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Cover Feature: Synthesis and Photophysical Properties of Hexabenzocoronene-Tetrabenzoporphyrin Architectures (Eur. J. Org. Chem. 40/2020)

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European Journal of Organic Chemistry 2020年第40期2020卷

作者： Michael Ruppel Lampros-Pascal Gazetas Dr. Dominik Lungerich Dr. Norbert Jux Department of Chemistry and Pharmacy & Interdisciplinary Center for Molecular Materials (ICMM) Friedrich-Alexander University Erlangen-Nuremberg Nikolaus-Fiebiger-Str. 10 91058 Erlangen Germany Institute for Basic Science (IBS) 50 Yonsei-ro Seodaemun-gu Center for Nanomedicine 03722 Seoul Republic of Korea Graduate Program of Nano Biomedical Engineering (NanoBME) Advanced Science Institute Yonsei University 03722 Seoul Republic of Korea

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Generation of terahertz transients from Co2Fe0.4Mn0.6Si-Heusler-alloy/normal-metal nanobilayers excited by femtosecond optical pulses

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Physical Review Research 2021年第4期3卷 043025-043025页

作者： Sarah Heidtfeld Roman Adam Takahide Kubota Koki Takanashi Derang Cao Carolin Schmitz-Antoniak Daniel E. Bürgler Fangzhou Wang Christian Greb Genyu Chen Ivan Komissarov Hilde Hardtdegen Martin Mikulics Roman Sobolewski Shigemasa Suga Claus M. Schneider Research Centre Jülich Peter Grünberg Institute 52425 Jülich Germany Faculty of Physics University of Duisburg-Essen 47048 Duisburg Germany Institute for Materials Research Tohoku University Sendai 980-8577 Japan Center for Spintronics Research Network Tohoku University Sendai 980-8577 Japan Center for Science and Innovation in Spintronics (Core Research Cluster) Tohoku University Sendai 980-8577 Japan College of Physics National Demonstration Center for Experimental Applied Physics Education Qingdao University Qingdao 266071 China Materials Science Graduate Program University of Rochester Rochester New York 14627 USA Laboratory for Laser Energetics University of Rochester Rochester New York 14623 USA Department of Electrical and Computer Engineering University of Rochester Rochester New York 14627 USA Belarusian State University of Informatics and Radioelectronics Minsk 220013 Belarus Research Centre Jülich Ernst Ruska Centre for Microscopy and Spectroscopy with Electrons 52425 Jülich Germany Department of Physics and Astronomy University of Rochester Rochester New York 14627 USA The Institute of Scientific and Industrial Research Osaka University Ibaraki Osaka 567-0047 Japan Department of Physics University of California Davis Davis California 95616 USA

We generated pulses of electromagnetic radiation in the terahertz (THz) frequency range by optical excitation of Co2Fe0.4Mn0.6Si (CFMS)/normal-metal (NM) bilayer structures. The CFMS is a Heusler alloy showing a band gap in one spin channel and is therefore a half metal. We compared the THz emission efficiency in a systematic manner for four different CFMS/NM bilayers, where NM was either Pt, Ta, Cr, or Al. Our measurements show that the THz intensity is highest for a Pt capping. We also demonstrate the tunability of the THz amplitude by varying the magnetic field for all four bilayers. We attribute the THz generation to the inverse spin Hall effect. In order to investigate the role of the interface in THz generation, we measured the spin mixing conductance for each CFMS/NM bilayer using a ferromagnetic resonance method. We found that the spin-orbit coupling cannot completely describe the THz generation in the bilayers and that the spin transmission efficiency of the CFMS/NM interface and the spin diffusion length, as well as the oxidation of the NM layer, play crucial roles in the THz emission process.

关键词： Inverse spin Hall effect Magnetism Spin injection Spin pumping Spintronics Ferromagnetic resonance Terahertz time-domain spectroscopy

