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Aqueous batteries:from laboratory to market

国家科学评论（英文版） 2023年第11期10卷 85-88页

作者： Xikun Zhang Pengcheng Xing Thomas L.Madanu Jing Li Jie Shu Bao-Lian Su Laboratory of Inorganic Materials Chemistry(CMI) University of NamurBelgium School of Materials Science and Chemical Engineering Ningbo UniversityChina Laboratory of Inorganic Materials Chemistry(CMI) University of NamurBelgium State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyChina

As estimated up to 2022,global installed capacity of lithium-ion batteries(LIBs)has increased dramatically from 148 to 580 GWh in the past five *** wide range of applications is mainly at-tributed to their high energy density,ex-cellent cycle life,and low self-discharge rate[1].However,with the continuous promotion of the applications in various fields,the limitations of LIBs have be-come apparent,such as high cost and safety issues.

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BaTiO_(3)/Polyurethane Dielectric Composites with Diels-Alder Bond for Improved Self-Healing Properties

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Journal of Renewable materials 2022年第9期10卷 2355-2364页

作者： unlong Yao Wei Nie Zhengguang Sun Huan Yang Yu Guan Lin Gao Xueliang Jiang Mujie Guo Chuanxi Xiong Hubei Key Laboratory of Plasma Chemistry and Advanced Materials School of Materials Science and EngineeringWuhan Institute of TechnologyWuhan430205China Ministry-of-Education Key Laboratory for the Green Preparation and Application of Functional Materials Hubei UniversityWuhan430062China Key Laboratory of Green Chemical Engineering Process of Ministry of Education Wuhan Institute of TechnologyWuhan430205China School of Chemistry and Environmental Engineering Jianghan UniversityWuhan430056China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing and School of Materials Science and EngineeringWuhan University of TechnologyWuhan430070China

In general,self-healing dielectric composites are mainly composed of polar hydrogen bonds,which have high hydrophilicity and are unsuitable for humid *** composite with Diels-Alder(D-A)bond contains covalent bonds,it can be adopted as an efficient self-healing ***,we construct self-healing barium titanate(BT)/polyurethane(PU)dielectric composites by adopting PU with D-A bond as matrix(BT/PU-DA).The prepared 10%BT/PU-DA composite exhibits superior self-healing ability than that of ***,its dielectric constant can reach 9.3 with a loss of only 0.04 at 1000 Hz and maintain 93%repair efficiency of tensile *** experimental analysis suggests the introduction of D-A bond can enhance the thermostability and self-healing ability of BT/PU-DA *** addition,the incorporation of BT nanoparticles and D-A bond in the self-healing composite contributes to the lower dielectric loss and excellent tensile strength after *** adopted strategy is a promising and facile approach to develop highly efficient selfhealing dielectric material,which will be conducive to reuse and sustainable development of the electronic packaging material in aqueous medium or wet environment.

关键词： Diels-Alder bond self-healing dielectric properties tensile strength polyurethane

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synthesis of highly sinterable MgO powders for IR transparent ceramics

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Ceramics International 2025年

作者： Zhi, Yongli Mei, Bingchu Li, Weiwei Cheng, Jing Luo, Peng State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China Jianghuai Advance Technology Center Hefei230000 China

MgO transparent ceramics (TCS) have attracted great interests in the field of infrared window materials due to its wide transmission range, excellent thermal conductivity, and balanced mechanical properties. To date, research on MgO transparent ceramics predominantly relies on commercial MgO powders by spark plasma sintering (SPS). Herein, we report highly sinterable MgO powders synthesized by co-precipitation method, which exhibits pure phase and particle size of 75 nm. When sintered at 950 °C under 45 MPa for 2 h by hot pressed (HP) method, the transmittance of the MgO ceramic sample with the thickness of 2 mm achieved 76.9 % at 0.4 μm and 88.3 % at 5 μm. These optical properties are comparable to or even superior to MgO TCS produced through SPS method. This work shows that the MgO particles synthesized via the co-precipitation method are suitable for producing high optical quality of MgO infrared (IR) transparent ceramics. © 2025

关键词： Thermal conductivity

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High Conduction Band Inorganic Layers for Distinct Enhancement of Electrical Energy Storage in Polymer Nanocomposites

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Nano-Micro Letters 2022年第9期14卷 221-236页

作者： Yingke Zhu Zhonghui Shen Yong Li Bin Chai Jie Chen Pingkai Jiang Xingyi Huang Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing State Key Laboratory of Metal Matrix CompositesDepartment of Polymer Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240People’s Republic of China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Center of Smart Materials and DevicesWuhan University of TechnologyWuhan 430070People’s Republic of China Institute of Applied and Physical Chemistry and Center for Environmental Research and Sustainable Technology University of Bremen28359 BremenGermany

