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Fluorine-Containing Passivation Layer via Surface Chelation for Inorganic Perovskite Solar Cells

Angewandte Chemie 2022年第6期135卷

作者： Hao Zhang Prof. Wanchun Xiang Xuejiao Zuo Xiaojing Gu Shiang Zhang Yachao Du Zhiteng Wang Yali Liu Haifeng Wu Peijun Wang Qingyue Cui Hang Su Prof. Qingwen Tian Prof. Shengzhong (Frank) Liu Key Laboratory of Applied Surface and Colloid Chemistry Ministry of Education Shaanxi Key Laboratory for Advanced Energy Devices Shaanxi Engineering Lab for Advanced Energy Technology School of Materials Science and Engineering Shaanxi Normal University No. 620 West Chang'an Avenue Xi'an 710119 P. R. China Contribution: Data curation (lead) Formal analysis (lead) Investigation (lead) Writing - original draft (supporting) Contribution: Conceptualization (lead) Data curation (lead) Writing - original draft (lead) Contribution: Formal analysis (supporting) Investigation (supporting) Contribution: Data curation (supporting) Formal analysis (equal) Investigation (equal) Contribution: Data curation (supporting) Investigation (supporting) Contribution: Data curation (supporting) Formal analysis (supporting) State Key Laboratory of Organic-Inorganic Composites Key Lab of Biomedical Materials of Natural Macromolecules Ministry of Education Beijing Laboratory of Biomedical Materials Beijing University of Chemical Technology No. 15 East Road North Third Ring Chaoyang District Beijing 100029 P. R. China Contribution: Conceptualization (lead) Data curation (lead) Funding acquisition (lead) Project administration (lead) Supervision (lead) Validation (lead) Visualization (lead) Writing - review & editing (lead) Dalian National Laboratory for Clean Energy iChEM Dalian Institute of Chemical Physics Chinese Academy of Sciences No. 457 Zhongshan Road Dalian Liaoning 116023 P. R. China Contribution: Project administration (lead) Supervision (lead) Validation (lead) Writing - review & editing (equal)

Minimizing surface defect is vital to further improve power conversion efficiency (PCE) and stability of inorganic perovskite solar cells (PSCs). Herein, we designed a passivator trifluoroacetamidine (TFA) to suppress CsPbI 3− x Br x film defects. The amidine group of TFA can strongly chelate onto the perovskite surface to suppress the iodide vacancy, strengthened by additional hydrogen bonds. Moreover, three fluorine atoms allow strong intermolecular connection via intermolecular hydrogen bonds, thus constructing a robust shield against moisture. The TFA-treated PSCs exhibit remarkably suppressed recombination, yielding the record PCEs of 21.35 % and 17.21 % for 0.09 cm 2 and 1.0 cm 2 device areas, both of which are the highest for all-inorganic PSCs so far. The device also achieves a PCE of 39.78 % under indoor illumination, the highest for all-inorganic indoor photovoltaic devices. Furthermore, TFA greatly improves device ambient stability by preserving 93 % of the initial PCE after 960 h.

关键词： Chelation Defect Passivation Inorganic Perovskite Solar Cells

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Mapping essential urban land use categories in China(EULUC-China):preliminary results for 2018

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Science Bulletin 2020年第3期65卷 182-187页

作者： Peng Gong Bin Chen Xuecao Li Han Liu Jie Wang Yuqi Bai Jingming Chen Xi Chen Lei Fang Shuailong Feng Yongjiu Feng Yali Gong Hao Gu Huabing Huang Xiaochun Huang Hongzan Jiao Yingdong Kang Guangbin Lei Ainong Li Xiaoting Li Xun Li Yuechen Li Zhilin Li Zhongde Li Chong Liu Chunxia Liu Maochou Liu Shuguang Liu Wanliu Mao Changhong Miao Hao Ni Qisheng Pan Shuhua Qi Zhehao Ren Zhuoran Shan Shaoqing Shen Minjun Shi Yimeng Song Mo Su Hoi Ping Suen Bo Sun Fangdi Sun Jian Sun Lin Sun Wenyao Sun Tian Tian Xiaohua Tong Yihsing Tseng Ying Tu Hong Wang Lan Wang Xi Wan Zongming Wang Tinghai Wu Yaowen Xie Jian Yang Jun Yang Man Yuan Wenze Yue Hongda Zeng Kuo Zhang Neng Zhang Tao Zhang Yu Zhang Feng Zhao Yichen Zheng Qiming Zhou Nicholas Clinton Zhiliang Zhu Bing Xu Ministry of Education Key Laboratory for Earth System Modeling Department of Earth System ScienceTsinghua UniversityBeijing 100084China Tsinghua Urban Institute Tsinghua UniversityBeijing 100084China Center for Healthy Cities Institute for China Sustainable UrbanizationTsinghua UniversityBeijing 100084China Department of Land Air and Water ResourcesUniversity of CaliforniaDavisCA 95616-8627USA Department of Geological and Atmospheric Sciences Iowa State UniversityAmesIA 50011USA State Key Laboratory of Remote Sensing Science Institute of Remote Sensing and Digital EarthChinese Academy of SciencesBeijing 100101China AI for Earth Laboratory Cross-Strait InstituteTsinghua UniversityBeijing 100084China International Institute for Earth System Sciences Nanjing UniversityNanjing 210093China Research Center for Ecology and Environment of Central Asia Chinese Academy of SciencesUrumchi 830011China Key Laboratory of Forest Ecology and Management Institute of Applied EcologyChinese Academy of SciencesShenyang 110016China National Engineering Laboratory for Applied Technology in Forestry&Ecology in South China College of Life Science and TechnologyCentral South University of Forestry and TechnologyChangsha 410004China College of Surveying&Geo-Informatics Tongji UniversityShanghai 200092China Department of Urban Planning College of Architecture and Urban PlanningTongji UniversityShanghai 200092China Beijing Institute of Urban Planning Beijing 100045China Department of Urban Planning School of Urban DesignWuhan UniversityWuhan 430072China College of Earth Sciences Jilin UniversityChangchun 130061China Research Center for Digital Mountain and Remote Sensing Application Institute of Mountain Hazards and EnvironmentChinese Academy of SciencesChengdu 610041China Institute of Remote Sensing and Geographic Information System School of Earth and Space SciencesPeking UniversityBeijing 100871China Department of Urban and Regional Planning School of Geography and PlanningSun Yat-sen Univ

