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2024 IEEE International Conference on Computational Electromagnetics, ICCEM 2024

作者： Tserkezis, C. POLIMA-Center For Polariton-driven Light-Matter Interactions University of Southern Denmark Campusvej 55 Odense MDK-5230 Denmark

ISBN: (纸本)9798350383317

The surface-response formalism (SRF) embodied by the Feibelman d parameters offers a promising route for bridging the gap between the classical and quantum worlds in plasmonics. Without radically affecting the description of the system (typically one or more few-nm scatterers) in terms of Maxwell's equations and the bulk permittivity, SRF introduces effects of atomistic/solid-state origin via modification of the boundary conditions at the surface of the scatterer, and the inclusion of quantum effects through surface polarisation and current densities. Here we discuss the influence of these corrections on both the far-field spectra of the scatterers and on their coupling to quantum emitters. © 2024 IEEE.

关键词： Maxwell equations

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Surface-Response Formalism for light–matter interactions in Mesoscopic Plasmonics

Surface-Response Formalism for Light–Matter Interactions in...

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IEEE International Conference on Computational Electromagnetics (ICCEM)

作者： C. Tserkezis POLIMA-Center for Polariton-driven Light-Matter Interactions University of Southern Denmark Odense M Denmark

ISBN: (数字)9798350383317

ISBN: (纸本)9798350383324

The surface-response formalism (SRF) embodied by the Feibelman $d$ parameters offers a promising route for bridging the gap between the classical and quantum worlds in plasmonics. Without radically affecting the description of the system (typically one or more few-nm scatterers) in terms of Maxwell's equations and the bulk permittivity, SRF introduces effects of atomistic/solid-state origin via modification of the boundary conditions at the surface of the scatterer, and the inclusion of quantum effects through surface polarisation and current densities. Here we discuss the influence of these corrections on both the far-field spectra of the scatterers and on their coupling to quantum emitters.

关键词： Couplings Atomic measurements Plasmons Computational electromagnetics Boundary conditions Permittivity Maxwell equations

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Tunable nonlinear excitonic optical response in biased bilayer graphene

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Physical Review B 2024年第8期110卷 085433页

作者： M. F. C. Martins Quintela N. M. R. Peres T. Garm Pedersen Department of Physics and (INL) Av. Mestre José Veiga 4715-330 Braga Portugal Department of Materials and Production POLIMA–Center for Polariton-driven Light-Matter Interactions

Biased bilayer graphene (BBG) is an important system for studies of excitonic effects in graphene-based systems, with its easily tunable band gap. This band gap is governed by an external gate voltage, allowing one to tune the optical response of the system. In this paper, we study the excitonic linear and nonlinear optical responses of Bernal-stacked BBG as a function of the gate voltage, both for in-plane (IP) and out-of-plane (OOP) directions. Based on a semianalytical model of the electronic structure of BBG describing the influence of gate voltage on excitonic binding energies, we focus our discussion on both the IP and OOP excitonic responses. Both linear and second harmonic generation nonlinear responses are shown to be very sensitive to the gate voltage, as both the interband momentum matrix elements and the band gap of the system will vary greatly with bias potential.

关键词： Electrical conductivity Excitons Optical conductivity Optoelectronics Bilayer graphene

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Fourier analysis of near-field patterns generated by propagating polaritons

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Physical Review Applied 2024年第1期22卷 014076-014076页

作者： Minsoo Jang Sergey G. Menabde Fatemeh Kiani Jacob T. Heiden Vladimir A. Zenin N. Asger Mortensen Giulia Tagliabue Min Seok Jang School of Electrical Engineering Laboratory of Nanoscience for Energy Technologies (LNET) School of Engineering (STI) Center for Nano Optics POLIMA – Center for Polariton-driven Light-Matter Interactions Danish Institute for Advanced Study

Scattering-type scanning near-field optical microscope (s-SNOM) has become an essential tool to study polaritons—quasiparticles of light coupled to collective charge oscillations—via direct probing of their near field with a spatial resolution far beyond the diffraction limit. However, extraction of the polariton’s complex propagation constant from the near-field images requires subtle considerations that have not received the necessary attention so far. In this study, we discuss important yet overlooked aspects of the near-field analysis. First, we experimentally demonstrate that the sample orientation inside the s-SNOM may significantly affect the near-field interference pattern of mid-infrared polaritons, leading to an error in momentum measurement up to 7.7%, even for the modes with an effective index of 12.5. Second, we establish a methodology to correctly extract the polariton damping rate from the interference fringes depending on their origin—i.e., the s-SNOM nanotip or the material edge. Overall, our work provides a unified framework for the accurate extraction of the polariton momentum and damping from the near-field interference fringes.

