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Correction to: Porous yttria-stabilized zirconia ceramics with low thermal conductivity via a novel foam-gelcasting method

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Journal of materials Science 2022年第1期57卷 790-790页

作者： Meng, Xuanyu Xu, Jie Zhu, Jiatong Zhao, Jia Li, Zhuolun Pawlikowska, Emilia Szafran, Mikołaj Gao, Feng State Key Laboratory of Solidification Processing MIIT Key Laboratory of Radiation Detective Material and Device NPU-QMUL Joint Research Institute of Advanced Materials and Structures (JRI-AMAS) School of Material Science and Engineering Northwestern Polytechnical University Xi’an China Research and Development Institute of Northwestern Polytechnical University in Shenzhen Shenzhen China Institute of High Pressure Physics of the Polish Academy of Sciences Warsaw Poland Faculty of Chemistry Warsaw University of Technology Warsaw Poland

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Two-Second-Annealed 2D/3D Perovskite Films with Graded Energy Funnels and Toughened Heterointerfaces for Efficient and Durable Solar Cells

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Angewandte Chemie 2023年第38期135卷

作者： Dr. Xueqing Chang Dr. Jun-Xing Zhong Sibo Li Dr. Qin Yao Yuxuan Fang Guo Yang Ying Tan Prof. Qifan Xue Prof. Longbin Qiu Dr. Qingqian Wang Prof. Yong Peng Prof. Wu-Qiang Wu MOE Key Laboratory of Bioinorganic and Synthetic Chemistry Lehn Institute of Functional Materials School of Chemistry Sun Yat-sen University Guangzhou 510006 P. R. China School of chemistry and Materials Science Guangdong University of Education Guangzhou 510303 P.R. China SUSTech Energy Institute for Carbon Neutrality Department of Mechanical and Energy Engineering Southern University of Science and Technology Shenzhen 518055 P. R. China School of Chemistry and Chemical Engineering Harbin Institute of Technology Harbin 150001 P. R. China State Key Laboratory of Luminescent Materials and Devices Institute of Polymer Optoelectronic Materials and Devices School of Materials Science and Engineering South China University of Technology 381 Wushan Road Guangzhou 510640 P. R. China Institute of Physics Henan Academy of Sciences Mingli Road 266-38 Zhengzhou 450046 P. R. China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 Hubei P. R. China Contribution: Conceptualization (lead) Project administration (lead) Supervision (lead) Writing - review & editing (lead)

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Amine‐Responsive Disassembly of AuI–CuIDouble Salts for Oxidative Carbonylation

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Angewandte Chemie 2019年第5期132卷

作者： Yanwei Cao Jian‐Gong Yang Yi Deng Shengchun Wang Qi Liu Chaoren Shen Wei Lu Chi‐Ming Che Yong Chen Lin He State Key Laboratory for Oxo Synthesis and Selective Oxidation (OSSO) Suzhou Research Institute of LICP Lanzhou Institute of Chemical Physics (LICP) Chinese Academy of Sciences (CAS) Lanzhou 730000 China University of Chinese Academy of Sciences Beijing 100049 China Key Laboratory of Photochemical Conversion and Optoelectronic Materials & CAS-HKU Joint Laboratory on New Materials Technical Institute of Physics and Chemistry CAS Beijing 100190 China The Institute for Advanced Studies College of Chemistry and Molecular Sciences Wuhan University Wuhan 430072 China Department of Chemistry South University of Science and Technology of China Shenzhen Guangdong 518055 China State Key Laboratory of Synthetic Chemistry & Department of Chemistry The University of Hong Kong Pokfulam Road Hong Kong SAR China

A sensitive amine‐responsive disassembly of self‐assembled Au I ‐Cu I double salts was observed and its utilization for the synergistic catalysis was enlightened. Investigation of the disassembly of [Au(NHC) 2 ][CuI 2 ] revealed the contribution of Cu‐assisted ligand exchange of N‐heterocyclic carbene (NHC) by amine in [Au(NHC) 2 ] + and the capacity of [CuI 2 ] − on the oxidative step. By integrating the implicative information coded in the responsive behavior and inherent catalytic functions of d 10 metal complexes, a catalyst for the oxidative carbonylation of amines was developed. The advantages of this method were clearly reflected on mild reaction conditions and the significantly expanded scope (51 examples); both primary and steric secondary amines can be employed as substrates. The cooperative reactivity from Au and Cu centers, as an indispensable prerequisite for the excellent catalytic performance, was validated in the synthesis of (un)symmetric ureas and carbamates.