Land use reflects human activities on *** land use is the highest level human alteration on Earth,and it is rapidly changing due to population increase and *** areas have widespread effects on local hydrology,climate,biodiversity,and food production[1,2].However,maps,that contain knowledge on the distribution,pattern and composition of various land use types in urban areas,are limited to city *** mapping standard on data sources,methods,land use classification schemes varies from city to city,due to differences in financial input and skills of mapping *** address various national and global environmental challenges caused by urbanization,it is important to have urban land uses at the national and global scales that are derived from the same or consistent data sources with the same or compatible classification systems and mapping *** is because,only with urban land use maps produced with similar criteria,consistent environmental policies can be made,and action efforts can be compared and assessed for large scale environmental ***,despite of the fact that a number of urban-extent maps exist at global scales[3,4],more detailed urban land use maps do not exist at the same *** at big country or regional levels such as for the United States,China and European Union,consistent land use mapping efforts are rare[5,6](e.g.,https://***/open_land_use/).

关键词： EULUC-China 土地利用类型

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A Hypothesis on the Function of High-Valent Fe in NiFe (Hydr)oxide in the Oxygen-Evolution Reaction

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Angewandte Chemie 2024年第6期137卷

作者： Nader Akbari Jafar Hussain Shah Cejun Hu Subhajit Nandy Pavlo Aleshkevych Rile Ge Sumbal Farid Changchang Dong Liang Zhang Keun Hwa Chae Wei Xie Taifeng Liu Junhu Wang Mohammad Mahdi Najafpour Department of Chemistry Institute for Advanced Studies in Basic Sciences (IASBS) Zanjan 45137-66731 Iran CAS Key Laboratory of Science and Technology on Applied Catalysis Mössbauer Effect Data Center Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian 116023 China Key Lab of Advanced Energy Materials Chemistry (Ministry of Education) Renewable Energy Conversion and Storage Center College of Chemistry Nankai University Tianjin 300071 China Advanced Analysis Center Korea Institute of Science and Technology Seoul 02792 Republic of Korea Institute of Physics Polish Academy of Sciences Warsaw 02-668 Poland School of Environmental and Chemical Engineering Jiangsu University of Science and Technology Zhenjiang 212100 China National and Local Joint Engineering Research Center for Applied Technology of Hybrid Nanomaterials Henan University Kaifeng 475004 China Department of Chemistry Sharif University of Technology Tehran 11155-9516 Iran

This study investigated the dynamic changes in NiFe (hydr)oxide and identified the role of high-valent Fe in the oxygen-evolution reaction (OER) within alkaline media via in situ techniques. Several high-valent Fe ions were found to remain considerably stable in the absence of potential in NiFe (hydr)oxide, even 96 hours after the OER. For Ni 2+ hydroxide treated with 57 Fe ions, where Fe sites are introduced onto the surface of Ni 2+ hydroxide, no Fe 4+ species were detected at the rate-determining step (RDS). The findings of this study suggested that the oxidation of bulk Fe ions, similar to Ni ions, to high valent forms, is charge accumulation without a direct role in OER; these results offered a novel perspective on manipulating Fe states to optimize OER efficacy. The prevailing hypothesis suggested that trace amounts of high-valent Fe ions, notably those on the surface, directly participate in OER.

