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Wear behavior of dental glass-ceramics: a scoping review on the damage of opposing tooth enamel surfaces

Biotribology 2020年 21卷

作者： Souza, Júlio C.M. Silva, Cristina S. Caramês, João Henriques, Bruno Novaes de Oliveira, Antonio P. Silva, Filipe S. Gomes, José R. Center for MicroElectroMechanical Systems (CMEMS-UMINHO) University of Minho Campus Azurém Guimarães 4800-058 Portugal University Institute of Heal Sciences (IUCS) CESPU Gandra PRD Portugal School of Dentistry Universidade de Lisboa Lisboa Portugal Post-Graduate Program in Mechanical Engineering (POSMEC) Dept. of Mechanical Engineering (EMC) Federal University of Santa Catarina (UFSC) Florianópolis 88040-900 SC Brazil Laboratory of Glass-Ceramic Materials (VITROCER) Dept. of Mechanical Engineering (EMC) Federal University of Santa Catarina (UFSC) Florianópolis SC Brazil

The main aim of this study was to perform a scoping review on the wear behaviour of recent dental glass-ceramics and its influence on the damage of opposing tooth enamel surfaces. Relevant in vivo and in vitro studies reported significant damage on enamel surfaces after friction against current glass-ceramics and therefore different parameters have been studied such as the glass-ceramic type, wear set up, environment, and surface treatment. The opposing enamel loss in volume, weight, or vertical measurement shown by previous studies is significantly higher when compared to enamel-by-enamel wear values. In fact, high values of hardness and elastic modulus of glass-ceramics combined with rough surfaces can result in detrimental effects on the tooth enamel surfaces. Restorative dental materials must withstand masticatory loads in combination with aesthetic benefits and high biocompatibility. Nevertheless, elastic modulus, hardness, and roughness of glass-ceramics should be adjusted to decrease the damage on tooth enamel surfaces. © 2020 Elsevier Ltd

关键词： Friction Glass-ceramics Restorative dental materials Wear

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Mixed-linker strategy for suppressing structural flexibility of metal-organic framework membranes for gas separation

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Communications Chemistry 2023年第1期6卷 1-12页

作者： Chung-Kai Chang Yen-Chun Lin Yi-Pei Li Dun-Yen Kang Ting-Rong Ko Tsai-Yu Lin Heng-Liang Wu Hyun Jung Yu Jong Suk Lee Department of Chemical Engineering National Taiwan University No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan International Graduate Program of Molecular Science and Technology National Taiwan University (NTU-MST) No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan Center of Atomic Initiative for New Materials National Taiwan University No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan Center for Condensed Matter Sciences National Taiwan University No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan Department of Chemical and Biomolecular Engineering Sogang University Baekbeom-ro 35 Mapo-gu Seoul 04107 Republic of Korea

Structural flexibility is a critical issue that limits the application of metal-organic framework (MOF) membranes for gas separation. Herein we propose a mixed-linker approach to suppress the structural flexibility of the CAU-10-based (CAU = Christian-Albrechts-University) membranes. Specifically, pure CAU-10-PDC membranes display high separation performance but at the same time are highly unstable for the separation of CO2/CH4. A partial substitution (30 mol.%) of the linker PDC with BDC significantly improves its stability. Such an approach also allows for decreasing the aperture size of MOFs. The optimized CAU-10-PDC-H (70/30) membrane possesses a high separation performance for CO2/CH4(separation factor of 74.2 and CO2permeability of 1,111.1 Barrer under 2 bar of feed pressure at 35°C). A combination of in situ characterization with X-ray diffraction (XRD) and diffuse reflectance infrared Fourier transform (DRIFT) spectroscopy, as well as periodic density functional theory (DFT) calculations, unveils the origin of the mixed-linker approach to enhancing the structural stability of the mixed-linker CAU-10-based membranes during the gas permeation tests.

