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Thermo-Electric Powered High energy-Density Hybrid Supercapattery for Driving Overall Water Splitting: A Novel Trifunctional Builder for Self-Powered Hydrogen Production

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Small 2025年 e2504667页

作者： Liyakath Ali, Noor Ul Haq Mohamed Saleem, Mohamed Sadiq Sathyaseelan, Arunprasath Krishnan, Vignesh Pazhamalai, Parthiban Saj, Anandhan Ayyappan Kim, Sang-Jae Nanomaterials & System Lab Major of Mechatronics Engineering Faculty of Applied Energy System Jeju National University Jeju 63243 South Korea Research Institute of New Energy Industry (RINEI) Jeju National University Jeju 63243 South Korea Nanomaterials & System Lab Major of Mechanical System Engineering College of Engineering Jeju National University Jeju 63243 South Korea Green Hydrogen Glocal Leading Research Center (gH2-RC) Jeju National University Jeju 63243 South Korea

Integrated electrochemical energy devices with multifunctionality are evolving as an auspicious way to lift up energy technology. However, the challenge is utilizing a single-electrode material for multifunctional applications is essential to minimize the manpower and overall cost of the system. Herein, a novel and cost-effective self-powered aqueous electrochemical energy device (SAEED) is proposed via integrating asymmetric supercapattery (ASD) and water-splitting (WS) devices utilizing Cu₃Mo₂O₉ (CMD) nanostructures on Ni-foam (prepared via hydrothermal method) as a trifunctional electrode. First, the Cu₃Mo₂O₉/Ni electrode is examined for the supercapacitor, which shows the faradaic-type of charge-storage behavior with a superior specific capacity of 588.88 mAh g⁻¹. The Cu₃Mo₂O₉ǁgraphene ASD is constructed, which shows high energy storage performance with high device capacitance and energy/power densities and 98% retention capacitance over 5000 cycles. Second, the electrocatalyst behavior of the Cu₃Mo₂O₉/Ni electrode is explored, which reveals impressive HER/OER performance with lower overpotential (HER-120 mV at 10 mA cm⁻²/OER-310 mV at 50 mA cm⁻²) values. As a proof-of-concept, an SAEED was developed that contains a thermoelectric generator, Cu₃Mo₂O₉ǁgraphene ASD, and a beaker-type electrolyzer operating at a voltage of 1.58 V to eliminate power loss and intermittent issues for sustainable and uninterrupted production of H₂. © 2025 The Author(s). Small published by Wiley-VCH GmbH.

关键词： asymmetric supercapattery copper molybdate nanostructures power regulator self-powered hydrogen production thermo-electric charging water-splitting

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Insight into spin polarization, Fermi surface, band structure and Thermophysical properties of Sc₂ZrSi inverse Heusler

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Chemical Physics 2025年 596卷

作者： Yousuf, Saleem Masood, Khalid Bin Iqbal, Shahzad Alsahli, Abdulaziz Abdullah Bhat, Masroor Ahmad Mir, Arshid Department of Physics Sri Pratap College Srinagar J&K India Faculty of Applied Energy System Major of Electronic Engineering Jeju National University Jeju 63243 South Korea Department of Botany and Microbiology Faculty of Science King Saud University Riyadh 11451 Saudi Arabia

The origin of half-metallicity, spin behavior, thermoelectrics and thermodynamics of inverse full-Heusler Sc2ZrSi alloy are explored using the density functional theory (DFT). The calculation of ground state energy, c... 详细信息

The origin of half-metallicity, spin behavior, thermoelectrics and thermodynamics of inverse full-Heusler Sc₂ZrSi alloy are explored using the density functional theory (DFT). The calculation of ground state energy, confirm the XA-type structure with Hg₂CuTi-prototype structure with F-43 m space group symmetries. Band structure and occupation of density of states at the Fermi level convey the semiconducting nature with an indirect band gap of 0.52 eV. Semi-classical Boltzmann transport theory is used to determine various thermoelectric coefficients to infer about its capability as waste heat recovery system. The Seebeck coefficient and electrical conductivity measurements also convey semiconducting band structure over all chemical potentials. The thermoelectric efficiency measured through zT calculation with a value of 0.5 at 1200 K, convey the material can be used as high temperature thermoelectric material. The thermodynamics using Debye temperature, specific heat and thermal expansion coefficient define low anharmonicity and low lattice thermal conductivity of the material. The overall thermophysical assets suggest the material has a potential stand for spintronic and thermoelectric applications. © 2025 Elsevier B.V.

