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International Conference on power engineering 2021, ICOPE 2021

作者： Wen, Du Zhou, Qulan Pan, Yuqing Chen, Xiaole Li, Na State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University China

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Analytical solution for temperature distribution in functionally graded cylindrical shells under convective cooling

Analytical solution for temperature distribution in function...

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作者： Emamian, Amin Amiri Delouei, Amin Karimnejad, Sajjad Jing, Dengwei International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China Department of Mechanical Engineering University of Bojnord Bojnord Iran Mechanical Engineering Department Shahrood University of Technology Shahrood Iran

In the current study, an analytical solution for the temperature distribution in a cylindrical shell that is made of functionally graded material is obtained. The general boundary condition is considered for achieving the solution, and particularly convective cooling plays the dominant role in this problem. The obtained solution is first verified against the numerical data, and then, the credibility of the solution for studying practical problems is tested employing two illustrative test cases with various boundary conditions. Parametric studies are done to evaluate some significant parameters, including material constant, boundary conditions, and convection on temperature distribution. It is seen that boundary condition plays a dominant role in the cooling rate. Material constant does not have a significant effect on the temperature distribution. The current study can be hired to better the design and production process of cylindrical shells made of functionally graded material. © 2021 John Wiley & Sons, Ltd.

关键词： Functionally graded materials

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Experimental study on the CO-SCR performance of honeycomb-based Fe-Cu/RHA catalyst

Experimental study on the CO-SCR performance of honeycomb-ba...

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International Conference on power engineering 2021, ICOPE 2021

作者： Pan, Yuqing Li, Na Wen, Du Ran, Shiyuan Wu, Chenyang Zhou, Qulan State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University China

The combustion process of carbon-based fuels will produce CO. If CO can be used as a reducing agent to remove NO, the goal of removing NO and unburned carbon (UBC) simultaneously can be achieved. When rice husk ash (RHA) rich in amorphous SiO2 is used to support Fe-Cu metal oxides, its huge specific surface area and non-lattice microstructure can reduce the reaction temperature, so that Fe-Cu/RHA catalyst has a high performance of selective catalytic reduction of NO by CO (CO-SCR). The paper used honeycomb ceramic to support Fe-Cu/RHA catalyst, and studied the effects of preparation method, active ingredient loading and reaction conditions on the CO-SCR performance of integral catalyst. The experimental results showed that the integral catalyst obtained by the heating and stirring method was better than the room temperature method. The conversion rates of CO and NO of the integral catalyst increased with the increase of the active ingredient loading. Besides, the oxygen concentration had little effect on the conversion rates of NO and CO. The conversion rate of CO to CO2 increased with the increase of temperature, and it could reach up to 98%. The conversion rate of NO to N2 fluctuated slightly as the temperature increased. © 2021 The Japan Society of Mechanical Engineers.

关键词： Selective catalytic reduction

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Experimental Study on Preparation of Amorphous SiO2 by Fluidized Bed Combstion of Rice Husk

Experimental Study on Preparation of Amorphous SiO2 by Fluid...

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International Conference on power engineering 2021, ICOPE 2021

作者： Tan, Jingkao Zhou, Qulan Yao, Yashu Li, Na State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University China

Rice husk ash contains SiO2 with a mass fraction of 87%-97%. Through controlled combustion under suitable conditions, SiO2 in rice husk ash will be amorphous, with high activity and rich porosity, which can be applied to construction, silicon preparation and adsorption *** it is necessary to study the effects of combustion parameters on the quality of RHA. Compared to conventional boiler furnace, the fluidized bed combustor has a lower combustion temperature and a longer residence time, which is suitable for the production of high quality amorphous rice husk ash. In this thesis, the effects of fluidized bed combustion parameters on the quality of RHA will be studied to provide guidance for amorphous SiO2 preparation by combustion control in boiler. On the existing 15kw bench-scale fluidized bed system, experiments were made to study the effects of fluidized bed combustion parameters on the quality of RHA. The rice husk combustion curve was comprehensively depicted, and the rice husk ash was analyzed by BET analysis, XRD scanning and thermogravimetric analysis. Therefore, the casual relationship between rice husk combustion process and RHA quality was evaluated comprehensively. © 2021 The Japan Society of Mechanical Engineers.