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Overcoming small-bandgap charge recombination in visible and NIR-light-driven hydrogen evolution by engineering the polymer photocatalyst structure

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Nature communications 2024年第1期15卷 707页

作者： Mohamed Hammad Elsayed Mohamed Abdellah Ahmed Zaki Alhakemy Islam M A Mekhemer Ahmed Esmail A Aboubakr Bo-Han Chen Amr Sabbah Kun-Han Lin Wen-Sheng Chiu Sheng-Jie Lin Che-Yi Chu Chih-Hsuan Lu Shang-Da Yang Mohamed Gamal Mohamed Shiao-Wei Kuo Chen-Hsiung Hung Li-Chyong Chen Kuei-Hsien Chen Ho-Hsiu Chou Department of Chemistry Faculty of Science Al-Azhar University Nasr City 11884 Cairo Egypt. Institute of Atomic and Molecular Sciences Academia Sinica Taipei 10617 Taiwan. Center for Condensed Matter Sciences National Taiwan University Taipei 10617 Taiwan. Department of Chemical Engineering National Tsing Hua University Hsinchu 300044 Taiwan. Department of Chemistry United Arab Emirates University Al Ain P.O. Box 15551 United Arab Emirates. Department of Chemistry Qena Faculty of Science South Valley University 83523 Qena Egypt. Chemical Physics and NanoLund Lund University 22100 Lund Sweden. Chemistry Department Faculty of Science Al-Azhar University Assiut 71542 Egypt. Sustainable Chemical Science and Technology Taiwan International Graduate Program Taipei Taiwan. Department of Applied Chemistry National Yang Ming Chiao Tung University Hsinchu 30010 Taiwan. Institute of Chemistry Academia Sinica 128 Sec 2 Academia Rd. Nankang Taipei 11529 Taiwan. Institute of Photonics Technologies National Tsing Hua University Hsinchu 300044 Taiwan. Center of Atomic Initiative for New Materials National Taiwan University Taipei 10617 Taiwan. Department of Chemical Engineering National Chung Hsing University Taichung 40227 Taiwan. Department of Materials and Optoelectronic Science Center for Functional Polymers and Supramolecular Materials National Sun Yat-Sen University Kaohsiung 804 Kaohsiung Taiwan. Department of Physics National Taiwan University Taipei 10617 Taiwan. Department of Chemical Engineering National Tsing Hua University Hsinchu 300044 Taiwan. hhchou@mx.nthu.edu.tw.

Designing an organic polymer photocatalyst for efficient hydrogen evolution with visible and near-infrared (NIR) light activity is still a major challenge. Unlike the common behavior of gradually increasing the charge recombination while shrinking the bandgap, we present here a series of polymer nanoparticles (Pdots) based on ITIC and BTIC units with different π-linkers between the acceptor-donor-acceptor (A-D-A) repeated moieties of the polymer. These polymers act as an efficient single polymer photocatalyst for H2 evolution under both visible and NIR light, without combining or hybridizing with other materials. Importantly, the difluorothiophene (ThF) π-linker facilitates the charge transfer between acceptors of different repeated moieties (A-D-A-(π-Linker)-A-D-A), leading to the enhancement of charge separation between D and A. As a result, the PITIC-ThF Pdots exhibit superior hydrogen evolution rates of 279 µmol/h and 20.5 µmol/h with visible (>420 nm) and NIR (>780 nm) light irradiation, respectively. Furthermore, PITIC-ThF Pdots exhibit a promising apparent quantum yield (AQY) at 700 nm (4.76%).

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AAA + ATPase Thorase inhibits mTOR signaling through the disassembly of the mTOR complex 1

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Nature Communications 2022年第1期13卷 4836页

