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Correction to: SARS-CoV-2 removal with a polyurethane foam composite

Environmental science and pollution research international 2023年第8期30卷 22033页

作者： Guilherme Pereira Schoeler Thays França Afonso Carolina Faccio Demarco Victor Dos Santos Barboza Tito Roberto Sant'anna Cadaval Andrei Valerão Igansi Marcos Alexandre Gelesky Janice Luehring Giongo Rodrigo de Almeida Vaucher Rafael de Avila Delucis Robson Andreazza Postgraduate Program in Environmental Sciences Center for Engineering Federal University of Pelotas R. Benjamin Constant 989 Pelotas RS CEP 96010-020 Brazil. Postgraduate Program in Materials Science and Engineering Federal University of Pelotas R. Gomes Carneiro 01 Pelotas RS CEP 96010-610 Brazil. Graduate Program in Biochemistry and Bioprospecting Research Laboratory in Biochemical and Molecular Biology of Microorganisms (LaPeBBiOM) Federal University of Pelotas RS Av. Eliseu Maciel Campus Universitário s/n Capão Do Leão CEP 96160-000 Brazil. School of Chemistry and Food Federal University of Rio Grande Av. Itália Km 8 s/n Rio Grande RS CEP 96203-000 Brazil. Postgraduate Program in Environmental Sciences Center for Engineering Federal University of Pelotas R. Benjamin Constant 989 Pelotas RS CEP 96010-020 Brazil. robsonandreazza@yahoo.com.br. Postgraduate Program in Materials Science and Engineering Federal University of Pelotas R. Gomes Carneiro 01 Pelotas RS CEP 96010-610 Brazil. robsonandreazza@yahoo.com.br.

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Bilayer osteochondral graft in rabbit xenogeneic transplantation model comprising sintered 3D-printed bioceramic and human adipose-derived stem cells laden biohydrogel

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Journal of Biological engineering 2023年第1期17卷 74-74页

作者： Lee, Chih-Yun Nedunchezian, Swathi Lin, Sung-Yen Su, Yu-Feng Wu, Che-Wei Wu, Shun-Cheng Chen, Chung-Hwan Wang, Chih-Kuang Ph.D. Program in Life Sciences College of Life Science Kaohsiung Medical University Kaohsiung 80708 Taiwan Regenerative Medicine and Cell Therapy Research Center Kaohsiung Medical University Kaohsiung 80708 Taiwan Orthopaedic Research Center College of Medicine Kaohsiung Medical University Kaohsiung 80708 Taiwan Department of Medicinal and Applied Chemistry College of Life Science Kaohsiung Medical University Kaohsiung 80708 Taiwan Departments of Orthopaedics School of Medicine College of Medicine Kaohsiung Medical University Kaohsiung 80708 Taiwan Department of Orthopaedics Kaohsiung Medical University Hospital Kaohsiung Medical University Kaohsiung 80708 Taiwan Department of Orthopaedics Kaohsiung Municipal Ta-Tung Hospital Kaohsiung Medical University Kaohsiung 80145 Taiwan Faculty of Post-Baccalaureate Medicine College of Medicine Kaohsiung Medical University Kaohsiung 80756 Taiwan Department of Surgery Division of Neurosurgery Kaohsiung Medical University Hospital Kaohsiung Medical University Kaohsiung 80708 Taiwan Department of Nursing Asia University Taichung 41354 Taiwan Ph.D. Program in Biomedical Engineering College of Medicine Kaohsiung Medical University Kaohsiung 80708 Taiwan Graduate Institute of Medicine College of Medicine Kaohsiung Medical University Kaohsiung 80708 Taiwan

