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Confined gas transport in low-dimensional materials

International Journal of Smart and Nano Materials 2024年第1期15卷 127-164页

作者： Hongwei Duan Zeyu Zhuang Jing Yang Shengping Zhang Luda Wang National Key Laboratory of Advanced Micro and Nano Manufacture Technology School of Integrated CircuitsPeking UniversityBeijingChina Academy for Advanced Interdisciplinary Studies and Center for Nanochemistry Beijing Science and Engineering Center for NanocarbonsPeking UniversityBeijingChina Beijing Advanced Innovation Center for Integrated Circuits BeijingChina Technology Innovation Center of Graphene Metrology and Standardization for State Market Regulation Beijing Graphene instituteBeijingChina

Gas transport under confinement exhibits a plethora of physical and chemical phenomena that differ from those observed in bulk media,owing to the deviations of continuum description at the molecular *** biological systems,gas channels play indispen-sable roles in various physiological functions by regulating gas transport across cell ***,investigating gas trans-port under such confinement is crucial for comprehending cellular physiological ***,leveraging these underlying mechanisms can enable the construction of bioinspired artificial nanofluidic devices with tailored gas transport properties akin to those found in biological *** review provides a comprehensive summary of confined gas transport mechanisms,focusing on the unique effects arising from ***,we categorize nanoconfinement spaces based on dimensionality to elucidate their control over gas transport ***,we highlight the potential of bioinspired smart gas membranes that mimic precise modulation of transportation observed in *** conclude,we present a concise outlook on the challenges and opportunities in this rapidly expanding field.

关键词： Nanofluidics gas transport transport mechanism low-dimensional materials smart membranes

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A pyrazine based metal-organic framework for selective removal of copper from strongly acidic solutions

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Frontiers of Environmental science & Engineering 2023年第3期17卷 75-86页

作者： Jiachuang Shao Penghui Shao Mingming Peng Min Li Ziwei Yao Xiuqin Xiong Caiting Qiu Yufan Zheng Liming Yang Xubiao Luo Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle National-Local Joint Engineering Research Center of Heavy Metals Pollutants Control and Resource utilizationNanchang Hangkong UniversityNanchang 330063China Department of Chemical Engineering Chongqing University of Science and TechnologyChongqing 401331China

The selective capture of copper from strongly acidic solutions is of vital importance from the perspective of sustainable development and environmental *** organic frameworks(MOFs)have attracted the interest of many scholars for adsorption due to their fascinating physicochemical characteristics,including adjustable structure,strong stability and ***,pz-UiO-66 containing a pyrazine structure is successfully synthesized for the efficient separation of copper from strongly acidic *** copper removal at low pH values is accomplished by using this material that is not available in previously reported metal–organic ***,the material exhibits excellent adsorption capacity,with a theoretical maximum copper uptake of 247 mg/*** proven by XPS and FT-IR analysis,the coordination of pyrazine nitrogen atoms with copper ions is the dominant adsorption mechanism of copper by *** work provides an opportunity for efficient and selective copper removal under strongly acidic conditions,and promises extensive application prospects for the removal of copper in the treatment for acid metallurgical wastewater.

关键词： Pyrazine Metal-organic frameworks Copper removal Strong acidity High selectivity

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Advances on jarosite residue detoxification and reutilization: a review

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Environmental science and Pollution Research 2025年第7期32卷 3571-3592页

作者： Chen, Mengjun Wang, Rong Fan, Wei Wang, Jiqin Zeng, Xiangfei Han, Yunhui Liang, Qian Huang, Rong Zhou, Songshan Shu, Jiancheng Ministry of Education Southwest University of Science and Technology 59 Qinglong Road Mianyang621010 China School of National Defense & Nuclear Science and Technology Southwest University of Science and Technology 59 Qinglong Road Mianyang621010 China Inner Mongolia JiuKeKangRui Environmental Protection Technology Co Ltd Inner Mongolia Ordos017000 China School of Environment Key Laboratory of Yellow River and Huai River Water Environment and Pollution Control Ministry of Education Henan Normal University Xinxiang453007 China

Jarosite residues are typical hazardous waste byproducts generated during the iron removal process in hydrometallurgical solutions. The jarosite process is widely used for iron removal in zinc hydrometallurgy;jarosite disposal has become a significant barrier to sustainable development in the industry. During this process, jarosite residues entrain and co-precipitate with heavy metals, which are hazardous but valuable. To better understand jarosite residue pollution control and circular recycling, we reviewed related research conducted over the past two decades, analyzed their characteristics, discussed state-of-the-art technologies for jarosite residue detoxification and reutilization, and proposed feasible suggestions for jarosite circular reutilization. We hope that this review helps solve the problem of jarosite residues and promote the sustainable development of the zinc hydrometallurgical industry. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2025.

