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10th International Conference on Theoretical and Applied Physics, ICTAP 2020

作者： Nazarudin Hasibuan, M.P.H. Haryadi, B. Nurhayati Ulyarti Hadiyanto Chemical Engineering FST University of Jambi Jambi Indonesia Energy and Nano Material Centre LPPM Universitas Jambi Jambi Indonesia Center of Excellent on Bio-Geo Material and Energy Universitas Jambi Jambi Indonesia Department of Enviromental Study Program University of Jambi Jambi Indonesia Department of Science Education Program University of Jambi Jambi Indonesia

Bioenergy is one of the renewable energies which is predicted to be a main energy in the next few years. It can play the important role to change the current fossil fuel-based energy into a green energy which has a low carbon footprint. A research about how to develop a bioenergy have been done by a lot of reseacher. However, especially in Indonesia, there is just few research to study about bioenergy from societal aspects poin of view such as the understanding and awarness of bioenergy among citizens. In this research, we have investigated senior high school students' knowledge, perceptions, and attitudes interconected to bioenergy with online survery. The survey instrument used in the study was adopted from P. Halder's study. The data was collected from students at senior high school th (SMAN 10) Jambi City. The results showed that the students awareness of bioenergy perceived from school, home, and social media have significant effects on their knowledge, perceptions and attitudes related to bioenergy. Among 211 students as respondent (N), we found 70.62% believe that they understand well the concept about bioenergy, 5.21% believe that they understand it very well, and the rest believe that they do not understand it. This understanding reflects to their willingness to use a bioenergy in their daily life, in which 71.70% respondents agree to use bioenergy, 25.47% respondents can not decide, and only 2.83% do not want to use it. To find the relationship among the variables, a multiple regression was conducted. A statistical analysis showed that the model for knowledge as a function of attitudes and perception does not fit the data therefore this model is rejected. However, both model for attitudes as function of perception and knowledge, and also perception as function of attitudes and knowldeges fit the data hence the models are accepted. In other words, attitudes of students who will use/not use bioenergy, is significantly affected by their perception about bioen

关键词： Students

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Magnetochiral Tunneling in Paramagnetic Co1/3NbS2

arXiv

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arXiv 2024年

作者： Lim, Seongjoon Singh, Sobhit Huang, Fei-Ting Pan, Shangke Wang, Kefeng Kim, Jaewook Kim, Jinwoong Vanderbilt, David Cheong, Sang-Wook Rutgers Center for Emergent Materials Department of Physics and Astronomy PiscatawayNJ08854 United States Department of Mechanical Engineering University of Rochester RochesterNY14627 United States Materials Science Program University of Rochester RochesterNY14627 United States State Key Laboratory Base of Novel Function Materials and Preparation Science School of Material Sciences and Chemical Engineering Ningbo University Zhejiang Ningbo315211 China Department of Physics and Astronomy Rutgers University PiscatawayNJ08854 United States

Electric currents have the intriguing ability to induce magnetization in nonmagnetic crystals with sufficiently low crystallographic symmetry. Some associated phenomena include the non-linear anomalous Hall effect in polar crystals and the nonreciprocal directional dichroism in chiral crystals when magnetic fields are applied. In this work, we demonstrate that the same underlying physics is also manifested in the electronic tunneling process between the surface of a nonmagnetic chiral material and a magnetized scanning probe. In the paramagnetic but chiral metallic compound Co1/3NbS2, the magnetization induced by the tunneling current is shown to become detectable by its coupling to the magnetization of the tip itself. This results in a contrast across different chiral domains, achieving atomic-scale spatial resolution of structural chirality. To support the proposed mechanism, we used first-principles theory to compute the chirality-dependent current-induced magnetization and Berry curvature in the bulk of the material. Our demonstration of this magnetochiral tunneling effect opens up a new avenue for investigating atomic-scale variations in the local crystallographic symmetry and electronic structure across the structural domain boundaries of low-symmetry nonmagnetic crystals. © 2024, CC BY.

