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Effect of chemical and biological additives on production of biogas from coffee pulp silage

Scientific Reports 2023年第1期13卷 1-11页

作者： Getachew, Mengizam Tsegaye Hiruy, Andualem Mekonnen Mazharuddin, Majid Mohiuddin Mamo, Tadios Tesfaye Feseha, Temesgen Aragaw Mekonnen, Yedilfana Setarge Center for Environmental Science College of Natural and Computational Sciences Addis Ababa University Addis Ababa Ethiopia Institute of Atomic and Molecular Sciences Academia Sinica Taipei Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica Taipei 11529 Taiwan Institute of Physics Academia Sinica Taipei 11529 Taiwan Department of Chemistry National Taiwan University Taipei 10617 Taiwan

Energy is the foundation of the global economy and is essential to human survival. Nevertheless, more than 60% of it comes from fossil fuels. That is not a replenished and scarce source. However, a sizable amount of organic waste is generated every minute throughout the world and can be used as a raw material to produce renewable energy. Among them, Coffee processing generates a huge amount of solid and liquid waste that is organic and can serve as raw material for biofuel production. Since coffee beans and powder are Ethiopia’s main exports, coffee pulp is easily accessible. Therefore, the main goal of this project is to convert this waste, which largely consists of organic materials, into a valuable product called Methane. The purity and yield of methane productivity are significantly influenced by the type of additives we use. This work systematically investigates the effect of chemical and biological additives on the productivity and purity of the Biogas from the coffee pulp silage in batch systems under mesophilic temperature (38 °C) for different ensiling periods and additive proportions. The chemical additives recorded the maximum biogas production (2980 ml) at an ensiling period of 40 days with high purity of about 70% biogas. The minimum Biogas was recorded at the ensiling period of 10 days by the control (T1) treatments, which was 634 ml. This work proves that biological additives produced the highest quality and quantity of Biogas from coffee silage. © 2023, The Author(s).

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Optogenetic Neural Probes: Fiberless, High-Density, Artifact-Free Neuromodulation : (Invited)

Optogenetic Neural Probes: Fiberless, High-Density, Artifact...

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International Electron Devices Meeting (IEDM)

作者： Eunah Ko Kanghwan Kim Mihály Vöröslakos Sungjin Oh György Buzsáki Kensall D. Wise Euisk Yoon Department of Electrical Engineering and Computer Science University of Michigan Ann Arbor MI USA Center for BioMicrosystems Brain Science Institute Korea Institute of Science and Technology Seoul Korea Neuroscience Institute Langone Medical Center New York University New York NY USA Department of Biomedical Engineering University of Michigan Ann Arbor MI USA Center for Nanomedicine Institute for Basic Science (IBS) and Graduate Program of Nano Biomedical Engineering (Nano BME) Advanced Science Institute Yonsei University Seoul Korea

ISBN: (纸本)9781665489607

Evolution of “Michigan Probes” has enabled unraveling the connectivity of neurons at cellular resolution and their dynamic interaction within and across brain areas that underlie behavioral and cognitive functions. Recently, micro-LEDs were monolithically integrated for optogenetic neuromodulation at scale without requiring external optical fiber connection. The ‘hectoSTAR’ micro-LED optoelectrode features 256 recording electrodes and 128 stimulation micro-LEDs in four silicon micro-needle shanks, covering a large volume with 1.3-mm × 0.9-mm cross-sectional area located as deep as 6 mm inside the brain. Technical challenges to overcome in scaling of optogenetic probes will be discussed, followed by future direction.

