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Detection of Picric Acid by Terpy-Based Metallo- Supramolecular Fluorescent Coordination Polymers in Aqueous Media

Chinese Journal of Chemistry 2017年第4期35卷 447-456页

作者： Zhongyu Ding Hongqing Li Wanqing Gao Yiquan Zhang Chunhua Liu Yuanyuan Zhu School of Chemistry and Chemical Engineering Hefei University of Technology and Anhui Key Laboratory of Advanced Functional Materials and Devices Hefei Anhui 230009 China Jiangsu Provincial Key Laboratory for Numerical Simulation of Large Scale Complex Systems (NSLSCS) School of Physical Science and Technology Nanjing Normal University Nanjing Jiangsu 210023 China

The synthesis of two linear terpy-based metallo-supramolecular fluorescent coordination polymers through 1 ： 1 complexation of Zn^2＋ and Cd^2＋ ions with ditopic terpyridine ligand was reported. The dispersibility of P1 and P2 was significantly improved in organic solvent and water through the introduction of hydrophilic oligo-ethyoxy side chain. Two polymers displayed yellow light emission both in solution and the solid state due to the intra-ligand charge transfer （ILCT） between the d^10 metal ions and the conjugated spacer unit. These coordination polymers were explored as fluorescent chemosensors for detecting picric acid in aqueous media, displaying high sensitivity and good selectivity. In addition, test strips were prepared from these polymers and exhibited the practical potential of detecting the NACs pollutants in the outdoor water for public safety and security.

关键词： coordination polymer fluorescent chemosensors nitroaromatic explosives picric acid aqueous media

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Mining and measurement of vocational skills and their association rules based on big data 17

Mining and measurement of vocational skills and their associ...

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2017 International Conference on Digital technology in Education, ICDTE 2017

作者： Wan, Jian Chen, Bin Bin Si, Huayou School of Computer Science and Technology Hangzhou Dianzi University Zhejiang China Key Laboratory of Complex Systems Modeling and Simulation Ministry of Education China

ISBN: (纸本)9781450352833

In recent years, researches on vocational skills are very extensive, most of them concentrated on vocational skills training, effect of vocational skill competition, vocational education and vocational skill identification and so on. But, there is very little research on the inner relationship among vocational skill based on big data. To address the issue, from LinkedIn we first collect tens of thousands of member profiles with vocational skills as empirical data. And then, we dig out high-frequency vocational skills and apply correlation analysis method to explore correlation characteristics of vocational skills. According to our studying, we figure out that there exist a large number of association rules, some of which have very high degrees of confidence, lift, and support. This research reveals the intrinsic association among different vocational skills. These relationships can reflect the general behavior and cognitive rules of human beings. We hope that our research results can provide a theoretical base for other research areas of vocational skills, such as vocational skill training, vocational skill mining, and identification of vocational skills. © 2017 Association for Computing Machinery.

关键词： Association rules

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Dynamic State Estimation Using Event-Trigger Master-Slave Nonlinear Filter for WAMS Applications

Dynamic State Estimation Using Event-Trigger Master-Slave No...

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Data Driven Control and Learning systems (DDCLS)

作者： Qing Yuan Fengdi Zhang Hengheng Gong Luyu Li Sen Li Xiaozhong Liao Zhen Li Xiangdong Liu School of Automation and Key Laboratory for Intelligent Control & Decision on Complex Systems Beijing Institute of Technology Beijing P. R. China National Key Laboratory of Science and Technology on Aerospace Intelligence Control Beijing P. R. China Beijing Institute of Radio Measurement Beijing P. R. China

ISBN: (纸本)9781538626191

The real-time state estimation becomes greatly important with the wide application of phasor measurement unit (PMU) in distributed generation (DG) for wide-area measurement systems (WAMS). In view of estimation, particle filter (PF) is capable of providing the best performance but at the cost of heavy computation burden. Besides, the growing grid size sustainably boosts the amount of data communication from PMU, causing the congestion. An event-trigger master-slave nonlinear filter (ET-MSNF) is proposed to guarantee the estimation accuracy and get the communication bandwidth relieved. The local slave filter at the generator node carries out the local estimation and event-trigger strategy using unscented transformation, which is identical to the center slave. The master filter at the center is designed using Monte Carlo method to improve the center's estimation accuracy by the cooperation with the center slave. Such master-slave filtering structure can fully utilize the computation capability both at the center and node. simulation on the standard IEEE 39-bus system verify the performance of ET-MSNF.