关键词： Magnetization

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High-Performance Silicon Anodes Enabled by Multifunctional Ultrafine Silica Nanoparticle-Embedded Carbon Coatings for Lithium-Ion Batteries

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Advanced Energy materials 2025年第0期

作者： Sun, Zhefei Yin, Quanzhi Zhou, Shenghui Chen, Haoyu Wen, Sifan Yang, Huiping Wu, Xiaoyu Pan, Jianhai Han, Jiajia Yang, Hui Zhuang, Zilong Feng, Shijie Zhang, Li Peng, Dong-Liang Zhang, Qiaobao State Key Laboratory of Physical Chemistry of Solid Surfaces College of Materials Xiamen University Xiamen361005 China State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical Engineering Tan Kah Kee Innovation Laboratory Collaborative Innovation Center of Chemistry for Energy Materials Xiamen University Fujian Xiamen361005 China State Key Laboratory of Material Processing and Die & Mould Technology Department of Mechanics School of Aerospace Engineering Huazhong University of Science and Technology Hubei Wuhan430074 China Department of Mechanical Engineering University of Wisconsin-Madison MadisonWI53706 United States Materials Science and Engineering Program University of California San Diego La JollaCA92093 United States Longmen Laboratory Henan Luoyang471023 China

Silicon (Si) holds immense promise as viable anode for next-generation high-energy-density Li-ion batteries (LIBs). However, its poor ionic/electronic conductivity and significant volumetric changes during cycling lead to rapidly deteriorated LIB performance. Here, a novel multifunctional coating featuring ultrafine SiO2 nanoparticles (2-C) to resolve these challenges is proposed. This unique uSiO2-C coating provides high-efficient electron and ion transport pathways, while also improves interfacial stability and mitigates volume changes during cycling, thereby enhancing the conductivity and structural integrity of Si@uSiO2-C, as corroborated by extensive experimental and computational studies. In addition, the abundant interfaces in uSiO2-C coating facilitate Li+ transport and the evenly distributed ultrafine SiO2 nanoparticles impart high electrochemical reactivity and mechanical robustness. Consequently, the Si@uSiO2-C anode achieves a high reversible capacity of 2093 mAh g−1 at 0.2 A g−1, with a high initial Coulombic efficiency of 88.3%, superior rate capability and durability (1000 cycles, 928 mAh g−1 at 1.0 A g−1, 75% capacity retention). Full cells paired with commercial LiFePO4 cathodes demonstrate high cyclability, maintaining 80% capacity retention over 500 cycles at 4 C. This work highlights the vital role of multifunctional coating in promoting the electrochemical performance of Si-based anodes for high-performance LIBs. © 2025 Wiley-VCH GmbH.

关键词： SiO2 nanoparticles

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Multifunctional polyimides containing triarylamine for electrochromic flexible device, photodetector and resistance memory device

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Multifunctional materials 2021年第3期4卷

作者： Gao, Yanyu Zhai, Minghao Sui, Yan Li, Dongxu Lin, Xiaoxue Pan, Shijia Pan, Qingjiang Niu, Haijun Wang, Wen Key Laboratory of Functional Inorganic Material Chemistry Ministry of Education Department of Macromolecular Science and Engineering School of Chemical. Chemical Engineering and Materials Heilongjiang University Harbin150086 China School of Materials Science and Engineering Harbin Institute of Technology Harbin150080 China

Integrating different functions in one material will decrease the volume, responding time, and price of device. Polyimides (PIs) are the optimal candidates because of excellent flexible mechanics, thermal stability, and transparent properties. In this work, a series of multifunctional flexible PIs were designed and synthesized from a novel functional triarylamine for electrochromic (EC) device. The PIs show promising application in EC with the efficiency of 205 cm2 C-1, memory devices with the ON/OFF ratio of 3.7 × 104, and photodetectors with a limit being of 0.07 V. Furthermore, the flexible EC device of PI-3 (short for PI 3 made of 4,4'-(hexafluoroisopropylidene) diphthalic anhydride) keeps excellent stability, and the optical contrast does not decrease even after 2000 cycles. © 2021 IOP Publishing Ltd.

