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Exploring multiple phases and first-order phase transitions in Kármán Vortex Street

Science China(Physics,Mechanics & Astronomy) 2024年第11期67卷 47-54页

作者： Xu Li Xing Xiang Tingting Xue Limin Wang Xiaosong Chen School of Systems Science and Institute of Nonequilibrium Systems Beijing Normal UniversityBeijing 100875China State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy ofSciencesBeijing 100190China School of Chemical Engineering University of Chinese Academy of SciencesBeijing 100049China

Kármán Vortex Street, a fascinating phenomenon of fluid dynamics, has intrigued the scientific community for a long time. Many researchers have dedicated their efforts to unraveling the essence of this intriguing flow pattern. Here, we apply the lattice Boltzmann method with curved boundary conditions to simulate flows around a circular cylinder and study the emergence of Kármán Vortex Street using the eigen microstate approach, which can identify phase transition and its order-parameter. At low Reynolds number, there is only one dominant eigen microstate W_(1) of laminar flow. At Re_(c)^(1)= 53.6, there is a phase transition with the emergence of an eigen microstate pair W^(2,3) of pressure and velocity fields. Further at Re_(c)^(2)= 56, there is another phase transition with the emergence of two eigen microstate pairs W^(4,5) and W^(6,7). Using the renormalization group theory of eigen microstate,both phase transitions are determined to be first-order. The two-dimensional energy spectrum of eigen microstate for W^(1), W^(2,3) after Re_(c)^(1), W^(4-7) after Re_(c)^(2) exhibit-5/3 power-law behavior of Kolnogorov's K41 theory. These results reveal the complexity and provide an analysis of the Kármán Vortex Street from the perspective of phase transitions.

关键词： Kármán Vortex Street first-order phase transition eigen microstate approach renormalization group theory of eigen microstate

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A brief review of preparation and applications of monolithic aerogels in atmospheric environmental purification

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Journal of Environmental Sciences 2025年第3期149卷 209-220页

作者： Linfeng Nie Shuangde Li Mengjie Cao Ning Han Yunfa Chen State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Key Laboratory of Science&Technology on Particle Materials Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China

Monolithic aerogels are promising candidates for use in atmospheric environmental purification due to their structural advantages,such as fine building block size together with high specific surface area,abundant pore structure,***,monolithic aerogels possess a unique monolithic macrostructure that sets them apart from aerogel powders and nanoparticles in practical environmental clean-up *** review delves into the available synthesis strategies and atmospheric environmental applications of monolithic aerogels,covering types of monolithic aerogels including SiO_(2),graphene,metal oxides and their combinations,along with their preparation *** particular,recent developments for VOC adsorption,CO_(2)capture,catalytic oxidation of VOCs and catalytic reduction of CO_(2)are ***,challenges and future opportunities for monolithic aerogels in the atmospheric environmental purification field are *** reviewprovides valuable insights for designing and utilizing monolithic aerogel-based functional materials.

关键词： Monolithic aerogel Environmental purification Catalysis Adsorption

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Ionic liquid-trimetallic electrocatalytic system for C–O bond cleavage in lignin model compounds and lignin under ambient conditions

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Nano Research 2024年第4期17卷 2420-2428页

作者： Guangyong Liu Yumiao Lu JunFeng Lu Yanlei Wang Shijing Liang Hongyan He Lilong Jiang National Engineering Research Center of Chemical Fertilizer Catalyst Fuzhou UniversityFuzhou 350002China CAS Key Laboratory of Green Process and Engineering State Key Laboratory of Multiphase Complex SystemsBeijing Key Laboratory of Ionic Liquids Clean ProcessInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China Longzihu New Energy Laboratory Zhengzhou Institute of Emerging Industrial TechnologyZhengzhou 450000China

Electrocatalytic depolymerization of lignin into value-added chemicals offers a promising technique to make biorefining ***,we report a robust trimetallic PdNiBi electrocatalyst for reductive C–O bond cleavage of different lignin model dimers and oxidized lignin under mild *** reduction reaction proceeds with complete substrate conversion and excellent yields toward monomers of phenols(80%–99%)and acetophenones(75%–96%)in the presence of an ionic liquid electrolyte with operational *** experimental investigations together with density functional theory(DFT)calculations reveal that the outstanding performance of the catalyst results from the synergistic effect of the metal elements,which facilitates the easier formation of a key Cαradical intermediate and the facile desorption of the as-formed products at the *** results open up new opportunities for lignin valorization through the green electrocatalytic approach.

