检索结果-内蒙古大学图书馆

SSRN 2022年

作者： Liu, Jing-Nan Zhang, Meng-Meng Zhang, Lin-Xin Di, Jiang-Lei Zhao, Jian-Lin Gao, Ming Sun, Yue-Dong Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering University of Shanghai for Science and Technology Shanghai200093 China MOE Key Laboratory of Material Physics and Chemistry under Extraordinary Conditions Shaanxi Key Laboratory of Optical Information Technology School of Physical Science and Technology Northwestern Polytechnical University Shaanxi Xi’an710129 China Advanced Institute of Photonics Technology School of Information Engineering Guangdong Provincial Key Laboratory of Information Photonics Technology Guangdong University of Technology Guangzhou51006 China

To study the heat and mass transfer between evaporating water film and air in limited space, the temperature and humidity distributions of air near the flowing water film was measured using dual-wavelength digital holographic interference (DHI). The holograms were recorded by CMOS with two different wavelengths of 532 nm and 671 nm. We derived the relationships between the phase changes reconstructed from the holograms and the air temperature and humidity changes based on the Edlen formulas. A experimental model was built to generate steady water film and demonstrate the heat and mass transfer in air countercurrent to the water film, which flows down on the copper plate. The model has two symmetrical tunnels isolated by a copper plate in the middle, allowing to compare the cases of heat mass transfer with and without evaporation. The relative measurement errors of temperature and humidity are less than x% and y%, respectively, by comparing the reconstructed results with the sensor measured values. Based on the measurement results, the concept, feature transfer distance (FTD), is proposed, which characterizes the intensity of heat and mass transfer. By analyzing FTD, the main influencing factors of heat and mass transfer were obtained. © 2022, The Authors. All rights reserved.

关键词： Evaporation

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High loading cotton cellulose-based aerogel self-standing electrode for Li-S batteries

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Science Bulletin 2020年第10期65卷 803-811,M0003页

作者： Heng Mao Limin Liu Lei Shi HuWu Jinxin Lang Ke Wang Tianxiang Zhu Yiyang Gao Zehui Sun Jing Zhao Guoxin Gao Dongyang Zhang Wei Yan Shujiang Ding Xi’an Key Laboratory of Sustainable Energy Materials Chemistry State Key Laboratory of Electrical Insulation and Power EquipmentDepartment of Applied ChemistrySchool of ScienceXi’an Jiaotong UniversityXi’an 710049China Department of Environmental Science and Engineering State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China

Lithium-sulfur(Li-S) batteries have attracted considerable attention due to their high energy density(2600 Wh kg-1). However, its commercialization is hindered seriously by the low loading and utilization rate of sulfur cathodes. Herein, we designed the cellulose-based graphene carbon composite aerogel(CCA) self-standing electrode to enhance the performance of Li-S batteries. The CCA contributes to the mass loading and utilization efficiency of sulfur, because of its unique physical structure: low density(0.018 g cm-3), large specific surface area(657.85 m2 g-1), high porosity(96%), and remarkable electrolyte adsorption(42.25 times). Compared to Al(about 49%), the CCA displayed excellent sulfur use efficiency(86%) and could reach to high area capacity of 8.60 mAh cm-2 with 9.11 mgS loading. Meanwhile,the CCA exhibits the excellent potential for pulse sensing applications due to its flexibility and superior sensitivity to electrical response signals.

关键词： Cellulose-based graphene aerogel Self-standing electrode High sulfur loading Lithium-sulfur battery Pulse sensing

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Customizable Ligand Exchange for Tailored Surface Property of Noble Metal Nanocrystals

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Research 2020年第1期2020卷 292-303页

作者： Qikui Fan Hao Yang Juan Ge Shumeng Zhang Zhaojun Liu Bo Lei Tao Cheng Youyong Li Yadong Yin Chuanbo Gao Frontier Institute of Science and Technology State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’anShaanxi 710054China Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesJoint International Research Laboratory of Carbon-Based Functional Materials and DevicesSoochow UniversitySuzhouJiangsu 215123China Department of Chemistry University of CaliforniaRiversideCalifornia 92521USA

