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Robust, Ultrafast and Reversible Photoswitching in Bulk Polymers Enabled by Octupolar Molecule Design

Angewandte Chemie 2024年第16期136卷

作者： Long Fang Ziwei Lin Yang Zhang Bin Ye Jing Li Qishan Ran Xiaotong Wang Meijia Yang Prof. Zhongke Yuan Prof. Xiaofeng Lin Prof. Dingshan Yu Prof. Xudong Chen Prof. Quan Li Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education Key Laboratory of High Performance Polymer-based Composites of Guangdong Province GBRCE for Functional Molecular Engineering School of Chemistry Sun Yat-sen University Guangzhou 510006 China School of Computer Science and Engineering Sun Yat-sen University Guangzhou 510275 China Institute of Applied Physics and Materials Engineering University of Macau Taipa Macao SAR 999078 China School of Chemical Engineering and Light Industry Guangdong University of Technology Guangzhou 510006 China Guangdong Laboratory of Chemistry and Fine Chemical Industry Jieyang Center Jieyang 515200 China Institute of Advanced Materials and School of Chemistry and Chemical Engineering Southeast University Nanjing 211189 China Materials Science Graduate Program Kent State University Kent OH 44242 USA

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Piecewise Polynomial Interpolation function approach for solving nonlinear programming problems with disjoint feasible regions: Mathematical proofs

arXiv

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arXiv 2020年

作者： Pinheiro, Ricardo B.N.M. Balbo, Antonio R. Nepomuceno, Leonardo Post-graduate program in Electrical Engineering Engineering Faculty Univ Estadual Paulista - UNESP Bauru–SP Brazil Department of Electrical Engineering in the Engineering Faculty Univ Estadual Paulista - UNESP Bauru–SP Brazil Department of Mathematics Science Faculty Univ Estadual Paulista - UNESP Bauru–SP Brazil

The Piecewise Polynomial Interpolation (PPI) function approach is aimed at solving nonlinear programming problems with disjoint feasible regions. In such problems, disjointedness is generally associated with prohibited operating zones, which correspond to bands of values that a variable is not allowed to assume. An analytical implication of such prohibited operating zones is to make the objective function, as well as its domain, discontinuous. The PPI function approach consists in replacing the constraints associated with prohibited operating zones by an equivalent set of equality and inequality constraints, thereby allowing the application of any efficient gradient-based optimization method for solving the equivalent problem. In this paper, we present the definition of the PPI function and provide the mathematical proofs for its properties. Copyright © 2020, The Authors. All rights reserved.

关键词： Constraint theory

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Correction to: Corrosion Resistant Boron-Modified Ferritic and Austenitic Stainless Steels Designed by CALPHAD

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Metallurgical and materials Transactions A 2021年第7期52卷 3190-3190页

作者： dos Santos, E. R. da Silva, W. A. Koga, G. Y. Bolfarini, C. Zepon, G. Graduate Program in Materials Science and Engineering Federal University of Sao Carlos Sao Carlos Brazil Department of Materials Engineering Federal University of Sao Carlos Sao Carlos Brazil

A correction to this paper has been published: https://***/10.1007/s11661-021-06290-w

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CCL5 Protects Cortical Neuron Function by Regulating M2 Microglia Activation After Mild Traumatic Brain Injury