关键词： Generators Monte Carlo methods Phasor measurement units Master-slave Wide area measurements State estimation

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Synthesizing and controlling helical indirect exchange interactions at nonequilibrium

arXiv

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arXiv 2018年

作者： Liu, Tingting Ren, Jie Tong, Peiqing Department of Physics Institute of Theoretical Physics Nanjing Normal University Nanjing210023 China Center for Phononics and Thermal Energy Science China-EU Joint Center for Nanophononics Shanghai Key Laboratory of Special Artificial Microstructure Materials and Technology School of Physics Science and Engineering Tongji University Shanghai200092 China Jiangsu Key Laboratory for Numerical Simulation of Large Scale Complex Systems Nanjing Normal University Nanjing210023 China

We study the nonequilibrium effects of spin and/or electric currents on the helical indirect exchange interactions of local spins that embedded in general open electronic systems. Especially, besides the synthesized anisotropic Heisenberg interactions, we find that the synthetic helical indirect exchange interactions possess two parts: antisymmetric (Dzyaloshinskii-Moriya interaction) and symmetric (Kaplan-Shekhtman-Entin-WohlmanAharony interaction), which are all formulated in terms of Keldysh nonequilibrium Green's functions. The presence of either spin-orbit coupling or spin polarized currents alone is able to synthesize and control the antisymmetric Dzyaloshinskii-Moriya exchange interactions, as the same direction as spin splitting. However, the appearance of symmetric Kaplan-Shekhtman-Entin-Wohlman-Aharony interactions requires both, i.e., the spin-orbit coupling and spin polarized currents with different splitting directions. Our results show the detailed scheme of controlling the sign, magnitude, and direction of indirect Dzyaloshinskii-Moriya vectors and Kaplan-Shekhtman-Entin-Wohlman-Aharony interactions at nonequilibrium in open quantum devices. Copyright © 2018, The Authors. All rights reserved.

关键词： Embedded systems

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Boson Sampling with 20 Input Photons and a 60-Mode Interferometer in a 1014-Dimensional Hilbert Space

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Physical Review Letters 2019年第25期123卷 250503-250503页

作者： Hui Wang Jian Qin Xing Ding Ming-Cheng Chen Si Chen Xiang You Yu-Ming He Xiao Jiang L. You Z. Wang C. Schneider Jelmer J. Renema Sven Höfling Chao-Yang Lu Jian-Wei Pan Hefei National Laboratory for Physical Sciences at Microscale and Department of Modern Physics University of Science and Technology of China Hefei 230026 People’s Republic of China Shanghai Branch CAS Center for Excellence and Synergetic Innovation Center in Quantum Information and Quantum Physics University of Science and Technology of China Shanghai 201315 People’s Republic of China State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information Technology (SIMIT) Chinese Academy of Sciences 865 Changning Road Shanghai 200050 China Technische Physik Physikalisches Instität and Wilhelm Conrad Röntgen-Center for Complex Material Systems Universitat Würzburg Am Hubland D-97074 Würzburg Germany Adaptive Quantum Optics Group Mesa+ Institute for Nanotechnology University of Twente P.O. Box 217 7500 AE Enschede Netherlands SUPA School of Physics and Astronomy University of St. Andrews St. Andrews KY16 9SS United Kingdom

