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Synergizing 3D-printed structure and sodiophilic interface enables highly efficient sodium metal anodes

Chinese Chemical Letters 2024年第11期35卷 528-534页

作者： Changyuan Bao Yunpeng Jiang Haoyin Zhong Huaizheng Ren Junhui Wang Binbin Liu Qi Zhao Fan Jin Yan Meng Chong Jianguo Sun Fei Wang Bo Wang Ximeng Liu Dianlong Wang John Wang School of Chemical and Environmental Engineering Yancheng Teachers UniversityYancheng 224007China MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage State Key Laboratory of Urban Water Resource and EnvironmentSchool of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbin 150001China Department of Materials Science and Engineering National University of SingaporeSingapore 117575Singapore Institute of Materials Research and Engineering Agency for ScienceTechnology and Research(ASTAR)Singapore 138634Singapore

Sodium(Na)metal batteries have gained increasing attention more recently,owing to their high energy densities and cost efficiencies,but are severely handicapped by the unsatisfactory Coulombic efficiency(CE)and cycling stability stemming from dendrite growth on Na *** this study,we developed a strategy of direct ink writing(DIW)3D printing combined with electroless deposition to construct a hierarchical Cu grid coated with a dense nanoscale Ag interfacial layer as the host material for Na *** sodiophilic Ag interface contributes to a fall in the Na nucleation energy,hence enabling uniform Na deposition on each 3D-printed *** constructed 3D-printed structure can effectively moderate the electric-field distribution and lower the local current density for relieving Na inhomogeneous growth,as confirmed by finite element simulation and Na plating/stripping morphology evolution *** particular,the unique 3D structure also promotes the lateral growth of Na,thus the volume change of Na metal was accommodated to stabilize the solid electrolyte interphase(SEI).As a result,the CE of the half-cell can reach 99.9%at the current density of 1 m A/cm^(2)after 300 cycles and the full-cell exhibits outstanding electrochemical performance(capacity retention of 91.0%after 500 cycles at 2 C).

关键词： 3D-printed host Sodiophilic interface Dendrite-free High reversibility Sodium metal batteries

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Metagenomic insights into responses of microbial population and key functional genes to fulvic acid during partial nitritation

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Journal of environmental sciences 2023年第2期124卷 952-962页

作者： Li Zhang Shuang Lan Quanhao Dou Shiwei Hao Yueping Wang Xiaoxuan Wang Ruoyan Zhang Yongzhen Peng Jiachun Yang National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery EngineeringBeijing University of TechnologyBeijing 100124China Shuifa Shandong Water Development Group Co.Ltd. Shandong 274200China

The long-term impact of fulvic acid(FA)on partial nitritation(PN)systemwas initially examined in this *** obtained results revealed that the FA lower than 50 mg/L had negligible effect on the nitrite accumulation rate(NAR nearly 100%)and ammonium removal rate(ARR 56.85%),while FA over 50 mg/L decreased ARR from 56.85%to 0.7%.Sludge characteristics analysis found that appropriate FA(<50 mg/L)exposure promoted the settling performance and granulation of PN sludge by removing Bacteroidetes and accumulating *** analysis of metagenomics suggested that the presence of limited FA(0-50 mg/L)stimulated the generation of NADH,which favors the denitrification and nitrite *** negative impact of FA on the PN system could be divided into two ***,limited FA(50-120 mg/L)was decomposed by Anaerolineae to stimulate the growth and propagation of heterotrophic bacteria(Thauera).Increasing heterotrophs competed with AOB(Nitrosomonas)for dissolved oxygen,causing AOB to be eliminated and ARR to ***,when FA dosage was over 120 mg/L,Anaerolineae were inhibited and heterotrophic bacteria reduced,resulting in the abundance of AOB ***,the ammonium transformation pathway was suppressed because genes amoABC and hao were obviously reduced,leading to the deterioration of reactor ***,these results provide theoretical guidance for the practical application of PN for the treatment of FA-containing sewage.

