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arXiv 2020年

作者： Tyner, Alexander C. Sur, Shouvik Puggioni, Danilo Rondinelli, James M. Goswami, Pallab Graduate Program in Applied Physics Northwestern University EvanstonIL60208 United States Department of Physics and Astronomy Northwestern University EvanstonIL60208 United States Department of Materials Science and Engineering Northwestern University IL60208 United States Northwestern Argonne Institute for Science and Engineering EvanstonIL60208 United States

Usually the quantum spin Hall states are expected to possess gapless, helical edge modes. Are there clean, non-interacting, quantum spin Hall states without gapless, edge modes? We show the generic, n-fold-symmetric, momentum planes of three-dimensional, stable Dirac semi-metals, which are orthogonal to the direction of nodal separation are examples of such generalized quantum spin Hall systems. We demonstrate that the planes lying between two Dirac points and the celebrated Bernevig-Zhang-Hughes model support identical quantized, non-Abelian Berry flux of magnitude 2π. Consequently, both systems exhibit spin-charge separation in response to electromagnetic, π-flux vortex. The Dirac points are identified as the unit-strength, monopoles of SO(5) Berry connections, describing topological quantum phase transitions between generalized, quantum spin Hall and trivial insulators. Our work identifies precise bulk invariant and quantized response of Dirac semimetals and shows that many two-dimensional higher-order topological insulators can be understood as generalized quantum spin Hall systems, possessing gapped edge states. Copyright © 2020, The Authors. All rights reserved.

关键词： Fruits

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A genuine correlation in piezoelectric properties of two-dimensional materials: A high-throughput computational study

arXiv

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arXiv 2020年

作者： Arlı, Cihan Kocabaş, Tugbey Çakır, Deniz Sevik, Cem Department of Materials Science and Engineering Institute of Graduate Program Eskisehir Technical University Eskiehir TR26555 Turkey Department of Physics and Astrophysics University of North Dakota Grand ForksND58202 United States Department of Mechanical Engineering Faculty of Engineering Eskisehir Technical University Eskiehir TR26555 Turkey

The rational design of two-dimensional piezoelectric materials has recently garnered increasing interest because of harnessing these materials in technological applications, including sensor technology, actuating devices, energy harvesting, and medical applications. Several materials possessing high piezoelectric response have been reported so far, but a high-throughput first-principles approach to estimate the piezoelectric potential of layered materials has not been performed yet. In this respect, we systematically investigated the piezoelectric (e11, d11) and elastic (C11 and C12) properties of 108 thermodynamically stable two-dimensional (2D) semiconductor materials by employing first-principle methods. Our calculations found a notable difference between the relaxed ion coefficients calculated with GGA and LDA functionals, indicating a strong exchange-correlation functional dependence. Nevertheless, both functionals yield the same trends for the elastic constants and piezoelectric coefficients. Our high-throughput approach demonstrates that the materials containing Group-V elements produce notably high piezoelectric strain constants, d11 > 40 pmV−1, and 42 of considered materials have the e11 coefficient higher than MoS2 insomuch as BrSSb has one of the largest d11 with a value of 503.6 pmV−1. Besides, we established simple empirical models to estimate the d11 coefficients by utilizing the relative ionic motion in the unit cell and the polarizability of the individual elements in the compounds. The proposed models, tested for both exchange-correlation functionals, are successful in estimating the piezoelectric constants of the studied materials with sufficient accuracy. Copyright © 2020, The Authors. All rights reserved.

关键词： Piezoelectricity

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Retraction notice to "Personal protective equipment-derived pollution during Covid-19 era: A critical review of ecotoxicology impacts, intervention strategies, and future challenges" [Sci. Total Environ. 887(2023) 164164]

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The science of the total environment 2025年 967卷 178758页