关键词： Quality control

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MULTIPLE SOLVERS FOR IMPLICIT TEMPERATURE CALCULATION OF HEAT CONDUCTION WITH THE MPS METHOD 15

MULTIPLE SOLVERS FOR IMPLICIT TEMPERATURE CALCULATION OF HEA...

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15th World Congress on Computational Mechanics and 8th Asian Pacific Congress on Computational Mechanics: Pursuing the Infinite Potential of Computational Mechanics, WCCM-APCOM 2022

作者： Li, Sijun Zhong, Yubao Cai, Qinghang Xiao, Xinkun Guo, Kailun Chen, Ronghua Tian, Wenxi Qiu, Suizheng Su, Guanghui School of Nuclear Science and Technology Shaanxi Key Laboratory of Advanced Nuclear Energy and Technology State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

In this study, an implicit algorithm and different solvers are applied to the Moving Particle Semi-Implicit (MPS) method for temperature calculation. The original MPS method uses an explicit method for temperature calculation and is limited by time increment due to diffusion number. In this paper, the heat conduction of plates with Dirichlet boundary condition and Neumann boundary condition is studied. The accuracy of explicit and implicit calculation of plate heat transfer cases are compared. In addition, different solvers are compared. Consequently, it is shown that the error of the implicit algorithm is not much different from the original one. And CG is still the better solver, CGS is also a superior solver. The implicit algorithm increases the size of a single time step by a maximum of 50 times (original diffusion number is 0.2), while the calculation time of a single time step does not increase Substantially, so it has a significant effect on the acceleration of calculation. © 2022 WCCM-APCOM 2022 - 15th World Congress on Computational Mechanics and 8th Asian Pacific Congress on Computational Mechanics: Pursuing the Infinite Potential of Computational Mechanics. All rights reserved.

关键词： Heat conduction

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Electrochemical evolution of a metal oxyhydroxide surface on two-dimensional layered metal phosphorus trisulfides enables the oxidation of amine to nitrile

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Carbon Energy 2025年第3期7卷 133-147页

作者： Binglan Wu Karim Harrath Marshet Getaye Sendeku Tofik Ahmed Shifa Yuxin Huang Jing Tai Fekadu Tsegaye Dajan Kassa Belay Ibrahim Xueying Zhan Zhenxing Wang Elisa Moretti Ying Yang Fengmei Wang Alberto Vomiero State Key Laboratory of Chemical Resource Engineering College of ChemistryBeijing University of Chemical TechnologyBeijingChina CAS Key Laboratory of Nanosystem and Hierarchical Fabrication National Center for Nanoscience and Technology(NCNST)BeijingChina Shaanxi Provincial Key Laboratory of Electroanalytical Chemistry Key Laboratory of Synthetic and Natural Functional Molecule of the Ministry of EducationCollege of Chemistry&Materials ScienceNorthwest UniversityXi'anChina State Key Laboratory of Multiphase Flow in Power Engineering International Research Center for Renewable EnergyXi'an Jiaotong UniversityShaanxiChina Fundamental Science Center of Rare Earths Ganjiang Innovation AcademyChinese Academy of ScienceGanzhouChina Ocean Hydrogen Energy R&D Center Research Institute of Tsinghua University in ShenzhenShenzhenChina Department of Molecular Sciences and Nanosystems Ca'Foscari University of VeniceVenezia MestreItaly Testing and Analysis Center Institute of Chemistry Chinese Academy of SciencesBeijingChina Department of Engineering Sciences and Mathematics Division of Materials ScienceLuleåUniversity of TechnologyLuleåSweden

