检索结果-内蒙古大学图书馆

Braiding fractional quantum Hall quasiholes on a superconducting quantum processor

Physical Review B 2023年第6期108卷 064303-064303页

作者： Ammar Kirmani Derek S. Wang Pouyan Ghaemi Armin Rahmani Physics Department City College of the City University of New York New York 10031 USA IBM Quantum IBM T.J. Watson Research Center Yorktown Heights 10598 USA Physics Program Graduate Center of City University of New York New York 10031 USA Department of Physics and Astronomy and Advanced Materials Science and Engineering Center Western Washington University Bellingham Washington 98225 USA

Direct experimental detection of anyonic exchange statistics in fractional quantum Hall systems by braiding the excitations and measuring the wave-function phase is an enormous challenge. Here, we use a small, noisy quantum computer to emulate direct braiding within the framework of a simplified model applicable to a thin cylinder geometry and measure the topological phase. Our algorithm first prepares the ground state with two quasiholes. It then applies a unitary operation controlled by an ancilla, corresponding to a sequence of adiabatic evolutions that take one quasihole around the other. We finally extract the phase of the wave function from measuring the ancilla with a compound error mitigation strategy. Our results point out an avenue for studying braiding statistics in fractional Hall states.

关键词： Anyons Fractional quantum Hall effect Quantum algorithms Superconducting devices

来源：评论

学校读者我要写书评

暂无评论

Far-Field Subwavelength Acoustic Computational Imaging with a Single Detector

引用

Physical Review Applied 2022年第1期18卷 014046-014046页

作者： Yuan Tian Hao Ge Xiu-Juan Zhang Xiang-Yuan Xu Ming-Hui Lu Yun Jing Yan-Feng Chen National Laboratory of Solid State Microstructures and Department of Materials Science and Engineering Nanjing University Nanjing 210093 China The Institute of Acoustics of the Chinese Academy of Sciences Beijing 100190 China Collaborative Innovation Center of Advanced Microstructures Nanjing 210093 China Graduate Program in Acoustics The Pennsylvania State University University Park Pennsylvania 16802 USA

Acoustic imaging techniques suffer from the diffraction limit due to the loss of evanescent waves that carry subwavelength information of objects. To overcome the diffraction limit, the evanescent components have to be collected and measured. Most of the existing methods targeting this task rely on expensive detector arrays and inefficient near-field point-by-point scanning. Here, we propose and experimentally demonstrate the realization of a far-field acoustic subwavelength imaging method based on a single stationary detector. Specifically, we utilize a series of masks to structure the detected field, so that the evanescent wave information is encoded into the propagating waves due to spatial frequency convolution between the object and masks. Our study shows that, by combining the principles of computational imaging and metalens, high-quality images of a subwavelength object can be reconstructed in the far field, even in the presence of unwanted scatterers. Our work provides a robust method for far-field acoustic subwavelength imaging, which could bring possibilities for acoustic microscopy and could further be applied to medical ultrasonography, underwater sonar, and ultrasonic nondestructive evaluation.

关键词： Acoustic metamaterials Acoustic modeling Acoustics Ghost imaging

来源：评论

学校读者我要写书评

暂无评论

Rapid Electronic Transport Channel of Co-P with Mo in a Heterostructure Embedded with P, N Dual Doped Porous Carbon for Electrocatalytic Oxygen and Hydrogen Evolution

引用

ChemNanoMat 2024年第7期10卷

作者： Dey, Tapan Rajput, Anubha Jhaa, Gaurav Matsagar, Babasahab M. Chen, Norman C.-R Kumar, Nitish Salunkhe, Rahul Wu, Kevin C.-W. Chakraborty, Biswarup Dutta, Saikat Electrochemical Energy & Sensor Research Laboratory Amity Institute of Click Chemistry Research & Studies Amity University Noida India Department of Chemistry Indian Institute of Technology Delhi Hauz Khas New Delhi110016 India Chemical Information Sciences Laboratory Department of Chemistry Pondicherry University Kalapet Pondicherry605014 India Department of Chemical Engineering National Taiwan University No. 1 Sec. 4 Roosevelt Road Taipei10617 Taiwan Molecular Science and Technology Program Taiwan International Graduate Program Academia Sinica Taiwan Materials Research Laboratory Department of Physics Indian Institute of Technology Jammu Jammu India Department of Chemical Engineering and Materials Science Yuan Ze University Taoyuan Chung-Li Taiwan Department of Chemical Engineering Chung Yuan Christian University No. 200 Zhongbei Rd. Zhongli Dist. Taoyuan City320 Taiwan