关键词： DFT Inverse full-Heuslers Mechanical properties Spintronics Thermodynamics Thermoelectrics

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Recent trends,challenges,and perspectives in piezoelectric-driven self-chargeable electrochemical supercapacitors

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Carbon energy 2022年第5期4卷 833-855页

作者： Karthikeyan Krishnamoorthy Parthiban Pazhamalai Sindhuja Manoharan Noor Ul Haq Liyakath Ali Sang-Jae Kim Nanomaterials&System Lab Major of Mechatronics EngineeringFaculty of Applied Energy SystemJeju National UniversityJejuSouth Korea Research Institute of Energy New Industry Jeju National UniversityJejuSouth Korea Nanomaterials&System Lab Major of Mechanical System EngineeringCollege of EngineeringJeju National UniversityJejuSouth Korea

The increasing demand for wearable electronic devices has resulted in tremendous progress in research on energy harvesting and storage devices/*** storage devices require a power source to charge them,whereas energy harvesting devices require a storage compartment to store the harvested energy for sustainable ***,a piezoelectrically driven self-charging supercapacitor power cell(SCSPC)was developed to harvest and store electrical energy in a solitary system to determine the potential impact of these two types of energy devices for wearable electronic *** review describes the recent advances in piezoelectric-driven SCSPCs in terms of device configuration,piezoelectric separator,electrolyte types,electrode materials,current collectors,and system *** review focuses specifically on the principles and mechanism of the self-charging process that occurred in the SCSPCs and the use of a promising piezo electrochemical spectroscopic tool to realize the piezo electrochemical energy transfer and storage process in the ***,the current challenges and new perspectives for future developments in the emerging area of SCSPCs or integrated energy devices are discussed.

关键词： electrospinning integrated energy cell mechanical energy piezoelectric separators piezoelectrochemical spectroscopy self-charging supercapacitor power cell

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Upcycling end of lithium cobalt oxide batteries to electrocatalyst for oxygen reduction reaction in direct methanol fuel cell via sustainable approach

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Journal of energy Chemistry 2023年第7期82卷 148-157,I0004页

作者： Keyru Serbara Bejigo Kousik Bhunia Jungho Kim Chaehyeon Lee Seoin Back Sang-Jae Kim Nanomaterials&System Lab Major of Mechatronics EngineeringFaculty of Applied Energy SystemJeju National UniversityJeju 63243Republic of Korea Nanomaterials&System Lab Major of Mechanical System EngineeringCollege of EngineeringJeju National UniversityJeju 63243Republic of Korea Research Institute of New Energy Industry(RINEI) Jeju National UniversityJeju 63243Republic of Korea Department of Chemical and Biomolecular Engineering Institute of Emergent MaterialsSogang UniversitySeoul 04107Republic of Korea

Recycling spent lithium-ion batteries(SLIBs)has become essential to preserve the environment and reclaim vital resources for sustainable *** typical SLIBs recycling concentrated on separating valuable components had limitations,including high energy consumption and complicated separation *** work suggests a safe hydrometallurgical process to recover usable metallic cobalt from depleted LiCoO_(2)batteries by utilizing citric acid as leachant and hydrogen peroxide as an oxidizing agent,with ethanol as a selective precipitating *** anode graphite was also recovered and converted to graphene oxide(GO).The above components were directly resynthesized to cobaltintegrated nitrogen-doped graphene(Co@NG).The Co@NG showed a decent activity towards oxygen reduction reaction(ORR)with a half-wave potential of 0.880 V ***,almost similar to Pt/C(0.888 V ***)and with an onset potential of 0.92 V *** metal-nitrogen-carbon(Co-N-C)having the highest nitrogen content has decreased the barrier for ORR since the reaction was enhanced for Co@NG-800,as confirmed by density functional theory(DFT)*** Co@NG cathode catalyst coupled with commercial Pt-Ru/C as anode catalyst exhibits excellent performance for direct methanol fuel cell(DMFC)with a peak power density of 34.7 mW cm^(-2)at a discharge current density of120 m A cm^(-2)and decent stability,indicating the promising utilization of spent battery materials in DMFC ***,lithium was recovered from supernatant as lithium carbonate by coprecipitation *** work avoids sophisticated elemental separation by utilizing SLIBs for other renewable energy applications,lowering the environmental concerns associated with recycling.