关键词： Partial nitritation Fulvic acid Microbial community Functional genes Metagenomic

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The suitability assessment on site selection for bottom seeding scallop culture based on analytic hierarchy process

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Journal of Oceanology and Limnology 2024年第2期42卷 647-663页

作者： Ziniu ZHANG Zhenyan WANG Guihua LI Meihan ZHAO Wenjian LI School of Earth Sciences and Engineering Shandong University of Science and TechnologyQingdao 266590China Key Laboratory of Marine Geology and Environment Institute of OceanologyChinese Academy of SciencesQingdao 266071China Laboratory for Marine Mineral Resources National Laboratory for Marine Science and TechnologyQingdao 266237China University of Chinese Academy of Sciences Beijing 100049China

Scallop culture is an important way of bottom-seeding marine ranching,which is of great significance to improve the current situation of fishery ***,there are some problems in site-selection evaluation of marine ranching,such as imperfect criteria system,complex structure,untargeted criteria quantification,*** addition,no site-selection evaluation method of bottom-seeding culture areas for scallops is ***,we established a hierarchy structure model according to the analytic hierarchy process(AHP)theory,in which social,physical,chemical,and biological environments are used as main criteria,and marine functional zonation,water depth,current,water temperature,salinity,substrate type,water quality,sediment quality,red tide,phytoplankton,and zooplankton are used as sub-criteria,on which a multi-parameter evaluation system is set ***,the dualism method,assignment method,and membership function method were used to quantify sub-criteria,and a quantitative evaluation for the entire criteria was added,including the evaluation and analysis of two types of unsuitable environmental *** overall consideration in scallop yield,quality,and marine ranching construction objectives,the weight of the main criteria could be *** grades in the suitability corresponding to the evaluation result were divided,and the Python language was used to create an evaluation system for efficient calculation and intuitive presentation of the evaluation *** marine cases were simulated based on existing survey data,and the results prove that the method is feasible for evaluating and analyzing the site selection of bottom-seeding culture areas for scallops under various environmental *** proposed evaluation method can be promoted for the site selection of bottom-seeding marine *** study provided theoretical and methodological references for the site selection evaluation of other types of marine ranching.

关键词： marine ranching bottom-seeding scallops site selection evaluation analytic hierarchy process evaluation system

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Mechanical pressing method for making high-quality perovskite single crystals

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Journal of Semiconductors 2023年第11期44卷 1-4页

作者： Chenglin Wang Jie Sun Jiangzhao Chen Cong Chen Liming Ding State Key Laboratory of Reliability and Intelligence of Electrical Equipment School of Materials Science and EngineeringHebei University of TechnologyTianjin 300401China Faculty of Materials Science and Engineering Kunming University of Science and TechnologyKunming 650093China Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190China Macao Institute of Materials Science and Engineering(MIMSE) Macao University of Science and TechnologyMacao 999078China

Halide perovskites show excellent photovoltaic properties[1−4].However,the preparation of high-quality perovskite crystals remains a great challenge,which limits their *** materials applied to photodetectors mainly include polycrystalline thin films and single *** solution methods are used to prepare polycrystalline thin films,and the films are full of defects such as voids and grain boundaries[5−7].Compared to polycrystalline thin films,perovskite single crystals possess high crystallinity and low defect density[8−10].Photodetectors based on perovskite single crystals exhibit excellent performance[11].However,the size limitation of single crystals hinders their application in photodetectors[12].

关键词： perovskite polycrystalline hinder

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Polysulfide modified PtCu intermetallic nanocatalyst with enrichment realizes efficient electrooxidation ethanol to CO_(2)

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Nano Research 2024年第4期17卷 2320-2327页

