检索结果-内蒙古大学图书馆

In-situ nonvolatile and volatile modulation for optical neural networks

Advanced Photonics 2023年第5期5卷 1-2页

作者： Carlos A.Ríos Ocampo University of Maryland Department of Materials Science&EngineeringCollege ParkMarylandUnited States University of Maryland Institute for Research in Electronics and Applied PhysicsCollege ParkMarylandUnited States

High-performance integrated optical memristors are crucial in developing optical neural networks based on in-memory *** devices are building blocks capable of modulating the transmission of a propagating mode in a multilevel and nonvolatile fashion,thus allowing storage and multiplication of analog signals in the same device.1 Chalcogenide phase change materials(PCMs)are candidates for high-performance devices.

关键词： optical networks neural

来源：评论

学校读者我要写书评

暂无评论

High energy storage density in NaNbO_(3) antiferroelectrics with double hysteresis loop

引用

Journal of Materiomics 2024年第5期10卷 1026-1035页

作者： Li Ma Zhenpei Chen Gengguang Luo Zhiyi Che Chao Xu Dongliang Shan Zhenyong Cen Qin Feng Xiyong Chen Toyohisa Fujita Ye Zhu Yunya Liu Jing-Feng Li Shujun Zhang Nengneng Luo State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures School of ResourcesEnvironment and MaterialsGuangxi UniversityNanning530004China School of Chemistry and Chemical Engineering Guangxi UniversityNanning530004China Department of Applied Physics Research Institute for Smart EnergyThe Hong Kong Polytechnic UniversityHung HomKowloonHong KongChina Key Laboratory of Low Dimensional Materials and Application Technology of Ministry of Education School of Materials Science and EngineeringXiangtan UniversityXiangtan411105HunanChina State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing100084China Institute for Superconducting and Electronic Materials Australian Institute of Innovative MaterialsUniversity of WollongongWollongongNSW2500Australia

Antiferroelectrics(AFEs)possess great potential for high performance dielectric capacitors,due to their distinct double hysteresis loop with high maximum polarization and low remnant ***,the well-known NaNbO_(3) lead-free antiferroelectric(AFE)ceramic usually exhibits square-like P–E loop related to the irreversible AFE P phase to ferroelectric(FE)Q phase transition,yielding low recoverable energy storage density(Wrec).Herein,significantly improved Wrec up to 3.3 J/cm^(3) with good energy storage efficiency(η)of 42.4% was achieved in Na_(0.7)Ag_(0.3)Nb_(0.7)Ta_(0.3)O_(3)(30Agsingle bond30Ta)ceramic with well-defined double P–E loop,by tailoring the A-site electronegativity with Ag+and B-site polarizability with Ta^(5+).The Transmission Electron Microscope,Piezoresponse Force Microscope and in-situ Raman spectra results verified a good reversibility between AFE P phase and high-field-induced FE Q *** improved stability of AFE P phase,being responsible for the double P–E loop and improved Wrec,was attributed to the decreased octahedral tilting angles and cation *** mechanism was revealed by synchrotron X-ray diffraction and Scanning Transmission Electron *** work provides a good paradigm for achieving double P–E loop and high energy storage density in NaNbO_(3)-based ceramics.

关键词： Sodium niobate Antiferroelectrics Double hysteresis loop Energy storage performance Reversibility

来源：评论

学校读者我要写书评

暂无评论

Enabling stable 4.6 V LiCoO_(2) cathode through oxygen charge regulation strategy

引用

Journal of Energy Chemistry 2023年第1期76卷 557-565,I0014页

作者： Wen Zhang Xiaoyu Zhang Fangyuan Cheng Meng Wang Jing Wan Yuyu Li Jia Xu Yi Liu Shixiong Sun Yue Xu Chun Fang Qing Li Jiantao Han Yunhui Huang State Key Laboratory of Material Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074HubeiChina Department of Applied Physics Chongqing UniversityChongqing 401331China Key Laboratory of Optoelectronic Chemical Materials and Devices of Ministry of Education Jianghan UniversityWuhan 430056HubeiChina