Reconstruction of severe osteochondral defects in articular cartilage and subchondral trabecular bone remains a challenging problem. The well-integrated bilayer osteochondral graft design expects to be guided the chondrogenic and osteogenic differentiation for stem cells and provides a promising solution for osteochondral tissue repair in this study. The subchondral bone scaffold approach is based on the developed finer and denser 3D β-tricalcium phosphate (β-TCP) bioceramic scaffold process, which is made using a digital light processing (DLP) technology and the novel photocurable negative thermo-responsive (NTR) bioceramic slurry. Then, the concave-top disc sintered 3D-printed bioceramic incorporates the human adipose-derived stem cells (hADSCs) laden photo-cured hybrid biohydrogel (HG + 0.5AFnSi) comprised of hyaluronic acid methacryloyl (HAMA), gelatin methacryloyl (GelMA), and 0.5% (w/v) acrylate-functionalized nano-silica (AFnSi) crosslinker. The 3D β-TCP bioceramic compartment is used to provide essential mechanical support for cartilage regeneration in the long term and slow biodegradation. However, the apparent density and compressive strength of the 3D β-TCP bioceramics can be obtained for ~ 94.8% theoretical density and 11.38 ± 1.72 MPa, respectively. In addition, the in vivo results demonstrated that the hADSC + HG + 0.5AFnSi/3D β-TCP of the bilayer osteochondral graft showed a much better osteochondral defect repair outcome in a rabbit model. The other word, the subchondral bone scaffold of 3D β-TCP bioceramic could accelerate the bone formation and integration with the adjacent host cancellous tissue at 12 weeks after surgery. And then, a thicker cartilage layer with a smooth surface and uniformly aligned chondrocytes were observed by providing enough steady mechanical support of the 3D β-TCP bioceramic scaffold. © 2023, The Author(s).

关键词： Bioceramic scaffold Digital light processing Gelatin methacryloyl Hyaluronic acid methacryloyl Osteochondral Tissue engineering

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Expression of concern: Microchip-based structure determination of low-molecular weight proteins using cryo-electron microscopy

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Nanoscale 2024年第9期16卷 4919页

作者： Michael A Casasanta G M Jonaid Liam Kaylor William Y Luqiu Maria J Solares Mariah L Schroen William J Dearnaley Jarad Wilson Madeline J Dukes Deborah F Kelly Department of Biomedical Engineering Pennsylvania State University University Park PA 16802 USA. Debkelly@psu.edu. Materials Research Institute Pennsylvania State University University Park PA 16802 USA. Bioinformatics and Genomics Graduate Program Huck Institutes of the Life Sciences Pennsylvania State University University Park PA 16802 USA. Molecular Cellular and Integrative Biosciences Graduate Program Huck Institutes of the Life Sciences Pennsylvania State University University Park PA 16802 USA. Department of Electrical and Computer Engineering Duke University Durham NC 27708 USA. RayBiotech Life Peachtree Corners GA 30092 USA. Applications Science Protochips Inc. Morrisville NC 27560 USA.

Expression of concern for 'Microchip-based structure determination of low-molecular weight proteins using cryo-electron microscopy' by Michael A. Casasanta , , 2021, , 7285-7293, https://***/10.1039/D1NR00388G.

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Magnetoelectric memory function with optical readout

arXiv

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arXiv 2017年

作者： Kocsis, V. Penc, K. Rõõm, T. Nagel, U. Vít, J. Romhányi, J. Tokunaga, Y. Taguchi, Y. Tokura, Y. Kézsmárki, I. Bordács, S. Wako Saitama351-0198 Japan Department of Physics Budapest University of Technology and Economics and MTA-BME Lendület Magneto-optical Spectroscopy Research Group Budapest1111 Hungary Institute for Solid State Physics and Optics Wigner Research Centre for Physics Hungarian Academy of Sciences P.O.B. 49 BudapestH-1525 Hungary National Institute of Chemical Physics and Biophysics Tallinn12618 Estonia Institute of Physics ASCR Na Slovance 2 Prague 8182 21 Eue Faculty of Nuclear Science and Physical Engineering Czech Technical University Břehová 7 Prague 1115 19 Eue Okinawa Institute of Science and Technology Graduate University Onna-sonOkinawa904-0395 Japan Department of Advanced Materials Science University of Tokyo Kashiwa277-8561 Japan Quantum-Phase Electronics Center Department of Applied Physics University of Tokyo Tokyo113-8656 Japan Department of Applied Physics University of Tokyo Hongo Tokyo113-8656 Japan Experimental Physics 5 Center for Electronic Correlations and Magnetism Institute of Physics University of Augsburg Augsburg86159 Germany Hungarian Academy of Sciences Premium Postdoctor Program Budapest1051 Hungary