It is highly desirable,while still challenging,to obtain noble metal nanocrystals with custom capping ligands,because their colloidal synthesis relies on specific capping ligands for the shape control while conventional ligand exchange processes suffer from“the strong replaces the weak”limitation,which greatly hinders their ***,we report a general and effective ligand exchange approach that can replace the native capping ligands of noble metal nanocrystals with virtually any type of ligands,producing flexibly tailored surface *** key is to use diethylamine with conveniently switchable binding affinity to the metal surface as an intermediate *** a strong ligand,it in its original form can effectively remove the native ligands;while protonated,it loses its binding affinity and facilitates the adsorption of new ligands,especially weak ones,onto the metal *** this means,the irreversible order in the conventional ligand exchange processes could be *** efficacy of the strategy is demonstrated by mutual exchange of the capping ligands among cetyltrimethylammonium,citrate,polyvinylpyrrolidone,and *** novel strategy significantly expands our ability to manipulate the surface property of noble metal nanocrystals and extends their applicability to a wide range of fields,particularly biomedical applications.

关键词： properties replace mutual

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Chemical looping based ammonia production--A promising pathway for production of the noncarbon fuel

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Science Bulletin 2022年第20期67卷 2124-2138,M0004页

作者： Qinghua Lai Tianyi Cai Shik Chi Edman Tsang Xia Chen Runping Ye Zhenghe Xu Morris D.Argyle Dong Ding Yongmei Chen Jianji Wang Armistead G.Russell Ye Wu Jian Liu Maohong Fan College of Engineering and Applied Science University of WyomingLaramie WY 82071USA School of Energy and Power Engineering Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power EngineeringUniversity of Shanghai for Science and TechnologyShanghai 200093China Wolfson Catalysis Department of ChemistryUniversity of OxfordOxford Ox13QRUK College of Chemistry and Chemical Engineering Ocean University of ChinaQingdao 266100China State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Department of Chemical and Materials Engineering University of AlbertaEdmonton Alberta T6G1H9Canada Department of Chemical Engineering Brigham Young UniversityProvo UT 84602USA Idaho National Laboratory Idaho Falls ID83415USA College of Chemistry Beijing University of Chemical TechnologyBejing 100029China School of Chemistry and Environmental Science Henan Normal UniversityXinxiang 453007China School of Civil and Environmental Engineering Georgia Institute of TechnologyAtlanta GA 30332USA MIIT Key Laboratory of Thermal Control of Electronic Equipment School of Power EngineeringNanjing University of Science&TechnologyNanjing 210094China DICP-Surrey Joint Centre for Future Materials Department of Chemical and Process Engineeringand Advanced Technology InstituteUniversity of SurreyGuilford Surrey GU27XH UK

Ammonia, primarily made with Haber-Bosch process developed in 1909 and winning two Nobel prizes, is a promising noncarbon fuel for preventing global warming of 1.5 °C above pre-industrial levels. However,the undesired characteristics of the process, including high carbon footprint, necessitate alternative ammonia synthesis methods, and among them is chemical looping ammonia production(CLAP) that uses nitrogen carrier materials and operates at atmospheric pressure with high product selectivity and energy efficiency. To date, neither a systematic review nor a perspective in nitrogen carriers and CLAP has been reported in the critical area. Thus, this work not only assesses the previous results of CLAP but also provides perspectives towards the future of CLAP. It classifies, characterizes, and holistically analyzes the fundamentally different CLAP pathways and discusses the ways of further improving the CLAP performance with the assistance of plasma technology and artificial intelligence(AI).

关键词： Ammonia synthesis Chemical looping Nitrogen carrier Renewable fuels Energy carrier

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Thermal-mechanical coupling behavior analysis of solid-state constrained component in advanced nuclear energy system

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Energy 2025年 330卷

作者： Xuan Yang Quan Li Jing Zhang Yingwei Wu Yanan He Chenxi Li Mingjun Wang Kailun Guo Chenglong Wang G.H. Su Wenxi Tian Suizheng Qiu State Key Laboratory of Multiphase Flow in Power Engineering School of Nuclear Science and Technology Xi'an Jiaotong University Xi'an 710049 China Science and Technology on Reactor System Design Technology Laboratory Nuclear Power Institute of China Chengdu 610213 China