关键词： electrocatalytic depolymerization lignin Ionic liquids density functional theory(DFT)calculation

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On the determination of particle impact breakage in selection function

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Particuology 2022年第6期20卷 117-132页

作者： Li Ge Wang Ruihuan Ge Xizhong Chen Process Systems Enterprise HammersmithLondonUK Department of Chemical and Biological Engineering University of SheffieldUK Process and Chemical Engineering School of EngineeringUniversity College CorkIreland

This paper presents a thorough study of particle impact breakage in selection function with a unified breakage *** impact mode and breakage pattern for particulate materials are classified based on a significant review of well-established impact *** was found that the lack of a unified breakage criterion to determine the breakage probability disables a direct comparison of particle breakage propensity from different impact loading *** literature breakage models to describe the breakage probability are reviewed where the advantage and drawback of these models are *** sourced literature breakage models are compared with the zeolite breakage datasets in a unified breakage criterion to evaluate the model performance.A novel computational modelling workflow for a milling process is proposed to provide a guidance in implementing the digital twin in milling process *** breakage probability models,*** selection functions are comprehensively assessed in population balance model to examine the model *** model simplicity and fidelity in the model assessment are specifically discussed and the value of digital twin in substantially reducing the experimental trials is highlighted.

关键词： Impact breakage Breakage criteria Breakage model assessment Selection function Population balance model Digital twin

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process control Principles for Scalable Electrolysis systems

Process Control Principles for Scalable Electrolysis Systems

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International Conference on Emerging Technologies and Factory Automation (ETFA)

作者： Julius Lorenz Anselm Klose Hannes Lange Tobias Kock Leon Urbas Chair of Process Control Systems TUD Dresden University of Technology Dresden Germany Process to Order Lab TUD Dresden University of Technology Dresden Germany Process Systems Engineering Group TUD Dresden University of Technology Dresden Germany

The scale up of hydrogen production to large scale production systems demands a structured approach to control these systems. With suitable control principles, optimization for operation can be achieved whilst maintaining flexibility. In this paper, existing control strategies are analyzed and compared for large scale electrolysis systems. It is argued, how modularization can enable the optimal distribution of set-points and enables the systems for capacity extension. An initial implementation in MATLAB is presented, showing the feasibility of the proposed power distribution concept.

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Flexible process control for Scalable Electrolysis systems

Flexible Process Control for Scalable Electrolysis Systems

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Electrical, Computer and Energy Technologies (ICECET), International Conference on

Large-scale water electrolysis systems are built from a multitude of stack units. These stack units have to be controlled during operation. The question arises how process control of the system can be designed in that way, that scalable, extendable but also optimal operation of the stack units becomes possible. To achieve this goal, existing process control strategies from literature are analyzed. The requirements resulting from the inherent numbering up of stack units are described and an approach for an adaptable optimized process control strategy considering the system properties is proposed. The proposed process control strategy is implemented in a modeled electrolysis system and evaluated regarding the stated criteria. The results could show, that the inherent modularization of electrolysis systems can be used in advantage for a scalable operation.

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Deposition of thin TiO_(2)films on fluorophlogopite particle surface by CVD in fluidized bed reactor to prepare silver pearlescent pigments

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Particuology 2024年第6期89卷 88-98页

作者： Ming Liu Guoqiang Shao Pengpeng Lv Jun Li Qingshan Zhu State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemical Engineering University of Chinese Academy of SciencesBeijing 100049China

Two critical parameters:Glossiness and chromaticity space of pearlescent pigments were evaluated based on crystallinity and grain *** the roughness and the vertical distance evolution along the surface of deposited TiO_(2)film are affected by the *** optimal crystallinity of TiO_(2)was deposited at the temperature of 350℃.The TiCl4 concentration effectively changed the grain ***,the high flow rate of fluidizing gas and optimal gas–solid ratio(<0.11 m^(3)/(kg h))restricted the change of TiCl_(4)concentrations in fluidized bed *** this case,the grain size of the deposited TiO_(2)film was about 55 *** on the grain size,the color of pearlescent pigments was adjusted by controlling the film thickness based on TiO_(2)***,the silver pearlescent pigment with high glossiness was prepared by chemical vapor deposition method in a fluidized bed reactor.

