检索结果-内蒙古大学图书馆

Small molecule probes for the specific imaging of monoamine oxidase A and monoamine oxidase B

iRADIOLOGY 2024年第2期2卷 191-215页

作者： Yi Fang Zhengping Chen Min Yang NHC Key Laboratory of Nuclear Medicine Jiangsu Key Laboratory of Molecular Nuclear MedicineJiangsu Institute of Nuclear MedicineWuxiJiangsu ProvinceChina Key Laboratory of Organic Synthesis of Jiangsu Province College of ChemistryChemical Engineering and Materials ScienceSoochow UniversitySuzhouJiangsu ProvinceChina

Monoamine oxidases(MAOs)are a class of flavin enzymes that are mainly present in the outer membrane of mitochondria and play a crucial role in maintaining the homeostasis of monoamine neurotransmitters in the central nervous ***,expression of MAOs is associated with the functions of peripheral *** of MAOs is relevant in a variety of diseases such as neurodegenerative diseases,heart failure,metabolic disor-ders,and *** oxidases have two isoenzymes,namely,monoamine oxidase A(MAO-A)and monoamine oxidase B(MAO-B).Therefore,the development of reliable and specific methods to detect these two isoenzymes is of great significance for the in-depth understanding of their functions in biological systems,and for further promoting the clinical diag-nosis and treatment of MAO-related *** review mainly focuses on the advances in small molecular probes for the specific imaging of MAO-A and MAO-B,including radiolabeled probes,fluorescent probes,and a 19F magnetic resonance imaging *** addition,applications of these probes for detecting MAO expression levels in cells,tissues,animal models,and patients are ***,the challenges and perspectives of developing novel MAO imaging probes are also highlighted.

关键词： monoamine oxidases radiolabeled probes fluorescent probes 19F MRI probe bioimaging diseases

来源：评论

学校读者我要写书评

暂无评论

Investigation of He retention in W through combined He characterization methods and cluster dynamics model

引用

nuclear science and Techniques 2025年第3期36卷 201-213页

作者： Jie Qiu Xun-Xiang Hu Cong-Yi Li Wendy Garcia Tan Shi Sha Xue Jamie L.Weaver HHeather Chen-Mayer Brian D.Wirth SJTU Paris Elite Institute of Technology Shanghai Jiao Tong UniversityShanghai 200240China Department of Nuclear Engineering University of TennesseeKnoxvilleTN 37996USA School of Physics Sichuan UniversityChengdu 610065China Oak Ridge National Laboratory Oak RidgeTN 37830USA Global Institute of Future Technology Shanghai Jiao Tong UniversityShanghai 200240China School of Nuclear Science and Technology Xi’an Jiaotong UniversityXi’an 710049China Nuclear Engineering Program The Ohio State UniversityColumbusOH 43210USA Material Measurement Laboratory National Institute of Standards and TechnologyGaithersburgMD 20899USA

Tungsten(W)is the leading plasma-facing candidate material for the International Thermonuclear Experimental Reactor and next-generation fusion *** impact of synergistic helium(He),irradiation-induced microstructural changes,and the corresponding thermal-mechanical property degradation of W are critically important but are not well understood *** the performance of W in fusion environments requires understanding the fundamentals of He-defect interactions and the resultant He bubble nucleation and growth in *** this study,He retention in helium-ion-implanted W was assessed using neutron depth profiling(NDP),laser ablation mass spectrometry(LAMS),and thermal desorption spectroscopy(TDS)following 10 keV room-temperature He implantation at various *** three experimental techniques enabled the determination of the He depth profile and retention in He-implanted W.A cluster dynamics model based on the diffusion-reaction rate theory was applied to interpret the experimental *** model successfully predicted the He spatial depth-dependent profile in He-implanted W,which was in good agreement with the LAMS *** model also successfully captured the major features of the He desorption spectra observed in the THDS *** NDP quantified total He concentration values for the samples;they were similar to those estimated by ***,the depth profiles from NDP and LAMS were not comparable due to several *** combination of modeling and experimentation enabled the identification of possible trapping sites for He in W and the evolution of He-defect clusters during the TDS thermal annealing process.