With the advantage of phase change heat transfer, heat pipes have the potential to replace flowing coolants for removing fission heat from nuclear reactors. However, the solid-state constrained heat transfer configuration poses mutual constraints between mechanical properties and heat transfer, and their long-term thermal-mechanical coupling behavior requires further investigation. Currently, research on long-term behavior is limited to either individual/local system components or a single physical field. In this paper, an analysis method for coupled thermal-mechanical behavior is proposed and verified, comprehensively considering thermal-mechanical properties, interactions between components, and the fission gas release. This method is employed to analyze the operating characteristics of a solid-state constrained component. The results indicate that prolonged operation leads to complete contact between structural components, generating high contact pressure that enhances heat transfer but increases creep. The release of gaseous fission products, accumulated over operating time, results in a synchronous increase in both gap and external contact pressures, reaching 5.2 MPa and 4.8 MPa, respectively. This process reduces the gas gap conductance, leading to elevated system peak temperatures and a reduction in temperature safety margins by 43 K. After heat pipe failure, continued operation significantly increases the local creep strain, up to 3.9 times that under normal conditions. The gap size and fuel gap pressure should be optimized to enhance gap heat transfer and reduce component creep. Excessive fission gas release should be avoided in fuel configuration. Reducing the system power following a single heat pipe failure can mitigate component creep and extend the operational lifespan.

关键词： Electric heating

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Mxene-Derived Ni/Tio2-X/Ti3c2 Catalyst for Enhanced Photothermal Co2 Methanation: Unraveling the Roles of Photoexcited Carriers

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SSRN 2025年

作者： Sun, Fan Xin, Yu Xing, Xueli Lou, Jiahui Wang, Qiliang Hong, Hui International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing100190 China School of Aeronautics and Astronautics University of Chinese Academy of Sciences Beijing100049 China Huaneng Clean Energy Research Institute Beijing102209 China Shandong Institute of Advanced Technology Jinan250100 China Department of Architecture and Built Environment University of Nottingham NottinghamNG7 2RD United Kingdom Institute of Engineering Thermophysics China

Photothermal catalysis has emerged as a promising approach for CO2 conversion, which combines photo and thermal energy to drive catalytic reactions efficiently. While light can lower activation barriers and enhance reaction rates, the interplay between light and heat within the catalytic framework remains largely unexplored. In this study, we investigate the critical role of photoexcited carriers in enhancing catalytic performance under solar irradiation, unraveling their contribution to the CO2-to-CH4 conversion process. A multilayer accordion-like Ni/TiO2-x/Ti3C2 catalyst, which exhibits excellent photothermal and photoelectric response characteristics was fabricated for efficient photothermal CO2 methanation. Experimental results demonstrated that introduction of light during thermal catalysis markedly enhanced the CO2 conversion rate, with a 55% increase achieved at 275 ºC. Furthermore, the required temperature for maximum CO2 conversion rate was reduced by 50 ºC compared to the thermal-driven process. Meanwhile, the effects of concentrated ratio and incident wavelength on CO2 conversion were also examined, revealing a synergistic effect between photogenerated carriers and thermal energy. Further characterizations, including steady-state and transient photoluminescence spectroscopy, in-situ XPS, in-situ EPR, in-situ DRITFs, were employed to elucidate the enhancement mechanisms of photogenerated carriers in the catalytic reaction. At the same time, an outdoor experimental prototype was developed to verify the feasibility of photogenerated carrier-thermal synergistically driven CO2 methanation. The findings provide valuable insights into the role of photo-generated carriers in photothermal CO2 methanation, offering new perspectives for the design of efficient photothermal catalysts and advancing solar catalytic CO2 conversion technologies. © 2025, The Authors. All rights reserved.