关键词： Fluidized bed chemical vapor deposition TiO_(2)film deposition Pearlescent pigment Free powder restrain Crystal growth

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Towards Usability of process Models for Co-Simulation-Based Operability Analysis of Modular Electrolysis Plants 29

Towards Usability of Process Models for Co-Simulation-Based ...

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29th IEEE International Conference on Emerging Technologies and Factory Automation, ETFA 2024

作者： Mock, Michael Viedt, Isabell Urbas, Leon Tud Dresden University of Technology Process Control Systems Dresden Germany Tud Dresden University of Technology Process to Order Lab Dresden Germany

ISBN: (纸本)9798350361230

The increasing need for simulation-based analysis along the life-cycle of modern process plants introduces new requirements and limitations in the development of simulation models. In the context of modular plants, according to VDI 2776, the distributed knowledge arises as a challenge in enabling system simulations. Co-simulation can enable a provider-independent simulation of chemical processes, but the co-simulation interfaces need further standardization to be efficiently integrated in the modular plant life-cycle. This paper works toward the usability of process models for co-simulation to support standardization efforts and make simulation models more usable and re-usable. To increase the usability of co-simulation in the process industry by working towards a common standard, two co-simulation standards, namely the Functional Mock-Up Interface and the CAPE-OPEN standard, are semantically linked. A use-case for a co-simulation-based operability analysis of a heterogeneous electrolysis plant is presented and necessary model requirements and interfaces are defined. Criteria to assess the compatibility of the model interfaces as a first step of a usability analysis are collected and presented. With the available requirements and interface specifications Functional Mock-Up Units can be created and the shown use-case can be carried out. Challenges regarding the potential integration of varying thermophysical properties have been pointed out and methods to overcome these challenges in the context of usability have been outlined. © 2024 IEEE.

关键词： Mockups

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Observer-based stabilization for discrete nonlinear semi-Markov jump singularly perturbed models with mode-switching delay

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Science China(Information Sciences) 2025年第4期68卷 389-390页

作者： Wenhai QI Runkun LI Ju H.PARK Zheng-Guang WU Huaicheng YAN School of Engineering Qufu Normal University Department of Electrical Engineering Yeungnam University Institute of Cyber-Systems and Control Zhejiang University Key Laboratory of Smart Manufacturing in Energy Chemical Process of Ministry of Education East China University of Science and Technology

Semi-Markov jump systems(S-MJMs) not only characterize hybrid systems but also address the limitations of Markov jump systems(MJMs) [1–3]. Due to their ability to exhibit multi-time-scale features, singularly perturbed models(SPMs) effectively model practical systems influenced by multiple time-scale phenomena [4]. In this study, the observer-based output feedback controller is asynchronous with the original system due to the time delay in the controller mode switching. A nonlinear plant with singularly perturbed parameters(SPPs) is represented using an interval type-2(IT2) fuzzy model [5].

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Formation control and path planning of multi-robot systems via large language models

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Science China(Information Sciences) 2025年第5期68卷 72-88页

作者： Dong XUE Xuanjie ZHOU Ming WANG Fangzhou LIU Key Laboratory of Smart Manufacturing in Energy Chemical Process Ministry of EducationEast China University of Science and Technology Research Institute of Intelligent Control and Systems School of Astronautics Harbin Institute of Technology

Existing path planning and coordination control methods for multi-robot systems(MRS) typically rely on predefined rules and rudimentary algorithms. However, these methods often struggle to adapt flexibly to complex environments and to adjust motion targets appropriately. To address this challenge, this study presents a large language model(LLM)-assisted framework. By integrating textual descriptions of complex motion constraints, robot information, and local environmental data as inputs, LLMs generate motion objectives and translate them into executable control commands for the robots, thereby achieving coordinated control and path planning. This framework facilitates the generation, maintenance, and reshaping of formations in MRSs during path planning, applicable to both obstacle-free and obstacle-avoidance environments. Simulation results demonstrate that LLM-based control strategies enhance the autonomy, adaptability, flexibility, and robustness of MRS by processing complex information, making intelligent decisions, adapting to environmental changes, and handling disturbances and uncertainties.

关键词： multi-robot systems formation control path planning obstacle avoidance large language models

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