关键词： NiFe (hydr)oxide oxygen evolution reaction high-valent Fe4+ in situ techniques electrocatalysts alkaline conditions mechanism active sites

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Wide-Bandgap Perovskite Solar Cell Using a Fluoride-Assisted Surface Gradient Passivation Strategy

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Angewandte Chemie 2023年第11期135卷

作者： Nan Yan Yan Gao Junjie Yang Zhimin Fang Jiangshan Feng Prof. Xiaojun Wu Prof. Tao Chen Prof. Shengzhong (Frank) Liu Key Laboratory of Applied Surface and Colloid Chemistry Ministry of Education Shaanxi Key Laboratory for Advanced Energy Devices Shaanxi Engineering Lab for Advanced Energy Technology School of Materials Science and Engineering Shaanxi Normal University Xi'an 710119 China Contribution: Data curation (lead) Formal analysis (lead) Investigation (lead) Methodology (lead) Writing - original draft (lead) Writing - review & editing (lead) Hefei National Laboratory for Physical Sciences at Microscale Department of Materials Science and Engineering University of Science and Technology of China Hefei 230026 China Contribution: Software (lead) Contribution: Methodology (equal) Validation (supporting) Contribution: Formal analysis (equal) Funding acquisition (lead) Investigation (equal) Writing - original draft (equal) Writing - review & editing (equal) Contribution: Funding acquisition (supporting) Investigation (supporting) Writing - original draft (equal) Writing - review & editing (equal) Dalian National Laboratory for Clean Energy iChEM Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian 116023 China Contribution: Formal analysis (supporting) Funding acquisition (lead) Investigation (equal) Project administration (lead) Resources (lead) Supervision (lead) Writing - original draft (supporting) Writing - review & editing (supporting)

Wide-band gap (1.68 eV) perovskite solar cells (PSCs) are important components of perovskite/Si tandem devices. However, the efficiency of wide band gap PSCs has been limited by their huge open-circuit voltage ( V oc ) deficit due to non-radiative recombination. Deep-level acceptor defects are identified as the major killers of V oc , and they can be effectively improved by passivation with ammonium salts. Theoretical calculation predicts that increasing the distance between F and −NH 3 + of fluorinated ammonium can dramatically enhance the electropositivity of −NH 3 + terminals, thus providing strong adsorption onto the negatively charged I A and I Pb anti-site defects. Characterizations further confirm that surface gradient passivation employing p -FPEAI demonstrates the most efficient passivation effect. Consequently, a record-efficiency of 21.63 % with the smallest V oc deficit of 441 mV is achieved for 1.68 eV-band gap inverted PSCs. Additionally, a flexible PSC and 1 cm 2 opaque device also deliver the highest PCEs of 21.02 % and 19.31 %, respectively.

关键词： Defects Fluoride Open-Circuit Voltage Deficit Perovskite Wide Band Gap

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Author Correction: Mapping annual 10-m soybean cropland with spatiotemporal sample migration

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Scientific data 2024年第1期11卷 565页

作者： Hongchi Zhang Zihang Lou Dailiang Peng Bing Zhang Wang Luo Jianxi Huang Xiaoyang Zhang Le Yu Fumin Wang Linsheng Huang Guohua Liu Shuang Gao Jinkang Hu Songlin Yang Enhui Cheng Key Laboratory of Digital Earth Science Aerospace Information Research Institute Chinese Academy of Sciences Beijing 100094 China. International Research Center of Big Data for Sustainable Development Goals Beijing 100094 China. University of Chinese Academy of Sciences Beijing 100094 China. Key Laboratory of Digital Earth Science Aerospace Information Research Institute Chinese Academy of Sciences Beijing 100094 China. pengdl@***. International Research Center of Big Data for Sustainable Development Goals Beijing 100094 China. pengdl@***. Key Laboratory of Digital Earth Science Aerospace Information Research Institute Chinese Academy of Sciences Beijing 100094 China. zhangbing@***. University of Chinese Academy of Sciences Beijing 100094 China. zhangbing@***. Jiangxi Nuclearindustry Surveying and Mapping Institute Group Co. Ltd Nanchang 330038 China. College of Land Science and Technology China Agricultural University Beijing 100083 China. Geospatial Sciences Center of Excellence Department of Geography Geospatial Sciences South Dakota State University Brookings SD 57007 USA. Department of Earth System Science Tsinghua University Beijing 100084 China. Institute of Applied Remote Sensing & Information Technology Zhejiang University Hangzhou 310058 China. National Engineering Research Center for Agro-Ecological Big Data Analysis & Application Anhui University Hefei 230601 China. Innovation Academy for Microsatellites Chinese Academy of Sciences Shanghai 200120 China.

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Study of ϒ production in pPb collisions at √sNN=8.16 TeV

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Journal of High Energy Physics 2018年第11期2018卷 1-36页

