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A review on waste-based biochar adsorbent for adsorption process in Batik wastewater treatment

AIP Conference Proceedings 2023年第1期2580卷

作者： Elfi Yulia Estiyanti Ekawati Bambang Sunendar Purwasasmita Doctoral Program of Engineering Physics Faculty of Industrial Technology Institut Teknologi Bandung Indonesia 40116 Center for Instrumentation Technology and Automation Institut Teknologi Bandung Indonesia 40116 Engineering Physics Research Program Faculty of Industrial Technology Institut Teknologi Bandung Indonesia 40116 Advanced Material Processing Department of Engineering Physics Faculty of Industrial Technology Institut Teknologi Bandung Indonesia 40116

The adsorption process in the batik wastewater treatment that containing heavy metals is still quite challenging. Batik waste that exceeds the quality standard can cause environmental pollution and health problems. The green technology method to use waste to treat waste has also attracted tremendous attention to recent research that aims to produce adsorbents. It has a significant role in the adsorption process. Organic carbonaceous biochar is typically rich in carbon, highly porous structure, and charged surface. It makes this biochar highly potential for adsorbent application. The characteristics of biochar depend on the raw material and the manufacturing process. This review provides the latest studies and development of the adsorption process and biochar adsorbent in batik wastewater treatment applications. Also, it describes the challenges thoroughly. Hopefully, this review will provide new inspiration for advancing future studies in the adsorption process for batik wastewater treatment.

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Profile of bovine teeth potency as hydroxyapatite scaffold

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AIP Conference Proceedings 2023年第1期2536卷

作者： Endanus Harijanto Anita Yuliati Prihartini Widiyanti Dental Material Department Faculty of Dentistry Universitas Airlangga Surabaya Indonesia Biomedical Engineering Study Program Department of Physics Faculty of Science and Technology Universitas Airlangga Surabaya Indonesia

Background: Bone destructions in the oral cavity are due to trauma, chronic infection, congenital malformations, or resection surgery, most often by using an autologous bone graft technique. The problem using this technique are limited donors and suppliers, high cost, host potential imune response becauce accepts foreign bone tissue also potential transmission diseases. Another solution in tissue engineering techniques is using the scaffold. Hidroxyapatite is one of the osteoconductive potentialy ceramic materials in scaffold fabrication. Objective: To prove that bovine teeth hydroxyapatite have characteristic as scaffold for bone tissue regeneration. Methods: HA was obtained by calcining bovine teeth at 1000°C for 3 hours, Fourier Transform Infra Red Spectroscopy (FTIR) test , Energy Dispersive X-Ray (EDX) test and X-Ray Diffraction (XRD) test. Results: Bovine teeth hydroxyapatite to showed of hydroxyl, phosphate and carbonate functional groups (FTIR test). Average Ca/P=1.97. Conclusion: Hydroxyapatite from bovine teeth has potency as scaffold through the chemistry and physical characteristics.

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Synthesis, Characterization, and performance test of modified Zeolite-Si/Al nanocomposite from pumice and waste cans using slow pyrolysis process for removal pollutant parameters from hard water

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Environmental Nanotechnology, Monitoring and Management 2023年 20卷

作者： Gusti Wibowo, Yudha Sudibyo Rianjanu, Aditya Taher, Tarmizi Susanti, Noni Karo Karo, Pulung Suprihatin Iman Supriyatna, Yayat Prasetyo, Erik Bahfie, Fathan Amin, Muhammad Syarifuddin, Hutwan Safitri, Hana Khairurrijal, Khairurrijal Department of Mining Engineering Institut Teknologi Sumatera Lampung-35365 Indonesia Research Center for Mining Technology National Research and Innovation Agency Lampung Indonesia Department of Material Engineering Institut Teknologi Sumatera Lampung-35365 Indonesia Department of Environmental Engineering Institut Teknologi Sumatera Lampung-35365 Indonesia Physics Department Universitas Lampung Lampung Indonesia Department of Environmental Science Postgraduate Program Universitas Jambi Jambi 36122 Indonesia Laboratory of Mine Environmental Department of Mining Engineering Institut Teknologi Sumatera Lampung-35365 Indonesia Department of Physics Institut Teknologi Sumatera Lampung-36365 Indonesia Department of Physics Institut Teknologi Bandung Bandung 40132 Indonesia Center for Green and Sustainable Materials Institut Teknologi Sumatera Indonesia

