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High-performance 110 kVp hard x-ray detector based on all-crystalline-surface passivated perovskite single crystals

InfoMat 2024年第8期6卷 97-110页

作者： Juyoung Ko Beomjun Park Jangwon Byun Sandeep Pandey Ajin Jo Joo-Hong Lee Wonho Lee Jin-Wook Lee Nam-Gyu Park Man-Jong Lee Department of Chemistry Konkuk UniversitySeoulRepublic of Korea Advanced Crystal Material/Device Research Center Konkuk UniversitySeoulRepublic of Korea Health Science Research Center Korea UniversitySeoulRepublic of Korea Department of Nano Engineering and Department of Nano Science and Technology SKKU Advanced Institute of Nanotechnology(SAINT)Sungkyunkwan UniversitySuwonRepublic of Korea SKKU Institute of Energy Science&Technology(SIEST) Sungkyunkwan UniversitySuwonRepublic of Korea Department of Health and Environmental Science Korea UniversitySeoulRepublic of Korea School of Chemical Engineering Center for Antibonding Regulated CrystalsSungkyunkwan UniversitySuwonRepublic of Korea

Halide perovskite single crystals(SCs)have attracted much attention for their application in high-performance x-ray detectors owing to their desirable properties,including low defect density,high mobility–lifetime product(μτ),and long carrier diffusion ***,suppressing the inherent defects in perovskites and overcoming the ion migration primarily caused by these defects remains a *** study proposes a facile process for dipping Cs0.05FA0.9MA0.05PbI3 SCs synthesized by a solution-based inverse temperature crystallization method into a 2-phenylethylammonium iodide(PEAI)solution to reduce the number of defects,inhibit ion migration,and increase x-ray *** to conventional spin coating,this simple dipping process forms a two-dimensional PEA2PbI4 layer on all SC surfaces without further treatment,effectively passivating all surfaces of the inherently defective SCs and minimizing ion *** a result,the PEAI-treated perovskite SC-based x-ray detector achieves a record x-ray sensitivity of 1.3×10^(5)μC Gyair^(-1) cm^(-2) with a bias voltage of 30 V at realistic clinical dose rates of 1–5 mGy s^(-1)(peak potential of 110 kVp),which is 6 times more sensitive than an untreated SC-based detector and 3 orders of magnitude more sensitive than a commercialα-Se-based ***,the PEAI-treatedperovskite SC-based x-ray detector exhibits a low detection limit(73 nGy s^(-1)),improved x-ray response,and clear x-ray images by a scanning method,highlighting the effectiveness of the PEAI dipping approach for fabricating next-generation x-ray detectors.

关键词： 2D PEA2PbI4 layers clinical dose rates perovskite single crystals phenethylammonium iodide(PEAI) surface passivation x-ray sensitivity

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Herceptin-Positive Breast Cancer Treatment via Immunoliposomes Triggered by High-Frequency Ultrasound and Microbubbles 17

Herceptin-Positive Breast Cancer Treatment via Immunoliposom...

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17th IEEE International Conference on Nano/Molecular Medicine and engineering, NANOMED 2024

作者： Abuwatfa, Waad H. Anjum, Shabana Pitt, William Husseini, Ghaleb A. American University of Sharjah Material Science and Engineering PhD Program College of Arts and Sciences Sharjah United Arab Emirates American University of Sharjah Department of Chemical and Biological Engineering Sharjah United Arab Emirates Brigham Young University Department of Chemical Engineering ProvoUT84604 United States

ISBN: (纸本)9798331516994

Functionalizing chemotherapeutics-loaded liposomes with monoclonal antibodies can enhance their specificity and minimize side effects. Targeting the human epidermal growth factor receptor 2 (HER2), overexpressed in HER2-positive breast cancer, is achievable by coating liposomes with an anti-HER2 monoclonal antibody. This study focused on synthesizing doxorubicin (DOX)-loaded immunoliposomes functionalized with anti-HER2 (HER-lip). The release of the drug from these immunoliposomes was triggered by high-frequency ultrasound (HFUS) and microbubbles, which acted as exogenous cavitation-enhancing agents. The platform was evaluated for size, lipid content, protein concentration, stability, and controlled release profiles. In vitro assessments were also performed, including the MTT assay for cell viability and flow cytometry to evaluate drug uptake. This innovative drug delivery system shows potential for combined therapeutic and diagnostic applications, improving personalized cancer care and treatment. © 2024 IEEE.

