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Dual-Functional Organotelluride Additive for Highly Efficient Sulfur Redox Kinetics and Lithium Regulation in Lithium–Sulfur Batteries

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Energy & Environmental Materials 2023年第3期6卷 126-133页

作者： Wei Zhang Fenfen Ma Qiang Wu Ziqi Zeng Wei Zhong Shijie Cheng Xin Chen Jia Xie State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China GuSu Laboratory of Materials SuzhouJiangsu 215123China State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

High energy density and low cost made lithium–sulfur(Li–S)batteries appealing for the next-generation energy storage ***,their commercial viability is seriously challenged by serious polysulfide shuttle effect,sluggish sulfur kinetics,and uncontrollable dendritic Li ***,a dual-functional electrolyte additive,diphenyl ditelluride(DPDTe)is reported for Li–S *** sulfur cathodes,DPDTe works as a redox mediator to accelerate redox kinetics of sulfur,in which Te radical-mediated catalytic cycle at the solid–liquid interface contributes significantly to the whole *** lithium anodes,DPDTe can react with lithium metal to form a smooth and stable organic–inorganic hybrid solid-electrolyte interphase(SEI),enabling homogeneous lithium deposition for suppressing dendrite ***,the Li–S battery with DPDTe exhibits remarkable cycling stability and superb rate capability,with a high capacity up to 1227.3 mAh g^(-1)and stable cycling over 300 ***,a Li–S pouch cell with DPDTe is evaluated as the proof of *** work demonstrates that organotelluride compounds can be used as functional electrolyte additives and offers new insights and opportunities for practical Li–S batteries.

关键词： electrolyte additive Li anode Li2 S deposition Li–S battery sulfur kinetics

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Enhancing solid-state lithium metal battery performance via indium-based modification of electrolytes and lithium metal surfaces:mechanistic insights and optimization

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Science China Chemistry 2025年第3期68卷 1144-1158页

作者： Zhongkai Wu Chen Liu Ziling Jiang Lin Li Siwu Li Chaochao Wei Qiyue Luo Xia Chen Long Zhang Shijie Cheng Chuang Yu State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China School of Chemistry and Chemical Engineering Huazhong University of Science and TechnologyWuhan 430074China Interdisciplinary Research Center of Smart Sensors Academy of Advanced Interdisciplinary ResearchXidian UniversityXi’an 710126China College of Physics and Energy Fujian Normal UniversityFuzhou 350117China

Argyrodite-based solid-state lithium metal batteries exhibit significant potential as next-generation energy storage ***,their practical applications are constrained by the intrinsic poor stability of argyrodite towards Li metal and exposure to air/***,an indium-involved modification strategy is employed to address these *** optimized doping yields a high Li-ion conductivity of 7.5 mS cm^(-1)for Li_(5.54)In_(0.02)PS_(4.47)O_(0.03)Cl_(1.5)electrolyte,accompanied by enhanced endurance against air/moisture and bare Li *** retains 92.0%of its original conductivity after exposure to air at a low dew point of-60℃in dry ***,a composite layer comprising Li-In alloy and Li F phases is generated on the surface of lithium metal anode via the reaction between InF_(3)and molten *** layer effectively mitigates Li dendrite growth by creating a physical barrier from the robust LiF phase,while the Li-In alloy induces uniform Li-ion deposition and accelerates Li transport dynamics across the interphase between the solid electrolyte/Li ***,the In-doped electrolyte facilitates the in-situ generation of Li-In alloy within its voids,reducing local current density and further inhibiting lithium dendrite ***,the combination of the Li_(5.54)In_(0.02)PS_(4.47)O_(0.03)Cl_(1.5)electrolyte and the InF_(3)@Li anode provides exceptional electrochemical performances in both symmetric cells and solid-state lithium metal batteries across different operating ***,the LiNbO_(3)@LiNi_(0.7)Co_(0.2)Mn_(0.1)O_(2)/Li_(5.54)In_(0.02)PS_(4.47)O_(0.03)Cl_(1.5)/InF_(3)@Li cell delivers a high discharge capacity of 167.8 mAh g^(-1)at 0.5 C under 25℃and retains 80.0%of its initial value after 400 *** work offers a viable strategy for designing functional interfaces with enhanced stability for sulfide-based solid-state lithium batteries.