The ultimate goal of multiferroic research is the development of new-generation non-volatile memory devices1, the so-called magnetoelectric (ME) memories, where magnetic bits are controlled via electric fields without the application of electrical currents subject to dissipation. This low-power operation exploits the entanglement of the magnetization and the electric polarization coexisting in multiferroic materials2,3. Here we demonstrate the optical readout of ME memory states in the antiferromagnetic (AFM) and antiferroelectric (AFE) LiCoPO4, based on the strong absorption difference of THz radiation between its two types of ME domains. This unusual contrast is attributed to the dynamic ME effect of the spin-wave excitations, as confirmed by our microscopic model, which also captures the characteristics of the observed static ME effect. Our proof-of-principle study, demonstrating the control and the optical readout of ME domains in LiCoPO4, lays down the foundation for future ME memory devices based on antiferroelectric-antiferromagnetic insulators. Copyright © 2017, The Authors. All rights reserved.

关键词： Digital storage

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A Photo- and Thermo-Driven Azoarene-Based Circularly Polarized Luminescence Molecular Switch in a Liquid Crystal Host

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Angewandte Chemie 2023年第48期135卷

作者： Wenxin Kang Yuqi Tang Xianyu Meng Siyang Lin Xinfang Zhang Prof. Jinbao Guo Prof. Quan Li Key Laboratory of Carbon Fibers and Functional Polymers Ministry of Education and College of Materials Science and Engineering Beijing University of Chemical Technology Beijing 100029 China Contribution: Investigation (lead) Writing - original draft (equal) Writing - review & editing (supporting) Institute of Advanced Materials and School of Chemistry and Chemical Engineering Southeast University Nanjing 211189 China Contribution: Investigation (supporting) Writing - original draft (supporting) Writing - review & editing (supporting) Materials Science Graduate Program Kent State University Kent OH 44242 USA Contribution: Conceptualization (equal) Funding acquisition (equal) Investigation (supporting) Project administration (lead) Writing - original draft (lead) Writing - review & editing (equal) Contribution: Conceptualization (equal) Funding acquisition (equal) Investigation (supporting) Supervision (lead) Writing - original draft (supporting) Writing - review & editing (equal)

The development of chiral optical active materials with switchable circularly polarized luminescence (CPL) signals remains a challenge. Here an azoarene-based circularly polarized luminescence molecular switch, ( S, R, S )-switch 1 and ( R, R, R )-switch 2 , are designed and prepared with an ( R )-binaphthyl azo group as a chiral photosensitive moiety and two ( S )- or ( R )-binaphthyl fluorescent molecules with opposite or the same handedness as chiral fluorescent moieties. Both switches exhibit reversible trans/cis isomerization when irradiated by 365 nm UV light and 520 nm green light in solvent and liquid crystal (LC) media. In contrast with the control ( R, R, R )-switch 2 , when switch 1 is doped into nematic LCs, polarization inversion and switching-off of the CPL signals are achieved in the resultant helical superstructure upon irradiation with 365 nm UV and 520 nm green light, respectively. Meanwhile, the fluorescence intensity of the system is basically unchanged during this switching process. In particular, these variations of the CPL signals could be recovered after heating, realizing the true sense of CPL reversible switching. Taking advantage of the unique CPL switching, the proof-of-concept for “a dual-optical information encryption system” based on the above CPL active material is demonstrated.

关键词： Chirality Inversion Cholesteric Liquid Crystal Circularly Polarized Luminescence Information Encryption Molecular Switch

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Tunable plasmonic ultrastrong coupling: Emulating dicke physics at room temperature

arXiv

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arXiv 2021年

作者： Yahiaoui, Riad Chase, Zizwe A. Kyaw, Chan Tay, Fuyang Baydin, Andrey Noe, G. Timothy Song, Junyeob Kono, Junichiro Agrawal, Amit Bamba, Motoaki Searles, Thomas A. Department of Physics and Astronomy Howard University WashingtonDC20059 United States Department of Electrical and Computer Engineering Rice University HoustonTX70005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Smalley-Curl Institute Rice University HoustonTX77005 United States Physical Measurement Laboratory National Institute of Standards and Technology GaithersburgMD20899 United States Department of Physics and Astronomy Rice University HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Maryland NanoCenter University of Maryland College ParkMD20742 United States The Hakubi Center for Advanced Research Kyoto University Kyoto606-8502 Japan Department of Physics I Kyoto University Kyoto606-8502 Japan Department of Physics Massachusetts Institute of Technology CambridgeMA02139 United States