Dielectric polymer nanocomposites are considered as one of the most promising candidates for high-power-density electrical energy storage *** nanofillers with high insulation property are frequently introduced into fluoropolymer to improve its breakdown strength and energy storage ***,inorganic nanofillers are thought to introducing traps into polymer matrix to suppress leakage ***,how these nanofillers effect the leakage current is still ***,high dopant(>5 vol%)is prerequisite for distinctly improved energy storage performance,which severely deteriorates the processing and mechanical property of polymer nanocomposites,hence brings high technical complication and ***,boron nitride nanosheet(BNNS)layers are utilized for substantially improving the electrical energy storage capability of polyvinylidene fluoride(PVDF)*** reveal that the high conduction band minimum of BNNS produces energy barrier at the interface of adjacent layers,preventing the electron in PVDF from passing through inorganic layers,leading to suppressed leakage current and superior breakdown *** by improved Young’s modulus(from 1.2 GPa of PVDF to 1.6 GPa of nanocomposite),significantly boosted discharged energy density(14.3 J cm^(-3)) and charge-discharge efficiency(75%)are realized in multilayered nanocomposites,which are 340 and 300% of PVDF(4.2 J cm^(-3),25%).More importantly,thus remarkably boosted energy storage performance is accomplished by marginal *** work offers a new paradigm for developing dielectric nanocomposites with advanced energy storage performance.

关键词： Boron nitride nanosheet Conduction band Efficiency Energy density Barrier

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Electronegativity-Induced Single-Ion Conducting Polymer Electrolyte for Solid-state Lithium Batteries

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Energy & Environmental materials 2023年第4期6卷 40-48页

作者： Tianyi Hou Yumin Qian Dinggen Li Bo Xu Zhenyu Huang Xueting Liu Haonan Wang Bowen Jiang Henghui Xu Yunhui Huang State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement Ministry of EducationSchool of PhysicsBeijing Institute of TechnologyBeijing 100081China School of Energy and Power Engineering Huazhong University of Science and TechnologyWuhan 430074China Jiangsu Jitri-Hust Intelligent Equipment Technology Nanjing 210000China

The application of solid polymer electrolytes(SPEs)is severely impeded by the insufficient ionic conductivity and low Li^(+)transference numbers(t_(Li)^(+)).Here,we report an iodine-driven strategy to address both the two longstanding issues of SPEs *** lodine-containing groups introduced on polymer chains effectively attract Li^(+)ions,facilitate Li^(+)transport,and promote the dissociation of Li ***,iodine is also favorable to alleviate the strong O-Li^(+)coordination through a Lewis acidbase interaction,further improving the ionic conductivity and t_(Li)^(+).As a proof of concept,an iodinated single-ion conducting polymer electrolyte(IPE)demonstrates a high ionic conductivity of 0.93 mS cm^(-1)and a high t_(Li)^(+)of 0.86 at 25℃,which is among the best results ever reported for ***,symmetric Li/Li cells with IPE achieve a long-term stability over 2600 h through the in-situ formed LiF-rich *** a result,Li-S battery with IPE maintains a high capacity of 623.7 mAh g^(-1)over 300 cycles with an average Coulombic efficiency of 99%.When matched with intercalation cathode chemistries,Li/IPE/LiFePO_(4)and Li/IPE/LiNi_(0.8)Mn_(0.1)Co_(0.1)O_(2)solid-state batteries also deliver high-capacity retentions of 95%and 97%at 0.2 C after 120 cycles,respectively.

关键词： iodine lithium polymer electrolytes single-ion conducting solid-state batteries

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Julolidine functionalized benzimidazoline-doped fullerene derivatives for efficient and stable perovskite solar cells

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Interdisciplinary materials 2024年第3期3卷 369-379页

作者： Yanqing Zhu Chenglong Li JiaHui Chen Yuxi Zhang Jianfeng Lu Min Hu Wangnan Li Fuzhi Huang Yi-Bing Cheng Hyesung Park Shengqiang Xiao State Key Laboratory of Silicate Materials for Architectures Wuhan University of TechnologyWuhanChina State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhanChina School of Electronic and Electrical Engineering Hubei Province Engineering Research Centre for Intelligent Micro-Nano Medical Equipment and Key TechnologiesWuhan Textile UniversityWuhanChina Hubei Key Laboratory of Low Dimensional Optoelectronic Material and Devices Hubei University of Arts and ScienceXiangyangHubeiChina KU-KIST Graduate School of Converging Science and Technology Korea UniversitySeoulRepublic of Korea Department of Integrative Energy Engineering Korea UniversitySeoulRepublic of Korea Hubei Key Laboratory of Fuel Cell WuhanChina