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Magnetic Control of Soft Chiral Phonons in PbTe

arXiv

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arXiv 2021年

作者： Baydin, Andrey Hernandez, Felix G.G. Rodriguez-Vega, Martin Okazaki, Anderson K. Tay, Fuyang Timothy Noe, G. Katayama, Ikufumi Takeda, Jun Nojiri, Hiroyuki Rappl, Paulo H.O. Abramof, Eduardo Fiete, Gregory A. Kono, Junichiro Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Smalley-Curl Institute Rice University HoustonTX77005 United States Instituto de Física Universidade de São Paulo SP São Paulo05508-090 Brazil Theoretical Division Los Alamos National Laboratory Los AlamosNM87545 United States Laboratório Associado de Sensores e Materiais Instituto Nacional de Pesquisas Espaciais SP São José dos Campos12201-970 Brazil Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Physics Graduate School of Engineering Science Yokohama National University Yokohama240-8501 Japan Institute for Materials Research Tohoku University Sendai980-8577 Japan Department of Physics Northeastern University BostonMA02115 United States Department of Physics Massachusetts Institute of Technology CambridgeMA02139 United States Department of Physics and Astronomy Rice University HoustonTX77005 United States Department of Material Science and NanoEngineering Rice University HoustonTX77005 United States

PbTe crystals have a soft transverse optical phonon mode in the terahertz frequency range, which is known to efficiently decay into heat-carrying acoustic phonons, resulting in anomalously low thermal conductivity. Here, we studied this phonon via polarization-dependent terahertz spectroscopy. We observed softening of this mode with decreasing temperature, indicative of incipient ferroelectricity, which we explain through a model including strong anharmonicity with a quartic displacement term. In magnetic fields up to 25 T, the phonon mode splits into two modes with opposite handedness, exhibiting circular dichroism. Their frequencies display Zeeman splitting together with an overall diamagnetic shift with increasing magnetic field. Using a group-theoretical approach, we demonstrate that these observations are the result of magnetic field-induced morphic changes in the crystal symmetries through the Lorentz force exerted on the lattice ions. Thus, our study reveals a novel process of controlling phonon properties in a soft ionic lattice by a strong magnetic field. Copyright © 2021, The Authors. All rights reserved.

关键词： Magnetic fields

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Plasma-Derived Nanoclusters for Site-Specific Multimodality Photo/Magnetic Thrombus Theranostics

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Advanced Healthcare materials 2023年第28期12卷 e2301504页

作者： Liu, Chia-Hung Liu, Ming-Che Jheng, Pei-Ru Yu, Jiashing Fan, Yu-Jui Liang, Jia-Wei Hsiao, Yu-Cheng Chiang, Chih-Wei Bolouki, Nima Lee, Jyh-Wei Hsieh, Jang-Hsing Mansel, Bradley W Chen, Yan-Ting Nguyen, Hieu Trung Chuang, Er-Yuan Department of Urology School of Medicine College of Medicine Taipei Medical University 250 Wu-Hsing Street Taipei11031 Taiwan TMU Research Center of Urology and Kidney Taipei Medical University 250 Wu-Hsing Street Taipei11031 Taiwan Department of Urology Shuang Ho Hospital Taipei Medical University 291 Zhongzheng Road Zhonghe District New Taipei City23561 Taiwan Clinical Research Center Taipei Medical University Hospital Taipei11031 Taiwan School of Dental Technology College of Oral Medicine Taipei Medical University Taipei11031 Taiwan Graduate Institute of Biomedical Materials and Tissue Engineering International Ph.D. Program in Biomedical Engineering Graduate Institute of Biomedical Optomechatronics School of Biomedical Engineering Research Center of Biomedical Device Innovation Entrepreneurship Education Center College of Interdisciplinary Studies Taipei Medical University Taipei11031 Taiwan Department of Chemical Engineering College of Engineering National Taiwan University Taipei106 Taiwan Department of Orthopedics Taipei Medical University Taipei11031 Taiwan Department of Orthopedics Taipei Medical University Hospital Taipei11031 Taiwan Department of Physical Electronics Faculty of Science Masaryk University Brno60177 Czech Republic Department of Materials Engineering Ming Chi University of Technology New Taipei City24301 Taiwan Center for Plasma and Thin Film Technologies Ming Chi University of Technology New Taipei City24301 Taiwan National Synchrotron Radiation Research Center Hsinchu Science Park Hsinchu30076 Taiwan Department of Orthopedics and Trauma Faculty of Medicine University of Medicine and Pharmacy at Ho Chi Minh City Ho Chi Minh City700000 Viet Nam Cell Physiology and Molecular Image Research Center Taipei Medical University Wan Fang Hospital Taipei11696 Taiwan Precision Medicine and Translational Cancer Research Center Taipei Medical University Hospital Taipei11031 Taiwan

