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Crystalline-magnetism action in biomimetic mineralization of calcium carbonate

Chinese Journal of Chemical engineering 2023年第7期59卷 146-152页

作者： Chaoqun Wu Xun Liu Fujun Yao Xin Yang Yan Wang Wenyuan Hu State Key Laboratory of Environment-friendly Energy Materials Southwest University of Science and TechnologyMianyang 621000China Materials Science and Engineering Southwest University of Science and TechnologyMianyang 621000China National Health Commission Key Laboratory of Nuclear Technology Medical Transformation Mianyang Central HospitalMianyang 621010China

The influence of minor environmental factors,such as the geomagnetic field,on the biomineralization of nacres,is often ignored but a great deal of research has confirmed its important role in the normal mineralization of calcium *** the geomagnetic field is weak,its cumulative effects need to be considered given that the biomineralization process can take ***,the authors of this paper have investigated the effects of weak magnetic fields(25 Gs or 50 Gs)on calcium carbonate mineralization and analyzed the mechanism *** results show that even a weak magnetic field conduces to the formation of vaterite or aragonite,in the induction order of precursor→vaterite→*** stronger the magnetic field and the longer the time,the more obvious the induction *** effect of a magnetic field is strongest in the aging stage and weakest in the solution *** by egg-white protein and by a magnetic field inhibit each other,but they both restrict particle *** findings highlight the importance of minor environmental factors for biomineralization and can serve as a reference for biomimetic preparation of a CaCO_(3)nacre-like structure and for anti-scale technology for circulating cooling water.

关键词： Biomimetic mineralization Calcium carbonate Magnetic field Egg-white protein

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Insights into the mechanism of the deterioration of mainstream partial nitritation/anammox under low residual ammonium

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Journal of environmental sciences 2023年第4期126卷 29-39页

作者： Yandong Yang Yiming Jiang Yanan Long Jiarui Xu Changqing Liu Liang Zhang Yongzhen Peng School of Environmental and Municipal Engineering Qingdao University of TechnologyQingdao 266033China National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery EngineeringBeijing University of TechnologyBeijing 100124China

Residual ammonium is a critical parameter affecting the stability of mainstream partial nitritation/anammox(PN/A), but the underlying mechanism remains unclear. In this study,mainstream PN/A was established and operated with progressively decreasing residual ammonium. PN/A deteriorated as the residual ammonium decreased to below 5 mg/L, and this was paralleled by a significant loss in anammox activity in situ and an increasing nitrite oxidation rate. Further analysis revealed that the low-ammonium condition directly decreased anammox activity in situ via two distinct mechanisms. First, anammox bacteria were located in the inner layer of the granular sludge, and thus were disadvantageous when competing for ammonium with ammonium-oxidizing bacteria(AOB) in the outer layer. Second, the complete ammonia oxidizer(comammox) was enriched at low residual ammonium concentrations because of its high ammonium affinity. Both AOB and comammox presented kinetic advantages over anammox bacteria. At high residual ammonium concentrations,nitrite-oxidizing bacteria(NOB) were effectively suppressed, even when their maximum activity was high due to competition for nitrite with anammox bacteria. At low residual ammonium concentrations, the decrease in anammox activity in situ led to an increase in nitrite availability for nitrite oxidation, facilitating the activation of NOB despite the dissolved oxygen limitation(0.15–0.35 mg/L) for NOB persisting throughout the operation. Therefore, the deterioration of mainstream PN/A at low residual ammonium was primarily triggered by a decline in anammox activity in situ. This study provides novel insights into the optimized design of mainstream PN/As in engineering applications.

关键词： Mainstream partial nitritation/anammox Residual ammonium Granular sludge Comammox

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Interlinked water and sediment microplastics in the Laizhou Bay of China

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Journal of Oceanology and Limnology 2025年第2期43卷 446-458页

作者： Hong CHEN Fenghua JIANG Jingxi LI Wei CAO Di ZHANG Futao ZHANG Shiliang WANG Chengjun SUN College of Safety and Environmental Engineering Shandong University of Science and TechnologyQingdao 266590China Key Laboratory of Analytical Technology Development and Offshore Eco-Environment Conservation First Institute of OceanographyMinistry of Natural ResourcesQingdao 266061China Qingdao National Laboratory of Marine Science and Technology Laboratory of Marine Drugs and Biological ProductsQingdao 266071China

