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Lead-free perovskite Cs_(2)AgBiBr_(6)photodetector detecting NIR light driven by titanium nitride plasmonic hot holes

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Photonics Research 2024年第3期12卷 522-533页

作者： ZIJIAN LIU YUYING XI WENBO ZENG TING JI WENYAN WANG SITONG GUO LINLIN SHI RONG WEN YANXIA CUI GUOHUI LI College of Physics College of Electronic Information and Optical EngineeringKey Laboratory of Advanced Transducers and Intelligent Control System of Ministry of EducationTaiyuan University of TechnologyTaiyuan 030024China Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan 030032China

Lead-free perovskite Cs_(2)AgBiBr_(6)manifests great potential in developing high-performance,environmentally friendly,solution-processable photodetectors(PDs).However,due to the relatively large energy bandgap,the spectrum responses of Cs_(2)AgBiBr_(6)PDs are limited to the ultraviolet and visible region with wavelengths shorter than 560 *** this work,a broadband Cs_(2)AgBiBr_(6)PD covering the ultraviolet,visible,and near infrared(NIR)range is demonstrated by incorporating titanium nitride(TiN)nanoparticles that are prepared with the assistance of self-assembled polystyrene sphere *** addition,an atomically thick Al2O3layer is introduced at the interface between the Cs_(2)AgBiBr_(6)film and TiN nanoparticles to alleviate the dark current deterioration caused by nanoparticle *** a result,beyond the spectrum range where Cs_(2)AgBiBr_(6)absorbs light,the external quantum efficiency(EQE)of the TiN nanoparticle incorporated Cs_(2)AgBiBr_(6)PD is enhanced significantly compared with that of the control,displaying enhancement factors as high as 2000 over a broadband NIR wavelength *** demonstrated enhancement in EQE arises from the photocurrent contribution of plasmonic hot holes injected from TiN nanoparticles into Cs_(2)AgBiBr_(6).This work promotes the development of broadband solution-processable perovskite PDs,providing a promising strategy for realizing photodetection in the NIR region.

关键词： perovskite titanium ultraviolet

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High-performance self-powered ultraviolet to near-infrared photodetector based on WS_(2)/InSe van der Waals heterostructure

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Nano Research 2023年第5期16卷 7851-7857页

作者： Jinping Chen Zhen Zhang Yi Ma Jiying Feng Xiaoyu Xie Xiaoxuan Wang Aoqun Jian Yuanzheng Li Zhuxin Li Heng Guo Yizhi Zhu Qiannan Cui Zengliang Shi Chunxiang Xu State Key Laboratory of Bioelectronics School of Biological Science and Medical EngineeringSoutheast UniversityNanjing 210096China Micro Nano System Research Center Key Laboratory of Advanced Transducers and Intelligent Control System of the Ministry of Education&College of Information Engineering and ComputerTaiyuan University of TechnologyTaiyuan 030024China Key Laboratory of UV-Emitting Materials and Technology of Ministry of Education Northeast Normal UniversityChangchun 130024China

van der Waals heterostructures(vdWHs)based on two-dimensional(2D)materials without the crystal lattice matching constraint have great potential for high-performance optoelectronic ***,a WS_(2)/InSe vdWH photodiode is proposed and fabricated by precisely stacking InSe and WS_(2)flakes through an all-dry transfer *** WS_(2)/InSe vdWH forms an n–n heterojunction with strong built-in electric field due to their intrinsic n-type semiconductor characteristics and energy-band alignments with a large Fermi level offset between WS_(2)and *** a result,the device displays excellent photovoltaic behavior with a large open voltage of 0.47 V and a short-circuit current of 11.7 nA under 520 nm light ***,a fast rising/decay time of 63/76μs,a large light on/off ratio of 105,a responsivity of 61 mA/W,a high detectivity of 2.5×10^(11) Jones,and a broadband photoresponse ranging from ultraviolet to near-infrared(325–980 nm)are achieved at zero *** study provides a strategy for developing high-performance self-powered broadband photodetectors based on 2D materials.