关键词： Heavy metals

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Halogenated Thienoacene Derivatives with Improved Emission Properties

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Chemical Research in Chinese Universities 2024年第4期40卷 699-703页

作者： ZHANG Jingmei MENG Zhihao ZHEN Yonggang HE Ping YU Panpan HU Wenping Advanced Innovation Center for Soft Matter Science and Engineering State Key Laboratory of Organic-Inorganic CompositesBeijing University of Chemical TechnologyBeijing100029P.R.China Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan430074P.R.China State Key Laboratory of Fine Chemicals Dalian University of TechnologyDalian116024P.R.China Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province China West Normal UniversityNanchong637000P.R.China Key Laboratory of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education Jiangxi Normal UniversityNanchang330022P.R.China MOE Key Laboratory of Organic Integrated Circuits&Tianjin Key Laboratory of Molecular Optoelectronic Sciences Department of ChemistrySchool of SciencesTianjin UniversityTianjin300072P.R.China

Thienoacenes is one of most important groups of semiconducting materials due to the high stability and superior ***,there are scarce studies on the emission properties of thienoacenes to ***,we synthesized fluorinated and chlorinated dibenzo[d,d’]thieno[3,2-b;4,5-b’]dithiophenes(DBTDTs)derivatives F6-DBTDT and Cl6-DBTDT by sulfoxide cyclization,significantly lowering the energy levels relative to the parent compound *** to single crystal structure analysis,F6-DBTDT molecules adopt one-dimensional slipped stacking with closeπ-πinteractions of 3.43Å(1Å=0.1 nm),which is different from the parent compound DBTDT with herringbone stacking ***,the halogenated DBTDT derivatives exhibit enhanced emission properties both in solution and in the solid state,opening up possiblities to improve photoluminescence of thienoacences by halogenation.

关键词： Thienoacene Halogenation Photoluminescence Aggregation structure

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Genome-resolved metagenomic analysis reveals different functional potentials of multiple Candidatus Brocadia species in a full-scale swine wastewater treatment system

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Frontiers of Environmental science & Engineering 2023年第1期17卷 13-25页

作者： Yabing Meng Depeng Wang Zhong Yu Qingyun Yan Zhili He Fangang Meng School of Environmental Science and Engineering Sun Yat-sen UniversityGuangzhou 510275China Guangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology Sun Yat-sen UniversityGuangzhou 510275China National Engineering Laboratory for Pollution Control and Waste Utilization in Livestock and Poultry Production Changsha 410125China Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai) Zhuhai 519082China

The increasing application of anammox processes suggests their enormous potential for nitrogen removal in wastewater treatment ***,the functional potentials and ecological differentiation of cooccurring anammox species in complex ecosystems have not been well ***,by utilizing functional reconstruction and comparative genome analysis,we deciphered the cooccurring mechanisms of four Candidatus Brocadia species that were spontaneously enriched in a full-scale swine wastewater treatment *** analysis indicated that species SW172 and SW745 were closely related to *** caroliniensis and *** sapporoensis,respectively,whereas the dominant species SW510 and SW773,with a total average abundance of 34.1%,were classified as novel species of the genus *** reconstruction revealed that the novel species SW510 can encode both cytochrome cd1-type nitrite reductase and hydroxylamine oxidase for nitrite *** contrast,the detected respiratory pentaheme cytochrome c nitrite reductase and acetate kinase genes suggested that SW773 likely reduced nitrite to ammonium with acetate as a carbon ***,the presence of genes encoding urease and cyanase indicated that both novel species can use diverse organic nitrogen compounds in addition to ammonia and nitrite as *** together,the recovery and comparative analysis of these anammox genomes expand our understanding of the functional differentiation and cooccurrence of the genus *** in wastewater treatment systems.

关键词： Anammox Candidatus Brocadia Functional potential Cooccurring mechanisms Swine wastewater treatment facilities

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Method for Evaluating the Performance of Aircraft Collaborative Decision-Making Based on Dynamic Bayesian Network

Method for Evaluating the Performance of Aircraft Collaborat...