作者： Aaij, R. Abellán Beteta, C. Adeva, B. Adinolfi, M. Aidala, C.A. Ajaltouni, Z. Akar, S. Albicocco, P. Albrecht, J. Alessio, F. Alexander, M. Alfonso Albero, A. Alkhazov, G. Alvarez Cartelle, P. Alves, A.A. Amato, S. Amerio, S. Amhis, Y. An, L. Anderlini, L. Andreassi, G. Andreotti, M. Andrews, J.E. Appleby, R.B. Archilli, F. d’Argent, P. Arnau Romeu, J. Artamonov, A. Artuso, M. Arzymatov, K. Aslanides, E. Atzeni, M. Audurier, B. Bachmann, S. Back, J.J. Baker, S. Balagura, V. Baldini, W. Baranov, A. Barlow, R.J. Barsuk, S. Barter, W. Bartolini, M. Baryshnikov, F. Batozskaya, V. Batsukh, B. Battig, A. Battista, V. Bay, A. Beddow, J. Bedeschi, F. Bediaga, I. Beiter, A. Bel, L.J. Belin, S. Beliy, N. Bellee, V. Belloli, N. Belous, K. Belyaev, I. Ben-Haim, E. Bencivenni, G. Benson, S. Beranek, S. Berezhnoy, A. Bernet, R. Berninghoff, D. Bertholet, E. Bertolin, A. Betancourt, C. Betti, F. Bettler, M.O. van Beuzekom, M. Bezshyiko, Ia. Bhasin, S. Bhom, J. Bifani, S. Billoir, P. Birnkraut, A. Bizzeti, A. Bjørn, M. Blago, M.P. Blake, T. Blanc, F. Blusk, S. Bobulska, D. Bocci, V. Boente Garcia, O. Boettcher, T. Bondar, A. Bondar, N. Borghi, S. Borisyak, M. Borsato, M. Bossu, F. Boubdir, M. Bowcock, T.J.V. Bozzi, C. Braun, S. Brodski, M. Brodzicka, J. Brossa Gonzalo, A. Brundu, D. Buchanan, E. Buonaura, A. Burr, C. Bursche, A. Buytaert, J. Byczynski, W. Cadeddu, S. Cai, H. Calabrese, R. Calladine, R. Calvi, M. Calvo Gomez, M. Camboni, A. Campana, P. Campora Perez, D.H. Capriotti, L. Carbone, A. Carboni, G. Cardinale, R. Cardini, A. Carniti, P. Carson, L. Carvalho Akiba, K. Casse, G. Cassina, L. Cattaneo, M. Cavallero, G. Cenci, R. Chamont, D. Chapman, M.G. Charles, M. Charpentier, Ph. Chatzikonstantinidis, G. Chefdeville, M. Chekalina, V. Chen, C. Chen, S. Chitic, S.-G. Chobanova, V. Chrzaszcz, M. Chubykin, A. Ciambrone, P. Cid Vidal, X. Ciezarek, G. Clarke, P.E.L. Clemencic, M. Cliff, H.V. Closier, J. Coco, V. Coelho, J.A.B. Cogan, J. Cogneras, E. Cojocariu, L. Collins, P. Colombo, T. Comerma-Montells, A. Contu, A. Coombs, G. Centro Brasileiro de Pesquisas Físicas (CBPF) Rio de Janeiro Brazil Universidade Federal do Rio de Janeiro (UFRJ) Rio de Janeiro Brazil Center for High Energy Physics Tsinghua University Beijing China Institute Of High Energy Physics (ihep) Beijing China Univ. Grenoble Alpes Univ. Savoie Mont Blanc CNRS IN2P3-LAPP Annecy France Clermont Université Université Blaise Pascal CNRS/IN2P3 LPC Clermont-Ferrand France Aix Marseille Univ CNRS/IN2P3 CPPM Marseille France LAL Univ. Paris-Sud CNRS/IN2P3 Université Paris-Saclay Orsay France LPNHE Sorbonne Université Paris Diderot Sorbonne Paris Cité CNRS/IN2P3 Paris France I. Physikalisches Institut RWTH Aachen University Aachen Germany Fakultät Physik Technische Universität Dortmund Dortmund Germany Max-Planck-Institut für Kernphysik (MPIK) Heidelberg Germany Physikalisches Institut Ruprecht-Karls-Universität Heidelberg Heidelberg Germany School of Physics University College Dublin Dublin Ireland INFN Sezione di Bari Bari Italy INFN Sezione di Bologna Bologna Italy INFN Sezione di Ferrara Ferrara Italy INFN Sezione di Firenze Firenze Italy INFN Laboratori Nazionali di Frascati Frascati Italy INFN Sezione di Genova Genova Italy INFN Sezione di Milano-Bicocca Milano Italy INFN Sezione di Milano Milano Italy INFN Sezione di Cagliari Monserrato Italy INFN Sezione di Padova Padova Italy INFN Sezione di Pisa Pisa Italy INFN Sezione di Roma Tor Vergata Roma Italy INFN Sezione di Roma La Sapienza Roma Italy Nikhef National Institute for Subatomic Physics Amsterdam Netherlands Nikhef National Institute for Subatomic Physics and VU University Amsterdam Amsterdam Netherlands Henryk Niewodniczanski Institute of Nuclear Physics Polish Academy of Sciences Kraków Poland AGH - University of Science and Technology Faculty of Physics and Applied Computer Science Kraków Poland National Center for Nuclear Research (NCBJ) Warsaw Poland Horia Hulubei National Institute of Physics and Nuclear Engineering Bucharest

The production of ϒ(nS) mesons (n = 1, 2, 3) in pPb and Pbp collisions at a centre-of-mass energy per nucleon pair sNN=8.16 TeV is measured by the LHCb experiment, using a data sample corresponding to an integrated luminosity of 31.8 nb⁻¹. The ϒ(nS) mesons are reconstructed through their decays into two opposite-sign muons. The measurements comprise the differential production cross-sections of the ϒ(1S) and ϒ(2S) states, their forward-to-backward ratios and nuclear modification factors. The measurements are performed as a function of the transverse momentum p_T and rapidity in the nucleon-nucleon centre-of-mass frame y^* of the ϒ(nS) states, in the kinematic range p_T < 25 GeV/c and 1.5 < y^* < 4.0 (−5.0 < y^* < −2.5) for pPb (Pbp) collisions. In addition, production cross-sections for ϒ(3S) are measured integrated over phase space and the production ratios between all three ϒ(nS) states are determined. Suppression for bottomonium in proton-lead collisions is observed, which is particularly visible in the ratios. The results are compared to theoretical models.[Figure not available: see fulltext.] © 2018, The Author(s).

