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Frontiers in Optics + Laser Science 2021, FiO+LS 2021 - Part of Frontiers in Optics, FiO 2021

作者： Boddeti, Ashwin K. Guan, Jun Sentz, Tyler Juarez, Xitali Newman, Ward Cortes, Cristian Odom, Teri W. Jacob, Zubin School of Electrical and Computer Engineering Birck Nanotechnology Center Purdue University West LafayetteIN47907 United States Graduate Program in Applied Physics Northwestern University EvanstonIL60208 United States Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States Intel Corporation BeavertonOR97007 United States Center for Nanoscale Materials Argonne National Laboratory LemontIL60439 United States Graduate Program in Applied Physics Department of Materials Science and Engineering Department of Chemistry Northwestern University EvanstonIL60208 United States

We observe long-range dipole-dipole interactions in a plasmonic lattice. Fluorescence lifetime measurements show density-dependent non-exponential decay dynamics over 800nm mean nearest-neighbour separation distances ... 详细信息

ISBN: (纸本)9781557528209

关键词： Plasmonics

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Nanoslot-Induced Ultrastrong Phonon-Photon and Phonon-Phonon Coupling in Hybrid Organic-Inorganic Perovskites 16

Nanoslot-Induced Ultrastrong Phonon-Photon and Phonon-Phonon...

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16th Pacific Rim Conference on Lasers and Electro-Optics, CLEO-PR 2024

作者： Kim, Dasom Hou, Jin Lee, Geon Agrawal, Ayush Kim, Sunghwan Zhang, Hao Bao, Di Baydin, Andrey Wu, Wenjing Tay, Fuyang Huang, Shengxi Hagenmüller, Daivd Chia, Elbert E. M. Kim, Dai-Sik Seo, Minah Mohite, Aditya D. Kono, Junichiro Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Sensor System Research Center Korea Institute of Science and Technology Seoul02792 Korea Republic of Department of Physics and Astronomy Seoul National University Seoul08826 Korea Republic of Department of Chemical and Biomolecular Engineering Rice University HoustonTX77005 United States Ulsan44919 Korea Republic of Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University 637371 Singapore Smalley-Curl Institute Rice University HoustonTX77005 United States Université de Strasbourg Cnrs Strasbourg67000 France KU-KIST Graduate School of Converging Science and Technology Korea University Seoul02841 Korea Republic of Department of Physics and Astronomy Rice University HoustonTX77005 United States

Methods for harnessing vibrational states are desired for phonon-based technologies. We realized ultrastrong coupling of two phonon modes in perovskite materials induced by ultrastrong coupling with a common photonic ... 详细信息

ISBN: (纸本)9798350372076

关键词： Organic-inorganic materials

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High-Order Nonlinear Electrophoresis in a Nematic Liquid Crystal

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Physical Review Letters 2024年第15期132卷 158102-158102页

作者： Mojtaba Rajabi Taras Turiv Bing-Xiang Li Hend Baza Dmitry Golovaty Oleg D. Lavrentovich Advanced Materials and Liquid Crystal Institute Kent State University Kent Ohio 44242 USA Department of Physics Kent State University Kent Ohio 44242 USA College of Electronic and Optical Engineering & College of Flexible Electronics (Future Technology) Nanjing University of Posts and Telecommunications Nanjing 210023 China Department of Mathematics The University of Akron Akron Ohio 44325-4002 USA Materials Science Graduate Program Kent State University Kent Ohio 44242 USA

Electrophoresis is the motion of particles relative to a surrounding fluid driven by a uniform electric field. In conventional electrophoresis, the electrophoretic velocity grows linearly with the applied field. Nonlinear effects with a quadratic speed vs field dependence are gaining research interest since an alternating current field could drive them. Here, we report on the giant nonlinearity of electrophoresis in a nematic liquid crystal in which the speed grows with the fourth and sixth powers of the electric field. The mechanism is attributed to the shear thinning of the nematic environment induced by the moving colloid. The observed giant nonlinear effect dramatically enhances the efficiency of electrophoretic transport.

关键词： Electrophoresis Non-Newtonian fluids Nonlinear dynamics in fluids Colloids Liquid crystals Nematic liquid crystals Optical microscopy Rheology techniques

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Transferable screened range-separated hybrid functionals for electronic and optical properties of van der Waals materials

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Physical Review materials 2023年第10期7卷 104001-104001页

作者： María Camarasa-Gómez Ashwin Ramasubramaniam Jeffrey B. Neaton Leeor Kronik Department of Molecular Chemistry and Materials Science Weizmann Institute of Science Rehovoth 7610001 Israel Department of Mechanical and Industrial Engineering University of Massachusetts Amherst Amherst Massachusetts 01003 USA Materials Science and Engineering Graduate Program University of Massachusetts Amherst Amherst Massachusetts 01003 USA Department of Physics University of California Berkeley California 94720 USA Materials Sciences Division Lawrence Berkeley National Laboratory Berkeley California 94720 USA Kavli Energy NanoSciences Institute at Berkeley University of California Berkeley California 94720 USA