Traditional thrombolytic therapeutics for vascular blockage are affected by their limited penetration into thrombi, associated off-target side effects, and low bioavailability, leading to insufficient thrombolytic efficacy. It is hypothesized that these limitations can be overcome by the precisely controlled and targeted delivery of thrombolytic therapeutics. A theranostic platform is developed that is biocompatible, fluorescent, magnetic, and well-characterized, with multiple targeting modes. This multimodal theranostic system can be remotely visualized and magnetically guided toward thrombi, noninvasively irradiated by near-infrared (NIR) phototherapies, and remotely activated by actuated magnets for additional mechanical therapy. Magnetic guidance can also improve the penetration of nanomedicines into thrombi. In a mouse model of thrombosis, the thrombosis residues are reduced by ≈80% and with no risk of side effects or of secondary embolization. This strategy not only enables the progression of thrombolysis but also accelerates the lysis rate, thereby facilitating its prospective use in time-critical thrombolytic treatment. © 2023 Wiley-VCH GmbH.

关键词： Diseases

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UNDERWATER INSPECTION FOR WELDING AND OVERHAUL

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NAVAL ENGINEERS JOURNAL 1993年第5期105卷 37-42页

作者： MITTLEMAN, J SWAN, L John Mittleman:is a mechanical engineer at the Naval Surface Warfare Center Dahlgren Division Coastal Systems Station in Panama City Florida. His Primary Responsibilities are in the development of underwater nondestructive testing equipment for use by fleet divers and inspectors. He also performs research in the characterization of metal microstructure through ultrasonic scattering measurements. Mr. Mittleman received his BS from Cornell University in 1969 and science master's in ocean engineering from the Massachusetts Institute of Technology in 1970. His research currently supports doctoral studies with Iowa State University. Mr. Mittleman received the American Society of Naval Engineer's Solberg Award in 1981 for his contributions to underwater ship hull inspection. Mr. Mittleman is a member of ASNE ASNT ASTM IoD Sigma Xi Tau Beta Pi and Phi Kappa Phi. Lisa Swan:is a mechanical engineer at the Naval Surface Warfare Center in Panama City Florida. She is involved in nondestructive testing engineering primarily in the underwater arena. Ms. Swan holds a bachelor of science in materials engineering from North Carolina State University. She is a graduate of the Federal Women's Executive Leadership Program. Ms. Swan is a member of ASNT.

Significant progress has been made in making underwater ultrasonic thickness gauging and magnetic particle inspections available to the fleet. Under sponsorship from the Naval Sea Systems Command, Director of Ocean engineering, Underwater Ship Husbandry Division (NavSea 00C5), the Coastal Systems Station has developed complete hardware packages supporting these two nondestructive test methods, and has introduced them to military inspectors at a shore intermediate maintenance activity, a destroyer tender, and a naval shipyard. Performance trials conducted prior to taking the systems to the field have been accepted by NavSea, Ships' Concepts Group, materials Subgroup, Metals Division (NavSea 5142) as evidence that these inspections can reliably be performed underwater. Avenues for certifying specially trained divers and inspectors are being developed;for the first time the Navy will have all of the elements in place for underwater inspections satisfying the requirements of Mil-Std-271 (Requirements for Nondestructive Testing Methods) and the Naval Ships' Technical Manual Chapter 074. Underwater ultrasonic thickness gauging has also been slated for use in the fleet, as data from laboratory and field trials have consistently shown that reliable results can be obtained by a team comprising a certified topside inspector and a diver. In tests performed at the Ship Repair Facility (SRF), Yokosuka, underwater readings were compared to those taken in dry dock by SRF inspectors, and independently by contract inspectors. On the basis of approximately 800 locations, differences between the data sets were found to be randomly distributed, with a standard deviation on the order of 0.02''. This level of accuracy is largely sufficient to distinguish plate which will need replacement during overhaul, or plate which is thick enough to weld on.

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Correction: Shear-induced polydomain structures of nematic lyotropic chromonic liquid crystal disodium cromoglycate

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Soft matter 2021年第21期17卷 5444页

作者： Hend Baza Taras Turiv Bing-Xiang Li Ruipeng Li Benjamin M Yavitt Masafumi Fukuto Oleg D Lavrentovich Department of Physics Kent State University Kent OH 44242 USA. olavrent@kent.edu and Advanced Materials and Liquid Crystal Institute Kent State University Kent OH 44242 USA. Advanced Materials and Liquid Crystal Institute Kent State University Kent OH 44242 USA and Materials Science Graduate Program Kent State University Kent OH 44242 USA. National Synchrotron Light Source II Brookhaven National Laboratory Upton NY 11973 USA. National Synchrotron Light Source II Brookhaven National Laboratory Upton NY 11973 USA and Department of Materials Science and Chemical Engineering Stony Brook University Stony Brook NY 11794 USA. Department of Physics Kent State University Kent OH 44242 USA. olavrent@kent.edu and Advanced Materials and Liquid Crystal Institute Kent State University Kent OH 44242 USA and Materials Science Graduate Program Kent State University Kent OH 44242 USA.