作者： Mehedi Hasan Abu Reza Md Towfiqul Islam Most Mastura Munia Farjana Jion Md Naimur Rahman Susmita Datta Peu Arnob Das A B M Mainul Bari Md Saiful Islam Subodh Chandra Pal Aznarul Islam Tasrina Rabia Choudhury Md Refat Jahan Rakib Abubakr M Idris Guilherme Malafaia Department of Disaster Management Begum Rokeya University Rangpur 5400 Bangladesh. Department of Disaster Management Begum Rokeya University Rangpur 5400 Bangladesh Department of Development Studies Daffodil International University Dhaka 1216 Bangladesh. Department of Geography and Environmental Science Begum Rokeya University Rangpur 5400 Bangladesh. Department of Agriculture Hajee Mohammad Danesh Science and Technology University Dinajpur 5200 Bangladesh. Department of Mechanical Engineering Rajshahi University of Engineering & Technology 6 Rajshahi 6204 Bangladesh. Department of Industrial and Production Engineering Bangladesh University of Engineering and Technology Dhaka 1000 Bangladesh. Department of Soil Science Patuakhali Science and Technology University Dumki Patuakhali 8602 Bangladesh. Department of Geography The University of Burdwan Bardhaman 713104 West Bengal India. Department of Geography Aliah University 17 Gorachand Road Kolkata 700 014 West Bengal India. Analytical Chemistry Laboratory Chemistry Division Atomic Energy Centre Dhaka (AECD) Bangladesh Atomic Energy Commission Dhaka 1000 Bangladesh. Department of Fisheries and Marine Science Faculty of Science Noakhali Science and Technology University Noakhali Bangladesh. Department of Chemistry College of Science King Khalid University Abha 62529 Saudi Arabia Research Center for Advanced Materials Science (RCAMS) King Khalid University Abha Saudi Arabia. Post-Graduation Program in Conservation of Cerrado Natural Resources Goiano Federal Institute Urutaí GO Brazil Post-Graduation Program in Ecology Conservation and Biodiversity Federal University of Uberlândia Uberlândia MG Brazil Post-Graduation Program in Biotechnology and Biodiversity Federal University of Goiás Goiânia GO Brazil.

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Double affinity ligands modified graphene enabled orientation-controllable cryo-EM sample preparation

Double affinity ligands modified graphene enabled orientatio...

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第七届全国冷冻电子显微学与结构生物学专题研讨会

作者：程航 Liming Zheng Nan Liu Jie Xu Congyuan Huang Ye Lu Hailin Peng Yanan Chen Hong-Wei Wang Ministry of Education Key Laboratory of Protein Sciences Beijing Advanced Innovation Center for Structural BiologySchool of Life SciencesTsinghua University Tsinghua-Peking Joint Center for Life Sciences Tsinghua University Center for Nanochemistry Beijing Science and Engineering Center for NanocarbonsBeijing National Laboratory for Molecular SciencesCollege of Chemistry and Molecular EngineeringPeking University Joint Graduate Program of Peking-Tsinghua-NIBS School of Life SciencesTsinghua University Academy for Advanced Interdisciplinary Studies Peking University School of Materials Science and Engineering Tianjin University Beijing Frontier Research Center for Biological Structures Tsinghua University

With the development of both hardwares and softwares of cryo-electron microscopy (cryo-EM),high- resolution structures of macromolecules have been increasingly ***,the robustness and generality of this technique are severely challenged by the air-water interface and preferred orientation issues during specimen preparation,which practically take plenty of efforts to overcome,especially for those hard *** we reported double-modified graphene (DMG) as the supporting material in cryo-EM sample preparation by covalently modified graphene membrane with two different affinity ligands,

关键词： DMG Double affinity ligands modified graphene enabled orientation-controllable cryo-EM sample preparation

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Physical characteristics of modified cassava flour wastewater at room temperature

Physical characteristics of modified cassava flour wastewate...

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International Conference on Food science and Technology 2018, ICFST 2018

作者： Yaqin, N. Al-Baarri, A.N. Legowo, A.M. Widayat Budihardjo, M.A. Program of Environmental Science School of Post-Graduate Studies Diponegoro University Semarang Indonesia Food Technology Department Faculty of Animal and Agricultural Sciences Diponegoro University Semarang Indonesia Chemical Engineering Department Faculty of Engineering Diponegoro University Semarang Indonesia Center of Research and Services Diponegoro University Semarang Indonesia Department of Environmental Engineering Faculty of Engineering Diponegoro University Indonesia

Cassava is an agricultural material that is considered as important raw resources in the industrial sector. The benefits are even greater after being modified using lactic acid bacteria. However, the mocaf industry often causes water and air pollution. Environmental problems arise after the fermentation process. Determination problems with lightness, TDS (Total Dissolved Solid), conductivity and pH analysis are required to measure the impact to the environment. This research was used waste water from mocaf during 3 days fermentation. The wastewater had the highest color level (Lightness) on initial day of fermentation at 83.7±3.73 and then decrease along the day of fermentation at the averages of 65.2±2.0. The highest TDS was resulted from the mocaf wastewater at a value of 1218 ± 4.6 ppm which continued to decline until day 4. The conductivity and pH showed a decrease along the day of fermentation. As conclusion, physical characteristic of wastewater from mocaf production could be analyzed specifically and determined through color, TDS, conductivity, and pH. © 2019 Published under licence by IOP Publishing Ltd.