We developed a molybdenum (Mo)-doped cobalt (Co)-heterostructure embedded on a phosphorous (P) and nitrogen (N) dual-doped porous carbon which exhibits an intrinsic electronic transport channel of Co to Mo and P. The P,Mo,O−Co/PNC/NF (NF=Nickel foam) electrode offers 335 mV overpotential at 10 mA cm−2 in OER as compared with PMA-ZIF67-NC/NF and ZIF67-NC/NF electrode with an overpotential of 357 and 373 mV respectively. Linear sweep voltammetry (LSV) of overall water splitting (OWS) supports that the current density gradually increased at a cell potential of 1.6 V with a maximum of 40 mA with a corresponding cell potential of 1.79 V at a current density of 10 mA cm−2. Density functional theory (DFT) calculations for water adsorption on optimized [111] surface of Co, CoMo, and CoMoP2 with adsorbed H2O and corresponding lattice determine the electron density difference of [111] surface with adsorbed H2O for Eads (eV) 4.23 corresponds to adsorption energy for CoMoP2. XANE-EXAFS spectroscopy of P,Mo,O−Co/PNC at Co K edge and Mo K edge suggests the presence of higher valence of both Cox+ and Mox+ without metallic Co and Mo and Co−P and Mo−P bonds as major structural units due to phosphidation as determined by R-space FT-EXAFS spectra. © 2024 Wiley-VCH GmbH.

关键词： Cobalt

来源：评论

学校读者我要写书评

暂无评论

Influence of Grain Size on Strain-Induced Phase Transformation in a Crconi Multi-Principal Element Alloy

SSRN

引用

SSRN 2024年

作者： Bertoli, Gustavo Clarke, Amy J. Kaufman, Michael J. Kiminami, Claudio Shyint Gil Coury, Francisco Colorado School of Mines George S. Ansell Department of Metallurgical and Materials Engineering 1500 Illinois St. GoldenCO80401 United States Federal University of São Carlos Graduate Program in Materials Science and Engineering Rod. Washington Luis km 235 SP-310 SP São Carlos13565-905 Brazil Sigma Manufacturing Sciences Division Los Alamos National Laboratory Los AlamosNM87545 United States Federal University of São Carlos Department of Materials Engineering Rod. Washington Luis km 235 SP-310 SP São Carlos13565-905 Brazil

A Cr40Co40Ni20 (at.%) alloy with different grain sizes was analyzed through in-situ synchrotron X-ray diffraction during tensile testing. The FCC starting structure underwent a partial strain-induced transformation to HCP (TRIP effect) and the percent transformed was measured throughout the deformation. The critical stress required to form a certain HCP fraction was shown to follow a Hall-Petch relation (σ = σ0,HCP + KHCPd-0.5), with the Hall-Petch slope being approximately the same for yield stress and TRIP effect (Ky ~ KHCP ~ 650 MPa/μm-0.5). The HCP fraction and HCP formation rate are controlled by the strain level, being insensitive to grain size in terms of strain. Furthermore, this work developed a Hall-Petch-based model that correlates the applied stress, the transformed phase fraction, and the initial FCC grain size. It predicts the stress required to form a certain HCP fraction, or the fraction formed when a certain stress is applied. We also proposed a mechanism to explain the grain size dependence of the TRIP effect and discuss how the TRIP effect and its early activation in the Cr40Co40Ni20 alloy provide high work-hardening capacity, which improves ductility and toughness. Here, a refined FCC grain size (1.3 μm) was shown to increase the yield stress by at least 100% (417 → 834 MPa), compared to a coarser grain material (22.4 μm), while maintaining a high ductility of 41%. This work contributes to a better understanding of the deformation mechanisms, mainly the strain-induced phase transformation (TRIP), highlighting their impact and importance on mechanical properties. © 2024, The Authors. All rights reserved.

关键词： Ductility

来源：评论

学校读者我要写书评

暂无评论

Protein folding as a jamming transition

arXiv

引用

arXiv 2024年

作者： Grigas, Alex T. Liu, Zhuoyi Logan, Jack A. Shattuck, Mark D. O’Hern, Corey S. Graduate Program in Computational Biology and Bioinformatics Yale University New HavenCT06520 United States Integrated Graduate Program in Physical and Engineering Biology Yale University New HavenCT06520 United States Department of Mechanical Engineering and Materials Science Yale University New HavenCT06520 United States Benjamin Levich Institute and Physics Department The City College of New York New YorkNY10031 United States Department of Physics Yale University New HavenCT06520 United States Department of Applied Physics Yale University New HavenCT06520 United States

Proteins fold to a specific functional conformation with a densely packed hydrophobic core that controls their stability. We develop a geometric, yet all-atom model for proteins that explains the universal core packing fraction of φc = 0.55 found in experimental measurements. We show that as the hydrophobic interactions increase relative to the temperature, a novel jamming transition occurs when the core packing fraction exceeds φc. The model also recapitulates the global structure of proteins since it can accurately refold to native-like structures from partially unfolded states. © 2024, CC BY.

