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arXiv 2020年

作者： Jiménez-Ángeles, Felipe Harmon, Katherine Nguyen, Trung Dac Fenter, Paul de la Cruz, Monica Olvera Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States Applied Physics Graduate Program Northwestern University EvanstonIL60208 United States Department of Chemical and Biological Engineering Northwestern University EvanstonIL60208 United States Chemical Sciences and Engineering Division Argonne National Laboratory LemontIL60439 United States Department of Physics and Astronomy Northwestern University EvanstonIL60208 United States Department of Chemistry Northwestern University EvanstonIL60208 United States

Water mediates electrostatic interactions via the orientation of its dipoles around ions, molecules, and interfaces. This induced water polarization consequently influences multiple phenomena. In particular, water polarization modulated by nanoconfinement affects ion adsorption and transport, biomolecular self-assembly, and surface chemical reactions. Therefore, it is of paramount importance to understand how water-mediated interactions change at the nanoscale. Here we show that near the graphene surface anion-cation interactions do not obey the translational and isotropic symmetries of Coulomb’s law. We identify a new property, referred to as non-reciprocity, which describes the non-equivalent and directional interaction between two oppositely charged ions near the confining surface when their positions with respect to the interface are exchanged. Specifically, upon exchange of the two ions’ positions along the surface normal direction the interaction energy changes by about 5kBT. In both cases, confinement enhances the attraction between two oppositely charged ions near the graphene surface, while intercalation of one ion into the graphene layers shifts the interaction to repulsive. While the water permittivity in confinement is different from that in bulk, the effects observed here via molecular dynamics simulations and X-ray reflectivity experiments cannot be accounted for by current permittivity models. Our work shows that the water structure is not enough to infer electrostatic interactions near interfaces. Copyright © 2020, The Authors. All rights reserved.

关键词： Ions

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Thermal valorisation extracts of selected agro-waste for human pathogen antibacterial NiO nanoparticles synthesis

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materials Today: Proceedings 2021年 36卷 559-565页

作者： L.C. Razanamahandry A.C. Nwanya A.K.H. Bashir C.M. Furqan J. Sackey A.E. Ameh G. Kavitha E. Manikandan S.K.O. Ntwampe E. Fosso-Kankeu F. Ezema M. Maaza UNESCO-UNISA Africa Chair in Nanoscience’s/Nanotechnology Laboratories (U2AC2N) College of Graduate Studies University of South Africa (UNISA) Muckleneuk Ridge P O Box 392 Pretoria South Africa Nanosciences African NETWORK (NANOAFNET) Materials Research Department (MRD) iThemba LABS-National Research Foundation (NRF) 1 Old Faure Road 7129 P O Box722 Somerset West Western Cape Province South Africa Department of Physics and Astronomy University of Nigeria Nsukka Enugu State Nigeria Preston Institute of Nano Science and Technology (PINSAT) Preston University Kohat Islamabad Campus Pakistan Enivronmental and Nano Science Research Group Department of Chemistry University of the Western Cape Bellville 7535 Cape Town South Africa Post Graduate (P.G.) & Research Dept. of Physics A M Jain College Meenembakkam-600114 University of Madras Chennai India Department of Physics TUCAS Campus Thennangur-604408 Thiruvalluvar University Vellore India Bioresource Engineering Research Group (BioERG) Cape Peninsula University of Technology P.O. Box 652 Cape Town 8000 South Africa Department of Chemical Engineering Faculty of Engineering and the Built EnvironmentCape Peninsula University of Technology PO Box 1906 Bellville 7535 Cape Town South Africa Water Pollution Monitoring and Remediation Initiatives Research Group School of Chemical and Minerals Engineering North-West University Private Bag X1290 Potchefstroom 2520 South Africa