关键词： Fermentation

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Alternation of Magnetic Anisotropy Accompanied by Metal-Insulator Transition in Strained Ultrathin Manganite Heterostructures

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Physical Review Applied 2021年第6期15卷 064019-064019页

作者： Masaki Kobayashi Le Duc Anh Masahiro Suzuki Shingo Kaneta-Takada Yukiharu Takeda Shin-ichi Fujimori Goro Shibata Arata Tanaka Masaaki Tanaka Shinobu Ohya Atsushi Fujimori Department of Electrical Engineering and Information Systems The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-8656 Japan Center for Spintronics Research Network The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-8656 Japan Institute of Engineering Innovation Graduate School of Engineering The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-8656 Japan PRESTO JST 4-1-8 Honcho Kawaguchi Saitama 332-0012 Japan Department of Physics The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-0033 Japan Materials Sciences Research Center Japan Atomic Energy Agency Sayo-gun Hyogo 679-5148 Japan Department of Applied Physics Tokyo University of Science Katsushika Tokyo 125-8585 Japan Quantum Matter Program Graduate School of Advanced Science and Engineering Hiroshima University Higashi-Hiroshima 739-8530 Japan Department of Applied Physics Waseda University Okubo Shinjuku Tokyo 169-8555 Japan

A fundamental understanding of the interfacial magnetic properties in ferromagnetic heterostructures is essential for utilizing ferromagnetic materials for spintronic device applications. Here, we investigate the interfacial magnetic and electronic structures of epitaxial single-crystalline LaAlO3(LAO)/La0.6Sr0.4MnO3(LSMO)/Nb:SrTiO3(Nb:STO) heterostructures with varying LSMO layer thicknesses, in which the magnetic anisotropy strongly changes with the LSMO thickness due to the delicate balance between strains originating from both the Nb:STO and LAO layers, using x-ray magnetic circular dichroism and photoemission spectroscopy. We successfully detect the clear change of the magnetic behavior of the Mn ions concomitant with the thickness-dependent metal-insulator transition. Our results suggest that the double-exchange interaction induces ferromagnetism in the metallic LSMO film under tensile strain caused by the STO substrate, while the superexchange interaction determines the magnetic behavior in the insulating LSMO film under compressive strain originating from the top LAO layer. The change in strain, depending on LSMO layer thickness, is confirmed by scanning transmission electron microscopy. Based on those findings, the formation of a magnetic dead layer near the LAO/LSMO interface is attributed to competition between the superexchange interaction via Mn 3d3z2−r2 orbitals under compressive strain and the double-exchange interaction via the 3dx2−y2 orbitals. These findings provide key aspects of ferromagnetic oxide heterostructures for the development of spintronic device applications.

关键词： Electronic structure Ferromagnetism Magnetic anisotropy Metal-insulator transition Spintronics Transition metal oxides Photoemission spectroscopy X-ray magnetic circular dichroism

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Photonic analog of bilayer graphene

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Physical Review B 2021年第21期103卷 214311-214311页

作者： Mourad Oudich Guangxu Su Yuanchen Deng Wladimir Benalcazar Renwen Huang Nikhil J. R. K. Gerard Minghui Lu Peng Zhan Yun Jing Graduate Program in Acoustics The Pennsylvania State University University Park Pennsylvania 16802 USA Université de Lorraine CNRS Institut Jean Lamour F-54000 Nancy France National Laboratory of Solid State Microstructures Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China School of Physics Nanjing University Nanjing 210093 China Department of Physics The Pennsylvania State University University Park Pennsylvania 16801 USA Department of Mechanical and Aerospace Engineering North Carolina State University Raleigh North Carolina 27695 USA Department of Materials Science and Engineering Nanjing University Nanjing Jiangsu 210093 China