Correction for 'Shear-induced polydomain structures of nematic lyotropic chromonic liquid crystal disodium cromoglycate' by Hend Baza et al., Soft Matter, 2020, 16, 8565-8576.

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Study of structural, electronic, optical and mechanical properties of K₂ScCuF₆ and K₂YCuF₆ perovskites via DFT calculations

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Results in Physics 2024年 62卷

作者： Amina Uzair, Muhammad Sohail Khan, Amir Quraishi, A.M. Almahri, Albandary Soliyeva, Mukhlisa Tirth, Vineet Algahtani, Ali Abdullah Mohammed, Rawaa M. Sarker, Mahidur R. Hadia, N.M.A. Zaman, Abid Department of Physics Bacha Khan University Charsadda Pakistan Department of Physics University of Peshawar KP Peshawar 25120 Pakistan Department of Energy Systems Research Ajou University Suwon 16499 South Korea Department of Electrical Engineering College of Engineering Qassim University Buraydah 51452 Saudi Arabia Department of Chemistry College of Science and Humanities in Prince Sattam Bin Abdulaziz University Al-Kharj 11942 Saudi Arabia Department of Physics and Teaching Methods Tashkent State Pedagogical University Tashkent Uzbekistan Mechanical Engineering Department College of Engineering King Khalid University Asir Abha 61421 Saudi Arabia Research Center for Advanced Materials Science (RCAMS) King Khalid University Asir Guraiger Abha 61413 Saudi Arabia Department of Physics Government Post Graduate College Karak 27200 Pakistan Ph.D in clinical microbiology College of Nursing Al-Mustaqbal University Iraq Institute of Visual Informatics Universiti Kebangsaan Malaysia Selangor Bangi 43600 Malaysia Universidad de Diseño Innovación y Tecnología UDIT Av. Alfonso XIII 97 Madrid 28016 Spain Department of Physics College of Science Jouf University Al-Jouf Sakaka 2014 Saudi Arabia Department of Physics Riphah International University Islamabad 44000 Pakistan

Owing to their outstanding performance, environmental friendliness and stability, perovskite materials are becoming very important for solar cells, renewable energy sources and thermoelectric generators. This work uses the first-principles approach to explore the structural, electronic, optical and elastic characteristics of K₂ScCuF₆ and K₂YCuF₆ double perovskites. The negative formation energy in Birch-Murnaghan confirms the stability of the compounds in Fm3m (2 2 5) space group. The analysis of the electronic properties concluded that both K₂ScCuF₆ and K₂YCuF₆ are narrow band gap semiconductors materials, having 1.2 and 2.3 eV of bandgap energies, respectively. This was further verified by the density of states. The mechanical stability, ductility and anisotropic nature of the compounds was shown by analyzing their elastic constants. In addition, the optical properties showed transparency at low energy values but showed both transmission and absorption characteristics at higher energy levels. These interesting results imply that K₂ScCuF₆ and K₂YCuF₆ have significant potential in solar cells, light-emitting diodes (LEDs), smart windows, displays and sensors. © 2024 The Author(s)

关键词： Density Functional Theory Elastic behaviors Opto-electronic properties Pb-free Double perovskite

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Fast Water Transport in UTSA-280 via a Knock-Off Mechanism

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Angewandte Chemie 2023年第39期135卷

作者： Cheng-Hsun Hsu Hsin-Yu Yu Ho Jun Lee Pei-Hao Wu Shing-Jong Huang Jong Suk Lee Tsyr-Yan Yu Yi-Pei Li Dun-Yen Kang Department of Chemical Engineering National Taiwan University No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan Department of Chemical and Biomolecular Engineering Sogang University Baekbeom-ro 35 Mapo-gu Seoul 04107 Republic of Korea Institute of Atomic and Molecular Sciences Academia Sinica Taipei Taiwan Instrumentation Center National Taiwan University Taipei 10617 Taiwan Institute of Emergent Materials Sogang University 35 Baekbeom-ro Mapo-gu Seoul 04107 Republic of Korea International Graduate Program of Molecular Science and Technology (NTU-MST) National Taiwan University Taipei 10617 Taiwan Molecular Science and Technology Program Taiwan International Graduate Program (TIGP) Academia Sinica Taipei 11529 Taiwan Center of Atomic Initiative for New Materials National Taiwan University No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan

