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SSRN 2025年

作者： Liu, Yunlian Liu, Mingkai Shen, Yuanhui Li, Yang Gai, Zhongrui Zhang, Ruqi Pan, Ying Jin, Hongguang Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing100190 China University of Chinese Academy of Sciences Beijing100049 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China

The integrated CO2 capture and conversion (ICCC) has emerged as a promising and cost-effective pathway for achieving carbon neutrality. However, limited energy-efficient pathways and durable materials for ICCC systems remains challenging. This study proposes a novel approach that synergistically integrates CO2 capture and conversion through a unified chemical framework. The method employs Li-based sorbents for CO2 capture, coupled with CH4-driven sorbent regeneration that is seamlessly integrated with chemical looping dry reforming of methane (CLDRM), enabling in-situ CO2 conversion. By coupling sorbent regeneration with CLDRM, this system enhances decarbonation kinetics through Le Chatelier's principle via continuous CO2 conversion. One-step calcination synthesized Li-based sorbents particles exhibit stable CO2 capture capacity of 5.25 mmol·g-1 within 15 min per cycle, maintaining 7.5-15% operational efficiency over 40 cycles at 600 ℃. In CLDRM, hydrogen radicals from CH4 dissociation promote the conversion of CO2 to intermediates, lowering the apparent activation energy of sorbents regeneration by 29.2%. Through systematic optimization in a fixed-bed reactor, we achieved 90% CO2 uptake and 85% CH4 conversion, with syngas production rates reaching 13.71 mL·min-1·g-1. Notably, the H2/CO molar ratio in syngas stabilizes ~1.6, aligns with iron-based Fischer-Tropsch and methanol synthesis to produce valuable fuels. This integrated system maintains >80% syngas purity with © 2025, The Authors. All rights reserved.

关键词： Activation energy

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Large eddy simulation on the wake characteristics of linearly stratified flow past a sphere

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Scientific Reports 2025年第1期15卷 1-13页

作者： Xia, Tianci Wei, Na Shi, Liuliu School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai 200093 China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering Shanghai 200093 China Key Laboratory of Power Machinery and Engineering of Ministry of Education Shanghai Jiao Tong University Shanghai 200240 China

In this study, Large Eddy Simulation (LES) has been employed to examine the influence of the Froude number (Fr) on the linearly stratified wake and internal waves behind a sphere at a subcritical Reynolds number of Re = 3700. Six distinct sets of models with varying Fr (Fr = 0.05, 0.25, 0.5, 1, 2, ∞) have been chosen to establish density linear stratification through the use of a User Defined Function (UDF). The analysis focuses on the impact of stratification on wake characteristics, velocity distribution, and the structure of internal waves within stratified flow. It is evident that density stratification plays a pivotal role in shaping wake structure. Notably, in stratified flows, wakes exhibit unique characteristics including the generation of internal waves, suppression of vertical velocity, and the emergence of oscillating wake patterns. The study reveals that a decrease in the Froude number leads to heightened vertical suppression of the wake and increased anisotropy of the velocity distribution. Furthermore, as the Froude number ascends from 0.05 to 2, the wake undergoes a transition from quasi-two-dimensional vortex shedding to three-dimensional turbulence. © The Author(s) 2025.

关键词： Froude number Internal wave Linearly stratified flow Wake

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AN EXPERIMENTAL INVESTIGATION ON THE INTERFACIAL WAVES IN AIR-WATER TWO-PHASE flow WITHIN HORIZONTAL PIPELINES

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Chinese Journal of Chemical engineering 1997年第4期5卷 34-42页

作者：李广军郭烈锦陈学俊 National Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

By using two-parallel conductance probes,the instantaneous film thickness of gas-liquidtwo-phase flow within a horizontal plexiglass pipe of 50mm inner diameter was *** pipe was 6680mm *** wave patterns were distinguished through statisticalanalysis of signals of film *** pattern maps were obtained and compared with resultsof former *** characteristics of the interfacial waves,such as time-averaged film thickness,wave height,wave propagation speed,wavelength and wave frequency,were systematically *** effect of the exit structure of the test section on interfacial waves was experimentally examined.