Selective oxidation of amines to imines through electrocatalysis is an attractive and efficient way for the chemical industry to produce nitrile compounds,but it is limited by the difficulty of designing efficient catalysts and lack of understanding the mechanism of ***,we demonstrate a novel strategy by generation of oxyhydroxide layers on two-dimensional iron-doped layered nickel phosphorus trisulfides(Ni1-xFexPS_(3))during the oxidation of benzylamine(BA).In-depth structural and surface chemical characterizations during the electrocatalytic process combined with theoretical calculations reveal that Ni(1-x)FexPS_(3) undergoes surface reconstruction under alkaline conditions to form the metal oxyhydroxide/phosphorus trichalcogenide(NiFeOOH/Ni1-xFexPS_(3))***,the generated heterointerface facilitates BA oxidation with a low onset potential of 1.39 V and Faradaic efficiency of 53%for benzonitrile(BN)*** calculations further indicate that the as-formed NiFeOOH/Ni1-xFexPS_(3) heterostructure could offer optimum free energy for BA adsorption and BN desorption,resulting in promising BN synthesis.

关键词： 2D layered materials benzylamine oxidation metal phosphorus trichalcogenides surfacereconstructed heterostructure

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Reduction kinetics of SrFeO_(3−δ)/CaO∙MnO nanocomposite as effective oxygen carrier for chemical looping partial oxidation of methane

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Frontiers of Chemical Science and engineering 2022年第12期16卷 1726-1734页

作者： Xinhe Wang Liuqing Yang Xiaolin Ji Yunfei Gao Fanxing Li Junshe Zhang Jinjia Wei State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China School of Chemical Engineering and Technology Xi’an Jiaotong UniversityXi’an 710049China Institute of Clean Coal Technology East China University of Science and TechnologyShanghai 200237China Department of Chemical and Biomolecular Engineering North Carolina State UniversityRaleighNC 27695USA

Chemical looping reforming of methane is a novel and effective approach to convert methane to syngas,in which oxygen transfer is achieved by a redox *** lots of efforts have been made to develop high-performance redox materials,a few studies have focused on the redox *** this work,the kinetics of SrFeO_(3−δ)–CaO∙MnO nanocomposite reduction by methane was investigated both on a thermo-gravimetric analyzer and in a packed-bed *** the methane reduction,combustion occurs before the partial oxidation and there exists a transition between *** weight loss due to combustion increases,but the transition region becomes less inconspicuous as the reduction temperature *** weight loss associated with the partial oxidation is much larger than that with *** rate of weight loss related to the partial oxidation is well fitted by the Avrami–Erofeyev equation with n=3(A3 model)with an activation energy of 59.8 kJ∙mol^(‒1).The rate law for the partial oxidation includes a solid conversion term whose expression is given by the A3 model and a methane pressure-dependent term represented by a power *** partial oxidation is half order with respect to methane *** proposed rate law could well predict the reduction kinetics;thus,it may be used to design and/or analyze a chemical looping reforming reactor.

关键词： chemical looping reforming SrFeO_(3−δ) CaO·MnO nanocomposite reduction kinetics Avrami–Erofeyev model pressure-dependent term

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In Situ Synthesis of Cu_(3)P/P-Doped g-C_(3)N_(4)Tight 2D/2D Heterojunction Boosting Photocatalytic H2 Evolution

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Chinese Journal of Chemistry 2023年第2期41卷 173-180页

作者： Fangyong Hou Feng Liu Haochen Wu Muhammad Qasim Yi Chen Yang Duan Zhibo Feng Maochang Liu International Research Center for Renewable Energy&State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'anShaanxi 710049China School of Electronic Engineering Jiujiang UniversityJiujiangJiangxi 332005China Gree Altairnano New Energy Inc ZhuhaiGuangdong 519040China Suzhou Academy of Xi'an Jiao tong University SuzhouJiangsu 215123China