Quantum computing experiments are moving into a new realm of increasing size and complexity, with the short-term goal of demonstrating an advantage over classical computers. Boson sampling is a promising platform for such a goal; however, the number of detected single photons is up to five so far, limiting these small-scale implementations to a proof-of-principle stage. Here, we develop solid-state sources of highly efficient, pure, and indistinguishable single photons and 3D integration of ultralow-loss optical circuits. We perform experiments with 20 pure single photons fed into a 60-mode interferometer. In the output, we detect up to 14 photons and sample over Hilbert spaces with a size up to 3.7×1014, over 10 orders of magnitude larger than all previous experiments, which for the first time enters into a genuine sampling regime where it becomes impossible to exhaust all possible output combinations. The results are validated against distinguishable samplers and uniform samplers with a confidence level of 99.9%.

关键词： Boson sampling Quantum computation Quantum optics Quantum simulation

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Opportunities for Fundamental Physics Research with Radioactive Molecules

arXiv

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arXiv 2023年

作者： Arrowsmith-Kron, Gordon Athanasakis-Kaklamanakis, Michail Au, Mia Ballof, Jochen Berger, Robert Borschevsky, Anastasia Breier, Alexander A. Buchinger, Fritz Budker, Dmitry Caldwell, Luke Charles, Christopher Dattani, Nike de Groote, Ruben P. DeMille, David Dickel, Timo Dobaczewski, Jacek Düllmann, Christoph E. Eliav, Ephraim Engel, Jonathan Fan, Mingyu Flambaum, Victor Flanagan, Kieran T. Gaiser, Alyssa N. Garcia Ruiz, Ronald F. Gaul, Konstantin Giesen, Thomas F. Ginges, Jacinda S.M. Gottberg, Alexander Gwinner, Gerald Heinke, Reinhard Hoekstra, Steven Holt, Jason D. Hutzler, Nicholas R. Jayich, Andrew Karthein, Jonas Leach, Kyle G. Madison, Kirk W. Malbrunot-Ettenauer, Stephan Miyagi, Takayuki Moore, Iain D. Moroch, Scott Navratil, Petr Nazarewicz, Witold Neyens, Gerda Norrgard, Eric B. Nusgart, Nicholas Pašteka, Lukáš F. Petrov, Alexander N. Plaß, Wolfgang R. Ready, Roy A. Reiter, Moritz Pascal Reponen, Mikael Rothe, Sebastian Safronova, Marianna S. Scheidenerger, Christoph Shindler, Andrea Singh, Jaideep T. Skripnikov, Leonid V. Titov, Anatoly V. Udrescu, Silviu-Marian Wilkins, Shane G. Yang, Xiaofei Facility for Rare Isotope Beams Michigan State University East LansingMI48824 United States Experimental Physics Department CERN Geneva 23CH-1211 Switzerland KU Leuven Department of Physics and Astronomy Instituut voor Kern- en Stralingsfysica LeuvenB-3001 Belgium CERN Geneva Switzerland Johannes Gutenberg-Universität Mainz Mainz Germany Accelerator Systems Department CERN Geneva 231211 Switzerland Fachbereich Chemie Philipps-Universität Marburg Hans-Meerwein-Straße 4 Marburg35032 Germany Van Swinderen Institute for Particle Physics and Gravity University of Groningen Netherlands Institute of Physics University of Kassel Heinrich-Plett-Str. 40 Kassel34132 Germany McGill University Canada Helmholtz-Institut GSI Helmholtzzentrum fur Schwerionenforschung and Johannes Gutenberg University Mainz55128 Germany Department of Physics University of California at Berkeley BerkeleyCA94720-7300 United States JILA NIST University of Colorado BoulderCO80309 United States Department of Physics University of Colorado BoulderCO80309 United States TRIUMF 4004 Wesbrook Mall VancouverBCV6T 2A3 Canada University of Western Ontario 1151 Richmond St. N. LondonONN6A 5B7 Canada HPQC Labs WaterlooON Canada HPQC College WaterlooON Canada Instituut voor Kern- en Stralingsfysica KU Leuven Leuven Belgium Department of Physics University of Jyväskylä Jyväskylä Finland University of Chicago ChicagoIL United States Argonne National Laboratory LemontIL United States GSI Helmholtzzentrum für Schwerionenforschung GmbH Darmstadt64291 Germany II. Physikalisches Institut Justus-Liebig-Universität Gießen Gießen 35392 Germany School of Physics Engineering and Technology University of York Heslington YorkYO10 5DD United Kingdom Institute of Theoretical Physics Faculty of Physics University of Warsaw ul. Pasteura 5 WarsawPL-02-093 Poland Department of Chemistry - TRIGA Site Johannes Gutenberg University Fritz-Strassmann-Weg 2 Mainz55128 Germany GSI He