关键词： interfacial waves two-phase flow conductance probe

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Teardrop-like micro pin fin coated nanotube arrays chip for enhancement of flow boiling electronics cooling

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International Journal of Thermal Sciences 2025年 214卷

作者： Chen, Hongqiang Gao, Quan Ma, Xiang Li, Kai Du, Wangfang Li, Caifeng Zhang, Yonghai Wei, Jinjia School of Chemical Engineering and Technology Xi'an Jiaotong University 28 Xianning West Road Shaanxi Xi'an710049 China Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China National Microgravity Laboratory Institute of Mechanics Chinese Academy of Sciences Beijing100190 China School of Engineering Science University of Chinese Academy of Sciences Beijing100149 China Xi'an Shaangu Power Co. Ltd. Xi'an710075 China

Phase change flow boiling heat transfer in microchannel is a very efficient thermal management mode for high-power electronics/devices cooling. However, achieving comprehensive enhancement of flow boiling heat transfer performance at low power consumption is still challenging. Herein, we devised and manufactured a teardrop-like micro-pin-fin coated stable copper hydroxide nanotubes array chip surfaces (S-Nanotube), demonstrating their exceptional enhancement in flow boiling heat transfer efficiency. A series of experiments were conducted using HFE-7100 as a working fluid within a semi-open microchannel. Compared to the smooth surface, the critical heat flux (CHF) and the maximum boiling heat transfer coefficient (HTC) of the S-Nanotube is increased by 82.1 % (from 45.1 to 72.9 and then to 82.1 W/cm2) and 140.5 % (from 5955 to 11,325 and then to 14,316 W/m2·K) at extremely low-pressure drop (≤4 kPa), showing a high coefficient of performance (COP). The temperature of the onset of nucleate boiling on the S-Nanotube surface is reduced by 26.4 %, and the heat flux is greatly increased in a small wall temperature variations (ΔT ≤ 10 °C). In situ observation and analysis of the surface properties and the bubble dynamics, the S-Nanotube chip promotes the phase change heat transfer process by providing massive nucleation sites, reducing bubbles size and residence time, and enhancing the wicking wetting capacity. These findings provide guidance for the rational design of boiling heat transfer-enhanced surfaces and heat sinks and point the way to achieving efficient thermal management of power devices. © 2025 Elsevier Masson SAS

关键词： Electronic cooling

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Numerical Study of Multi-Factor Coupling Effects on Energy Conversion Performance of Nanofluidic Reverse Electrodialysis

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Frontiers in Heat and Mass Transfer 2025年第2期23卷 507-528页

作者： Hao Li Cunlu Zhao Jinhui Zhou Jun Zhang Hui Wang Yanmei Jiao Yugang Zhao School of Physical and Mathematical Sciences Nanjing Tech UniversityNanjing211816China MOE Key Laboratory of Thermo-Fluid Science and Engineering Xi’an Jiaotong UniversityXi’an710049China Key Laboratory of Unsteady Aerodynamics and Flow Control Ministry of Industry and Information TechnologyNanjing University of Aeronautics and AstronauticsNanjing210016China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power EngineeringUniversity of Shanghai for Science and TechnologyShanghai200093China Key Laboratory of Icing and Anti/De-icing China Aerodynamics Research and Development CenterMianyang621000China

Based on the rapid advancements in nanomaterials and nanotechnology,the Nanofluidic Reverse Electrodialysis(NRED)has attracted significant attention as an innovative and promising energy conversion strategy for extracting sustainable and clean energy fromthe salinity gradient ***,the scarcity of research investigating the intricate multi-factor coupling effects on the energy conversion performance,especially the trade-offs between ion selectivity and mass transfer in nanochannels,of NRED poses a great challenge to achieving breakthroughs in energy conversion *** numerical study innovatively investigates the multi-factor coupling effect of three critical operational factors,including the nanochannel configuration,the temperature field,and the concentration difference,on the energy conversion processes of *** this work,a dimensionless amplitude parameter s is introduced to emulate the randomly varied wall configuration of nanochannels that inherently occur in practical applications,thereby enhancing the realism and applicability of our *** results reveal that the application of a temperature gradient,which is oriented in opposition to the concentration gradient,enhances the ion transportation and selectivity simultaneously,leading to an enhancement in both output power and energy conversion ***,the increased fluctuation of the nanochannel wall from s=0 to s=0.08 improves ion selectivity yet raises ion transport resistance,resulting in an enhancement in output power and energy conversion efficiency but a slight reduction in ***,with increasing the concentration ratio cH/cL from 10 to 1000,either within a fixed temperature field or at a constant dimensionless amplitude,the maximumpower consistently attains its optimal value at a concentration ratio of 100 but the cation transfer number experiences amonotonic decrease across this entire range of concentration ***,uponmodifying the ope

关键词： Salinity gradient energy nanofluidic reverse electrodialysis energy conversion nanochannel configuration multi-factor coupling effect

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Effect of surface roughness on corrosion behaviour of stainless steel in supercritical CO 2

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Journal of Materials Research and Technology 2025年 36卷 4946-4954页

作者： Liyong Cao Wenyan Zhang Chongjun Jiang Hui Wang Hong An Chao Ye Jiyun Ren Xiaole Huang Lei Deng China University of Xihua Chengdu 610039 China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an 710049 China China University of Petroleum-Beijing Beijing 102249 China PipeChina Gansu Branch Lanzhou 730070 China Zhengzhou Yutong Group Co. Ltd. Zhengzhou 450000 China

