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Construction of dual Z-scheme Ag3VO4–BiVO4/InVO4 photocatalysts using vanadium source from spent catalysts for contaminated water treatment and bacterial inactivation

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Chemosphere 2024年 363卷 142746页

作者： Lee, Kuen-Chan Hsu, Shih-Chieh Huang, Jen-Hsien Wang, Kuan-Syun Pang, Wei Kong Hu, Chih-Wei Jiang, Yi-Jhen Cho, Er-Chieh Weng, Huei Chu Liu, Ting-Yu Department of Science Education National Taipei University of Education No. 134 Sec. 2 Heping E. Road Da-an District Taipei City106 Taiwan PhD Program in Medical Neuroscience College of Medical Science and Technology Taipei Medical University 250 Wuxing Street Taipei City110 Taiwan Department of Chemical and Materials Engineering Tamkang University No. 151 Yingzhuan Road Tamsui District New Taipei City25137 Taiwan Department of Green Material Technology Green Technology Research Institute CPC Corporation No.2 Zuonan Rd. Nanzi District Kaohsiung City81126 Taiwan Department of Materials Engineering Ming Chi University of Technology New Taipei City243303 Taiwan Faculty of Engineering Institute for Superconducting & Electronic Materials University of Wollongong WollongongNSW Australia National Synchrotron Radiation Research Center 101 Hsin-Ann Road Hsinchu Science Park Hsinchu30076 Taiwan School of Pharmacy College of Pharmacy Taipei Medical University 250 Wuxing Street Taipei City110 Taiwan Department of Mechanical Engineering Chung Yuan Christian University No. 200 Chungpei Road Chungli District Taoyuan City32023 Taiwan Department of Chemical Engineering and Materials Science Yuan Ze University Taoyuan City32003 Taiwan College of Engineering & Center for Sustainability and Energy Technologies Chang Gung University Taoyuan33302 Taiwan

Vanadate-based photocatalysts have recently attracted substantial attention owing to their outstanding photocatalytic activity for degrading organic pollutants and generating energy via photocatalytic processes. However, the relatively high price of vanadium has hindered the development of vanadate-based photocatalysts for various applications. Spent catalysts obtained from oil refineries typically contain a significant quantity of vanadium, making them valuable for recovery and utilization as precursors for the production of high-value-added photocatalysts. In this study, we transformed the V present in spent catalysts produced by the petrochemical industry into ternary vanadate-based photocatalysts [BiVO4/InVO4/Ag3VO4 (BVO/IVO/AVO, respectively)] designed for water remediation. The ternary composites revealed an enhanced photocatalytic capability, which was 1.42 and 5.1 times higher than those of the binary BVO/IVO and pristine AVO due to the facilitated charge separation. The ternary photocatalysts not only effectively treated wastewater containing various organic dyes, such as methylene blue (MB), rhodamine 6G (R6G), and brilliant green (BG), but also exhibited remarkable photocatalytic performance in the degradation of antibiotics, reduction of Cr(VI), and bacterial inactivation. This paper proposes a feasible route for recycling industrial waste as a source of vanadium to produce highly efficient vanadate-based photocatalysts. © 2024 Elsevier Ltd

关键词： Water pollution

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Cold atmospheric plasma-enabled platelet vesicle incorporated iron oxide nano-propellers for thrombolysis

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materials Today Bio 2023年 23卷 100876页