作者： Shuanglong Zhou Zheng Lv Liang Zhao Dan Zhang Zuocao Wang Yu Dai Bin Li Olga Starostenko Jianping Lai Lei Wang Key Laboratory of Eco-chemical Engineering Ministry of EducationTaishan scholar advantage and characteristic discipline team of Eco-chemical process and technologyLaboratory of Inorganic Synthesis and Applied ChemistryCollege of Chemistry and Molecular EngineeringQingdao University of Science and TechnologyQingdao 266042China College of Foreign Languages Qingdao City UniversityQingdao 266106China College of Materials Science and Engineering Qingdao University of Science and TechnologyQingdao 266042China Institute of Macromolecular Chemistry of the National Academy of Sciences of Ukraine Kyiv 02160Ukraine Shandong Engineering Research Center for Marine Environment Corrosion and Safety Protection College of Environment and Safety EngineeringQingdao University of Science and TechnologyQingdao 266042China

The main problem faced by ethanol oxidation reaction(EOR)includes low activity,poor selectivity,and *** the study,we found that polysulfide modified on the surface of PtCu intermetallic(IM)/C can simultaneously enrich hydroxyl and ethanol,which could effectively improve the catalytic activity,CO_(2) selectivity,and durability of *** mass activity and the specific activity of the product in 1 M KOH electrolyte reached 17.83 A·mgPt^(-1) and 24.67 mA·cm^(-2).The CO_(2) selectivity of polysulfide modified product achieved 93.5%,which was 30 folds higher than Pt/*** addition,the catalyst showed high catalytic *** mechanism study demonstrates that the surface modified polysulfide could significantly boost the enrichment effect of ethanol and hydroxyl species,accelerating C–C bond cleavage and CO oxidation.

关键词： Pt CO_(2) selectivity enrichment effect ethanol oxidation reaction(EOR) electrocatalyst

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Comparative Study of Proton and Heavy Ion-induced Damages for GaN-based HEMTs 24

Comparative Study of Proton and Heavy Ion-induced Damages fo...

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8th International Conference on Electronic Information technology and Computer engineering, EITCE 2024

作者： Wu, Zhipeng Huang, Huixiang Yang, Jianqun Lei, Zhifeng Cui, Xiuhai Ma, Teng Peng, Chao School of Opto-electronic and Communication Engineering Xiamen University of Technology Fujian Xiamen China National Key Laboratory of Material Behavior and Evaluation Technology in Space Environment Harbin Institute of Technology Heilongjiang Harbin China Science and Technology on Reliability Physics and Application of Electronic Component Laboratory China Electronic Product Reliability and Environmental Testing Research Institute Guangdong Guangzhou China

ISBN: (纸本)9798400710094

The variations of the radiation damage induced by radiation from protons and heavy ions on Cascode GaN HEMTs are comparatively studied. 300 MeV proton and 500 MeV heavy ion irradiation are carried out for AlGaN/GaN HEMTs. Findings from the study indicate that exposure to a proton flux of 300 MeV, reaching a cumulative level of 1×1011 cm-2, leads to a reduction in the output current. Concurrently, there is a downward adjustment of 0.27 volts in the turn-on voltage, along with a 5.59% decline in the peak transconductance. Following irradiation, the creation of traps within the device’s channel layer results in a decline in its electrical efficiency. Under 500 MeV heavy ion irradiation with a total fluence of 3.167×105cm-2, a significant leakage current increase is observed when a drain bias of 100 volts is applied. An enhancement in the output current is observed, accompanied by a 0.11V downward adjustment in the voltage at which the channel forms and a significant 70.17% diminution in peak transconductance. Additionally, instances of single event burnout (SEB) are detectable when the drain bias exceeds 150 V. © 2024 Copyright held by the owner/author(s).

关键词： Gallium nitride

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Degradation properties of fulvic acid and its microbially driven mechanism from a partial nitritation bioreactor through multi-spectral and bioinformatic analysis

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Journal of environmental sciences 2024年第1期135卷 318-331页

作者： Quanhao Dou Li Zhang Tingjun Dong Zixuan Song Xuepeng Fan Yongzhen Peng Xiayan Wang Jiachun Yang National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery EngineeringBeijing University of TechnologyBeijing 100124China Department of Chemistry and Biology Center of Excellence for Environmental Safety and Biological EffectsBeijing Key Laboratory for Green Catalysis and SeparationBeijing University of TechnologyBeijing 100124China Environmental Protection Development Group Co. Ltd.Shandong 250101China

