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Two-step superconductor-insulator transitions in iron chalcogenide superconductors

Physical Review B 2025年第6期111卷 L060506-L060506页

作者： Li Xu Zefeng Lin Wenxin Cheng Xuewei Wang Mingyang Qin Xingyu Jiang Liping Zhang Juan Xu Peiyu Xiong Beijing National Laboratory for Condensed Matter Physics Institute of Physics Chinese Academy of Sciences Beijing 100190 China School of Physical Sciences University of Chinese Academy of Sciences Beijing 100049 China Department of Materials Science and Engineering Southern University of Science and Technology Shenzhen 518055 China Beijing Academy of Quantum Information Sciences Beijing 100193 China School of Physics and Technology Wuhan University Wuhan 430072 China

The superconductor-insulator transition is an archetypal example of a quantum phase transition that plays a crucial role in physics and statistical mechanics. Belonging to different universality classes, the classical and quantum percolative transitions usually manifest in different systems and are studied separately. Here, we fabricate thickness-gradient FeyTe1−xSex (FTS) films and observe the existence of these two transitions. Variation in the film thickness, which controls substrate misfit and leads to a modification of Fe concentration, results in a superconducting quantum percolative transition. By exposing FTS films to air, we observe a shift in electrical resistivity behavior and a superconducting classical percolative transition. FTS films subjected to the two treatments exhibit very similar phase diagrams, except for different critical exponents. Remarkably, we identify a two-step superconductor-insulator transition at low temperature, where the appearance of superconductive zero resistivity coincides with a sign change in the temperature derivative of electrical resistivity in the normal state. Our analysis can provide a universal scheme to categorize the superconductor-insulator transition in various copper-oxide and iron-based superconductors.

关键词： Iron-based Superconductors

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Giant phonon-skyrmion coupling in ferromagnet/heavy metal heterostructures

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Physical Review B 2024年第6期110卷 064423-064423页

作者： Egor Savostin Vitaliy Lomakin Program in Materials Science and Engineering Center for Memory and Recording Research Department of Electrical and Computer Engineering

The strong impact of the strain-induced Dzyaloshinskii-Moriya interaction (SIDMI) on the magnetization dynamics of skyrmions in nanomagnetic structures is demonstrated. The effects of SIDMI are characterized by skyrmion equations (SEs) of motion and magnetoelastic (ME) equations. The study is performed on a model system of MgO/CoFe/Pt stacked on a piezoelectric substrate. The results demonstrate a major nonlinear amplification in both the first- and higher-harmonic magnitudes of the skyrmion breathing mode due to SIDMI. Remarkably, this enhancement can trigger a skyrmion collapse, enabling its deletion with ultraweak strain-induced excitations. The SIDMI effect is shown to be much more significant than the conventional ME effect. These findings open different avenues for the efficient manipulation of nanomagnetic structures through strain.

关键词： Exchange interaction Magnetic interactions Magnetization dynamics Magnetoacoustic effect Micromagnetism Spin dynamics

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Influence of extended interactions on spin dynamics in one-dimensional cuprates

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Physical Review B 2024年第16期110卷 165118页

作者： Ta Tang Daniel Jost Brian Moritz Thomas P. Devereaux Stanford Institute for Materials and Energy Sciences Department of Applied Physics Department of Materials Science and Engineering Geballe Laboratory for Advanced Materials

Quasi-one-dimensional (1D) materials provide a unique platform for understanding the importance and influence of extended interactions on the physics of strongly correlated systems due to their relative structural simplicity and the existence of powerful theoretical tools well adapted to one spatial dimension. Recently, this was highlighted by anomalous observations in the single-particle spectral function A(q,ω) of 1D cuprate chain compounds, measured by angle-resolved photoemission spectroscopy (ARPES), which were explained by the presence of a long-range attractive interaction. Such an extended interaction should leave its fingerprints on other observables, notably the dynamical spin structure factor S(q,ω), measured by neutron scattering or resonant inelastic x-ray scattering. Starting from a simple Hubbard Hamiltonian in 1D and using time-dependent density matrix renormalization group methods, we show that the presence of long-range attractive coupling, directly through an instantaneous Coulomb interaction V or retarded electron-phonon (el-ph) coupling, can introduce significant spectral weight redistribution in S(q,ω) across a wide range of doping. This underscores the significant impact that extended interactions can have on dynamical correlations among particles, and the importance of properly incorporating this influence in modeling. Our results demonstrate that S(q,ω) can provide a sensitive experimental constraint, which complements ARPES measurements, in identifying key interactions in 1D cuprates, beyond the standard Hubbard model.