Waste management stays a challenge in developing countries. This research reports on the valorisation of agro-waste for the synthesis of nickel oxide nanoparticles (NiO NPs), useful as antibacterial agents to assure the sustainable use of renewable waste resources for human health protection. Agro-waste extracts from Persea americana seed, Zea mays silk and Eucalyptus globulus leaves were used as chelating agents in combination with nickel nitrate to synthesis NiO NPs. Optical, physical and chemical characteristics of synthesised NiO NPs were analysed by Ultraviolet spectroscopy studies (UV–VIS analysis), X-ray powder diffraction (XRD) and Scanning Electron Microscopy (SEM); Fourier Transform Infrared analysis (FTIR) and Energy Dispersive X-Ray Spectroscopy (EDS), respectively. Antibacterial activity of each synthesised NiO-NPs was determined by cell culture in nutrient agar using well diffusion method. The UV–VIS results showed the formation of NiO NPs at wavelength range 300 – 400 nm. The XRD patterns demonstrated the crystalline form of the NiO NPs with a lattice face-centered cubic with average size of 14, 18 and 19 nm for NiO NPs from Persea americana seed, Zea mays silk and Eucalyptus globulus leaves, respectively. SEM images revealed the spherical, pleomorphism and nanosheet surface shape of the synthesised NiO NPs. Chemical elements K, P, Mg, Na, C and O were detected by EDS analysis as forming part of the elemental composition of the NiO NPs synthesised. Chemical bending between O–H, C–H, C–C and C-N was observed using FTIR. Furthermore, antibacterial studies showed the efficacy of all the NiO NPs synthesised against pathogen microbial growth with the largest inhibition zone (IZ) of 26 mm for the NiO NPs from Eucalyptus globulus leaves being observed. Therefore, Eucalyptus globulus leaves are recommended to synthesise NiO NPs for antibacterial applications.

关键词： Antibacterial Eucalyptus globulus Green nanomaterials NiO Persea americana Zea mays

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Developing self-adaptive microservice systems: Challenges and directions

arXiv

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arXiv 2019年

作者： Mendonça, Nabor C. Jamshidi, Pooyan Garlan, David Pahl, Claus Post Graduate Program in Applied Informatics University of Fortaleza FortalezaCE Brazil Computer Science and Engineering Department University of South Carolina ColumbiaSC United States School of Computer Science Carnegie Mellon University PittsburghPA United States Faculty of Computer Science Free University of Bozen-Bolzano Bozen-Bolzano Italy

A self-adaptive system can dynamically monitor and adapt its behavior to preserve or enhance its quality attributes under uncertain operating conditions. This article identifies key challenges for the development of microservice applications as self-adaptive systems, using a cloud-based intelligent video surveillance application as a motivating example. It also suggests potential new directions for addressing most of the identified challenges by leveraging existing microservice practices and technologies. Copyright © 2019, The Authors. All rights reserved.

关键词： Adaptive systems

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Phase transitions in the frustrated Ising ladder with stoquastic and nonstoquastic catalysts

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Physical Review Research 2021年第4期3卷 043013-043013页

作者： Kabuki Takada Shigetoshi Sota Seiji Yunoki Bibek Pokharel Hidetoshi Nishimori Daniel A. Lidar Department of Physics Tokyo Institute of Technology Yokohama Kanagawa 226-8503 Japan Computational Materials Science Research Team RIKEN Center for Computational Science (R-CCS) Kobe Hyogo 650-0047 Japan Computational Condensed Matter Physics Laboratory RIKEN Cluster for Pioneering Research (CPR) Wako Saitama 351-0198 Japan Computational Quantum Matter Research Team RIKEN Center for Emergent Matter Science (CEMS) Wako Saitama 351-0198 Japan Department of Physics University of Southern California Los Angeles California 90089 USA Center for Quantum Information Science & Technology University of Southern California Los Angeles California 90089 USA Institute of Innovative Research Tokyo Institute of Technology Yokohama Kanagawa 226-8503 Japan Graduate School of Information Sciences Tohoku University Sendai Miyagi 980-8579 Japan RIKEN Interdisciplinary Theoretical and Mathematical Sciences Program (iTHEMS) Wako Saitama 351-0198 Japan Department of Electrical & Computer Engineering and Department of Chemistry University of Southern California Los Angeles California 90089 USA

The role of nonstoquasticity in the field of quantum annealing and adiabatic quantum computing is an actively debated topic. We study a strongly-frustrated quasi-one-dimensional quantum Ising model on a two-leg ladder to elucidate how a first-order phase transition with a topological origin is affected by interactions of the ±XX-type. Such interactions are sometimes known as stoquastic (negative sign) and nonstoquastic (positive sign) “catalysts”. Carrying out a symmetry-preserving real-space renormalization group analysis and extensive density-matrix renormalization group computations, we show that the phase diagrams obtained by these two methods are in qualitative agreement with each other and reveal that the first-order quantum phase transition of a topological nature remains stable against the introduction of both XX-type catalysts. This is the first study of the effects of nonstoquasticity on a first-order phase transition between topologically distinct phases. Our results indicate that nonstoquastic catalysts are generally insufficient for removing topological obstacles in quantum annealing and adiabatic quantum computing.

