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arXiv 2017年

作者： Tawfik, Sherif Abdulkader Ali, Sajid Fronzi, Marco Kianinia, Mehran Tran, Toan Trong Stampfl, Catherine Aharonovich, Igor Toth, Milos Ford, Michael J. School of Mathematical and Physical Sciences University of Technology Sydney UltimoNSW2007 Australia Department of Physics GC University Faisalabad Allama Iqbal Road Faisalabad38000 Pakistan International Research Centre for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an Shaanxi710049 China School of Physics University of Sydney NSW2006 Australia

Hexagonal boron nitride (hBN) has recently emerged as a fascinating platform for room-temperature quantum photonics due to the discovery of robust visible light single-photon emitters. In order to utilize these emitters, it is necessary to have a clear understanding of their atomic structure and the associated excitation processes that give rise to this single photon emission. Here we perform density-functional theory (DFT) and constrained DFT calculations for a range of hBN point defects in order to identify potential emission candidates. By applying a number of criteria on the electronic structure of the ground state and the atomic structure of the excited states of the considered defects, and then calculating the Huang-Rhys (HR) factor, we find that the CBVN defect, in which a carbon atom substitutes a boron atom and the opposite nitrogen atom is removed, is a potential emission source with a HR factor of 1.66, in good agreement with the experimental HR factor. We calculate the photoluminescence (PL) line shape for this defect and find that it reproduces a number of key features in the the experimental PL lineshape. Copyright © 2017, The Authors. All rights reserved.

关键词： III-V semiconductors

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Facile Synthesis of Bulk Au-Co-Coox-Ceox@Iron Ball and its Photocatalytic Application in 4-Nitrophenol Degradation

SSRN

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SSRN 2023年

作者： Sun, Li Qiao, Zhili Zhi, Yuan Zhang, Hua Dou, Binlin Shan, Yuejin Huang, Weijia School of Energy and Power Engineering University of Shanghai for Science and Technology Jun Gong Road 516 Shanghai200093 China R&D Department Shanghai Minrula Biotechnology Co.Ltd Building 15 Haji Sixth Road 218 Shanghai201306 China Department of Material and Environmental Chemistry Research Division of Functional Materials Design Utsunomiya University Yoto 7-1-2 Utsunomiya321-8585 Japan Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering China

Bulk noble metal-semiconductor composites can be chosen as photocatalysts to carry out the continuous-flow (C-F) degradation of 4-nitrophenol (4-NP) whereas their preparation is complex and uncontrollable. Here, bulk Au/Co-CC@iron ball is designed and prepared by a facile and controllable route without any toxic chemical. The bulk Au/Co-CC@iron ball shows excellent photocatalytic activity and reusability for the 4-NP degradation, which can be ascribed to the synergistic action of active components and foliated iron ball surface. Furthermore, the highly active Au/Co-CC@iron ball is used as packing material to construct a new-type of packed reactor, by which the C-F degradation of 4-NP is successfully achieved. As-fabricated packed reactor and its tandem module exhibit superior photocatalytic performance for the C-F degradation of 4-NP. Noteworthy, based on the tandem module with six reactors, the removal rate of 4-NP can reach up to 2750 µmol/h. Meanwhile, the reactor and its module display satisfactory operational stability and reusability in the C-F degradation of 4-NP. Clearly, the provided route is effective for the preparation of bulk noble metal-semiconductor composites with exceptional performance, which can also be a prospective strategy to obtain bulk packing materials to serve for the C-F degradation. © 2023, The Authors. All rights reserved.

关键词： Precious metals

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Theoretical investigation on heat-electricity decoupling technology of low-pressure steam turbine renovation for CHPs

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IOP Conference Series: Earth and Environmental Science 2019年第4期227卷

作者： Qingbo Hu Kun Wang Li Zhang Liansheng Zhou Rong Chen Shan Wang Yu Zhang Guohao Li Tianjin Electric Power Science & Research Institute Tianjin 300384 State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiao Tong University Xi'an 710049.

