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arXiv 2022年

作者： Hou, Jin Li, Wenbin Zhang, Hao Sidhik, Siraj Blancon, Jean-Christophe Even, Jacky Kanatzidis, Mercouri G. Mohite, Aditya D. Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Department of Chemical and Biomolecular Engineering Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley‐Curl Institute Rice University HoustonTX77005 United States INSA de Rennes CNRS UMR 6082 Rennes35708 France Department of Chemistry Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States

Two-dimensional (2D) halide perovskites have emerged as semiconductor platforms for realizing efficient and durable optoelectronic devices. However, the reproducible synthesis of 2D perovskite crystals with desired layer thickness (or n value) greater than 2, has been an enduring challenge due to the lack of kinetic control (temperature, time, stoichiometry) for each layer thickness. Here, we demonstrate a novel method term as the kinetically controlled space confinement (KCSC) for the deterministic growth of phase pure Ruddlesden-Popper (RP) and Dion-Jacobson (DJ) 2D perovskites. The phase-pure growth was achieved by progressively increasing the temperature (fixed time) or the crystallization time (fixed temperature), which allowed for an acute control of the crystallization kinetics. We also observe a systematic transformation from a lower n-value to n=3, 4, 5, 6 in 2D perovskites. In-situ photoluminescence spectroscopy and imaging suggest that the progressive transformation from lower to higher n-value occurs via intercalation of excess precursor ions. These experiments enabled the development of a machine learning assisted multi-parameter phase diagram, which predicts the growth of 2D phase with a specific n-value. © 2022, CC BY.

关键词： Perovskite

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Chiral anomaly and Weyl orbit in three-dimensional Dirac semimetal Cd3As2 grown on Si

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Nanotechnology 2024年第16期35卷 165002-165002页

作者： Lin, Wei-Chen Tsai, Peng-Ying Zou, Jia-Zhu Lee, Jie-Ying Kuo, Chun-Wei Lee, Hsin-Hsuan Pan, Ching-Yang Yang, Cheng-Hsueh Chen, Sheng-Zong Wang, Jyh-Shyang Jiang, Pei-Hsun Liang, Chi-Te Chuang, Chiashain Taiwan International Graduate Program Academia Sinica Taipei115 Taiwan Department of Engineering and System Science National Tsing Hua University Hsinchu300 Taiwan Graduate Institute of Applied Physics National Taiwan University Taipei106 Taiwan National Taiwan University Taipei106 Taiwan Department of Electronic Engineering Chung Yuan Christian University Taoyuan320 Taiwan Department of Physics Chung Yuan Christian University Taoyuan320 Taiwan Department of Physics National Taiwan Normal University 106 Taiwan Research Center for Semiconductor Materials and Advanced Optics Chung Yuan Christian University Taoyuan320 Taiwan

Preparing Cd3As2, which is a three-dimensional (3D) Dirac semimetal in certain crystal orientation, on Si is highly desirable as such a sample may well be fully compatible with existing Si CMOS technology. However, there is a dearth of such a study regarding Cd3As2 films grown on Si showing the chiral anomaly. Here, for the first time, we report the novel preparation and fabrication technique of a Cd3As2 (112) film on a Si (111) substrate with a ZnTe (111) buffer layer which explicitly shows the chiral anomaly with a nontrivial Berry’s phase of π. Despite the Hall carrier density ( n 3 D ≈ 9.42 × 10 17 cm−3) of our Cd3As2 film, which is almost beyond the limit for the portents of a 3D Dirac semimetal to emerge, we observe large linear magnetoresistance in a perpendicular magnetic field and negative magnetoresistance in a parallel magnetic field. These results clearly demonstrate the chiral magnetic effect and 3D Dirac semimetallic behavior in our silicon-based Cd3As2 film. Our tailoring growth of Cd3As2 on a conventional substrate such as Si keeps the sample quality, while also achieving a low carrier concentration. © 2024 IOP Publishing Ltd.