关键词： Classical optics Nanophotonics Phonon polariton Surface & interfacial phenomena Nanotechnology Surfaces Scanning near-field optical microscopy

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Moiré excitons in biased twisted bilayer graphene under pressure

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Physical Review B 2024年第3期110卷 035405-035405页

作者： V. G. M. Duarte D. R. da Costa N. M. R. Peres L. K. Teles A. J. Chaves Departamento de Física Centro de Física das (INL) Avenida Mestre José Veiga 4715-330 Braga Portugal POLIMA—Center for Polariton-driven Light-Matter Interactions

Using the tight-binding model, we report a gap opening in the energy spectrum of a twisted bilayer graphene under the application of pressure, that can be further amplified by the presence of a perpendicular bias voltage. The valley edges are located along the K−Γ path of the superlattice Brillouin zone, with the band gap reaching values up to 200 meV in the single-particle picture. Employing the formalism of the semiconductor Bloch equations, we observe an enhancement of the band gap due to the electron-electron interaction, with a renormalization of the band gap of about 160 meV. From the solution of the corresponding Bethe-Salpeter equation, we show that this system supports highly anisotropic bright excitons whose electrons and holes are strongly hybridized between the adjacent layers.

关键词： Excitons Bilayer graphene Twisted heterostructures Bethe-Salpeter equation Random phase approximation Tight-binding model

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Organic-inorganic polaritonics: Linking Frenkel and Wannier-Mott excitons

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Physical Review B 2025年第20期111卷 L201404-L201404页

作者： V. G. M. Duarte A. J. Chaves N. M. R. Peres Department of Physics Aeronautics Institute of Technology 12228-900 São José dos Campos SP Brazil International Iberian Nanotechnology Laboratory (INL) Avenida Mestre José Veiga P-4715-330 Braga Portugal POLIMA—Center for Polariton-driven Light–Matter Interactions University of Southern Denmark Campusvej 55 DK-5230 Odense M Denmark Centro de Física (CF-UM-UP) and Departamento de Física Universidade do Minho P-4710-057 Braga Portugal

In recent years, organic materials have emerged as promising candidates for a variety of light-harvesting applications ranging from the infrared to the visible regions of the electromagnetic spectrum. Their enhanced excitonic binding energies and large transition dipole moments enable strong coupling with light, with some systems already reaching the ultrastrong-coupling regime. In contrast, a wide range of two-dimensional (2D) materials has been extensively explored in the literature, exhibiting high exciton stability and strong electron-hole coupling due to reduced screening effects. In this Letter, we present a microscopic model describing the interaction of 2D materials and organic molecular aggregates in an optical cavity. We predict the formation of a hybrid Wannier-Mott-Frenkel exciton polariton with an enhanced Rabi splitting, exceeding that of the pure organic cavity by several tens of meV. To elucidate this phenomenon, we examine a cavity with 2D tungsten sulfide and a cyanine dye, where this enhancement corresponds to a 5% increase relative to the organic cavity. The complementary characteristics of Wannier-Mott and Frenkel excitons enable the formation of tunable polariton states that merge into a single hybrid state as a function of detuning, allowing for dual Rabi splitting mechanisms. This provides a promising platform for exploring quantum optical phenomena in both the strong- and ultrastrong-coupling regimes.

关键词： Organic-inorganic materials

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Quantum-informed plasmonics for strong coupling: the role of electron spill-out

arXiv

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arXiv 2023年

作者： Bundgaard, Ida Juliane Hansen, Christian Nicolaisen Stamatopoulou, P. Elli Tserkezis, Christos POLIMA Center for Polariton-driven Light-Matter Interactions University of Southern Denmark Campusvej 55 Odense MDK-5230 Denmark

The effect of nonlocality on the optical response of metals lies at the forefront of research in nanoscale physics and, in particular, quantum plasmonics. In alkali metals, nonlocality manifests predominantly as electron density spill-out at the metal boundary, and as surface-enabled Landau damping. For an accurate description of plasmonic modes, these effects need be taken into account in the theoretical modelling of the material. The resulting modal frequency shifts and broadening become particularly relevant when dealing with the strong interaction between plasmons and excitons, where hybrid modes emerge and the way they are affected can reflect modifications of the coupling strength. Both nonlocal phenomena can be incorporated in the classical local theory by applying a surface-response formalism embodied by the Feibelman parameters. Here, we implement surface-response corrections in Mie theory to study the optical response of spherical plasmonic–excitonic composites in core–shell configurations. We investigate sodium, a jellium metal dominated by spill-out, for which it has been anticipated that nonlocal corrections should lead to an observable change in the coupling strength, appearing as a modification of the width of the mode splitting. We show that, contrary to expectations, the influence of nonlocality on the anticrossing is minimal, thus validating the accuracy of the local response approximation in strong-coupling photonics. © 2023, CC BY.