作者： Jheng, Pei-Ru Chiang, Chia-Che Kang, Jiunn-Horng Fan, Yu-Jui Wu, Kevin C.-W. Chen, Yan-Ting Liang, Jia-Wei Bolouki, Nima Lee, Jyh-Wei Hsieh, Jang-Hsing Chuang, Er-Yuan Graduate Institute of Nanomedicine and Medical Engineering Graduate Institute of Biomedical Materials and Tissue Engineering Institute of Biomedical Optomechatronics International Ph.D. Program in Biomedical Engineering School of Biomedical Engineering College of Biomedical Engineering Professional Master Program in Artificial Intelligence in Medicine College of Medicine Taipei Medical University Taipei11031 Taiwan Department of Physical Medicine and Rehabilitation Taipei Medical University Hospital Taipei Taiwan Institute of Biomedical Engineering & Nanomedicine National Health Research Institute Keyan Road Zhunan Miaoli City350 Taiwan Department of Chemical Engineering National Taiwan University No.1 Sec. 4 Roosevelt Rd Taipei10617 Taiwan Department of Plasma Physics and Technology Faculty of Science Masaryk University Brno Czech Republic Center for Plasma and Thin Film Technologies Ming Chi University of Technology New Taipei City Taiwan Department of Materials Engineering Ming Chi University of Technology New Taipei City Taiwan Cell Physiology and Molecular Image Research Center Taipei Medical University-Wan Fang Hospital Taipei11696 Taiwan

A new approach to treating vascular blockages has been developed to overcome the limitations of current thrombolytic therapies. This approach involves biosafety and multimodal plasma-derived theranostic platelet vesicle incorporating iron oxide constructed nano-propellers platformed technology that possesses fluorescent and magnetic features and manifold thrombus targeting modes. The platform is capable of being guided and visualized remotely to specifically target thrombi, and it can be activated using near-infrared phototherapy along with an actuated magnet for magnetotherapy. In a murine model of thrombus lesion, this proposed multimodal approach showed an approximately 80 % reduction in thrombus residues. Moreover, the new strategy not only improves thrombolysis but also boosts the rate of lysis, making it a promising candidate for time-sensitive thrombolytic therapy. © 2023 The Authors

关键词： Infrared devices

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A theoretical investigation of some N-hydroxymethyl amino acids as corrosion inhibitors for mild steel 59th

A theoretical investigation of some N-hydroxymethyl amino ac...

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59th International Scientific Conference of Riga Technical University (RTU) Section of materials science and Applied Chemistry, MSAC 2018

作者： Özdemir, Emre Gece, Gökhan Advanced Technologies Material Science and Engineering Program Graduate School of Natural and Applied Sciences Bursa Technical University Bursa Turkey Department of Chemistry Faculty of Engineering and Natural Sciences Bursa Technical University Bursa Turkey

ISBN: (纸本)9783035714074

In this study the dependence of corrosion inhibition and microbial effects of four N-hydroxymethylated amino acids on their molecular and electronic structure was analyzed using density functional theory calculations. Quantum chemical parameters, such as highest occupied molecular orbital energy (EHOMO), lowest unoccupied molecular orbital energy (ELUMO), energy gap (ΔE) were calculated at the B3LYP/6-311G++(d,p) basis set. Although no simple relationship between the inhibition performance and the calculated data could be discerned, the comparison of inactivation rate constants with energetic parameters suggested that microbial effects of the compounds can be explained in terms of their side chain disparities. © 2019 Trans Tech Publications, Switzerland

关键词： Density functional theory

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Microscopic picture of paraelectric perovskites from structural prototypes

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Physical Review Research 2022年第1期4卷 L012042-L012042页

作者： Michele Kotiuga Samed Halilov Boris Kozinsky Marco Fornari Nicola Marzari Giovanni Pizzi Theory and Simulation of Materials (THEOS) National Centre for Computational Design and Discovery of Novel Materials (MARVEL) École Polytechnique Fédérale de Lausanne CH-1015 Lausanne Switzerland Designed Material Technologies LLC P.O. Box 14548 Richmond Virginia 23221-9998 USA John A. Paulson School of Engineering and Applied Sciences Harvard University 29 Oxford Street Cambridge Massachusetts 02138 USA Robert Bosch LLC Research and Technology Center Cambridge Massachusetts 02139 USA Department of Physics and Science of Advanced Materials Program Central Michigan University Mt. Pleasant Michigan 48859 USA