关键词： II-VI semiconductors

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Improving the Performance of Asphalt Mixtures with Highly Acidic Aggregates in Central Vietnam Using Modifier Based on Styrene-Butadiene-Styrene and Rosin Resin

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Journal of materials in Civil engineering 2025年第7期37卷

作者： Nguyen, Lan Ngoc Lee, Hosin David Bui, Lam Tung Kim, Young-Ik Truong, Van Quyet Nguyen, May Huu Nguyen, Du Van Dept. of Construction Materials Faculty of Construction Engineering Univ. of Transport and Communications No. 03 Cau Giay Hanoi100000 Viet Nam Dept. of Civil and Environmental Engineering Iowa Technology Institute The Univ. of Iowa Iowa CityIA52242 United States Research Dept. Hansoo Natech Co. Ltd. 6-20 Yuseong-daero 1205beon-gil Yuseong-gu Daejeon34104 Korea Republic of Civil and Environmental Engineering Program Graduate School of Advanced Science and Engineering Hiroshima Univ. 1-4-1 Kagamiyama Higashi-Hiroshima Hiroshima739-8527 Japan Faculty of Civil Engineering Univ. of Transport and Communications Campus in Ho Chi Minh City Ho Chi Minh City700000 Viet Nam

In Central Vietnam, the aggregate typically originates from highly acidic rocks containing a significant amount of silicon dioxide (SiO2), leading to poor adhesion quality with virgin asphalt binder. Hence, the asphalt mixture production usually needs to utilize adhesion promoters. Based on the chemical compositions of the sample aggregate (up to 72.3% SiO2), research has been conducted to introduce an adhesive agent called rubber modified compound (RMC-160), which is composed of styrene-butadiene-styrene (SBS) with petroleum hydrocarbon resin, treated clay and mineral oil. This article presents the research findings regarding the adhesion effectiveness of RMC-160-modified asphalt binder to high acid-based aggregate through laboratory and field tests, along with the mixture performance under both short-term oven aging (STOA) and long-term oven aging (LTOA). The test results exhibited remarkable effects, whereby the asphalt binder modified with RMC-160 additive significantly increased the adhesion level from Grade 2 to Grade 4, and the asphalt mixtures containing RMC-160 had lower rutting and higher cracking tolerance (CTIndex) under both the STOA and LTOA conditions. © 2025 American Society of Civil Engineers.

关键词： Silicon oxides

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Development of high on/off current ratio in p-type copper oxide thin-film transistors with a back-end-of-line compatible process

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Journal of Vacuum science and Technology A: Vacuum, Surfaces and Films 2024年第5期42卷

作者： Kuo, Chi-Yuan Lin, Wei-Chen Lo, Tsung-Tien Shen, Ching-Hsuan Shen, Ming-Yu Lee, Chia-Chan Lin, Chi-Ping Lin, Yuang-Ming Huang, Haw-Tyng Yeh, Po-Chun Chen, Hsin-Chu Wu, Chih-I Graduate Institute of Photonics and Optoelectronic Department of Electrical Engineering National Taiwan University Taipei106 Taiwan Program of Quantum Technology and Advanced Material College of Science National Tsing Hua University Hsinchu300 Taiwan Institute of Innovative Semiconductor Manufacturing National Sun Yat-sen University Kaohsiung804 Taiwan Institute of Advanced Semiconductor Packaging and Testing National Sun Yat-sen University Kaohsiung804 Taiwan Department of Materials Science and Engineering National Taiwan University Taipei106 Taiwan Electronic and Optoelectronic System Research Laboratories Industrial Technology Research Institute Hsinchu300 Taiwan

The objective of this study is to develop an efficient process to synthesize wafer scale p-type cuprous oxide (Cu2O) with the back-end-of-line (BEOL) compatible process (2/Si substrates followed by rapid thermal oxidation to oxidize it into large-area, uniform Cu2O. Bottom-gate Cu2O thin-film transistors (TFTs) were fabricated as gate dielectric on 100 nm thermal oxide. The results of the ID-VG curve demonstrate that we have successfully fabricated BEOL-compatible p-type Cu2O TFTs. The drain-off current can be achieved to 0.1 pA, with the highest on/off ratio reaching up to 6 orders. Significantly, the TFT with an on/off ratio of 106 is sufficient to meet the requirements for digital circuit applications, including logic circuits, and the BEOL-compatible process (2O TFTs. © 2024 Author(s).