关键词： Density matrix renormalization group Spin dynamics Cuprates

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Electronic structure and optical spectra of MSi2N4 (M = Mo, Ta, V) materials with single-atom decoration: a first-principles study

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Journal of materials Chemistry C 2023年第43期11卷 15097-15105页

作者： Wu, Tzu-Cheng Liao, Yin-Song Kao, Jui-Cheng Chou, Jyh-Pin Department of Physics National Tsing Hua University Hsinchu300044 Taiwan The Affiliated Senior High School of National Taiwan Normal University Taipei10658 Taiwan Tsing Hua Interdisciplinary Program National Tsing Hua University Hsinchu300044 Taiwan Department of Materials Science and Engineering National Tsing Hua University Hsinchu300044 Taiwan Department of Materials Science and Engineering National Yang Ming Chiao Tung University Hsinchu30010 Taiwan Department of Physics National Changhua University of Education Changhua50007 Taiwan

MoSi2N4 has outstanding potential for applications in electronics, spintronics, and semiconducting fabrication. This attractive scenario can be attributed to its remarkable electronic properties. In this study, we investigate the electronic structure and optical spectra of the MSi2N4 (M = Mo, Ta, and V) materials with single atom (H, N, and O) decoration using first-principles calculations. Pristine MoSi2N4 and VSi2N4 are semiconductors, and TaSi2N4 shows the half-metal properties. Decorating MoSi2N4 with single hydrogen and nitrogen atoms induces a magnetic moment. Single oxygen decorated TaSi2N4 does not change its intrinsic electronic properties, which is suitable for spintronic applications. On top of that, the semiconductor VSi2N4 can be turned into a half-metal via single hydrogen atom decoration. The absorption spectra demonstrate an enhancement in optical absorption for VSi2N4 after the decoration with a single nitrogen atom. Single atom decoration is one of the effective methods of tailoring the electronic properties of the two-dimensional MoSi2N4 family. Our findings can accelerate the development of the advanced electronic devices. © 2023 The Royal Society of Chemistry.

关键词： Silicon compounds

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Structural,magnetic and antibacterial properties of manganese-substituted magnetite ferrofluids

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International Journal of Minerals,Metallurgy and materials 2023年第7期30卷 1417-1426页

作者： Blessy Babukutty Deepalekshmi Ponnamma Swapna S.Nair Jiya Jose Saritha G.Bhat Sabu Thomas Department of Physics Central University of KeralaKasargod 671314India Materials Science and Technology Program College of Arts and SciencesQatar UniversityP.O.Box 2713DohaQatar Department of Biotechnology Cochin University of Science and TechnologyKalamasseryKeralaIndia Department of Chemistry Mahatma Gandhi UniversityKottayam 686560KeralaIndia

Manganese-substituted magnetite ferrofluids(FFs)Mnx Fe_(1-x)Fe_(2)O_(4)(x=0–0.8)were prepared in this work through a chemical coprecipitation *** controlled growth of FF nanomaterials for antibacterial activities is challenging,and therefore,very few reports are available on the *** research focuses on stabilizing aqueous FFs with the tetramethylammonium hydroxide surfactant to achieve high *** characterization reveals nanoparticles of 5–11 nm formed by the chemical reaction and nanocrystalline nature,as evident from structural ***-substituted magnetic FFs are analyzed for their structural,functional,and antibacterial performance according to the Mn-substituent *** studies show a high blue shift for Mn^(2+)-substituted Mnx Fe_(1-x)Fe_(2)O_(4)with the theoretical correlation of optical band gaps with the Mn *** superparamagnetic nature of substituted FFs causes zero coercivity and remanence,which consequently influence the particle size,cation distribution,and spin *** structural and functional performance of the FFs is correlated with the antibacterial activity,finally demonstrating the highest inhibition zone formation for Mnx Fe_(1-x)Fe_(2)O_(4)FFs.