We highlight with first-principles molecular dynamics the persistence of intrinsic 〈111〉 Ti off-centerings for BaTiO3 in its cubic paraelectric phase. Intriguingly, these are inconsistent with the Pm3¯m space group often used to atomistically model this phase using density-functional theory or similar methods. Therefore, we deploy a systematic symmetry analysis to construct representative structural models in the form of supercells that satisfy a desired point symmetry but are built from the combination of lower-symmetry primitive cells. We define as structural prototypes the smallest of these that are both energetically and dynamically stable. Remarkably, two 40-atom prototypes can be identified for paraelectric BaTiO3; these are also common to many other ABO3 perovskites. These prototypes can offer structural models of paraelectric phases that can be used for the computational engineering of functional materials. Last, we show that the emergence of B-cation off-centerings and the primitive-cell phonon instabilities is controlled by the equilibrium volume, in turn, dictated by the filler A cation.

关键词： Crystal symmetry Ferroelectricity Structural order parameter Paraelectrics

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Bioenergy knowledge, perception and attitude among students at Jambi state senior high school

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Journal of Physics: Conference Series 2021年第1期1816卷

作者： Nazarudin M P H Hasibuan B Haryadi Nurhayati Ulyarti Hadiyanto Chemical Engineering FST University of Jambi Jambi Indonesia Energy and Nano Material Centre LPPM Universitas Jambi Jambi Indonesia Center of Excellent on Bio-Geo Material and Energy Universitas Jambi Jambi Indonesia Master of Enviromental Study Program University of Jambi Jambi Indonesia Master of Science Education Program University of Jambi Jambi Indonesia

Bioenergy is one of the renewable energies which is predicted to be a main energy in the next few years. It can play the important role to change the current fossil fuel-based energy into a green energy which has a low carbon footprint. A research about how to develop a bioenergy have been done by a lot of reseacher. However, especially in Indonesia, there is just few research to study about bioenergy from societal aspects poin of view such as the understanding and awarness of bioenergy among citizens. In this research, we have investigated senior high school students' knowledge, perceptions, and attitudes interconected to bioenergy with online survery. The survey instrument used in the study was adopted from P. Halder's study. The data was collected from students at senior high school th (SMAN 10) Jambi City. The results showed that the students awareness of bioenergy perceived from school, home, and social media have significant effects on their knowledge, perceptions and attitudes related to bioenergy. Among 211 students as respondent (N), we found 70.62% believe that they understand well the concept about bioenergy, 5.21% believe that they understand it very well, and the rest believe that they do not understand it. This understanding reflects to their willingness to use a bioenergy in their daily life, in which 71.70% respondents agree to use bioenergy, 25.47% respondents can not decide, and only 2.83% do not want to use it. To find the relationship among the variables, a multiple regression was conducted. A statistical analysis showed that the model for knowledge as a function of attitudes and perception does not fit the data therefore this model is rejected. However, both model for attitudes as function of perception and knowledge, and also perception as function of attitudes and knowldeges fit the data hence the models are accepted. In other words, attitudes of students who will use/not use bioenergy, is significantly affected by their perception about bioen

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Measurement and analysis of thermal conductivity of ceramic particle beds for solar thermal energy storage

arXiv

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arXiv 2021年

作者： Chung, Ka Man Zeng, Jian Adapa, Sarath Reddy Feng, Tianshi Bagepalli, Malavika V. Loutzenhiser, Peter G. Albrecht, Kevin J. Ho, Clifford K. Chen, Renkun Material Science and Engineering Program University of California San Diego San DiegoCA92093 United States Department of Mechanical and Aerospace Engineering University of California San Diego San DiegoCA92093 United States George W. Woodruff School of Mechanical Engineering Georgia Institute of Technology AtlantaGA30332-0405 United States Concentrating Solar Technologies Department Sandia National Laboratories 1515 Eubank Blvd. SE AlbuquerqueNM87123 United States