关键词： Thin film transistors

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Injectable cross-linked hyaluronic acid hydrogels with epigallocatechin gallate loading as vitreous substitutes

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International Journal of Biological Macromolecules 2024年第Part1期275卷 133467页

作者： Chen, Huai-An Tai, Yi-Ning Hsieh, Erh-Hsuan Thacker, Minal Lin, I-Chan Tseng, Ching-Li Lin, Feng-Huei Graduate Institute of Biomedical Materials and Tissue Engineering College of Biomedical Engineering Taipei Medical University Shuang-Ho Campus New Taipei City Taiwan Institute of Biomedical Engineering College of Medicine & College of Engineering National Taiwan University Taipei City Taiwan 17W Hong Kong Science Park Hong Kong Department of Ophthalmology Wan Fang Hospital Taipei Medical University Taipei City Taiwan Department of Ophthalmology School of Medicine College of Medicine Taipei Medical University Taipei City Taiwan International Ph. D. Program in Biomedical Engineering College of Biomedical Engineering Taipei Medical University Shuang-Ho Campus New Taipei City Taiwan Research Center of Biomedical Device College of Biomedical Engineering Taipei Medical University Taipei City Taiwan International Ph. D. Program in Cell Therapy and Regenerative Medicine College of Medicine Taipei Medical University Taipei City Taiwan National Health Research Institutes Miaoli County Taiwan

Hyaluronic acid (HA) serves as a vitreous substitute owing to its ability to mimic the physical functions of native vitreous humor. However, pure HA hydrogels alone do not provide sufficient protection against potential inflammatory risks following vitrectomy. In this study, HA was crosslinked with 1,4-butanediol diglycidyl ether (BDDE) to form HA hydrogels (HB). Subsequently, the anti-inflammatory agent epigallocatechin gallate (EGCG) was added to the hydrogel (HBE) for ophthalmic applications as a vitreous substitute. The characterization results indicated the successful preparation of HB with transparency, refractive index, and osmolality similar to those of native vitreous humor, and with good injectability. The anti-inflammatory ability of HBE was also confirmed by the reduced expression of inflammatory genes in retinal pigment epithelial cells treated with HBE compared with those treated with HB. In a New Zealand white rabbit model undergoing vitreous substitution treatment, HBE 50 (EGCG 50 μM addition) exhibited positive results at 28 days post-surgery. These outcomes included restored intraocular pressure, improved electroretinogram responses, minimal increase in corneal thickness, and no inflammation during histological examination. This study demonstrated the potential of an injectable HA-BDDE cross-linked hydrogel containing EGCG as a vitreous substitute for vitrectomy applications, offering prolonged degradation time and anti-inflammatory effects postoperatively. © 2024 The Authors

关键词： Hyaluronic acid

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High‑Performance Thick Cathode Based on Polyhydroxyalkanoate Binder for Li Metal Batteries

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Advanced Fiber materials 2024年第1期6卷 214-228页

作者： Dong Hyuk Kang Minhyuck Park Jeonghun Lee Chan Yeol Kim Jimin Park Youn‑Ki Lee Jong Chan Hyun Son Ha Jin Hwan Kwak Juhee Yoon Hyemin Kim Hyun Soo Kim Do Hyun Kim Sangmin Kim Ji Yong Park Robin Jang Seung Jae Yang Hee‑Dae Lim Se Youn Cho Hyoung‑Joon Jin Seungjin Lee Yunil Hwang Young Soo Yun KU‑KIST Graduate School of Converging Science and Technology Korea University145 Anam‑roSeongbuk‑guSeoul 02841South Korea Carbon Composite Materials Research Center Korea Institute of Science and Technology(KIST)92 Chundong‑roBongdong‑eupWanju‑gunJeollabuk‑do 55324South Korea Energy Storage Research Center Korea Institute of Science and Technology(KIST)514‑gil Hwaraong‑roSeoul 02792South Korea Program in Environmental and Polymer Engineering Inha University100 Inha‑ro Michuhol‑guIncheon 22212South Korea Advanced Analysis Data Center Korea Institute of Science and Technology(KIST)514‑gil Hwaraong‑roSeoul 02792South Korea Advanced Nanohybrids Laboratory Department of Chemistry and Chemical EngineeringInha University100 Inha‑roMichuhol‑guIncheon 22212South Korea CJ CheilJedang Corporation 55 Gwanggyo‑ro 42Beon‑gilYeongtong‑guSuwon 16495South Korea Department of Chemical Engineering Hanyang University222 Wangsimni‑roSeongdong‑guSeoul 04763South Korea Department of Integrative Energy Engineering Korea University145 Anam‑roSeongbuk‑guSeoul 02841South Korea