关键词： manganese ferrofluids homogeneity antibacterial stability

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Flexible artificial synapse based on single-crystalline BiFeO_(3) thin film

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Nano Research 2022年第3期15卷 2682-2688页

作者： Zhen Zhao Amr Abdelsamie Rui Guo Shu Shi Jianhui Zhao Weinan Lin Kaixuan Sun Jingjuan Wang Junling Wang Xiaobing Yan Jingsheng Chen Key Laboratory of Brain-like Neuromorphic Devices and Systems of Hebei Province College of Electron and Information EngineeringHebei UniversityBaoding 071002China Department of Materials Science and Engineering Nanyang Technological UniversitySingapore 639798Singapore Department of Materials Science and Engineering National University of SingaporeSingapore 117576Singapore Department of Physics Southern University of Science and TechnologyShenzhen 518055China

Realization of functional flexible artificial synapse is a significant step toward neuromorphic ***,a flexible artificial synapse based on ferroelectric tunnel junctions(FTJs)is demonstrated,using BiFeO_(3)(BFO)thin film as the functional *** inorganic single crystalline FTJs grown on rigid perovskite substrates at high temperatures are integrated with the flexible plastic substrates,by using the water-soluble Sr_(3)Al_(2)O_(6)(SAO)as the sacrificial layer and the following *** transferred freestanding BFO thin film exhibits excellent ferroelectric ***,the memristive properties and the brain-like synaptic learning performance of the flexible FTJs are *** results show that multilevel resistance states were maintained well of the flexible artificial synapse,together with their stable synaptic learning *** work indicates the promising opportunity of ferroelectric thin film based flexible synapse used in the future neuromorphic computing system.

关键词： flexible ferroelectricity memristor artificial synapse

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Exploring the Correlation Between Surface Roughness, Surface Energy, Nano-indentation, Electrical Properties, and Magnetic Characteristics of Annealed Co40Fe40Dy20 Thin Films Deposited on Si(100) Substrates

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Journal of Electronic materials 2024年第8期53卷 4498-4511页

作者： Liu, Wen-Jen Chang, Yung-Huang Hsu, Shuo-Ting Fern, Chi-Lon Chen, Yuan-Tsung Tsao, Shin-Ying Lin, Shih-Hung Department of Materials Science and Engineering I-Shou University Kaohsiung840 Taiwan Bachelor Program in Industrial Technology National Yunlin University of Science and Technology 123 University Road Section 3 Yunlin Douliou64002 Taiwan Graduate School of Materials Science National Yunlin University of Science and Technology 123 University Road Section 3 Yunlin Douliou64002 Taiwan Department of Electronic Engineering National Yunlin University of Science and Technology 123 University Road Section 3 Yunlin Douliou64002 Taiwan

The impact of film thickness and annealing temperature on the structural, electrical, magnetic, and mechanical properties of cobalt–iron–dysprosium (Co40Fe40Dy20 ) thin films deposited on Si(100) substrates have been investigated. X-ray diffraction (XRD) analysis confirmed the film's crystalline microstructure, featuring dysprosium oxide, Dy2O3(440), and cobalt oxide, Co2O3(422) and Co2O3(511), crystallographic phases. Surface energy measurements indicated a noticeable reduction in surface energy following annealing treatments, which could be ascribed to the alleviation of residual stress and enhanced atomic arrangement, resulting in a more stable film structure with reduced surface energy. The film exhibited a decreasing trend in hardness with increasing thickness, and film resistivity was significantly responsive to alterations in thickness and annealing temperature. Notably, the Co40Fe40Dy20 film demonstrated exceptional characteristics, featuring a high saturation magnetization (Ms) of 675 emu/cm3 and a low coercivity (Hc) of 9.5 Oe. Further analysis of magnetic domains and hysteresis loops revealed that larger and brighter domains were associated with higher Hc. To sum up, the surface roughness of CoFeDy films under various annealing temperatures played a pivotal role in shaping their magnetic, electrical, adhesive, and optical characteristics. An improved low-frequency alternating current magnetic susceptibility (χac) value was achieved by minimizing the pinning effect on domain walls through surface smoothing. Moreover, smoother surfaces displayed heightened carrier conductivity, resulting in a decrease in electrical resistance. On the whole, Co40Fe40Dy20 films exhibited outstanding soft magnetic properties, encompassing high saturation magnetization, low coercivity, exceptional mechanical attributes, and decreased surface energy. Graphical Abstract: (Figure presented.) © The Minerals, Metals & materials Society 2024.