关键词： Monoclonal antibodies

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Guided organic exciton-polaritons on patterned distributed Bragg reflectors at room temperature

Guided organic exciton-polaritons on patterned distributed B...

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CLEO: Fundamental science, CLEO:FS 2024 - Part of Conference on Lasers and Electro-Optics, CLEO 2024

作者： Liu, Bin Horowitz, Jeffrey Forrest, Stephen R. Department of Electrical Engineering and Computer Science University of Michigan Ann ArborMI48109 United States Department of Physics University of Michigan Ann ArborMI48109 United States Department of Material Science and Engineering University of Michigan Ann ArborMI48109 United States

We demonstrate guided long-range excitation energy transport mediated by exciton-polaritons on different patterned distributed Bragg reflectors at room temperature, which results from strong coupling between organic e... 详细信息

ISBN: (纸本)9781957171395

关键词： Distributed Bragg reflectors

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Bubble-pen lithography:Fundamentals and applications

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Aggregate 2022年第4期3卷 85-100页

作者： Pavana Siddhartha Kollipara Ritvik Mahendra Jingang Li Yuebing Zheng Walker Department of Mechanical Engineering The University of Texas at AustinAustinTexasUSA Department of Electrical and Computer Engineering The University of Texas at AustinAustinTexasUSA Material Science and Engineering Program Texas Materials InstituteThe University of Texas at AustinAustinTexasUSA

Developing on-chip functional devices requires reliable fabrication methods with high resolution for miniaturization,desired components for enhanced performance,and high throughput for fast prototyping and mass ***,laser-based bubble-pen lithography(BPL)has been developed to enable sub-micron linewidths,in situ synthesis of custom materials,and on-demand patterning for various functional components and *** exploits Marangoni convection induced by a laser-controlled microbubble to attract,accumulate,and immobilize particles,ions,and molecules onto different *** years have witnessed tremendous progress in theory,engineering,and application of BPL,which motivated us to write this ***,an overview of experimental demonstrations and theoretical understandings of BPL is ***,we discuss the advantages of BPL and its diverse applications in quantum dot displays,biological and chemical sensing,clinical diagnosis,nanoalloy synthesis,and *** conclude this review with our perspective on the challenges and future directions of BPL.

关键词： additive manufacturing capillary flow lithography marangoni convection microbubbles sensing

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Interface engineering and Anion engineering of Mo-Based Heterogeneous Electrocatalysts for Hydrogen Evolution Reaction

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Energy & Environmental materials 2023年第1期6卷 87-104页

作者： Zehao Yin Xuan Liu Siru Chen Tingli Ma Yanqiang Li State Key Laboratory of Fine Chemicals School of Chemical EngineeringDalian University of TechnologyPanjin CampusPanjin 124221China School of Material and Chemical Engineering Centre for Advanced Materials ResearchZhongyuan University of TechnologyZhengzhou 450007China Department of Materials Science and Engineering China Jiliang UniversityHangzhou 310018China Graduate School of Life Science and Systems Engineering Kyushu Institute of TechnologyKitakyushu Fukuoka 808-0196Japan

Development and utilization of hydrogen energy is an effective way to achieve carbon neutrality,only hydrogen production through electrolytic water splitting meets the goal of zero carbon *** facilitate the large-scale commercialization of water splitting devices,the development of highly efficient and low-cost catalysts to reduce the energy consumption is ***_(2)has been regarded as a promising electrocatalyst to replace platinum in hydrogen evolution reaction due to its low price and unique 2D layered ***,the poor conductivity and inert basal planes of MoS_(2)limited its wide-spread ***,researches have demonstrated that the conductivity and active sites of MoS_(2)can be improved by heteroatoms doping or constructing of heterogeneous *** this review,the recent progress of Mo-based catalysts are summarized centered on MoS_(2)based on interface engineering and anion engineering,including MoS_(2)–MoO_(2),MoS_(2)–Mo_(2)C,MoS_(2)–MoN_(x),MoS_(2)–MoP,and MoS_(2)–MoSe_(2).The preparation method,structure,and performance of the catalysts are introduced and the possible mechanism behind the improved catalytic activity are revealed to give readers an overall comprehension on the progress of the Mo-based electrocatalysts for hydrogen evolution *** addition,an outlook on future opportunities and development directions of Mo-based catalysts are proposed to facilitate the development of Mo-based catalysts for hydrogen production.