This study employed multispectral techniques to evaluate fulvic acid(FA)compositional characteristic and elucidate its biodegradation mechanisms during partial nitritation(PN)*** showed that FA removal efficiency(FRE)decreased from 90.22 to 23.11%when FA concentrations in the reactor were increased from 0 to 162.30 mg/L,and that molecular size,degree of aromatization and humification of the effluent FA macromolecules all increased after *** population analysis indicated that the proliferation of the Comamonas,OLB12 and Thauera exhibit high FA utilization capacity in lower concentrations(<50.59 mg/L),promoting the degradation and removal of macromolecular *** addition,the sustained increase in external FA may decrease the abundance of above functional microorganisms,resulting in a rapid drop in ***,from the genetic perspective,the elevated FA levels restricted carbohydrate(ko00620,ko00010 and ko00020)and nitrogen(HAO,AMO,NIR and NOR)metabolism-related pathways,thereby impeding FA removal and total nitrogen loss associated with N_(2)O emissions.

关键词： Partial nitritation Fulvic acid 3DEEM-PARAFAC UV/Vis Microbially driven mechanism

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Adsorption of typical gasoline vapor emitted from service stations by commercial activated carbon:static/dynamic adsorption and kinetics simulation

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Frontiers of environmental science & engineering 2025年第3期19卷 87-98页

作者： Wei Hu Quanming Liang Dan Lu Beibei Li Biqi Ren Qingye Luan Jia Liu Wenjun Liang Yuhu Huang National Engineering Research Center of Urban Environmental Pollution Control Beijing Key Laboratory of Urban Atmospheric Volatile Organic Compounds Control Technology and ApplicationsBeijing Municipal Research Institute of Eco-Environmental ProtectionBeijing 100037China Key Laboratory of Beijing on Regional Air Pollution Control Faculty of Environment and LifeBeijing University of TechnologyBeijing 100124China Institute of Urban Safety and Environmental Science Beijing Academy of Science and TechnologyBeijing 100054China

Gasoline vapor emissions from service stations significantly affect urban *** the research on the mechanisms and effectiveness of gasoline vapor removal is limited,this study innovatively investigates the static and dynamic adsorption of xylene—a typical gasoline vapor and one of the most active secondary organic aerosol(SOA)species—by commercial activated carbon(AC).The results showed that the saturation static adsorption capacity(Q_(e))of 12 ACs varied from 0.9 to 870.7 mg/g,which correlated with the specific surface area(SSA)and pore *** them,11#and 12#ACs were identified as the most effective adsorbents for typical gasoline vapor *** maximum dynamic Q_(e) increased from 301.5 to 414.3 mg/g when the initial xylene concentration rose from 918 to 2008 mg/m^(3) for 11#AC,and from 201.4 to 406.2 mg/g when the initial xylene concentration increased from 589 to 2120 mg/m^(3) for 12#*** findings implied a direct correlation between higher initial xylene concentrations and greater dynamic Q_(e) values,with static Q_(e) values surpassing dynamic *** adsorption kinetics simulation were analyzed by the pseudo-first-order(PFO)and pseudo-second-order(PSO)*** kinetics results demonstrated that the PFO was more effective in characterizing the adsorption of xylene onto ACs(R2>0.989),indicating that the adsorption of typical gasoline vapor by ACs primarily involves physical *** findings of static/dynamic adsorption and kinetics provide valuable guidance for practical applications of gasoline vapor removal in service stations.