Hard water is one of crucial problems in the world due to its pollutant parameters. Adsorption is a promising method for treating hard water because of its benefits such as low-cost, easy to use, acceptable, and easy to maintenance. In this study, we utilized zeolite functionalized with silicon/aluminum (Ze-Si/Al) as adsorbent materials for hard water treatment. Ten different ratios of Si/Al were added into zeolite by modifying the solid waste source concentration (pumice and cans). The optimum sample was then further tested with different parameters including contact time, dye concentration, and isotherm models. The zeolite-Si/Al adsorbent was characterized by Scanning Electron Microscope (SEM), X-Ray Diffraction (XRD), and X-Ray Fluorescence (XRF). Results of this study have showed that the best functionalized zeolite was that with Si/Al ratio 0.67, which has higher sorption ability. In contact time test, the equilibrium was reached after 300 min. This study also informed that the concentration of dyes will give impact on removal of pollutant parameters. Isotherm model of Ze-Si/Al fitted with Langmuir method. This study also discussed the potential development and future research direction. Thus, this study is a crucial report to develop the information about waste utilization as source of Si/Al to increasing quality of zeolite. © 2023 Elsevier B.V.

关键词： Adsorption Hard water Wastewater Wastewater treatment zeolite-Si/Al

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Effects of chain-chain interaction on the configuration of short-chain alkanethiol self-assembled monolayers on a metal surface

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Journal of Chemical physics 2024年第21期160卷 214711-214711页

作者： Liao, Chia-Li Faizanuddin, Syed Mohammed Haruyama, Jun Liao, Wei-Ssu Wen, Yu-Chieh Department of Chemistry National Taiwan University Taipei 10617 Taiwan Institute of Physics Academia Sinica Taipei 11529 Taiwan Taiwan International Graduate Program Academia Sinica Taipei 11529 Taiwan Department of Engineering and System Science National Tsing Hua University Hsinchu 300044 Taiwan Solid State Chemistry Laboratory Cluster for Pioneering Research RIKEN Wako 351-0198 Japan Center for Emerging Material and Advanced Devices National Taiwan University Taipei 10617 Taiwan

Surface-specific sum frequency generation vibrational spectroscopy is applied to study the molecular configuration of short-chain n-alkanethiol self-assembled monolayers (SAMs with n = 2-6) on the Au surface. For monolayers with n ≥ 3, the alkanethiols are upright-oriented, with the CH₃ tilt angle varying between ∼33° and ∼46° in clear even-odd dependency. The ethanethiol monolayer (n = 2) is, however, found to exhibit a distinct lying-down configuration with a larger methyl tilt angle (67°-79°) and a smaller CH₂ tilt angle (56°-68°). Such a unique configurational transition from n = 2 to n ≥ 3 discloses the steric effect owing to chain-chain interaction among neighboring molecules. Through density functional theory calculations, the transition is further confirmed to be energetically favorable for thiols on a defective reconstructed Au(111) surface but not on the pristine one. Our study highlights the roles of the chain-chain interaction and the substrate surface atomic structure when organizing SAMs, offering a strategic pathway for exploiting their applications. © 2024 Author(s).

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Technology Roadmap for Flexible Sensors

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ACS NANO 2023年第6期17卷 5211-5295页