To study the effect of surface roughness on the corrosion behavior of austenitic steels in supercritical CO 2 , the corrosion experiments were conducted on 304 and 310S stainless steels at 550 °C and 15 MPa. The corroded samples were characterized using XRD and SEM-EDS. The results demonstrate that surface roughness significantly affects the morphology and structure of the oxide films formed on 310S stainless steel. Samples prepared with varying surface roughness (grounded using from 200# to 1000# metallographic abrasive papers) showed that rougher surfaces tend to develop denser oxide layers, whereas smoother surfaces exhibit relatively loose and porous oxide films. Despite these differences in oxide structure, the overall corrosion weight gain remained largely unaffected, indicating minimal oxide shedding from 310S steel. The oxidation product is mainly Cr 2 O 3 . For 304 stainless steel, surface roughness was found to influence the composition of surface oxides. Both 200# and 1000# samples formed loose, porous oxide films prone to spallation, with the primary constituents being Fe 3 O 4 , (Fe, Cr) 3 O 4 and Fe 2 O 3 . Because the content of (Fe, Cr) 3 O 4 and Fe 3 O 4 of the former is higher, more voids appear in the oxide film, leading to spallation within the first 100 h of exposure. The rougher surface showed a more pronounced loss of oxide. But for the 600# sample, the main component is Fe 2 O 3 . Carburization was observed to intensify with increasing surface roughness in both materials. Notably, the 200# sample of 310S stainless steel exhibited more severe carburization compared to the 1000# sample of 304 stainless steel.

关键词： Supercritical CO 2 Corrosion Austenitic stainless steels Surface roughness Oxidation

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A 3D-dimensional interconnected structured poly (m-phenylene isophthalamide) nanofiber separator with Li1.5Al0.5Ge1.5(PO4)3 for high-safety lithium-sulfur batteries

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Journal of power Sources 2025年 645卷

作者： Liu, Jianwei Zhu, Lei Chai, Qinqin Sun, Shiyi Yang, Xiaomeng Sun, Jingyun Zhang, Yating Zhu, Youyu Yan, Wei College of Chemistry and Chemical Engineering Xi'an University of Science and Technology Shaanxi Xi'an710054 China Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiao tong University Shaanxi Xi'an710049 China Xi'an Hantang Analysis & Test Co. Ltd Shaanxi Xi'an710201 China

Safety concerns have consistently presented substantial obstacles to the widespread adoption of lithium-sulfur (Li-S) batteries. Conventional polyolefin separators, which are characterized by low flash points and insufficient mechanical strength, pose potential safety hazards, including risks of fire and explosion under extreme operating conditions. In this study, we introduce a thermally stable and non-flammable poly-m-phenyleneisophthalamide (PMIA)-based multifunctional separator (L-PMIA separator), which is enhanced with lithium aluminum germanium phosphate (Li1.5Al0.5Ge1.5(PO4)3 or LAGP) fillers. By incorporating g high-ionic-conductivity LAGP and establishing an interconnected framework, this design effectively mitigates the issues of particle agglomeration and uneven commonly ion transport associated with traditional separators. The L-PMIA separator demonstrates remarkable mechanical strength (with a tensile strength of 8.5 MPa and a puncture force of 0.72 N) and thermal stability (showing no dimensional shrinkage even at 200 °C), while also facilitating the formation of continuous ion channels that inhibit lithium dendrite growth. Consequently, Li-S batteries utilizing the 4L-PMIA separator demonstrated a reversible capacity of 4.97 mAh cm−2 after 150 cycles, even under conditions of high sulfur loading (6.75 mg cm−2), limited electrolyte availability (E/S = 7), and elevated temperatures. This approach offers novel insights for the development of future energy storage systems characterized by enhanced safety and performance. © 2025 Elsevier B.V.

关键词： Lithium sulfur batteries

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Detachment Size Measurement of Two Interacting Bubble Plumes Formed at Neighboring Needles Using an Acoustic Method

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Chinese Journal of Chemical engineering 1999年第2期7卷 145-153页

作者：向宇孙科霞郭烈锦陈学俊 National Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

Detachment size determination with an acoustic method has been carried out for two interacting bubble plumes formed at neighboring needles in quiescent water. Two sets of needle pairs, one with 1.5mm and 0.8mm inner diameters and the other with the equal 1.5mm inner diameters, were separately used as the bubble pair injectors in the experiments. Consequently, four typical patterns of bubble plumes interaction could be observed in the two cases of needle pair matches. Through measuring the pressure pulses radiated by the bubble pairs immediately after their 'pinching-off ' and by making use of a sophisticated relation between oscillation frequency of volume mode and radius of gas bubble, the detachment size of the bubble plumes have been determined from the amplitude/frequency spectrum of the sound pressure pulses. The experimental results demonstrate that the acoustical method is valid in both of the interacting and non-interacting circumstances in bubble field and the bubble size measurements by this acoustical method agree well with the measurements from photographic analysis. Finally, a comparison has been made on the strong and weak points of the acoustical method with the other size determination methods.