关键词： Carbamate Doppelsalze Harnstoff Oxidative Carbonylierung Synergistische Katalyse

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Daytime radiative cooling dressings for accelerating wound healing under sunlight

Nature Chemical Engineering

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Nature Chemical Engineering 2024年第4期1卷 301-310页

作者： Qian Zhang Xueyang Wang Bin Zhu Hanyu Fu Shining Zhu Jia Zhu Xingfang Xiao Weilin Xu Chao Qi Song Hu Wei Li National Laboratory of Solid State Microstructures College of Engineering and Applied Sciences Jiangsu Key Laboratory of Artificial Functional Materials Collaborative Innovation Center of Advanced Microstructures Frontiers Science Center for Critical Earth Material Cycling Nanjing University Nanjing P. R. China State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile University Wuhan P. R. China School of Sustainable Energy and Resources Nanjing University Suzhou P. R. China Department of Pharmacy Wuhan No.1 Hospital (Wuhan Hospital of Traditional Chinese and Western Medicine) Wuhan P. R. China GPL Photonics Laboratory State Key Laboratory of Luminescence Science and Technology Changchun Institute of Optics Fine Mechanics and Physics Chinese Academy of Sciences Changchun P. R. China

The process of wound healing is sensitive to various factors of the local environment, including temperature, humidity and sterility. However, due to lack of efficient thermal regulation in existing wound dressings, the perturbed local environment and oxidative stress caused by an increased wound temperature under outdoor sunlight inevitably impacts wound healing. Here we demonstrate a daytime radiative cooling dressing based on a polyamide 6/silk fibroin bilayer that reduces the thermal load for skin wounds under sunlight illumination. The mid-infrared transparent polyamide 6 and the biocompatible silk fibroin together endow a high mid-infrared emissivity (~0.94) and sunlight reflectivity (~0.96), thus achieving a temperature of ~7 °C below ambient under direct sunlight. When used for repairing mouse skin full-thickness injuries under sunlight, we observed an accelerated wound healing rate compared with that of commercial dressings. This work therefore offers a promising strategy for passive temperature regulation to accelerate wound healing under sunlight.

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Front Cover: Molecular Engineering of Zinc-Porphyrin Sensitisers for p-Type Dye-Sensitised Solar Cells (ChemPlusChem 7/2018)

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ChemPlusChem 2018年第7期83卷 542-542页

作者： Dr. Jianfeng Lu Dr. Zonghao Liu Narendra Pai Liangcong Jiang Prof. Dr. Udo Bach Dr. Alexandr N. Simonov Prof. Dr. Yi-Bing Cheng Prof. Dr. Leone Spiccia School of Chemistry Monash University Clayton Victoria 3800 Australia School of Optical and Electronic Information Huazhong University of Science and Technology Wuhan 430074 China Department of Materials Science and Engineering Monash University Clayton Victoria 3800 Australia Department of Chemical Engineering Monash University Clayton Victoria 3800 Australia CSIRO Clayton Victoria 3168 Australia ARC Centre of Excellence for Exciton Science Monash University Clayton Victoria 3800 Australia ARC Centre of Excellence for Electromaterials Science Monash University Clayton Victoria 3800 Australia State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 China Deceased December 2016

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Direct Atomic-Level Imaging of Zeolites: Oxygen, Sodium in Na-LTA and Iron in Fe-MFI

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Angewandte Chemie 2020年第44期132卷

作者： Mayoral A. Zhang Q. Zhou Y. Chen P. Ma Y. Monji T. Losch P. Schmidt W. Schüth F. Hirao H. Yu J. Terasaki O. Centre for High-resolution Electron Microscopy (CħEM) School of Physical Science and Technology ShanghaiTech University 393 Middle Huaxia Road Shanghai Pudong 201210 China Institute of Materials Science of Aragon (ICMA) Spanish National Research Council (CSIC) Advanced Microscopy Laboratory (LMA) University of Zaragoza 12 Calle de Pedro Cerbuna Zaragoza 50009 Spain Key Laboratory of Biomedical Polymers-Ministry of Education College of Chemistry and Molecular Sciences Wuhan University Wuhan 430072 China Zhiyuan College & School of Chemistry and Chemical Engineering Shanghai Jiao Tong University 800 Dongchuan Road Shanghai 200240 China Hitachi Solutions East (Japan) Ltd. Sendai Japan Department of Heterogeneous Catalysis Max-Planck-Institut für Kohlenforschung Kaiser-Wilhelm-Platz 1 Mülheim an der Ruhr 45470 Germany Department of Chemistry City University of Hong Kong Tat Chee Avenue Kowloon Hong Kong SAR China State Key Laboratory of Inorganic Synthesis and Preparative Chemistry College of Chemistry International Center of Future Science Jilin University Changchun 130012 China Department of Materials and Environmental Chemistry Stockholm University Stockholm Sweden

Zeolites are becoming more versatile in their chemical functions through rational design of their frameworks. Therefore, direct imaging of all atoms at the atomic scale, basic units (Si, Al, and O), heteroatoms in the framework, and extra-framework cations, is needed. TEM provides local information at the atomic level, but the serious problem of electron-beam damage needs to be overcome. Herein, all framework atoms, including oxygen and most of the extra-framework Na cations, are successfully observed in one of the most electron-beam-sensitive and lowest framework density zeolites, Na-LTA. Zeolite performance, for instance in catalysis, is highly dependent on the location of incorporated heteroatoms. Fe single atomic sites in the MFI framework have been imaged for the first time. The approach presented here, combining image analysis, electron diffraction, and DFT calculations, can provide essential structural keys for tuning catalytically active sites at the atomic level. © 2020 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA.