关键词： Adiabatic quantum optimization Phase transitions by order Quantum spin models Density matrix renormalization group Renormalization group

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Serial stimuli-responsive theranostic nanomaterials for cancer therapy and imaging

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Coordination Chemistry Reviews 2025年 542卷

作者： Malairaj Sathuvan Karthikeyan Narayanan Hyunsik Hong Raju Vivek Saiyi Zhong Kit-Leong Cheong Juyoung Yoon Guosheng Song Heemin Kang Ramar Thangam Centre for Advanced Studies in Botany University of Madras Guindy Campus Chennai 600 025 Tamilnadu India Center for Biotechnology and Interdisciplinary Studies Rensselaer Polytechnic Institute Troy New York 12180 United States Department of Materials Science and Engineering Korea University Seoul 02841 Republic of Korea Bio-Nano Theranostics Research Laboratory Department of Zoology Bharathiar University Coimbatore 641 046 Tamil Nadu India Guangdong Provincial Key Laboratory of Aquatic Product Processing and Safety College of Food Science and Technology Guangdong Ocean University Zhanjiang 524088 China Department of Biology College of Science Shantou University Shantou 515063 Guangdong China Department of Chemistry and Nanoscience Ewha Womans University Seoul 03760 Republic of Korea Graduate Program in Innovative Biomaterials Convergence Ewha Womans University Seoul 03760 Republic of Korea State Key Laboratory of Chemo/Biosensing and Chemometrics College of Chemistry and Chemical Engineering Hunan University Changsha 410082 China College of Medicine Korea University Seoul 02841 Republic of Korea

Traditional cancer drug therapies face major challenges, including high recurrence rates, systemic toxicity, and drug resistance. Serial stimuli-responsive (SSR) nanomaterials offer substantial advantages over single-stimulus systems for diagnosis and treatment by facilitating precise, adaptable, and effective drug delivery and triggering multiple disease site-specific on-demand responses tailored for personalized treatment of heterogeneous dynamic tumors under real-time monitoring. In this review, we highlight the transformative role of SSR nanomaterials with theranostic abilities. We explore SSR-associated innovative drug delivery systems based on smart nanomaterials, such as liposomes, dendrimers, polymeric nanoparticles, and micelles, which can be serially activated by endogenous stimuli, such as the pH and enzymes, or exogenous stimuli, such as heat, light, a magnetic field, and ultrasound. To our knowledge, this review is the first to discuss the design of smart nanomaterials for SSR multimodal cancer theranostics. We emphasize the emerging field of imaging-guided therapy, wherein theranostic agents facilitate the real-time monitoring of drug pharmacokinetics and therapeutic responses, allowing for the development of personalized treatment strategies targeting different tumor sites. Finally, we anticipate the role of SSR nanomaterials in transforming cancer-theranostic modalities for more effective and personalized therapies.

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Tunneling spectroscopy of c-axis epitaxial cuprate junctions

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Physical Review B 2020年第22期101卷 224512-224512页

作者： Panpan Zhou Liyang Chen Ilya Sochnikov Tsz Chun Wu Matthew S. Foster Anthony T. Bollinger Xi He Ivan Božović Douglas Natelson Department of Physics and Astronomy Rice University Houston Texas 77005 USA Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston Texas 77005 USA Department of Physics University of Connecticut Storrs Connecticut 06269 USA Brookhaven National Laboratory Upton New York 11973–5000 USA Department of Chemistry Yale University New Haven Connecticut 06520 USA Department of Electrical and Computer Engineering Rice University Houston Texas 77005 USA Department of Materials Science and NanoEngineering Rice University Houston Texas 77005 USA