关键词： two-dimensional materials van der Waals heterostructure self-powered photodetector photocurrent

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Broadband Optical Nonlinearities and Ultrafast Carrier Dynamics of GO-CuS Hybrid Film

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Journal of Lightwave Technology 2025年第11期43卷 5381-5389页

作者： Zhang, Xuefeng Bai, Xuli Liu, Xiaofei Wang, Dan Han, Hong Xiao, Zhengguo Zhang, Jianguo Nie, Zhongquan Taiyuan University of Technology College of Materials Science and Engineering Institute of New Carbon Materials Taiyuan030024 China Taiyuan University of Technology Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Electronic Information and Optical Engineering Taiyuan030024 China Taiyuan Institute of Technology Department of Science Taiyuan030008 China Tongren University Department of Physics and Electronic Engineering Tongren China National University of Defense Technology College of Advanced Interdisciplinary Studies Changsha410073 China

We report the broadband optical nonlinearities and ultrafast carrier dynamics of GO doped with CuS nanoparticles (GO-CuS) following the femtosecond pulse lasers. Both the pure GO and GO-CuS hybrid films are first synthesized by the vacuum filter deposition method and their optical nonlinearities are then examined in the wide wavelength range (400 nm-1064 nm) based on the femtosecond Z-scan technique. The results reveal that, compared to the pristine GO, the introduction of CuS not only makes the GO-CuS hybrid film switched from saturated absorption to reverse saturated absorption possible, but also achieves strong broadband optical nonlinear absorption responses and optical limiting effects. It is demonstrated that the strongest nonlinear absorption coefficient (∼3.6×10-7 m/W) appears at 400 nm excitation, which is dozens of times larger than that under the illumination of 1064 nm. By leveraging the femtosecond pump-probe technique, we further study the ultrafast carrier dynamics of the GO-CuS hybrid film carrying the fast and slow relaxation processes. Moreover, the physical mechanisms behind these excellent nonlinear optical responses are elucidated. The findings presented here indicate that the GO-CuS hybrid film can be regarded as a potential promising candidate in various ultrafast photonics devices. © 1983-2012 IEEE.

关键词： Femtosecond lasers

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Grain size control in quasi-two-dimensional perovskite thin film via intermediate phase engineering for efficient bound exciton generation

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Science China Materials 2024年第12期67卷 3925-3931页

作者： Guohui Li Wenhui Zhao Kai Lin Kefan Zhao Yujing Wang Aohua Niu Rong Weng Kaibo Zheng Yanxia Cui College of Electronic Information and Optical Engineering Key Laboratory of Interface Science and Engineering in Advanced MaterialsKey Lab of Advanced Transducers and Intelligent Control System of Ministry of EducationTaiyuan University of TechnologyTaiyuan 030024China Chemical Physics Division and NanoLund Lund UniversityBox 12422100LundSweden

Quasi-two dimensional(2D)perovskites have emerged as a promising class of materials due to their remarkable photoluminescence efficiency,which stems from their exceptionally high exciton binding *** spatial confinement of excitons within smaller grain sizes could enhance the formation of biexcitons leading to higher radiative recombination ***,the synthesis of high-quality quasi-2D perovskite thin films with controllable grain sizes remains a challenging *** this study,we present a facile method for achieving quasi-2D perovskite thin films with controllable grain sizes ranging from 500 to 900 *** is accomplished by intermediate phase engineering during the film fabrication *** results demonstrate that quasi-2D perovskite films with smaller grain sizes exhibit more efficient bound exciton generation and a reduced stimulated emission threshold down to 15.89µJ cm^(−2).Furthermore,femtosecond transient absorption measurements reveal that the decay time of bound excitons is shorter in quasi-2D perovskites with smaller grain sizes compared to that of those with larger grains at the same pump density,which is 230.5 *** observation suggests a more efficient exciton recombination process in the smaller grain size *** findings would offer a promising approach for the development of efficient bound exciton lasers.