To explore the relationship of microplastic pollution in different media in marine environment,microplastics in the surface seawater and sediments of Laizhou Bay,Bohai Sea,North China,were *** samples were collected using a pre-concentrator equipped with a 20-μm mesh size sieve,and sediment samples were collected by a box *** shape,color,size,and type of microplastics were obtained by a stereomicroscope and a Fourier transform infrared spectrometer(ATR-μ-FT-IR).Results show that the abundance of microplastics in the surface seawater of Laizhou Bay was 858.3±573.2 items/m~3,and that of microplastics in sediments was 151.0±77.4 items/kg dry weight(d.w.)The microplastics in seawater and sediments were mainly ***,the microplastics in seawater were mainly transparent,and those in sediments were transparent and *** highest proportion of microplastics in seawater was rayon(77.48%),followed by polyethylene terephthalate(PET,13.17%).The highest proportion of microplastics in sediments was rayon(73.66%),followed by PET(8.90%).The size of microplastics in 1000-2000μm accounted for the largest proportion of 28.54%in seawater,while that in 500-1000μm took 27.93%in *** in seawater and sediment showed medium-level *** seawater,microplastic abundance was higher in offshore and nearshore areas of *** sediment,microplastic abundance was higher in offshore and nearshore areas of *** results of the principal component analysis(PCA)indicated that microplastics in sediment exhibited greater stability compared to those in *** microplastics in seawater and sediment show a positive correlation in terms of shape and plastic type,while exhibiting a negative correlation in terms of ***,microplastics in sediments were smaller in size,and those in seawater and sediments had consistent size distribution characteristics in space.

关键词： microplastic Laizhou Bay sediment seawater correlation

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High density sampling reveals the spatiotemporal characteristics of microbial communities in a full-scale municipal wastewater treatment plant

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Frontiers of environmental science & engineering 2025年第2期19卷 135-149页

作者： Zhaoyang Li Liang Zhang Jinghan Li Da Kang Jialin Li Shujun Zhang Xiaoyu Han Bin Ma Yongzhen Peng National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery EngineeringBeijing University of TechnologyBeijing 100124China Beijing Drainage Group Co. Ltd.(BDG)Beijing 100022China College of Environment and Ecology Institute of Tropical Agriculture and ForestryHainan UniversityHaikou 570228China

Insights into the microbial communities in municipal wastewater treatment plants(WWTPs)are critical for the optimization of biological nutrient removal ***,our understanding about the spatiotemporal characteristics of the microbial communities in WWTPs remains *** the present study,264 samples were collected biweekly from four spatially independent corridors in a typical municipal *** annual compositional and metagenomic characteristics were investigated based on multiple ecological indicators using statistical *** results revealed that the microbial community compositions from the four corridors showed significantly high similarities,as revealed by the statistical analysis at the operational taxonomic unit(OTU)*** with the OTU level results,the functionality of the microbial communities in the four independent corridors also showed significant *** comparison,the dynamics of the microbial community over the year showed two successional peaks of the microbial communities with the spatial similarity,and this resulted in three alternative stable states of the microbial communities in a calendar *** microbial communities only drifted in July and November,suggesting an uneven community succession pattern driven by seasonal variation in environmental *** functional characteristics were found to be relatively conservative compared to the microbial community succession,which revealed the decoupling between the composition and functionality of the microbial community in the municipal *** present study provides an in-depth overview of the microbial communities in a municipal WWTP and will be useful for the establishment of the connection between ecological characteristics and the operational stability of WWTPs.