LiCoO_(2) is the preferred cathode material for consumer electronic products due to its high volumetric energy density. However, the unfavorable phase transition and surface oxygen release limits the practical application of LiCoO_(2)at a high-voltage of 4.6 V to achieve a higher energy density demanded by the market. Herein, both bulk and surface structures of LiCoO_(2)are stabilized at 4.6 V through oxygen charge regulation by Gd-gradient doping. The enrichment of highly electropositive Gd on LiCoO_(2) surface will increase the effective charge on oxygen and improve the oxygen framework stability against oxygen *** the other hand, Gd ions occupy the Co-sites and suppress the unfavorable phase transition and microcrack. The modified LiCoO_(2) exhibits superior cycling stability with capacity retention of 90.1% over 200 cycles at 4.6 V, and also obtains a high capacity of 145.7 m Ah/g at 5 C. This work shows great promise for developing high-voltage LiCoO_(2) at 4.6 V and the strategy could also contribute to optimizing other cathode materials with high voltage and large capacity, such as cobalt-free high-nickel and lithiumrich manganese-based cathode materials.

关键词： Li-ion batteries 4.6 V LiCoO_(2) Gd-gradient doping Oxygen charge Cycle stability

来源：评论

学校读者我要写书评

暂无评论

Localization effect in single crystal of RuAs_(2)

引用

Chinese physics B 2024年第4期33卷 195-200页

作者：易哲铠刘琪光双魁徐升岳小宇梁慧李娜周颖吴丹丹孙燕李秋菊程鹏夏天龙孙学峰王义炎 Anhui Key Laboratory of Magnetic Functional Materials and Devices Institute of Physical Science and Information TechnologyAnhui UniversityHefei 230601China Department of Physics and Key Laboratory of Strongly-Coupled Quantum Matter Physics University of Science and Technology of ChinaHefei 230026China Department of Physics and Beijing Key Laboratory of Opto-electronic Functional Materials&Micro-nano Devices Renmin University of ChinaBeijing 100872China School of Optical and Electronic Information Suzhou City UniversitySuzhou 215104China School of Physics and Optoelectronic Engineering Anhui UniversityHefei 230601China Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China

We report the magnetotransport and thermal properties of RuAs_(2) single ***_(2) exhibits semiconductor behavior and localization *** crossover from normal state to diffusive transport in the weak localization(WL)state and then to variable range hopping(VRH)transport in the strong localization state has been *** transitions can be reflected in the measurement of resistivity and Seebeck *** magnetoresistance(NMR)emerges with the appearance of localization effect and is gradually suppressed in high magnetic *** temperature dependent phase coherence length extracted from the fittings of NMR also indicates the transition from WL to *** measurement of Hall effect reveals an anomaly of temperature dependent carrier concentration caused by localization *** findings show that RuAs_(2) is a suitable platform to study the localized state.

关键词： weak localization variable range hopping RuAs_(2) single crystal

来源：评论

学校读者我要写书评

暂无评论

Porous Indium Nanocrystals on Conductive Carbon Nanotube Networks for High-Performance CO_(2)-to-Formate Electrocatalytic Conversion

引用

Energy & Environmental materials 2024年第4期7卷 413-421页

作者： Liangping Xiao Rusen Zhou Tianqi Zhang Xiaoxiang Wang Renwu Zhou Patrick J.Cullen Kostya(Ken)Ostrikov Department of Physics Research Institute for Biomimetics and Soft MatterFujian Provincial Key Laboratory for Soft Functional MaterialsJiujiang Research InstituteXiamen UniversityXiamen 361005China School of Chemistry and Physics QUT Centre for Materials Science and QUT Centre for a Waste-Free WorldQueensland University of Technology(QUT)Brisbane QLD 4000Australia School of Chemical and Biomolecular Engineering University of SydneySydney NSW 2006Australia