关键词： Tokamak nuclear reactor Nondestructive detection

来源：评论

学校读者我要写书评

暂无评论

Na-22 for Safeguarding and Mass Accounting of Molten Salt Systems

Na-22 for Safeguarding and Mass Accounting of Molten Salt Sy...

引用

2023 Transactions of the American nuclear Society Winter Conference and Expo, ANS 2023

作者： Zile, Matthew Van Kauffman, Andrew Herminghuysen, Kevin Li, Shelly Simpson, Michael Kandlakunta, Praneeth Cao, Guoping Cao, Lei R. Nuclear Engineering Program Department of Mechanical and Aerospace Engineering Ohio State University United States Nuclear Reactor Laboratory College of Engineering Ohio State University United States Department of Materials Science and Engineering University of Utah.Idaho National Laboratory United States

The Na-22based radioactive tracer dilution (RTD) technique has been previously demonstrated for mass accounting in small quantities of clean molten salt for bench top testing. While the concept of RTD has proven to be a promising method, it has lacked further validation in large-scale quantities and in fuel-bearing salt. Towards that end, two research initiatives are on-going at The Ohio State University (OSU) and Idaho National laboratory (INL) to address these challenges. Current work at OSU is focused on evaluating the RTD using the full gamma-ray spectrum of fission products produced by irradiating fuel bearing salt, i.e., UCl3-MgCl2-KCl in a 500-kW research reactor. The INL team has successfully demonstrated the RTD for mass determination using an 8-kg LiCl-KCl-UCl3salt for uranium electrorefining and is currentlyseeking to validate the tracer method with large(about 60 kg)molten salt system(bearing fission products) in an oxide reduction (OR) facility for spent nuclear fuel (SNF) reprocessing. © 2023 American nuclear Society. All rights reserved.

关键词： Fission products

来源：评论

学校读者我要写书评

暂无评论

Band convergence boosted high thermoelectric performance of Zintl compound Mg_(3)Sb_(2) achieved by biaxial strains

引用

Journal of Materiomics 2022年第5期8卷 1086-1094页

作者： Suiting Ning Shan Huang Ziye Zhang Ning Qi Man Jiang Zhiquan Chen Xinfeng Tang Hubei Nuclear Solid Physics Key Laboratory Department of PhysicsWuhan UniversityWuhan430072China Department of Nuclear Engineering and Technology School of Energy and Power EngineeringHuazhong University of Science and TechnologyWuhan430073China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan430070China

Mg_(3)Sb_(2) as a Zintl compound is a promising thermoelectric material with the intrinsically low lattice thermal conductivity and excellent n-type electrical properties,but its p-type electrical transport properties are ***,the thermoelectric performance of Mg_(3)Sb_(2) under the effect of biaxial strain is investigated by using first-principles method and Boltzmann transport *** application of biaxial strain enables tuning the band structure of Mg_(3)Sb_(2) in such a way that the band degeneracy of both the conduction band and valence band *** the biaxial strain increases,the Seebeck coefficient of ptype Mg_(3)Sb_(2) has a remarkable increase,leading to a significant improvement in power *** is mainly ascribed to the achievement of valence band orbital ***,the lattice thermal conductivity exhibits very slight biaxial strain dependence within the strain range considered in this work,which increases from 1.28 to 1.62 W m^(-1) K^(-1) at 300 ***,the highest ZT of p-type Mg_(3)Sb_(2) at 700 K can be up to 2.6 along the in-plane direction under-2.5%biaxial strain,which is almost three times that of the unstrained *** realization of high thermoelectric performance of p-type Mg_(3)Sb_(2) will promote its practical applications as thermoelectric generators.