关键词： Polyimides

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Efficient Ceo2/Zno Heterojunction for Enhanced Heterogenous Photocatalytic Application

SSRN

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SSRN 2024年

作者： Li, Honglin Wu, Rong Ji, Jun Liu, Yue Zhao, Jiahui Sahar, Shafaq Zeb, Akif College of Chemistry and Material Engineering Chao Hu University Hefei238000 China School of Energy Materials and Chemical Engineering Hefei University Hefei City230601 China Key Laboratory of Resource Comprehensive Utilization of Chaohu University Chaohu University Hefei238000 China MOE Key Laboratory of Macromolecular Synthesis and Functionalization Department of Polymer Science and Engineering Zhejiang University 866 Yuhangtang Rd Hangzhou310058 China Hunan Joint International Laboratory of Advanced Materials and Technology for Clean Energy College of Materials Science and Engineering Hunan University Changsha410082 China Surface and Materials Technology Institute of Materials Engineering University of Siegen Paul-Bonatz-Straße 9-11 Siegen57076 Germany

Organic pollutants pose a significant challenge due to their toxicity and potential carcinogenicity, posing a severe threat to the environment and human health. Heterogeneous photocatalysts offer promising advantages over traditional water purification methods due to their tunable electronic properties such as bandgap, easy separation from the reaction solution and formidable nanostructures. Herein, we prepare a CeO2/ZnO heterostructure via simple hydrothermal synthesis. The electronic structure of this nanocomposite was tuned to achieve a band gap of ~2.94 eV, which was between the individual bandgaps of CeO2 and ZnO nanoparticles. In addition, the mixed valence character of Ce further enhanced the electronic properties of the CeO2/ZnO heterostructure. The photocatalytic performance of CeO2, ZnO and CeO2/ZnO heterostructure was evaluated and it was found that CeO2/ZnO heterostructure with a Zn/Ce ratio of 0.2 exhibited the highest photocatalytic activity and the degradation efficiency was 99.28% after irradiation for 60 min. It was mainly ascribed to the heterojunction structure of the CeO2/ZnO nanocomposite, leading to a higher separation efficiency of electron-hole pairs and generating more superoxide radicals, which in turn improved the photocatalytic activity effectively. © 2024, The Authors. All rights reserved.

关键词： II-VI semiconductors

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Ogden material Calibration via Magnetic Resonance Cartography, Parameter Sensitivity, and Variational System Identification

arXiv

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arXiv 2022年

作者： Nikolov, Denislav P. Srivastava, Siddhartha Abeid, Bachir A. Scheven, Ulrich M. Arruda, Ellen M. Garikipati, Krishna Estrada, Jonathan B. Department of Mechanical Engineering University of Michigan United States Department of Biomedical Engineering University of Michigan United States Program in Macromolecular Science and Engineering University of Michigan United States Department of Mathematics University of Michigan United States Michigan Institute for Computational Discovery and Eng. University of Michigan United States

Contemporary material characterisation techniques that leverage deformation fields and the weak form of the equilibrium equations face challenges in the numerical solution procedure of the inverse characterisation problem. As material models and descriptions differ, so too must the approaches for identifying parameters and their corresponding mechanisms. The widely-used Ogden material model can be comprised of a chosen number of terms of the same mathematical form, which presents challenges of parsimonious representation, interpretability, and stability. Robust techniques for system identification of any material model are important to assess and improve experimental design, in addition to their centrality to forward computations. Using fully 3D displacement fields acquired in silicone elastomers with our recently-developed magnetic resonance cartography (MR-u) technique on the order of > 20, 000 points per sample, we leverage PDE-constrained optimisation as the basis of variational system identification of our material parameters. We incorporate the statistical F-test to maintain parsimony of representation. Using a new, local deformation decomposition locally into mixtures of biaxial and uniaxial tensile states, we evaluate experiments based on an analytical sensitivity metric, and discuss the implications for experimental design. © 2022, CC BY-NC-ND.

关键词： Inverse problems

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Active tuning of plasmon damping via light induced magnetism

arXiv

引用

arXiv 2022年

作者： Cheng, Oscar Hsu-Cheng Zhao, Boqin Brawley, Zachary Son, Dong Hee Sheldon, Matthew Department of Chemistry Texas A&M University College Station TX United States Center for Nanomedicine Institute for Basic Science Graduate Program of Nano Biomedical Engineering Advanced Science Institute Yonsei University Seoul Korea Republic of Department of Material Science and Engineering Texas A&M University College Station TX United States

