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Unveiling the Interfacial Properties of Organic Single-Crystal Hole-Transporting Layers for High-Performance Light-Emitting

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SmartMat 2025年第1期6卷 227-238页

作者： Gao-Da Ye I Su-Heng Li I Ran Ding |Runda Guo?|Hu Zhang|Ze-Qing Liu|Fangxu Yang|Lingjie Sun|Yansong Li|Xiaobo Du|Xi-Bin WangI Lei Wang|Yue-Feng Liu|Hong-Hua Fang|Yu Liu|Bin Xu|Jing Feng Istate Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchunChina I 2wuhan National Laboratory for OptoelectronicsHuazhong University of Science and TechnologyWuhanChina I 3State Key Laboratory of Supermolecular Structures and MaterialsThe Institute of Theoretical ChemistryJilin UniversityChangchunChina I Department of ChemistrySchool of ScienceKey Laboratory of Organic Integrated CircuitsMinistry of Education and TianjinKey Laboratory of Molecular Optoelectronic SciencesTianjin UniversityTianjinChina I'BOE Technology Group Co.Ltd.BeijingChina I°Department of Precision InstrumentState Key Laboratory of Precision Measurement Technology and InstrumentsTsinghua UniversityBeijingChina

Organic single crystals with long-range molecular periodic ordering ensure superior charge-transport properties and low defect density,which have been considered promising candidates for charge-transporting materials in organic light-emitting devices(OLEDs).The functional interfaces of OLEDs play a critical role in charge-transporting and light-emitting behaviors,while the interfacial properties of organic single crystals in OLEDs and their impact on device performance have been rarely ***,two typical organic single crystals,1,4-bis(4-methylstyryl)benzene(BSB-Me)and 2,6-diphenylanthracene(DPA)with different molecular formulas and packing structures,are introduced as the single-crystal hole-transporting layers(HTLs)for a systematic investigation of the interfacial properties between single-crystal HTLs and active emissive ***-Me single-crystal HTLs offer satisfied surface wettability and enhanced interfacial interaction,which dominate the charge-transporting and light-emitting behaviors of the *** improved interfacial properties are responsible for the superior light out-coupling efficiency of BSB-Me single-crystal OLEDs with efficient exciton recombination and minimal Joule heat *** consequence,BSB-Me single-crystal OLEDs exhibit a maximum luminance of 50,170 cd/m?and a peak EQE of 8.78%,which are better than DPA-based ***,BSB-Me single-crystal HTLs with favorable interfacial properties enable large-area OLEDs withuniform EL emission over thewhole light-emitting area of1mm×1mm.

关键词： electroluminescence interfacial properties OLEDs organic single crystals single-crystal HTLs

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Quantitative characterisation of the influence of different environmental factors on coal spontaneous combustion

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Journal of Thermal Analysis and Calorimetry 2024年第18期149卷 10241-10264页

作者： Zhao, Jingyu Wang, Chen Song, Jiajia Lu, Shiping Deng, Jun Zhang, Yanni Shu, Chi-Min School of Safety Science and Engineering Xi’an University of Science and Technology Xi’an710054 China Shaanxi Key Laboratory of Prevention and Control of Coal Fire Shaanxi Xi’an710054 China Department of Safety Health and Environmental Engineering National Yunlin University of Science and Technology Yunlin64002 Taiwan