SSRN

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SSRN 2022年

作者： Tsai, Yih-Jeng Ho, Man-Hau Yen, Chia-Hung Wang, Jia-Yi Burnouf, Thierry Chen, Chia-Yen Wang, Yun Chiang, Yung-Hsiao Hoffer, Barry J. Chou, Szu-Yi Department of Otolaryngology Head and Neck Surgery Shin Kong Wu HoSu Memorial Hospital Taipei Taiwan School of Medicine Fu Jen Catholic University New Taipei City Taiwan Ph.D. Program in Medical Neuroscience College of Medical Science and Technology Taipei Medical University National Health Research Institute Taiwan Graduate Institute of Neural Regenerative Medicine College of Medical Science and Technology Taipei Medical University Taipei Taiwan Department of Biological Science and Technology National Pingtung University of Science and Technology Neipu Pingtung91201 Taiwan Graduate Institute of Medical Sciences College of Medicine Taipei Medical University Taipei11031 Taiwan Department of Neurosurgery Taipei Medical University Hospital Taipei11031 Taiwan Neuroscience Research Center Taipei Medical University Taipei11031 Taiwan International PhD Program in Biomedical Engineering College of Biomedical Engineering Taipei Medical University Taipei Taiwan Graduate Institute of Biomedical Materials and Tissue Engineering College of Biomedical Engineering Taipei Medical University Taipei Taiwan NeuroTMULille International Laboratory Taipei Medical University Taipei Taiwan International PhD Program in Cell Therapy and Regeneration Medicine College of Medicine Taipei Medical University Taipei Taiwan Brain and Consciousness Research Centre TMU Shuang Ho Hospital New Taipei City Taiwan Center for Neuropsychiatric Research National Health Research Institutes Zhunan Miaoli County Taiwan Department of Surgery School of Medicine College of Medicine Taipei Medical University 11031 Taiwan Department of Neurosurgery Case Western Reserve University School of Medicine ClevelandOH United States Scientist Emeritus National Institutes of Health United States International Master Program in Medical Neuroscience College of Medical Science and Technology Taipei Medical University Taipei Taiwan

Cytokines and chemokines play important roles in inflammation and repair following brain injury. M1 microglia are pro-inflammatory which produce cytokines and lead to neural injury;in contrast, M2 microglia are anti-inflammatory, release neurotrophic factors, and promote neural repair processes. Chemokine CCL5, increased after TBI, shows a neuroprotective function by reducing oxidative stress. CCL5 may contribute to the balance between oxidative stress and immune responses after brain injury. Herein, we investigated the role of CCL5 in microglial polarization after mild traumatic brain injury, focusing on the cerebral cortex.C57BL/6 and CCL5 knockout (CCL5-KO) mice were given a mild traumatic brain injury (TBI) using weight-drop. Neurological parameters such as motor and sensory functions were analyzed by mNSS score, accelerating rotarod, beam walking, and adhesive removal tests. Oxidative stress and neuron damage were measured by NADPH oxidase activity, hypoxyloprobe staining and FJC. Performance of motor and sensory functions in both WT and CCL5-KO mice were impaired after brain injury which recovered after 7 days-post-injury (dpi) in the WT group but only after 14 days in the CCL5-KO mouse group. RT-qPCR analysis revealed that pro-inflammation cytokines - IL-1β, TNF-α, and IL-6 were higher in CCL5-KO mice compared to WT mice at 4 and 14 dpi. In contrast, M2-like microglia markers - IL-10 and Agr-1 were increased in WT mouse cortical tissue at 4 dpi. Oxidative stress increased both M1 and M2- related cytokine expression in BV2 cells treated with H 2 O 2;CCL5 treatment increased M2- but suppressed M1- related cytokine gene activation. Intranasal delivery of CCL5 reduced neuronal oxidative stress, increased IL-10 expression and improved motor and sensory functions in CCL5-KO mice after brain *** summary, CCL5, which alters immune responses and protects neurons from TBI damage, has an important function in regulating M2-like microglial polarization during post-

关键词： Polarization

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Sharma et al. Reply:

引用

Physical Review Letters 2022年第21期128卷 219602-219602页

作者： Keshav Sharma Nathalia L. Costa Yoong Ahm Kim Hiroyuki Muramatsu Newton M. Barbosa Neto Luiz G. P. Martins Jing Kong Alexandre Rocha Paschoal Paulo T. Araujo Department of Physics and Astronomy University of Alabama Tuscaloosa 35487 Alabama USA Department of Physics Federal University of Ceara Fortaleza 60455-760 Ceara Brazil Department of Polymer Engineering School of Polymer Science and Engineering and Alan G. MacDiarmid Energy Research Institute Chonnam National University 77 Yongbong-ro Buk-gu Gwangju 61186 Republic of Korea Research Institute for Supra-Materials Shinshu University 4-17-1 Wakasato 380-8553 Nagano Japan Institute of Natural Sciences Graduate Program in Physics Federal University of Para Belem 66075-110 Brazil Department of Physics Massachusetts Institute of Technology Cambridge 02139 Massachusetts USA Department of Electrical Engineering and Computer Science Massachusetts Institute of Technology Cambridge 02139 Massachusetts USA

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Prediction of Fluctuations in a Chaotic Cancer Model Using Machine Learning