关键词： Activated sludge Microbial community Spatial similarity Successional pattern Metagenomics

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Towards optimized tensor code generation for deep learning on sunway many-core processor

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Frontiers of Computer science 2024年第2期18卷 1-15页

作者： Mingzhen LI Changxi LIU Jianjin LIAO Xuegui ZHENG Hailong YANG Rujun SUN Jun XU Lin GAN Guangwen YANG Zhongzhi LUAN Depei QIAN State Key Laboratory of Software Development Environment Beijing 100191China School of Computer Science and Engineering Beihang UniversityBeijing 100191China National University of Singapore Singapore 119077Singapore State Key Laboratory of Mathematical Engineering and Advanced Computing Wuxi 214000China Science and Technology on Special System Simulation Laboratory Beijing Simulation Center Beijing 100854China Department of Computer Science and Technology Tsinghua UniversityBeijing 100084China

The flourish of deep learning frameworks and hardware platforms has been demanding an efficient compiler that can shield the diversity in both software and hardware in order to provide application *** the existing deep learning compilers,TVM is well known for its efficiency in code generation and optimization across diverse hardware *** the meanwhile,the Sunway many-core processor renders itself as a competitive candidate for its attractive computational power in both scientific computing and deep learning *** paper combines the trends in these two ***,we propose swTVM that extends the original TVM to support ahead-of-time compilation for architecture requiring cross-compilation such as *** addition,we leverage the architecture features during the compilation such as core group for massive parallelism,DMA for high bandwidth memory transfer and local device memory for data locality,in order to generate efficient codes for deep learning workloads on *** experiment results show that the codes generated by swTVM achieve 1.79x improvement of inference latency on average compared to the state-of-the-art deep learning framework on Sunway,across eight representative *** work is the first attempt from the compiler perspective to bridge the gap of deep learning and Sunway processor particularly with productivity and efficiency in *** believe this work will encourage more people to embrace the power of deep learning and Sunwaymany-coreprocessor.

关键词： sunway processor deep learning compiler code generation performance optimization

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Honeycomb-like biochar framework coupled with Fe_(3)O_(4)/FeS nanoparticles as efficient heterogeneous Fenton catalyst for phenol degradation

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Journal of environmental sciences 2024年第2期136卷 390-399页

作者： Aihua Cheng Yi He Xiaohe Liu Chi He Department of Environmental Engineering College of Geology and EnvironmentXi’an University of Science and TechnologyXi’an 710054China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an 710049China National Engineering Laboratory for VOCs Pollution Control Material and Technology University of Chinese Academy of SciencesBeijing 101408China

Achieving an efficient and stable heterogeneous Fenton reaction over a wide pH range is of great significance for wastewater ***,a pollen-derived biochar catalyst with a unique honeycomb-like structure,coupled with the dispersion of magnetic Fe_(3)O_(4)/FeS(Fe/S)nanoparticles,was synthesized by simple impregnation precursor,followed by *** prepared Fe/S-biochar catalyst demonstrated outstanding phenol degradation efficiency across a wide pH range,with 98%of which eliminated even under neutral conditions(pH 7.0).The high catalytic activity was due to the multilevel porous structure of pollenderived biochar provided enough active sites and allowed for better electron transfer,then increases oxidation ability to promote the ***,the acid microenvironment formed by SO_(4)^(2-)group from Fe/S composite extended the pH range for Fenton reaction,and S^(2-)facilitated the conversion of≡Fe^(3+)to≡Fe^(2+),resulting in remarkable degradation ***,biochar can effectively promote cycling stability by limiting Fe *** work may provide a general strategy for designing 3D framework biochar-based Fe/S catalysts with excellent performance for heterogeneous Fenton reactions.

关键词： Biomass Biochar Fenton reaction Fe_(3)O_(4)/FeS(Fe/S) Phenol degradation

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Construction of a Cu@hollow TS-1 nanoreactor based on a hierarchical full-spectrum solar light utilization strategy for photothermal synergistic artificial photosynthesis

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Carbon Energy 2024年第2期6卷 25-36页

作者： Sixian Zhu Qiao Zhao Hongxia Guo Li Liu Xiao Wang Xiwei Qi Xianguang Meng Wenquan Cui Hebei Key Laboratory for Environment Photocatalytic and Electrocatalytic Materials College of Chemical EngineeringNorth China University of Science and TechnologyTangshanChina School of Materials Science and Engineering National Institute for Advanced MaterialsTKL of Metal and Molecule-Based Material ChemistryNankai UniversityTianjinChina Hebei Iron and Steel Laboratory TangshanChina