Circularly polarized optical excitation of plasmonic nanostructures causes coherent circulating motion of their electrons, which in turn, gives rise to strong optically induced magnetization— a phenomenon known as the inverse Faraday effect (IFE). In this study we report how the IFE also significantly decreases plasmon damping. By modulating the optical polarization state incident on achiral plasmonic nanostructures from linear to circular, we observe reversible increases of reflectance by 78% as well as simultaneous increases of optical field concentration by 35.7% under 109 W/m2 continuous wave (CW) optical excitation. These signatures of decreased plasmon damping were also monitored in the presence of an externally applied magnetic field (0.2 T). The combined interactions allow an estimate of the light-induced magnetization, which corresponds to an effective magnetic field of ~1.3 T during circularly polarized CW excitation (109 W/m2). We rationalize the observed decreases in plasmon damping in terms of the Lorentz forces acting on the circulating electron trajectories. Our results outline strategies for actively modulating intrinsic losses in the metal, and thereby, the optical mode quality and field concentration via opto-magnetic effects encoded in the polarization state of incident light. Copyright © 2022, The Authors. All rights reserved.

关键词： Damping

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Coal Structure: Visualizing Micropore Distributions Through Hierarchical 3D Pore Modeling for a Bituminous Coal 38

Coal Structure: Visualizing Micropore Distributions Through ...

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38th Annual International Pittsburgh Coal Conference 2021: Clean Coal-based Energy/Fuels and the Environment, PCC 2021

作者： Lu, Guanwen Watson, Justin K. Mathews, Jonathan P. Leone Family Department of Energy and Mineral Engineering The EMS Energy Institute Pennsylvania State University University ParkPA16802 United States China University of Mining & Technology Xuzhou221008 China Department of Material Science and Engineeing Nuclear Engineering Program Florida University GainesvilleFL32661 United States

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Room-temperature multiple ligands-tailored SnO_(2) quantum dots endow in situ dual-interface binding for upscaling efficient perovskite photovoltaics with high V_(OC)

引用

Light(science & Applications) 2021年第12期10卷 2467-2481页

作者： Zhiwei Ren Kuan Liu Hanlin Hu Xuyun Guo Yajun Gao Patrick W.K.Fong Qiong Liang Hua Tang Jiaming Huang Hengkai Zhang Minchao Qin Li Cui Hrisheekesh Thachoth Chandran Dong Shen Ming-Fai Lo Annie Ng Charles Surya Minhua Shao Chun-Sing Lee Xinhui Lu Frédéric Laquai Ye Zhu Gang Li Department of Electronic and Information Engineering Research Institute for Smart Energy(RISE)Guangdong-Hong Kong-Macao(GHM)Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and DevicesThe Hong Kong Polytechnic UniversityHung HomKowloonHong KongChina Department of Electrical and Computer Engineering Nazarbayev UniversityNur-SultanKazakhstan The Hong Kong Polytechnic University Shenzhen Research Institute Shenzhen 518057China Hoffmann Institute of Advanced Materials Shenzhen Polytechnic7098 Liuxian BoulevardShenzhen 518055China Department of Applied Physics The Hong Kong Polytechnic UniversityHung HomKowloonHong KongChina Department of Chemical and Biological Engineering The Hong Kong University of Science and TechnologyClear Water BayKowloonHong KongChina King Abdullah University of Science and Technology(KAUST) KAUST Solar Center(KSC)Physical Sciences and Engineering Division(PSE)Material Science and Engineering Program(MSE)Thuwal 23955-6900Kingdom of Saudi Arabia Department of Physics The Chinese University of Hong KongShatin 999077 Hong KongChina Center of Super-Diamond and Advanced Films(COSDAF) Department of ChemistryCity University of Hong KongHong KongChina

The benchmark tin oxide(SnO_(2))electron transporting layers(ETLs)have enabled remarkable progress in planar perovskite solar cell(PSCs).However,the energy loss is still a challenge due to the lack of“hidden interface”*** report a novel ligand-tailored ultrafine SnO_(2) quantum dots(QDs)via a facile rapid room temperature ***,the ligand-tailored SnO_(2) QDs ETL with multi-functional terminal groups in situ refines the buried interfaces with both the perovskite and transparent electrode via enhanced interface binding and perovskite *** novel ETLs induce synergistic effects of physical and chemical interfacial modulation and preferred perovskite crystallization-directing,delivering reduced interface defects,suppressed non-radiative recombination and elongated charge carrier *** conversion efficiency(PCE)of 23.02%(0.04 cm^(2))and 21.6%(0.98 cm^(2),V_(OC) loss:0.336 V)have been achieved for the blade-coated PSCs(1.54 eV E_(g))with our new ETLs,representing a record for SnO_(2) based blade-coated ***,a substantially enhanced PCE(V_(OC))from 20.4%(1.15 V)to 22.8%(1.24 V,90 mV higher V_(OC),0.04 cm^(2) device)in the blade-coated 1.61 eV PSCs system,via replacing the benchmark commercial colloidal SnO_(2) with our new ETLs.