A system of N two-level atoms cooperatively interacting with a photonic field can be described as a single giant atom coupled to the field with interaction strength ∝ √N. This enhancement, known as Dicke cooperativity in quantum optics, has recently become an indispensable element in quantum information technology based on strong light-matter coupling. Here, we extend the coupling beyond the standard light-matter interaction paradigm, emulating Dicke cooperativity in a terahertz metasurface with N meta-atoms. Cooperative enhancement manifested in the form of matter-matter coupling, through the hybridization of localized surface plasmon resonance in individual meta-atoms and surface lattice resonance due to the periodic array of the meta-atoms. By varying the lattice constant of the array, we observe a clear anticrossing behavior, a signature of strong coupling. Furthermore, through engineering of the capacitive split-gap in the meta-atoms, the coupling rate was cooperatively enhanced into the ultrastrong coupling regime by a factor of √N. This room-temperature technology serves as a convenient quantum emulator of the dynamics of a qubit with a giant dipole moment coherently driven by a single bosonic field. Copyright © 2021, The Authors. All rights reserved.

关键词： Atoms

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In-situ observation of hydrogen nanobubbles formation on graphene surface by AFM-SECM

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Electrochimica Acta 2024年 493卷

作者： Kholimatussadiah, Septia Hsu, Chia-Ling Ke, Shang-Wei Chou, Tsu-Chin Wu, Yung-Fu Yakimova, Rositsa Kumatani, Akichika Chen, Kuei-Hsien Chen, Li-Chyong Du, He-Yun Department of Physics National Taiwan University Taipei 10617 Taiwan Nano Science and Technology Taiwan International Graduate Program Academia Sinica Taipei 10617 Taiwan Center for Condensed Matter Sciences National Taiwan University Taipei 10617 Taiwan Center of Atomic Initiative for New Materials National Taiwan University Taipei 10617 Taiwan Department of Chemical Engineering Ming Chi University of Technology New Taipei City24301 Taiwan Institute of Atomic and Molecular Sciences Academia Sinica Taipei 10617 Taiwan Institute of Analytical and Environmental Sciences National Tsing Hua University Hsinchu 300044 Taiwan Department of Physics Chemistry and Biology Linköping University SE-581 83 Linköping Sweden Institute of Engineering Innovation School of Engineering The University of Tokyo Tokyo 113-8656 Japan Saitama 332-0012 Japan Tohoku University Sendai980-8577 Japan Battery Research Center of Green Energy Ming Chi University of Technology New Taipei City24301 Taiwan Biochemical Technology R&D Center Ming Chi University of Technology New Taipei City24301 Taiwan Center for Sustainability and Energy Technologies Chang Gung University Taoyuan City33302 Taiwan

Gas bubble evolution is an important phenomenon in many electrochemical processes and it is highly sensitive to the surface properties. Here we visualize the gas bubble dynamics on the surface of different graphene substrates during hydrogen evolution reaction (HER) using atomic force microscopy combined with scanning electrochemical microscopy. The low overpotential and low surface hydrophobicity of few-layer graphene formed on C-phase SiC causes the uniform distribution of hydrogen nanobubbles, which easily depart from the surface during the reaction. Conversely, the high overpotential and more hydrophobic surface of HOPG induces hydrogen bubbles to linger on the surface for an extended duration, leading to its accumulation and the subsequent formation of microbubbles. This in-situ nanoscale electrochemical mapping of hydrogen bubble dynamics provides new insight into electrocatalytic HER that occurs on non-metal electrodes. © 2024 Elsevier Ltd

关键词： Graphene

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EMPRESS. IX. Extremely Metal-Poor Galaxies are Very Gas-Rich Dispersion-Dominated Systems: Will JWST Witness Gaseous Turbulent High-z Primordial Galaxies?