关键词： Thermoelectric First-principles Crystal field splitting energy Band convergence

来源：评论

学校读者我要写书评

暂无评论

Transport and magnetic properties of Hund's metal CaRuO3 under strain modulation

引用

Physical Review B 2024年第4期110卷 L041403-L041403页

作者： Zhen Wang Arjyama Bordoloi Zhaoqing Ding Enling Wang Xiaofeng Wu Zeguo Lin Mingyu Yang Chenxu Liu Jinglin Zhou Meng Meng Fang Yang Qinghua Zhang Xiaoran Liu Sobhit Singh Huan-hua Wang Jiandong Guo Beijing National Laboratory for Condensed Matter Physics and School of Nuclear Science and Technology Department of Mechanical Engineering School of Physical Sciences Materials Science Program

We synthesized CaRuO3 (001) thin films on a set of substrates and investigated their electronic and magnetic properties via combining magnetotransport measurements with first-principles density-functional theory calculations. The experimental results indicate that a moderate strain can introduce the Kondo effect in the system, leading to a significant modulation of the non-Fermi liquid behavior. Moreover, when the strain reaches a certain threshold, the system undergoes a metal-semiconductor transition, accompanied by a transition from a nonmagnetic state to a plausible G-type antiferromagnetic state. We attribute the observed phenomena in CaRuO3 to strain-induced disruption of the delicate balance between the itinerant and the local Ru 4d electrons. These findings shed light on the intriguing magnetic and non-Fermi liquid behavior of CaRuO3, systematically tailored by heteroepitaxial strain.

关键词： Density of states Kondo effect Transport phenomena Ruthenates Ultrathin films Density functional calculations Physical deposition Resistivity measurements Strain engineering X-ray diffraction X-ray reflectivity

来源：评论

学校读者我要写书评

暂无评论

A lithiated gel polymer electrolyte with superior interfacial performance for safe and long-life lithium metal battery

引用

Journal of Energy Chemistry 2021年第4期30卷 313-322页

作者： Jia-Jia Yuan Chuang-Chao Sun Li-Feng Fang You-Zhi Song Yan Yan Ze-Lin Qiu Yu-Jie Shen Han-Ying Li Bao-Ku Zhu Key Laboratory of Macromolecular Synthesis and Functionalization(Ministry of Education) Department of Polymer Science and EngineeringZhejiang UniversityHangzhou 310027ZhejiangChina Institute of Nuclear and New Energy Technology Tsinghua UniversityBeijing 100084China

Rechargeable lithium metal batteries(LMBs)have gained much attention ***,the short lifespan and safety issues restrict their commercial *** we report a novel gel polymer electrolyte(GPE)based on lithiated poly(vinyl chloride-r-acrylic acid)(PVCAALi)to realize dendritesuppressing and long-term stable lithium metal *** chains ensure the quick gelation process and high electrolyte uptake,and lithiated PAA segments enable the increase of mechanical strength,acceleration of lithium-ion transmission and improvement of interfacial *** GPE showed much higher mechanical strength compared with other free-standing GPEs in previous *** displays a superior ionic conductivity of 1.50 m S cm^(-1) and a high lithium-ion transference number of 0.59 at room ***,the lithiated GPE exhibits excellent interfacial compatibility with lithium metal *** symmetrical cells with PVCAALi GPE yield low hysteresis of 50 m V over1000 h at 1.0 m A cm^(-2).And the possible mechanism of the lithiated GPE with improved lithium-ion transfer and interfacial property was ***,both the Li4Ti5O12/Li and lithium-sulfur(Li-S)cells assembled with PVCAALi GPE show outstanding electrochemical performance,retaining high discharge capacities of 133.8 m Ah g^(-1) and 603.8 m Ah g^(-1) over 200 cycles,*** work proves excellent application potential of the highly effective and low-cost PVCAALi GPE in safe and long-life LMBs.

关键词： Lithiation Gel polymer electrolyte Lithium dendrite Safety Lithium metal battery

来源：评论

学校读者我要写书评

暂无评论

FeNi@CNS nanocomposite as an efficient electrochemical catalyst for N_(2)-to-NH_(3) conversion under ambient conditions

引用

Journal of Materials science & Technology 2022年第8期103卷 59-66页

作者： Tayiba Ilyas Fazal Raziq Nasir Ilyas Liuxin Yang Sharafat Ali Amir Zada Syedul Hasnain Bakhtiar Yong Wang Huahai Shen Liang Qiao School of Physics University of Electronic Science and Technology of ChinaChengdu 610054China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 10084China Department of Chemistry Abdul Wali Khan University of MardanMardanKPK 23200Pakistan Laboratory of Living Materials at the State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Institute of Nuclear Physics and Chemistry Chinese Academy of Engineering PhysicsMianyang 621900China