Thick cathodes can overcome the low capacity issues,which mostly hamper the performance of the conventional active cathode materials,used in rechargeable Li ***,the typical slurry-based method induces cracking and flaking during the fabrication of thick *** addition,a significant increase in the charge-transfer resistance and local cur-rent overload results in poor rate capabilities and cycling stabilities,thereby limiting electrode *** this study,a synergistic dual-network combination strategy based on a conductive nanofibrillar network(CNN)and a nano-bridging amor-phous polyhydroxyalkanoate(aPHA)binder is used to demonstrate the feasibility of constructing a high-performance thick *** CNN and aPHA dual network facilitates the fabrication of a thick cathode(≥250μm thickness and≥90 wt%active cathode material)by a mass-producible slurry *** thick cathode exhibited a high rate capability and excel-lent cycling *** addition,the thick cathode and thin Li metal anode pair(Li//t-NCM)exhibited an optimal energy performance,affording high-performance Li metal batteries with a high areal energy of~25.3 mW h cm^(-2),a high volumetric power density of~1720 W L^(-1),and an outstanding specific energy of~470 W h kg^(-1)at only 6 mA h cm^(-2).

关键词： Thick cathode Polyhydroxyalkanoate binder Nano-bridging Conductive nano-fibrillar network Lithium metal battery

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Manipulating Fano coupling in an opto-thermoelectric field

arXiv

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arXiv 2024年

作者： Lin, Linhan Lepeshov, Sergey Krasnok, Alex Huang, Yu Jiang, Taizhi Peng, Xiaolei Korgel, Brian A. Alu, Andrea Zheng, Yuebing State Key Laboratory of Precision Measurement Technology and Instruments Department of Precision Instrument Tsinghua University Beijing100084 China Department of Electrical and Photonics Engineering DTU Electro Technical University of Denmark Building 343 Kgs. LyngbyDK-2800 Denmark Department of Electrical and Computer Engineering Florida International University MiamiFL33174 United States School of Physics and Electronics Hunan University Changsha410082 China Mc Ketta Department of Chemical Engineering The University of Texas at Austin AustinTX78712 United States Materials Science & Engineering Program Texas Materials Institute The University of Texas at Austin AustinTX78712 United States Department of Electrical and Computer Engineering The University of Texas at Austin AustinTX78712 United States Advanced Science Research Center City University of New York New YorkNY10031 United States Physics Program Graduate Center City University of New York NY10016 United States Walker Department of Mechanical Engineering The University of Texas at Austin AustinTX78712 United States

Fano resonances in photonics arise from the coupling and interference between two resonant modes in structures with broken symmetry. They feature an uneven and narrow and tunable lineshape, and are ideally suited for optical spectroscopy. Many Fano resonance structures have been suggested in nanophotonics over the last ten years, but reconfigurability and tailored design remain challenging. Herein, we propose an all-optical "pick-and-place" approach aimed at assemble Fano metamolecules of various geometries and compositions in a reconfigurable manner. We study their coupling behavior by in-situ dark-field scattering spectroscopy. Driven by a light-directed opto-thermoelectric field, silicon nanoparticles with high quality-factor Mie resonances (discrete states) and low-loss BaTiO3 nanoparticles (continuum states) are assembled into all-dielectric heterodimers, where distinct Fano resonances are observed. The Fano parameter can be adjusted by changing the resonant frequency of the discrete states or the light polarization. We also show tunable coupling strength and multiple Fano resonances by altering the number of continuum states and discrete states in dielectric heterooligomers. Our work offers a general design rule for Fano resonance and an all-optical platform for controlling Fano coupling on demand. Copyright © 2024, The Authors. All rights reserved.