关键词： Optical fibers Electrodes Brain Optogenetics Silicon Recording Optical fiber devices

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Enhanced electrochemical performance of a LiFePO4 cathode with an environmentally friendly pectin/polyethylene glycol binder

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Journal of Power Sources 2024年 613卷

作者： Chen, Yan-Ruei Chen, Liang-Yu Chung, Chin-Yi Su, Yu-Hsuan Wu, Feng-Yu Hsu, Tsung-Ming Chi, Po-Wei Wu, Phillip M. Chang-Liao, Kuei-Shu Tang, Hong-Yi Wu, Maw-Kuen Institute of Physics Academia Sinica 128 Section 2 Academia Road Taipei11529 Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Tsing Hua University 128 Section 2 Academia Road Taipei11529 Taiwan Department of Engineering and System Science National Tsing Hua University 101 Section 2 Kuang-Fu Road Hsinchu300044 Taiwan College of Science National Chung Hsing University 145 Xingda Road South District Taichung402 Taiwan Department of Applied Chemistry National Chi-Nan University 1 University Road Puli Nantou545301 Taiwan

The advancement of lithium-ion battery technology relies on the development of materials that not only improve performance but also align with environmental sustainability. This work presents a novel water-based pectin-PEG binder for LiFePO4 cathodes that combines eco-friendliness with electrochemical innovation. The binder material is made by mixing pectin, a flexible natural substance, with polyethylene glycol through a radical copolymerization process. This combination gives the binder both flexibility and a boost in electrical performance. Our experimental results demonstrate that LFP cathodes with this binder have an intriguing self-healing ability in comparison with the conventional PVDF binder, enhanced charge-discharge capacities, improved cycling stability, and higher ionic conductivity. Specifically, electrodes utilizing the pectin-PEG binder exhibit an impressive retention of discharge capacity. They maintain roughly 150 mAh g−1 after 500 cycles at 1C with 99% retention, and about 141 mAh g−1 with 97% retention at 3C. Cyclic voltammetry (CV) confirms that the PP binder maintains its ionic diffusion properties at high sweep rates, whereas galvanostatic intermittent titration technique reveals a much higher lithium ion diffusion coefficient (DLi+) within the operational voltage range of the LFP-PP250 electrodes. These findings establish an attractive direction for the development of electrodes for high-energy density, sustainable lithium-ion batteries. © 2024 Elsevier B.V.

关键词： Lithium compounds

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Solution-Processed and Room-Temperature Spin Light-Emitting Diode Based on Quantum Dots/Chiral Metal-Organic Framework Heterostructure

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Advanced Functional Materials 2023年第19期33卷

作者： Mustaqeem, Mujahid Chou, Pi-Tai Kamal, Saqib Ahmad, Naveed Lin, Jia-Yu Lu, Yu-Jung Lee, Xing-Hao Lin, Kung-Hsuan Lu, Kuang-Lieh Chen, Yang-Fang Nano-Science and Technology Program Taiwan International Graduate Program Institute of Physics Academia Sinica Taipei106 Taiwan Department of Physics National Taiwan University No. 1 Section 4 Roosevelt Rd Taipei10617 Taiwan Department of Chemistry National Taiwan University No. 1 Section 4 Roosevelt Rd Taipei10617 Taiwan Institute of Chemistry Academia Sinica Taipei115 Taiwan Department of Materials Science and Engineering National Taiwan University of Science and Technology Taipei10607 Taiwan Research Center for Applied Sciences Academia Sinica Taipei115024 Taiwan Institute of Physics Academia Sinica Taipei11529 Taiwan

Spin optoelectronics is an indispensable key for the future development of spintronics. In conventional spin light emitting diodes (LEDs), spin-polarized carrier pairs are injected electrically into the light emitting layer and create circularly polarized light (CPL). Generally, spin-polarized carriers are accomplished using ferromagnetic contacts or applying an external magnetic field, which will produce several drawbacks, including low temperature operation, low spin-polarized carriers injection efficiency, etc. To circumvent the existing shortcomings, here, an alternative approach is proposed and achieves spin-polarized LEDs at room temperature based on quantum dots (QDs)/chiral metal-organic framework heterojunction without using ferromagnetic contacts or magnetic fields. The spin-polarized injected layer composed of self-assembled monolayer (SAM)/Chiral-MOF ([Sr(9,10-adc)(DMAc)2]n)) film, which produces spin-polarized holes with spin orientation, determining the polarization and strength of circularly polarized electroluminescence (CP-EL). The spin-QLED emits CP-EL at a rate of 12.24% efficiency, which provides an excellent alternative to generate new functionality for conventional QLEDs. The approach is anticipated to be very useful, enabling to offer a general methodology for generating not yet realized spin optoelectronic devices. © 2023 Wiley-VCH GmbH.