关键词： Heavy Ion Experiments

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Prompt Λ _c ⁺ production in pPb collisions at √sNN=5.02 TeV

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Journal of High Energy Physics 2019年第2期2019卷 1-26页

作者： Aaij, R. Adeva, B. Adinolfi, M. Aidala, C.A. Ajaltouni, Z. Akar, S. Albicocco, P. Albrecht, J. Alessio, F. Alexander, M. Alfonso Albero, A. Ali, S. Alkhazov, G. Alvarez Cartelle, P. Alves, A.A. Amato, S. Amerio, S. Amhis, Y. An, L. Anderlini, L. Andreassi, G. Andreotti, M. Andrews, J.E. Appleby, R.B. Archilli, F. d’Argent, P. Arnau Romeu, J. Artamonov, A. Artuso, M. Arzymatov, K. Aslanides, E. Atzeni, M. Audurier, B. Bachmann, S. Back, J.J. Baker, S. Balagura, V. Baldini, W. Baranov, A. Barlow, R.J. Barsuk, S. Barter, W. Baryshnikov, F. Batozskaya, V. Batsukh, B. Battista, V. Bay, A. Beddow, J. Bedeschi, F. Bediaga, I. Beiter, A. Bel, L.J. Beliy, N. Bellee, V. Belloli, N. Belous, K. Belyaev, I. Ben-Haim, E. Bencivenni, G. Benson, S. Beranek, S. Berezhnoy, A. Bernet, R. Berninghoff, D. Bertholet, E. Bertolin, A. Betancourt, C. Betti, F. Bettler, M.O. van Beuzekom, M. Bezshyiko, Ia. Bhasin, S. Bhom, J. Bifani, S. Billoir, P. Birnkraut, A. Bizzeti, A. Bjørn, M. Blago, M.P. Blake, T. Blanc, F. Blusk, S. Bobulska, D. Bocci, V. Boente Garcia, O. Boettcher, T. Bondar, A. Bondar, N. Borghi, S. Borisyak, M. Borsato, M. Bossu, F. Boubdir, M. Bowcock, T.J.V. Bozzi, C. Braun, S. Brodski, M. Brodzicka, J. Brossa Gonzalo, A. Brundu, D. Buchanan, E. Buonaura, A. Burr, C. Bursche, A. Buytaert, J. Byczynski, W. Cadeddu, S. Cai, H. Calabrese, R. Calladine, R. Calvi, M. Calvo Gomez, M. Camboni, A. Campana, P. Campora Perez, D.H. Capriotti, L. Carbone, A. Carboni, G. Cardinale, R. Cardini, A. Carniti, P. Carson, L. Carvalho Akiba, K. Casse, G. Cassina, L. Cattaneo, M. Cavallero, G. Cenci, R. Chamont, D. Chapman, M.G. Charles, M. Charpentier, Ph. Chatzikonstantinidis, G. Chefdeville, M. Chekalina, V. Chen, C. Chen, S. Chitic, S.-G. Chobanova, V. Chrzaszcz, M. Chubykin, A. Ciambrone, P. Cid Vidal, X. Ciezarek, G. Clarke, P.E.L. Clemencic, M. Cliff, H.V. Closier, J. Coco, V. Coelho, J.A.B. Cogan, J. Cogneras, E. Cojocariu, L. Collins, P. Colombo, T. Comerma-Montells, A. Contu, A. Coombs, G. Coquereau, S. Corti, G. Corvo, M. Costa Sobra Centro Brasileiro de Pesquisas Físicas (CBPF) Rio de Janeiro Brazil Universidade Federal do Rio de Janeiro (UFRJ) Rio de Janeiro Brazil Center for High Energy Physics Tsinghua University Beijing China Univ. Grenoble Alpes Univ. Savoie Mont Blanc CNRS IN2P3-LAPP Annecy France Clermont Université Université Blaise Pascal CNRS/IN2P3 LPC Clermont-Ferrand France Aix Marseille Univ CNRS/IN2P3 CPPM Marseille France LAL Univ. Paris-Sud CNRS/IN2P3 Université Paris-Saclay Orsay France LPNHE Sorbonne Université Paris Diderot Sorbonne Paris Cité CNRS/IN2P3 Paris France I. Physikalisches Institut RWTH Aachen University Aachen Germany Fakultät Physik Technische Universität Dortmund Dortmund Germany Max-Planck-Institut für Kernphysik (MPIK) Heidelberg Germany Physikalisches Institut Ruprecht-Karls-Universität Heidelberg Heidelberg Germany School of Physics University College Dublin Dublin Ireland INFN Sezione di Bari Bari Italy INFN Sezione di Bologna Bologna Italy INFN Sezione di Ferrara Ferrara Italy INFN Sezione di Firenze Firenze Italy INFN Laboratori Nazionali di Frascati Frascati Italy INFN Sezione di Genova Genova Italy INFN Sezione di Milano-Bicocca Milano Italy INFN Sezione di Milano Milano Italy INFN Sezione di Cagliari Monserrato Italy INFN Sezione di Padova Padova Italy INFN Sezione di Pisa Pisa Italy INFN Sezione di Roma Tor Vergata Roma Italy INFN Sezione di Roma La Sapienza Roma Italy Nikhef National Institute for Subatomic Physics Amsterdam Netherlands Nikhef National Institute for Subatomic Physics and VU University Amsterdam Amsterdam Netherlands Henryk Niewodniczanski Institute of Nuclear Physics Polish Academy of Sciences Kraków Poland AGH - University of Science and Technology Faculty of Physics and Applied Computer Science Kraków Poland National Center for Nuclear Research (NCBJ) Warsaw Poland Horia Hulubei National Institute of Physics and Nuclear Engineering Bucharest-Magurele Romania Petersburg Nuclear Physics Institute