The electrocatalytic nitrogen reduction reaction(NRR)has emerged as a promising renewable energy source and a feasible strategy as an alternative to Haber-Bosch ammonia(NH_(3))***,finding an efficient and cost-effective robust catalyst to activate and cleave the extremely strong triple bond in nitrogen(N_(2))for electrocatalytic NRR is still a ***,a FeNi@CNS nanocomposite as an efficient catalyst for N_(2) fixation under ambient conditions is *** FeNi@CNS nanocomposite was prepared by a simple water bath process and *** FeNi@CNS is demonstrated to be a highly efficient NRR catalyst,which exhibits better NRR performance with exceptional Faradaic efficiency of 9.83%and an NH_(3) yield of 16.52μg h^(−1) cm^(−2) in 0.1 M Na_(2)SO_(4) aqueous ***,high stability and reproducibility with consecutive 6 cycles for two hours are also demonstrated throughout the NRR electrocatalytic process for 12 ***,the FeNi@CNS catalyst encourages N_(2) adsorption and activation as well as effectively suppressing competitive ***,this earth-abundant FeNi@CNS catalyst with a subtle balance of activity and stability has excellent potential in NRR industrial applications.

关键词： Electrocatalytic nitrogen reduction Transition-metal alloy FeNi@CNS catalyst N_(2)fixation to NH_(3)

来源：评论

学校读者我要写书评

暂无评论

Pt_(1)/Ni_(6)Co_(1)layered double hydroxides/N-doped graphene for electrochemical non-enzymatic glucose sensing by synergistic enhancement of single atoms and doping

引用

Nano Research 2023年第1期16卷 318-324页

作者： Baojun Long Peiyu Cao Yuanmeng Zhao Qianqian Fu Yan Mo Yueming Zhai Juejing Liu Xingyi Lyu Tao Li Xiaofeng Guo Changsheng Shan Minghua Zeng Ministry-of-Education Key Laboratory for the Synthesis and Application of Organic Functional Molecules College of Chemistry and Chemical EngineeringHubei UniversityWuhan 430062China Key Laboratory for the Chemistry and Molecular Engineering of Medicinal Resources School of Chemistry and Pharmaceutical SciencesGuangxi Normal UniversityGuilin 541004China The Institute for Advanced Studies(IAS) Wuhan UniversityWuhan 430072China Material Science and Engineering Program Washington State UniversityPullmanWA 99164USA Department of Chemistry and Alexandra Navrotsky Institute for Experimental Thermodynamics Washington State UniversityPullmanWA 99164USA X-ray Science Division Argonne National LaboratoryArgonneIL 60439USA Department of Chemistry and Biochemistry Northern Illinois UniversityDeKalbIL 60115USA

The development of novel single-atom catalysts is important for highly efficient electrochemical catalysis and *** this work,a novel Pt single atoms(SAs)supported on Ni_(6)Co_(1)layered double hydroxides/nitrogen-doped graphene(Pt_(1)/Ni_(6)Co_(1)LDHs/NG)was constructed for electrochemical enzyme-free catalysis and sensing towards *** loading of Pt single atoms increases with doping of Co atoms that generate more anchoring sites for Pt *** resulting Pt_(1)/Ni_(6)Co_(1)LDHs/NG exhibits low oxidative potential of 0.440 V with high sensitivity of 273.78μA·mM^(−1)·cm^(−2)toward glucose,which are 85 mV lower and 15 times higher than those of Ni(OH)_(2),***_(1)/Ni_(6)Co_(1)LDHs/NG also shows excellent selectivity and great stability during 5-week *** and experimental results show that the boosted performance of Pt_(1)/Ni_(6)Co_(1)LDHs/NG originates from its stronger binding energy with glucose and the synergistic effect of Pt SAs,Co doping,and *** work provides a general strategy of designing highly active SACs for extending their application in electrochemical sensing.