Coal spontaneous combustion (CSC) events pose hazards to miners, infrastructure, and the environment. To mitigate some of the risk of CSC, this study explored the influence of airflow rate (AFR), oxygen concentration (OxyC), and heating rate (HR) on CSC. A temperature programmed experiment was used to examine a coal sample under different AFRs, OxyCs, and HRs. The characteristic temperature was determined using index gas growth rate analysis, and the characteristic parameters were shown. The apparent activation energy (Ea) of the sample was computed by the Arrhenius equation, and variance analysis was employed to quantitatively characterise the impact of different environmental factors on the characteristic parameters of the coal samples. The experimental results show that the critical temperature of the coal samples ranges between 65 and 75 °C, and the cracking temperature ranges between 115 and 130 °C, dividing the low-temperature oxidation process of coal into three stages: before the critical temperature, between the critical temperature and the cracking temperature, and after the cracking temperature. An AFR of 120 mL min−1 was identified as the optimal level;exceeding or falling below this value inhibits the coal-oxygen reaction. Increasing OxyC and reducing HR improves coal oxidation. Compared to the same samples under AFR and HR conditions, the Ea of coal under oxygen conditions is lower, ranging between 20 and 35 kJ mol−1, while under AFR and HR conditions, the Ea is not less than 30 kJ mol−1, indicating a stronger tendency for spontaneous combustion under oxygen conditions. AFR substantially affects the oxygen consumption rate, CH4, and exothermic intensity at all stages, with a partial η2 of 0.6. Before the critical temperature, OxyC has the greatest impact on CO2;between the critical temperature and the cracking temperature, OxyC has the greatest impact on CO;and after the cracking temperature, OxyC has the greatest impact on CO, CO2, C2H4, and C2H6, wit

关键词： Activation energy

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3D-printed MoS_(2)/Ni electrodes with excellent electro-catalytic performance and long-term stability for dechlorination of florfenicol

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Journal of Environmental sciences 2024年第3期137卷 420-431页

作者： Jianhui Xu Pengxu Wang Shenggui Chen Lei Li Dan Li Yunfei Zhang Qi Wu Jinhong Fan LumingMa School of Environment and Civil Engineering Dongguan University of TechnologyDongguan 523808China School of Art and Design Guangzhou Panyu PolytechnicGuangzhou 511483China National Engineering Research Center for Urban Pollution Control State Key Laboratory of Pollution Control and Resources ReuseCollege of Environmental Science and EngineeringTongji UniversityShanghai 200092China Dongguan Institute of Science and Technology Innovation Dongguan University of TechnologyDongguan 523808China School of Mechanical Engineering Dongguan University of TechnologyDongguan 523808China

Here,we report the production of 3D-printed MoS_(2)/Ni electrodes(3D-MoS_(2)/Ni)with longterm stability and excellent performance by the selective laser melting(SLM)*** a cathode,the obtained 3D-MoS_(2)/Ni could maintain a degradation rate above 94.0%for forfenicol(FLO)when repeatedly used 50 times in *** also found that the removal rate of FLO by 3D-MoS_(2)/Ni was about 12 times higher than that of 3D-printed pure Ni(3D-Ni),attributed to the improved accessibility of H^(*).In addition,the electrochemical characterization results showed that the electrochemically active surface area of the 3D-MoS_(2)/Ni electrode is about 3-fold higher than that of the 3D-Ni electrode while the electrical resistance is 4 times *** on tert-butanol suppression,electron paramagnetic resonance and triple quadrupole mass spectrometer experiments,a“dual path”mechanism and possible degradation pathway for the dechlorination of FLO by 3D-MoS_(2)/Ni were ***,we also investigated the impacts of the cathode potential and the initial pH of the solution on the degradation of ***,this study reveals that the SLM 3D printing technique is a promising approach for the rapid fabrication of high-stability metal electrodes,which could have broad application in the control of water contaminants in the environmental field.

关键词： 3D-print Electroreduction MoS_(2)/Ni Antibiotic Florfenicol

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Research on the combined polishing technology for high precision ZnS optical element fabrication 4

Research on the combined polishing technology for high preci...

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Advanced Optical Manufacturing Technologies and Applications 2024, AOMTA 2024 and 4th International Forum of Young Scientists on Advanced Optical Manufacturing, YSAOM 2024

作者： Zhao, Xinqi Hu, Hao Chen, Fulei Chen, Yun Laboratory of Science and Technology on Integrated Logistics Support National University of Defense Technology Changsha410073 China Hu’nan Key Laboratory of Ultra-precision Machining Technology Changsha410073 China National University of Defense Technology Changsha410073 China