Ever-increasing emissions of anthropogenic carbon dioxide(CO_(2))cause global environmental and climate *** by biological photosynthesis,developing effective strategies NeuNlto up-cycle CO_(2)into high-value organics is *** CO_(2)reduction reaction(CO_(2)RR)is highly promising to convert CO_(2)into economically viable carbon-based chemicals or fuels under mild process ***,mesoporous indium supported on multi-walled carbon nanotubes(mp-In@MWCNTs)is synthesized via a facile wet chemical *** mp-In@MWCNTs electrocatalysts exhibit high CO_(2)RR performance in reducing CO_(2)into *** outstanding activity(current density-78.5 mA cm^(-2)),high conversion efficiency(Faradaic efficiency of formate over 90%),and persistent stability(∼30 h)for selective CO_(2)-to-formate conversion are *** outstanding CO_(2)RR process performance is attributed to the unique structures with mesoporous surfaces and a conductive network,which promote the adsorption and desorption of reactants and intermediates while improving electron *** findings provide guiding principles for synthesizing conductive metal-based electrocatalysts for high-performance CO_(2)conversion.

关键词： CO_(2)RR conductive network electrocatalysts formate

来源：评论

学校读者我要写书评

暂无评论

High glass transition temperature dopant-free hole transport material via D-A-π-A-D-strategy for perovskite solar cell

引用

Rare Metals 2024年第12期43卷 6373-6383页

作者： Cheng-Hui Liao Li-Gang Yuan Yi-Heng Zhang Wei-Ya Zhu Min-Chao Qin Zhi-Bo He Jie-Lin Huang Hao-Lin Xiao Zhi-Heng Li Xin-Hui Lu Ke-You Yan Yuan Li State Key Laboratory of Luminescent Materials and Devices Institute of Polymer Optoelectronic Materials and DevicesSchool of Materials Science and EngineeringSouth China University of TechnologyGuangzhou510640China School of Environment and Energy State Key Laboratory of Luminescent Materials and DevicesGuangdong Provincial Key Laboratory of Solid Wastes Pollution Control and RecyclingSouth China University of TechnologyGuangzhou510000China Department of Physics The Chinese University of Hong KongHong Kong999077China

Despite the great leap forward perovskite solar cells(PSCs)have achieved in power conversion efficiency,the device instability remains one of the major problems plaguing its ***-free hole transport material(HTM)has been widely studied as an important strategy to improve the stability of PSCs due to its avoidance of moisture-sensitive dopants and cumbersome doping *** this work,a series of dopant-free HTMs L1F,L2F and L3F based on D-A-π-A-D configuration were synthesized through two steps of reaction.L3F presents a high glass transition temperature of 1800C and thermal decomposition temperature of ***,electron paramagnetic resonance signals of L1F,L2F and L3F powders indicate the open-shell quinoidal diradical resonance structure in their aggregation state due to aggregation-induced radical *** these HTMs present higher hole mobility than dopant-free Spiro-OMeTAD,and the dopant-free L3F-based PSC device achieves the highest power conversion efficiency of 17.6%among *** addition,due to the high hydrophobic properties of L1F,L2F and L3F,the perovskite films spin-coated with these HTMs exhibit higher humidity stability than doped *** results demonstrate a promising design strategy for high glass transition temperature dopant-free hole transport *** open-shell quinoid-radical organic semiconductors are not rational candidates for dopant-free HTMs for PSC devices.

关键词： Perovskite solar cells Dopant-free Hole transport materials D-A-π-A-D High glass transition temperature

来源：评论

学校读者我要写书评

暂无评论

Over 18.2% efficiency of layer–by–layer all–polymer solar cells enabled by homoleptic iridium(Ⅲ)carbene complex as solid additive

引用

science Bulletin 2024年第18期69卷 2862-2869页

作者： Hang Zhou Yingjie Sun Miao Zhang Yuheng Ni Fenghua Zhang Sang Young Jeong Tianhuan Huang Xiong Li Han Young Woo Jian Zhang Wai-Yeung Wong Xiaoling Ma Fujun Zhang Key Laboratory of Luminescence and Optical Information(Ministry of Education) Beijing Jiaotong UniversityBeijing 100044China Department of Applied Biology and Chemical Technology and Research Institute for Smart Energy The Hong Kong Polytechnic UniversityHong Kong 999077China Department of Physics Beijing Technology and Business UniversityBeijing 100048China Organic Optoelectronic Materials Laboratory Department of ChemistryCollege of ScienceKorea UniversitySeoul 02841Republic of Korea School of Materials Science and Engineering Engineering Research Center of Electronic Information Materials and DevicesMinistry of EducationGuangxi Key Laboratory of Information MaterialsGuilin University of Electronic TechnologyGuilin 541004China Tangshan Research Institute of Beijing Jiaotong University Tangshan 063000China