作者： Luo, Yifei Abidian, Mohammad Reza Ahn, Jong-Hyun Akinwande, Deji Andrews, Anne M. Antonietti, Markus Bao, Zhenan Berggren, Magnus Berkey, Christopher A. Bettinger, Christopher John Chen, Jun Chen, Peng Cheng, Wenlong Cheng, Xu Choi, Seon-Jin Chortos, Alex Dagdeviren, Canan Dauskardt, Reinhold H. Di, Chong-an Dickey, Michael D. Duan, Xiangfeng Facchetti, Antonio Fan, Zhiyong Fang, Yin Feng, Jianyou Feng, Xue Gao, Huajian Gao, Wei Gong, Xiwen Guo, Chuan Fei Guo, Xiaojun Hartel, Martin C. He, Zihan Ho, John S. Hu, Youfan Huang, Qiyao Huang, Yu Huo, Fengwei Hussain, Muhammad M. Javey, Ali Jeong, Unyong Jiang, Chen Jiang, Xingyu Kang, Jiheong Karnaushenko, Daniil Khademhosseini, Ali Kim, Dae-Hyeong Kim, Il-Doo Kireev, Dmitry Kong, Lingxuan Lee, Chengkuo Lee, Nae-Eung Lee, Pooi See Lee, Tae-Woo Li, Fengyu Li, Jinxing Liang, Cuiyuan Lim, Chwee Teck Lin, Yuanjing Lipomi, Darren J. Liu, Jia Liu, Kai Liu, Nan Liu, Ren Liu, Yuxin Liu, Yuxuan Liu, Zhiyuan Liu, Zhuangjian Loh, Xian Jun Lu, Nanshu Lv, Zhisheng Magdassi, Shlomo Malliaras, George G. Matsuhisa, Naoji Nathan, Arokia Niu, Simiao Pan, Jieming Pang, Changhyun Pei, Qibing Peng, Huisheng Qi, Dianpeng Ren, Huaying Rogers, John A. Rowe, Aaron Schmidt, Oliver G. Sekitani, Tsuyoshi Seo, Dae-Gyo Shen, Guozhen Sheng, Xing Shi, Qiongfeng Someya, Takao Song, Yanlin Stavrinidou, Eleni Su, Meng Sun, Xuemei Takei, Kuniharu Tao, Xiao-Ming Tee, Benjamin C. K. Thean, Aaron Voon-Yew Trung, Tran Quang Wan, Changjin Wang, Huiliang Wang, Joseph Wang, Ming Wang, Sihong Wang, Ting Wang, Zhong Lin Weiss, Paul S. Wen, Hanqi Xu, Sheng Xu, Tailin Yan, Hongping Yan, Xuzhou Yang, Hui Yang, Le Yang, Shuaijian Yin, Lan Yu, Cunjiang Yu, Guihua Yu, Jing Yu, Shu-Hong Yu, Xinge Zamburg, Evgeny Zhang, Haixia Zhang, Xiangyu Zhang, Xiaosheng Zhang, Xueji Zhang, Yihui Zhang, Yu Zhao, Siyuan Zhao, Xuanhe Zheng, Yuanjin Zheng, Yu-Qing Zheng, Zijian Zhou, Tao Zhu, Bowen Zhu, Ming Zhu, Rong Zhu, Yangzhi Zhu, Yong Zou, Guijin Chen, Xiaodong 08-03 Innovis Singapore 138634 Republic of Singapore Innovative Centre for Flexible Devices (iFLEX) School of Materials Science and Engineering Nanyang Technological University Singapore 639798 Singapore Department of Biomedical Engineering University of Houston Houston Texas 77024 United States School of Electrical and Electronic Engineering Yonsei University Seoul 03722 Republic of Korea Department of Electrical and Computer Engineering The University of Texas at Austin Austin Texas 78712 United States Microelectronics Research Center The University of Texas at Austin Austin Texas 78758 United States Department of Chemistry and Biochemistry California NanoSystems Institute and Department of Psychiatry and Biobehavioral Sciences Semel Institute for Neuroscience and Human Behavior and Hatos Center for Neuropharmacology University of California Los Angeles Los Angeles California 90095 United States Colloid Chemistry Department Max Planck Institute of Colloids and Interfaces 14476 Potsdam Germany Department of Chemical Engineering Stanford University Stanford California 94305 United States Laboratory of Organic Electronics Department of Science and Technology Campus Norrköping Linköping University 83 Linköping Sweden Wallenberg Initiative Materials Science for Sustainability (WISE) and Wallenberg Wood Science Center (WWSC) SE-100 44 Stockholm Sweden Department of Materials Science and Engineering Stanford University Stanford California 94301 United States Department of Biomedical Engineering and Department of Materials Science and Engineering Carnegie Mellon University Pittsburgh Pennsylvania 15213 United States Department of Bioengineering University of California Los Angeles Los Angeles California 90095 United States School of Chemistry Chemical Engineering and Biotechnology Nanyang Technological University Singapore 637457 Singapore Nanobionics Group Department of Chemical and Biological Engineering Monash University Clayton Australia 3800 Monash