SSRN

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SSRN 2022年

作者： Sayari, Elaheh da Silva, Sidney Tiago Iarosz, Kelly C. Viana, Ricardo L. Szezech, José Danilo Batista, Antonio Marcos Post-Graduation in Science State University of Ponta Grossa PR Ponta Grossa Brazil Federal University of Paraná PR Curitiba Brazil Faculdade de Telêmaco Borba FATEB Telêmaco Borba Paraná Brazil Graduate Program in Chemical Engineering Federal Technological University of Paraná PR Ponta Grossa Brazil Department of Physics Federal University of Paraná PR Curitiba Brazil Institute of Physics University of São Paulo SP São Paulo Brazil Mathematics and Statistics Department State University of Ponta Grossa PR Ponta Grossa Brazil

Cancer is a group of diseases and the second leading cause of death according to World Health Organization. Mathematical and computational methods have been used to explore the cancer cells spread and the mechanism of their growth. We study a cancer model that exhibits both periodic and chaotic attractors. It describes the interactions among host, effector immune, and cancer cells. It is observed fluctuations in the population of cells. The fluctuation range can be associated with the appearance of tumour cells. In this work, we use machine learning algorithms for the prediction of fluctuations. We show that our machine learning classification is able to identify fluctuations that are associated with the growth rate of cancer cells. © 2022, The Authors. All rights reserved.

关键词： Cancer cells

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Application of Emerging Innovations in Microbiome science to Space Development and Settlement Systems 73

Application of Emerging Innovations in Microbiome Science to...

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73rd International Astronautical Congress, IAC 2022

作者： Nastasi, Nicholas Anderson, Matthew Z. Balasubrahmaniam, Neeraja Bope, Ashleigh Britt, Rodney D. Cochran, Samuel J. Gill, Samuel J. Hegarty, Bridget Lee, Jiyoung Stamps, Blake W. Stickney, Amanda Taylor, Christopher G. Tram, Nguyen K. Van Dusen, John Varaljay, Vanessa A. Weir, Mark H. Horack, John M. Oglesbee, Michael Sullivan, Matthew B. Dannemiller, Karen C. Department of Civil Environmental & Geodetic Engineering Ohio State University ColumbusOH United States Division of Environmental Health Sciences College of Public Health Ohio State University ColumbusOH United States Environmental Sciences Graduate Program Ohio State University ColumbusOH United States Department of Microbiology College of Arts and Sciences Ohio State University ColumbusOH United States Department of Microbial Infection and Immunity Ohio State University ColumbusOH United States Center for Perinatal Research The Abigail Wexner Research Institute Nationwide Children's Hospital Department of Pediatrics Ohio State University ColumbusOH United States Department of Civil and Environmental Engineering Case School of Engineering Case Western Reserve University ClevelandOH United States Department of Food Science and Technology Ohio State University ColumbusOH United States Infectious Diseases Institute Ohio State University ColumbusOH United States Soft Matter Materials Branch Materials and Manufacturing Directorate Air Force Research Laboratory Wright - Patterson AFBOH United States Department of Plant Pathology College of Food Agriculture and Environmental Science Ohio State University ColumbusOH United States Department of Anesthesiology & Pain Medicine Nationwide Children's Hospital ColumbusOH United States Airman Systems Directorate 711th Human Performance Wing Air Force Research Laboratory WPAFBOH United States Sustainability Institute Ohio State University ColumbusOH United States Department of Mechanical and Aerospace Engineering College of Engineering John Glenn College of Public Affairs Ohio State University ColumbusOH United States Department of Veterinary Biosciences College of Veterinary Medicine Ohio State University ColumbusOH United States Center of Microbiome Science Ohio State University ColumbusOH United States