关键词： Activated carbon Gasoline vapor Xylene Dynamic adsorption Breakthrough curve

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Sulfhydryl-modified zeolite A with exceptional strontium adsorption selectivity

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science China Chemistry 2025年第5期68卷 1847-1858页

作者： Lingyi Li Lanxing Ren Dong Wang Junchang Chen Qi Guo Yuting Zhao Fuqiang Zhao Linwei He Jie Li Wenqi Zhang Lijuan Song Long Chen Lixi Chen Bin Wang Lin Zhu Tao Duan Zhifang Chai Shuao Wang State Key Laboratory of Radiation Medicine and Protection School for Radiological and Interdisciplinary Sciences (RAD-X)and Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education InstitutionsSoochow University School of Science Harbin Institute of Technology (Shenzhen) School of Chemistry and Chemical Engineering Hunan Province Key Laboratory for the Design and Application of Actinide ComplexesUniversity of South China Radioactive Waste Technology and Radiochemistry Research Department China Nuclear Power Technology Research Institute Co.Ltd. State Key Laboratory of Environment-Friendly Energy Materials School of National Defence Science & TechnologySouthwest University of Science and Technology

Efficient removal of trace radiostrontium from contaminated highly saline wastewater,such as seawater,remains a critical but challenging task due to the coexistence of large excess of hard cations like Na+,K+,Mg2+and particularly Ca2+,which shares similar physicochemical properties with Sr2+.Herein,we successfully boosted the selectivity by a sulfhydryl-functionalized NaA zeolite（SH-NaA） via ion exchange coupled with reinforced soft-soft interactions between sulfhydryl groups and Sr2+.Remarkably,SH-NaA achieved a 99.8%removal efficiency of Sr2+in the presence of a tenfold excess of Ca2+,with a distribution coefficient（Kd） of 4.98×10～5mL/*** effectiveness of SH-NaA in accurately capturing Sr2+was further validated by its superior dynamic adsorption performance in natural seawater compared to pristine NaA *** experiments highlighted SH-NaA’s exceptional Sr2+removal efficiency（qm=233.36 mg/g）,rapid adsorption kinetics（1 min）,superior decontamination depth（Kd=6.71×10～5mL/g）,and robust irradiation stability（400 kGy γ-ray）.X-ray photoelectron spectroscopy（XPS） and in situ Fouriertransform infrared（FTIR） analyses underscored the pivotal role of sulfhydryl groups in Sr2+*** functional theory（DFT） calculations revealed that the sulfhydryl-functionalized NaA zeolite exhibits the best selectivity toward Sr2+,with an interaction energy of-2.55 *** findings demonstrate that organic group functionalized zeolites hold significant promise for environmental remediation applications.

关键词： strontium selectivity adsorption seawater sulfhydryl NaA zeolite

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Dimethylammonium cation stabilizes all-inorganic perovskite solar cells

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Journal of Semiconductors 2023年第3期44卷 4-8页

作者： Zuolin Zhang Mengjia Li Jie Sun Cong Chen Jiangzhao Chen Liming Ding State Key Laboratory of Reliability and Intelligence of Electrical Equipment School of Materials Science and EngineeringHebei University of TechnologyTianjin 300401China Key Laboratory of Optoelectronic Technology&Systems(MoE) College of Optoelectronic EngineeringChongqing UniversityChongqing 400044China Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190China Macao Institute of Materials Science and Engineering(MIMSE) Macao University of Science and TechnologyMacao 999078China

Facing the poor environmental stability of traditional methylammonium or formamidinium-based lead halide per-ovskites,scientists turn their attention to inorganic lead hal-ide perovskites(ILHPs)with narrow bandgaps,excellent thermal stability and reduced ion migration compared to their organic/inorganic counterparts[1−4].Up to now,the PCEs for ILHP solar cells exceed 21%[5].Especially,the preferred black ILHP(***3)with the smallest bandgap of~1.7 eV and single-halide composition for avoiding phase separation is crucial for high-performance single-junction solar cells and can be applied in tandem devices as the top cells[6,7].However,small Cs+(167 pm)in CsPbI3 with a tolerance factor close to 0.8 is unsuitable for the 3D PbI3-framework[8].The mis-matched size of cations will induce lattice strain and the per-ovskite spontaneously transforms to undesired non-photoact-ive yellow phase(δ-phase,like NH4CdCl3)(Fig.1(a))[9,10].There-fore,improving lattice symmetry and reducing lattice strain are the strategies for inhibiting the phase transition of ILHPs.

关键词： inorganic perovskite ammonium

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