Water and other small molecules frequently coordinate within metal-organic frameworks (MOFs). These coordinated molecules may actively engage in mass transfer, moving together with the transport molecules, but this phenomenon has yet to be examined. In this study, we explore a unique water transfer mechanism in UTSA-280, where an incoming water molecule can displace a coordinated molecule for mass transfer. We refer to this process as the “knock-off” mechanism. Despite UTSA-280 possessing one-dimensional channels, the knock-off transport enables water movement along the other two axes, effectively simulating a pseudo-three-dimensional mass transfer. Even with a relatively narrow pore width, the knock-off mechanism enables a high water flux in the UTSA-280 membrane. The knock-off mechanism also renders UTSA-280 superior water/ethanol diffusion selectivity for pervaporation. To validate this unique mechanism, we conducted 1 H and 2 H solid-state NMR on UTSA-280 after the adsorption of deuterated water. We also derived potential energy diagrams from the density functional theory to gain atomic-level insight into the knock-off and the direct-hopping mechanisms. The simulation findings reveal that the energy barrier of the knock-off mechanism is marginally lower than the direct-hopping pathway, implying its potential role in enhancing water diffusion in UTSA-280.

关键词： Diffusion Knock-off Mechanism Membrane Metal-Organic Frameworks Water Transport

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Implementation Method CUSUM To Determine The Accident Prone Areas in Web Based

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Journal of Physics: Conference Series 2018年第1期1114卷

作者： Rozzi Kesuma Dinata Dahlan Abdullah H Hartono Cut Ita Erliana Berliana Kusuma Riasti Akbar Iskandar Ifit Novita Sari Nurmawati Ricardo Freedom Nanuru Lusi Dwi Putri Rosida Tiurma Manurung S. Sriadhi A A Saleh T Astari Muammar Khaddafi Department of Informatics Universitas Malikussaleh Aceh Indonesia Department of Computer Science STMIK IBBI Medan Indonesia Department of Industrial Engineering Universitas Malikussaleh Aceh Indonesia Department of Informatics Universitas Sebelas Maret Surakarta. Indonesia Department of Informatics STMIK AKBA Makassar Indonesia Departement of: Social Science Education Program Post Graduate Program Universitas Kanjuruhan Malang Malang Indonesia Faculty of industry Technique University of 45 Surabaya Indonesia Universitas Kristen Indonesia Maluku Ambon Indonesia Department of Civil Engineering Universitas Lancang Kuning Pekanbaru Indonesia Graduate Program in Scientific Psychology Universitas Kristen Maranatha Indonesia Department of Electrical Engineering Universitas Negeri Medan Indonesia Statistics Financial & Social Sciences Research Group Indonesia Department of Elementary School Teacher Education STKIP Citra Bangsa Aceh Utara Aceh Indonesia Department of Accounting Universitas Malikussaleh Aceh Indonesia

At the Unit Laka Lantas Polres Lhokseumawe determining accident-prone areas on roads in Lhokseumawe still using manual systems. Determination of accident-prone areas are less effective because the police Unit Laka Lantas Polres Lhokseumawe just using the data of the last year and had to repeatedly calculate manually accident-prone areas based on the number of human casualties. In this study the system implementation CUSUM method (Cummulative Summary) to determine the accident-prone areas designed using the web-based programming language PHP. In this system there are three processes to determine areas prone to accidents, the accident rate calculations based on the weighted severity, blacksite calculations using the Z-Score method for determining areas prone to accident blackspots and calculations using the CUSUM method to determine the critical points of an accident. The data used are secondary data obtained from the Police Unit Laka Lantas Polres Lhokseumawe years 2009-2013.

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Retraction: Implementation Method CUSUM To Determine The Accident Prone Areas in Web Based (J. Phys.: Conf. Ser. 1114 012093)

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Journal of Physics: Conference Series 2018年第1期1114卷

This paper was retracted by IOP Publishing on 12 December 2018. This paper was published due to a technical error and was not intended to be included in this journal. Retraction published: 8 February 2019

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