关键词： quasi-2D perovskite intermediate phase engineering bound exciton generation grain size control

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Boosting external quantum efficiency of a WSe_(2) photodetector across visible and NIR spectra through harnessing plasmonic hot electrons

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Photonics Research 2024年第9期12卷 1846-1857页

作者： LINLIN SHI ZIYANG ZHAO JINYANG JIAO TING JI WENYAN WANG YANXIA CUI GUOHUI LI College of Electronic Information and Optical Engineering Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of EducationKey Laboratory of Advanced Transducers and Intelligent Control System of Ministry of EducationTaiyuan University of TechnologyTaiyuan 030024China Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan 030032China

The layered two-dimensional material tungsten diselenide(WSe_(2))has triggered tremendous interests in the field of optoelectronic devices due to its exceptional carrier transport ***,the limited absorption of WSe_(2) in the near infrared(NIR)band poses a challenge for the application of WSe_(2) photodetectors in night vision,telecommunication,***,the enhanced performance of the WSe_(2) photodetector is demonstrated through the incorporation of titanium nitride nanoparticles(TiN NPs),complemented by an atomically-thick Al_(2)O_(3) layer that aids in suppressing the dark *** is demonstrated that TiN NPs can dramatically enhance the absorption of light in the proposed WSe_(2) photodetector in the NIR *** enhancement boosts photocurrent responses through the generation of plasmonic hot electrons,leading to external quantum efficiency(EQE)enhancement factors of 379.66%at 850 nm and 178.47%at 1550 *** work presents,for the first time,to our knowledge,that the WSe_(2) photodetector is capable of detecting broadband light spanning from ultraviolet to the telecommunication range,all achieved without the reliance on additional semiconductor *** achievement opens avenues for the advancement of cost-effective NIR photodetectors.

关键词： quantum titanium exceptional

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3D bioprinting of in vitro porous hepatoma models:establishment,evaluation,and anticancer drug testing

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Bio-Design and Manufacturing 2024年第2期7卷 137-152页

作者： Xiaoyuan Wang Zixian Liu Qianqian Duan Boye Zhang Yanyan Cao Zhizhong Shen Meng Li Yanfeng Xi Jianming Wang Shengbo Sang Shanxi Key Laboratory of Micro Nano Sensors and Artificial Intelligence Perception College of Electronic Information and Optical EngineeringTaiyuan University of TechnologyTaiyuan 030024China Key Lab of Advanced Transducers and Intelligent Control System of the Ministry of Education Taiyuan University of TechnologyTaiyuan 030024China Shanxi Institute of 6D Artificial Intelligence Biomedical Science Taiyuan 030031China Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan 030024China Department of Pathology Shanxi Provincial Cancer HospitalTaiyuan 030024China General Hospital of Taiyuan Iron and Steel Company Taiyuan 030809China

Traditional tumor models do not tend to accurately simulate tumor growth in vitro or enable personalized treatment and are particularly unable to discover more beneficial targeted *** address this,this study describes the use of threedimensional(3D)bioprinting technology to construct a 3D model with human hepatocarcinoma SMMC-7721 cells(3DP-7721)by combining gelatin methacrylate(GelMA)and poly(ethylene oxide)(PEO)as two immiscible aqueous phases to form a bioink and innovatively applying fluorescent carbon quantum dots for long-term tracking of *** GelMA(10%,mass fraction)and PEO(1.6%,mass fraction)hydrogel with 3:1 volume ratio offered distinct pore-forming characteristics,satisfactorymechanical properties,and biocompatibility for the creation of the 3DP-7721 *** analysis and quantitative real-time fluorescence polymerase chain reaction(PCR)were used to evaluate the biological properties of the *** with the two-dimensional culture cell model(2D-7721)and the 3D mixed culture cell model(3DM-7721),3DP-7721 significantly improved the proliferation of cells and expression of tumor-related proteins and ***,we evaluated the differences between the three culture models and the effectiveness of antitumor drugs in the three models and discovered that the efficacy of antitumor drugs varied because of significant differences in resistance proteins and genes between the three *** addition,the comparison of tumor formation in the three models found that the cells cultured by the 3DP-7721 model had strong tumorigenicity in nude *** evaluation of the levels of biochemical indicators related to the formation of solid tumors showed that the 3DP-7721 model group exhibited pathological characteristics of malignant tumors,the generated solid tumors were similar to actual tumors,and the deterioration was *** research therefore acts as a foundation for the application of 3DP-7721 models in drug devel

