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TiZrHfNb refractory high-entropy alloys with twinning-induced plasticity

Journal of materials science & Technology 2024年第20期187卷 72-85页

作者： Shubin Wang Da Shu Peiying Shi Xianbing Zhang Bo Mao Donghong Wang Peter.K.Liaw Baode Sun Shanghai Key Lab of Advanced High-temperature Materials and Precision Forming and State Key Lab of Metal Matrix Composites School of Materials Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China Shanghai Institute of Applied Physics Chinese Academy of SciencesShanghai 201800China Department of Mechanical and Energy Engineering Southern University of Science and TechnologyShenzhen 518055China Department of Materials Science and Engineering The University of TennesseeKnoxvilleTN37996USA

The twinning-induced plasticity(TWIP)effect has been widely utilized in austenite steels,β-Ti alloys,and recently developed face-centered-cubic(FCC)high-entropy alloys(HEAs)to simultaneously enhance the tensile strength and *** this study,for the first time,the TWIP effect through hierarchical{332}<113>mechanical twinning has been successfully engineered into the TiZrHfNb refractory HEAs by decreasing temperature and tailoring the content of Nb to destabilize the BCC *** cryogenic tem-perature,the comprehensive hierarchical{332}<113>mechanical twins are activated in TiZrHfNb_(0.5) alloy from micro-to nanoscale and progressively segment the BCC grains into nano-scale islands during de-formation,ensuring sustainable strain hardening capability and eventually achieving a substantial 35%uniform tensile *** addition,at 77 K,the tensile strength and uniform elongation of TiZrHfNbx alloys can further be adjusted by a moderate increase of *** results above shed new light on the de-velopment of high-performance refractory HEAs with a high and adjustable strength and ductility com-bination down to the cryogenic temperature.

关键词： Refractory high-entropy alloys Cryogenic temperature Twinning induced plasticity Hierarchical twins Tensile properties

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Imaging and structure analysis of ferroelectric domains,domain walls,and vortices by scanning electron diffraction

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npj Computational materials 2024年第1期10卷 2154-2161页

作者： Ursula Ludacka Jiali He Shuyu Qin Manuel Zahn Emil Frang Christiansen Kasper A.Hunnestad Xinqiao Zhang Zewu Yan Edith Bourret István Kézsmárki Antonius T.Jvan Helvoort Joshua Agar Dennis Meier Department of Materials Science and Engineering NTNU Norwegian University of Science and TechnologyTrondheimNorway Department of Computer Science and Engineering Lehigh UniversityBethlehemPAUSA Department of Mechanical Engineering and Mechanics Drexel UniversityPhiladelphiaPAUSA Experimental Physics V University of AugsburgAugsburgGermany Department of Physics NTNU Norwegian University of Science and TechnologyTrondheimNorway Department of Physics ETH ZurichZürichSwitzerland Materials Sciences Division Lawrence Berkeley National LaboratoryBerkeleyCAUSA

Direct electron detectors in scanning transmission electron microscopy give unprecedented possibilities for structure analysis at the *** electronic and quantum materials,this new capability gives access to,for example,emergent chiral structures and symmetry-breaking distortions that underpin functional *** nanoscale structural features with statistical significance,however,is complicated by the subtleties of dynamic diffraction and coexisting contrast mechanisms,which often results in a low signal-to-noise ratio and the superposition of multiple signals that are challenging to deconvolute.