关键词： Li_(5.5)PS_(4.5)Cl_(1.5)solid electrolyte In_(2)O_(3)dual-doping InF_(3)surface-modification chemical/electrochemical stability electrochemical performance

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Simultaneously enhancing erosion and compression resistance:designing AlCoCrFeNi high-entropy alloy strengthened Ag-based contacts

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Rare Metals 2024年第9期43卷 4476-4492页

作者： Xiao-Yang Xue Zhe Wang Hui-Ling Nie Zhao Yuan Jun Wang Chang-Hu Xu Kai Wen Cong-Hao Yu School of Materials Science and Engineering Xi’an Polytechnic UniversityXi’an 710048China School of Physics Xi’an Jiaotong UniversityXi’an 710049China Key Laboratory of Pulsed Power Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Designing microstructures and unveiling dynamic erosion mechanisms remain important challenges for Ag-based *** simultaneously enhance erosion and compression resistance,an Al Co Cr Fe Ni high-entropy alloy(HEA)is introduced into Ag-based materials to fabricate novel Ag-HEA contacts with island-and skeletonrestricted *** arc erosion experimental results reveal that the skeleton-restricted HEA microstructure is the key factor in reducing the hill and crater morphologies of the contact surface,effectively delaying material transfer between the movable and stationary *** molten bridge evolution and compressive deformation behavior of Ag-HEA contacts with various microstructures are investigated using molecular dynamics(MD)*** results indicate that the constraint of Ag atom diffusion in the molten pool and the involvement of HEA atoms in the molten bridge are the primary mechanisms for improving erosion *** skeleton-restricted HEA microstructure reduces the total energy and structural stability of the molten bridge system and promotes its fracture and ***,the synergistic effect of the twin and Lomerz–Cottrell lock structures can hinder dislocation glide,generating dispersed and small-area stacking faults in the Ag matrix and mitigating the concentration of shear ***,the skeleton-restricted HEA microstructure contributes positively to compression *** study presents a novel approach to designing Ag-based contacts.

关键词： Electrical contact materials High entropy alloys Arc erosion Molecular dynamics Microstructures

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“In-N-out” design enabling high-content triethyl phosphate-based non-flammable and high-conductivity electrolytes for lithium-ion batteries

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Science China Chemistry 2024年第2期67卷 724-731页

作者： Mengchuang Liu Fenfen Ma Zicheng Ge Ziqi Zeng Qiang Wu Hui Yan Yuanke Wu Sheng Lei Yanli Zhu Shijie Cheng Jia Xie State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan430074China School of Chemistry and Chemical Engineering Huazhong University of Science and TechnologyWuhan430074China GuSu Laboratory of Materials Suzhou215123China Institute of Metal Research Chinese Academy of SciencesShenyang110000China State Key Laboratory of Explosion Science and Technology Beijing Institute of TechnologyBeijing100081China

Safety issues related to flammable electrolytes in lithium-ion batteries(LIBs) remain a major challenge for their extended *** use of non-flammable phosphate-based electrolytes has proved the validity in inhibiting the combustion of ***,the strong interaction between Li^(+) and phosphate leads to a dominant solid electrolyte interphase(SEI) with limited electronic shielding,resulting in the poor Li^(+) intercalation at the graphite(Gr) anode when using high-phosphate-content *** mitigate this issue and improve Li^(+) insertion,we propose an “In-N-Out” strategy to render phosphates “noncoordinative”.By employing a combination of strongly polar solvents for a “block effect” and weakly polar solvents for a “drag effect”,we reduce the Li^(+)–phosphate *** a result,phosphates remain in the electrolyte phase(“In”),minimizing their impact on the incompatibility with the Gr electrode(“Out”).We have developed a non-flammable electrolyte with high triethyl phosphate(TEP) content(>60 wt.%),demonstrating the excellent ion conductivity(5.94 mS cm^(-1) at 30 ℃) and reversible Li^(+) intercalation at a standard concentration(~1 mol L^(-1)).This approach enables the manipulation of multiple electrolyte functions and holds the promise for the development of safe electrochemical energy storage systems using non-flammable electrolytes.

关键词： lithium-ion batteries graphite anode high-phosphate-content electrolytes non-flammable electrolyte excellent ion conductivity standard concentration

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The Impact Analysis of Line Inductance on System Amplitude and Frequency Stability in the Converter Interfaced System 6

The Impact Analysis of Line Inductance on System Amplitude a...

