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The origins of catalytic selectivity for the electrochemical conversion of carbon dioxide to methanol

Nano Research 2024年第1期17卷 5-17页

作者： Tian Wang Yating Wang Yuhang Li Chunzhong Li Key Laboratory for Ultrafine Materials of Ministry of Education Shanghai Engineering Research Center of Hierarchical NanomaterialsFrontiers Science Center for Materiobiology and Dynamic ChemistrySchool of Materials Science and EngineeringEast China University of Science&TechnologyShanghai 200237China School of Chemical Engineering East China University of Science&TechnologyShanghai 200237China

The electrocatalytic conversion of carbon dioxide(CO_(2))into useful fuels and chemical feedstocks is an emerging route to alleviate global warming and reduce reliance on fossil ***(CH_(3)OH),as one of the most significant and widely used liquid fuels that can be generated by CO_(2)reduction,is essential in the chemical *** this minireview,we unravel the origins of the selective formation of CH_(3)OH via CO_(2)reduction,including catalyst composition designs,local structure modulations,and electrolyte/catalyst interface ***,the remaining challenges and perspectives for the CO_(2)-to-CH_(3)OH reduction are proposed.

关键词： methanol carbon dioxide(CO_(2))reduction reaction electrochemistry electrocatalyst catalyst-electrolyte interface

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Structure-performance relationship between denitration performance and catalytic interface morphologies of MnCeO_(x)/P84 catalytic filters

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Journal of Rare Earths 2025年第3期43卷 516-525,I0004页

作者： Bo Yang Yujie Lei Maosen Ni Liuying Wang Qiong Huang Mindong Chen Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology(CICAEET) Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution ControlSchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjing210044China

MnCeO_(x)/P84 catalytic filters with spherical,flower-like,cubic and rod-like catalytic interfaces were synthesized respectively,and their catalytic activities in the NH_(3)-SCR reaction were *** MnCeO_(x)/P84 catalytic filter with spherical catalytic interfaces(recorded as S-MnCeO_(x)/P84)exhibits the best catalytic denitration *** NO_(x)removal efficiency of S-MnCeO_(x)/P84 reaches the highest value of 98.6%at 160℃when the catalyst loading is 100 g/m^(2).At the same time,S-MnCeO_(x)/P84 exhibits good SO_(2)resistance and stability,achieving a NO_(x)removal rate of 83%at 190℃with 30 ppm SO_(2).The characterization results illustrate that the MnCeO_x active component in S-MnCeO_(x)/P84 is present in weak crystalline states,tightly wrapped around the surface of the filter fiber,and uniformly dispersed,and the mesopore is the main pore structure of the S-MnCeO_(x)/P84,which can provide a channel for the catalytic reaction to *** the same time,transmission electron microscopy(TEM)characterization shows that y-MnO_(2)is the main form of MnO_(2)in the S-MnCeO_(x)/*** analysis of H_(2)temperature programmed reduction(H_(2)-TPR).NH_(3)temperature programmed desorption(NH_(3)-TPD)and in-situ diffuse reflectance infrared spectra(DRIFTS)show that S-MnCeO_(x)/P84 has good redox ability at 100-200℃and has abundant Lewis acid sites and Bronsteds acid sites,which provides an important guarantee for its superior low-temperature NH_(3)-SCR denitration performance.

关键词： Catalytic filter Nitrogen oxides(NO_x) Denitration Catalytic interface Rare earths

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Polyetherketoneketone/carbon fiber composites with an amorphous interface prepared by solution impregnation

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新型炭材料（中英文） 2024年第4期39卷 692-702页

作者： ZHANG Feng LI Bo-lan JIAO Meng-xiao LI Yan-bo WANG Xin YANG Yu YANG Yu-qiu ZHANG Xiao-hua MOE Key Laboratory of Textile Science&Technology College of TextilesInnovation Center for Textile Science and TechnologyDonghua UniversityShanghai 201620China Key Laboratory of Carbon Materials National Engineering Laboratory for Carbon Fiber TechnologyInstitute of Coal ChemistryChinese Academy of SciencesTaiyuan 030001China

Interfacial adhesion between carbon fibers(CF)and polyetherketoneketone(PEKK)is a key factor that affects the mechanical performances of their *** is therefore of great importance to impregnate the CF bundles with PEKK as effi-ciently as *** report that PEKK with a good dispersion in a mixed solution of 4-chlorophenol and 1,2-dichloroethane can be introduced onto CF surfaces by solution impregnation and curing at 280,320,340 and 360℃.The excellent wettability or infiltra-tion of the PEKK solution guarantees a full covering and its tight binding to CFs,making it possible to evaluate the interfacial shear strength(IFSS)with the microdroplet *** interior of the CF bundles is completely and uniformly filled with PEKK by solu-tion impregnation,leading to a high interlaminar shear strength(ILSS).The maximum IFSS and ILSS reached 107.8 and 99.3 MPa,*** superior shear properties are ascribed to the formation of amorphous PEKK in the small spaces between CFs.