关键词： properties structure ferroelectric

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Aerosol jet printing of surface acoustic wave microfluidic devices

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Microsystems & Nanoengineering 2024年第1期10卷 231-242页

作者： Joseph Rich Brian Cole Teng Li Brandon Lu Hanyu Fu Brittany N.Smith Jianping Xia Shujie Yang Ruoyu Zhong James L.Doherty Kanji Kaneko Hiroaki Suzuki Zhenhua Tian Aaron D.Franklin Tony Jun Huang Department of Biomedical Engineering Duke UniversityDurhamNC 27708USA Department of Electrical and Computer Engineering Duke UniversityDurhamNC 27708USA Department of Mechanical Engineering Virginia Polytechnic Institute and State UniversityBlacksburgVA 24061USA Thomas Lord Department of Mechanical Engineering and Materials Science Duke UniversityDurhamNC 27708USA Deptartment of Precision Mechanics Faculty of Science and EngineeringChuo UniversityTokyo 112-8551Japan Department of Chemistry Duke UniversityDurhamNC 27708USA

The addition of surface acoustic wave(SAW)technologies to microfluidics has greatly advanced lab-on-a-chip applications due to their unique and powerful attributes,including high-precision manipulation,versatility,integrability,biocompatibility,contactless nature,and rapid ***,the development of SAW microfluidic devices is limited by complex and time-consuming micro/nanofabrication techniques and access to cleanroom facilities for multistep photolithography and vacuum-based *** simplify the fabrication of SAW microfluidic devices with customizable dimensions and functions,we utilized the additive manufacturing technique of aerosol jet *** successfully fabricated customized SAW microfluidic devices of varying materials,including silver nanowires,graphene,and poly(3,4-ethylenedioxythiophene)polystyrene sulfonate(PEDOT:PSS).To characterize and compare the acoustic actuation performance of these aerosol jet printed SAW microfluidic devices with their cleanroom-fabricated counterparts,the wave displacements and resonant frequencies of the different fabricated devices were directly measured through scanning laser Doppler ***,to exhibit the capability of the aerosol jet printed devices for lab-on-a-chip applications,we successfully conducted acoustic streaming and particle concentration ***,we demonstrated a novel solution-based,direct-write,single-step,cleanroom-free additive manufacturing technique to rapidly develop SAW microfluidic devices that shows viability for applications in the fields of biology,chemistry,engineering,and medicine.

关键词： printing wave fluid

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mechanically robust bamboo node and its hierarchically fibrous structural design

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National science Review 2023年第2期10卷 199-211页

作者： Si-Ming Chen Si-Chao Zhang Huai-Ling Gao Quan Wang LiChuan Zhou Hao-Yu Zhao Xin-Yu Li Ming Gong Xiao-Feng Pan Chen Cui Ze-Yu Wang YongLiang Zhang HengAn Wu Shu-Hong Yu Department of Chemistry Institute of Biomimetic Materials & Chemistry Anhui Engineering Laboratory of Biomimetic MaterialsDivision of Nanomaterials & Chemistry Hefei National Research Center for Physical Sciences at the Microscale Institute of Energy Hefei Comprehensive National Science Center University of Science and Technology of China CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Modern MechanicsEngineering and Materials Science Experiment CenterUniversity of Science and Technology of China Institute of Innovative Materials (I2M) Department of Materials Science and EngineeringDepartment of Chemistry Southern University of Science and Technology

Although short bamboo nodes function in mechanical support and fluid exchange for bamboo survival,their structures are not fully understood compared to unidirectional fibrous ***,we identify the spatial heterostructure of the bamboo node via multiscale imaging strategies and investigate its me chanical properties by multimodal mechanical *** find three kinds of hierarchical fiber reinforcement schemes that originate from the bamboo node,including spatially tightened interlocking,triaxial interconnected scaffolding and isotropic *** reinforcement schemes,built on porous vascular bundles,microfibers and more-refined twist-aligned nanofibers,govern the structural stability of the bamboo via hierarchical *** addition,the spatial liquid transport associated with these multiscale fibers within the bamboo node is experimentally verified,which gives perceptible evidence for life-indispensable multidirectional fluid *** functional integration of mechanical reinforcement and liquid transport reflects the fact that the bamboo node has opted for elaborate structural optimization rather than ingredient *** study will advance our understanding of biological materials and provide insight into the design of fiber-reinforced structures and biomass utilization.

