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2019 Transactions of the American nuclear Society, ANS 2019

作者： Albarqi, Mubarak Alsulami, Raed Graham, Joseph Nuclear Engineering Program Missouri University of Science and Technology 222 Fulton Hall 301 W. 14th St. RollaMO65409 United States Nuclear Sciences Research Institute King Abdulaziz City for Science and Technology Kingdom of Saudi Arabia P.O Box 6086 Riyadh11442 Saudi Arabia

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Concurrent operando neutron imaging and diffraction analysis revealing spatial lithiation phase evolution in an ultra-thick graphite electrode

arXiv

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arXiv 2024年

作者： Strobl, Markus Baur, Monica E. Samothraktis, Stavros Malamud, Florencia Zhang, Xiaolong Tung, Patrick K.M. Schmidt, Søren Woracek, R. Lee, J. Kiyanagi, Ryoji Kuhn, Luise Theil Segev, Inbal Gavish Ein-Eli, Yair PSI Center for Neutron and Muon Sciences Villigen5232 Switzerland Niels Bohr Institut University of Copenhagen Denmark Department of Energy Conversion and Storage Technical University of Denmark Kongens LyngbyDK-2800 Denmark Research Technology Services [ResTech UNSW Sydney Kensington2052 Australia DMSC European Spallation Source Lyngby Denmark European Spallation Source P.O. Box 176 LundS - 221 00 Sweden J-PARC Center Japan Atomic Energy Agency Tokai319-1195 Japan Soreq Nuclear Research Center [SNRC Yavne Israel Department of Material Science and Engineering Technion Israel Institute of Technology Haifa3200003 Israel Grand Technion Energy Program [GTEP Technion Haifa3200003 Israel Israel National Institute for Energy Storage [INIES Technion Haifa3200003 Israel

Energy efficient, safe and reliable Li-ion batteries (LIBs) are required for a wide range of applications. Charging capabilities of thick electrodes still holding their stored high-energy is a most desirable characteristic in future advanced LIBs. The introduction of ultra-thick graphite anode meets limitations in internal electrode transport properties, leading to Li-ion gradients with detrimental consequences for battery cell performance and lifetime. Yet, there is a lack of experimental tools capable of providing a complete view of local processes and evolving gradients within such thick electrodes. Here, we introduce a multi-modal operando measurement approach, enabling quantitative spatio-temporal observations of Li concentrations and intercalation phases in ultra-thick, graphite electrodes. Neutron imaging and diffraction concurrently provide correlated information from the macroscopic scale of the cell and electrode down to the crystallographic scale portraying the intercalation and deintercalation processes. In particular, the evolving formation of the solid electrolyte interphase (SEI), observation of gradients in total lithium content, as well as in the formation of ordered LixC6 phases and trapped lithium have been mapped throughout the first charge-discharge cycle of the cell. Different lithiation stages co-exist during charging and discharging of an ultra-thick composite graphite-based electrode;delayed lithiation and delithiation processes are observed at the central region of the electrode, while the SEI formation, potential plating and dead lithium are predominantly found closer to the interface with the separator. The study furthermore emphasizes the potential of the method to study Li ion diffusion and the kinetics of lithiation phase formation in advanced ultra-thick electrodes. Specifically, the relation of dead Li and SEI formation to the different Li phase stages can be mapped. Copyright © 2024, The Authors. All rights reserved.

关键词： Solid electrolytes

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Neural network coupled with MCNP for neutron depth profiling

Neural network coupled with MCNP for neutron depth profiling

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2019 Transactions of the American nuclear Society, ANS 2019

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Comparison between OSEM and FBP reconstruction algorithms for the qualitative and quantitative interpretation of brain DAT-SPECT using an anthropomorphic striatal phantom: implications for the practice

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Research on Biomedical engineering 2020年第1期36卷 77-88页