The artificial photosynthesis technology has been recognized as a promising solution for CO_(2) *** catalysis has been proposed as a novel strategy to promote the efficiency of artificial photosynthesis by coupling both photochemistry and ***,strategies for maximizing the use of solar spectra with different frequencies in photothermal catalysis are urgently ***,a hierarchical full-spectrum solar light utilization strategy is *** on this strategy,a Cu@hollow titanium silicalite-1 zeolite(TS-1)nanoreactor with spatially separated photo/thermal catalytic sites is designed to realize high-efficiency photothermal catalytic artificial *** space-time yield of alcohol products over the optimal catalyst reached 64.4μmol g−1 h−1,with the selectivity of CH3CH2OH of 69.5%.This rationally designed hierarchical utilization strategy for solar light can be summarized as follows:(1)high-energy ultraviolet light is utilized to drive the initial and difficult CO_(2) activation step on the TS-1 shell;(2)visible light can induce the localized surface plasmon resonance effect on plasmonic Cu to generate hot electrons for H2O dissociation and subsequent reaction steps;and(3)low-energy near-infrared light is converted into heat by the simulated greenhouse effect by cavities to accelerate the carrier *** work provides some scientific and experimental bases for research on novel,highly efficient photothermal catalysts for artificial photosynthesis.

关键词： artificial photosynthesis full spectrum nanoreactors photothermal catalysis

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Time-dependent color-tunable room temperature phosphorescence from unusual conformational transitions in phenothiazine polymers under UV irradiation

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science China Chemistry 2025年第3期68卷 1091-1098页

作者： Jiwen Lu Yifan Niu Chanjuan Jin Chengheng Wu Hanyu Wang Yan Guan Ping Wang Xinghe Fan Key Lab of Environment-Friendly Chemistry and Application of Ministry of Education Key Laboratory of Polymeric Materials and Application Technology of Hunan ProvinceKey Laboratory of Advanced Functional Polymer Materials of CollegesUniversities of Hunan ProvinceCollege of ChemistryXiangtan UniversityXiangtan 411105China Beijing National Laboratory for Molecular Sciences Key Laboratory of Polymer Chemistry and Physics of Ministry of EducationCenter for Soft Matter Science and EngineeringCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China

Achieving color-tunable room-temperature phosphorescence(RTP),especially including blue RTP from a single-component polymer still faces a formidable ***,we wisely choose conformation-dependent phenothiazine with trifluoromethyl substituent as the side group of the phosphor monomer(Cz PT)and then copolymerize it with N-isopropylacrylamide(NIPAM)through photopolymerization to obtain polymers PPCz ***-dependent color-tunable phosphorescence from unusual quasi-equatorial(eq)to quasi-axial(ax)conformers are obtained,and the RTP color changes from orange(550 nm)to blue(470 nm)with phosphorescence lifetime up to 0.96 *** theoretical calculations confirm that the quasi-axial conformer is the preferred structure that facilitates the formation of intramolecular hydrogen bonds on the trifluoromethyl *** EPR spectra illustrate that the persistent UV irradiation generates radical cations to induce the conformational transitions first,followed by photopolymerization immobilizing the ax conformation in PPCz *** of data encryption and anti-counterfeiting are fabricated to show prompt and delayed multicolor *** work affords a simple and feasible avenue for two-dimensional color tunable room temperature phosphorescence from a single-component polymer.

关键词： polymeric room temperature phosphorescence color-tunable phosphorescence conformation-dependent time-dependent blue phosphorescence

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An assessment of the CMIP6 performance in simulating Arctic sea ice volume flux via Fram Strait

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Advances in Climate Change Research 2024年第4期15卷 584-595页

作者： Hui-Yan KUANG Shao-Zhe SUN Yu-Fang YE Shao-Yin WANG Hai-Bo BI Zhuo-Qi CHEN Xiao CHENG School of Geospatial Engineering and Science Sun Yat-sen UniversitySouthern Marine Science and Engineering Guangdong Laboratory(Zhuhai)Zhuhai 519082China Key Laboratory of Comprehensive Observation of Polar Environment(Sun Yat-sen University) Ministry of EducationZhuhai 519082China CAS Key Laboratory of Marine Geology and Environment Institute of OceanologyChinese Academy of Sciences(CAS)Qingdao 266071China Laboratory for Marine Geology Qingdao National Laboratory for Marine Science and Technology Qingdao 266237China