关键词： Room temperature

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Structural, Morphological, Optical, and Antibacterial Activities of Zinc Oxide nanopowders: A Comparative Study of Green and Soft Chemical Synthesis

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Advances in Materials science and Engineering 2022年第0期2022卷

作者： Siriya Pushpa, K. Catherine Sakthivel, P. Saravanakumar, K. Anuradha, N. Sankaranarayanan, R.K. Paulraj, Mosae Selvakumar Post-Graduate and Research Department of Physics Bon Secours College for Women Tamil Nadu Thanjavur613006 India Centre for Materials Science Department of Physics Science and Humanities Faculty of Engineering Karpagam Academy of Higher Education Coimbatore641021 India Mallasamudram Tamil Nadu Namakkal637503 India Centre for Nano Science and Technology Department of Chemistry Chennai Institute of Technology Tamil Nadu Kundrathur600069 India AUW Chemistry Hub Science and Math Program Asian University for Women Chattogram Bangladesh

Zinc oxide, a well-known inorganic metal oxide in nanoparticle form, has outstanding antibacterial properties. In this work, the authors focus on determining ZnO nanoparticles’ structural, optical, and antibacterial activity. A simple soft chemical route synthesizes C-ZnO nanoparticles chemically, while the green synthesis method is used to prepare G-ZnO nanoparticles. Ocimum tenuiflorum leaf extract was used to prepare G-ZnO nanopowders. These samples are investigated and compared in terms of their structural, morphological, optical, and antibacterial properties. According to XRD investigations, the synthesized ZnO nanopowders possess a hexagonal structure. The particle size of G-ZnO is smaller than that of C-ZnO nanoparticles. The XPS result revealed the binding and interactions between molecules. The FTIR study confirmed the presence of molecules and their vibrations. UV-vis-DRS spectroscopy was used to investigate optical properties such as reflectance and band gap. The grain size of the G-ZnO nanopowders was decreased, and oxygen vacancy was produced. The antibacterial efficiency of plant extracts against two different bacterial strains, S. aureus (Gram-positive) and *** (Gram-negative), has been studied and reported. Copyright © 2022 K. Catherine Siriya Pushpa et al.

关键词： ZnO nanoparticles

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technology Roadmap for Flexible Sensors

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ACS nano 2023年第6期17卷 5211-5295页