The accurate description of electronic properties and optical absorption spectra is a long-standing challenge for density functional theory. Recently, the introduction of screened range-separated hybrid (SRSH) functionals for solid-state materials has allowed for the calculation of fundamental band gaps and optical absorption spectra that are in very good agreement with many-body perturbation theory. However, since solid-state SRSH functionals are typically tuned to reproduce the properties of bulk phases, their transferability to low-dimensional structures, which experience substantially different screening than in the bulk, remains an open question. In this work, we explore the transferability of SRSH functionals to several prototypical van der Waals materials, including transition-metal sulfides and selenides, indium selenide, black phosphorus, and hexagonal boron nitride. Considering the bulk and a monolayer of these materials as limiting cases, we show that the parameters of the SRSH functional can be determined systematically, using only the band-edge quasiparticle energies of these extremal structural phases as fitting targets. The resulting SRSH functionals can describe both electronic band structures and optical absorption spectra with accuracy comparable to more demanding ab initio many-body perturbation theory (GW and Bethe-Salpeter equation) approaches. Selected examples also demonstrate that the SRSH parameters, obtained from the bulk and monolayer reference structures, display good accuracy for band structures and optical spectra of bilayers, indicating a degree of transferability that is independent of the fitting procedure.

关键词： 2-dimensional systems Density functional theory First-principles calculations GW method

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TiCu-CMC/PDA coatings with long-term antimicrobial activity and cytocompatibility for surface engineering of implants

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Surface and Coatings Technology 2025年 509卷

作者： Zheng, Xiaosong Jiang, Yehao Zheng, Fazhan Xiang, Long Zhou, Lili Liang, Wenlang Huang, Nan Leng, Yongxiang Akhavan, Behnam Jing, Fengjuan Institute of Biomedical Engineering College of Medicine Southwest Jiaotong University Sichuan Chengdu610031 China Key Laboratory of Advanced Technologies of Materials Ministry of Education School of Materials Science and Engineering Southwest Jiaotong University Chengdu610031 China School of Engineering University of Newcastle CallaghanNSW2308 Australia Precision Medicine Program New Lambton HeightsNSW2305 Australia School of Biomedical Engineering University of Sydney SydneyNSW2006 Australia School of Physics University of Sydney SydneyNSW2006 Australia Sydney Nano Institute University of Sydney SydneyNSW2006 Australia

Long-term antibacterial effects and favourable biocompatibility are crucial to sustaining the long-term application of medical devices such as cardiac implantable devices, orthopedic devices, hernia meshes, and catheters. This study reports the development of sodium carboxymethyl cellulose/polydopamine films on Ti[sbnd]Cu coatings (TiCu-CMC/PDA) with long-term antimicrobial effects and cytocompatibility for surface engineering of implants. The TiCu-CMC/PDA coatings demonstrate sustained antimicrobial efficacy, maintaining bacterial inhibition rates above 99.6 % after aging in simulated body fluid (SBF) at 37 °C for 60 days. This remarkable antibacterial performance is primarily driven by the controlled release of copper ions during aging, complemented by surface copper's contribution to antimicrobial effects. Further, the TiCu-CMC/PDA coatings exhibit high cell viability and proliferation with negligible cytotoxicity, attributed to the regulated copper ion release. However, the endothelial cell viability on TiCu-CMC/PDA coatings decreased with aging due to the formation of copper ion complexes and CuO/Cu(OH)2, as well as increased surface roughness and hydrophilicity over time. The technology offers a simple and controllable approach to fabricating TiCu-CMC/PDA coatings, providing a pathway for the design of long-term antibacterial biomedical devices, including cardiovascular and orthopedic implants. © 2024

关键词： Antibiotics

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Supplementary information for "Low-loss silicon nitride Kerr-microresonators fabricated with metallic etch masks via metal lift-off"

arXiv

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arXiv 2025年

作者： Colación, Gabriel M. Rukh, Lala Buck, Franco Drake, Tara E. Optical Science & Engineering Program University of New Mexico AlbuquerqueNM87106 United States Center for High Technology Materials University of New Mexico AlbuquerqueNM87106 United States Department of Physics & Astronomy University of New Mexico AlbuquerqueNM87106 United States