关键词： perovskite interface quantum

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Recent trend of metal promoter role for CO₂ hydrogenation to C₁ and C₂₊ products

引用

South African Journal of Chemical engineering 2023年 44卷 14-30页

作者： Sholeha, Novia Amalia Holilah, Holilah Bahruji, Hasliza Ayub, Athirah Widiastuti, Nurul Ediati, Ratna Jalil, Aishah Abdul Ulfa, Maria Masruchin, Nanang Nugraha, Reva Edra Prasetyoko, Didik College of Vocational Studies Bogor Agricultural University (IPB University) Jalan Kumbang No. 14 Bogor 16151 Indonesia Research Center for Biomass and Bioproducts National Research and Innovation Agency of Indonesia (BRIN) Cibinong 16911 Indonesia Department Chemistry Faculty of Science and Data Analytics Institut Teknologi Sepuluh Nopember Kampus ITS Keputih Surabaya Sukolilo 60111 Indonesia Centre of Advanced Material and Energy Science Universiti Brunei Darussalam Jalan Tungku Link BE 1410 Brunei Darussalam Department of Chemical Engineering Faculty of Chemical and Energy Engineering Universiti Teknologi Malaysia 81310 UTM Skudai Johor Johor Bahru Malaysia Centre of Hydrogen Energy Institute of Future Energy Universiti Teknologi Malaysia Skudai 81310 UTM Skudai Johor Johor Bahru Malaysia Chemistry Education Study Program Faculty of Teacher Training and Education Sebelas Maret University Jl. Ir. Sutami 36A Surakarta 57126 Indonesia Research Collaboration Center for Biomass and Biorefinery between BRIN and Universitas Padjadjaran Jatinangor 45363 Indonesia Department of Chemical Engineering Faculty of Engineering Universitas Pembangunan Nasional “Veteran” Jawa Timur East Java Surabaya 60294 Indonesia

CO2 hydrogenation as sustainable route for generation of value-added carbon feedstock is identified as green pathway for mitigation of greenhouse gasses emission. CO2 methanation is one of the promising solutions, whi... 详细信息

CO₂ hydrogenation as sustainable route for generation of value-added carbon feedstock is identified as green pathway for mitigation of greenhouse gasses emission. CO₂ methanation is one of the promising solutions, which only requires reactions at atmospheric pressure while utilizing metal catalysts to overcome kinetic limitations. Metal catalysts can be promoted to alter reducibities, CO₂ adsorption capacities, and H_2[sbnd]CO₂ dissociation potential. The role of metal promoter such as rare earth elements (Ce, Mn, Co, and La) and alkali and alkali earth metal (Li, Na, Ca, and K) will be discussed within the scope of CO₂ methanation. The aspect of catalysts modification towards hydrogen dissociation potential and surface oxygen vacancy will be emphasized to enhance selectivity for methane. Another pathway for CO₂ hydrogenation is via further conversion into longer chain molecules such as olefin and ethanol. The benefit of metal promoter will be discussed in this review on the effect towards promoting C[sbnd]C coupling reaction for producing longer chain alcohol and light olefin. The strategies to develop active catalysts for the coupling reaction of C[sbnd]C will be emphasized with the promoter introduction. For the hydrogenation of CO₂ to longer chain molecules, the main metal catalysts Ni, Pd, Rh, and Co, and their modification with promoter such as Ga, Cu, and alkali metal Na, K will be discussed. A critical analysis of the CO₂ methanation mechanism and further C[sbnd]C reaction to longer chain molecules will be discussed, particularly the effect of metal promoters to stabilize the intermediate and maneuver the catalytic reaction pathway into the desired products. © 2023 The Author(s)

关键词： C1 products C2+ products CO2 Hydrogenation Metal promoter

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