关键词： biological materials bamboo node hierarchical fiber structural reinforcement functional integration

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Recent advances in tip-enhanced Raman spectroscopy probe designs

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Nano Research 2023年第4期16卷 5555-5571页

作者： Da Xu Boqun Liang Yaodong Xu Ming Liu Department of Electrical and Computer Engineering University of California-RiversideRiversideCalifornia 92521USA Materials Science and Engineering program University of California-RiversideRiversideCalifornia 92521USA

Tip-enhanced Raman spectroscopy(TERS)imaging is a super-resolution imaging technique that features the merits of both surface-enhanced Raman spectroscopy(SERS)and scanning probe microscopy(SPM),such as the high chemical sensitivity from the former and the nanoscale spatial resolution from the *** advantages make TERS an essential nanospectroscopic characterization technique for chemical analysis,materials science,bio-sensing,*** probes,the most critical factor determining the TERS imaging quality,are expected to provide a highly confined electromagnetic hotspot with a minimized scattering background for the generation of Raman signals with high spatial *** two decades of development,numerous probe design concepts have been proposed and *** review provides a comprehensive overview of the state-of-the-art TERS probe designs,from the working mechanism to the practical *** start with reviewing the recent development of TERS configurations and the corresponding working mechanisms,including the SPM platforms,optical excitation/collection techniques,and probe preparation *** then review the emerging novel TERS probe designs,including the remote-excitation probes,the waveguide-based nanofocusing probes,the metal-coated nanofocusing probes,the nanowire-assisted selective-coupling probes,and the tapered metal-insulator-metal *** discussion focuses on a few critical aspects,including the surface-plasmon-polariton(SPP)hotspot excitation technique,conversion efficiency,working frequency,and *** the end,we review the latest TERS applications and give a perspective on the future of TERS.

关键词： tip-enhanced Raman spectroscopy plasmonics scanning probe microscopy nanoscale imaging nanophotonics nanofocusing

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Accelerated discovery of eutectic compositionally complex alloys by generative machine learning

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npj Computational materials 2024年第1期10卷 1091-1102页

作者： Z.Q.Chen Y.H.Shang X.D.Liu Y.Yang Department of Mechanical Engineering City University of Hong KongHong KongChina City University of Hong Kong(Dongguan) DongguanGuangdongChina College of Mechatronics and Control Engineering Shenzhen UniversityShenzhenChina Department of Materials Science and Engineering City University of Hong KongKowloonChina Department of System Engineering College of EngineeringCity University of Hong KongKowloonChina

Eutectic alloys have garnered significant attention due to their promising mechanical and physical properties,as well as their technological ***,the discovery of eutectic compositionally complex alloys(ECCAs)(*** entropy eutectic alloys)remains a formidable challenge in the vast and intricate compositional space,primarily due to the absence of readily available phase *** address this issue,we have developed an explainable machine learning(ML)framework that integrates conditional variational autoencoder(CVAE)and artificial neutral network(ANN)models,enabling direct generation of *** overcome the prevalent problem of data imbalance encountered in data-driven ECCA design,we have incorporated thermodynamicsderived data descriptors and employed K-means clustering methods for effective data *** our ML framework,we have successfully discovered dual-or even tri-phased ECCAs,spanning from quaternary to senary alloy systems,which have not been previously reported in the *** findings hold great promise and indicate that ourML framework can play a pivotal role in accelerating the discovery of technologically significant ECCAs.