Humans rely increasingly on sensors to address grand challenges and to improve quality of life in the era of digitalization and big data. For ubiquitous sensing, flexible sensors are developed to overcome the limitations of conventional rigid counterparts. Despite rapid advancement in bench-side research over the last decade, the market adoption of flexible sensors remains limited. To ease and to expedite their deployment, here, we identify bottlenecks hindering the maturation of flexible sensors and propose promising solutions. We first analyze continued...challenges in achieving satisfactory sensing performance for real-world applications and then summarize issues in compatible sensor-biology interfaces, followed by brief discussions on powering and connecting sensor networks. Issues en route to commercialization and for sustainable growth of the sector are also analyzed, highlighting environmental concerns and emphasizing nontechnical issues such as business, regulatory, and ethical considerations. Additionally, we look at future intelligent flexible sensors. In proposing a comprehensive roadmap, we hope to steer research efforts towards common goals and to guide coordinated development strategies from disparate communities. Through such collaborative

关键词： soft materials mechanics engineering flexible electronics conformable sensors bioelectronics human-machine interfaces body area sensor networks technology translation sustainable electronics

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A three-stage magnetic phase transition revealed in ultrahigh-quality van der Waals magnet CrSBr

arXiv

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arXiv 2022年

作者： Liu, Wenhao Guo, Xiaoyu Schwartz, Jonathan Xie, Hongchao Dhale, Nikhil Sung, Suk Hyun Kondusamy, Aswin L.N. Wang, Xiqu Zhao, Haonan Berman, Diana Hovden, Robert Zhao, Liuyan Lv, Bing Department of Physics The University of Texas at Dallas RichardsonTX75080 United States Department of Physics University of Michigan Ann ArborMI48109 United States Department of Material Science and Engineering University of Michigan Ann ArborMI48109 United States Department of Chemistry University of Houston HoustonTX77004 United States Department of Materials Science and Engineering University of North Texas DentonTX76203 United States Applied Physics Program University of Michigan Ann ArborMI48109 United States Department of Materials Science & Engineering The University of Texas at Dallas RichardsonTX75080 United States

van der Waals (vdW) magnets are receiving ever-growing attention nowadays due to their significance in both fundamental research on low-dimensional magnetism and potential applications in spintronic devices. High crystalline quality of vdW magnets is key for maintaining intrinsic magnetic and electronic properties, especially when exfoliated down to the 2D limit. Here, ultrahigh-quality air-stable vdW CrSBr crystals are synthesized using the direct vapor-solid synthesis method. The high single crystallinity and spatial homogeneity have been thoroughly evidenced at length scales from sub-mm to atomic resolution by X-ray diffraction, second harmonic generation, and scanning transmission electron microscopy. More importantly, specific heat measurements of these ultrahigh quality CrSBr crystals show three thermodynamic anomalies at 185K, 156K, and 132K, revealing a stage-by-stage development of the magnetic order upon cooling, which is also corroborated with the magnetization and transport results. Our ultrahigh-quality CrSBr can further be exfoliated down to monolayers and bilayers easily, paving the way to integrate them into heterostructures for spintronic and magneto-optoelectronic applications. Copyright © 2022, The Authors. All rights reserved.

关键词： Magnetism

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Simulation-trained machine learning models for Lorentz transmission electron microscopy

APL Machine Learning

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APL Machine Learning 2024年第2期2卷

作者： Arthur R. C. McCray Alec Bender Amanda Petford-Long Charudatta Phatak Material Science Division Argonne National Laboratory Lemont Illinois 60439 USA Applied Physics Program Northwestern University Evanston Illinois 60208 USA Department of Materials Science and Engineering Northwestern University Evanston Illinois 60208 USA