Heterojunction design in a two-dimensional(2D)fashion has been deemed beneficial for improving the photocatalytic activity of g-C_(3)N_(4)because of the promoted interfacial charge transfer,yet still facing ***,we construct a novel 2D/2D Cu_(3)P nanosheet/P-doped g-C_(3)N_(4)(PCN)nanosheet heterojunction photocatalyst(PCN/Cu_(3)P)through a simple in-situ phosphorization treatment of 2D/2D CuS/g-C_(3)N_(4)composite for photocatalytic H2 *** demonstrate that the 2D lamellar structure of both CuS and g-C_(3)N_(4)could be well reserved in the phosphorization process,while CuS and g-C_(3)N_(4)in-situ transformed into Cu_(3)P and PCN,respectively,leading to the formation of PCN/Cu_(3)P tight 2D/2D *** to the large contact area provided by intimate face-to-face 2D/2D structure,the PCN/Cu_(3)P photocatalyst exhibits significantly enhanced charge separation efficiency,thus achieving a boosted visible-light-driven photocatalytic *** highest rate for H2 evolution reaches 5.12 umol·h^(-1),nearly 24 times and 368 times higher than that of pristine PCN and g-C_(3)N_(4),*** work represents an excellent example in elaborately con-structing g-C_(3)N_(4)-based 2D/2D heterostructure and could be extended to other photocatalyst/co-catalyst system.

关键词： Photocatalysis Water splitting 2D/2D heterojunction g-C_(3)N_(4) Energy conversion Charge transfer Nanosheet photocatalyst

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Genetically engineered nifA mutations in Rhodobacter capsulatus to enhance ammonium tolerance and hydrogen production

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International Journal of Hydrogen Energy 2025年 144卷 252-261页

作者： Zixuan Gao Xintong Gao Yu Ma Zhixuan Jiao Minmin Wang Xuefang Mu Jiali Feng Wen Cao Liejin Guo State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 Shaanxi China College of Biology and Oceanography Weifang University Weifang 261061 Shandong China

NifA, the activator of nitrogenase, is sensitive to ammonium concentration, particularly within its N-terminal domain. In this work, genetically engineered mutants with N-terminal deletions of the nifA1 and nifA2 genes were constructed using overlap extension PCR to reduce the inhibitory effect of ammonium on nitrogenase expression in Rhodobacter capsulatus SB1003. Under 3 mM NH 4 + , the hydrogen production rate of ZX03 ( nifA1 - , nifA2 - ) reached 0.65 mmol L −1 h −1 , with a 31.2 % increase in hydrogen production compared to the wild-type. When 8 mM NH 4 + was used as the sole nitrogen source, H 2 production in all strains decreased substantially compared to 5 mM NH 4 + . However, ZX03 demonstrated a 5.2-fold enhancement in hydrogen production relative to the wild-type under 8 mM NH 4 + , underscoring its improved ammonium tolerance. During hydrogen production, the gene expression levels of nifA and nifH in all mutant strains were significantly up-regulated under ammonium conditions compared to the wild-type. These findings reveal distinct roles of nifA1 and nifA2 in ammonium tolerance and hydrogen production.

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Toward the influence of fluid convection on filtered drag force in fluidized gas-particle flows

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Powder Technology 2025年 460卷

作者： Jiang, Ju Yuan, Shouzheng Chen, Xiao Yang, Bolun Zhou, Qiang School of Chemical Engineering and Technology Xi'an Jiaotong University Xi'an710049 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

Mesoscale drag modeling for gas-solid flows is typically based on fully-periodic systems where fluid convection is insignificant. This study examines a series of 2D sudden-expanded fluidized beds (SEFBs) to investigate the effects of fluid convection on the filtered drag force. A priori analysis indicates that the volumetric force induced by convection has a notable impact on the filtered drag force, and correlations of drag force using traditional markers (such as solid volume fraction, slip velocity, and filter size) fail to provide accurate predictions. In contrast, the gas-phase pressure gradient shows a good correlation with drag force when strong convection is present. Posterior tests in the SEFBs with several existing drag models reveal that the predictive capacity of drag models constructed with traditional markers declines under conditions with strong convection, whereas the drag model incorporating the gas-phase pressure gradient still performs well. © 2025 Elsevier B.V.

关键词： Drag coefficient

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