作者： Luo, Yifei Abidian, Mohammad Reza Ahn, Jong-Hyun Akinwande, Deji Andrews, Anne M. Antonietti, Markus Bao, Zhenan Berggren, Magnus Berkey, Christopher A. Bettinger, Christopher John Chen, Jun Chen, Peng Cheng, Wenlong Cheng, Xu Choi, Seon-Jin Chortos, Alex Dagdeviren, Canan Dauskardt, Reinhold H. Di, Chong-an Dickey, Michael D. Duan, Xiangfeng Facchetti, Antonio Fan, Zhiyong Fang, Yin Feng, Jianyou Feng, Xue Gao, Huajian Gao, Wei Gong, Xiwen Guo, Chuan Fei Guo, Xiaojun Hartel, Martin C. He, Zihan Ho, John S. Hu, Youfan Huang, Qiyao Huang, Yu Huo, Fengwei Hussain, Muhammad M. Javey, Ali Jeong, Unyong Jiang, Chen Jiang, Xingyu Kang, Jiheong Karnaushenko, Daniil Khademhosseini, Ali Kim, Dae-Hyeong Kim, Il-Doo Kireev, Dmitry Kong, Lingxuan Lee, Chengkuo Lee, Nae-Eung Lee, Pooi See Lee, Tae-Woo Li, Fengyu Li, Jinxing Liang, Cuiyuan Lim, Chwee Teck Lin, Yuanjing Lipomi, Darren J. Liu, Jia Liu, Kai Liu, Nan Liu, Ren Liu, Yuxin Liu, Yuxuan Liu, Zhiyuan Liu, Zhuangjian Loh, Xian Jun Lu, Nanshu Lv, Zhisheng Magdassi, Shlomo Malliaras, George G. Matsuhisa, Naoji Nathan, Arokia Niu, Simiao Pan, Jieming Pang, Changhyun Pei, Qibing Peng, Huisheng Qi, Dianpeng Ren, Huaying Rogers, John A. Rowe, Aaron Schmidt, Oliver G. Sekitani, Tsuyoshi Seo, Dae-Gyo Shen, Guozhen Sheng, Xing Shi, Qiongfeng Someya, Takao Song, Yanlin Stavrinidou, Eleni Su, Meng Sun, Xuemei Takei, Kuniharu Tao, Xiao-Ming Tee, Benjamin C. K. Thean, Aaron Voon-Yew Trung, Tran Quang Wan, Changjin Wang, Huiliang Wang, Joseph Wang, Ming Wang, Sihong Wang, Ting Wang, Zhong Lin Weiss, Paul S. Wen, Hanqi Xu, Sheng Xu, Tailin Yan, Hongping Yan, Xuzhou Yang, Hui Yang, Le Yang, Shuaijian Yin, Lan Yu, Cunjiang Yu, Guihua Yu, Jing Yu, Shu-Hong Yu, Xinge Zamburg, Evgeny Zhang, Haixia Zhang, Xiangyu Zhang, Xiaosheng Zhang, Xueji Zhang, Yihui Zhang, Yu Zhao, Siyuan Zhao, Xuanhe Zheng, Yuanjin Zheng, Yu-Qing Zheng, Zijian Zhou, Tao Zhu, Bowen Zhu, Ming Zhu, Rong Zhu, Yangzhi Zhu, Yong Zou, Guijin Chen, Xiaodong 08-03 Innovis Singapore 138634 Republic of Singapore Innovative Centre for Flexible Devices (iFLEX) School of Materials Science and Engineering Nanyang Technological University Singapore 639798 Singapore Department of Biomedical Engineering University of Houston Houston Texas 77024 United States School of Electrical and Electronic Engineering Yonsei University Seoul 03722 Republic of Korea Department of Electrical and Computer Engineering The University of Texas at Austin Austin Texas 78712 United States Microelectronics Research Center The University of Texas at Austin Austin Texas 78758 United States Department of Chemistry and Biochemistry California NanoSystems Institute and Department of Psychiatry and Biobehavioral Sciences Semel Institute for Neuroscience and Human Behavior and Hatos Center for Neuropharmacology University of California Los Angeles Los Angeles California 90095 United States Colloid Chemistry Department Max Planck Institute of Colloids and Interfaces 14476 Potsdam Germany Department of Chemical Engineering Stanford University Stanford California 94305 United States Laboratory of Organic Electronics Department of Science and Technology Campus Norrköping Linköping University 83 Linköping Sweden Wallenberg Initiative Materials Science for Sustainability (WISE) and Wallenberg Wood Science Center (WWSC) SE-100 44 Stockholm Sweden Department of Materials Science and Engineering Stanford University Stanford California 94301 United States Department of Biomedical Engineering and Department of Materials Science and Engineering Carnegie Mellon University Pittsburgh Pennsylvania 15213 United States Department of Bioengineering University of California Los Angeles Los Angeles California 90095 United States School of Chemistry Chemical Engineering and Biotechnology Nanyang Technological University Singapore 637457 Singapore Nanobionics Group Department of Chemical and Biological Engineering Monash University Clayton Australia 3800 Monash