Stoichiometric silicon nitride has emerged as a widely used integratedphotonic material owing to its high index of refraction, nonlinear opticalproperties, and broad transparency window spanning visible to mid-IRfrequencies. However, silicon nitride is generally more resistant to reactiveion etching than are typical etch masks made of polymer-based resist. Thisnecessitates resist layers that are significantly thicker than the siliconnitride and results in mask patterns which are tall and narrow. Thesehigh-aspect-ratio patterns inhibit the plasma transport of reactive ionetching, which leads to difficulties in accurately reproducing dimensions andcreating well-defined, vertical waveguide sidewalls. In this work, we overcomethese challenges by developing a metallic etch mask that provides a 30:1nitride-to-metal etch rate ratio, representing a near 20-fold reduction in therequired mask thickness. We demonstrate the quality of this technique byetching microring resonators with near-vertical waveguide sidewalls andintrinsic quality factors of over 1 million. Leveraging the low optical loss ofour resonators, we generate optical frequency combs with more than an octave ofbandwidth and dual dispersive waves. These results establish metal lift-off asa viable and easy-to-implement technique capable of producing low optical losswaveguides. © 2025, CC BY.

关键词： Aspect ratio

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Optimization of Printing Parameters for Printing of Ordinary Portland Cement using a Custom-made 3D Printer 21

Optimization of Printing Parameters for Printing of Ordinary...

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21st International Union of materials Research Societies International Conference in Asia, IUMRS-ICA 2021

作者： Chaiyotha, D. Pinitsoontorn, S. Chindaprasirt, P. Payakaniti, P. Materials Science and Nanotechnology Program Department of Physics Faculty of Science Khon Kaen University Khon Kaen40002 Thailand NANOTEC -KKU RNN on Nanomaterials Research and Innovation for Energy Khon Kaen University Khon Kaen40002 Thailand Sustainable Infrastructure Research and Development Center Department of Civil Engineering Faculty of Engineering Khon Kaen University Khon Kaen40002 Thailand

3D printing techniques have recently received a lot of attention as a new technique for forming construction materials, due to benefits over the traditional cast. In this research, ordinary Portland cement (OPC) paste was formed using a 3D extruder. Optimized mixture and printing parameters were determined. Compressive strengths of the printed and the traditionally casted OPC paste were measured after the specimens were cured in saturated limewater for 7, 14 and 28 days, respectively. The result led to the conclusion that the most suitable mixture for printing was achieved at the water to cement ratio of 0.35 with water reducing and retarding admixture added. The optimum printing parameters were the printing speed of 60 mm/min and the feed rate of 120 ml/s. Compressive strength of the 5 x 5 x 5 cm3 hollowed and filled cubic printed specimens, were compared with casted cement paste. The strengths of both the printed and the casted specimens were higher with longer curing durations. The highest levels of strength were achieved at 12.36 MPa on the printed specimens and 80.88 MPa when testing the casted samples. © Published under licence by IOP Publishing Ltd.

关键词： 3D printers

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Visualizing Field-free Deterministic Magnetic Switching of all–van der Waals Spin-Orbit Torque System Using Spin Ensembles in Hexagonal Boron Nitride

arXiv

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arXiv 2025年

作者： Zhang, Xi Zhou, Jingcheng Hu, Chaowei Deng, Kuangyin Wang, Chuangtang Agarwal, Nishkarsh Jin, Hanshang Al-Matouq, Faris A. Xu, Stelo Trivedi, Roshan S. Li, Senlei Rathi, Sumedh Lu, Hanyi Jiang, Zhigang Taufour, Valentin Hovden, Robert Zhao, Liuyan Cheng, Ran Xu, Xiaodong Chu, Jiun-Haw Du, Chunhui Rita Wang, Hailong School of Physics Georgia Institute of Technology AtlantaGA30332 United States Department of Physics University of Washington SeattleWA98105 United States Department of Electrical and Computer Engineering University of California RiversideCA92521 United States Department of Physics University of Michigan Ann ArborMI48109 United States Department of Materials Science and Engineering University of Michigan Ann ArborMI48109 United States Department of Physics and Astronomy University of California DavisCA95616 United States Department of Physics University of California San Diego La Jolla CA92093 United States Applied Physics Program University of Michigan Ann ArborMI48109 United States Department of Physics and Astronomy University of California RiversideCA92521 United States Department of Materials Science and Engineering University of Washington SeattleWA98105 United States

Recently, optically active spin defects embedded in van der Waals (vdW) crystals have emerged as a transformative quantum sensing platform to explore cutting-edge materials science and quantum physics. Taking advantage of excellent solid-state integrability, this new class of spin defects can be arranged in controllable nanoscale proximity of target materials in vdW heterostructures, showing great promise for improving spatial resolution and field sensitivity of current sensing technologies. Building on this state-of-the-art measurement platform, here we report hexagonal boron nitride-based quantum imaging of field-free deterministic magnetic switching of room-temperature two-dimensional magnet Fe3GaTe2 in an all-vdW spin-orbit torque (SOT) system. By visualizing SOT-driven variations of nanoscale Fe3GaTe2 magnetic stray field profile under different conditions, we have revealed how the observed magnetic switching evolves from deterministic to indeterministic behavior due to the interplay between out-of-plane spins, in-plane spins and Joule heating. This understanding, which is otherwise difficult to access by conventional transport measurements, offers valuable insights on material design, testing, and evaluation of next-generation vdW spintronic devices. Copyright © 2025, The Authors. All rights reserved.