The prompt production of Λ c + baryons is studied in proton-lead collisions collected with the LHCb detector at the LHC. The data sample corresponds to an integrated luminosity of 1.58 nb −1 recorded at a nucleon-nuc... 详细信息

The prompt production of Λ _c ⁺ baryons is studied in proton-lead collisions collected with the LHCb detector at the LHC. The data sample corresponds to an integrated luminosity of 1.58 nb ⁻¹ recorded at a nucleon-nucleon centre-of-mass energy of sNN=5.02 TeV. Measurements of the differential cross-section and the forwardbackward production ratio are reported for Λ _c ⁺ baryons with transverse momenta in the range 2 < p _T < 10 GeV/c and rapidities in the ranges 1.5 < y ^∗ < 4.0 and −4.5 < y ^∗ < −2.5 in the nucleon-nucleon centre-of-mass system. The ratio of cross-sections of Λ _c ⁺ baryons and D ⁰ mesons is also reported. The results are compared with next-to-leading order calculations that use nuclear parton distribution functions.[Figure not available: see fulltext.] © 2019, The Author(s).

关键词： Charm physics Forward physics Heavy Ion Experiments Heavy quark production

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Integrating Chemical Pre-Potassiation with Pre-Modulated KF-Rich Electrolyte Interfaces for Dual-Carbon Potassium Ion Hybrid Capacitor

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Angewandte Chemie 2023年第9期135卷

作者： Yong Qian Bei Wu Yang Li Zhen Pan Dr. Shuai Feng Dr. Ning Lin Prof. Yitai Qian Hefei National Laboratory for Physical Sciences at the Microscale Department of Applied Chemistry University of Science and Technology of China Hefei 230026 P. R. China Contribution: Conceptualization (lead) Formal analysis (lead) Investigation (lead) Methodology (lead) Writing - original draft (lead) Contribution: Software (equal) Visualization (lead) Contribution: Data curation (equal) Resources (equal) College of Chemistry and Chemical Engineering Taishan University Shandong 271021 P. R. China Contribution: Resources (equal) Visualization (equal) Contribution: Funding acquisition (lead) Writing - review & editing (lead) Contribution: Funding acquisition (equal)

Herein, a chemical pre-potassiation strategy via simultaneously treating both glucose derived carbon (GDC) anode and commercial activated carbon (CAC) cathode in potassium-naphthalene-tetrahydrofuran solution is developed for potassium ion hybrid capacitor (PIHC). Combined with in situ and ex situ characterizations, a radical reaction between pre-potassiation reagent and carbon electrodes is confirmed, which not only deactivates electrochemical irreversible sites, but also promotes to pre-form a uniform and dense KF-rich electrolyte film on the electrodes. As a result, the pre-potassiation treatment presents multiple advantages: (I) the initial Coulombic efficiency (CE) of the GDC anode increases from 45.4 % to 84.0 % with higher rate capability; (II) the CAC cathode exhibits the improved cycling CEs and stability due to the enhanced resistance to electrolyte oxidation at 4.2 V; (III) the assembled PIHC achieves a high energy density of 172.5 Wh kg −1 with cycling life over 10000 cycles.

