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Defined High Molar Mass Poly(2‐Oxazoline)s

Angewandte Chemie 2018年第47期130卷

作者： Bryn D. Monnery Valentin V. Jerca Ondrej Sedlacek Bart Verbraeken Rachel Cavill Richard Hoogenboom Supramolecular Chemistry Group Centre of Macromolecular Chemistry (CMaC) Department of Organic and Macromolecular Chemistry Ghent University Krijgslaan 281—S4 9000 Gent Belgium Centre of Organic Chemistry “Costin D. Nenitzescu” Romanian Academy Spl. Independentei 202B 060023 Bucharest Romania Department of Data Science and Knowledge Engineering Maastricht University Bouillonstraat 8–10 6211 LH Maastricht The Netherlands

Poly(2‐alkyl‐2‐oxazoline)s (PAOx) are regaining interest for biomedical applications. However, their full potential is hampered by the inability to synthesise uniform high‐molar mass PAOx. In this work, we proposed alternative intrinsic chain transfer mechanisms based on 2‐oxazoline and oxazolinium chain‐end tautomerisation and derived improved polymerization conditions to suppress chain transfer, allowing the synthesis of highly defined poly(2‐ethyl‐2‐oxazoline)s up to ca. 50 kDa (dispersity ( Ð ) <1.05) and defined polymers up to at least 300 kDa ( Ð <1.2). The determination of the chain transfer constants for the polymerisations hinted towards the tautomerisation of the oxazolinium chain end as most plausible cause for chain transfer. Finally, the method was applied for the preparation of up to 60 kDa molar mass copolymers of 2‐ethyl‐2‐oxazoline and 2‐methoxycarbonylethyl‐2‐oxazoline.

关键词： Kationische Polymerisationen Polymere Ringöffnungspolymerisationen Tautomerisierungen

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Author Correction: Altered structural brain asymmetry in autism spectrum disorder in a study of 54 datasets

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Nature communications 2021年第1期12卷 7260页

作者： Merel C Postema Daan van Rooij Evdokia Anagnostou Celso Arango Guillaume Auzias Marlene Behrmann Geraldo Busatto Filho Sara Calderoni Rosa Calvo Eileen Daly Christine Deruelle Adriana Di Martino Ilan Dinstein Fabio Luis S Duran Sarah Durston Christine Ecker Stefan Ehrlich Damien Fair Jennifer Fedor Xin Feng Jackie Fitzgerald Dorothea L Floris Christine M Freitag Louise Gallagher David C Glahn Ilaria Gori Shlomi Haar Liesbeth Hoekstra Neda Jahanshad Maria Jalbrzikowski Joost Janssen Joseph A King Xiang Zhen Kong Luisa Lazaro Jason P Lerch Beatriz Luna Mauricio M Martinho Jane McGrath Sarah E Medland Filippo Muratori Clodagh M Murphy Declan G M Murphy Kirsten O'Hearn Bob Oranje Mara Parellada Olga Puig Alessandra Retico Pedro Rosa Katya Rubia Devon Shook Margot J Taylor Michela Tosetti Gregory L Wallace Fengfeng Zhou Paul M Thompson Simon E Fisher Jan K Buitelaar Clyde Francks Department of Language & Genetics Max Planck Institute for Psycholinguistics Nijmegen The Netherlands. Department of Cognitive Neuroscience Donders Institute for Brain Cognition and Behaviour Donders Centre for Cognitive Neuroimaging Radboud University Medical Centre Nijmegen The Netherlands. Bloorview Research Institute Holland Bloorview Kids Rehabilitation Hospital and Department of Pediatrics University of Toronto Toronto ON USA. Child and Adolescent Psychiatry Department Gregorio Marañón General University Hospital School of Medicine Universidad Complutense IiSGM CIBERSAM Madrid Spain. Institut de Neurosciences de la Timone UMR 7289 Aix Marseille Université CNRS Marseille France. Department of Psychology Carnegie Mellon University Pittsburgh PA USA. Laboratory of Psychiatric Neuroimaging (LIM-21) Departamento e Instituto de Psiquiatria Hospital das Clinicas HCFMUSP Faculdade de Medicina Universidade de Sao Paulo Sao Paulo SP Brazil. IRCCS Stella Maris Foundation viale del Tirreno 331 56128 Pisa Italy. Department of Clinical and Experimental Medicine University of Pisa Pisa Italy. Department of Child and Adolescent Psychiatry and Psychology Hospital Clinic Psychiatry Unit Department of Medicine 2017SGR881 University of Barcelona IDIBAPS CIBERSAM Barcelona Spain. Department of Forensic and Neurodevelopmental Sciences Institute of Psychiatry Psychology & Neuroscience King's College London London UK. Institute for Pediatric Neuroscience NYU Child Study Center New York NY USA. Department of Psychology Ben-Gurion University of the Negev Beer Sheva Israel. Brain Center Rudolf Magnus Department of Psychiatry University Medical Center Utrecht Utrecht The Netherlands. Department of Child and Adolescent Psychiatry Psychosomatics and Psychotherapy University Hospital Goethe University Frankfurt am Main Frankfurt Germany. Imaging Genetics Center Mark and Mary Stevens Neuroimaging and Informatics Institute Keck School of Medicine of USC University o