关键词： detachment size determination sound pressure pulses acoustical method bubble interaction bubble plumes

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Thermodynamics analyses on a novel CHP system integrated with multi-grade thermal energy storage

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Journal of Energy Storage 2025年 106卷

作者： Liu, Rongtang Zhang, Kezhen Qin, Yuanzhi Wan, Kaidi Xu, Can Liu, Ming Ningbo Institute of Technology Beihang University Ningbo315800 China Xi'an Thermal Power Research Institute Co. Ltd. Xi'an710054 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China Dongfang Boiler Co. Ltd. of Dongfang Electric Group Chengdu611731 China

The high penetration level of intermittent renewable power necessitates the crucial requirement for combined heat and power systems to possess both high efficiency and flexibility. However, the heat-controlled operation modes of traditional combined heat and power systems impose limitations on their efficiency and flexibility. Therefore, it is of great significance to develop a heat-power decoupling technology that exhibits exceptional efficiency and flexibility. A novel combined heat and power system integrated with multi-grade thermal energy storage is proposed in this study. Thermodynamic analysis models of all operational conditions are developed, and the comprehensive characteristics of efficiency and operational flexibility for the proposed system are assessed by taking a 330 MW system as an example. Results show that the proposed system can decrease/increase 16.05 MW/30.96 MW power loads comparing with the reference system during the charging/discharging periods under the design condition. Energy efficiency of the proposed system can reach 49.40 %, which is improved by 1.66 percentage points. Exergy analysis reveals the exergy destruction order for the proposed system, and shows that the combustion and heat transfer in the boiler are the major process of exergy dissipation. Moreover, operation strategies of the proposed system during charging-discharging cycle are explored and formulated under off-design condition, suggesting that thermodynamic performances of the novel system under various conditions even extreme conditions exhibits exceptional properties. The maximum heat load of the proposed system can be improved by 46.78 % comparing with the reference system, and the maximum improvement of power load capacity during charging-discharging cycle is 14.58 percentage points. This study provides a promising approach for multi-grade thermal energy storage to improve the comprehensive characteristics of combined heat and power systems. © 2024

关键词： Charge storage

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Low-energy and accelerated hydrogen release from MgH2–5 wt% NaTiOxH catalyzed hydrogen storage reactor by graphite responsive microwave

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Journal of Magnesium and Alloys 2025年

作者： Wang, Bofei Wu, Zhen Liu, Honghao Yang, Fusheng Zhang, Zaoxiao Yao, Jing Li, Qian Cao, Hujun Li, Bo State Key Laboratory of Fluorine & Nitrogen Chemicals School of Chemical Engineering and Technology Xi'an Jiaotong University Xi'an710049 China State Key Laboratory of Multiphase Flow for Power Engineering Xi'an Jiaotong University Xi'an710049 China National Engineering Research Center for Magnesium Alloys Chongqing University Chongqing400044 China Dalian National Laboratory for Clean Energy Dalian Institute of Chemical Physics Chinese Academy of Sciences Dalian116023 China Faculty of Engineering Electrical Energy Management Group University of Bristol BristolBS8 1QU United Kingdom

Owing to high thermal stability and large reaction enthalpy, MgH2 has high reaction temperatures and sluggish reaction kinetics in the dehydrogenation process, which consumes lots of energy. To achieve hydrogen release with low energy consumption, accelerated reaction rate, and high heating uniformity, this paper proposes a novel method of graphite responsive microwave-assisted thermal management with NaTiOxH catalyst. A multi-physics model of the 5 wt% NaTiOxH catalyzed MgH2 reactor integrated with a microwave generator is developed to investigate the reaction, heat and mass transfer process of hydrogen release. It is found that the graphite responsive microwave heating method could improve the temperature uniformity of reaction bed, reduce the energy consumption by at least 10.71% and save the hydrogen release time by 53.49% compared with the traditional electric heating method. Moreover, the hydrogen desorption thermodynamics could be improved with the increase of microwave power. The hydrogen release time is shortened by 19.55% with the increase of 20 W microwave power. Meanwhile, it is also concluded that the microwave excitation frequency of 2.1 GHz and the graphite content of 2 wt% have better heating performance. Therefore, it can be verified that the graphite responsive microwave heating helps to low-energy and accelerated hydrogen release from MgH2 hydrogen storage reactor. © 2025

关键词： Reaction rates

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