Molecules containing short-lived, radioactive nuclei are uniquely positioned to enable a wide range of scientific discoveries in the areas of fundamental symmetries, astrophysics, nuclear structure, and chemistry. Recent advances in the ability to create, cool, and control complex molecules down to the quantum level, along with recent and upcoming advances in radioactive species production at several facilities around the world, create a compelling opportunity to coordinate and combine these efforts to bring precision measurement and control to molecules containing extreme nuclei. In this manuscript, we review the scientific case for studying radioactive molecules, discuss recent atomic, molecular, nuclear, astrophysical, and chemical advances which provide the foundation for their study, describe the facilities where these species are and will be produced, and provide an outlook for the future of this nascent field. Copyright © 2023, The Authors. All rights reserved.

关键词： Molecules

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Synthesizing and controlling helical indirect exchange interactions out of equilibrium

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Physical Review B 2018年第18期98卷 184426-184426页

作者： Tingting Liu Jie Ren Peiqing Tong Department of Physics and Institute of Theoretical Physics Nanjing Normal University Nanjing 210023 P. R. China Center for Phononics and Thermal Energy Science China-EU Joint Center for Nanophononics Shanghai Key Laboratory of Special Artificial Microstructure Materials and Technology School of Physics Science and Engineering Tongji University Shanghai 200092 P. R. China Jiangsu Key Laboratory for Numerical Simulation of Large Scale Complex Systems Nanjing Normal University Nanjing 210023 P. R. China

We study the nonequilibrium effects of spin and/or electric currents on the helical indirect exchange interactions of local spins that embedded in general open electronic systems. Especially, besides the synthesized anisotropic Heisenberg interactions, we find that the synthetic helical indirect exchange interactions possess two parts: antisymmetric (Dzyaloshinskii-Moriya interaction) and symmetric (Kaplan-Shekhtman-Entin-Wohlman-Aharony interaction), which are all formulated in terms of Keldysh nonequilibrium Green's functions. The presence of either spin-orbit coupling or spin polarized currents alone is able to synthesize and control the antisymmetric Dzyaloshinskii-Moriya exchange interactions, as the same direction as spin splitting. However, the appearance of symmetric Kaplan-Shekhtman-Entin-Wohlman-Aharony interactions requires both, i.e., the spin-orbit coupling and spin polarized currents with different splitting directions. Our results show the detailed scheme of controlling the sign, magnitude, and direction of indirect Dzyaloshinskii-Moriya vectors and Kaplan-Shekhtman-Entin-Wohlman-Aharony interactions at nonequilibrium in open quantum devices.