Drawing inspiration from bilayer graphene, this paper introduces its photonic analog comprising two stacked graphenelike photonic crystals that are coupled in the near field through spoof surface plasmons. Beyond the twist degree of freedom that can radically alter the band structure of the bilayer photonic graphene, the photonic dispersion can be also tailored via the interlayer coupling which exhibits an exponential dependence on the distance between the two photonic crystals. We theoretically, numerically, and experimentally characterize the band structures of AA- and AB-stacked bilayer photonic graphene, as well as for twisted bilayer photonic graphene with even and odd sublattice exchange symmetries. Furthermore, we numerically predict the existence of magic angles in bilayer photonic graphene, which are associated with ultraflat bands resulting from interlayer hybridization. Finally, we demonstrate that the bilayer photonic graphene at a particular twist angle satisfying even sublattice exchange symmetry is a high-order photonic topological insulator. The proposed bilayer photonic graphene could constitute a useful platform for identifying new quantum materials and inspiring next-generation photonic devices with new degrees of freedom and emerging functionality.

关键词： Photonic crystals Plasmonics Surface plasmons

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Spectral evidence for unidirectional charge density wave in detwinned BaNi2As2

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Physical Review B 2023年第8期108卷 L081104-L081104页

作者： Yucheng Guo Mason Klemm Ji Seop Oh Yaofeng Xie Bing-Hua Lei Luca Moreschini Cheng Chen Ziqin Yue Sergey Gorovikov Tor Pedersen Matteo Michiardi Sergey Zhdanovich Andrea Damascelli Jonathan Denlinger Makoto Hashimoto Donghui Lu Chris Jozwiak Aaron Bostwick Eli Rotenberg Sung-Kwan Mo Rob G. Moore Junichiro Kono Robert J. Birgeneau David J. Singh Pengcheng Dai Ming Yi Department of Physics and Astronomy Rice University Houston Texas 77005 USA Advanced Light Source Lawrence Berkeley National Laboratory Berkeley California 94720 USA Department of Physics University of California Berkeley California 94720 USA Department of Physics and Astronomy University of Missouri Columbia Missouri 65211 USA Materials Science Division Lawrence Berkeley National Laboratory Berkeley California 94720 USA Department of Physics University of Oxford Oxford OX1 3PU United Kingdom Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston Texas 77005 USA Canadian Light Source Inc. 44 Innovation Boulevard Saskatoon SK S7N 2V3 Canada Department of Physics and Astronomy University of British Columbia Vancouver British Columbia V6T 1Z1 Canada Quantum Matter Institute University of British Columbia Vancouver British Columbia V6T 1Z4 Canada Max Planck Institute for Chemical Physics of Solids Nöthnitzer Straße 40 01187 Dresden Germany Stanford Synchrotron Radiation Lightsource SLAC National Accelerator Laboratory Menlo Park California 94025 USA Materials Science and Technology Division Oak Ridge National Laboratory Oak Ridge Tennessee 37831 USA Department of Electrical and Computer Engineering Rice University Houston Texas 77005 USA Smalley-Curl Institute Rice University Houston Texas 77005 USA Department of Materials Science and NanoEngineering Rice University Houston Texas 77005 USA Department of Chemistry University of Missouri Columbia Missouri 65211 USA

In the iron-based superconductors, unconventional superconductivity emerges in proximity to intertwined electronic orders consisting of an electronic nematic order and a spin density wave (SDW). Recently, BaNi2As2, like its well-known iron-based analog BaFe2As2, has been discovered to host a symmetry-breaking structural transition but coupled to a unidirectional charge density wave (CDW) instead of SDW, providing a novel platform to study intertwined orders. Here, through a systematic angle-resolved photoemission spectroscopy study combined with a detwinning B1g uniaxial strain, we identify distinct spectral evidence of band evolution due to the structural transition as well as CDW-induced band folding. In contrast to the nematicity and spin density wave in BaFe2As2, the structural and CDW order parameters in BaNi2As2 are observed to be strongly coupled and do not separate in the presence of uniaxial strain. Furthermore, no nematic band splitting is resolved above the structural transition. Our measurements point to a likely lattice origin of the CDW order in BaNi2As2.