作者： Umanah, George K. E. Abalde-Atristain, Leire Khan, Mohammed Repon Mitra, Jaba Dar, Mohamad Aasif Chang, Melissa Tangella, Kavya McNamara, Amy Bennett, Samuel Chen, Rong Aggarwal, Vasudha Cortes, Marisol Worley, Paul F. Ha, Taekjip Dawson, Ted M. Dawson, Valina L. Neuroregeneration and Stem Cell Programs Institute for Cell Engineering Johns Hopkins University School of Medicine Baltimore 21205 MD United States Department of Neurology Johns Hopkins University School of Medicine Baltimore 21205 MD United States Cellular and Molecular Medicine Graduate Program Johns Hopkins University School of Medicine Baltimore 21205 MD United States Department of Materials Science and Engineering University of Illinois at Urbana-Champaign Urbana 61801 IL United States Department of Biophysics and Biophysical Chemistry Johns Hopkins University Baltimore 21205 MD United States Solomon H. Snyder Department of Neuroscience Johns Hopkins University School of Medicine Baltimore 21205 MD United States Departments of Biophysics and Biophysical Chemistry Biophysics and Biomedical Engineering JHU Howard Hughes Medical Institute Baltimore 21205 MD United States Department of Pharmacology and Molecular Sciences Johns Hopkins University School of Medicine Baltimore 21205 MD United States Department of Physiology Johns Hopkins University School of Medicine Baltimore 21205 MD United States Division of Neuroscience National Institute of Neurological Disorders and Stroke National Institutes of Health Bethesda MD United States Vollum Institute Oregon Health & Science University Portland 97239 OR United States

The mechanistic target of rapamycin (mTOR) signals through the mTOR complex 1 (mTORC1) and the mTOR complex 2 to maintain cellular and organismal homeostasis. Failure to finely tune mTOR activity results in metabolic dysregulation and disease. While there is substantial understanding of the molecular events leading mTORC1 activation at the lysosome, remarkably little is known about what terminates mTORC1 signaling. Here, we show that the AAA + ATPase Thorase directly binds mTOR, thereby orchestrating the disassembly and inactivation of mTORC1. Thorase disrupts the association of mTOR to Raptor at the mitochondria-lysosome interface and this action is sensitive to amino acids. Lack of Thorase causes accumulation of mTOR-Raptor complexes and altered mTORC1 disassembly/re-assembly dynamics upon changes in amino acid availability. The resulting excessive mTORC1 can be counteracted with rapamycin in vitro and in vivo. Collectively, we reveal Thorase as a key component of the mTOR pathway that disassembles and thus inhibits mTORC1. © 2022, The Author(s).

关键词： Cell signalling Lysosomes Mechanisms of disease

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Current md forcefields fail to capture key features of protein structure and fluctuations: a case study of cyclophilin a and t4 lysozyme

arXiv

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arXiv 2020年

作者： Mei, Zhe Grigas, Alex T. Treado, John D. Corres, Gabriel Melendez Vuorte, Maisa Sammalkorpi, Maria Regan, Lynne Levine, Zachary A. O’Hern, Corey S. Department of Chemistry Yale University New HavenCT06520 United States Integrated Graduate Program in Physical and Engineering Biology Yale University New HavenCT06520 United States Graduate Program in Computational Biology and Bioinformatics Yale University New HavenCT06520 United States Department of Mechanical Engineering and Materials Science Yale University New HavenCT06520 United States Department of Biology UPR Humacao Puerto RicoHumacao00792 Puerto Rico Department of Chemistry and Materials Science School of Chemical Engineering Aalto University Aalto Finland Department of Bioproducts and Biosystems School of Chemical Engineering Aalto University Aalto Finland Institute of Quantitative Biology Biochemistry and Biotechnology Center for Synthetic and Systems Biology School of Biological Sciences University of Edinburgh Edinburgh United Kingdom Department of Pathology Yale School of Medicine New HavenCT06520 United States Department of Molecular Biophysics and Biochemistry Yale University New HavenCT06520 United States Department of Physics Yale University New HavenCT06520 United States Department of Applied Physics Yale University New HavenCT06520 United States