The vertical phase distribution of active layers plays a vital role in balancing exciton dissociation and cha rge transport for achieving efficient polymer solar cells(PSCs).The layer-by-layer(LbL)PSCs are commonly prepared by using sequential spin-coating method from donor and acceptor solutions with distinct solvents and solvent *** enhanced exciton dissociation is expected in the LbL PSCs with efficient charge transport in the relatively neat donor or acceptor *** this work,a series of LbL all-polymer solar cells(APSCs)were fabricated with PM6 as donor and PY-DT as acceptor,and triplet material m-Ir(CPmPB)_(3)is deliberately incorporated into PY-DT layer to prolong exciton lifetimes of active *** power conversion efficiency(PCE)of LbL APSCs is improved to 18.24%from 17.32%by incorporating 0.3 wt%m-Ir(CPMPB)_(3)in PY-DT layer,benefiting from the simultaneously enhanced short-circuit current density(Isc)of 25.17 mA cm^(-2)and fill factor(FF)of 74.70%.The enhancement of PCE is attributed to the efficient energy transfer of m-Ir(CPmPB)_(3)to PM6 and PY-DT,resulting in the prolonged exciton lifetime in the active layer and the increased exciton diffusion *** efficient energy transfer from m-Ir(CPmPB)_(3)to PM6 and PY-DT layer can be confirmed by the increased photoluminescence(PL)intensity and the prolonged PL lifetime of PM6 and PY-DT in PM6+m-Ir(CPmPB)_(3)and PY-DT+m-Ir(CPmPB)_(3)*** study indicates that the triplet material as solid additive has great potential in fabricating efficient LbL APSCs by prolonging exciton lifetimes in active layers.

关键词： Layer-by-layer All-polymer solar cells Additive strategy Triplet material Energy transfer

来源：评论

学校读者我要写书评

暂无评论

Ultrathin NiO/Ni_(3)S_(2)Heterostructure as Electrocatalyst for Accelerated Polysulfide Conversion in Lithium-Sulfur Batteries

引用

Energy & Environmental materials 2023年第6期6卷 182-190页

作者： Chunqiao Jin Pengbo Zhai Jianli Tang Liuxiang Huo Qianqian He Yan Ye Lingxi Qiu Kai Jiang Liyan Shang Yawei Li Yongji Gong Zhigao Hu Junhao Chu Department of Materials School of Physics and Electronic ScienceTechnical Center for Multifunctional Magneto-Optical Spectroscopy(Shanghai)Engineering Research Center of Nanophotonics&Advanced Instrument(Ministry of Education)East China Normal UniversityShanghai 200241China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan Shanxi 030006China School of Materials Science and Engineering Beihang UniversityBeijing 100191China

The practical application of Lithium-Sulfur batteries largely depends on highly efficient utilization and conversion of sulfur under the realistic condition of high-sulfur content and low electrolyte/sulfur *** design of heterostructure electrocatalysts with abundant active sites and strong interfacial electronic interactions is a promising but still challenging strategy for preventing shuttling of polysulfides in lithium-sulfur ***,ultrathin nonlayered NiO/Ni_(3)S_(2)heterostructure nanosheets are developed through topochemical transformation of layered Ni(OH)_(2)templates to improve the utilization of sulfur and facilitate stable cycling of *** a multifunction catalyst,NiO/Ni_(3)S_(2)not only enhances the adsorption of polysulfides and shorten the transport path of Li ions and electrons but also promotes the Li_(2)S formation and transformation,which are verified by both in-situ Raman spectroscopy and electrochemical ***,the cell with NiO/Ni_(3)S_(2)as electrocatalyst delivers an area capacity of 4.8 mAh cm^(-2)under the high sulfur loading(6 mg cm^(-2))and low electrolyte/sulfur ratio(4.3 pL mg^(-1)).The strategy can be extended to 2D Ni foil,demonstrating its prospects in the construction of electrodes with high gravimetric/volumetric energy *** designed electrocatalyst of ultrathin nonlayered heterostructure will shed light on achieving high energy density lithium-sulfur batteries.