关键词： Chemical Pre-Potassiation Strategy Higher Rate Capability KF-Rich Electrolyte Interface Radical Reaction the Resistance to Electrolyte Oxidation

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INTRODUCTION

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Bulletin of the American Meteorological Society 2024年第8期105卷 S1-S11页

作者： Boyer, T. Blunden, J. Dunn, R.J.H. NOAA/NESDIS National Centers for Environmental Information Silver Spring Maryland NOAA/NESDIS National Centers for Environmental Information Asheville North Carolina Met Office Hadley Centre Exeter United Kingdom European Centre for Medium-Range Weather Forecasts Reading United Kingdom University of Maryland College Park Maryland Scripps Institution of Oceanography University of California San Diego La Jolla California NOAA/NWS National Centers for Environmental Prediction Climate Prediction Center College Park Maryland Brandenburg University of Technology (BTU) Cottbus-Senftenberg Germany Servicio Meteorológico Nacional Buenos Aires Argentina NOAA/OAR Physical Sciences Laboratory Boulder Colorado European Centre for Medium-Range Weather Forecasts Bonn Germany Center for Geophysical Research and School of Physics University of Costa Rica San José Costa Rica Department of Meteorology and National Centre for Earth Observation University of Reading Reading United Kingdom Centro Nacional de Monitoramento e Alertas de Desastres Naturais CEMADEN São Paulo Brazil Université Grenoble Alpes Institut des Géosciences de l’Environnement IRD CNRS Grenoble INP Grenoble France Hampton University Hampton Virginia Seychelles Meteorological Authority Mahe Seychelles Section for Glaciers Ice and Snow Norwegian Water Resources and Energy Directorate Oslo Norway National Research Institute for Agriculture Food and Environment (INRAE) CARRTEL Université Savoie Mont Blanc Thonon les Bains France Graduate School of Agriculture Osaka Metropolitan University Sakai Japan Science Faculty Universidad Nacional de Colombia Bogotá Colombia University of Bremen Bremen Germany NOAA Global Monitoring Laboratory Boulder Colorado Servicio Nacional de Meteorología e Hidrología del Perú Lima Perú Centro de Investigaciones sobre Desertificación – Spanish National Research Council (CSIC-UV-GVA) Valencia Spain Hydro-Climate Extremes Lab (H-CEL) Ghent University Ghent Belgium Department o

In 2023, La Niña conditions that generally prevailed in the eastern Pacific Ocean from mid-2020 into early 2023 gave way to a strong El Niño by October. Atmospheric concentrations of Earth’s major greenhouse gases—carbon dioxide, methane, and nitrous oxide—all increased to record-high levels. The annual global average carbon dioxide concentration in the atmosphere rose to 419.3±0.1 ppm, which is 50% greater than the pre-industrial level. The growth from 2022 to 2023 was 2.8 ppm, the fourth highest in the record since the 1960s. The combined short-term effects of El Niño and the long-term effects of increasing levels of heat-trapping gases in the atmosphere contributed to new records for many essential climate variables reported here. The annual global temperature across land and oceans was the highest in records dating as far back as 1850, with the last seven months (June–December) having each been record warm. Over land, the globally averaged temperature was also record high. Dozens of countries reported record or near-record warmth for the year, including China and continental Europe as a whole (warmest on record), India and Russia (second warmest), and Canada (third warmest). Intense and widespread heatwaves were reported around the world. In Vietnam, an all-time national maximum temperature record of 44.2°C was observed at Tuong Duong on 7 May, surpassing the previous record of 43.4°C at Huong Khe on 20 April 2019. In Brazil, the air temperature reached 44.8°C in Araçuaí in Minas Gerais on 20 November, potentially a new national record and 12.8°C above normal. The effect of rising temperatures was apparent in the cryosphere, where snow cover extent by June 2023 was the smallest in the 56-year record for North America and seventh smallest for the Northern Hemisphere overall. Heatwaves contributed to the greatest average mass balance loss for Alpine glaciers around the world since the start of the record in 1970. Due to rapid volume loss beginning in 2021, St. A

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Evidence of a J/ψΛstructure and observation of excited■^(-)states in the■b^(-)→J/ψΛK^(-) decay

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Science Bulletin 2021年第13期66卷 1278-1287,M0003页