Humans rely increasingly on sensors to address grand challenges and to improve quality of life in the era of digitalization and big data. For ubiquitous sensing, flexible sensors are developed to overcome the limitations of conventional rigid counterparts. Despite rapid advancement in bench-side research over the last decade, the market adoption of flexible sensors remains limited. To ease and to expedite their deployment, here, we identify bottlenecks hindering the maturation of flexible sensors and propose promising solutions. We first analyze continued...challenges in achieving satisfactory sensing performance for real-world applications and then summarize issues in compatible sensor-biology interfaces, followed by brief discussions on powering and connecting sensor networks. Issues en route to commercialization and for sustainable growth of the sector are also analyzed, highlighting environmental concerns and emphasizing nontechnical issues such as business, regulatory, and ethical considerations. Additionally, we look at future intelligent flexible sensors. In proposing a comprehensive roadmap, we hope to steer research efforts towards common goals and to guide coordinated development strategies from disparate communities. Through such collaborative

关键词： soft materials mechanics engineering flexible electronics conformable sensors bioelectronics human-machine interfaces body area sensor networks technology translation sustainable electronics

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Impact of zinc doping on physical and photoelectrochemical properties of Bi2O3 nanoparticles for biosensor application

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Ceramics International 2025年

作者： Abdelfatah, Mahmoud Goher, Nermeen El-Shaer, Abdelhamid Hashim, H. Physics Department Faculty of Science Kafrelsheikh University Kafrelsheikh33516 Egypt Nano Science and Technology Program Faculty of Science Kafrelsheikh University Kafrelsheikh33516 Egypt Physics Department Faculty of Science Tanta University Tanta31527 Egypt

Many people lose their life due to diabetes each year as it is one of the most prevalent chronic illnesses, so that nanomaterials such Bi2O3 could employed in the fabrication of electrodes for glucose detection. Low-cost co-precipitation method was used to synthesize pure and (1 %, 3 %, 5 %) Zn-doped Bi2O3 NPs. XRD, Raman, SEM, TEM, EDX, UV–Vis, PL, Mott Schottky, and EIS measurements were employed to examine the characteristics of the fabricated nanoparticles. The XRD data showed that pure and Zn-doped Bi2O3 NPs have a monoclinic structure with decreasing in crystallite size from 24 to 11 nm as Zn ion concentration rises. Raman spectra showed that Bi-O stretches are related to the broad peaks at higher frequency modes of 526, 442, and 312 cm−1, while lattice vibrations are linked to the other sharp peaks at 91, 115, 147, 182, and 208 cm−1. From SEM results, Zn ion concentrations affect the size of agglomerated particles and the surface appearance of all samples. TEM micrographs showed average particle size of 24 and 10 nm for pure and 5 % Zn -doped Bi2O3 NPs. UV–Vis spectra displayed strong absorption bands with band gap energy increasing from 2.86 to 2.89 eV with increasing Zn ion concentration. PL analysis showed that the intensity of the spectra reduced with the increase in Zn doping with blue-green emission bands concentrated at 525 nm. The EIS investigation presented that with increasing Zn ion content rises, the charge transfer resistance of all the manufactured samples lowers. Mott-Schottky measurements revealed that the donor density of pure and Zn-doped α Bi2O3 NPs increased from 9.3 × 1019 cm−3 to 1.3 × 1020 cm−3. The chronoamperometry analysis displayed that the measured current was found to rise from 0.02 to 0.04 mA with increasing glucose where the sensitivity of fabricated biosensor increased from 0.31 to 2.3 μA mM−1 cm−2 with Zn doping process. Our outcomes show that Zn-doped Bi2O3 nanoparticles are promising candidates for biosensor applications. ©

关键词： Lattice vibrations

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A green recyclable Li3VO4-pectin electrode exhibiting pseudocapacitive effect as an advanced anode for lithium-ion battery

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Journal of Energy Storage 2023年 72卷

作者： Su, Yu-Hsuan Chung, Chin-Yi Chen, Yan-Ruei Wu, Feng-Yu Lin, Ya-Huei Chi, Po-Wei Wu, Phillip M. Paul, Tanmoy Lin, Hwai-En Chang-Liao, Kuei-Shu Wang, Sea-Fue Wu, Maw-Kuen Institute of Physics Academia Sinica 128 Section 2 Academia Road Taipei11529 Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Tsing Hua University 128 Section 2 Academia Road Taipei11529 Taiwan Department of Engineering and System Science National Tsing Hua University 101 Section 2 Kuang-Fu Road Hsinchu300044 Taiwan 1 Section 3 Zhongxiao E. Rd. Taipei106 Taiwan 1 Section 3 Zhongxiao E. Road Taipei106 Taiwan Research Institute for Sustainable Energy TCG Centres for Research and Education in Science and Technology BIPL Building Salt Lake Kolkata700091 India