The power grid peaking capacity is insufficient due to the increasing installed capacity of renewable power. Moreover, it is also restricted by the operation mode of combined heat and power units (CHPs), the minimum electricity loads of which are determined by the heat load. It is significant to study the heat-electricity decoupling technologies for CHPs. Therefore, the low-pressure steam turbine renovation technology is studied in this paper with a 300MW unit as reference case. Results show that the minimum electric load rate and the coal consumption are decreased, and the heat-electricity ratio is increased significantly for CHP with low-pressure steam turbine renovation. When the heat load is 1200 GJ/h, the minimum electric load rate and coal consumption with low-pressure steam turbine renovation can be reduced by 32.4 and 30.9 % respectively. The heat-electricity ratio can be increased by 68.8 % after renovation of low-pressure steam turbine.

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Non-Hermitian delocalization in a 2D photonic quasicrystal

arXiv

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arXiv 2023年

作者： Zhang, Zhaoyang Liang, Shun Septembre, Ismaël Yu, Jiawei Huang, Yongping Liu, Maochang Zhang, Yanpeng Xiao, Min Malpuech, Guillaume Solnyshkov, Dmitry Key Laboratory for Physical Electronics and Devices The Ministry of Education Shaanxi Key Lab of Information Photonic Technique School of Electronic Science and Engineering Faculty of Electronics and Information Xi’an Jiaotong University Xi’an710049 China Institut Pascal PHOTON-N2 Université Clermont Auvergne CNRS Clermont INP Clermont-FerrandF-63000 France International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Department of Physics University of Arkansas FayettevilleAR72701 United States National Laboratory of Solid State Microstructures School of Physics Nanjing University Nanjing210093 China Paris75231 France

Quasicrystals show long-range order, but lack translational symmetry. So far, theoretical and experimental studies suggest that both Hermitian and non-Hermitian quasicrystals show localized eigenstates. This localization is due to the fractal structure of the spectrum in the Hermitian case and to the transition to diffusive bands via exceptional points in the non-Hermitian case. Here, we present an experimental study of a dodecagonal (12-fold) photonic quasicrystal based on electromagnetically-induced transparency in a Rb vapor cell. The transition to a quasicrystal is obtained by superposing two honeycomb lattices at 30◦ with a continuous tuning of their amplitudes. Non-Hermiticity is controlled independently. We study the spatial expansion of a probe wavepacket. In the Hermitian case, the wavepacket expansion is suppressed when the amplitude of the second lattice is increased (quasicrystal localization). We find a new regime, where increasing the non-Hermitian potential in the quasicrystal enhances spatial expansion, with the C12 symmetry becoming visible in the wavepacket structure. This real-space expansion is due to a k-space localization on specific quasicrystal modes. Our results show that the non-Hermitian quasicrystal behavior is richer than previously thought. The localization properties of the quasicrystals can be used for beam tailoring in photonics, but are also important in other fields. Copyright © 2023, The Authors. All rights reserved.

关键词： Quasicrystals

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Boosted Photocatalytic Co2 Reduction by Induced Electromotive Force in Rotating Magnetic Field

SSRN

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SSRN 2023年

作者： Lu, Danchen Ren, Yuqi Yang, Ya Cheng, Miao Wang, Ke Wang, Nan Liu, Maochang Zhou, Jiancheng Chen, Wenshuai Li, Naixu School of Chemistry and Chemical Engineering Southeast University No.2 Dongnandaxue Road Jiangsu Nanjing211189 China CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-nano Energy and Sensor Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of Sciences Beijing101400 China Key Laboratory of Bio-Based Material Science and Technology Ministry of Education Northeast Forestry University No. 26 Hexing Road Harbin150040 China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University No.28 Xianning West Road Shaanxi Xi'An710049 China