关键词： Van der Waals forces

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Computational design of anisotropic stealthy hyperuniform composites with engineered directional scattering properties

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Physical Review E 2023年第4期108卷 045306-045306页

作者： Wenlong Shi David Keeney Duyu Chen Yang Jiao Salvatore Torquato Materials Science and Engineering Arizona State University Tempe Arizona 85287 USA Materials Research Laboratory University of California Santa Barbara California 93106 USA Department of Physics Arizona State University Tempe Arizona 85287 USA Department of Chemistry Princeton University Princeton New Jersey 08544 USA Department of Physics Princeton University Princeton New Jersey 08544 USA Princeton Institute of Materials Princeton University Princeton New Jersey 08544 USA Program in Applied and Computational Mathematics Princeton University Princeton New Jersey 08544 USA

Disordered hyperuniform materials are an emerging class of exotic amorphous states of matter that endow them with singular physical properties, including large isotropic photonic band gaps, superior resistance to fracture, and nearly optimal electrical and thermal transport properties, to name but a few. Here we generalize the Fourier-space-based numerical construction procedure for designing and generating digital realizations of isotropic disordered hyperuniform two-phase heterogeneous materials (i.e., composites) developed by Chen and Torquato [Acta Mater. 142, 152 (2018)] to anisotropic microstructures with targeted spectral densities. Our generalized construction procedure explicitly incorporates the vector-dependent spectral density function χ̃V(k) of arbitrary form that is realizable. We demonstrate the utility of the procedure by generating a wide spectrum of anisotropic stealthy hyperuniform microstructures with χ̃V(k)=0 for k∈Ω, i.e., complete suppression of scattering in an “exclusion” region Ω around the origin in Fourier space. We show how different exclusion-region shapes with various discrete symmetries, including circular-disk, elliptical-disk, square, rectangular, butterfly-shaped, and lemniscate-shaped regions of varying size, affect the resulting statistically anisotropic microstructures as a function of the phase volume fraction. The latter two cases of Ω lead to directionally hyperuniform composites, which are stealthy hyperuniform only along certain directions and are nonhyperuniform along others. We find that while the circular-disk exclusion regions give rise to isotropic hyperuniform composite microstructures, the directional hyperuniform behaviors imposed by the shape asymmetry (or anisotropy) of certain exclusion regions give rise to distinct anisotropic structures and degree of uniformity in the distribution of the phases on intermediate and large length scales along different directions. Moreover, while the anisotropic exclusion regions

关键词： Amorphous materials Complex materials Simulated annealing

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Metallization of colloidal crystals

arXiv

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arXiv 2021年

作者： Ehlen, Ali Lopez-Rios, Hector de la Cruz, Monica Olvera Applied Physics Program Northwestern University Department of Materials Science and Engineering Northwestern University

Colloidal crystals formed by size-asymmetric binary particles co-assemble into a wide variety of colloidal compounds with lattices akin to ionic crystals. Recently, a transition from a compound phase with a sublattice of small particles to a metal-like phase in which the small particles are delocalized has been predicted computationally and observed experimentally. In this colloidal metallic phase, the small particles roam the crystal maintaining the integrity of the lattice of large particles, as electrons do in metals. A similar transition also occurs in superionic crystals, termed sublattice melting. Here, we use energetic principles and a generalized molecular dynamics (MD) model of a binary system of functionalized nanoparticles (NPs) to analyze the transition to sublattice delocalization in different co-assembled crystal phases as a function of temperature (T), number of grafted chains on the small particles, and number ratio between the small and large particles ns:nl. We find that ns:nl is the primary determinant of crystal type due to energetic interactions and interstitial site filling, while the number of grafted chains per small particle determines the stability of these crystals. We observe first-order sublattice delocalization transitions as T increases, in which the host lattice transforms from low- to high-symmetry crystal structures, including A20 → BCT → BCC, Ad → BCT → BCC, and BCC → BCC/FCC → FCC transitions and lattices. Analogous sublattice transitions driven primarily by lattice vibrations have been seen in some atomic materials exhibiting an insulator-metal transition also referred to as metallization. We also find minima in the lattice vibrations and diffusion coefficient of small particles as a function of ns:nl, indicating enhanced stability of certain crystal structures for ns:nl values that form compounds. © 2021, CC BY.

关键词： Molecular dynamics

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