ISBN: (数字)9781510683037

ISBN: (纸本)9781510683020

ZnS crystal is a multispectral infrared optical material with excellent optical and mechanical properties. Due to its large brittle properties, low hardness, and poor machining performance, Single Point Diamond Ultra Precision Turning technology (SPDT) is the effective fabrication method for ZnS at present. However, the machining accuracy of the SPDT method is limited by the principle of "error copying", which cannot meet the application of high precision applications. Moreover, the traditional polishing method cannot achieve the high efficiency of surface shape accuracy and surface quality improvement of aspherical elements. In order to meet the demands of high precision surface shape and high surface quality of ZnS aspherical optical components, a new combined polishing technology which consists of Magnetorheological Finishing (MRF) and Small Tool Polishing (STP) technology is presented and researched in this paper. Firstly, the Magnetorheological Finishing method is used to achieve the deterministic convergence of surface figure error rapidly. The quantified relationship between process parameters and process defects is established through a series of experiments. Through the optimization of MRF polishing fluid and processing parameters, the surface quality is controlled from sharp deterioration while removing the cutting knife lines. Then STP method is used to improve the surface quality while maintaining the surface figure accuracy. This combined polishing technology is conducted through validation experiments on the ZnS experimental sample. The surface figure error is reduced by 3 times after polishing and the surface roughness is below Ra 1nm. This result validates the effectiveness of the combined polishing technology proposed in the paper. © 2024 SPIE.

关键词： Cutting fluids

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Prospects for the transformation and development of carbon storage in abandoned mines of coal enterprises from the perspective ofcarbon neutrality

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International Journal of Coal science & technology 2023年第3期10卷 24-40页

作者： Xin Lyu Tong Zhang Liang Yuan Juejing Fang State Key Laboratory of Mining Response and Disaster Prevention and Control in Deep Coal Mines Anhui University of Science and TechnologyHuainan 232001China Institute of Energy Hefei Comprehensive National Science CenterHefei230031China

Under the carbon neutrality goal,coal enterprises must seek breakthroughs from abandoned mines,develop new resources in the new era,turn problems into countermeasures,and participate in the carbon emissions market,for contributing to the accomplishment of the national strategic goal of carbon *** this end,we investigated the relevant national policies and regulations to clarify the boundaries disclosed by the carbon information of enterprises,understood the development direction of carbon storage in abandoned mines,and clarified the transformation and development of carbon storage in aban-doned *** made a few suggestions:(1)China should learn from its past experience and other countries to develop the energy industry with Chinese characteristics and reform the economic system.(2)Coal enterprises must actively respond to the national carbon information disclosure policy,clarify their own responsibilities and carbon emission boundaries.(3)It is necessary to proactively obtain advanced knowledge and plan carbon storage pathways for abandoned mines.(4)Devel-opment problems of coal enterprises should be deduced using ***'dual carbon'goals should be achieved steadily step-by-step.(5)Three measures,*** the existing resource structure,coordinating the information of abandoned mines,and promoting the cultivation of scientific and technological talents.

关键词： Mining engineering Abandoned mines Carbon neutrality Carbon emission rights Carbon tax

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Multi-particle quantum walks on 3D integrated photonic chip

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Light(science & Applications) 2024年第12期13卷 3129-3138页

作者： Wen-Hao Zhou Xiao-Wei Wang Ruo-Jing Ren Yu-Xuan Fu Yi-Jun Chang Xiao-Yun Xu Hao Tang Xian-Min Jin Center for Integrated Quantum Information Technologies(IQIT) School of Physics and Astronomy and State Key Laboratory of Advanced Optical Communication Systems and NetworksShanghai Jiao Tong UniversityShanghai 200240China Hefei National Laboratory Hefei 230088China School of Artificial Intelligence Science and Technology University of Shanghai for Science and TechnologyShanghaiChina Institute of Photonic Chips University of Shanghai for Science and TechnologyShanghaiChina Chip Hub for Integrated Photonics Xplore(CHIPX) Shanghai Jiao Tong UniversityWuxi 214000China TuringQ Co. Ltd.Shanghai 200240China

Quantum walks provide a speed-up in computational power for various quantum algorithms and serve as inspiration for the construction of complex graph *** pioneering works have been dedicated to expanding the experimental state space and the complexity of ***,these experiments are mostly limited to small experimental scale,which do not reach a many-body level and fail to reflect the multi-particle quantum interference effects among non-adjacent ***,we present a quantum walk with three photons on a two-dimensional triangular lattice,which is mapped to a 19×19×19 high-dimensional state space and constructs a complex graph with 6859 nodes and 45,486 *** utilizing the statistical signatures of the output combinations and incorporating machine learning techniques,we successfully validate the nonclassical properties of the *** implementation provides a paradigm for exponentially expanding the state space and graph complexity of quantum walks,paving the way for surmounting the classical regime in large-scale quantum simulations.