关键词： electrocatalysis heterostructure hydrogen evolution reaction Mo-based catalysts

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Evaluating the Efficiency of CuInGaSe2 Based Solar Cells: CuSCN Hole Transport Layer (HTL) Effect 3

Evaluating the Efficiency of CuInGaSe2 Based Solar Cells: Cu...

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2024 3rd International Conference on Advances in Modern Physics sciences and engineering Technology, ICPSET 2024

作者： Zaidi, B. Mekhaznia, N. Ullah, M.S. Al-Dmour, H. Department of Physics Faculty of Material Sciences University of Batna 1 Batna Algeria Department of Material Sciences SESNV-Faculty Echahid Cheikh Larbi Tebessi University Tebessa Algeria Department of Electrical and Computer Engineering Florida Polytechnic University Lakeland United States Department of Physics Faculty of Science Mutah University Mutah61710 Jordan

Copper indium gallium disulfide (CuInGaSe2) or (CIGS) based solar cells are emerging solar cell structures that have attracted significant interest in recent years. In this research, a SCAPS-1D simulator was used to investigate the performance of the proposed CIGS based solar cell under the effect of a copper (I) thiocyanate (CuSCN) hole transport layer (HTL). Different photovoltaic parameters, such as the efficiency, short circuit current density (Jsc) and open-circuit voltage (Voc), are observed with respect to the doping concentration, temperature, and thickness. A comparative study is presented between a hole transport layer (HTL) and without an HTL. The simulation results demonstrate that the HTL has a significant impact and plays a major role in improving the performance of the proposed CIGS solar cell structure compared to that without the HTL. This research outlines a structured guide for both the manufacturing process and achievement of cost-effective, highly efficient solar cells. © 2024 Institute of Physics Publishing. All rights reserved.

关键词： Gallium compounds

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Towards sustainable H2 evolution by using an algal-electro-photosynthetic process: The mediator selection alternates the electron sources for Chlorella sorokiniana SU-1

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International Journal of Hydrogen Energy 2023年第46期48卷 17409-17419页

作者： Li, Shiue-Lin Liao, En-Ci Lin, Yu-Jun Lu, Yun-Ju Zhang, Yu-Sheng Tseng, Yen-Tzu Jiang, Yu-Jie Chiang, Tzu-Hao Gao, Zhi-Xiang Li, Pei-Xuan Chang, Jo-Shu Department of Environmental Science and Engineering Tunghai University Taichung40704 Taiwan Department of Chemical and Material Engineering Tunghai University Taichung40704 Taiwan Department of Chemical Engineering National Cheng Kung University Tainan701 Taiwan Research Center for Smart Sustainable Circular Economy Tunghai University Taichung40704 Taiwan Department of Chemical Engineering and Materials Science Yuan Ze University Chung-Li32003 Taiwan

Chlorella sorokiniana SU-1 is employed on the graphite-felt anode of a two-chamber cell connecting potentiostat (+0.4 V vs Ag/AgCl) to study its photoelectrochemical characteristics. Among the mediators selected, the current significantly reached 1.5 mA and 4.0 mA, respectively, when 0.3 mM 2,6-dimethoxy-1,4-benzoquinone and 5.5 mM ferricyanide were spiked. To give significant hydrogen evolution, the applied direct-circuit voltage could be reduced from 2.0 to 1.3 V (producing 1.5 mL-H2 h−1) due to the assistance of the algae-attached anode and platinum-mesh cathode. The current was boosted by spiking 0.2 g L−1 glucose under light/dark conditions. When using ferricyanide as a mediator, the current oscillated under alternating light-on/off conditions, while for 2,6-dimethoxy-1,4-benzoquinone, the increase or decrease of the current was clearly responding to the light going on and off. The microscopic observation of the SU-1 cell attachment indicates successful development by offering adequate illumination and electrode surfaces. © 2023 Hydrogen Energy Publications LLC

关键词： Anodes

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Non-contact Burst Monitoring via Dual Fiber Fabry-Perot Interferometers

Non-contact Burst Monitoring via Dual Fiber Fabry-Perot Inte...