关键词： Charge density waves Nematic phase transition Iron-based superconductors Angle-resolved photoemission spectroscopy

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Electron Transfer Enhanced by a Minimal Energetic Driving Force at the Organic-Semiconductor Interface

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Angewandte Chemie 2024年第37期136卷

作者： Hiroto Iwasaki Keisuke Fujimoto Koki Banno Qing-jun Shui Yutaka Majima Masaki Takahashi Seiichiro Izawa Laboratory for Materials and Structures Tokyo Institute of Technology 4259 Nagatsuta-cho Midori-ku Yokohama Kanagawa 226-8503 Japan Applied Chemistry Program Graduate School of Advanced Science and Engineering Hiroshima University 1-4-1 Kagamiyama Higashi-Hiroshima Hiroshima 739-8527 Japan Department of Applied Chemistry Faculty of Engineering Shizuoka University 3-5-1 Johoku Chuo-ku Hamamatsu Shizuoka 432-8561 Japan Precursory Research for Embryonic Science and Technology (PRESTO) Japan Science and Technology Agency (JST) 4-1-8 Honcho Kawaguchi Saitama 332-0012 Japan

The energetic driving force for electron transfer must be minimized to realize efficient optoelectronic devices including organic light-emitting diodes (OLEDs) and organic photovoltaics (OPVs). Exploring the dynamics of a charge-transfer (CT) state at an interface leads to a comprehension of the relationship between energetics, electron-transfer efficiency, and device performance. Here, we investigate the electron transfer from the CT state to the triplet excited state (T 1 ) in upconversion OLEDs with 45 material combinations. By analyzing the CT emission and the singlet excited-state emission from triplet–triplet annihilation via the dark T 1 , their energetics and electron-transfer efficiencies are extracted. We demonstrate that the CT→T 1 electron transfer is enhanced by the stronger CT interaction and a minimal energetic driving force (<0.1 eV), which is explained using the Marcus theory with a small reorganization energy of <0.1 eV. Through our analysis, a novel donor–acceptor combination for the OLED is developed and shows an efficient blue emission with an extremely low turn-on voltage of 1.57 V. This work provides a solution to control interfacial CT states for efficient optoelectronic devices without energy loss.

关键词： electron transfer Marcus theory organic optoelectronic devices organic light-emitting diodes organic photovoltaics

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Localized growth drives spongy mesophyll morphogenesis

arXiv

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arXiv 2022年

作者： Treado, John D. Roddy, Adam B. Théroux-Rancourt, Guillaume Zhang, Liyong Ambrose, Chris Brodersen, Craig Shattuck, Mark D. O’Hern, Corey S. Department of Mechanical Engineering & Materials Science Integrated Graduate Program in Physical and Engineering Biology Yale University New HavenCT06520 United States Institute of Environment Department of Biological Sciences Florida International University MiamiFL33199 United States University of Natural Resources and Life Sciences Vienna Department of Integrative Biology and Biodiversity Research Institute of Botany Vienna1180 Austria Department of Biology College of Arts and Science University of Saskatchewan SaskatoonS7N 5E2 Canada School of the Environment Yale University New HavenCT06520 United States Department of Physics Benjamin Levich Institute City College of New York New YorkNY10031 United States Department of Physics Department of Applied Physics Yale University New HavenCT06520 United States

The spongy mesophyll is a complex, porous tissue found in plant leaves that enables carbon capture and provides mechanical stability. Unlike many other biological tissues, which remain confluent throughout development, the spongy mesophyll must develop from an initially confluent tissue into a tortuous network of cells with a large proportion of intercellular airspace. How the airspace in the spongy mesophyll develops while the cells remain mechanically stable remains unknown. Here, we used computer simulations of deformable particles to develop a purely mechanical model for the development of the spongy mesophyll tissue. By stipulating that (1) cell perimeter grows only near voids, (2) cells both form and break adhesive bonds, and (3) the tissue pressure remains constant, the computational model was able to recapitulate the developmental trajectory of the microstructure of the spongy mesophyll observed in Arabidopsis thaliana leaves. Robust generation of pore space in the spongy mesophyll requires a balance of cell growth, adhesion, stiffness and tissue pressure to ensure cell networks remain both porous yet mechanically robust. The success of this mechanical model of tissue growth and porosity evolution suggests that simple physical principles can coordinate and drive the development of complex plant tissues like the spongy mesophyll. © 2022, CC BY.

关键词： Tissue

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