关键词： 3D bioprinting Hepatoma tumor models Drug screening Antitumor drug development

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Simultaneously realizing thermal and electromagnetic cloaking by multi-physical null medium

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Opto-Electronic Science 2024年第2期3卷 45-59页

作者： Yichao Liu Xiaomin Ma Kun Chao Fei Sun Zihao Chen Jinyuan Shan Hanchuan Chen Gang Zhao Shaojie Chen Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi ProvinceCollege of Electronic Information and Optical EngineeringTaiyuan University of TechnologyTaiyuan 030024China

Simultaneously manipulating multiple physical fields plays an important role in the increasingly complex integrated systems,aerospace equipment,biochemical productions,*** on-chip systems with high integration level,the precise and efficient control of the propagation of electromagnetic waves and heat fluxes simultaneously is particularly *** this study,we propose a graphical designing method(i.e.,thermal-electromagnetic surface transformation)based on thermal-electromagnetic null medium to simultaneously control the propagation of electromagnetic waves and thermal fields according to the pre-designed paths.A thermal-electromagnetic cloak,which can create a cloaking effect on both electromagnetic waves and thermal fields simultaneously,is designed by thermal-electromagnetic surface transformation and verified by both numerical simulations and experimental *** thermal-electromagnetic surface transformation proposed in this study provides a new methodology for simultaneous controlling on electromagnetic and temperature fields,and may have significant applications in improving thermal-electromagnetic compatibility problem,protecting of thermal-electromagnetic sensitive components,and improving efficiency of energy usage for complex onchip systems.

关键词： transformation optics multi-physical cloak null medium

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3D printed-electrospun PCL/hydroxyapatite/MWCNTs scaffolds for the repair of subchondral bone

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Regenerative Biomaterials 2023年第1期10卷 294-305页

作者： Yanyan Cao Lei Sun Zixian Liu Zhizhong Shen Wendan Jia Peiyi Hou Shengbo Sang College of Information Science and Engineering Hebei North UniversityZhangjiakou 075000China Shanxi Key Laboratory of Micro Nano Sensors&Artificial Intelligence Perception College of Information and ComputerTaiyuan University of TechnologyTaiyuan 030024China Key Lab of Advanced Transducers and Intelligent Control System of the Ministry of Education Taiyuan University of TechnologyTaiyuan 030024China Shanxi Research Institute of 6D Artificial Intelligence Biomedical Science Taiyuan 030031China

Osteochondral defect caused by trauma or osteoarthritis exhibits a major challenge in clinical treatment with limited symptomatic effects at *** regeneration and remodeling of subchondral bone play a positive effect on cartilage regeneration and further promotes the repair of osteochondral *** use of the strengths of each preparation method,the combination of 3D printing and electrospinning is a promising method for designing and constructing multi-scale scaffolds that mimic the complexity and hierarchical structure of subchondral bone at the microscale and nanoscale,*** this study,the 3D printed-electrospun poly(ɛ-caprolactone)/nano-hydroxyapatites/multi-walled carbon nanotubes(PCL/nHA/MWCNTs)scaffolds were successfully constructed by the combination of electrospinning and layer-by-layer 3D *** resulting dual-scale scaffold consisted of a dense layer of disordered nanospun fibers and a porous microscale 3D scaffold layer to support and promote the ingrowth of subchondral ***,the biomimetic PCL/nHA/MWCNTs scaffolds enhanced cell seeding efficiency and allowed for higher cell-cell interactions that supported the adhesion,proliferation,activity,morphology and subsequently improved the osteogenic differentiation of bone marrow mesenchymal stem cells in ***,this study elucidates that the construction of 3D printed-electrospun PCL/nHA/MWCNTs scaffolds provides an alternative strategy for the regeneration of subchondral bone and lays a foundation for subsequent in vivo studies.