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Identifying the best machine learning algorithms for brain tumor segmentation, progression assessment, and overall survival prediction in the BRATS challenge

arXiv

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arXiv 2018年

作者： Bakas, Spyridon Reyes, Mauricio Jakab, Andras Bauer, Stefan Rempfler, Markus Crimi, Alessandro Shinohara, Russell Takeshi Berger, Christoph Ha, Sung Min Rozycki, Martin Prastawa, Marcel Alberts, Esther Lipkova, Jana Freymann, John Kirby, Justin Bilello, Michel Fathallah-Shaykh, Hassan M. Wiest, Roland Kirschke, Jan Wiestler, Benedikt Colen, Rivka Kotrotsou, Aikaterini Lamontagne, Pamela Marcus, Daniel Milchenko, Mikhail Nazeri, Arash Weber, Marc-Andr Mahajan, Abhishek Baid, Ujjwal Gerstner, Elizabeth Kwon, Dongjin Acharya, Gagan Agarwal, Manu Alam, Mahbubul Albiol, Alberto Albiol, Antonio Albiol, Francisco J. Alex, Varghese Allinson, Nigel Amorim, Pedro H.A. Amrutkar, Abhijit Anand, Ganesh Andermatt, Simon Arbel, Tal Arbelaez, Pablo Avery, Aaron Azmat, Muneeza Pranjal, B. Bai, Wenjia Banerjee, Subhashis Barth, Bill Batchelder, Thomas Batmanghelich, Kayhan Battistella, Enzo Beers, Andrew Belyaev, Mikhail Bendszus, Martin Benson, Eze Bernal, Jose Bharath, Halandur Nagaraja Biros, George Bisdas, Sotirios Brown, James Cabezas, Mariano Cao, Shilei Cardoso, Jorge M. Carver, Eric N. Casamitjana, Adri Castillo, Laura Silvana Cat, Marcel Cattin, Philippe Cérigues, Albert Chagas, Vinicius S. Chandra, Siddhartha Chang, Yi-Ju Chang, Shiyu Chang, Ken Chazalon, Joseph Chen, Shengcong Chen, Wei Chen, Jefferson W. Chen, Zhaolin Cheng, Kun Choudhury, Ahana Roy Chylla, Roger Clrigues, Albert Colleman, Steven Colmeiro, Ramiro German Rodriguez Combalia, Marc Costa, Anthony Cui, Xiaomeng Dai, Zhenzhen Dai, Lutao Daza, Laura Alexandra Deutsch, Eric Ding, Changxing Dong, Chao Dong, Shidu Dudzik, Wojciech Eaton-Rosen, Zach Egan, Gary Escudero, Guilherme Estienne, Tho Everson, Richard Fabrizio, Jonathan Fan, Yong Fang, Longwei Feng, Xue Ferrante, Enzo Fidon, Lucas Fischer, Martin French, Andrew P. Fridman, Naomi Fu, Huan Fuentes, David Gao, Yaozong Gates, Evan Gering, David Gholami, Amir Gierke, Willi Glocker, Ben Gong, Mingming Gonzlez-Vill, Sandra Grosges, T. Guan, Yuanfang Guo, Sheng Gupta, Sudeep Han, Woo-Sup Han, Il Song Harmuth, Ko Center for Biomedical Image Computing and Analytics University of Pennsylvania PhiladelphiaPA United States Department of Radiology Perelman School of Medicine University of Pennsylvania PhiladelphiaPA United States Department of Pathology and Laboratory Medicine Perelman School of Medicine University of Pennsylvania PhiladelphiaPA United States Institute for Surgical Technology and Biomechanics University of Bern Bern Switzerland Center for MR-Research University Children's Hospital Zurich Zurich Switzerland Support Centre for Advanced Neuroimaging Inselspital Institute for Diagnostic and Interventional Neuroradiology Bern University Hospital Bern Switzerland University Hospital of Zurich Zurich Switzerland Center for Clinical Epidemiology and Biostatistics University of Pennsylvania Philadelphia United States Image-Based Biomedical Modeling Group Technical University of Munich Munich Germany Icahn School of Medicine Mount Sinai Health System New YorkNY United States Leidos Biomedical Research Inc. Frederick National Laboratory for Cancer Research FrederickMD21701 United States Cancer Imaging Program National Cancer Institute National Institutes of Health BethesdaMD20814 United States Department of Neurology University of Alabama at Birmingham BirminghamAL United States Department of Diagnostic Radiology University of Texas MD Anderson Cancer Center HoustonTX United States Department of Psychology Washington University St. LouisMO United States Neuroimaging Informatics and Analysis Center Washington University St. LouisMO United States Department of Radiology Washington University St. LouisMO United States Institute of Diagnostic and Interventional Radiology Pediatric Radiology and Neuroradiology University Medical Center Rostock Ernst-Heydemann-Str. 6 Rostock18057 Germany Tata Memorial Centre Homi Bhabha National Institute Mumbai India Shri Guru Gobind Singhji Institute of Engineering and Technology Nanded India NVIDIA Santa Clara