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2024 International Conference on Electronics and Devices, Computational science, ICEDCS 2024

作者： Zhang, Wenbo Yu, Boxiao Tong, Jiahui Li, Jing Beijing Electro-Mechanical Engineering Institute National Key Laboratory of Complex System Control and Intelligent Agent Cooperation Beijing China Beijing Institute of Technology School of Computer Science and Technology Beijing China

ISBN: (纸本)9798331527624

This research addresses the challenge of assessing equipment decision-making effectiveness in environments characterized by uncertainty and multiple influencing factors. We propose a novel approach involving the creation and optimization of a dynamic Bayesian network-based model tailored for equipment decision-making processes. The model facilitates a systematic evaluation of decision-making effectiveness by incorporating various factors, including equipment performance, environmental conditions, and enemy defensive capabilities. A comprehensive assessment system has been developed to simulate the penetration capabilities of different equipment through enemy defenses. Moreover, this study identifies potential errors in the effectiveness evaluation model by analyzing its performance in typical scenarios, pinpointing areas for enhancement. © 2024 IEEE.

关键词： Decision-making Dynamic Bayesian networks Equipment Simulation Uncertainty Management

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A nonlinear wake model of a wind turbine considering the yaw wake steering

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Journal of Oceanology and Limnology 2024年第3期42卷 715-727页

作者： Yunzhou LI Zhiteng GAO Shoutu LI Suiping QI Xiaoyu TANG College of Meteorology and Oceanography National University of Defense TechnologyChangsha 410073China Multi-function Towing Tank School of Naval ArchitectureOcean and Civil EngineeringShanghai Jiao Tong UniversityShanghai 200240China School of Energy and Power Engineering Lanzhou University of TechnologyLanzhou 730050China Institute of Oceanographic Instrumentation Qilu University of Technology(Shandong Academy of Sciences)Qingdao 266061China State Key Laboratory of Industrial Control Technology College of Control Science and EngineeringZhejiang UniversityHangzhou 310027China Laoshan Laboratory Qingdao 266237China

Duo to fluctuations in atmospheric turbulence and yaw control strategies,wind turbines are often in a yaw *** predict the far wake velocity field of wind turbines quickly and accurately,a wake velocity model was derived based on the method of momentum conservation considering the wake steering of the wind turbine under yaw *** consider the shear effect of the vertical incoming wind direction,a two-dimensional Gaussian distribution function was introduced to model the velocity loss at different axial positions in the far wake region based on the assumption of nonlinear wake *** work also developed a“prediction-correction”method to solve the wake velocity field,and the accuracy of the model results was verified in wake experiments on the Garrad Hassan wind ***,a 33-kW two-blade horizontal axis wind turbine was simulated using this method,and the results were compared with the classical wake model under the same parameters and the computational fluid dynamics(CFD)simulation *** results show that the nonlinear wake model well reflected the influence of incoming flow shear and yaw wake steering in the wake velocity ***,computation of the wake flow for the Horns Rev offshore wind farm with 80 wind turbines showed an error within 8%compared to the experimental *** established wake model is less computationally intensive than other methods,has a faster calculation speed,and can be used for engineering calculations of the wake velocity in the far wakefield of wind turbines.

关键词： far wake wake model wake steering wind shear wind farm

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Mechanisms of sesamol and sesamin inhibitingα-glucosidase activity by spectroscopy and molecular docking

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Food Bioscience 2023年第3期53卷 1641-1648页

作者： Shijia Zhang Yiren Zhang Emad Karrar Qingzhe Jin Hui Zhang Gangcheng Wu Xingguo Wang State Key Laboratory of Food Science and Technology School of Food Science and TechnologyNational Engineering Research Center for Functional FoodInternational Joint Research Laboratory for Lipid Nutrition and SafetyCollaborative Innovation Center of Food Safety and Quality Control in Jiangsu ProvinceJiangnan UniversityChina International Joint Laboratory on Food Safety Jiangnan UniversityChina

Sesamol and sesamin inhibitα-glucosidase activity and may therefore be effective in treating type 2 diabetes,but their mechanisms remain ***,the inhibitory effects of sesamol and sesamin onα-glucosidase activity were analyzed by multispectral technique and molecular *** findings indicated that the sesamol and sesamin had a significant influence onα-glucosidase activity,with IC_(50) values of 0.96 mM and 0.33 mM,respectively,and their inhibition types were *** sesamol and sesamin quenched the fluorescence by a static quenching *** results of three-dimensional(3D)fluorescence,circular dichroism(CD)spectroscopy and Fourier transform infrared spectrometer(FT-IR)showed that both sesamol and sesamin had certain effects on the conformation ofα-*** docking results revealed that both sesamol and sesamin could spontaneously bind toα-glucosidase and form hydrogen bonds with some of the amino acid residues of the *** a result,this study sheds new light on sesamol/sesamin as a potentialα-glucosidase inhibitor.