Future human spaceflight beyond low-Earth orbit will bring substantial changes and new requirements to the development of fully sustainable, healthy indoor human environments across a range of gravitational, radiative, and thermal conditions. One key aspect is understanding (and potentially leveraging) microorganisms that must coexist with humans, plants, and animals in enclosed habitats (their microbiota or microbiomes). Modern, genome-resolved microbiome science provides an opportunity to better understand how we can utilize microbes to optimize space missions and protect human health and well-being long-term. Microorganisms will be critical to mission success due to their direct or indirect interactions with 1) humans, 2) other living systems (e.g., plant and animal life as a food source and for experimentation), and 3) the built environment. For example, the human gut microbiome is a complex community that has important implications for human health and performance that include mental health, nutrition intake, and immune system function. The health of plant microbiomes is also critical for sustainable, dependable, and nutritious food production. Humans, plants, and other living systems (e.g., animals used in experimentation) will also shed microbes into the built environment, which may impact human exposure, plant health, system integrity, and planetary protection from microbial contamination in both forward and reverse directions. Microbes from all three systems will interact, resulting in potentially important 'non-linear' system implications that must be understood for the overall long-term sustainability of hardware, crew, and other living systems. This paper discusses recent advances in technology that expand measurement capabilities to ultra-low-biomass samples and now allow for better understanding of microbial taxa, community structure and drivers, and functional capacity, which together will empower microbiome-optimized deep-space human exploration miss

关键词： Bacteria

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Zeeman polaritons as a platform for probing Dicke physics in condensed matter

arXiv

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arXiv 2024年

作者： Kritzell, T. Elijah Doumani, Jacques Asano, Tobias Yamada, Sota Tay, Fuyang Xu, Hongjing Yan, Han Katayama, Ikufumi Takeda, Jun Nevidomskyy, Andriy Nojiri, Hiroyuki Bamba, Motoaki Baydin, Andrey Kono, Junichiro Applied Physics Graduate Program Smalley-Curl Institute Rice University 6100 Main Street HoustonTX77005 United States Department of Electrical and Computer Engineering Rice University 6100 Main Street HoustonTX77005 United States Department of Physics Yokohama National University 79-5 Tokiwadai Hodogaya-ku Kanagawa Yokohama240-8501 Japan Department of Physics and Astronomy Rice University 6100 Main Street HoustonTX77005 United States Smalley-Curl Institute Rice University 6100 Main Street HoustonTX77005 United States Institute for Multidisciplinary Sciences Yokohama National University 79-5 Tokiwadai Hodogaya-ku Kanagawa Yokohama240-8501 Japan Institute for Materials Research Tohoku University 2-1-1 Katahira Aoba-ku Miyagi Sendai980-8577 Japan Rice Advanced Materials Institute Rice University 6100 Main Street HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University 6100 Main Street HoustonTX77005 United States

The interaction of an ensemble of two-level atoms and a quantized electromagnetic field, described by the Dicke Hamiltonian, is an extensively studied problem in quantum optics. However, experimental efforts to explore similar physics in condensed matter typically employ bosonic matter modes (e.g., phonons, magnons, and plasmons) that are describable as simple harmonic oscillators, i.e., an infinite ladder of equally spaced energy levels. Here, we examine ultrastrong coupling between a coherent light mode and an ensemble of paramagnetic spins, a finite-multilevel system, in Gd3Ga5O12. The electron paramagnetic resonance of Gd3+ ions is tuned by a magnetic field into resonance with a Fabry–Pérot cavity mode, resulting in the formation of spin–photon hybrid states, or Zeeman polaritons. We observe that the light–matter coupling strength, measured through the vacuum Rabi splitting, decreases with increasing temperature, which can be explained by the temperature-dependent population difference between the lower and higher-energy states, a trait of a finite-level system. This finding demonstrates that a spin–boson system is more compatible with the Dicke model and has advantages over boson–boson systems for pursuing experimental realizations of phenomena predicted for ultrastrongly coupled light–matter hybrids. Copyright © 2024, The Authors. All rights reserved.

关键词： Phonons

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Observation of the Magnonic Dicke Superradiant Phase Transition

arXiv

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arXiv 2024年

作者： Kim, Dasom Dasgupta, Sohail Ma, Xiaoxuan Park, Joong-Mok Wei, Hao-Tian Luo, Liang Doumani, Jacques Li, Xinwei Yang, Wanting Cheng, Di Kim, Richard H.J. Everitt, Henry O. Kimura, Shojiro Nojiri, Hiroyuki Wang, Jigang Cao, Shixun Bamba, Motoaki Hazzard, Kaden R.A. Kono, Junichiro Applied Physics Graduate Program Smalley–Curl Institute Rice University HoustonTX77005 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Ames National Laboratory AmesIA50011 United States Department of Physics and Astronomy Rice University HoustonTX77005 United States Department of Physics International Center of Quantum and Molecular Structures Materials Genome Institute Shanghai University Shanghai200444 China Department of Physics National University of Singapore 117551 Singapore Department of Physics and Astronomy Iowa State University AmesIA50011 United States Smalley–Curl Institute Rice University HoustonTX77005 United States DEVCOM Army Research Laboratory-South HoustonTX77005 United States Institute for Materials Research Tohoku University Sendai980-8577 Japan Department of Physics Yokohama National University Yokohama240-8501 Japan Department of Physics and Astronomy University of California DavisCA95616 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States