Battery system design and development is prioritizing environmentally friendly recycling processes to ensure a sustainable future for our planet. The reuse of active materials in Li-ion batteries is critical for this goal. Herein, we investigated the electrochemical performance of Li3VO4 (LVO) anode with pectin as a binder. Our Li-ion half-cells showed stable capacity of 230 mAh g−1 at a current density of 0.02 A g−1 after 100 cycles. In addition, we observed a novel enhanced specific capacity of 400 mAh g−1 during delithiation at a high current density of 1 A g−1, which did not occur during lithiation. This higher capacity was can be attributed to the pseudocapacitive lithium storage behavior in the LVO-pectin electrode, as identified by CV and EIS analyses. The heterostructure of LVO-pectin resulted in an interfacial surface charge that contributed to the capacity, as demonstrated by impedance spectroscopy in conjunction with the distribution of relaxation times. The utilization of pectin as an eco-friendly binder demonstrated nearly 90 % material recovery and 100 % capability for subsequent re-lithiation, indicating recyclability. Furthermore, the pseudocapacitive effect becomes increasingly dominant in regenerated LVO-pectin cells. These results exemplify a promising approach towards the development of environmentally friendly Li-ion batteries with high energy and power density. © 2023 Elsevier Ltd

关键词： Lithium-ion batteries

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Photothermal responsivity of van der Waals material-based nanomechanical resonators

arXiv

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arXiv 2022年

作者： Aguila, Myrron Albert C. Esmenda, Joshoua C. Wang, Jyh-Yang Lee, Teik-Hui Chen, Yen-Chun Yang, Chi-Yuan Lin, Kung-Hsuan Chang-Liao, Kuei-Shu Kafanov, Sergey Pashkin, Yuri A. Chen, Chii-Dong Department of Engineering and System Science National Tsing Hua University Hsinchu30013 Taiwan Nano Science and Technology Program Taiwan International Graduate Program National Tsing Hua University Academia Sinica Taiwan Institute of Physics Academia Sinica Nankang Taipei11529 Taiwan Department of Physics Lancaster University LancasterLA1 4YB United Kingdom

nanomechanical resonators made from van der Waals materials (vdW NMRs) provide a new tool for sensing absorbed laser power. The photothermal response of vdW NMRs, quantified from the resonant frequency shifts induced by optical absorption, is enhanced when incorporated in a Fabry-Perot (FP) interferometer. Along with the enhancement comes the dependence of the photothermal response on NMR displacement, which lacks investigation. Here, we address the knowledge gap by studying electromotively driven niobium diselenide drumheads fabricated on highly reflective substrates. We use a FP-mediated absorptive heating model to explain the measured variations of the photothermal response. The model predicts a higher magnitude and tuning range of photothermal responses on few-layer and monolayer NbSe2 drumheads, which outperform other clamped vdW drum-type NMRs at a laser wavelength of 532 nm. Further analysis of the model shows that both the magnitude and tuning range of NbSe2 drumheads scale with thickness, establishing a displacement-based framework for building bolometers using FP-mediated vdW NMRs. © 2022, CC BY.

关键词： Van der Waals forces

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Single-molecule localization microscopy of expanded mammalian centrioles unravels the ultrastructural constitution of distal appendages

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Biophysical journal 2023年第3S1期122卷 17a页

作者： Chang, Ting-Jui B Hsu, Jimmy C-C Yang, Tony Physics National Taiwan University Taipei City Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica Taipei City Taiwan Electrical Engineering National Taiwan University Taipei City Taiwan Electrical Engineering National Taiwan University Taipei City Taiwan Graduate Institute of Biomedical Electronics and Bioinformatics National Taiwan University Taipei City Taiwan

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