关键词： sesamol Sesamin α-glucosidase Inhibition mechanism Spectroscopy Molecular docking

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Molecular mechanisms of aflatoxin neurotoxicity and potential neuroprotective agents

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Food science and Human Wellness 2024年第5期13卷 2445-2455页

作者： Chongshan Dai Erjie Tian Hui Li Subhajit Das Gupta Zhihui Hao Zhanhui Wang Tony Velkov Jianzhong Shen National Key Laboratory of Veterinary Public Health and Safety Beijing Key Laboratory of Detection Technology for Animal-Derived Food SafetyCollege of Veterinary MedicineChina Agricultural UniversityBeijing 100193China Guangdong Laboratory for Lingnan Modern Agriculture Guangzhou 510642China College of Animal Science and Technology Henan University of Science and TechnologyLuoyang 471023China Beijing Key Laboratory of Diagnostic and Traceability Technologies for Food Poisoning Beijing Center for Disease Prevention and ControlBeijing 100013China Department of Internal Medicine University of Texas Southwestern Medical CenterDallas 75230USA Monash Biomedicine Discovery Institute Department of PharmacologyMonash UniversityVictoria 3800Australia

Aflatoxins(AFTs)represent one of the most notorious classes of deadly mycotoxins produced by certain fungi that are found on agricultural *** are highly toxic to mammals and are known to cause a series of detrimental effects,including neuro-,hepato-,nephron-,and *** this original review we summarize the mechanisms of aflatoxin-induced neurotoxicity and the clinical potential of novel neuroprotective *** B1(AFB1)is the most toxic congener among the 21 identified *** studies have shown that food borne exposure to AFB1 and/or its metabolites often leads to fatal neurotoxicity in animals and *** studies indicated that AFB1 exposure could induce abnormal behavioral changes,including anxiety,lethargy disorders,depression-like behavior,cognitive,learning and memory defects,and decreased feeding ***,AFB1 exposure has been associated with lipid peroxidation,ablation of non-enzymatic and enzymatic antioxidant defense systems and decreased neurotransmitter ***1 exposure has also been shown to induce DNA damage,apoptosis,pyroptosis,and mitochondrial dysfunction in the brain *** signaling pathways,including gasdermin D,toll like receptor 2(TLR2),TLR4,Akt,NF-κB,ERK/MAPK,protein kinase C(PKC),and mitochondrial apoptotic pathways have been shown to participate in AFB1-induced neuronal or astrocyte cell *** these pathways by small molecules(e.g.,quercetin,curcumin,and gallic acid,and dimethyl fumarate),Chinese herbal extracts(e.g.,Artichoke leaf extract,Chelidonium majus ethanolic extract,pumpkin extract,and Crocus sativus ***),and probiotic supplements could effectively improve AFB1-induced neurobehavioral abnormalities and *** date,the precise molecular mechanisms of AFB1-induced neurotoxicity and potential neuroprotective agents remain *** the present review,the clinical manifestations,molecular mechanisms,and potential neuroprotective agents of AFB1

关键词： Aflatoxin B1(AFB1) Neurotoxicity Molecular mechanisms Chemical preventions

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Enhancing corn stalk-based anaerobic digestion with different types of zero-valent iron added during the acidification stage:Performance and mechanism

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Journal of Environmental sciences 2024年第11期145卷 64-74页

作者： Xiang Liu Yue Liu Min Wang Qianzhen Deng Hao Yang College of Agricultural Science and Engineering Hohai UniversityNanjing 210098China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China National and Local Joint Engineering Research Center of Ecological Treatment Technology for Urban Water Pollution Wenzhou UniversityWenzhou 325035China Anhui Provincial Key Laboratory of Environmental Pollution Control and Resource Reuse Anhui Jianzhu UniversityHefei 230009China

Anaerobic digestion has been defined as a competitive approach to facilitate the recycling of corn ***,few studies have focused on the role of direct interspecies electron transfer(DIET)pathway in the acidification stage under the addition of different particle sizes of zero-valent iron(ZVI).In this study,three types of ZVI,namely iron filings,iron powder and nanoscale iron,were investigated,respectively,to enhance its high-value *** in volatile fatty acids(VFAs)and methane(CH4)production associated with the underlyingmechanisms were emphatically *** indicated that the addition of ZVI could increase the concentration of VFAs,with the most outstanding performance observed with the use of nanoscale ***,the conversion of propionic acid to acetic acid was driven by adding ZVI with no between-group differences in acidizing ***,the substrate was more fully utilized when supplied with iron powder compared with other groups in methanogenic phase,thereby displaying the maximumCH4 yield with a value of 263.1 mL/(g total solids(TS)).However,adding nanoscale iron could signally shorten the digestion time(T80),saving 7 days in comparison to the group of iron powder.

关键词： Zero-valent iron Corn stalk Anaerobic digestion Volatile fatty acids Methane

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