A systematic study was performed to measure the effective thermal conductivity of ceramic particle beds, a promising heat transfer and thermal energy storage media for concentrating solar power (CSP). The thermal conductivity of the ceramic particle beds was measured using a transient hot-wire (THW) method within a temperature range of room temperature to 700 oC, the target operating temperature of the next-generation CSP systems. Two different types of ceramic particles were examined: (1) CARBOBEAD HSP 40/70 and (2) CARBOBEAD CP 40/100 with the average particle sizes of ~ 400 μm and ~280 μm, respectively, and thermal conductivities ranging from ~0.25 W m-1 K-1 to ~0.50 W m-1 K-1 from 20 oC to 700 oC in both air and N2 gas. The gaseous pressure dependence of the thermal conductivity of the ceramic particle beds was also studied in the N2 environment to differentiate the contributions from gas conduction, solid conduction, and radiation. Calculations using the Zehner, Bauer, and Schlünder (ZBS) model showed good agreements with the measurements. Based on the model, it is concluded that the effective thermal conductivity of the packed particle beds is dominated by the gas conduction while the solid conduction and radiation contributes to about 20% of the effective thermal conductivity at high temperature. Copyright © 2021, The Authors. All rights reserved.

关键词： Heat storage

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A novel evolution-based recommendation system 12

A novel evolution-based recommendation system

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12th International Conference on Ubi-Media Computing, Ubi-Media 2019

作者： Chen, Yi-Cheng Chu, Yen-Lung Hui, Lin Chen, Sheng-Chih Thaipisutikul, Tipajin Weng, Kai-Ze Department of Information Management National Central University Taiwan Department of Computer Science and Information Engineering Tamkang University Taiwan Department of Innovative Information and Technology Tamkang University Taiwan Master's Program of Digital Content and Technologies College of Communication National ChengChi University Taiwan Department of Computer Science and Information Engineering National Central University Taiwan

ISBN: (纸本)9781728128207

Matrix factorization (MF) technique has been widely utilized in recommendation systems due to the precise prediction of users' interests. Prior MF-based methods adapt the overall rating to make the recommendation by extracting latent factors from users and items. However, in real applications, people's preferences usually vary with time;the traditional MF-based methods could not properly capture the change of users' interests. In this paper, by incorporating the recurrent neural network (RNN) into MF, we develop a novel recommendation system, M-RNN-F, to effectively describe the preference evolution of users over time. A learning model is proposed to capture the evolution pattern and predict the user preference in the future. The experimental results show that M-RNN-F performs better than other state-of-the-art recommendation algorithms. In addition, we conduct the experiments on real world dataset to demonstrate the practicability. © 2019 IEEE.

关键词： Recommender systems

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Terahertz Cavity Phonon Polaritons in the Deep-Strong Coupling Regime

Terahertz Cavity Phonon Polaritons in the Deep-Strong Coupli...

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International Conference on Infrared and Millimeter Waves

作者： Andrey Baydin Manukumara Manjappa Sobhan Subhra Mishra Hongjing Xu Jacques Doumani Fuyang Tay Dasom Kim Felix G. G. Hernandez Paulo H. O. Rappl Eduardo Abramof Ranjan Singh Junichiro Kono Department of Electrical and Computer Engineering Rice University Houston TX USA Smalley-Curl Institute Rice University Houston TX USA Department of Instrumentation and Applied Physics Indian Institute of Science Bangalore India Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University Singapore Department of Physics and Astronomy Rice University Houston TX USA Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston TX USA Instituto de Física Universidade de São Paulo São Paulo SP Brazil Laboratório Associado de Sensores e Materiais Instituto Nacional de Pesquisas Espaciais São José dos ampos SP Brazil Center for Disruptive Photonic Technologies The Photonics Institute Nanyang Technological University Singapore Department of Material Science and NanoEngineering Rice University Houston TX USA

We have studied the resonant and nonperturbative coupling of transverse optical phonons in lead telluride with photons in small-mode-volume terahertz cavities, observing a giant vacuum Rabi splitting on the order of the uncoupled phonon and cavity frequencies. Our terahertz time-domain spectroscopy experimental data, systematically collected as a function of sample thickness, temperature, and cavity length, can be well reproduced by our electromagnetic simulations. These results demonstrate that this uniquely tunable platform is promising for realizing and understanding predicted cavity-vacuum-induced ferroelectric instabilities, as well as for exploring applications of light-matter coupling in the ultra-and deep-strong coupling regimes in quantum technology.