关键词： Light polarization

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Generative Chemical Transformer: Neural Machine Learning of Molecular Geometric Structures from Chemical Language via Attention

arXiv

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arXiv 2021年

作者： Kim, Hyunseung Na, Jonggeol Lee, Won Bo School of Chemical and Biological Engineering Seoul National University Gwanak-ro 1 Gwanak-gu Seoul08826 Korea Republic of Department of Chemical Engineering and Materials Science Graduate Program in System Health Science and Engineering Ewha Womans University Seoul03760 Korea Republic of

Discovering new materials better suited to specific purposes is an important issue in improving the quality of human life. Here, a neural network that creates molecules that meet some desired conditions based on a deep understanding of chemical language is proposed (Generative Chemical Transformer, GCT). The attention mechanism in GCT allows a deeper understanding of molecular structures beyond the limitations of chemical language itself which cause semantic discontinuity by paying attention to characters sparsely. It is investigated that the significance of language models for inverse molecular design problems by quantitatively evaluating the quality of the generated molecules. GCT generates highly realistic chemical strings that satisfy both chemical and linguistic grammar rules. Molecules parsed from generated strings simultaneously satisfy the multiple target properties and vary for a single condition set. These advances will contribute to improving the quality of human life by accelerating the process of desired material discovery. Copyright © 2021, The Authors. All rights reserved.

关键词： Molecules

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Deformed Fredkin model for the ν=5/2 Moore-Read state on thin cylinders

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Physical Review Research 2024年第1期6卷 013105-013105页

作者： Cristian Voinea Songyang Pu Ammar Kirmani Pouyan Ghaemi Armin Rahmani Zlatko Papić School of Physics and Astronomy University of Leeds Leeds LS2 9JT United Kingdom Theoretical Division T-4 Los Alamos National Laboratory Los Alamos New Mexico 87545 USA Physics Department City College of the City University of New York New York 10031 USA Physics Program Graduate Center of City University of New York New York 10031 USA Department of Physics and Astronomy and Advanced Materials Science and Engineering Center Western Washington University Bellingham Washington 98225 USA

We propose a frustration-free model for the Moore-Read quantum Hall state on sufficiently thin cylinders with circumferences ≲7 magnetic lengths. While the Moore-Read Hamiltonian involves complicated long-range interactions between triplets of electrons in a Landau level, our effective model is a simpler one-dimensional chain of qubits with deformed Fredkin gates. We show that the ground state of the Fredkin model has high overlap with the Moore-Read wave function and accurately reproduces the latter's entanglement properties. Moreover, we demonstrate that the model captures the dynamical response of the Moore-Read state to a geometric quench, induced by suddenly changing the anisotropy of the system. We elucidate the underlying mechanism of the quench dynamics and show that it coincides with the linearized bimetric field theory. The minimal model introduced here can be directly implemented as a first step towards quantum simulation of the Moore-Read state, as we demonstrate by deriving an efficient circuit approximation to the ground state and implementing it on an IBM quantum processor.

关键词： Fractional quantum Hall effect Quantum computation Quantum many-body systems Strongly correlated systems Exact diagonalization Matrix product states

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Analytical modeling and decoupling of humidity effects in nanomechanical sensing based on sorption kinetics and viscoelastic stress relaxation

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Physical Review E 2025年第6期111卷 065407-065407页

作者： Meng-Qun Feng Kosuke Minami Yingcheng Zhou Genki Yoshikawa Research Center for Macromolecules and Biomaterials National Institute for Materials Science (NIMS) 1-1 Namiki Tsukuba Ibaraki 305-0044 Japan Materials Science and Engineering Graduate School of Pure and Applied Science University of Tsukuba 1-1-1 Tennodai Tsukuba Ibaraki 305-8571 Japan International Center for Young Scientists (ICYS) National Institute for Materials Science (NIMS) 1-1 Namiki Tsukuba Ibaraki 305-0044 Japan

Nanomechanical sensors have gained significant attention as powerful tools for detecting target analytes; however, their signals are often influenced by environmental humidity. In static mode operation, the sensing signals of nanomechanical sensors are obtained by a concentration-dependent sorption-induced mechanical strain/stress. In this study, we derive an analytical model to describe the response of viscoelastic material-coated nanomechanical sensors by incorporating humidity effects based on sorption kinetics and viscoelastic stress relaxation of receptor materials. This model is capable of reproducing the dynamic responses observed in the experiments under varying humidity conditions. Moreover, it allows for the subtraction of humidity effects, facilitating the precise isolation of analyte-specific signals. These results provide a theoretical framework for decoupling environmental background factors, such as humidity effects, in nanomechanical sensors.

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