Charge separation plays a crucial role in semiconductor-based photocatalytic CO2 conversion. Herein, we report a unique induced electric field, which can actively manipulate carrier behavior at the minuscule, leading to significantly boosted photocatalytic CO2 reduction in H2O vapor. The success relies on the development a monolithic photocatalyst made of a copper foam substrate and nanosized ZnO/NiO/Au heterostructures that can effectively couple a special rotating magnetic field (RMF). Specifically, the copper foam cuts the magnetic induction line, leading to the periodic generation of induced electric field. This induced electric field could significantly increase the carriers' density by preventing their recombination. Moreover, NiO and Au as the active sites for oxidation and reduction, respective, synergistically magnify this effect. As a result, compared with the photocatalytic reaction without adding RMF, the utilization rate of photogenerated electrons increases by 5.24 times after coupling RMF, with the yield of CO and CH4 improved by 5.50 times and 5.18 times. This strategy by integrating unique RMF into the reaction system provides new insights for improving photocatalytic CO2 conversion. © 2023, The Authors. All rights reserved.

关键词： Carbon dioxide

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Corrigendum to “Huge wave and drop entrainment mechanism in gas–liquid churn flow” [Chem. Eng. Sci. 108 (2013) 638–646]

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Chemical engineering Science 2017年 158卷 624-624页

作者： Ke Wang Bofeng Bai Weimin Ma State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi 710049 China Royal Institute of Technology (KTH) Stockholm 10691 Sweden

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Erosion of water-based fracturing fluid containing particles in a sudden contraction of horizontal pipe

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Journal of Physics: Conference Series 2017年第1期916卷

作者： Jiarui Cheng Yinping Cao Yihua Dou Zhen Li State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China. Department of Mechanical Engineering Xi'an Shiyou University Xi'an China.

A lab experiment was carried out to study the effects of pipe flow rate, particle concentration and pipe inner diameter ratio on proppant erosion of the reducing wall in hydraulic fracturing. The results show that the erosion rate and erosion distribution are different not only in radial direction but also in circumferential direction of the sample. The upper part of sample always has a minimum erosion rate and erosion area. Besides, the erosion rate of reducing wall is most affected by fluid flow velocity, and the erosion area is most sensitive to the change in the diameter ratio. Meanwhile, the erosion rate of reducing wall in crosslinked fracturing fluid is mainly determined by the fluid flowing state due to the high viscosity of the liquid. In general, the increase in flow velocity and diameter ratio not only cause the expansion of erosion-affected flow region in sudden contraction section, but also lead to more particles impact the wall.

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Numerical Study of Percolation and Seepage Behaviors in Ion-Adsorption-Type Rare Earth Ore Leaching Process

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Mathematical Problems in engineering 2023年第1期2023卷

作者： Dianyu, E. Su, Zhongfang Zeng, Jia Yang, Liuyimei Li, Jing Xu, Qiang Wang, Lin Cui, Jiaxin Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi University of Science and Technology Nanchang330013 China International Institute for Innovation Jiangxi University of Science and Technology Nanchang330013 China Ganjiang Innovation Academy Chinese Academy of Sciences Ganzhou341000 China ARC Research Hub for Computational Particle Technology Department of Chemical and Biological Engineering Monash University ClaytonVIC3800 Australia State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an710049 China Delft University of Technology Delft Netherlands

Ionic rare earth ore is a type of featured rare earth ore in China. Its mining process suffers from a long leaching cycle and considerable consumption of leaching agents. Improving mining efficiency requires a sound physical understanding of the leaching process. In this study, the CFD-based numerical model is used to analyze the physical process of leaching through porous media formed by particles. The simulation results indicate that a lower packing porosity and smaller particles packed granular porous medium result in much larger energy dissipation during seepage, and the energy dissipation increases with seepage velocity. It is found that when the seepage velocity increases to a certain high value, the energy dissipation exceeds the value predicted by Darcy's law, which is mainly caused by liquid turbulence. Additionally, the effect of particle shape is examined. The results show that the granular medium composed of prolate particles causes larger energy dissipation than oblate particles, and spherical particles play the least role. This phenomenon may result from the particle shape affecting the area of the frontal contact surface between particles and liquid. The results provide new insights into the fundamental understanding of percolation and seepage behaviors in the ion-adsorption-type rare earth ore leaching process. © 2023 E. Dianyu et al.