Fullerene derivatives are highly attractive materials in solar cells,organic thermoelectrics,and other ***,the intrinsic low electron mobility and electrical conductivity restrict their potential device performance,such as perovskite solar cells(PSCs).Herein,we successfully enhanced the electric properties and morphology of phenyl-C61-butyric acid methyl ester(PCBM)by n-doping it with a benzimidazoline derivative,9-(1,3-dimethyl-2,3-dihydro-1H-benzoimidazol-2-yl)-julolidine(JLBI-H)via a solution *** found the n-doping can not only improve the conductivity and optimize the band alignment but also enable the PCBM to have a constantly strong charge extraction ability in a wide temperature from 173 to 373 K,which guarantees a stable photovoltaic performance of the corresponding PSCs under a wide range of operating *** the JLBI-H-doped PCBM,we improved the efficiency from 17.9%to 19.8%,along with enhanced stability of the nonencapsulated devices following the aging protocol of ISOS-D-1.

关键词： charge extraction electron mobility n-doping PSCs wide operation temperature

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A review on electrocatalytic CO_(2) conversion via C-C and C-N coupling

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Carbon Energy 2024年第2期6卷 167-194页

作者： Zhuangzhi Zhang Sijun Li Zheng Zhang Zhou Chen Hua Wang Xianguang Meng Wenquan Cui Xiwei Qi Jiacheng Wang Hebei Provincial Laboratory of Inorganic Nonmetallic Materials College of Materials Science and EngineeringNorth China University of Science and TechnologyTangshanChina Key Laboratory of Luminescence Analysis and Molecular Sensing Ministry of EducationCollege of Chemistry and Chemical EngineeringSouthwest UniversityChongqingChina State Key Laboratory of New Textile Materials and Advanced Processing Technologies Hubei Key Laboratory of Biomass Fibers and Eco-Dyeing and FinishingCollege of Chemistry and Chemical EngineeringWuhan Textile UniversityWuhanChina College of Materials Xiamen UniversityXiamenChina Hebei Iron and Steel Laboratory TangshanChina Hebei Key Laboratory for Environment Photocatalytic and Electrocatalytic Materials College of Chemical EngineeringNorth China University of Science and TechnologyTangshanChina College of Metallurgy and Energy North China University of Science and TechnologyTangshanChina State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghaiChina Institute of Electrochemistry School of Materials Science and EngineeringTaizhou UniversityTaizhouChina

Electrochemical C-C and C-N coupling reactions with the conversion of abundant and inexpensive small molecules,such as CO_(2) and nitrogencontaining species,are considered a promising route for increasing the value of CO_(2) reduction *** development of high-performance catalysts is the key to the both electrocatalytic *** this review,we present a systematic summary of the reaction systems for electrocatalytic CO_(2) reduction,along with the coupling mechanisms of C-C and C-N bonds over outstanding electrocatalytic materials recently *** key intermediate species and reaction pathways related to the coupling as well as the catalyst-structure relationship will be also discussed,aiming to provide insights and guidance for designing efficient CO_(2) reduction systems.

关键词： C-C coupling C-N coupling CO_(2) conversion electrocatalysis urea synthesis

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Emerging strategies and developments in oxygen reduction reaction using high-performance platinum-based electrocatalysts

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Nano Research 2024年第5期17卷 3516-3532页

作者： Asad Ali Aatto Laaksonen Guo Huang Shahid Hussain Shuiping Luo Wen Chen Pei Kang Shen Jinliang Zhu Xiaoyan Ji Energy Engineering Division of Energy ScienceLuleåUniversity of Technology97187 LuleåSweden Department of Materials and Environmental Chemistry Arrhenius LaboratoryStockholm UniversitySE-10691 StockholmSweden Center of Advanced Research in Bionanoconjugates and Biopolymers “Petru Poni”Institute of Macromolecular ChemistryIasi 700469Romania State Key Laboratory of Materials-Oriented and Chemical Engineering Nanjing Tech UniversityNanjing 211816China College of Materials Science and Engineering Shenzhen UniversityShenzhen 518060China School of Resources Environment and MaterialsState Key Laboratory of Processing for Non-ferrous Metal and Featured MaterialsGuangxi UniversityNanning 530004China