关键词： quantum particle expanding

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Many-to-many GEO on-orbit refueling mission optimization under time-varying fuel demands via modified differential evolution 74

Many-to-many GEO on-orbit refueling mission optimization und...

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74th International Astronautical Congress, IAC 2023

作者： Li, Chuanjiang Han, Peng Zhang, Haibo Guo, Yanning Harbin Institute of Technology China Beijing Institute of Control Engineering National Key Laboratory of Science and Technology on Space Intelligent Control China

As a kind of on-orbit servicing technology, on-orbit refueling (OOR) has essential significance in prolonging the lifetime of satellites and decreasing the generation of space debris, especially for the expensive satellites located in geosynchronous orbit (GEO). Recently, several one-to-one mode-based OOR missions have been successfully conducted in space. To further reduce the economic cost, the mode of using several refuel satellites (RS) to refuel some dozens of client satellites (CS) in one mission has been proposed, that is, the many-to-many OOR mode. To maximize the efficiency of this mode, the mission optimization problem that determines the refueling sequence and time should be further investigated. The mission optimization is usually carried out before the OOR mission starts, and the fuel demand of CS is obtained in advance. However, the OOR mission for multiple GEO CSs usually takes a long time, and some temporarily unrefueled CSs may perform orbit maintenance by consuming the remaining fuel, leading to a time-varying fuel demand change. In this case, performing the initial mission optimization results may lead to efficiency reduction or even mission failure. To address this problem, in this paper, a many-to-many mode-based OOR mission optimization model is established considering the time-varying fuel demands, and a differential evolution (DE) based algorithm is designed to solve the problem. Firstly, a remaining fuel varying law is obtained according to the periodic orbit maintenance strategy of GEO CSs. Based on that, the mission profit model is further established. Then, by additionally considering several constraints like RS fuel capacity, mission duration, and orbital maneuver duration, the mission optimization model is established. Next, by taking the refueling sequence, the instant of refueling begins as the design variable, and a modified DE is designed to solve the problem. Unlike existing DE, a greedy-search-based mechanism generates high-qualit

关键词： differential evolution geosynchronous orbit on-orbit refueling time-varying fuel demands

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Multi-Task Learning-Enabled Automatic Vessel Draft Reading for Intelligent Maritime Surveillance

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IEEE Transactions on Intelligent Transportation Systems 2024年第5期25卷 4552-4564页

作者： Qu, Jingxiang Liu, Ryan Wen Zhao, Chenjie Guo, Yu Xu, Sendren Sheng-Dong Zhu, Fenghua Lv, Yisheng Wuhan University of Technology Hubei Key Laboratory of Inland Shipping Technology School of Navigation Wuhan430063 China State Key Laboratory of Maritime Technology and Safety Wuhan430063 China National Taiwan University of Science and Technology Graduate Institute of Automation and Control and the Advanced Manufacturing Research Center Taipei10617 Taiwan Institute of Automation State Key Laboratory of Multimodal Artificial Intelligence Systems Chinese Academy of Sciences Beijing100190 China