Atomically precise epitaxial structures are unique systems for tunneling spectroscopy that minimize extrinsic effects of disorder. We present a systematic tunneling spectroscopy study, over a broad doping, temperature, and bias range, in epitaxial c-axis La2−xSrxCuO4/La2CuO4/La2−xSrxCuO4 heterostructures. The behavior of these superconductor/insulator/superconductor (SIS) devices is unusual. Down to 20 mK there is complete suppression of c-axis Josephson critical current with a barrier of only 2 nm of La2CuO4, and the zero-bias conductance remains at 20–30% of the normal-state conductance, implying a substantial population of in-gap states. Tunneling spectra show greatly suppressed coherence peaks. As the temperature is raised, the superconducting gap fills in rather than closing at Tc. For all doping levels, the spectra show an inelastic tunneling feature at ∼80 meV, suppressed as T exceeds Tc. These nominally simple epitaxial cuprate junctions deviate markedly from expectations based on the standard Bardeen-Cooper-Schrieffer theory.

关键词： Coherence length Impurities in superconductors Josephson effect Quasiparticles & collective excitations Superconducting gap Superconducting phase transition d-wave Cuprates Heterostructures High-temperature superconductors Multilayer thin films Scanning tunneling spectroscopy

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A Dual-Responsive Liquid Crystal Elastomer for Multi-Level Encryption and Transient Information Display

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Angewandte Chemie 2023年第48期135卷

作者： Hong-Qin Wang Yuqi Tang Zi-Yang Huang Fang-Zhou Wang Peng-Fei Qiu Xinfang Zhang Prof. Cheng-Hui Li Prof. Quan Li State Key Laboratory of Coordination Chemistry School of Chemistry and Chemical Engineering Collaborative Innovation Center of Advanced Microstructures Nanjing University 210023 Nanjing China Contribution: Investigation (lead) Writing - original draft (lead) Writing - review & editing (supporting) Institute of Advanced Materials and School of Chemistry and Chemical Engineering Southeast University 211189 Nanjing China Contribution: Investigation (supporting) Writing - original draft (supporting) Writing - review & editing (supporting) Materials Science Graduate Program Kent State University 44242 Kent Ohio USA Contribution: Conceptualization (equal) Funding acquisition (equal) Investigation (supporting) Project administration (lead) Writing - original draft (supporting) Writing - review & editing (equal) Contribution: Conceptualization (equal) Funding acquisition (equal) Investigation (supporting) Supervision (lead) Writing - original draft (supporting) Writing - review & editing (equal)

Information security has gained increasing attention in the past decade, leading to the development of advanced materials for anti-counterfeiting, encryption and instantaneous information display. However, it remains challenging to achieve high information security with simple encryption procedures and low-energy stimuli. Herein, a series of strain/temperature-responsive liquid crystal elastomers (LCEs) are developed to achieve dual-modal, multi-level information encryption and real-time, rewritable transient information display. The as-prepared polydomain LCEs can change from an opaque state to a transparent state under strain or temperature stimuli, with the transition strains or temperatures highly dependent on the concentration of long-chain flexible spacers. Information encrypted by different LCE inks can be decrypted under specific strains or temperatures, leading to multi-level protection of information security. Furthermore, with the combination of the phase transition of polydomain LCEs and the photothermal effect of multi-walled carbon nanotubes (MWCNTs), we achieved a repeatable transient information display by using near-infrared (NIR) light as a pen for writing. This study provides new insight into the development of advanced encryption materials with versatility and high security for broad applications.

关键词： Dual-Responsive Information Display Liquid Crystal Elastomer Multi-Level Encryption Transparency Transition

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Retraction notice to "Pyrolysis: An effective technique for degradation of COVID-19 medical wastes" [Chemosphere 275 (2021) 130092]

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Chemosphere 2025年 370卷 143824页