Numerical models serve as an essential tool to investigate the causes and effects of Arctic sea ice *** the simulation capabilities of the most recent CMIP6 models in sea ice volume flux provides references for model applications and ***,reliable long-term simulation results of the ice volume fux contribute to a deeper understanding of the sea ice response to global climate *** this study,the sea ice volume flux through six Arctic gateways over the past four decades(1979-2014)were estimated in combination of satellite observations of sea ice concentration(SIC)and sea ice motion(SIM)as well as the Pan-Arctic Ice-Ocean Modeling and Assimilation System(PIOMAS)reanalysis sea ice thickness(SIT)*** simulation capability of 17 CMIP6 historical models for the volume flux through Fram Strait were quantitatively *** ice volume flux simulated from the ensemble mean of 17 CMIP6 models demonstrates better performance than that from the individual model,yet IPSL-CM6A-LR and EC-Earth3-Veg-LR outperform the ensemble mean in the annual volume flux,with Taylor scores of 0.86 and 0.50,***6 models display relatively robust capability in simulating the seasonal variations of volume *** them,CESM2-WACCM performs the best,with a correlation coefficient of 0.96 and a Taylor score of ***,NESM3 demonstrates the largest devi-ation from the observation/reanalysis data,with the lowest Taylor score of *** variability of sea ice volume flux is primarily influenced by SIM and SIT,followed by *** extreme large sea ice export through Fram Strait is linked to the occurrence of anomalously low air temperatures,which in turn promote increased SIC and SIT in the corresponding ***,the intensified activity of Arctic cyclones and Arctic dipole anomaly could boost the southward sea ice velocity through Fram Strait,which further enhance the sea ice outflow.

关键词： Sea ice volume flux CMIP6 models Fram Strait Attribution analysis

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2D phosphides heterostructures on titanium microfiltration membrane for enhanced ampere-level current density overall seawater splitting

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Nano Research 2025年第1期18卷 249-259页

作者： Wenjing Dai Xin Wang Yulong Ma Sisi He Ming Chen Zhaohui Yin Shuheng Tian Maolin Wang Shixiang Yu Hang Zhang Yuanzhe Wang Hong Wang Jianxin Li Faming Gao Bowen Cheng Yun Wang Zhen Yin Ding Ma Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-utilization College of Chemical Engineering and Materials ScienceTianjin University of Science and TechnologyTianjin 300457China State Key Laboratory of Biobased Fiber Manufacturing Technology Tianjin University of Science and TechnologyTianjin 300457China Haian Institute of High-Tech Research Nanjing UniversityHaian 226600China Beijing National Laboratory for Molecular Sciences College of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China State Key Laboratory of Separation Membranes and Membrane Processes Separation Membrane Science and Technology International Joint Research CentreTiangong UniversityTianjin 300387China Centre for Catalysis and Clean Energy School of Environment and ScienceGold Coast CampusGriffith UniversitySouthportQueensland 4222Australia

The advancement of direct seawater electrolysis is a significant step towards sustainable hydrogen production,addressing the critical need for renewable energy sources and efficient resource ***,direct seawater electrolysis has to face several challenges posed by the corrosiveness of highly concentrated chloride and the competitive chlorine evolution reaction(ClER).To overcome these issues,we designed a novel NiP_(2)@CoP electrocatalyst on a porous titanium microfiltration(Ti MF)*** obtained bifunctional NiP_(2)@CoP catalyst outperforms the Pt/C and IrO_(2),as evidenced by its low overpotentials of 192 and 425 mV at a current density of 500 mA·cm^(-2) for hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)in alkaline seawater(1 M KOH+0.5 M NaCl),***,only 231 and 569 mV overpotentials are required at the current density of 1500 mA·cm^(-2) towards HER and OER in alkaline seawater,*** importantly,no ClER was observed,demonstrating its excellent selectivity to *** selection of porous Ti MF membrane as an electrode substrate further enhances the performance by providing a robust structure that promotes the fast generation and release of gas *** promising outcomes obtained with NiP_(2)@CoP catalysts on Ti MF support,therefore,pave the way for the commercial viability of direct seawater electrolysis technologies at industrial-level current densities.

关键词： direct seawater electrolysis porous titanium microfiltration membrane phosphides heterostructures NiP_(2)@CoP electrocatalyst excellent selectivity to oxygen evolution reaction(OER)

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