关键词： Polyetherketoneketone Carbon fiber Wettability Amorphous adhesion Interfacial strength

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Ionic-electronic dual-conductor interface engineering and architecture design in layered lithium-rich manganese-based oxides

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Carbon Energy 2025年第2期7卷 24-40页

作者： Youyou Fang Yuefeng Su Jinyang Dong Jiayu Zhao Haoyu Wang Ning Li Yun Lu Yujia Wu Wenbo Li Ni Yang Xiaojuan Wu Feng Wu Lai Chen Beijing Key Laboratory of Environmental Science and Engineering School of Materials Science and EngineeringBeijing Institute of TechnologyBeijingChina Chongqing Innovation Center Beijing Institute of TechnologyChongqingChina Initial Energy Science&Technology(Xiamen)Co. LtdXiamenChina

The burgeoning growth in electric vehicles and portable energy storage systems necessitates advances in the energy density and cost-effectiveness of lithium-ion batteries(LIBs),areas where lithium-rich manganese-based oxide(LLO)materials naturally stand *** their inherent advantages,these materials encounter significant practical hurdles,including low initial Coulombic efficiency(ICE),diminished cycle/rate performance,and voltage fading during cycling,hindering their widespread *** response,we introduce an ionic-electronic dual-conductive(IEDC)surface control strategy that integrates an electronically conductive graphene framework with an ionically conductive heteroepitaxial spinel Li_(4)Mn_(5)O_(12)*** electrochemical and structural analyses demonstrate that this IEDC heterostructure effectively minimizes polarization,mitigates structural distortion,and enhances electronic/ionic *** functional theory calculations highlight an extensive Li^(+)percolation network and lower Li^(+)migration energies at the layered-spinel *** designed LLO cathode with IEDC interface engineering(LMOSG)exhibits improved ICE(82.9%at 0.1 C),elevated initial discharge capacity(296.7 mAh g^(-1)at 0.1 C),exceptional rate capability(176.5 mAh g^(-1)at 5 C),and outstanding cycle stability(73.7%retention at 5 C after 500 cycles).These findings and the novel dual-conductive surface architecture design offer promising directions for advancing highperformance electrode materials.

关键词： architecture design high-rate cyclability ionic-electronic dual-conductor layered lithiumrich manganese-based oxides lithium-ion battery

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Accurate quantification of the algebraic,multiplicative algebraic,and simultaneous iterative reconstruction techniques in ionosphere rebuilding based on the TIEGCM assessment

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Earth and Planetary Physics 2025年第1期9卷 117-126页

作者： Ao Qi HaiBing Ruan Institute of Space Weather Nanjing University of Information Science and TechnologyNanjing 210044China Key Laboratory of Geospace Environment University of Science&Technology of ChinaChinese Academy of SciencesHefei 230026China

The algebraic reconstruction technique(ART),multiplicative algebraic reconstruction technique(MART),and simultaneous iterative reconstruction technique(SIRT)are computational methodologies extensively utilized within the field of computerized ionospheric tomography(CIT)to facilitate three-dimensional reconstruction of the ionospheric ***,reconstruction accuracy elicits recurrent disputes over its practical application,and people usually attribute this issue to incomplete and uneven coverage of the *** Thermosphere Ionosphere Electrodynamics General Circulation Model(TIEGCM)offers a reasonable physics-based ionospheric background and is widely utilized in ionospheric *** use the TIEGCM simulations as the targeted ionosphere because the current measurements are far from able to realistically reproduce the ionosphere in *** designations of satellite measurements are conducted to investigate the limiting performance of CIT methods in ionospheric *** to common practice,electron density distributions from outputs of the International Reference Ionosphere(IRI)model are used as the iterative initial value in CIT *** outcomes suggest that despite data coverage,iterative initial conditions also play an essential role in ionospheric *** particular,in the longitudinal sectors where the iterative initial height of the F2-layer peak electron density(hmF2)differs substantially from the background densities,none of the three CIT methods can reproduce the exact background *** hmF2 is close but the ionospheric F2-layer peak density(NmF2)is different between the targeted background and initial conditions,the MART performs better than the ART and SIRT,as evidenced by the correlation coefficients of MART being above 0.97 and those of ART and SIRT being below *** summary,this investigation reveals the potential uncertainties in traditional CIT reconstruction,particularly when reali