关键词： Methanation

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Research on control strategies for rapid load decrease events in fluoride salt reactor-supercritical CO2 Brayton cycle systems

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Nuclear engineering and Design 2025年 439卷

作者： Shichang, Yun Xinyu, Li Dalin, Zhang Ping, Song Wenxi, Tian Suizheng, Qiu Guanghui, Su State Key Laboratory of Multiphase Flow in Power Engineering Shaanxi Key Laboratory of Advanced Nuclear Energy and Technology School of Nuclear Science and Technology Xi'an Jiaotong University Xi'an710049 China State Key Laboratory of Marine Thermal Power Technology Wuhan Second Ship Design and Research Institute Wuhan China

This study delves into the control strategies for the Fluoride-salt-cooled High-temperature Reactor-Supercritical CO2 (SCO2) Brayton cycle power generation system under rapid grid load reduction scenarios. By developing a dynamic simulation model, the system's dynamic response characteristics under rapid load changes were analyzed, and a combined control strategy emphasizing safety, speed, and economic efficiency was proposed. The research first compared the dynamic response characteristics and steady-state performance of different bypass configurations under load rejection conditions. The computational results indicate that all three bypass control systems exhibit excellent load-following capabilities, effectively responding to a 50 % load step change within 10 s. However, significant differences were observed in their steady-state thermodynamic performance: the upper cycle bypass control achieves the highest steady-state efficiency (η = 29.92 %), followed by the turbine bypass control (η = 27.50 %), with the heat source bypass control showing relatively lower efficiency (η = 26.49 %). Although the upper cycle bypass offers superior efficiency, it leads to a substantial increase in the working fluid flow through the compressor (ΔQ = 15 %) during operation, raising the risk of compressor blockage and necessitating additional flow restriction and anti-blocking interlock control systems. Considering system safety, control complexity, and engineering feasibility, the turbine bypass system, with its relative independence and lower operational risk, is deemed more suitable as the primary control strategy for load rejection conditions. Building on this, the study proposes a combined control strategy that leverages the strengths of both bypass control and inventory control. During the initial phase of rapid load reduction, the bypass control system quickly adjusts the turbine bypass valve opening to promptly respond to grid load changes, ensuring system frequency stability

关键词： Frequency stability

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Cavitation characteristics of rotary vane pump in aeroengine lubricating oil system and their effects on pump performance

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Hangkong Dongli Xuebao/Journal of Aerospace power 2025年第7期40卷

作者： Wang, Ge Wang, Yijin He, Denghui Yang, Lina Cao, Ming Bai, Bofeng State Key Laboratory of Eco-hydraulic in Northwest Arid Region of China Xi’an University of Technology Xi’an710048 China Department of Power Engineering Institute of Water Resources and Hydro-electric Engineering Xi’an University of Technology Xi’an710048 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Commercial Aircraft Engine Company Limited Aero Engine Corporation of China Shanghai200241 China Shanghai Center of Research for Commercial Aircraft Engine Engineering Techniques Shanghai200241 China

To meet the demand for high-performance oil pumps in the lubricating oil system of high thrust and high-speed aeroengines, numerical simulation was conducted on a new high-speed rotary vane oil pump. The Mixture multiphase flow model, Singhal full cavitation model, and renormalization group（RNG） k-Ε turbulence model were employed for numerical calculation, and the reliability of the numerical simulation method was verified through experiments. Then, cavitation characteristics of the rotary vane pump and its impact on pump performance under different inlet pressure and oil temperature conditions were analyzed. The results showed that the cavitation gas was mainly distributed in the volume chamber on the oil suction side, as well as on the suction surface of the rotary vane and near the inner wall of the rotor. With the decrease of inlet pressure and the increase of oil temperature, the cavitation phenomenon inside the rotary vane pump intensified, and the cavitation gas increased, which in turn led to a decrease in the average oil discharge flow rate at the pump outlet and a decrease in volumetric efficiency. When the inlet pressure dropped to 40 kPa and the temperature rose to 373.15 K, the average oil discharge flow rate and volumetric efficiency at the pump outlet both significantly decreased. The pressure pulsation at the monitoring point exhibited low-frequency and high-amplitude pulsation characteristics. The cavitation of the rotary vane pump affected not only its oil discharge and volumetric efficiency, but also the stable and reliable operation of the pump. © 2025 Beijing University of Aeronautics and Astronautics (BUAA). All rights reserved.