关键词： Hazardous materials spills

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Mechanical Su-Schrieffer-Heeger quasicrystal: Topology, localization, and mobility edge

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Physical Review B 2024年第19期109卷 195427-195427页

作者： D. A. Miranda T. V. C. Antão N. M. R Peres Centro de Física (CF-UM-UP) and Departamento de Física Department of Applied Physics (INL) Avenida Mestre José Veiga 4715-330 Braga Portugal POLIMA–Center for Polariton-driven Light-Matter Interactions

In this paper we discuss the topological transition between trivial and nontrivial phases of a quasiperiodic (Aubry-André like) mechanical Su-Schrieffer-Heeger model. We find that there exists a nontrivial boundary separating the two topological phases, and an analytical expression for this boundary is found. We discuss the localization of the vibrational modes using the calculation of the inverse participation ratio and access the localization nature of the states of the system. We find three different regimes: extended, localized, and critical, depending on the intensity of the Aubry-André spring. We further study the energy-dependent mobility edge (ME) separating localized from extended eigenstates and find its analytical expression for both commensurate and incommensurate modulation wavelengths, thus enlarging the library of models possessing analytical expressions for the ME. Our results extend previous results for the theory of fermionic topological insulators and localization theory in quantum matter to the classical realm.

关键词： Localization Topological materials Hybrid model Su-Schrieffer-Heeger model Topology

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A Dedicated Modelling Scheme for Nonclassical Optical Response from the Nanosphere-on-Mirror Structure

arXiv

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arXiv 2023年

作者： Yan, Xiaotian Tserkezis, Christos Mortensen, N. Asger Vandenbosch, Guy A.E. Zheng, Xuezhi KU Leuven LeuvenB-3001 Belgium POLIMA Center for Polariton-driven Light-Matter Interactions University of Southern Denmark Odense5230 Denmark

Within the framework of the T-matrix method, we present a modeling tool that predicts the optical response from the Nanosphere-on-Mirror (NSoM) construct. The nonclassical effects in metals are accounted for by the nonlocal hydrodynamic Drude model (NLHDM) or the surface response model (SRM). Two essential elements in the T-matrix method, i.e., the T-matrix of the sphere and the R matrix accounting for the effects of the mirror, have been fully upgraded to include longitudinal waves for the NLHDM and the augmented interface conditions for the SRM. The proposed tool is quantitatively validated both in the near and the far field by an in-house developed BEM solver for the NLHDM where the gap between the sphere and the mirror is as small as 1 nm. Two physical checks are performed, where the results from the classical local response model are compared with the ones from the NLHDM and the SRM. The observed shifts in resonances and reduced field enhancements in the gap region agree well with previous physical findings. The proposed tool may not only serve as a reference tool for other numerical methods, but also provides an ideal platform for investigating nonclassical optical processes in the NSoM, hence paving a semi-analytical way to understand the extreme optics at very small scales. © 2023, CC BY.

关键词： Mirrors

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Coexistence of one-dimensional and two-dimensional topology and genesis of Dirac cones in the chiral Aubry-André model

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Physical Review B 2024年第19期109卷 195436-195436页

作者： T. V. C. Antão D. A. Miranda N. M. R. Peres Department of Applied Physics Centro de Física das Universidade do Minho e do Porto (CFUMUP) e Departamento de Física (INL) Av Mestre José Veiga 4715-330 Braga Portugal POLIMA - Center for Polariton-driven Light-Matter Interactions

We construct a one-dimensional (1D) topological SSH-like model with chiral symmetry and a superimposed hopping modulation, which we call the chiral Aubry-André model. We show that its topological properties can be described in terms of a pair (C,W) of a two-dimensional (2D) Chern number C, stemming from a superspace description of the model, and a 1D winding number W, originating in its chiral symmetric nature. Thus, we showcase the explicit coexistence of 1D and 2D topology in a model composed of a single 1D chain. We detail the superspace description by showcasing how our model can be mapped to a Harper-Hofstadter model, familiar from the description of the integer quantum Hall effect, and analyze the vanishing field limit analytically. An extension of the method used for vanishing fields is provided in order to handle any finite fields, corresponding to hopping modulations both commensurate and incommensurate with the lattice. In addition, this formalism allows us to obtain certain features of the 2D superspace model, such as its number of massless Dirac nodes, purely in terms of topological quantities, computed without the need to go into momentum space.

关键词： Chern insulators Edge states Integer quantum Hall effect Landau levels Phononic crystals Topological insulators Waveguide arrays 1-dimensional systems 2-dimensional systems Quasicrystals Topological materials Su-Schrieffer-Heeger model Topological tools

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