Globular proteins undergo thermal fluctuations in solution, while maintaining an overall well-defined folded structure. In particular, studies have shown that the core structure of globular proteins differs in small, but significant ways when they are solved by x-ray crystallography versus solution-based NMR spectroscopy. Given these discrepancies, it is unclear whether molecular dynamics (MD) simulations can accurately recapitulate protein conformations. We therefore perform extensive MD simulations across multiple force fields and sampling techniques to investigate the degree to which computer simulations can capture the ensemble of conformations observed in experiments. By analyzing fluctuations in the atomic coordinates and core packing, we show that conformations sampled in MD simulations both move away from and sample a larger conformational space than the ensemble of structures observed in NMR experiments. However, we find that adding inter-residue distance restraints that match those obtained via Nuclear Overhauser Effect measurements enables the MD simulations to sample more NMR-like conformations, though significant differences between the core packing features in restrained MD and the NMR ensemble remain. Given that the protein structures obtained from the MD simulations possess smaller and less dense protein cores compared to those solved by NMR, we suggest that future improvements to MD forcefields should aim to increase the packing of hydrophobic residues in protein cores. © 2020, CC BY.

关键词： Molecular dynamics

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Road infrastructure asset management strategy and its impact on the environment

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IOP Conference Series: materials science and engineering 2020年第2期830卷

作者： K Priyatiningsih M Sutrisno Lecturer of Asset Management Study Program Politeknik Negeri Bandung Bandung 40012 Indonesia Student of Management Science Doctoral Program School of Post Graduate Universitas Pendidikan Indonesia Bandung Indonesia Lecturer of Civil Engineering Politeknik Negeri Bandung Bandung 40012 Indoenesia

The development of the economic sector is determined by services to the public through reforms that aim to place public satisfaction through the management of road infrastructure assets. Some research on road infrastructure assets still requires a deepening of studies related to the delivery of public services related to asset management systems. The purpose of this study is to find an appropriate road infrastructure asset management strategy through an integrated asset management system and asset management policies that can provide public satisfaction. This comprehensive approach to management strategies ensures that the performance of service provider assets is in line with the expectations of stakeholders including road users. This descriptive qualitative research is based on the perspective of road users as respondents, consisting of vehicle drivers from 50 transportation companies (people or goods) through interviews and observations. The results show aspects of asset performance based on the user's perspective there are five aspects, namely productivity, efficiency, effectiveness, use of resources and institutions and this performance is integrated in the asset management system related to policies from the management authority through service delivery namely quality and mobility, risk and use and maintenance of resources. The conclusion of this research is that road infrastructure asset services can be improved through the concept of road infrastructure asset management strategies in an integrated management system with five aspects of performance and more directed towards asset management policies related to the provision of road infrastructure asset services.

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Dielectric Nanospheres: Directional Modulation of Exciton Emission Using Single Dielectric Nanospheres (Adv. Mater. 20/2021)

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Advanced materials 2021年第20期33卷

作者： Jie Fang Mingsong Wang Kan Yao Tianyi Zhang Alex Krasnok Taizhi Jiang Junho Choi Ethan Kahn Brian A. Korgel Mauricio Terrones Xiaoqin Li Andrea Alù Yuebing Zheng Walker Department of Mechanical Engineering and Texas Materials Institute The University of Texas at Austin Austin TX 78712 USA Photonics Initiative Advanced Science Research Center City University of New York New York NY 10031 USA Department of Materials Science and Engineering Department of Physics Department of Chemistry and Center for 2-Dimensional and Layered Materials The Pennsylvania State University University Park PA 16802 USA McKetta Department of Chemical Engineering The University of Texas at Austin Austin TX 78712 USA Department of Physics The University of Texas at Austin Austin TX 78712 USA Physics Program Graduate Center City University of New York New York NY 10016 USA

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Self-assembled periodic nanostructures using martensitic phase transformations

arXiv

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arXiv 2020年

作者： Prakash, Abhinav Wang, Tianqi Bucsek, Ashley Truttmann, Tristan K. Fali, Alireza Cotrufo, Michele Yun, Hwanhui Kim, Jong-Woo Ryan, Philip J. Mkhoyan, K. Andre Alù, Andrea Abate, Yohannes James, Richard D. Jalan, Bharat Department of Chemical Engineering and Materials Science University of Minnesota – Twin Cities MinneapolisMN55455 United States Department of Aerospace Engineering and Mechanics University of Minnesota – Twin Cities MinneapolisMN55455 United States Department of Mechanical Engineering University of Michigan Ann ArborMI48109 United States Department of Physics and Astronomy University of Georgia AthensGA30602 United States Photonics Initiative Advanced Science Research Center City University of New York NY10031 United States Advanced Photon Source Argonne National Laboratory ArgonneIL60439 United States Physics Program Graduate Center City University of New York New YorkNY10016 United States