关键词： Vane pumps

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Construction of a Transient Multi-Physics Model of Solid Oxide Fuel Cell Fed by Biomass Syngas Considering the Carbon Deposition and Temperature Effect

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SSRN 2022年

作者： Zhu, Pengfei Yao, Jing Wu, Zhen Huang, Si-Min Abu Mansor, Mohd Radzi Yang, Fusheng Zhang, Zaoxiao School of Chemical Engineering and Technology Xi’an Jiaotong University Xi’an710049 China Guangdong Provincial Key Laboratory of Distributed Energy Systems Guangdong Provincial Engineering Research Center of Distributed Energy Systems Dongguan University of Technology Dongguan523808 China Department of Mechanical and Manufacturing Engineering University Kebangsaan Malaysia Selangor43600 Malaysia State Key Laboratory of Multiphase Flow for Power Engineering Xi’an Jiaotong University Xi’an710049 China

Carbon deposition is a thorny issue for the SOFC fueled by low carbon hydrocarbons such as biomass syngas. Moreover, long-term large temperature gradients would reduce SOFC durability. Regarding these two issues, a two dimensional transient multi-physical model considering carbon deposition and temperature effect is developed for SOFC in this work. Typically due to the carbon deposition, the SOFC anode porosity decreases from 0.5 to 0.26, and the reaction activity decreases from 1.0 to about 0.45 after running 140 day. Accordingly, the current density decreases by 1.6 % at t =42 d and 6% at t =140 d, which indicates the damage of SOFC durability compared to the durability target (1%/1000h) of commercial SOFC. The maximum temperature difference of the cell is predicted to be about 106 o C. It was found that the carbon deposition and large temperature gradient are closely related to the operating parameters. With the increase of operating voltage from 0.4 V to 0.8 V, the porosity and reaction activity respectively increase by 50% and 55%, and the maximum temperature difference is reduced from 150 o C to 16 o C after running 140 day. The increase of the inlet temperature could improve the overall temperature and decrease the porosity. Besides, the reduction in the ratio of CH 4 to H 2 O helps to suppress carbon deposition, thus to improving the performance. © 2022, The Authors. All rights reserved.

关键词： Solid oxide fuel cells (SOFC)

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Facile Synthesis of Bulk Au-Co-Coox-Ceox@Iron Ball and its Photocatalytic Application in 4-Nitrophenol Degradation

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SSRN 2023年

作者： Sun, Li Qiao, Zhili Zhi, Yuan Zhang, Hua Dou, Binlin Shan, Yuejin Huang, Weijia School of Energy and Power Engineering University of Shanghai for Science and Technology Jun Gong Road 516 Shanghai200093 China R&D Department Shanghai Minrula Biotechnology Co.Ltd Building 15 Haji Sixth Road 218 Shanghai201306 China Department of Material and Environmental Chemistry Research Division of Functional Materials Design Utsunomiya University Yoto 7-1-2 Utsunomiya321-8585 Japan Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering China

Bulk noble metal-semiconductor composites can be chosen as photocatalysts to carry out the continuous-flow (C-F) degradation of 4-nitrophenol (4-NP) whereas their preparation is complex and uncontrollable. Here, bulk Au/Co-CC@iron ball is designed and prepared by a facile and controllable route without any toxic chemical. The bulk Au/Co-CC@iron ball shows excellent photocatalytic activity and reusability for the 4-NP degradation, which can be ascribed to the synergistic action of active components and foliated iron ball surface. Furthermore, the highly active Au/Co-CC@iron ball is used as packing material to construct a new-type of packed reactor, by which the C-F degradation of 4-NP is successfully achieved. As-fabricated packed reactor and its tandem module exhibit superior photocatalytic performance for the C-F degradation of 4-NP. Noteworthy, based on the tandem module with six reactors, the removal rate of 4-NP can reach up to 2750 µmol/h. Meanwhile, the reactor and its module display satisfactory operational stability and reusability in the C-F degradation of 4-NP. Clearly, the provided route is effective for the preparation of bulk noble metal-semiconductor composites with exceptional performance, which can also be a prospective strategy to obtain bulk packing materials to serve for the C-F degradation. © 2023, The Authors. All rights reserved.

关键词： Precious metals

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