关键词： Density functional theory(DFT) Direct methanol fuel cell Leaching Nitrogen doping Oxygen reduction reaction Recycling Spent lithium-ion batteries

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Robust prediction-based control for unknown time-varying delays and disturbances in spherical motion platform

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Control engineering Practice 2025年 163卷

作者： Seong-Min Lee Sangheon Lee Hungsun Son Department of Mechanical Systems Engineering Jeju National University Jeju 63243 South Korea Major of Mechatronics Engineering and faculty of Applied Energy System Jeju National University Jeju 63243 South Korea School of Mechanical Engineering Kyungpook National University Daegu 41566 South Korea Department of Mechanical Engineering Ulsan National Institute of Science and Technology Ulsan 44919 South Korea

This paper presents a new prediction-based controller utilizing enhanced preview and state prediction methods to deal with unknown time-varying delays and disturbances. In practice, uncertain and variable time delays in virtual reality applications can lead to control instability and a significant reduction in the overall sense of realism. In this paper, a robust prediction-based control (RPC) is proposed for the spherical motion platform (SMP) to compensate for the effects of the time-varying delays and disturbances. The RPC comprises a preview strategy and state/disturbance prediction methods with an estimator to handle unknown time-varying delays. In addition, a newly proposed preview method improves the system’s ability to follow a time-varying reference trajectory. The stability analysis for the time-delayed system incorporating the RPC is conducted using the Lyapunov–Krasovskii approach. Numerical simulations and various experiments demonstrate that the RPC effectively leads the state to converge to the desired trajectory within an error bound under various conditions of time-varying delays in the presence of disturbances, whereas the existing controllers have limitations in reducing the desired control errors. Consequently, the results validate the feasibility and effectiveness of the RPC in real-world applications, demonstrating its robustness in handling time-varying delays through practical implementation on the SMP.

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Comprehensive Insight into the Mechanism, Material Selection and Performance Evaluation of Supercapatteries

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Nano-Micro Letters 2020年第7期12卷 43-88页

作者： Saravanakumar Balasubramaniam Ankita Mohanty Suresh Kannan Balasingam Sang Jae Kim Ananthakumar Ramadoss School for Advanced Research in Polymers Laboratory for Advanced Research in Polymeric MaterialsCentral Institute of Plastics Engineering and TechnologyBhubaneswar 751024India Department of Materials Science and Engineering Faculty of Natural SciencesNorwegian University of Science and Technology(NTNU)Trondheim 7491Norway Nanomaterials and Systems Laboratory Major of Mechatronics EngineeringFaculty of Applied Energy SystemJeju National UniversityJeju 63243Republic of Korea

Electrochemical energy storage devices(EESs)play a crucial role for the construction of sustainable energy storage system from the point of generation to the end user due to the intermittent nature of renewable ***,to meet the demand for next-generation electronic applications,optimizing the energy and power densities of EESs with long cycle life is the crucial *** e orts have been devoted towards the search for new materials,to augment the overall performance of the *** there are a lot of ongoing researches in this field,the performance does not meet up to the level of commercialization.A further understanding of the charge storage mechanism and development of new electrode materials are highly *** present review explains the overview of recent progress in supercapattery devices with reference to their various *** di erent charge storage mechanisms and the multiple factors involved in the performance of the supercapattery are described in ***,recent advancements in this supercapattery research and its electrochemical performances are ***,the challenges and possible future developments in this field are summarized.

关键词： Supercapattery energy density Power density Redox materials Carbon materials

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A Study on the Operation Method of Hybrid energy Storage system Connected with Wind Turbine

A Study on the Operation Method of Hybrid Energy Storage Sys...

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2018 IEEE International Conference on High Voltage engineering and Application, ICHVE 2018

作者： Kang, Min Hyeok Chae, Sang Heon Ahn, Jin Hong Kim, Gi Hoon Lee, Seong Hoon Yang, Seungmoo Kim, Ho Min Kim, Eel-Hwan Faculty of Applied Energy System Major of Electrical Engineering Jeju National University Jeju-si Korea Republic of

ISBN: (纸本)9781538650868

Nowadays, there are many wind farms around the world. However, intermittent characteristics of wind power output can cause unbalanced grid condition between demand load and generation resources, especially in isolated area such as Jeju Island located in the Republic of Korea. Grid operator of Jeju Island has often curtailed wind power output for the stability of Jeju power system. Therefore, this paper proposes not only installation of hybrid energy storage system (HESS) combining lithium-ion battery with water electrolysis device (WED), but also its operation algorithm to save controlled wind power output. This system will be focused on supplying electrical power stably to WED by using wind power generation and lithium-ion battery, because the WED should be always turned on to prevent lifetime degradation. The proposed method will be applied to simulation model including wind turbine generator, lithium-ion battery, WED and power conversion systems. The simulation results will be carried out using PSCAD/EMTDC program. © 2018 IEEE.