作者： Selvakumar Dharmaraj Veeramuthu Ashokkumar Rajesh Pandiyan Heli Siti Halimatul Munawaroh Kit Wayne Chew Wei-Hsin Chen Chawalit Ngamcharussrivichai (Deemed to be University) Chennai 603112 Tamil Nadu India. Center of Excellence in Catalysis for Bioenergy and Renewable Chemicals (CBRC) Faculty of Science Chulalongkorn University Bangkok 10330 Thailand. Department of Biochemistry Karpagam Academy of Higher Education (formerly Karpagam University) Pollachi Main Road Eachanari Post Coimbatore Tamil Nadu India. Chemistry Study Program Department of Chemistry Education Faculty of Mathematics and Science Education Universitas Pendidikan Indonesia Jl. Dr. Setiabudhi 229 Bandung 40154 Indonesia. School of Energy and Chemical Engineering Xiamen University Malaysia Jalan Sunsuria Bandar Sunsuria 43900 Sepang Selangor Malaysia College of Chemistry and Chemical Engineering Xiamen University Xiamen 361005 Fujian China. Department of Aeronautics and Astronautics National Cheng Kung University Tainan 701 Taiwan Research Center for Smart Sustainable Circular Economy Tunghai University Taichung 407 Taiwan Department of Mechanical Engineering National Chin-Yi University of Technology Taichung 411 Taiwan. Center of Excellence in Catalysis for Bioenergy and Renewable Chemicals (CBRC) Faculty of Science Chulalongkorn University Bangkok 10330 Thailand Center of Excellence on Petrochemical and Materials Technology (PETROMAT) Chulalongkorn University Pathumwan Bangkok 10330 Thailand.

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EMPRESS. IX. Extremely Metal-Poor Galaxies are Very Gas-Rich Dispersion-Dominated Systems: Will JWST Witness Gaseous Turbulent High-z Primordial Galaxies?

arXiv

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arXiv 2022年

作者： Isobe, Yuki Ouchi, Masami Nakajima, Kimihiko Ozaki, Shinobu Bouché, Nicolas F. Wise, John H. Xu, Yi Emsellem, Eric Kusakabe, Haruka Hattori, Takashi Nagao, Tohru Chiaki, Gen Fukushima, Hajime Harikane, Yuichi Hayashi, Kohei Hirai, Yutaka Kim, Ji Hoon Maseda, Michael V. Nagamine, Kentaro Shibuya, Takatoshi Sugahara, Yuma Yajima, Hidenobu Aoyama, Shohei Fujimoto, Seiji Fukushima, Keita Hatano, Shun Inoue, Akio K. Ishigaki, Tsuyoshi Kawasaki, Masahiro Kojima, Takashi Komiyama, Yutaka Koyama, Shuhei Koyama, Yusei Lee, Chien-Hsiu Matsumoto, Akinori Mawatari, Ken Moriya, Takashi J. Motohara, Kentaro Murai, Kai Nishigaki, Moka Onodera, Masato Ono, Yoshiaki Rauch, Michael Saito, Tomoki Sasaki, Rin Suzuki, Akihiro Takeuchi, Tsutomu T. Umeda, Hiroya Umemura, Masayuki Watanabe, Kuria Yabe, Kiyoto Zhang, Yechi Institute for Cosmic Ray Research The University of Tokyo 5-1-5 Kashiwanoha Chiba Kashiwa277-8582 Japan Department of Physics Graduate School of Science The University of Tokyo 7-3-1 Hongo Bunkyo Tokyo113-0033 Japan National Astronomical Observatory of Japan 2-21-1 Osawa Mitaka Tokyo181-8588 Japan University of Tokyo Chiba Kashiwa277-8583 Japan Univ Lyon Univ Lyon1 ENS de Lyon CNRS Centre de Recherche Astrophysique de Lyon UMR5574 Saint-Genis-LavalF-69230 France Center for Relativistic Astrophysics School of Physics Georgia Institute of Technology AtlantaGA30332 United States Department of Astronomy Graduate School of Science The University of Tokyo 7-3-1 Hongo Bunkyo Tokyo113-0033 Japan European Southern Observatory Karl-Schwarzschild-Straße 2 Garching85748 Germany Observatoire de Genéve Université de Genéve 51 Ch. des Maillettes Versoix1290 Switzerland 650 North A'ohoku Place HiloHI96720 United States Research Center for Space and Cosmic Evolution Ehime University Bunkyo-cho 2-5 Ehime Matsuyama790-8577 Japan Center for Computational Sciences University of Tsukuba Ten-nodai 1-1-1 Tsukuba Ibaraki305-8577 Japan Department of Physics and Astronomy University College London Gower Street LondonWC1E 6BT United Kingdom National Institute of Technology Ichinoseki College Hagisho Ichinoseki021-8511 Japan Astronomical Institute Tohoku University 6-3 Aoba Aramaki Aoba-ku Miyagi Sendai980-8578 Japan Department of Physics and Astronomy University of Notre Dame 225 Nieuwland Science Hall Notre DameIN46556 United States Astronomy Program Department of Physics and Astronomy Seoul National University 1 Gwanak-ro Gwanak-gu Seoul08826 Korea Republic of SNU Astronomy Research Center Seoul National University 1 Gwanak-ro Gwanak-gu Seoul08826 Korea Republic of Department of Astronomy University of Wisconsin-Madison 475 N. Charter Street MadisonWI53706 United States Theoretical Astrophysics Department of Earth & Space S