关键词： eutectic alloys alloy

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Rapid Outgassing of Hydrophilic TiO_(2) Electrodes Achieves Long-Term Stability of Anion Exchange Membrane Water Electrolyzers

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Nano-Micro Letters 2025年第8期17卷 219-236页

作者： Shajahan Shaik Jeonghyeon Kim Mrinal Kanti Kabiraz Faraz Aziz Joon Yong Park Bhargavi Rani Anne Mengfan Li Hongwen Huang Ki Min Nam Daeseong Jo Sang-Il Choi Department of Chemistry and Green-Nano Materials Research Center Kyungpook National UniversityDaegu 41566South Korea Department of Mechanical Engineering Kyungpook National UniversityDaegu 41566South Korea Department of Chemistry and Chemistry Institute for Functional Materials Pusan National UniversityBusan 46241South Korea Department of Metallurgical and Materials Engineering National Institute of TechnologyRaipur 492010India College of Materials Science and Engineering Hunan UniversityChangsha 410082HunanPeople’s Republic of China

The state-of-the-art anion-exchange membrane water electrolyzers(AEMWEs)require highly stable electrodes for prolonged *** stability of the electrode is closely linked to the effective evacuation of H_(2) or O_(2) gas generated from electrode surface during the *** this study,we prepared a superhydrophilic electrode by depositing porous nickel–iron nanoparticles on annealed TiO_(2) nanotubes(NiFe/ATNT)for rapid outgassing of such nonpolar *** super-hydrophilic NiFe/ATNT electrode exhibited an overpotential of 235 mV at 10 mA cm^(−2) for oxygen evolution reaction in 1.0 M KOH solution,and was utilized as the anode in the AEMWE to achieve a current density of 1.67 A cm^(−2) at 1.80 *** addition,the AEMWE with NiFe/ATNT electrode,which enables effective outgassing,showed record stability for 1500 h at 0.50 A cm^(−2) under harsh temperature conditions of 80±3℃.

关键词： TiO_(2)nanotubes NiFe Super-hydrophilic electrode Oxygen evolution reaction Anion-exchange membrane water electrolyzer

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Fabrication and Characterization of Willemite Scaffolds Using Corn Stalk as a Novel Bio Template for Bone Tissue engineering Applications

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Journal of Bionic engineering 2023年第1期20卷 16-29页

作者： Zahra Yahay Seyed Mehdi Mirhadi Fariborz Tavangarian Department of Cellular Biotechnology Cell Science Research CenterRoyan Institute for BiotechnologyACECRIsfahan81593-58686Iran Department of Materials Engineering Shahreza BranchIslamic Azad UniversityShahrezaIsfahan86145-311Iran Mechanical Engineering Program School of ScienceEngineering and TechnologyPennsylvania State UniversityHarrisburgMiddletownPA17057USA

In this paper,we used Corn Stalk(CS)as a renewable and economical bio template to fabricate willemite scaffolds with the potential application in skull bone *** was used as a sacrificial template to synthesize the *** scaffolds with the chemical formula of Zn2SiO4 and pore size in the range of 3 to 10µm could be successfully synthesized by soaking CS in the willemite solution for 24 h and sintering at 950°C for 5 *** porosity of the samples was controlled by the soaking time(between 12 and 48 h)in the willemite solution from 5 to 35%,*** properties of these scaffolds showed a good approximation with cranial bone *** addition,cytotoxicity assays(MTT)were performed on Human Bone Marrow Stromal cells(HBMSc)and A172 human glioblastoma cell lines by direct and indirect culture methods to estimate their toxicity for bone and nerve cells,*** Phosphatase(ALP)activity and DAPI/Phalloidin cell staining were also performed to investigate the efficiency of the scaffolds for bone tissue engineering *** results showed that the scaffolds had good biocompatibility with both HBMSC and A172 cells,noticeable improvement on ALP activity,and great apatite formation ability in Simulated Body Fluid(SBF).All the evidence ascertained that willemite scaffolds made by corn stalks could be a useful candidate for bone tissue engineering applications.