关键词： computerized ionospheric tomography International Reference Ionosphere model Thermosphere Ionosphere Electrodynamics General Circulation model ionosphere

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A waterproof,environment-friendly,multifunctional,and stretchable thermoelectric fabric for continuous self-powered personal health signal collection at high humidity

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SusMat 2023年第5期3卷 709-720页

作者： Xinyang He Bingyi Li Jiaxin Cai Honghua Zhang Chengzu Li Xinxin Li Jianyong Yu Liming Wang Xiaohong Qin Key Laboratory of Textile Science&Technology Ministry of EducationCollege of TextilesDonghua UniversityShanghaiChina Center for Civil Aviation Composites College of TextilesDonghua UniversityShanghaiChina Innovation Center for Textile Science and Technology Donghua UniversityShanghaiChina

Thermoelectric sensors have attracted increasing attention in smart wearables due to the recognition of multiple signals in self-powered ***,present thermoelectric devices show disadvantages of low durability,weak wearability,and complex preparation processes and are susceptible to moisture in the microenvironment of the human body,which hinders their further application in wearable ***,we prepared a new thermoelectric fabric with thermoplastic polyurethane/carbon nanotubes(TPU/CNTs)by combining vacuum filtration and electrospraying *** TPU microsphere coating with good biocompatibility and environmental friendliness made the fabric worn directly and exhibits preferred water resistance,mechanical durability,and stability even after being bent 4000 times,stretched 1000 times,and washed 1000 ***,this fabric showed a Seebeck coefficient of 49μVK−1 and strain range of 250%and could collect signals well and avoided interference from *** on the biocompatibility and safety of the fabric,it can be fabricated into devices and mounted on the human face and elbow for long-term and continuous collection of data on the body’s motion and breathing simultaneously to provide collaborative support *** thermoelectric fabric-based sensor will show great potential in advanced smart wearables for health monitoring,motion detection,and human–computer interaction.

关键词： biocompatibility health monitor self-powered sensing thermoelectric fabrics waterproof

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A 4H-SiC trench IGBT with controllable hole-extracting path for low loss

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Chinese Physics B 2023年第4期32卷 714-718页

作者：吴丽娟刘恒宋宣廷陈星曾金胜邱滔张帮会 Hunan Provincial Key Laboratory of Flexible Electronic Materials Genome Engineering Changsha University of Science&TechnologyChangsha 410114China

A novel 4H-Si C trench insulated gate bipolar transistor(IGBT)with a controllable hole-extracting(CHE)path is proposed and investigated in this *** CHE path is controlled by metal semiconductor gate(MES gate)and metal oxide semiconductor gate(MOS gate)in the p-shield *** grounded p-shield region can significantly suppress the high electric field around gate oxide in Si C devices,but it weakens the conductivity modulation in the Si C trench IGBT by rapidly sweeping out *** effect can be eliminated by introducing the CHE *** CHE path is pinched off by the high gate bias voltage at on-state to maintain high conductivity modulation and obtain a comparatively low on-state voltage(VON).During the turn-off transient,the CHE path is formed,which contributes to a decreased turn-off loss(EOFF).Based on numerical simulation,the EOFFof the proposed IGBT is reduced by 89%compared with the conventional IGBT at the same VONand the VONof the proposed IGBT is reduced by 50%compared to the grounded p-shield IGBT at the same *** addition,the average power reduction for the proposed device can be 51.0%to 81.7%and 58.2%to 72.1%with its counterparts at a wide frequency range of 500 Hz to 10 k Hz,revealing a great improvement of frequency characteristics.