关键词： Lithium-ion batteries

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Tunable Phase-Engineered Polyhydroxybutyrate Fibrous Mat: An energy Autonomous, Temperature-Responsive Platform for Wearable Application

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Advanced Fiber Materials 2025年

作者： Sharma, Kusum Alluri, Nagamalleswara Rao Prasanna, Asokan Poorani Sathya Perumalsamy, Muthukumar Saj, Anandhan Ayyappan Ryu, Yeonkyeong Lee, Ju-Hyuck Park, Kwi-Il Kim, Sang-Jae Nanomaterials and System Lab Major of Mechatronics Engineering Faculty of Applied Energy System Jeju National University Jeju63243 Korea Republic of Research Institute of Automotive Parts and Materials Kyungpook National University Buk-Gu Daegu41566 Korea Republic of Department of Materials Science and Metallurgical Engineering Kyungpook National University Buk-Ku Daegu41566 Korea Republic of Department of Energy Science and Engineering Daegu Gyeongbuk Institute of Science and Technology 333 Techno Jungang-Daero Dalseong-Gun Daegu42988 Korea Republic of Nanomaterials and System Lab Major of Mechanical System Engineering College of Engineering Jeju National University Jeju63243 Korea Republic of Jeju National University Jeju63243 Korea Republic of Jeju National University Jeju63243 Korea Republic of

Biodegradable and biocompatible organic polymers play a pivotal role in designing the next generation of wearable smart electronics, reducing electronic waste and carbon emissions while promoting a toxin-free environment. Herein, an electrospun fibrous polyhydroxybutyrate (PHB) organic mat-based, energy-autonomous, skin-adaptable temperature sensor is developed, eliminating the need for additional storage or circuit components. The electrospun PHB mat exhibits an enhanced β-crystalline phase with a β/α phase ratio of 3.96 using 1,1,1,3,3,3-hexafluoro-2-propanol as a solvent. Solvent and film processing techniques were tailored to obtain high-quality PHB films with the desired thickness, flexibility, and phase conversion. The PHB mat-based temperature sensor (PHB–TS) exhibits a negative temperature coefficient of resistance, with a sensitivity of − 2.94%/°C and a thermistor constant of 4676 K, outperforming pure metals and carbon-based sensors. A triboelectric nanogenerator (TENG) based on the enhanced β-phase PHB mat was fabricated, delivering an output of 156 V, 0.43 µA, and a power density of 1.71 mW/m2. The energy-autonomous PHB–TS was attached to the index finger to monitor temperature changes upon contact with hot and cold surfaces, demonstrating good reliability and endurance. © Donghua University, Shanghai, China 2025.

关键词： Electrospinning

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Comparative thermodynamic performance assessment of two-stage cycle for various refrigerants

Comparative thermodynamic performance assessment of two-stag...

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作者： Yilmaz, Fatih Ozturk, Murat Selbaş, Reşat Department of Electrical and Energy Vocational School of Technical Science Aksaray University 68100 Turkey Department of Mechatronics Engineering Faculty of Technology Applied Science University of Isparta Cunur West Campus Isparta32200 Turkey Department of Energy System Engineering Faculty of Technology Applied Science University of Isparta Cunur West Campus Isparta32200 Turkey

In this paper, the thermodynamic performance evaluations of the two-stage cooling cycle are investigated comparatively for different refrigerants under the same operating conditions. Due to their environmentally friendly properties, CO2, R600, R600a, R161, and R134a are selected as the refrigerants. The change in energy performance coefficient (COPen) and exergy performance coefficient (COPex) of the defined cycle are investigated according to the various indicators, such as reference temperature, gas cooler outlet temperature and pressure. Results are shown that, at the evaporator temperature of -5°C and the gas cooler outlet temperature of 40°C, the COPen of the cooling cycle are 1.644, 1.603, 1.452, 2.0356 and 1.928 for the refrigerants CO2, R600, R600a, R161 and R134a, respectively. Furthermore, COPex of the cycle are computed as 25.94%, 15.57%, 14.07%, 19.73% and 18.68% for the same refrigerants in the same order. In addition, the overall exergy destruction rate of the cooling cycle for CO2 refrigerant is calculated as 145.69 kW. © 2019 Inderscience Enterprises Ltd.

关键词： Refrigerants

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Piezo-phototronic Dependent Enhanced Charge Transportation in SbSI Micro Rod Photodetector

Piezo-phototronic Dependent Enhanced Charge Transportation i...

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OptoElectronics and Communications Conference, OECC

作者： Yuvasree Purusothaman Nagamalleswara Rao Alluri Sang-Jae Kim Department of Mechatronics Engineering Nanomaterials and System Lab Faculty of Applied Energy System Jeju National University Republic of Korea

We demonstrate the enhancement of photocurrent response of antimony sulfoiodide (SbSI) based optical detector through piezo-phototronic effect. The band interface modulation via strain engineering exhibits fast switch... 详细信息

ISBN: (纸本)9781538691465

关键词： Strain Optical switches Photodetectors Photoconductivity Piezoelectric polarization Charge carriers

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