关键词： Magnetic susceptibility

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Terahertz phonon polariton concentrator based on perovskite oxides

Terahertz phonon polariton concentrator based on perovskite ...

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2023 Conference on Lasers and Electro-Optics, CLEO 2023

作者： Xu, Rui Lin, Tong Luo, Jiaming Chen, Xiaotong Blackert, Elizabeth R. Moon, Alyssa R. JeBailey, Khalil M. Zhu, Hanyu Department of Materials Science and Nano Engineering Rice University Houston United States Applied Physics Graduate Program Rice University Houston United States Program Rice University Houston United States

ISBN: (纸本)9781957171258

We report the experimental demonstration of surface phonon-polaritonic devices in a broad spectral range of 7-13 THz based on SrTiO3. We designed planar ultrafast concentrators that amplifies transient electric field by 6 times and measured an average field of 0.5 GV/m in an optically resolvable area in the far field. © 2023 The Author(s)

关键词： Perovskite

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Supercurrent through a single transverse mode in nanowire Josephson junctions

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Physical Review B 2025年第16期111卷 L161401-L161401页

作者： B. Zhang Z. Li H. Wu M. Pendharkar C. Dempsey J. S. Lee S. D. Harrington C. J. Palmstrøm S. M. Frolov Department of Physics and Astronomy University of Pittsburgh Pittsburgh Pennsylvania 15260 USA Department of Physics The Pennsylvania State University University Park Pennsylvania 16802 USA Electrical and Computer Engineering University of California Santa Barbara California 93106 USA Present address: Department of Materials Science and Engineering Stanford University Stanford CA 94305 USA. California NanoSystems Institute University of California Santa Barbara Santa Barbara California 93106 USA Present address: Department of Physics and Astronomy University of Tennessee Knoxville TN 37996 USA. Materials Department University of California Santa Barbara Santa Barbara California 93106 USA

Hybrid superconductor-semiconductor materials are fueling research in mesoscopic physics and quantum technology. Recently demonstrated smooth β-Sn superconductor shells, due to the increased induced gap, are expanding the available parameter space to new regimes. Fabricated on quasiballistic InSb nanowires, with careful control over the hybrid interface, Sn shells yield measurable switching currents even when nanowire resistance is of order 10kΩ. In this regime Cooper pairs travel through a purely one-dimensional quantum wire for at least part of their trajectory. Here, we focus on the evolution of proximity-induced supercurrent in magnetic field parallel to the nanowire. Long decay up to fields of 1T is observed. At the same time, the decay for higher occupied subbands is notably faster in some devices but not in others. We analyze this using a tight-binding numerical model that includes the Zeeman, orbital, and spin-orbit effects. When the first subband is spin polarized, we observe a dramatic suppression of supercurrent, which is also confirmed by the model and suggests an absence of significant triplet supercurrent generation.

关键词： Nanowires

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Higher-order topology in twisted multilayer systems:A review

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Chinese physics B 2025年第3期34卷 2-10页

作者： Chunbo Hua Dong-Hui Xu Key Laboratory of Artificial Micro-and Nanostructures of Ministry of Education and School of Physics and Technology Wuhan UniversityWuhan 430072China School of Electronic and Information Engineering Hubei University of Science and TechnologyXianning 437100China Department of Physics and Chongqing Key Laboratory for Strongly Coupled Physics Chongqing UniversityChongqing 400044China Center of Quantum Materials and Devices Chongqing UniversityChongqing 400044China

In recent years,there has been a surge of interest in higher-order topological phases(HOTPs)across various disciplines within the field of *** unique phases are characterized by their ability to harbor topological protected boundary states at lower-dimensional boundaries,a distinguishing feature that sets them apart from conventional topological phases and is attributed to the higher-order bulk-boundary ***-dimensional(2D)twisted systems offer an optimal platform for investigating HOTPs,owing to their strong controllability and experimental ***,we provide a comprehensive overview of the latest research advancements on HOTPs in 2D twisted multilayer *** will mainly review the HOTPs in electronic,magnonic,acoustic,photonic and mechanical twisted systems,and finally provide a perspective of this topic.

关键词： higher-order topology twisted multilayer systems van der Waals materials corner states

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