作者： Trevisan, Ana Carolina Raed, Michel David Tumas, Vitor Alexandre-Santos, Leonardo Pitella, Felipe Arriva Itikawa, Emerson Nobuyuki Silvah, Jose Henrique Kato, Mery Martinez, Edson Zangiacomi Achcar, Jorge Alberto Simões, Marcus Vinícius Wichert-Ana, Lauro Interunits Post-Graduation Program on Bioengineering. São Carlos School of Engineering University of São Paulo Bandeirantes 3900 São Carlos14048-900 Brazil Section of Nuclear Medicine Image Science and Medical Physics Center Department of Internal Medicine University of São Paulo Ribeirão PretoSP Brazil Department of Social Medicine University of São Paulo Ribeirão PretoSP Brazil Department of Neuroscience and Behavioral Sciences. Ribeirão Preto Medical School University of São Paulo Ribeirão PretoSP Brazil

Purpose: The aim of this study was to evaluate the effect of ordered subsets maximization expectation (OSEM) and filtered backprojection (FBP) reconstruction algorithms for the qualitative interpretation of DAT-SPECT. Methods: Data were acquired using an anthropomorphic striatal phantom and a gamma camera (SPECT/CT). Images were reconstructed using different values of the covariates applied in the OSEM and FBP algorithms (iteration, subsets, order, and cut-off frequency). Image quality was compared according to each set of covariates used in the reconstruction and extracted quantitative parameters of the image quality, such as C, CV RCR, and RSR, as well as the angular coefficients of the edges in regions of interest. Results: Variations in the order from 0 to 10 do not influence the image if a trustworthy cut-off frequency range for FBP (0.9 to 1.6) and OSEM (1.2 to 1.5) are used. For OSEM, the iteration value and the number of subsets that guarantee better quality were those suggested by the developer of the algorithm used (3i8s). Conclusion: For a quality image, it is necessary to use the range of values found for the covariables order and cut-off frequency of the Butterworth filter in the FBP and OSEM reconstruction. OSEM reconstruction shows superiority in the images compared with FBP when the recommended three iterations and eight subsets are used. In the quantitative analyses, the evaluation showed that increasing the number of updates while allowing a better distinction of certain areas, culminates with a degradation image, making it inappropriate for clinical. © 2020, Sociedade Brasileira de Engenharia Biomedica.

关键词： Phantoms

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Efficiency optimization of a positron moderator foil

Efficiency optimization of a positron moderator foil

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2019 Transactions of the American nuclear Society, ANS 2019

作者： Alsulami, Raed Albarqi, Mubarak Jaradat, S.Q. Graham, Joseph Usman, Shoaib Nuclear Engineering Program Missouri University of Science and Technology 222 Fulton Hall 301 W. 14th St. RollaMO65409 United States Nuclear Science Research Institute King Abdulaziz City for Science and Technology Kingdom of Saudi Arabia P.OBox 6086 Riyadh11442 Saudi Arabia Higher Colleges of Technology Abu Dhabi United Arab Emirates

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Tuning the Magnetization of Manganese (II) Carbonate by Intracrystalline Amino Acids

arXiv

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arXiv 2022年

作者： Lang, Arad Polishchuk, Iryna Confalonieri, Giorgia Dejoie, Catherine Maniv, Ariel Potashnikov, Daniel Caspi, El'Ad N. Pokroy, Boaz Department of Materials Science and Engineering The Russell Berrie Nanotechnology Institute Technion-Israel Institute of Technology Haifa32000 Israel ESRF The European Synchrotron Radiation Facility CS 40220 Grenoble Cedex 938043 France Physics Department Nuclear Research Centre Negev P.O. Box 9001 Beer-Sheva84190 Israel Israel Atomic Energy Commission P.O. Box 7061 Tel-Aviv61070 Israel The Nancy and Stephen Grand Technion Energy Program Technion-Israel Institute of Technology Haifa3200003 Israel

Incorporation of organic molecules into the lattice of inorganic crystalline hosts is a common phenomenon in biomineralization, and has been shown to alter various properties of the crystalline host. Taking this phenomenon as our source of inspiration, we show herein that incorporation of specific single amino acids into the lattice of manganese (II) carbonate strongly alters its inherent magnetic properties. At room temperature, the magnetic susceptibility of the amino-acid-incorporating paramagnetic MnCO3decreases, following a simple rule of mixtures. When cooled below the Néel temperature, however, the opposite trend is observed, namely an increase in magnetic susceptibility measured in a high magnetic field. Such an increase, accompanied by a drastic change in the Néel phase transformation temperature, results from a decrease in MnCO3orbital overlapping and the weakening of superexchange interactions. To our knowledge, this is the first time that the magnetic properties of a host crystal have been tuned via the incorporation of amino acids. © 2022, CC BY-SA.