arXiv

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arXiv 2022年

作者： Isobe, Yuki Ouchi, Masami Nakajima, Kimihiko Ozaki, Shinobu Bouché, Nicolas F. Wise, John H. Xu, Yi Emsellem, Eric Kusakabe, Haruka Hattori, Takashi Nagao, Tohru Chiaki, Gen Fukushima, Hajime Harikane, Yuichi Hayashi, Kohei Hirai, Yutaka Kim, Ji Hoon Maseda, Michael V. Nagamine, Kentaro Shibuya, Takatoshi Sugahara, Yuma Yajima, Hidenobu Aoyama, Shohei Fujimoto, Seiji Fukushima, Keita Hatano, Shun Inoue, Akio K. Ishigaki, Tsuyoshi Kawasaki, Masahiro Kojima, Takashi Komiyama, Yutaka Koyama, Shuhei Koyama, Yusei Lee, Chien-Hsiu Matsumoto, Akinori Mawatari, Ken Moriya, Takashi J. Motohara, Kentaro Murai, Kai Nishigaki, Moka Onodera, Masato Ono, Yoshiaki Rauch, Michael Saito, Tomoki Sasaki, Rin Suzuki, Akihiro Takeuchi, Tsutomu T. Umeda, Hiroya Umemura, Masayuki Watanabe, Kuria Yabe, Kiyoto Zhang, Yechi Institute for Cosmic Ray Research The University of Tokyo 5-1-5 Kashiwanoha Chiba Kashiwa277-8582 Japan Department of Physics Graduate School of Science The University of Tokyo 7-3-1 Hongo Bunkyo Tokyo113-0033 Japan National Astronomical Observatory of Japan 2-21-1 Osawa Mitaka Tokyo181-8588 Japan University of Tokyo Chiba Kashiwa277-8583 Japan Univ Lyon Univ Lyon1 ENS de Lyon CNRS Centre de Recherche Astrophysique de Lyon UMR5574 Saint-Genis-LavalF-69230 France Center for Relativistic Astrophysics School of Physics Georgia Institute of Technology AtlantaGA30332 United States Department of Astronomy Graduate School of Science The University of Tokyo 7-3-1 Hongo Bunkyo Tokyo113-0033 Japan European Southern Observatory Karl-Schwarzschild-Straße 2 Garching85748 Germany Observatoire de Genéve Université de Genéve 51 Ch. des Maillettes Versoix1290 Switzerland 650 North A'ohoku Place HiloHI96720 United States Research Center for Space and Cosmic Evolution Ehime University Bunkyo-cho 2-5 Ehime Matsuyama790-8577 Japan Center for Computational Sciences University of Tsukuba Ten-nodai 1-1-1 Tsukuba Ibaraki305-8577 Japan Department of Physics and Astronomy University College London Gower Street LondonWC1E 6BT United Kingdom National Institute of Technology Ichinoseki College Hagisho Ichinoseki021-8511 Japan Astronomical Institute Tohoku University 6-3 Aoba Aramaki Aoba-ku Miyagi Sendai980-8578 Japan Department of Physics and Astronomy University of Notre Dame 225 Nieuwland Science Hall Notre DameIN46556 United States Astronomy Program Department of Physics and Astronomy Seoul National University 1 Gwanak-ro Gwanak-gu Seoul08826 Korea Republic of SNU Astronomy Research Center Seoul National University 1 Gwanak-ro Gwanak-gu Seoul08826 Korea Republic of Department of Astronomy University of Wisconsin-Madison 475 N. Charter Street MadisonWI53706 United States Theoretical Astrophysics Department of Earth & Space S

We present kinematics of 6 local extremely metal-poor galaxies (EMPGs) with low metallicities (0.016 − 0.098 Z☉) and low stellar masses (104.7 − 107.6M☉). Taking deep medium-high resolution (R ∼ 7500) integral-field spectra with 8.2-m Subaru, we resolve the small inner velocity gradients and dispersions of the EMPGs with Hα emission. Carefully masking out sub-structures originated by inflow and/or outflow, we fit 3-dimensional disk models to the observed Hα flux, velocity, and velocity-dispersion maps. All the EMPGs show rotational velocities (vrot) of 5-23 km s−1 smaller than the velocity dispersions (σ0) of 17-31 km s−1, indicating dispersion-dominated (vrot/σ0 = 0.29−0.80 gas 0.9 − 1.0. Comparing our results with other Hα kinematics studies, we find that vrot/σ0 decreases and fgas increases with decreasing metallicity, decreasing stellar mass, and increasing specific star-formation rate. We also find that simulated high-z (z ∼ 7) forming galaxies have gas fractions and dynamics similar to the observed EMPGs. Our EMPG observations and the simulations suggest that primordial galaxies are gas-rich dispersion-dominated systems, which would be identified by the forthcoming James Webb Space Telescope (JWST) observations at z ∼ 7. Copyright © 2022, The Authors. All rights reserved.