关键词： Energy dissipation

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聚丙烯酸酯修饰铜电极用于电化学二氧化碳还原选择性生成多碳产物（英文）

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Science Bulletin 2024年第15期 2395-2404页

作者：石玉川张凯妮董崇礼 Ta Thi Thuy Nga 汪淼魏代星王佳琳王亦清沈少华 International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Department of Physics Tamkang University

Highly selective production of value-added multicarbon(C2+) products via electrochemical CO2reduction reaction（eCO2RR） on polycrystalline copper（Cu） remains ***,the facile surface modification using poly（α-ethyl cyanoacrylate）(PECA) is presented to greatly enhance the C2+selectivity for eCO2RR over polycrystalline Cu,with Faradaic efficiency（FE） towards C2+products increased from30.1% for the Cu electrode to 72.6% for the obtained Cu-PECA electrode at -1.1 V *** hydrogen electrode（RHE）.Given the well-determined FEs towards C2+products,the partial current densities for C2+production could be estimated to be-145.4 mA cm-2for the Cu-PECA electrode at -0.9 V *** in a homemade flow ***-situ spectral characterizations and theoretical calculations reveal that PECA featured with electron-accepting-C≡N and-COOR groups decorated onto the Cu electrode could inhibit the adsorption of *H intermediates and stabilize the *CO intermediates,given the redistributed interfacial electron density and the raised energy level of d-band center（Ed） of Cu active sites,thus facilitating the C-C coupling and then the C2+selective *** study is believed to be guidable to the modification of electrocatalysts and electrodes with polymers to steer the surface adsorption behaviors of reaction intermediates to realize practical eCO2RR towards value-added C2+products with high activity and selectivity.

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Activated Overall Water Splitting Over a Ni-Fe Layered Double Hydroxide Electrocatalyst by V Doping and Sulfuration

SSRN

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SSRN 2023年

作者： Wu, Wentong Peng, Lei Min, Boya Huang, Jie Liu, Saiya Lu, Kejian Lu, Shijian Jing, Dengwei Zheng, Mingsheng Liu, Maochang International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China No. 8 Oil Production Plant of PetroChina Changqing Oilfield Company Shaanxi Xi’an710016 China Carbon Neutrality Institute Jiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization China University of Mining and Technology Jiangsu Xuzhou221008 China Gree Altairnano New Energy Inc Zhuhai519040 China School of Chemistry and Biological Engineering University of Science and Technology Beijing Beijing100083 China

Ni-Fe layered double hydroxide (NiFe-LDH) is regarded as one of the promising non-noble electrocatalyst. However, the limited number of active sites and poor electrical conductivity impede its further development. Herein, we report the synthesis of a Ni foam supported NiFe-LDH electrocatalyst modified by V doping and vulcanization (NiFeV-S/NF). This modification endows the catalyst excellent property toward hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and overall water splitting. Only 211 mV and 127 mV of the overpotentials are required to achieve the current density of 10 mA cm-2 for OER and HER in 1 M KOH electrolyte, respectively. Particularly, the prepared NiFeV-S/NF could serve as a bifunctional electrocatalyst for overall water splitting, with a cell voltage of 1.573 V to reach a current density of 10 mA cm-2. In principle, the success relies on the intrinsically improved conductivity, increased specific surface area and the number of active sites, as well as the heterojunction structure of the catalyst. Therefore, this work provides a new idea for the design and preparation of more efficient noble-metal-free bifunctional electrocatalysts. © 2023, The Authors. All rights reserved.

关键词： Electrocatalysts

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