关键词： Dzyaloshinskii-Moriya interaction Exchange interaction Open quantum systems RKKY interaction Rashba coupling

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Rho-pion transition form factors in the kT factorization formulism revisited

arXiv

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arXiv 2018年

作者： Hua, Jun Cheng, Shan Zhang, Ya-Lan Xiao, Zhen-Jun Department of Physics and Institute of Theoretical Physics Nanjing Normal University Nanjing Jiangsu210023 China School of Physics and Microelectronics Science Hunan University Changsha Hunan410082 China Department of Faculty of Mathematics and Physics Huaiyin Institute of Technology Huaian Jiangsu223001 China Jiangsu Key Laboratory for Numerical Simulation of Large Scale Complex Systems Nanjing Normal University Nanjing Jiangsu210023 China

We revisit the evaluations for the spacelike and timelike ρπ transition form factors Fρπ(Q2) and Gρπ(Q2) with the inclusion of the the next-to-leading order (NLO) QCD contributions in the framework of the kT factorization theorem. The infrared divergence is regularized by the transversal momentum carried by external valence quarks, and ultimately absorbed into the meson wave functions. In the region of Q2 6 2 GeV2, where PQCD factorization apporach applicable, the NLO contribution can bring no larger than 35% enhancement to the spacelike form factor Fρπ(Q2). For the timelike form factor derived under the kinematic exchanging symmetry, this contribution is also under control when the momentum transfer squared is large enough. We also prolong our prediction into the small Q2 region by taking the Lattice QCD results into account, and subsequently obtain the coupling gρπγ = Gρπ(0) = 0.596. Copyright © 2018, The Authors. All rights reserved.

关键词： Approximation theory

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Rho-pion transition form factors in the kT-factorization formalism revisited

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Physical Review D 2018年第11期97卷 113002-113002页

作者： Jun Hua Shan Cheng Ya-lan Zhang Zhen-Jun Xiao Department of Physics and Institute of Theoretical Physics Nanjing Normal University Nanjing Jiangsu 210023 People’s Republic of China School of Physics and Microelectronics Science Hunan University Changsha Hunan 410082 People’s Republic of China Department of Faculty of Mathematics and Physics Huaiyin Institute of Technology Huaian Jiangsu 223001 People’s Republic of China Jiangsu Key Laboratory for Numerical Simulation of Large Scale Complex Systems Nanjing Normal University Nanjing Jiangsu 210023 People’s Republic of China

We revisit the evaluations for the spacelike and timelike ρπ transition form factors Fρπ(Q2) and Gρπ(Q2) with the inclusion of the next-to-leading order (NLO) QCD contributions in the framework of the kT-factorization theorem. The infrared divergence is regularized by the transversal momentum carried by external valence quarks, and ultimately absorbed into the meson wave functions. In the region of Q2≤2 GeV2, where the perturbative QCD factorization approach is applicable, the NLO contribution can bring no larger than 35% enhancement to the spacelike form factor Fρπ(Q2). For the timelike form factor derived under the kinematic exchanging symmetry, this contribution is also under control when the momentum transfer squared is large enough. We also prolong our prediction into the small Q2 region by taking the lattice QCD results into account, and subsequently obtain the coupling gρπγ=Gρπ(0)=0.596.

关键词： Form factors

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Using density peaks sentence clustering for update summary generation

Using density peaks sentence clustering for update summary g...

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2016 IEEE Canadian Conference on Electrical and Computer Engineering, CCECE 2016

作者： Wu, Guohua Guo, Yutian Key Laboratory of Complex Systems Modeling and Simulation Ministry of Education School of Computer Science and Technology Hangzhou Dianzi University China

ISBN: (纸本)9781467387217

Update summarization can be a daunting task in automatic text summarization. It aims to distill evolved messages from a collection of new articles, under the assumption that the reader has already browsed the previous articles. In this paper, a number of state-of-the-art approaches were reviewed for extracting update summarization and then a method called DPC-TS was proposed. This approach is derived from the DPC-based multi-documents summarization method, which was developed in 2015. In our study, a model was established by using the topic signature algorithm, to evaluate the novelty of sentences in update documents set. In addition, the scheme of calculating similarities between sentences and sentence selection approach was improved to ensure there are diversity topics in the summary. DPC-TS update documents summarization method is a simple and effective approach, which can be reproduced and deployed in real environment. © 2016 IEEE.

关键词： update summarization DPC topic signature dedicated physical channel signature algorithm Novelty Adjudication peaks

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