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Deep-Strong Coupling between Cavity Photons and Terahertz TO Phonons in PbTe

Deep-Strong Coupling between Cavity Photons and Terahertz TO...

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Conference on Lasers and Electro-Optics (CLEO)

作者： Andrey Baydin Manukumara Manjappa Sobhan Subhra Mishra Hongjing Xu Fuyang Tay Dasom Kim Felix G. G. Hernandez Paulo H. O. Rappl Eduardo Abramof Ranjan Singh Junichiro Kono Department of Electrical and Computer Engineering Rice University Houston Texas USA Smalley-Curl Institute Rice University Houston Texas USA Instrumentation and Applied Physics Department Indian Institute of Science Bangalore India Center for Disruptive Photonic Technologies The Photonics Institute Nanyang Technological University Singapore Department of Physics and Astronomy Rice University Houston Texas USA Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston Texas USA Instituto de Física Universidade de São Paulo São Paulo SP Brazil Laboratório Associado de Sensores e Materiais Instituto Nacional de Pesquisas Espaciais São José dos Campos SP Brazil Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University Singapore Department of Material Science and NanoEngineering Rice University Houston Texas USA

We have investigated the resonant coupling of photons with TO phonons in lead telluride in small-mode-volume terahertz cavities, observing a giant vacuum Rabi splitting on the order of the bare cavity–phonon frequency.

ISBN: (纸本)9781957171258

关键词： Electric fields Numerical simulation Optical constants Photons Physical vapor deposition Terahertz spectroscopy

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Terahertz Cavity Phonon Polaritons in Lead Telluride in the Deep-Strong Coupling Regime

arXiv

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arXiv 2025年

作者： Baydin, Andrey Manjappa, Manukumara Mishra, Sobhan Subhra Xu, Hongjing Doumani, Jacques Tay, Fuyang Kim, Dasom Rappl, Paulo H.O. Abramof, Eduardo Singh, Ranjan Hernandez, Felix G.G. Kono, Junichiro Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Smalley–Curl Institute Rice University HoustonTX77005 United States Rice Advanced Materials Institute Rice University HoustonTX77005 United States Instrumentation and Applied Physics Department Indian Institute of Science Bangalore560012 India Center for Disruptive Photonic Technologies The Photonics Institute Nanyang Technological University 639798 Singapore Department of Physics and Astronomy Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley–Curl Institute Rice University HoustonTX77005 United States Group of Research and Development in Materials and Plasma National Institute for Space Research São José dos Campos São Paulo12201-970 Brazil Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University 637371 Singapore Instituto de Física Universidade de São Paulo São Paulo05508-090 Brazil Department of Material Science and NanoEngineering Rice University HoustonTX77005 United States

Lead telluride is an important thermoelectric material due to its large Seebeck coefficient combined with its unusually low thermal conductivity that is related to the strong anharmonicity of phonons in this material. Here, we have studied the resonant and nonperturbative coupling of transverse optical phonons in lead telluride with cavity photons inside small-mode-volume metallic metasurface cavities that have photonic modes with terahertz frequencies. We observed a giant vacuum Rabi splitting on the order of the bare phonon and cavity frequencies. Through terahertz time-domain spectroscopy experiments, we systematically studied the vacuum Rabi splitting as a function of sample thickness, temperature, and cavity length. Under the strongest light–matter coupling conditions, the strength of coupling exceeded the bare phonon and cavity frequencies, putting the system into the deep-strong coupling regime. These results demonstrate that this uniquely tunable platform is promising for realizing and understanding predicted cavity-vacuum-induced ferroelectric instabilities and exploring applications of light–matter coupling in the ultrastrong and deep-strong coupling regimes in quantum technology. Copyright © 2025, The Authors. All rights reserved.

关键词： Phonons

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