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6th International Conference on Power and Energy technology, ICPET 2024

作者： Xu, Qiumeng Wang, Sicheng Yuan, Xiaoming State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic Engineering Huazhong University of Science and Technology Wuhan China

ISBN: (纸本)9798350375855

With the transition to cleaner energy sources, a high proportion of renewable devices often needs to be connected to the grid through long transmission lines, which increases the risk of system instability. The system is composed of device and network, both of which have influence on system stability. The impact of device control parameters on system stability has been widely studied, but the impact of network on system stability should not be overlooked. This paper focuses on the line inductance in the network. Firstly, it elucidates the implications of the system Amplitude and Frequency (A&F) stability, considering the dynamic characteristics of both device and the network. Secondly, it analyzes the high-order dynamic characteristics of the inherent relationship between the excitation of the amplitude/frequency of internal voltage and the response of active/reactive current, under the constraints imposed by line inductance in the network. This analysis reveals the essence of the dominant feature of this relationship, which is influenced by the system oscillation frequency. Finally, the system oscillation frequency was analyzed through closed-loop simulation, which affects the A&F stability of the system by affecting the energy storage capacity of the line inductance. This paper establishes a general understanding of the energy storage capacity of line inductor in the grid and lays the foundation for further understanding and analyzing of the mechanism of power system instability problems. © 2024 IEEE.

关键词： Frequency stability

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Multi-Objective Optimization of electromagneticthermal Coupling Performance for High-torquedensity PMSM based on Multi-dimensional Correction Techniques

Multi-Objective Optimization of Electromagneticthermal Coupl...

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2024 International Conference on Electrical Machines, ICEM 2024

作者： Li, Zequan Wang, Jin Sun, Lu Kang, Haoyu Liu, Liyang Zhou, Libing State Key Laboratory of Advanced Electromagnetic Technology Huazhong University of Science and Technology Wuhan China School of Electrical and Electronic Engineering Huazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Engineering and Technology Wuhan430074 China Guangzhou China Guangzhou511453 China

ISBN: (纸本)9798350370607

To address the precision limitation of traditional thermal models and the computational inefficiency of electromagnetic-thermal coupling finite element models, this work proposes a multidimensional correction-based electromagnetic-thermal coupling design optimization method for electric machines. Firstly, this method corrects the sensitive parameters in the analytical lumped parameters thermal network model (LPNM) based on prior information from historical experimental data to ensure the accuracy for thermal performance analysis. Subsequently, to enhance computational efficiency, a large number of low-fidelity (LF) samples are obtained using the corrected thermal model in a serial electromagnetic-thermal field calculation manner, complemented by a small number of high-fidelity (HF) samples obtained from the electromagnetic-thermal coupling simulation model. Then, by employing a transfer learning technique, the data information from the low- to high-fidelity sample sets is comprehensively utilized to train a multi-fidelity (MF) surrogate model for the final optimization. The proposed method applied to a high-torque-density aerospace propulsion permanent magnet synchronous motor (PMSM) with short-term strong overload capability, it not only significantly improves the accuracy of LPNM, but also reduces the training sample acquisition time by over 50% under the same model accuracy. Finally, a prototype is tested to validate the effectiveness of the proposed method. © 2024 IEEE.

关键词： Lumped parameter networks

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Power-to-Hydrogen by Electrolysis in Carbon Neutrality: technology Overview and Future Development

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CSEE Journal of Power and Energy Systems 2023年第4期9卷 1266-1283页

作者： Zhiyao Zhong Jiakun Fang Kewei Hu Danji Huang Xiaomeng Ai Xiaobo Yang Jinyu Wen Yuan Pan Shijie Cheng the State Key Laboratory of Advanced Electromagnetic Engineering and Technology Huazhong University of Science and TechnologyWuhan 430074China. Hitachi Energy Research Hitachi Energy(China)LimitedBeijing 100015China.

Power-to-hydrogen by electrolysis(PtHE)is a promising technology in the carbon-neutral evolution of *** not only contributes to renewable energy integration but also accelerates decarbonization in industrial sectors through green hydrogen *** paper presents a comprehensive review of PtHE ***,technical solutions in PtHE technology are introduced to clarify pros and cons of one ***,the multiphysics coupling and the multi-energy flow are investigated to reveal the insight mechanism during operation of compactly assembled industrial PtHE ***,the development trends of core components in PtHE plants,including electrocatalysts,electrode plates and operation strategy,are reviewed,*** thrusts needed for PtHE in carbon-neutral transition are also ***,three configurations of the PtHE plant in energy system integration are introduced,which can achieve renewable energy integration and efficient energy *** Terms-Carbon neutrality,power-to-hydrogen nby electrolysis(PtHE),multiphysics coupling,multidisciplinary.