关键词： density functional theory simulation Li-S batteries multifunction electrocatalyst NiO/Ni_(3)S_(2)heterostructures ultrathin nonlayered nanosheets

来源：评论

学校读者我要写书评

暂无评论

A Review of the Application of Digital Image Correlation to Micromechanical Studies of Polymer Electrolytes 2

A Review of the Application of Digital Image Correlation to ...

引用

2nd International Conference on Multidisciplinary engineering and Applied science, ICMEAS 2023

作者： Obi, Uchenna C. Sanni, Dahiru Abraham, Bernice Adeniji, Sharafadeen A. Offia-Kalu, Nkechi E. Amune, Daniel Anye, Vitalis C. Bello, Abdulhakeem African University of Science and Technology Department of Materials Science and Engineering Abuja Nigeria Nile University Department of Physics Abuja Nigeria African University of Science and Technology Theoretical and Applied Physics Abuja Nigeria

ISBN: (纸本)9798350358834

High-performing lithium-ion batteries (LIBs) necessitate a stable solid electrolyte. When batteries are subjected to external loads, the electrolytes in LIBs are susceptible to irregular deformation distributions, which may result in an asymmetrical porosity distribution. Therefore, these electrolytes must be mechanically robust to withstand pressures and loads, such as significant volumetric changes in anode materials, as well as to prevent dendrite formation, which reduces their efficiency and extends LIB's lifespan. Numerous research methods and tools have been used to examine the mechanical characteristics of LIB components, including tensile, compression, flexural, hardness, and viscoelasticity experiments conducted using the universal testing machine and nanoindentation machine. However, this study discusses the digital image correlation (DIC) technique to examine the mechanical properties of solid electrolytes on a microscopic scale and how this technique has been and can be successfully used to improve our understanding of the strain distribution and effects on LIBs when the solid electrolyte is loaded. © 2023 IEEE.

关键词： Lithium-ion batteries

来源：评论

学校读者我要写书评

暂无评论

Comparative Study of the Effects of Nano ZnO and CuO on the Biodegradation,Biocompatibility,and Antibacterial Properties of Micro-arc Oxidation Coating of Magnesium Alloy

引用

Acta Metallurgica Sinica(English Letters) 2024年第2期37卷 242-254页

作者： Ying Shen Xianfeng Shan Iniobong P.Etim Muhammad Ali Siddiqui Yang Yang Zewen Shi Xuping Su Junxiu Chen Key Laboratory of Materials Surface Science and Technology of Jiangsu Province Changzhou UniversityChangzhou213164China Department of Stomatology The Affiliated Xinhua Hospital of Dalian UniversityDalian116000China Department of Physics University of CalabarCalabar540242Nigeria Metallurgical Engineering Department NED University of Engineering and TechnologyUniversity RoadKarachi75270Pakistan Ningbo No.2 Hospital Ningbo315010China

This research systematically examined the degradation,antibacterial effects,and biocompatibility of micro-arc oxidation(MAO)coatings with nano CuO and ZnO on extruded Mg *** copper(Cu)and Zinc(Zn)possess antibacterial *** findings demonstrated that adding ZnO will appreciably reduce the degradation rate of MAO-coating alloy due to the self-sealing micro ***+MAO coating exhibited excellent antibacterial performance,with an antibacterial rate of over 90%within 6 h co-cultured with Staphylococcus ***,the antibacterial rate of ZnO+MAO coating reached 90%after 12 h *** test using MG63 cell indicated that the incorporation of CuO and ZnO did not notably affect the cell viability rate of the ***,after 14 days of culture,the CuO+MAO and ZnO+MAO coated samples exhibited higher alkaline phosphatase(ALP)activity than the MAO-coated and uncoated samples,suggesting favorable osteogenic properties.

关键词： Copper oxide Zinc oxide Micro-arc oxidation(MAO)coating Corrosion behavior Antibacterial characteristics

来源：评论

学校读者我要写书评

暂无评论

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案：

请选择收藏分类：

通借通还

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：