关键词： Amino acids

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Joint Observation of the Galactic Center with MAGIC and CTA-LST-1 38

Joint Observation of the Galactic Center with MAGIC and CTA-...

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38th International Cosmic Ray Conference, ICRC 2023

作者： Abe, Shotaro Berti, Alessio Di Pierro, Federico López-Coto, Rubén Moralejo, Abelardo Ohtani, Yoshiki Sitarek, Julian Strzys, Marcel Suda, Yusuke Vovk, Ievgen Abe, H. Abe, K. Abe, S. Abhir, J. Acciari, V.A. Aguasca-Cabot, A. Agudo, I. Alvarez Crespo, N. Aniello, T. Ansoldi, S. Antonelli, L.A. Aramo, C. Arbet-Engels, A. Cornelia, A. Artero, M. Asano, K. Aubert, P. Baack, D. Babić, A. Baktash, A. Bamba, A. Baquero Larriva, A. Baroncelli, L. Barres de Almeida, U. Barrio, J.A. Batkovic, I. Baxter, J. Becerra González, J. Bednarek, W. Bernardini, E. Bernardos, M.I. Bernete Medrano, J. Berti, A. Besenrieder, J. Bhattacharjee, P. Biederbeck, N. Bigongiari, C. Biland, A. Bissaldi, E. Blanch, O. Bonnoli, G. Bordas, P. Bošnjak, Ž. Bulgarelli, A. Burelli, I. Burmistrov, L. Buscemi, M. Busetto, G. Campoy-Ordaz, A. Cardillo, M. Caroff, S. Carosi, A. Carosi, R. Carrasco, M.S. Carretero-Castrillo, M. Cassol, F. Castro-Tirado, A.J. Cauz, D. Cerasole, D. Ceribella, G. Chai, Y. Cheng, K. Chiavassa, A. Chikawa, M. Chilingarian, A. Chytka, L. Cifuentes, A. Cikota, S. Colombo, E. Contreras, J.L. Cortina, J. Costantini, H. Covino, S. D’Amico, G. Dalchenko, M. D’Elia, V. Da Vela, P. Dazzi, F. De Angelis, A. de Bony de Lavergne, M. De Lotto, B. De Lucia, M. de Menezes, R. Del Peral, L. Deleglise, G. Delfino, M. Delgado, C. Delgado Mengual, J. della Volpe, D. Dellaiera, M. Del Popolo, A. Depaoli, D. Di Piano, A. Di Pierro, F. Di Pilato, A. Di Tria, R. Di Venere, L. Díaz, C. Dominik, R.M. Dominis Prester, D. Donini, A. Dorner, D. Doro, M. Eisenberger, L. Elsässer, D. Emery, G. Escudero, J. Fallah Ramazani, V. Fariña, L. Fattorini, A. Ferrara, G. Ferrarotto, F. Fiasson, A. Foffano, L. Font, L. Freixas Coromina, L. Fröse, S. Fukami, S. Fukazawa, Y. Garcia, E. Garcia López, R. Garczarczyk, M. Gasbarra, C. Gasparrini, D. Gasparyan, S. Gaug, M. Geyer, D. Giesbrecht Paiva, J. Giglietto, N. Giordano, F. Gliwny, P. Godinovic, N. Grau, R. Green, J. Green, D. Gunji, S. Günther, P. Hackfeld, J. Hadasch, D. Hahn, A. Institute for Cosmic Ray Research Kashiwa-no-ha 5-1-5 Kashiwa-shi Chiba Japan Max-Planck-Institut für Physik Föhringer Ring 6 München80805 Germany INFN Sezione di Torino Via P. Giuria 1 Torino10125 Italy Instituto de Astrofísica de Andalucía-CSIC Glorieta de la Astronomía s/n Granada18008 Spain The Barcelona Institute of Science and Technology Campus UAB Bellaterra Barcelona08193 Spain Faculty of Physics and Applied Informatics University of Lodz ul. Pomorska 149-153 Lodz90-236 Poland Physics Program Graduate School of Advanced Science and Engineering Hiroshima University Hiroshima739-8526 Japan Institute for Cosmic Ray Research University of Tokyo Japan Department of Physics Tokai University Japan ETH Zürich Switzerland Instituto de Astrofísica de Canarias Departamento de Astrofísica Universidad de La Laguna Spain Departament de Física Quàntica i Astrofísica Institut de Ciències del Cosmos Universitat de Barcelona IEEC-UB Spain EMFTEL department IPARCOS Universidad Complutense de Madrid Spain Italy INFN Sezione di Trieste Università degli Studi di Udine Italy Italy INAF Osservatorio Astronomico di Roma Italy INFN Sezione di Napoli Italy INFN Sezione di Padova Università degli Studi di Padova Italy LAPP Univ. Grenoble Alpes Univ. Savoie Mont Blanc CNRS-IN2P3 Annecy France Department of Physics TU Dortmund University Germany Croatia Universität Hamburg Institut für Experimentalphysik Germany Graduate School of Science University of Tokyo Japan Universidad del Azuay Ecuador INAF Osservatorio di Astrofisica e Scienza dello spazio di Bologna Italy Centro Brasileiro de Pesquisas Físicas Brazil CIEMAT Spain INFN Sezione di Bari Politecnico di Bari Italy INAF Osservatorio Astronomico di Brera Italy University of Geneva Département de physique nucléaire et corpusculaire Switzerland INFN Sezione di Catania Italy Departament de Física CERES-IEEC Universitat Autónoma de Barcelona Spain Italy Università di Pisa INFN Pisa Italy Aix Mars