Gliomas are the most common primary brain malignancies, with different degrees of aggressiveness, variable prognosis and various heterogeneous histologic sub-regions, i.e., peritumoral edematous/invaded tissue, necrotic core, active and non-enhancing core. This intrinsic heterogeneity is also portrayed in their radio-phenotype, as their sub-regions are depicted by varying intensity profiles disseminated across multi-parametric magnetic resonance imaging (mpMRI) scans, reflecting varying biological properties. Their heterogeneous shape, extent, and location are some of the factors that make these tumors difficult to resect, and in some cases inoperable. The amount of resected tumor is a factor also considered in longitudinal scans, when evaluating the apparent tumor for potential diagnosis of progression. Furthermore, there is mounting evidence that accurate segmentation of the various tumor sub-regions can offer the basis for quantitative image analysis towards prediction of patient overall survival. This study assesses the state-of-the-art machine learning (ML) methods used for brain tumor image analysis in mpMRI scans, during the last seven instances of the International Brain Tumor Segmentation (BraTS) challenge, i.e., 2012-2018. Specifically, we focus on i) evaluating segmentations of the various glioma sub-regions in pre-operative mpMRI scans, ii) assessing potential tumor progression by virtue of longitudinal growth of tumor sub-regions, beyond use of the RECIST/RANO criteria, and iii) predicting the overall survival from pre-operative mpMRI scans of patients that underwent gross total resection. Finally, we investigate the challenge of identifying the best ML algorithms for each of these tasks, considering that apart from being diverse on each instance of the challenge, the multi-institutional mpMRI BraTS dataset has also been a continuously evolving/growing dataset. Copyright © 2018, The Authors. All rights reserved.

关键词： Tumors

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Spatiotemporal activation time estimation improves noninvasive localization of cardiac electrical activity

Spatiotemporal activation time estimation improves noninvasi...