关键词： additive manufacturing 3D printing electrospinning subchondral bone

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Broadband source-surrounded cloak for on-chip antenna radiation pattern protection

arXiv

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arXiv 2025年

作者： Chen, Hanchuan Sun, Fei Liu, Yichao Fei, Hongming Chen, Zhihui Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Physics and Optoelectronic Engineering Taiyuan University of Technology Taiyuan030024 China

As the frequency range of electromagnetic wave communication continues to expand and the integration of integrated circuits increases, electromagnetic waves emitted by on-chip antennas are prone to scattering from electronic components, which limits further improvements in integration and the protection of radiation patterns. Cloaks can be used to reduce electromagnetic scattering;however, they cannot achieve both broadband and omnidirectional effectiveness simultaneously. Moreover, their operating modes are typically designed for scenarios where the source is located outside the cloak, making it difficult to address this problem. In this work, we propose a dispersionless air-impedance-matched metamaterial over the 2-8 GHz bandwidth that achieves an adjustable effective refractive index ranging from 1.1 to 1.5, with transmittance maintained above 93%. Based on this metamaterial, we introduce a broadband source-surrounded cloak that can guide electromagnetic waves from a broadband source surrounded by the cloak in any propagation direction to bypass obstacles and reproduce the original wavefronts outside the cloak. Thereby protecting the radiation pattern from distortion due to scattering caused by obstacles. Our work demonstrates significant potential for enhancing the integration density of integrated circuits and improving the operational stability of communication systems. Copyright © 2025, The Authors. All rights reserved.

关键词： Directional patterns (antenna)

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Wearable multichannel pulse condition monitoring system based on flexible pressure sensor arrays

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Microsystems & Nanoengineering 2022年第1期8卷 249-258页

作者： Jie Wang Yirun Zhu Zhiyong Wu Yunlin Zhang Jian Lin Tao Chen Huicong Liu Fengxia Wang Lining Sun Jiangsu Provincial Key Laboratory of Advanced Robotics School of Mechanical and Electric EngineeringSoochow UniversitySuzhou 215123China Micro Nano System Research Center Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education and Shanxi Province&College of Information EngineeringTaiyuan University of TechnologyTaiyuan 030024China Suzhou Institute of Nano-tech and Nanobionics Chinese Academy of SciencesSuzhou 215123China

Pulse diagnosis is an irreplaceable part of traditional Chinese medical ***,application of the traditional pulse monitoring method was restricted in the modernization of Chinese medical science since it was difficult to capture real signals and integrate obscure feelings with a modern data ***,a novel multichannel pulse monitoring platform based on traditional Chinese medical science pulse theory and wearable electronics was *** pulse sensing platform simultaneously detected pulse conditions at three pulse positions(Chi,Cun,and Guan).These signals were fitted to smooth surfaces to enable 3-dimensional pulse mapping,which vividly revealed the shape of the pulse length and width and compensated for the shortcomings of traditional single-point pulse ***,the pulse sensing system could measure the pulse signals from different individuals with different conditions and distinguish the differences in pulse *** addition,this system could provide full information on the temporal and spatial dimensions of a person’s pulse waveform,which is similar to the true feelings of doctors’*** innovative,cost-effective,easily designed pulse monitoring platform based on flexible pressure sensor arrays may provide novel applications in modernization of Chinese medical science or intelligent health care.

关键词： multichannel system replace

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