MAGIC is a system of two Imaging Atmospheric Cherenkov Telescopes (IACTs), designed to detect very-high-energy gamma rays, and is operating in stereoscopic mode since 2009 at the Observatorio del Roque de Los Muchachos in La Palma, Spain. In 2018, the prototype IACT of the Large-Sized Telescope (LST-1) for the Cherenkov Telescope Array, a next-generation ground-based gamma-ray observatory, was inaugurated at the same site, at a distance of approximately 100 meters from the MAGIC telescopes. Using joint observations between MAGIC and LST-1, we developed a dedicated analysis pipeline and established the threefold telescope system via software, achieving the highest sensitivity in the northern hemisphere. Based on this enhanced performance, MAGIC and LST-1 have been jointly and regularly observing the Galactic Center, a region of paramount importance and complexity for IACTs. In particular, the gamma-ray emission from the dynamical center of the Milky Way is under debate. Although previous measurements suggested that a supermassive black hole Sagittarius A* plays a primary role, its radiation mechanism remains unclear, mainly due to limited angular resolution and sensitivity. The enhanced sensitivity in our novel approach is thus expected to provide new insights into the question. We here present the current status of the data analysis for the Galactic Center joint MAGIC and LST-1 observations. © Copyright owned by the author(s) under the terms of the Creative Commons.

关键词： Cosmology

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Malware detection in critical infrastructures using the electromagnetic emissions of PLCs

Malware detection in critical infrastructures using the elec...