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2024 Conference on Lasers and Electro-Optics, CLEO 2024

作者： Wang, Ruixuan Homa, Daniel Dejneka, Zach Theis, Logan Wang, Anbo Pickrell, Gary Center for Photonics Technology The Bradley Department of Electrical and Computer Engineering Virginia Tech BlacksburgVA United States Center for Photonics Technology Department of Material Science and Engineering Virginia Tech BlacksburgVA United States

Introducing a dual Fabry-Perot sensor system for non-contact pipe burst monitoring. With a lab-standard dual-ferrule probe, we measure absolute distance from the pipe and differentiate bursting events from absolute dr... 详细信息

ISBN: (纸本)9781957171395

关键词： Fabry-Perot interferometers

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Recent Progress in the Auxiliary Phase Enhanced Flexible Piezocomposites

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Energy & Environmental materials 2025年第1期8卷 292-312页

作者： Xin Gao Mupeng Zheng Boyue Hou Junshu Wu Mankang Zhu Yunfan Zhang Ke Wang Bing Han College of Materials Science and Engineering Beijing University of TechnologyBeijing 100124China School of Basic Medical Sciences Capital Medical UniversityBeijing 100069China Department of Orthodontics Peking University School and Hospital of Stomatology&National Center of Stomatology&National Engineering Laboratory for Digital and Material Technology of Stomatology&NMPA Key Laboratory for Dental MaterialsBeijing 100089China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China

Piezocomposites with both flexibility and electromechanical conversion characteristics have been widely applied in various fields,including sensors,energy harvesting,catalysis,and biomedical *** the composition of piezocomposites or their preparation process,a category of materials is commonly employed that do not possess piezoelectric properties themselves but play a crucial role in performance *** this review,the concept of auxiliary phase is first proposed to define these materials,aiming to provide a new perspective for designing high-performance *** different categories of modulation forms of auxiliary phase in piezocomposites are systematically summarized,including the modification of piezo-matrix,the modification of piezo-fillers,and the construction of special *** category emphasizes the role of the auxiliary phase and systematically discusses the latest advancements and the physical mechanisms of the auxiliary phase enhanced flexible ***,a summary and future outlook of piezocomposites based on the auxiliary phase are provided.

关键词： auxiliary phase flexibility microstructure piezocomposites piezoelectricity

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NH_(4)Cl-assisted preparation of single Ni sites anchored carbon nanosheet catalysts for highly efficient carbon dioxide electroreduction

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Journal of materials science & Technology 2023年第11期142卷 1-9页

作者： Dan Ping Feng Yi Guiwei Zhang Shide Wu Shaoming Fang Kailong Hu Ben Bin Xu Junna Ren Zhanhu Guo Henan Provincial Key Laboratory of Surface&Interface Science Henan Engineering Research Center of Chemical Engineering Separation Process IntensificationSchool of Material and Chemical EngineeringZhengzhou University of Light IndustryZhengzhou 450002China School of Materials Science and Engineering Harbin Institute of TechnologyShenzhen 518055China Mechanical and Construction Engineering Faculty of Engineering and EnvironmentNorthumbria UniversityNewcastle upon Tyne NE18STUK College of Materials Science and Engineering Taiyuan University of Science and TechnologyTaiyuan 030024China Department of Chemical&Biomolecular Engineering Integrated Composites Lab(ICL)University of TennesseeKnoxvilleTN 37996USA

Single-atomic transition metal-nitrogen codoped carbon(M-N-C)are efficient substitute catalysts for noble metals to catalyze the electrochemical CO_(2) reduction reaction(CO_(2)RR).However,the uncontrolled aggregations of metal and serious loss of nitrogen species constituting the M-N_(x) active sites are frequently observed in the commonly used pyrolysis ***,single-atomic nickel(Ni)-based sheet-like electrocatalysts with abundant Ni-N_(4) active sites were created by using a novel ammonium chloride(NH_(4)Cl)-assited pyrolysis *** aberration correction electron microscopy and X-ray absorption fine structure analysis clearly revealed that Ni species are atomically dispersed and anchored by N in Ni-N_(4) *** addition of NH_(4)Cl optimized the mesopore size to 7-10 nm and increased the concentrations of pyridinic N(3.54 wt%)and Ni-N_(4)(3.33 wt%)*** synergistic catalytic effect derived from Ni-N_(4) active sites and pyridinic N species achieved an outstanding CO_(2) RR performance,presenting a high CO Faradaic efficiency(FE_(CO))up to 98% and a large CO partial current density of 8.5 mA cm^(-2) at a low potential of-0.62 V ***,the FE_(CO) maintains above 80% within a large potential range from -0.43 to -0.73 V *** work provides a practical and feasible approach to building highly active single-atomic catalysts for CO_(2) conversion systems.

关键词： CO_(2)reduction Electrocatalyst Single-atomic ni NH_(4)Cl Pyridinic N

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