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computers in Cardiology (CinC)

作者： Matthijs J.M. Cluitmans Jaume Coll-Font Burak Erem Dana Brooks Pietro Bonizzi Joël M.H. Karel Paul G.A. Volders Ralf L.M. Peeters Ronald L. Westra Department of Data Science and Knowledge Engineering Maastricht University Maastricht The Netherlands Department of Electrical & Computer Engineering Northeastern University Boston MA USA Boston Childrens Hospital Harvard Medical School Boston MA USA Department of Data Science and Knowledge Engineering Maastricht University The Netherlands CARIM School for Cardiovascular Diseases Maastricht University The Netherlands

ISBN: (纸本)9781509008964

Electrocardiographic imaging (ECGI) reconstructs epicardial potentials and electrograms from body-surface electrocardiograms and a torso-heart geometry. For clinical purposes, local activation and recovery times are often more useful than epicardial electrograms. However, noise and fractionation can affect estimation of activation and recovery times from reconstructed electrograms. Here, we employ a method for activation and recovery time estimation that detects the simultaneous presence of spatial and temporal features associated with a passing wavefront and evaluate this in a series of canine experiments. We show that estimation of activation times is more accurate when this spatiotemporal approach is used, however, recovery times are best determined with a temporal-only approach. Additional spatial smoothing further benefits activation and recovery time estimation in all cases. This results in a median beat origin localization error of only one centimeter, which could expedite catheter-based diagnostic evaluation and ablation in clinical settings.

关键词： Estimation Smoothing methods Spatiotemporal phenomena Electric potential Heart Imaging Electrodes

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Preface

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Lecture Notes in computer science (including subseries Lecture Notes in Artificial Intelligence and Lecture Notes in Bioinformatics) 2017年 10664 LNCS卷 V-X页

作者： Winands, Mark H. M. van den Herik, Jaap Kosters, Walter A. Department of Data Science and Knowledge Engineering Maastricht University MaastrichtLimburg Netherlands Leiden Centre of Data Science Leiden University LeidenZuid-Holland Netherlands Leiden Institute of Advanced Computer Science Leiden University LeidenZuid-Holland Netherlands

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SHREC'16 Track: Partial Shape Queries for 3D object retrieval 9

SHREC'16 Track: Partial Shape Queries for 3D object retrieva...

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9th Eurographics Workshop on 3D Object Retrieval, 3DOR 2016

作者： Pratikakis, I. Savelonas, M.A. Arnaoutoglou, F. Ioannakis, G. Koutsoudis, A. Theoharis, T. Tran, M.-T. Nguyen, V.-T. Pham, V.-K. Nguyen, H.-D. Le, H.-A. Tran, B.-H. To, Q.H. Truong, M.-B. Phan, T.V. Nguyen, M.-D. Than, T.-A. Mac, K.-N.C. Do, M.N. Duong, A.-D. Furuya, T. Ohbuchi, R. Aono, M. Tashiro, S. Pickup, D. Sun, X. Rosin, P.L. Martin, R.R. Democritus University of Thrace Department of Electrical and Computer Engineering Greece ATHENA Research Center Institute for Language and Speech Processing Greece Norwegian University of Science and Technology Department of Computer and Information Science Norway University of Science VNU-HCM Viet Nam University of Science University of Information Technology VNU-HCM Viet Nam University of Science John von Neumann Institute VNU-HCM Viet Nam University of Illinois Urbana-Champaign United States University of Information Technology VNU-HCM Viet Nam Graduate School of Medicine and Engineering University of Yamanashi Japan Knowledge Data Engineering Lab. Toyohashi University of Technology Japan School of Computer Science and Informatics Cardiff University United Kingdom

ISBN: (纸本)9783038680048

Despite numerous recent efforts, 3D object retrieval based on partial shape queries remains a challenging problem, far from being solved. The problem can be defined as: given a partial view of a shape as query, retrieve all partially similar 3D models from a repository. The objective of this track is to evaluate the performance of partial 3D object retrieval methods, for partial shape queries of various scan qualities and degrees of partiality. The retrieval problem is often found in cultural heritage applications, for which partial scans of objects query a dataset of geometrically distinct classes. © 2016 The Eurographics Association.