Two-level atoms coupled with single-mode cavity photons are predicted to exhibit a quantum phase transition when the coupling strength exceeds a critical value, entering a phase in which atomic polarization and photonic field are finite even at zero temperature and without external driving. However, this phenomenon, the superradiant phase transition (SRPT), is forbidden by a no-go theorem due to the existence of the diamagnetic term in the Hamiltonian. Here, we present spectroscopic evidence for a magnonic SRPT in ErFeO3, where the role of the photonic mode (two-level atoms) in the photonic SRPT is played by an Fe3+ magnon mode (Er3+ spins). The absence of the diamagnetic term in the Fe3+–Er3+ exchange coupling ensures that the no-go theorem does not apply. Terahertz and gigahertz magnetospectroscopy experiments revealed the signatures of the SRPT – a kink and a softening, respectively, of two spin–magnon hybridized modes at the critical point. Copyright © 2024, The Authors. All rights reserved.

关键词： Phase transitions

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Experimentally shock-induced melt veins in basalt: Improving the shock classification of eucrites

arXiv

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arXiv 2022年

作者： Ono, Haruka Kurosawa, Kosuke Niihara, Takafumi Mikouchi, Takashi Tomioka, Naotaka Isa, Junko Kagi, Hiroyuki Matsuzaki, Takuya Sakuma, Hiroshi Genda, Hidenori Sakaiya, Tatsuhiro Kondo, Tadashi Kayama, Masahiro Koike, Mizuho Sano, Yuji Murayama, Masafumi Satake, Wataru Matsui, Takafumi Planetary Exploration Research Center Chiba Institute of Technology 2-17-1 Tsudanuma Narashino Chiba275-0016 Japan Department of Applied Science Okayama University of Science 1-1 Ridaicho Kita-ku Okayama-shi700-0005 Japan The University Museum The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo113-0033 Japan 200 Monobe Otsu Kochi Nankoku783-8502 Japan Geochemical Research Center Graduate School of Science The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo113-0033 Japan Center for Advanced Marine Core Research Kochi University 200 Monobe Otsu Kochi Nankoku783-8502 Japan Research Center for Functional Materials National Institute for Materials Science 1-1 Namiki Ibaraki Tsukuba305-0044 Japan Earth–Life Science Institute Tokyo Institute of Technology 2-12-1 Ookayama Meguro-ku Tokyo152-8550 Japan Department of Earth and Space Science Graduate School of Science Osaka University 1-1 Machikaneyama Osaka Toyonaka560-0043 Japan Department of General Systems Studies Graduate School of Arts and Sciences The Univ. of Tokyo 3-8-1 Komaba Meguro-ku Tokyo153-8902 Japan Earth and Planetary Systems Science Program Graduate School of Advanced Science and Engineering Hiroshima University 1-3-1 Kagamiyama Higashi–Hiroshima Hiroshima739-8526 Japan Institute of Geo-Cosmology Chiba Institute of Technology 2-17-1 Tsudanuma Chiba Narashino275-0016 Japan

Basaltic rocks occur widely on the terrestrial planets and differentiated asteroids, including the asteroid 4 Vesta. We conducted a shock recovery experiment with decaying compressive pulses on a terrestrial basalt at Chiba Institute of Technology, Japan. The sample recorded a range of pressures, and shock physics modeling was conducted to add a pressure scale to the observed shock features. The shocked sample was examined by optical and electron microscopy, electron back-scattered diffractometry, and Raman spectroscopy. We found that localized melting occurs at a lower pressure (~10 GPa) than previously thought (>20 GPa). The shocked basalt near the epicenter represents "shock degree C" of a recently proposed classification scheme for basaltic eucrites and, as such, our results provide a pressure scale for the classification scheme. Finally, we estimated the total fraction of the basaltic eucrites classified as shock degree C to be ~15% by assuming the impact velocity distribution onto Vesta. © 2022, CC BY-NC-SA.

关键词： Basalt

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