关键词： Carbon neutrality power-to-hydrogennby electrolysis(PtHE) multiphysics coupling multidisciplinary.

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On the green aurora emission of Ar atmospheric pressure plasma

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Plasma Science and technology 2022年第5期24卷 195-204页

作者： Fengwu LIU Lanlan NIE Xinpei LU State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074People’s Republic of China

The Ar atmospheric pressure plasma was found to be an excellent laboratorial source for green aurora ***,the characteristic and production mechanism of the green aurora emission of the Ar atmospheric pressure plasma are still not *** this work,an Ar plasma in a long glass tube which emits intense green aurora light is *** the long glass tube,it can be concluded that the green aurora emission in the Ar plasma is not owing to the mixture of Ar plasma plume with the surrounding *** is also found that the green aurora emission often appeared beyond the active electrode when the active electrode is placed at the downstream of the gas *** green emission disappears when the traces amount of O_(2) or N_(2)(about 0.05%–0.07%)is added to *** is because the O_(2) molecules deactivate the upper state O(^(1)S),which results in the decrease of the green *** the other hand,when N_(2) is added,Ar metastable atoms are quenched by N_(2),which results in the decrease of O atoms and eventually leads to the decrease of the green emission *** intensity of the green aurora emission increases when the driving voltage frequency increases from 1 to 10 k *** importantly,it is found that the green aurora emission is not affected when a grounded stainless steel needle is in contact with the plasma ***,the green emission is not driven *** these findings are helpful for the understanding of the physics and its applications of atmospheric pressure plasma jet in space physics,laser physics and other application areas.

关键词： atmospheric pressure plasma jet plasma optical emission aurora emission

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A non‐equal gap distance dielectric barrier discharge:Between cone‐shape and cylinder‐shape electrodes

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High Voltage 2022年第1期7卷 98-105页

作者： Shaohui Jin Zhiyu Li Yubin Xian Lanlan Nie Xinpei Lu State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhanHubeiChina

A non‐equal gap distance dielectric barrier discharge(DBD)between cone‐shape and a cylinder‐shaped electrodes is *** DBD is driven by a nanosecond voltage *** the pulse frequency is 500 Hz or lower,ladder‐shape plasma with multiple plasma layers is generated within the gap,with a distance increasing from 1 to 7 *** to high‐speed photographs of the plasma captured by an intensified charge‐coupled camera detector camera,the ladder‐shaped plasma is formed owing to propa-gation of ring‐shaped plasma from the region of the short‐gap distance to the region of long‐gap distance with regular variations in its propagation *** propagation speed drops to zero and lasts for about 20-30 ns at the region of each plasma layer,which results in bright plasma *** electric field of the plasma layer at the region of the different gap distance is evaluated according to the optical emission intensity ratio R_(391)/_(394)of N_(2)^(+)at 391 nm and N_(2) at 394 *** obtained electric field drops from 8.1 to 6.4 kV/mm when the plasma is propagated from regions of gap distance of 2-5 *** the pulse frequency is increased to 1 kHz or higher,the discharge changes into a filamentary mode and the multiple‐layer plasma disappears.

关键词： cylinder shaped dielectric

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Real-time State Prediction Based Coordinated Control Strategy of LIQHYSMES

Real-time State Prediction Based Coordinated Control Strateg...

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2024 IEEE China International Youth Conference on Electrical engineering, CIYCEE 2024

作者： Liu, Qi Shi, Jing Zhou, Jiachen Cheng, Siwei Cheng, Qi School of Electrical and Electronic Engineering Huazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Engineering and Technology Wuhan430074 China

ISBN: (纸本)9798331530174

LIQHYSMES (Liquid hydrogen with superconducting magnetic energy storage) offers rapid response, substantial capacity, and low energy conversion losses, making it ideal for large scale renewable energy integration and power grid stability. However, challenges remain in fully coordinated utilization of the storage units and safe, stable operation of the storage magnets. Accurate state prediction and control are vital for the efficient operation and coordination of LIQHYSMES. This paper proposes a state prediction based LIQHYSMES coordinated control strategy. Firstly, a superconducting magnet state prediction model based on the random forest algorithm is established. Secondly, the coordinated control strategy is outlined. Finally, simulation analysis validates the prediction model and control strategy, demonstrating their accuracy and effectiveness. © 2024 IEEE.

关键词： Prediction models

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