We describe a novel approach for the rational design and synthesis of self-assembled periodic nanostructures using martensitic phase transformations. We demonstrate this approach in a thin film of perovskite SrSnO3 with reconfigurable periodic nanostructures consisting of regularly spaced regions of sharply contrasted dielectric properties. The films can be designed to have different periodicities and relative phase fractions via chemical doping or strain engineering. The dielectric contrast within a single film can be tuned using temperature and laser wavelength, effectively creating a variable photonic crystal. Our results show the realistic possibility of designing large-area self-assembled periodic structures using martensitic phase transformations with the potential of implementing "built-to-order" nanostructures for tailored optoelectronic functionalities. Copyright © 2020, The Authors. All rights reserved.

关键词： Thin films

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Frontispiece: Optical Characteristics of Hybrid Macrocycles with Dithienogermole and Tricoordinate Boron Units

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Chemistry – A European Journal 2021年第10期27卷

作者： Dr. Yohei Adachi Taishi Nabeya Keigo Kawakami Kosuke Yamaji Prof. Dr. Frieder Jäkle Prof. Dr. Joji Ohshita Applied Chemistry Program Graduate School of Advanced Science and Engineering Hiroshima University Higashi-Hiroshima 739-8527 Japan Department of Chemistry Rutgers University-Newark Newark NJ 07102 USA Division of Materials Model-Based Research Digital Monozukuri (Manufacturing) Education and Research Center Hiroshima University Higashi-Hiroshima 739-0046 Japan

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Corrigendum for “Review—Contemporary Progresses in Carbon-Based Electrode Material in Li-S Batteries” J. Electrochem. Soc. 169, 020530 2022

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Journal of The Electrochemical Society 2023年第11期170卷 119001-119001页

作者： Utkarsh Chadha Preetam Bhardwaj Sanjeevikumar Padmanaban Reyna Michelle Suneel Kevin Milton Neha Subair Akshat Pandey Mayank Khanna Divyansh Srivastava Rhea Mary Mathew Senthil Kumaran Selvaraj Murali Banavoth Prashant Sonar Badrish Badoni Nalamala Srinivasa Rao S. Gopa Kumar Arun Kumar Ray Amit Kumar Department of Manufacturing Engineering School of Mechanical Engineering (SMEC) Vellore Institute of Technology (VIT) Vellore Tamilnadu 632014 India Centre for Nanotechnology Research (CNR) School of Electronics Engineering (SENSE) Vellore Institute of Technology Vellore 632014 Tamil Nadu 632014 India Center for Electric Vehicles and Power Department of Electrical and Electronics Engineering Anna University Chennai-600025 India & Department of Energy Technology Aalborg University Esbjerg Denmark School of Chemical Engineering (SCHEME) Vellore Institute of Technology (VIT) Vellore Tamilnadu 632014 India Solar Cells and Photonics Research Laboratory School of Chemistry University of Hyderabad Hyderabad Telangana 500046 India Centre for Materials Science School of Chemistry and Physics Queensland University of Technology Brisbane QLD 4001 Australia Department of Physics Bal Ganga Degree College Sendul Kemar Tehri Garhwal Uttrakhand 249155 India Department of Chemistry Government Degree College Cumbum Prakasam Andhra Pradesh 523333 India Department of Electrical and Electronics Engineering Rohini College of Engineering and Technology Palkulam Anjugramam Tamilnadu 629401 India Department of Mechanical Engineering Hindu College of Engineering Sonipat Haryana-131001 India Department of Physics Radhey Hari Government Post Graduate College Kashipur Kumaun University Nainital Uttarakhand 244713 India

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