Understanding the collective behavior of complex spin textures, such as lattices of magnetic skyrmions, is of fundamental importance for exploring and controlling the emergent ordering of these spin textures and inducing phase transitions. It is also critical to understand the skyrmion–skyrmion interactions for applications such as magnetic skyrmion-enabled reservoir or neuromorphic computing. Magnetic skyrmion lattices can be studied using in situ Lorentz transmission electron microscopy (LTEM), but quantitative and statistically robust analysis of the skyrmion lattices from LTEM images can be difficult. In this work, we show that a convolutional neural network, trained on simulated data, can be applied to perform segmentation of spin textures and to extract quantitative data, such as spin texture size and location, from experimental LTEM images, which cannot be obtained manually. This includes quantitative information about skyrmion size, position, and shape, which can, in turn, be used to calculate skyrmion–skyrmion interactions and lattice ordering. We apply this approach to segmenting images of Néel skyrmion lattices so that we can accurately identify skyrmion size and deformation in both dense and sparse lattices. The model is trained using a large set of micromagnetic simulations as well as simulated LTEM images. This entirely open-source training pipeline can be applied to a wide variety of magnetic features and materials, enabling large-scale statistical studies of spin textures using LTEM.

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Direct writing of PVBVA/Ti3C2 Tx (MXene) triboelectric nanogenerators for energy harvesting and sensing applications

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Nano Energy 2025年 142卷

作者： Pratap, Ajay Rajabi Kouchi, Fereshteh Burgoyne, Hailey Curtis, Michael Rektor, Attila Seol, Myeong-Lok Mansoor, Naqsh E. Varghese, Tony Valayil Eixenberger, Josh Efaw, Corey M. Zuzelski, Matt Little, Isaac Fujimoto, Kiyo Deng, Zhangxian Shuck, Christopher E. Koehne, Jessica E. Estrada, David Micron School of Material Science and Engineering Boise State University BoiseID83725 United States Biomolecular Sciences Graduate Program Boise State University BoiseID83725 United States NASA Ames Research Center Universities Space Research Association Moffett Field CA94035 United States Department of Physics Boise State University BoiseID83725 United States Center for Advanced Energy Studies Boise State University BoiseID83725 United States Department of Mechanical and Biomedical Engineering Boise State University BoiseID83725 United States Idaho National Laboratory Idaho FallsID83415 United States A.J. Drexel Nanomaterials Institute and Department of Materials Science and Engineering Drexel University PhiladelphiaPA19104 United States Department of Chemistry and Chemical Biology Rutgers University PiscatawayNJ08854 United States

Triboelectric nanogenerators (TENGs) have gained recognition for their potential to convert mechanical energy into electrical energy, making them attractive for applications in healthcare, robotics, and human-device interfaces. However, many TENG devices rely on fluorinated polymers for high charge generation and involve complex fabrication processes, which limit their practicality and environmental sustainability. Here, we developed an eco-friendly composite of poly (vinyl butyral-co-vinyl alcohol-co-vinyl acetate) (PVBVA) and Ti₃C₂Tₓ MXene for extrusion printing onto aluminum foil substrates, enabling the additive manufacturing of TENGs. Experimental results indicate that integrating 5.5 mg mL-1 of MXene (P-MX 5.5) into PVBVA resulted in a power density of 760 mW·m⁻², with simultaneous improvements in open-circuit voltage (129 %) and short-circuit current (250 %), demonstrating enhanced charge transfer efficiency. Beyond aluminum foil-based devices, we further explored the fully printed P-MX 5.5 TENG by utilizing silver ink electrodes, eliminating the need for aluminum foil. This fully printed, flexible TENG was successfully used for real-time human motion sensing, demonstrating its ability to detect activities such as walking, running, knee bending, and jumping. Collectively, our additively manufactured and sustainable PVBVA-MXene TENG composites, including both aluminum-based and fully printed versions, show promise for future energy harvesters, sensors, wearable electronics, healthcare, and robotic applications. © 2025

关键词： Aluminum foil

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Two-step electronic response to magnetic ordering in a van der Waals ferromagnet

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Physical Review B 2024年第4期109卷 045416-045416页