关键词： Proteins

来源：评论

学校读者我要写书评

暂无评论

Role of the Ionomer in Supporting Electrolyte-Fed Anion Exchange Membrane Water Electrolyzers

ACS electrochemistry

引用

ACS electrochemistry 2025年第2期1卷 239-248页

作者： Emily K Volk Arielle L Clauser Melissa E Kreider Diego D Soetrisno Sunilkumar Khandavalli Joshua D Sugar Stephanie Kwon Shaun M Alia Advanced Energy Systems Graduate Program Colorado School of Mines Golden Colorado 80401 United States. Sandia National Laboratories Livermore California 94550 United States. Chemistry and Nanoscience Center National Renewable Energy Laboratory Golden Colorado 80401 United States. Materials Science Center National Renewable Energy Laboratory Golden Colorado 80401 United States. Department of Chemical and Biological Engineering Colorado School of Mines Golden Colorado 80401 United States.

While anion exchange membrane water electrolyzers (AEMWEs) have achieved significant performance advances in recent decades, overpotentials remain high relative to their proton exchange membrane water electrolyzer (PEMWE) counterparts, requiring AEMWE-specific catalyst layer design strategies to further advance this technology. In this work, the role of the ionomer in catalyst layer structure and quality, catalyst layer stability, and ion conduction for supporting electrolyte-fed AEMWEs is assessed for catalyst layers composed of NiFeO and PiperION TP85 from Versogen at variable ionomer contents (0-30 wt %) for tests up to 200 h. The results reveal that, for supporting electrolyte-fed AEM devices, the ionomer is not required for ion conduction through the catalyst layer. Instead, the ionomer is found to play a critical role in catalyst layer structure and stability, where intermediate ionomer contents lead to the lowest overpotentials, highest effective surface areas, and lowest catalyst layer resistances. Catalyst layer stability is found to be a function of both catalyst adhesion and ionomer loss. These results show that an ionomer may be selected which is not of the same chemistry as the anion exchange membrane, mitigating ionomer stability concerns throughout the catalyst layer and offering a pathway towards highly active and stable AEMWEs.

关键词：

来源：评论

学校读者我要写书评

暂无评论

engineering the directionality of hot carrier tunneling in plasmonic tunneling structures

arXiv

引用

arXiv 2023年

作者： Abbasi, Mahdiyeh Liao, Shusen Zhu, Yunxuan Natelson, Douglas Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Physics and Astronomy Engineering Rice University HoustonTX77005 United States Department of Materials Science and Nanoengineering Rice University HoustonTX77005 United States

Tunneling metal-insulator-metal (MIM) junctions can exhibit an open-circuit photovoltage (OCPV) response under illumination that may be useful for photodetection. One mechanism for photovoltage generation is hot carrier tunneling, in which photoexcited carriers generate a net photocurrent that must be balanced by a drift current in the open-circuit configuration. We present experiments in electromigrated planar MIM structures, designed with asymmetric plasmonic properties using Au and Pt electrodes. Decay of optically excited local plasmonic modes preferentially creates hot carriers on the Au side of the junction, leading to a clear preferred directionality of the hot electron photocurrent and hence a preferred polarity of the resulting OCPV. In contrast, in an ensemble of symmetric devices constructed from only one Au, polarity of the OCPV has no preferred direction. Copyright © 2023, The Authors. All rights reserved.

关键词： Plasmonics

来源：评论

学校读者我要写书评

暂无评论

An Innovative Real-Time Cell Viability Analysis: A Cutting-Edge Flexible Bioimpedance Sensor

SSRN

引用

SSRN 2023年

作者： Chou, Hsin-Yu Ching, Congo Tak-Shing Huang, Hui-Xuan Phan, Thien Luan Wang, Hui-Min David Department of Materials Science and Engineering National Chung Hsing University Taichung40227 Taiwan Ph.D. Program in Tissue Engineering and Regenerative Medicine National Chung Hsing University Taichung402 Taiwan Graduate Institute of Biomedical Engineering National Chung Hsing University Taichung40227 Taiwan Department of Electrical Engineering National Chi Nan University Nantou54561 Taiwan Department of Physic and Electronic Engineering Faculty of Physic and Engineering Physic Vietnam National University Ho Chi Minh City University of Science Viet Nam Graduate Institute of Medicine College of Medicine Kaohsiung Medical University Kaohsiung807 Taiwan Department of Medical Laboratory Science and Biotechnology China Medical University Taichung City404 Taiwan