作者： R.Aaij C.Abellán Beteta T.Ackernley B.Adeva M.Adinolfi H.Afsharnia C.A.Aidala S.Aiola Z.Ajaltouni S.Akar J.Albrecht F.Alessio M.Alexander A.Alfonso Albero Z.Aliouche G.Alkhazov P.Alvarez Cartelle S.Amato Y.Amhis L.An L.Anderlini A.Andreianov M.Andreotti F.Archilli A.Artamonov M.Artuso K.Arzymatov E.Aslanides M.Atzeni B.Audurier S.Bachmann M.Bachmayer J.J.Back S.Baker P.Baladron Rodriguez V.Balagura W.Baldini J.Baptista Leite R.J.Barlow S.Barsuk W.Barter M.Bartolini F.Baryshnikov J.M.Basels G.Bassi B.Batsukh A.Battig A.Bay M.Becker F.Bedeschi I.Bediaga A.Beiter V.Belavin S.Belin V.Bellee K.Belous I.Belov I.Belyaev G.Bencivenni E.Ben-Haim A.Berezhnoy *** D.Berninghoff H.C.Bernstein C.Bertella E.Bertholet A.Bertolin C.Betancourt F.Betti Ia.Bezshyiko S.Bhasin J.Bhom L.Bian M.S.Bieker S.Bifani P.Billoir M.Birch F.C.R.Bishop A.Bizzeti M.Bj┆rn M.P.Blago T.Blake F.Blanc S.Blusk D.Bobulska J.A.Boelhauve O.Boente Garcia T.Boettcher A.Boldyrev A.Bondar N.Bondar S.Borghi M.Borisyak M.Borsato J.T.Borsuk S.A.Bouchiba T.J.V.Bowcock A.Boyer C.Bozzi M.J.Bradley S.Braun A.Brea Rodriguez M.Brodski J.Brodzicka A.Brossa Gonzalo D.Brundu A.Buonaura C.Burr A.Bursche A.Butkevich J.S.Butter J.Buytaert W.Byczynski S.Cadeddu H.Cai R.Calabrese L.Calefice L.Calero Diaz S.Cali R.Calladine M.Calvi M.Calvo Gomez P.Camargo Magalhaes A.Camboni P.Campana A.F.Campoverde Quezada S.Capelli L.Capriotti A.Carbone G.Carboni R.Cardinale A.Cardini I.Carli P.Carniti L.Carus K.Carvalho Akiba A.Casais Vidal G.Casse M.Cattaneo G.Cavallero S.Celani J.Cerasoli A.J.Chadwick M.G.Chapman M.Charles Ph.Charpentier G.Chatzikonstantinidis C.A.Chavez Barajas M.Chefdeville C.Chen S.Chen A.Chernov S.-G.Chitic V.Chobanova S.Cholak M.Chrzaszcz A.Chubykin V.Chulikov P.Ciambrone M.F.Cicala X.Cid Vidal G.Ciezarek P.E.L.Clarke M.Clemencic H.V.Cliff J.Closier J.L.Cobbledick V.Coco J.A.B.Coelho J.Cogan E.Cogneras L.Cojocariu P.Collins T.Colombo L.Congedo A.Contu N.Cooke G.Coombs G.Corti C.M.Costa Sobral B.Couturier D.C.Craik J.Crkovská M.Cruz Torres R.Currie C.L.Da Silva E.Dall’ Centro Brasileiro de Pesquisas Físicas(CBPF) Rio de JaneiroBrazil Universidade Federal do Rio de Janeiro(UFRJ) Rio de JaneiroBrazil Center for High Energy Physics Tsinghua UniversityBeijingChina School of Physics State Key Laboratory of Nuclear Physics and Technology Peking UniversityBeijingChina University of Chinese Academy of Sciences BeijingChina Institute Of High Energy Physics(IHEP) BeijingChina Institute of Particle Physics Central China Normal UniversityWuhanHubeiChina Univ.Grenoble Alpes Univ.Savoie Mont BlancCNRSIN2P3-LAPPAnnecyFrance UniversitéClermont Auvergne CNRS/IN2P3LPCClermont-FerrandFrance Aix Marseille Univ CNRS/IN2P3CPPMMarseilleFrance UniversitéParis-Saclay CNRS/IN2P3IJCLabOrsayFrance Laboratoire Leprince-ringuet(llr) PalaiseauFrance LPNHE Sorbonne UniversitéParis Diderot Sorbonne Paris CitéCNRS/IN2P3ParisFrance I.Physikalisches Institut RWTH Aachen UniversityAachenGermany Fakultät Physik Technische Universität DortmundDortmundGermany Max-Planck-Institut für Kernphysik(MPIK) HeidelbergGermany Physikalisches Institut Ruprecht-Karls-Universität HeidelbergHeidelbergGermany School of Physics University College DublinDublinIreland INFN Sezione di Bari BariItaly INFN Sezione di Bologna BolognaItaly INFN Sezione di Ferrara FerraraItaly INFN Sezione di Firenze FirenzeItaly INFN Laboratori Nazionali di Frascati FrascatiItaly INFN Sezione di Genova GenovaItaly INFN Sezione di Milano-Bicocca MilanoItaly INFN Sezione di Milano MilanoItaly INFN Sezione di Cagliari MonserratoItaly Universita degli Studi di Padova Universita e INFNPadovaPadovaItaly INFN Sezione di Pisa PisaItaly INFN Sezione di Roma Tor Vergata RomaItaly INFN Sezione di Roma La Sapienza RomaItaly Nikhef National Institute for Subatomic Physics AmsterdamNetherlands Nikhef National Institute for Subatomic Physics and VU University Amsterdam AmsterdamNetherlands Henryk Niewodniczanski Institute of Nuclear Physics Polish Academy of Sciences KrakówPoland AGH-University of Science and Techno

First evidence of a structure in the J/ψΛinvariant mass distribution is obtained from an amplitude analysis of■b^(-)J/ψΛK^(-)*** observed structure is consistent with being due to a charmonium pentaquark with strangeness with a significance of 3.1r including systematic uncertainties and lookelsewhere *** mass and width are determined to be 4458:8±2:9t4:7-1:1 MeV and 17:3±6:5t8:0-5:7 MeV,respectively,where the quoted uncertainties are statistical and *** structure is also consistent with being due to two *** addition,the narrow excited■^(-)states,N■(1690)and■(1820),are seen for the first time in a■b^(-)decay,and their masses and widths are measured with improved *** analysis is performed using pp collision data corresponding to a total integrated luminosity of 9 fb^(-1),collected with the LHCb experiment at centre-of-mass energies of 7,8 and 13 TeV.

关键词： QCD Exotics Pentaquark Spectroscopy Quarkonium Particle and resonance production

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