关键词： single-atom catalysts electrochemical sensor layered double hydroxides nitrogen-doped graphene synergistic effect

来源：评论

学校读者我要写书评

暂无评论

Chemical and Microstructural Evaluation of Coatings for Yttrium Hydride Adjacent Materials

Chemical and Microstructural Evaluation of Coatings for Yttr...

引用

2024 nuclear and Emerging Technologies for Space, NETS 2024

作者： Shivprasad, A.P. Kohnert, C.A. Torrez, M.A. Tegtmeier, E. Emberley, C. Luther, E.P. Trellue, H.R. Materials Science and Technology Los Alamos National Laboratory Los AlamosNM United States Program Project Interface Los Alamos National Laboratory Los AlamosNM United States Sigma Division Los Alamos National Laboratory Los AlamosNM United States Nuclear Engineering and Nonproliferation Los Alamos National Laboratory Los AlamosNM United States

ISBN: (纸本)9780894487989

Yttrium hydride moderators enable more compact reactor designs for space nuclear applications. However, the high reactivity of yttrium hydride warrants investigation into barrier coatings to prevent chemical reactions between the hydride moderator and an adjacent material. The thermodynamics of coating-hydride systems were evaluated, and chemical interactions were explored through sintering of candidate coating materials with yttrium hydride. Resultant phases, microstructure, and chemical analyses were performed to determine viability of candidate coating materials. © 2024 AMERICAN nuclear SOCIETY. All rights reserved.

关键词： Moderators

来源：评论

学校读者我要写书评

暂无评论

Total conversion of centimeter-scale nickel foam into single atom electrocatalysts with highly selective CO_(2)electrocatalytic reduction in neutral electrolyte

引用

Nano Research 2023年第2期16卷 2003-2010页

作者： Qikui Fan Pengfei Gao Shan Ren Yunteng Qu Chuncai Kong Jian Yang Yuen Wu Ministry of Education Key Laboratory for Non-equilibrium Synthesis and Modulation of Condensed Matter Shaanxi Province Key Laboratory of Advanced Functional Materials and Mesoscopic PhysicsSchool of PhysicsXi’an Jiaotong UniversityXi’an 710049China Shenzhen Key Laboratory of Special Functional Materials Guangdong Research Center for Interfacial Engineering of Functional MaterialsCollege of Materials Science and EngineeringShenzhen UniversityShenzhen 518060China Northwest Institute of Nuclear Technology Xi’an 710024China Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123China State Key Laboratory of Photoelectric Technology and Functional Materials International Collaborative Center on Photoelectric Technology and Nano Functional MaterialsInstitute of Photonics and Photon-TechnologyNorthwest UniversityXi’an 710069China Department of Chemistry iChEM(Collaborative Innovation Center of Chemistry for Energy Materials)University of Science and Technology of ChinaHefei 230026China

To improve the atomic utilization of metals and reduce the cost of industrialization,the one-step total monoatomization of macroscopic bulk metals,as opposed to nanoscale metals,is *** this study,we used a thermal diffusion method to directly convert commercial centimeter-scale Ni foam to porous Ni single-atom-loaded carbon nanotubes(CNTs).As expected,owing to the coating of single-atom on porous,highly conductive CNT carriers,Ni single-atom electrocatalysts(Ni-SACs)exhibit extremely high activity and selectivity in CO_(2)electroreduction(CO_(2)RR),yielding a current density of>350 mA/cm^(2),a selectivity for CO of>91%under a flow cell configuration using a 1 M potassium chloride(KCl)*** on the superior activity of the Ni-SACs electrocatalyst,an integrated gas-phase electrochemical zero-gap reactor was introduced to generate a significant amount of CO current for potential practical *** overall current can be increased to 800 mA,while maintaining CO Faradaic efficiencies(FEs)at above 90%per unit *** findings and insights on the active site transformation mechanism for macroscopic bulk Ni foam conversion into single atoms can inform the design of highly active single-atom catalysts used in industrial CO_(2)RR systems.

关键词： Ni single atom electrocatalyst CO_(2)electroreduction to CO neutral electrolyte thermal diffusion

来源：评论

学校读者我要写书评

暂无评论

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案：

请选择收藏分类：

通借通还

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：