关键词： Galaxies

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Fluorescent phenylthiazoles: Application as latent fingermark and their cytotoxicity against NOK-SI cell line

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Chemical Data Collections 2021年 33卷

作者： Bruno Nunes da Rosa Kristiane de Cássia Mariotti Bruna Silveira Pacheco Caroline Carapina da Silva Neftalí Lenin Villarreal Carreño Caroline Nicolodi Tais Poletti Allison Carlos Assunção Silva Adriana Fernandes da Silva Janice Luehring Giongo Rodrigo de Almeida Vaucher Tiago Franco de Oliveira Claudio Martin Pereira de Pereira Laboratory of Lipidomics and Bioorganic Bioforensics Research Group Federal University of Pelotas 96010 900 Pelotas RS Brazil National Institute of Forensic Science and Technology (INCT Forensic) Porto Alegre (RS) Pelotas (RS) Brazil Identification Group Brazilian Federal Police 90610-093 Porto Alegre RS Brazil Materials Science and Engineering Technology Development Center Federal University of Pelotas 96010-000 Pelotas RS Brazil Post-Graduate Program in Dentistry Department of Restorative Dentistry Dental School Federal University of Pelotas 96010 Pelotas RS Brazil Laboratory of Biochemistry Research and Molecular Biology of Microorganisms (LaPeBBiOM) Federal University of Pelotas 96010-900 Pelotas RS Brazil Pharmacosciences Department Federal University of Health Sciences of Porto Alegre Porto Alegre RS Brazil

Fingerprints are unique to each individual who contributes to human identification in forensic cases. In this sense, the present work aimed to synthesize 1H-pyrazol-1-yl-4-phenylthiazoles and apply them as powder agents to reveal latent finger marks as an alternative and low cost related to powders found on the market. The compounds were characterized by infrared; fluorescence; 1H NMR; 13C NMR; laser diffractometer and SEM. In addition, cytotoxicity was also evaluated in oral keratinocytes showing high cell viability. The result of the hemolytic assay revealed that compound 2a does not present red cell cytotoxicity. The prepared powders were applied to fingermarks deposited on different surfaces providing quality visualization at level three so that human identification is possible.

关键词： Forensic chemistry Fingermark Thiazoles Cytotoxicity Development powder

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Correction: Interface structure, precursor rheology and dielectric properties of BaTiO3/PVDF–hfp nanocomposite films prepared from colloidal perovskite nanoparticles

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RSC Advances 2017年第73期7卷 45987-45987页

作者： Y. N. Hao K. Bi S. O’Brien X. H. Wang J. Lombardi F. Pearsall W. L. Li M. Lei Y. Wu L. T. Li State Key Laboratory of Information Photonics and Optical Communications School of Science Beijing University of Posts and Telecommunications Beijing 100876 China The Department of Chemistry and Biochemistry The City College of New York The Ph.D. Program in Chemistry The Graduate Center of the City University of New York New York NY 10016 USA State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and Engineering Tsinghua University Beijing 100084 China School of Journalism and Communication Beijing Normal University Beijing 100875 China

Correction for ‘Interface structure, precursor rheology and dielectric properties of BaTiO3/PVDF–hfp nanocomposite films prepared from colloidal perovskite nanoparticles’ by Y. N. Hao et al., RSC Adv., 2017, 7, 32...

Correction for ‘Interface structure, precursor rheology and dielectric properties of BaTiO₃/PVDF–hfp nanocomposite films prepared from colloidal perovskite nanoparticles’ by Y. N. Hao et al., RSC Adv., 2017, 7, 32886–32892.

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