作者： Han Wu Jian-Xin Zhu Lebing Chen Matthew W. Butcher Ziqin Yue Dongsheng Yuan Yu He Ji Seop Oh Bin Gao Jianwei Huang Shan Wu Cheng Gong Yucheng Guo Sung-Kwan Mo Jonathan Denlinger Donghui Lu Makoto Hashimoto Matthew B. Stone Alexander I. Kolesnikov Songxue Chi Junichiro Kono Andriy H. Nevidomskyy Robert J. Birgeneau Pengcheng Dai Ming Yi Department of Physics and Astronomy and Rice Center for Quantum Materials Rice University Houston Texas 77005 USA Theoretical Division Los Alamos National Laboratory Los Alamos New Mexico 87545 USA Center for Integrated Nanotechnologies Los Alamos National Laboratory Los Alamos New Mexico 87545 USA Department of Physics University of California at Berkeley Berkeley California 94720 USA Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston Texas 77005 USA Materials Sciences Division Lawrence Berkeley National Laboratory Berkeley California 94720 USA National Institute for Materials Science 1-1 Namiki Tsukuba Ibaraki 305-0044 Japan Department of Applied Physics Yale University New Haven Connecticut 06511 USA Department of Electrical and Computer Engineering and Quantum Technology Center University of Maryland College Park Maryland 20742 USA Advanced Light Source Lawrence Berkeley National Laboratory Berkeley California 94720 USA Stanford Synchrotron Radiation Lightsource SLAC National Accelerator Laboratory Menlo Park California 94025 USA Neutron Scattering Division Oak Ridge National Laboratory Oak Ridge Tennessee 37831 USA Department of Electrical and Computer Engineering Rice University Houston Texas 77005 USA Smalley-Curl Institute Rice University Houston Texas 77005 USA Department of Material Science and Nanoengineering Rice University Houston Texas 77005 USA Department of Materials Science and Engineering University of California Berkeley California 94720 USA

The two-dimensional material Cr2Ge2Te6 is a member of the class of insulating van der Waals (vdW) magnets. Here, using high resolution angle-resolved photoemission spectroscopy in a detailed temperature dependence study, we identify a clear response of the electronic structure to a dimensional crossover in the form of two distinct temperature scales marking onsets of modifications in the electronic structure. Specifically, we observe Te p-orbital-dominated bands to undergo changes at the Curie transition temperature TC while the Cr d-orbital-dominated bands begin evolving at a higher temperature scale. Combined with neutron scattering, density functional theory calculations, and Monte Carlo simulations, we find that the electronic system can be consistently understood to respond sequentially to the distinct temperatures at which in-plane and out-of-plane spin correlations exceed a characteristic length scale. Our findings reveal the sensitivity of the orbital-selective electronic structure for probing the dynamical evolution of local moment correlations in vdW insulating magnets.

关键词： Electronic structure Magnetic order Magnetic phase transitions Van der Waals systems Angle-resolved photoemission spectroscopy

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Response to Comment on (Novel two-dimensional porous graphitic carbon nitride C6N7 monolayer: A First-principle calculations [Appl. Phys. Lett. 2021, 119, 142102])

arXiv

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arXiv 2022年

作者： Bafekry, Asadollah Faraji, Mehrdad Fadlallah, Mohamed M. Sarsari, I. Abdolhosseini Jappor, Hamad R. Fazeli, Sara Ghergherehchi, Mitra Department of Radiation Application Shahid Beheshti University Tehran Iran Micro and Nanotechnology Graduate Program TOBB University of Economics and Technology Sogutozu Caddesi No 43 Sogutozu Ankara06560 Turkey Department of Physics Faculty of Science Benha University Benha13518 Egypt Department of Physics Isfahan University of Technology Isfahan84156-83111 Iran Department of Physics College of Education for Pure Sciences University of Babylon Hilla Iraq Department of Material Science and Engineering Sharif University of Technology PO Box 11155-9466 Tehran Iran Department of Electrical and Computer Engineering Sungkyunkwan University Suwon16419 Korea Republic of

Recently, reported a comments on the our paper [Appl. Phys. Lett. 119, 142102(2021)]. With our response, the APL journal rejected their non scientificcomments. There are some ambiguities about their claim: 1-They can check thephonon dispersion of their structure to see ZA out-of-plane mode. 2-They reportthe uniaxial stress-strain responses in Fig 2., which is unrelated to ourpaper. For a more helpful understanding of the mechanical properties of thenovel C6N7 monolayer, they can publish a paper. 3-They mentioned: Using the DFTmethod and with assuming a thickness of 3.35 A for the C6N7 monolayer based ongraphene thickness. Why did they choose this thickness while we know our C6N7monolayer is at without buckling? The distance of ZA out-of-plane movement ofions in C6N7 is different from Graphene. © 2022, CC BY.

关键词： Monolayers

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