The accurate and efficient vessel draft reading (VDR) is an important component of intelligent maritime surveillance, which could be exploited to assist in judging whether the vessel is normally loaded or overloaded. The computer vision technique with an excellent price-to-performance ratio has become a popular medium to estimate vessel draft depth. However, the traditional estimation methods easily suffer from several limitations, such as sensitivity to low-quality images, high computational cost, etc. In this work, we propose a multi-task learning-enabled computational method (termed MTL-VDR) for generating highly reliable VDR. In particular, our MTL-VDR mainly consists of four components, i.e., draft mark detection, draft scale recognition, vessel/water segmentation, and final draft depth estimation. We first construct a benchmark dataset related to draft mark detection and employ a powerful and efficient convolutional neural network to accurately perform the detection task. The multi-task learning method is then proposed for simultaneous draft scale recognition and vessel/water segmentation. To obtain more robust VDR under complex conditions (e.g., damaged and stained scales, etc.), the accurate draft scales are generated by an automatic correction method, which is presented based on the spatial distribution rules of draft scales. Finally, an adaptive computational method is exploited to yield an accurate and robust draft depth. Extensive experiments have been implemented on the realistic dataset to compare our MTL-VDR with state-of-the-art methods. The results have demonstrated its superior performance in terms of accuracy, robustness, and efficiency. The computational speed exceeds 40 FPS, which satisfies the requirements of real-time maritime surveillance to guarantee vessel traffic safety. © 2000-2011 IEEE.

关键词： Real time systems

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Time-Varying Formation Tracking control of Heterogeneous Multi-Agent Systems With Intermittent Communications and Directed Switching Networks

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IEEE/CAA Journal of Automatica Sinica 2025年第1期12卷 294-296页

作者： Yuhan Wang Zhuping Wang Hao Zhang Huaicheng Yan the Shanghai Research Institute for Intelligent Autonomous Systems Tongji University the National Key Laboratory of Autonomous Intelligent Unmanned Systems the Frontiers Science Center for Intelligent Autonomous System of Ministry of Education the College of Electronic and Information Engineering the Department of Control Science and Engineering Tongji University the Key Laboratory of Advanced Control and Optimization for Chemical Processes of Ministry of Education the School of Information Science and Engineering East China University of Science and Technology

Dear Editor,This letter is concerned with the problem of time-varying formation tracking for heterogeneous multi-agent systems(MASs) under directed switching networks. For this purpose, our first step is to present so... 详细信息

关键词： Switches Topology Observers Formation control Event detection Switched systems Multi-agent systems control theory Autonomous systems Stability

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Getting insights into gas-phase sulfation effect on catalytic performance of praseodymium oxides in NH_(3)-SCR of NO

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Journal of Rare Earths 2023年第6期41卷 952-958,I0005页

作者： Yandi Cai Peng Yang Qinglong Liu Kaili Ma Wenxin Ma Wang Song Qiuhui Qian Fei Gao Wei Tan Lin Dong State Key Laboratory of Pollution Control and Resource Reuse School of EnvironmentJiangsu Key Laboratory of Vehicle Emissions ControlCenter of Modern AnalysisKey Laboratory of Mesoscopic Chemistry of MOESchool of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Analysis and Testing Center Southeast UniversityNanjing 211189China National and Local Joint Engineering Laboratory of Municipal Sewage Resource Utilization Technology School of Environmental Science and EngineeringSuzhou University of Science and TechnologySuzhou 215009China

Sulfation treatment has been widely used to promote the catalytic performance of ceria(CeO_(2))based catalysts for the selective catalytic reduction of NO by NH_(3)(NH_(3)-SCR of NO).Praseodymium oxide(PrO_(x)),another commonly used rare earth material with similar structural properties as CeO_(2),also shows satistactory redox properties due to the facile redox cycle of Pr^(3+)■Pr^(4+).In this work,gas phase sulfation treatment with varied duration was performed on PrO_(x) at 200℃,and the NH_(3)-SCR activity of sulfated PrO_(x) was *** on the results of systematic characterizations(e.g.,N_(2)-physisorption,NH_(3) oxidation,NO oxidation,in situ diffuse Fourier transform infrared spectroscopy),it is revealed that the catalytic performance of sulfated PrO_(x)is highly dependent on the sulfation time(or the amount of sulfate species deposited on PrO_(x)),which has a significant impact on the competitive reaction between NH_(3) oxidation and NH_(3)-SCR of NO,thus determining the NH_(3)-SCR activity of PrO_(x).This work provides new insight into tuning the interaction between PrO_(x) surface and reactants(NO,NH_(3))via sulfation treatment,which cam guide the design and application of PrO_(x)based catalysts for NH_(3)-SCR of NO in the future.

关键词： NH_(3)-SCR Praseodymium oxides Sulfation treatment Surface acidity NH_(3)oxidation Rare earths

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