关键词： Corn stalk Bio template Bioactive ceramics-Scaffolds Bone tissue engineering

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Investigation on mechanical properties of hybrid polymer composites for automobile applications

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materials Today: Proceedings 2023年 74卷 73-79页

作者： Beer Mohamed, S. Anandhavasan, S. Basheer Ahamed, S. Ajayharish, R. Barathraj, B. Hariprakash, R. Ravichandran, M. Kaviarasu, C. Department of Materials Science Central University of Tamil Nadu Thiruvarur 610005 India Department of Mechanical Engineering Arasu Engineering College Kumbakonam 612501 India Department of Mechanical Engineering K.Ramakrishnan College of Engineering Trichy 621112 India

A novel epoxy-based hybrid polymer composite was developed and the effect of hybridization on the mechanical properties was investigated. Sisal fiber, polypropylene fiber, alumina trihydrate and nano silica are used for hybridization in epoxy resin matrix via hand layup process. Hardness and impact testing were conducted as per the standards ASTM D2240 and ASTM D256 respectively. Both sisal and polypropylene fibers (5 %wt.) without fillers have improved the hardness by 5.8 % and achieved an impact strength of 68 kJ/m2. A small addition of ATH (0.5 % wt.) as filler to inherit the fire retardancy has deteriorated the mechanical properties of hybrid polymers. However, the addition of nano silica (1.5 % wt.) as another filler along with ATH, sisal and polypropylene fibers has improved the mechanical properties, i.e., hardness and impact value of the epoxy resin-based hybrid polymer by 9.4 % and 85.7 % respectively by suppressing the ATH effect in the hybridization. © 2022

关键词： Polypropylenes

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Light-Material Interactions Using Laser and Flash Sources for Energy Conversion and Storage Applications

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Nano-Micro Letters 2024年第12期16卷 468-514页

作者： Jung Hwan Park Srinivas Pattipaka Geon-Tae Hwang Minok Park Yu Mi Woo Young Bin Kim Han Eol Lee Chang Kyu Jeong Tiandong Zhang Yuho Min Kwi-Il Park Keon Jae Lee Jungho Ryu Department of Mechanical Engineering(Department of Aeronautics Mechanical and Electronic Convergence Engineering)Kumoh National Institute of Technology61Daehak-RoGumiGyeongbuk 39177Republic of Korea Department of Materials Science and Engineering Pukyong National University45Yongso-RoNam-GuBusan 48513Republic of Korea Energy Technologies Area Lawrence Berkeley National LaboratoryBerkeleyCA 94720USA Department of Materials Science and Engineering Korea Advanced Institute of Science and Technology(KAIST)291 Daehak-RoYuseong-GuDaejeon 34141Republic of Korea Division of Advanced Materials Engineering Jeonbuk National UniversityJeonju 54896JeonbukRepublic of Korea School of Electrical and Electronic Engineering Harbin University of Science and TechnologyHarbin 150080People’s Republic of China Key Laboratory of Engineering Dielectrics and Its Application Ministry of EducationHarbin University of Science and TechnologyHarbin 150080People’s Republic of China Department of Materials Science and Metallurgical Engineering Kyungpook National University80 Daehak-RoBuk-GuDaegu 41566Republic of Korea School of Materials Science and Engineering Yeungnam UniversityDaehak-RoGyeongsan-Si 38541Gyeongsangbuk-doRepublic of Korea

This review provides a comprehensive overview of the progress in light-material interactions(LMIs),focusing on lasers and flash lights for energy conversion and storage *** discuss intricate LMI parameters such as light sources,interaction time,and fluence to elucidate their importance in material *** addition,this study covers various light-induced photothermal and photochemical processes ranging from melting,crystallization,and ablation to doping and synthesis,which are essential for developing energy materials and ***,we present extensive energy conversion and storage applications demonstrated by LMI technologies,including energy harvesters,sensors,capacitors,and *** the several challenges associated with LMIs,such as complex mechanisms,and high-degrees of freedom,we believe that substantial contributions and potential for the commercialization of future energy systems can be achieved by advancing optical technologies through comprehensive academic research and multidisciplinary collaborations.

关键词： Light Light-material interaction Nanomaterials Energy conversion and storage devices

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