关键词： controllable hole-extracting path energy loss frequency characteristics Si C insulated gate bipolar transistor(IGBT)

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Electrospun Polyacrylonitrile Membrane In Situ Modified with Cellulose Nanocrystal Anchoring TiO_(2)for Oily Wastewater Recovery

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Advanced Fiber Materials 2023年第6期5卷 2055-2068页

作者： Jiqing Lu Tian Bai Dong Wang Haijiao Yu Qingxiang Wang Zhaoxuan Niu Yi Hu Xueying Liu Guangping Han Wanli Cheng Key Laboratory of Bio‑Based Material Science&Technology of Ministry of Education Northeast Forestry UniversityHarbin 150040China

With the increasingly urgent demand for clean water resources and the growing emission of oily wastewater,high-flux oil/water separation materials with the special wettability are progressively *** nanocrystal(CNC)from renewable biomass has been utilized to fabricate oil/water separation membranes,but it is limited to enhancing mechanical ***,a wrinkled structure with abundant–OH is constructed on polyacrylonitrile(PAN)nanofibers via the CNC hybridization *** then,a super-hydrophilic nano-TiO_(2)shell is anchored tightly on the surface of the fiber by wrinkles and–*** CNC promotes significantly the in situ growth of TiO_(2),with the TiO_(2)loading ratio of up to 5.3%.The nano-TiO_(2)shell endows the obtained film with super-hydrophilicity and underwater super-oleophobicity,resulting in a visible increase of the permeation flux for the oil/water mixture from 1483 to 11,023 L m^(−2)h^(−1).Interestingly,the hierarchical structure facilitates the demulsification for oil-in-water emulsion stabilized by surfactant,allowing the obtained membrane to exhibit eminent antifouling property and high emulsion permeability of about 3,278 L m^(−2)h^(−1).This design strategy develops next-generation anchors for targeted modification on the non-reactive substrates and provides a novel pathway for fabricating oil/water separation membranes.

关键词： Electrospinning Cellulose nanocrystal TiO_(2) Core-shell structure Oil/water separation

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Breaking the boundaries of biological penetration depth:X-ray luminescence in light theranostics

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science China Chemistry 2024年第4期67卷 1056-1059页

作者： Zhijian Yang Qiaohong Xu Qiushui Chen Huanghao Yang New Cornerstone Science Laboratory Key Laboratory for Analytical Science of Food Safety and Biology of Ministry of EducationCollege of ChemistryFuzhou UniversityFuzhou 350002China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China

Advances in luminescence materials have markedly propelled research in light theranostics,spanning luminescence biosensing[1],in vivo optical imaging[2],photodynamic therapy[3],optogenetics[4],and related fields[5-7].Nevertheless,conventional light sources have limited penetration depths within deep tissues,and the current state of light theranostics in superficial tissues does not fulfill the requirements for deep tissue treatments in clinical applications.

关键词： luminescence light spanning

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Mid-wavelength InAs/GaSb type-Ⅱ superlattice barrier detector with nBn design and M barrier

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Optoelectronics Letters 2023年第10期19卷 577-582页

作者： LIU Zhaojun ZHU Lianqing LU Lidan DONG Mingli ZHANG Dongliang ZHENG Xiantong School of Opto-Electronic Engineering Changchun University of Science&TechnologyChangchun130022China Key Laboratory of the Ministry of Education for Optoelectronic Measurement Technology and Instrument Beijing Information Science&Technology UniversityBeijing100192China Key Laboratory of Optical Fiber Sensing and System Beijing Information Science&Technology UniversityBeijing100016China

This study reports the performance of an InAs/GaSb type-Ⅱ superlattices(T2SLs) detector with nBn structure for mid-wavelength infrared(MWIR) detection. An electronic band structure of M barrier is calculated using 8-band k·p method, and the nBn structure is designed with the M barrier. The detector is prepared by wet etching, which is simple in manufacturing process. X-ray diffraction(XRD) and atomic force microscope(AFM) characteristics indicate that the detector material has good crystal quality and surface morphology. The saturation bias of the spectral response measurements at 77 K is 300 m V, and the device is promising to work at a temperature of 140 K. Energy gap of T2SLs versus temperature is fitted by the Varshni curve, and zero temperature bandgap Eg(0), empirical coefficients α and β are extracted. A dark current density of 3.2×10-5A/cm2and differential resistance area(RA) product of 1.0×104Ω·cm2are measured at 77 K. The dominant mechanism of dark current at different temperature ranges is analyzed. The device with a 50% cutoff wavelength of 4.68 μm exhibits a responsivity of 0.6 A/W, a topside illuminated quantum efficiency of 20% without antireflection coating(ARC), and a detectivity of 9.17×1011cm·Hz1/2/W at 77 K and 0.3 V.

关键词： InAs/GaSb barrier structure

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