We present kinematics of 6 local extremely metal-poor galaxies (EMPGs) with low metallicities (0.016 − 0.098 Z☉) and low stellar masses (104.7 − 107.6M☉). Taking deep medium-high resolution (R ∼ 7500) integral-field spectra with 8.2-m Subaru, we resolve the small inner velocity gradients and dispersions of the EMPGs with Hα emission. Carefully masking out sub-structures originated by inflow and/or outflow, we fit 3-dimensional disk models to the observed Hα flux, velocity, and velocity-dispersion maps. All the EMPGs show rotational velocities (vrot) of 5-23 km s−1 smaller than the velocity dispersions (σ0) of 17-31 km s−1, indicating dispersion-dominated (vrot/σ0 = 0.29−0.80 gas 0.9 − 1.0. Comparing our results with other Hα kinematics studies, we find that vrot/σ0 decreases and fgas increases with decreasing metallicity, decreasing stellar mass, and increasing specific star-formation rate. We also find that simulated high-z (z ∼ 7) forming galaxies have gas fractions and dynamics similar to the observed EMPGs. Our EMPG observations and the simulations suggest that primordial galaxies are gas-rich dispersion-dominated systems, which would be identified by the forthcoming James Webb Space Telescope (JWST) observations at z ∼ 7. Copyright © 2022, The Authors. All rights reserved.

关键词： Galaxies

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Microchip-Based Structure Determination of Small Proteins Using Cryo-EM

SSRN

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SSRN 2020年

作者： Casasanta, Michael A. Jonaid, G.M. Kaylor, Liam Luqiu, William Y. Solares, Maria J. Schroen, Mariah L. Dearnaley, William J. Wilson, Jarad Dukes, Madeline J. Kelly, Deborah F. Department of Biomedical Engineering Pennsylvania State University University ParkPA16802 United States Materials Research Institute Pennsylvania State University University ParkPA16802 United States Bioinformatics and Genomics Graduate Program Huck Institutes of the Life Sciences Pennsylvania State University University ParkPA16802 United States Molecular Cellular and Integrative Biosciences Graduate Program Huck Institutes of the Life Sciences Pennsylvania State University University ParkPA16802 United States Department of Electrical and Computer Engineering Duke University DurhamNC27708 United States RayBiotech Life Peachtree CornersGA30092 United States Applications Science Protochips Inc MorrisvilleNC27560 United States

Interest in cryo-Electron Microscopy (EM) imaging has skyrocketed in recent years due to its pristine views of macromolecules and materials. As advances in instrumentation and computing algorithms spurred this progress, there is renewed focus to address specimen-related challenges. Here we contribute a microchip-based toolkit to perform complementary structural and biochemical analysis on low molecular-weight proteins. As a model system, we used the SARS-CoV-2 nucleocapsid (N) protein (48 kDa) due to its stability and important role in therapeutic development. Cryo-EM structures of the N protein monomer revealed a flexible N-terminal “top hat” motif and a helical-rich C-terminal domain. To complement our structural findings, we engineered microchip-based immunoprecipitation assays that led to the discovery of the first antibody binding site on the N protein. The data also facilitated molecular modeling of a variety of pandemic and common cold-related coronavirus proteins. Such insights may guide future pandemic-preparedness protocols through immuno-engineering strategies to mitigate viral outbreaks. © 2020, The Authors. All rights reserved.

关键词： Proteins

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