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Biogeography-based optimization for cluster analysis

Biogeography-based optimization for cluster analysis

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International Conference on computer, Communication and Computational sciences, ICCCCS 2016

作者： Wu, Xueyan Wang, Hainan Chen, Zhimin Lu, Zhihai Phillips, Preetha Wang, Shuihua Zhang, Yudong School of Computer Science and Technology Nanjing Normal University NanjingJiangsu210023 China Key Laboratory of Statistical Information Technology & Data Mining State Statistics Bureau ChengduSichuan610225 China School of Computer and Information Engineering Henan Normal University XinxiangHenan453000 China School of Electronic Information Shanghai Dianji University Shanghai200240 China Key Laboratory of Symbolic Computation & Knowledge Engineering of Ministry of Education Jilin University ChangchunJilin130012 China Guangxi Key Laboratory of Manufacturing System & Advanced Manufacturing Technology GuilinGuangxi541004 China School of Natural Sciences and Mathematics Shepherd University ShepherdstownWV25443 United States West Virginia School of Osteopathic Medicine 400 N Lee St LewisburgWV24901 United States Department of Electrical Engineering The City College of New York CUNY New YorkNY10031 United States State Key Lab of CAD & CG Zhejiang University HangzhouZhejiang310027 China Manchester Metropolitan University ManchesterM156BH United Kingdom

ISBN: (纸本)9789811037696

With the aim of resolving the issue of cluster analysis more precisely and validly, a new approach was proposed based on biogeography-based optimization (abbreviated as BBO) algorithm. (Method) First, we reformulated the problem with an optimization model based on the variance ratio criterion (VARAC). Then, BBO was presented to search the optimal solution of the VARAC. There are 400 data of four groups in the experimental dataset, which have the degrees of overlapping of three distinct scales. The first one is nonoverlapping, the second one is partial overlapping, and the last is severely overlapping. BBO algorithm was compared with three different state-of-the-art approaches. We ran every algorithm 20 times. In this experiment, our results demonstrate the maximum VARAC values that can be found by BBO. The conclusion is that BBO is predominant which is extremely quick for the issue of clustering analysis. © Springer Nature Singapore Pte Ltd. 2017.

关键词： Cluster analysis

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Introduction

Lecture Notes in Computer Science (including subseries Lectu...

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Lecture Notes in computer science (including subseries Lecture Notes in Artificial Intelligence and Lecture Notes in Bioinformatics) 2016年 9792 LNCS卷 1-8页

作者： González-Beltrán, Alejandra Osborne, Francesco Peroni, Silvio Oxford e-Research Centre University of Oxford Oxford United Kingdom Data Science Group Knowledge Media Institute The Open University Milton Keynes United Kingdom Digital and Semantic Publishing Laboratory Department of Computer Science and Engineering University of Bologna Bologna Italy

We provide the motivation and overview of the SAVE-SD workshop series and introduce the manuscripts that were accepted as part of these proceedings of the SAVE-SD 2016 edition. © Springer International Publishing...

ISBN: (纸本)9783319536361

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Preface

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CEUR Workshop Proceedings 2017年 1935卷

作者： Bastianelli, Emanuele D'Aquin, Mathieu Nardi, Daniele Knowledge Media Institute Open University United Kingdom Insight Centre for Data Analytics National University of Ireland Galway Ireland Department of Computer Science Control and Management Engineering Sapienza University of Rome Italy

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A framework to provide customized reuse of open corpus content for adaptive systems 15

A framework to provide customized reuse of open corpus conte...

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26th ACM Conference on Hypertext and Social Media, HT 2015

作者： Bayomi, Mostafa CNGL Centre for Global Intelligent Content Knowledge and Data Engineering Group School of Computer Science and Statistics Trinity College Dublin Ireland

ISBN: (纸本)9781450333955

One of the main services that Adaptive Systems offer to their users is the provision of content that is tailored to individual user's needs. Some Adaptive Systems use a closed corpus content that has been prepared for them a priori, hence, they accept only a narrow field of content. Furthermore, the content is tightly coupled with other parts of the system, which also hinders its reusability. To address these limitations, recent systems started to make use of open Web content to provide a wider variety of content. Previous approaches have attempted to harness the information available on the web by providing adaptive systems with customizable information objects. Since adaptive systems are evolving towards the Semantic Web and the use of ontologies, existing systems are limited by their ability to service these documents solely through keyword-based queries. In this research we propose a novel framework that extends existing content provision system, Slicepedia. Our framework uses the conceptual representation of content to segment it in a semantic manner. The framework removes unnecessary content from web pages, such as navigation bars, and then semantically reveals the structural representation of text to build a tree-like hierarchy. This tree can be traversed to obtain different levels of content granularity that facilitate content discoverability and adaptivity. © 2015 ACM.

关键词： Adaptive systems

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