关键词： annular bright-field analysis beam damage electron diffraction electron microscopy Zeolites

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Cover Picture: Bioinspired Color Switchable Photonic Crystal Silicone Elastomer Kirigami (Angew. Chem. Int. Ed. 26/2021)

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Angewandte Chemie International Edition 2021年第26期60卷

作者： Xintao Lai Jingsong Peng Prof. Qunfeng Cheng Prof. Antoni P. Tomsia Dr. Guanlei Zhao Prof. Lei Liu Prof. Guisheng Zou Prof. Yanlin Song Prof. Lei Jiang Prof. Mingzhu Li Key Laboratory of Green Printing Institute of Chemistry Chinese Academy of Sciences Beijing 100191 China School of Chemistry and Chemical Engineering University of Chinese Academy of Sciences Beijing 100049 China Key Laboratory of Bio-inspired Smart Interfacial Science and Technology of Ministry of Education School of Chemistry Beijing Advanced Innovation Center for Biomedical Engineering BUAA-UOW Joint Research Centre Beihang University Beijing 100191 China School of Materials Science and Engineering Zhengzhou University Zhengzhou 450001 China Department of Mechanical Engineering State Key Laboratory of Tribology Tsinghua University Beijing 100084 China Key Laboratory of Materials Processing and Mold (Zhengzhou University) Ministry of Education Zhengzhou 450002 China

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Titelbild: Bioinspired Color Switchable Photonic Crystal Silicone Elastomer Kirigami (Angew. Chem. 26/2021)

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Angewandte Chemie 2021年第26期133卷

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Bioinspired Color Switchable Photonic Crystal Silicone Elastomer Kirigami

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Angewandte Chemie 2021年第26期133卷

Bioinspired dynamic structural color has great potential for use in dynamic displays, sensors, cryptography, and camouflage. However, it is quite rare for artificial structural color devices to withstand thousands of cycles. Male hummingbird's crowns and gorgets are brightly colored, demonstrating frequent color switching that is induced by regulating the orientation of the feathers through movement of skin or joints. Inspired by this unique structural color modulation, we demonstrate a flexible, mechanically triggered color switchable sheet based on a photonic crystal (PhC)-coated polydimethylsiloxane (PDMS) kirigami (PhC-PDMS kirigami) made by laser cutting. Finite element modeling (FEM) simulation reveals that the thickness of PDMS kirigami and the chamfer at the incision induced by laser cutting both dominate the out-of-plane deformation through in-plane stretching. The bioinspired PhC-PDMS kirigami shows precisely programmable structural color and keeps the color very well after recycling over 10 000 times. This bioinspired PhC-PDMS kirigami also shows excellent viewability even in bright sunlight, high readability, robust functionality, technical flexibility, and mechanical durability, which are readily exploitable for applications, such as chromic mechanical monitors for the sports industry or for medical applications, wearable camouflage, and security systems.

关键词： bioinspired color switchable kirigami silicone elastomers

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Photo-driven Oxygen Vacancies Extends Charge Carrier Lifetime for Efficient Solar Water Splitting

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Angewandte Chemie 2021年第32期133卷

作者： Mao Sun Rui-Ting Gao Prof. Jinlu He Prof. Xianhu Liu Prof. Tomohiko Nakajima Prof. Xueyuan Zhang Prof. Lei Wang School of Chemistry and Chemical Engineering & Inner Mongolia Engineering and Technology Research Center for Catalytic Conversion and Utilization of Carbon Resource Molecules Inner Mongolia University 235 West University Street Hohhot 010021 China Key Laboratory of Materials Processing and Mold Ministry of Education Zhengzhou University Zhengzhou 450002 China Advanced Coating Technology Research Center National Institute of Advanced Industrial Science and Technology Tsukuba Central 5 1-1-1 Higashi Tsukuba Ibaraki 305-8565 Japan State Key Laboratory of Chemo/Biosensing and Chemometrics College of Chemistry and Chemical Engineering Hunan University Changsha 410082 China

A photocharge/discharge strategy is proposed to initiate the WO 3 photoelectrode and suppress the main charge recombination, which remarkably improves the photoelectrochemical (PEC) performance. The photocharged WO 3 surrounded by a 8–10 nm overlayer and oxygen vacancies could be operated more than 25 cycles with 50 h durability without significant decay on PEC activity. A photocharged WO 3 /CuO photoanode exhibits an outstanding photocurrent of 3.2 mA cm −2 at 1.23 V RHE with a low onset potential of 0.6 V RHE , which is one of the best performances of p-n heterojunction structure. Using nonadiabatic molecular dynamics combined with time-domain DFT, we clarify the prolonged charge carrier lifetime of photocharged WO 3 , as well as how electronic systems of photocharged WO 3 /CuO semiconductors enable the effective photoinduced electrons transfer from WO 3 into CuO. This work provides a feasible route to address excessive defects existed in photoelectrodes without causing extra recombination.

关键词： oxygen vacancies photocharging/discharging p-n heterojunctions solar water splitting tungsten

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