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2019 Transactions of the American nuclear Society, ANS 2019

作者： Kolias, Constantinos Borrelli, R.A. Barbara, Daniel Stavrou, Angelos Computer Science Department University of Idaho 1776 Science Center Drive Idaho FallsID United States Nuclear Engineering Program University of Idaho CAES 995 MK Simpson Boulevard Idaho FallsID United States Computer Science Department George Mason University 4400 University Drive FairfaxVA United States

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Thermodynamic modeling of the LiCl-KCl-LaCl 3 system with Bayesian model selection and uncertainty quantification

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Journal of Molecular Liquids 2025年 432卷

作者： Rushi Gong Shun-Li Shang Vitaliy G. Goncharov Cillian Cockrell Kostya Trachenko Paul A. Bingham Xiaofeng Guo Zi-Kui Liu Department of Materials Science and Engineering The Pennsylvania State University University Park PA 16802 United States Department of Chemistry Washington State University Pullman Washington 99164 United States Materials Science and Engineering Program Washington State University Pullman Washington 99164 United States Nuclear Futures Institute Bangor University Bangor LL57 1UT United Kingdom School of Physical and Chemical Sciences Queen Mary University of London Mile End Road London E1 4NS United Kingdom Materials and Engineering Research Institute Sheffield Hallam University Sheffield S1 1WB United Kingdom

Chloride molten salts are increasingly used in pyroprocessing techniques for the separation of lanthanides. Understanding their thermodynamic properties is essential for predicting their critical characteristics and optimizing the separation process. Various thermodynamic models, including the associate model, the two-sublattice ionic model, and the modified quasichemical model with quadruplet approximation (MQMQA), have been utilized to capture the complexity of molten salts. In the present work, the Bayes factor is used to guide the model selection process for the thermodynamic modeling of the KCl-LaCl 3 system and provide a statistical comparison of different models. The results indicate that the MQMQA model is the most favorable based on the available data. The LiCl-KCl-LaCl 3 system is further modeled with uncertainty quantification (UQ) using the MQMQA model. The thermodynamic properties of compounds in KCl-LaCl 3 are predicted by the quasiharmonic approach in terms of first-principles phonon calculations as a function of temperature. The calculated phase stability shows excellent agreement with experimental data, indicating that an appropriate thermodynamic model is important for accurately predicting the critical characteristics of complex molten salts.

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Development of an advanced SiPM camera for the Large Size Telescope of the Cherenkov Telescope Array Observatory 37

Development of an advanced SiPM camera for the Large Size Te...

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37th International Cosmic Ray Conference, ICRC 2021