There are many compounds to be used to treat cancer but still only 20% of proposed anticancer agents have been commercialized after clinical trials due to serious side effects and unsatisfactory results. To screen potential drugs precisely and quickly, this study develops a flexible bioimpedance sensor. The sensor is positive to detect the half maximal inhibitory concentration (IC50) of drugs real-time by analyzing phase angle changes during cell mortality. The best results are achieved using a probe separation of A12B34 at logarithmic frequencies of 163 Hz and 77.87 kHz. At these two frequencies, there is a linear relationship with the phase angle at 0% and 50% of the dead cells. Dividing the phase angle at the two frequencies shows a 17.98% change in the phase angle, which allows self-correction and insensitivity to the number of cells. A custom phase angle measurement device is developed for detection at 163 Hz and 77.87 kHz, respectively. This study develops a novel sensor that is precise, fast and allows high throughput analysis to detect the inhibition of cancer in real-time. This sensor is an alternative to traditional chemical detection methods because it is faster, cheaper and more accurate. © 2023, The Authors. All rights reserved.

关键词： Chemical detection

来源：评论

学校读者我要写书评

暂无评论

The investigation of the physical properties and bandgap engineering of the antimony trirutile phase-based magnesium under hydrostatic pressure

引用

Inorganic Chemistry Communications 2025年 179卷

作者： Rania Charif Rachid Makhloufi Oumnia Racha Selmi Sarah Chaba Mouna Wahidullah Khan Laboratory of Applied Chemistry (LCA) University of Biskra P.O. Box 145 07000 Biskra Algeria Department of Materials Science Dr. Yahia Fares University Algeria Post Graduate Program of Materials Science UFRGS Porto Alegre RS 91501-970 Brazil

The trirutile structure holds significant potential for use in affordable photovoltaic and optoelectronic devices. This manuscript examines MgSb 2 O 6 material structural, thermodynamic, electronic, optical, and mechanical properties utilizing density functional theory (DFT) simulations. Additionally, we investigate the effects of hydrostatic pressure ranging from 0 to 70 GPa on these physical properties. Our study presents the first theoretical framework for analyzing the behaviour of MgSb 2 O 6 under pressure, offering valuable insights into its properties. The compound retains a tetragonal crystal structure across this pressure range, and the derived lattice constants align with those reported in other experimental studies. Moreover, the thermal properties of the MgSb 2 O 6 compound have been determined, including enthalpy, free energy, heat capacity, entropy, and Debye temperature, which can support future experimental and theoretical investigations of this material. Due to their high Debye temperatures, the components under study exhibit relatively high melting points. The electronic density of states (DOS) and electronic band structures were evaluated with the GGA-PBE exchange correlation function, the results reveal that the direct (Γ-Γ) energy bandgap value increases and shifts in the ultraviolet spectrum by applying pressures from 0 to 70 GPa. The optical properties of the MgSb 2 O 6 compound are described in detail, including dielectric function, absorption, reflection, conductivity, and refractive index, which highlight the potential of this material for optoelectronic and engineering applications. The increase in the elastic modulus value indicates that MgSb 2 O 6 becomes stiffer under stress. The Poisson’s and Pugh’s ratios also show that the compound transforms from brittle to ductile when pressure is applied. Pressure significantly affects this material’s anisotropy factor, causing deviations from a spherical shape. This discovery brings up interestin

关键词：

来源：评论

学校读者我要写书评

暂无评论

Innentitelbild: Cucurbituril-Mediated Supramolecular Heterodimerisation and Photoinduced [2+2] Heterocycloaddition to Generate Unexpected Rotaxanes (Angew. Chem. 39/2024)

引用

Angewandte Chemie 2024年第39期136卷

作者： Dr. Shu Zhang Liyan Zhang Aocheng Chen Yi An Dr. Xu-Man Chen Prof. Hong Yang Prof. Quan Li Institute of Advanced Materials and School of Chemistry and Chemical Engineering Southeast University Nanjing 211189 China Materials Science Graduate Program Kent State University Kent OH-44242 USA

来源：评论

学校读者我要写书评

暂无评论

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案：

请选择收藏分类：

通借通还

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：