The global practical implementation of proton exchange membrane fuel cells(PEMFCs)heavily relies on the advancement of highly effective platinum(Pt)-based electrocatalysts for the oxygen reduction reaction(ORR).To achieve high ORR performance,electrocatalysts with highly accessible reactive surfaces are needed to promote the uncovering of active positions for easy mass *** this critical review,we introduce different approaches for the emerging development of effective ORR electrocatalysts,which offer high activity and *** strategies,including morphological engineering,geometric configuration modification via supporting materials,alloys regulation,core-shell,and confinement engineering of single atom electrocatalysts(SAEs),are discussed in line with the goals and requirements of ORR performance *** review the ongoing development of Pt electrocatalysts based on the syntheses,nanoarchitecture,electrochemical performances,and *** eventually explore the obstacles and research directions on further developing more effective electrocatalysts.

关键词： oxygen reduction reaction(ORR) Pt-based electrocatalysts proton exchange membrane fuel cells(PEMFCs) morphology and alloys strategies single atom electrocatalysts(SAEs)

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Aligne d nanofib ers incorporate d composite solid electrolyte for high-sensitivity oxygen sensing at medium temperatures

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Journal of materials Science & technology 2024年第14期181卷 189-197页

作者： Mengfei Zhang Lei Yao Yan Xing Jing Cheng Tianrang Yang Jianguo Liu Wei Pan Institute of Energy Power Innovation North China Electric Power UniversityBeijing 102206China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China Shenzhen Key Laboratory of Special Functional Materials Shenzhen Engineering Laboratory for Advanced Technology of CeramicsGuangdong Research Center for Interfacial Engineering of Functional MaterialsCollege of Materials Science and EngineeringShenzhen UniversityShenzhen 518060China New Energy Technology Engineering Lab of Jiangsu Province School of ScienceNanjing University of Posts&Telecommunications(NUPT)Nanjing 210003China

otentiometric oxygen sensors have been widely used in internal combustion engines,industrial boilers,and metallurgical heat treatment ***,traditional oxygen sensors based on yttria-stabilized zirconia(YSZ)electrolyte can only be operated at elevated temperatures(>750℃)due to their rela-tively low ionic *** this study,we present a highly efficient micro-oxygen sensor that can be operated at a temperature as low as 300℃.This micro-oxygen sensor incorporates a composite solid electrolyte,i.e.,well-aligned gadolinium-doped cerium oxide(CGO)nanofibers embedded within a YSZ matrix(YSZ/CGO_(f)).The arrays of CGO nanofibers in the YSZ matrix are parallel to the conduction direc-tion,providing rapid conducting channels for oxygen *** from this design,the composite electrolyte leads to a conductivity of four times higher than that of traditional YSZ solid electrolytes at low *** enhancement in conductivity is attributed to the presence of a defective interfacial region between CGO_(f)and YSZ,which promotes the mobility of oxygen *** strategy of constructing fast ionic conduction in the composite electrolyte by using well-aligned nanofibers may be considered for the design and optimization of other micro/nano-devices including sensors,batteries,and fuel cells.

关键词： Oxygen sensor Nanofibers Composite electrolyte Ionic conduction

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稀有金属材料与工程 2025年第2期54卷 311-318页

作者： Zhang Wenxin Zhang Xiankun Shi Lei Li Shengli Jiang Yuanning Wu Chuansong State Key Laboratory of Advanced Equipment and Technology for Metal Forming Shandong UniversityJinan 250061China Key Laboratory for Liquid-Solid Structure Evolution&Processing of Materials Ministry of EducationShandong UniversityJinan 250061China

Friction stir lap welding of AA2195 Al-Li alloy and Ti alloy was conducted to investigate the formation,microstructure,and mechanical properties of the *** show that under different welding parameters,with the decrease in welding heat input,the weld surface is *** Ti/Al joint interface is flat without obvious Ti and Al mixed structure,and the hook structure is not formed under optimal *** to the enhanced breaking effect of the stirring head,the hook structural defects and intermetallic compounds are more likely to form at the Ti/Al interface at high rotational speed of 1000 r/min,thereby deteriorating the mechanical properties of *** the heat input is beneficial to hardness enhancement of the aluminum alloy in the weld nugget *** the optimal parameters of rotation speed of 800 r/min and welding speed of 120 mm/min,the maximum tensile shear strength of joint is 289 N/mm.

关键词： Ti/Al dissimilar welding friction stir lap welding Ti alloy Al-Li alloy interface bonding mechanical property

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