作者： Bellato, M. Bergnoli, A. Bernasconi, E. Biland, A. Charbon, E. Corti, D. Gascón, D. Gómez, S. Ziȩtara, K. Abe, H. Aguasca, A. Agudo, I. Antonelli, L.A. Aramo, C. Armstrong, T. Artero, M. Asano, K. Ashkar, H. Aubert, P. Baktash, A. Bamba, A. Baquero Larriva, A. Baroncelli, L. Barres de Almeida, U. Barrio, J.A. Batkovic, I. Becerra González, J. Bernardos, M.I. Berti, A. Biederbeck, N. Bigongiari, C. Blanch, O. Bonnoli, G. Bordas, P. Bose, D. Bulgarelli, A. Burelli, I. Buscemi, M. Cardillo, M. Caroff, S. Carosi, A. Cassol, F. Cerruti, M. Chai, Y. Cheng, K. Chikawa, M. Chytka, L. Contreras, J.L. Cortina, J. Costantini, H. Dalchenko, M. De Angelis, A. de Bony de Lavergne, M. Deleglise, G. Delgado, C. Delgado Mengual, J. della Volpe, D. Depaoli, D. Di Pierro, F. Di Venere, L. Díaz, C. Dominik, R.M. Dominis Prester, D. Donini, A. Dorner, D. Doro, M. Elsässer, D. Emery, G. Escudero, J. Fiasson, A. Foffano, L. Fonseca, M.V. Freixas Coromina, L. Fukami, S. Fukazawa, Y. Garcia, E. Garcia López, R. Giglietto, N. Giordano, F. Gliwny, P. Godinovic, N. Green, D. Grespan, P. Gunji, S. Hackfeld, J. Hadasch, D. Hahn, A. Hassan, T. Hayashi, K. Heckmann, L. Heller, M. Herrera Llorente, J. Hirotani, K. Hoffmann, D. Horns, D. Houles, J. Hrabovsky, M. Hrupec, D. Hui, D. Hütten, M. Inada, T. Inome, Y. Iori, M. Ishio, K. Iwamura, Y. Jacquemont, M. Jimenez Martinez, I. Jouvin, L. Jurysek, J. Kagaya, M. Karas, V. Katagiri, H. Kataoka, J. Kerszberg, D. Kobayashi, Y. Kong, A. Kubo, H. Kushida, J. Lamanna, G. Lamastra, A. Le Flour, T. Longo, F. López-Coto, R. López-Moya, M. López-Oramas, A. Luque-Escamilla, P.L. Majumdar, P. Makariev, M. Mandat, D. Manganaro, M. Mannheim, K. Mariotti, M. Marquez, P. Marsella, G. Martí, J. Martinez, O. Martínez, G. Martínez, M. Marusevec, P. Mas, A. Maurin, G. Mazin, D. Mestre Guillen, E. Micanovic, S. Miceli, D. Miener, T. Miranda, J.M. Miranda, L.D.M. Mirzoyan, R. Mizuno, T. Molina, E. Montaruli, T. Monteiro, I. AQUA EPFL Neuchâtel Switzerland ETH Zurich Institute for Particle Physics Otto-Stern-Weg 5 Zurich8093 Switzerland Astronomical Observatory Jagiellonian University ul. Orla 171 Kraków30-244 Poland Institute for Cosmic Ray Research University of Tokyo Japan Departament de Física Quàntica i Astrofísica Institut de Ciències del Cosmos Universitat de Barcelona IEEC-UB Martí i Franquès 1 Barcelona08028 Spain Instituto de Astrofísica de Andalucía CSIC Spain INAF Osservatorio Astronomico di Roma Italy INFN Sezione di Napoli Italy Aix Marseille Univ CNRS IN2P3 CPPM Marseille France Barcelona Institute of Science and Technology Spain IRFU CEA Université Paris-Saclay France LAPP Univ. Grenoble Alpes Univ. Savoie Mont Blanc CNRS IN2P3 Annecy France Universität Hamburg Institut für Experimentalphysik Germany Graduate School of Science University of Tokyo Japan EMFTEL department IPARCOS Universidad Complutense de Madrid Spain INAF Osservatorio di Astrofisica e Scienza dello spazio di Bologna Centro Brasileiro de Pesquisas Físicas Brazil INFN Sezione di Padova Università degli Studi di Padova Via Marzolo 8 Padova35131 Italy Instituto de Astrofísica de Canarias Departamento de Astrofísica Universidad de La Laguna Spain Max-Planck-Institut für Physik Germany Department of Physics TU Dortmund University Germany Saha Institute of Nuclear Physics India INFN Sezione di Trieste Università degli Studi di Udine Italy INFN Sezione di Catania Italy University of Geneva Département de Physique Nucléaire et Corpusculaire 24 Quai Ernest Ansermet GenèveCH-1211 Switzerland Palacky University Olomouc Faculty of Science Czech Republic CIEMAT Port d’Informació Científica INFN Sezione di Torino via P. Giuria 1 Torino10125 Italy Dipartimento di Fisica Universitá degli Studi di Torino via P. Giuria 1 Torino10125 Italy INFN Sezione di Bari Università di Bari University of Rijeka Department of Physics Institute for Theoretical Physics and Astrophysics Universitä

Silicon photomultipliers (SiPMs) have become the baseline choice for cameras of the small-sized telescopes (SSTs) of the Cherenkov Telescope Array (CTA). On the other hand, SiPMs are relatively new to the field and covering large surfaces and operating at high data rates still are challenges to outperform photomultipliers (PMTs). The higher sensitivity in the near infra-red and longer signals compared to PMTs result in higher night sky background rate for SiPMs. However, the robustness of the SiPMs represents a unique opportunity to ensure long-term operation with low maintenance and better duty cycle than PMTs. The proposed camera for large size telescopes will feature 0.05◦ pixels, low power and fast front-end electronics and a fully digital readout. In this work, we present the status of dedicated simulations and data analysis for the performance estimation. The design features and the different strategies identified, so far, to tackle the demanding requirements and the improved performance are described. © Copyright owned by the author(s) under the terms of the Creative Commons.

关键词： Photomultipliers

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