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57th US Rock Mechanics/Geomechanics Symposium

作者： Fakher, Sherif Hassanin, Abdulla Tamer, Sara Eltohamy, Mohamed Abdelaty, Bassel Alsakkaf, Aseel Eldakar, Shams Petroleum and Energy Engineering The American University in Cairo Cairo Egypt Process and Product Development Unit The American University in Cairo Cairo Egypt Mechanical Engineering The American University in Cairo Cairo Egypt

ISBN: (纸本)9780979497582

One of the main solutions for carbon dioxide (CO2) emissions is carbon capture and storage. Carbon capture technologies, although abundant, are very costly and therefore their application is limited. This research introduces a novel technique for carbon capture that is extremely low in cost and applicable at atmospheric conditions with no pressurization requirements. This method is designed based on the utilization of waste material for sustainability and reduction in environmental impact. The selection of the material was the first step into determining the CO2 storage potential. The material selected was a fly ash produced as a byproduct of clinker manufacturing. The fly ash was then used in three different shapes including powder, cube, and hemi-spherical shape. Following this, the CO2 storage capacity was quantified based on the CO2 adsorption to the material. The shape was one of the most significant findings in this project as changing the shape and size of the fly ash resulted in a significant alteration of the adsorption capacity. The cycles of adsorption and desorption had no significant impact on the fly ash itself which indicated that it does not need to be replaced. This research introduces a small working model for a new design that can assist in carbon capture at ambient conditions. © 2023 57th US Rock Mechanics/Geomechanics Symposium. All Rights Reserved.

关键词： Fly ash

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Characterization of GaN-on-SiC Wafers using a Multi-Method Laser-Based Pump-Probe Technique 22

Characterization of GaN-on-SiC Wafers using a Multi-Method L...

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22nd InterSociety Conference on Thermal and Thermomechanical Phenomena in Electronic Systems, ITherm 2023

作者： Song, Yiwen Shoemaker, Daniel Kang, Kyuhwe Schuette, Michael Tweedie, James S. Sheppard, Scott T. Choi, Sukwon The Pennsylvania State University Department of Mechanical Engineering PA16802 United States Wolfspeed Rf Device and Process Development DurhamNC27703 United States

ISBN: (纸本)9798350321661

Gallium nitride (GaN) high electron mobility transistors (HEMTs) are key components of modern radio frequency (RF) power amplifiers. However, device self-heating negatively impacts both the performance and reliability of GaN HEMTs. Accordingly, laser-based pump-probe methods have been used to characterize the thermal resistance network of epitaxial material stacks that are used to fabricate HEMT structures. However, validation studies of these measurement results at the device level are lacking. In the present work, a GaN-on-SiC wafer was characterized using frequency-domain thermoreflectance and steady-state thermoreflectance techniques. The thermal conductivity of the GaN channel/buffer layer, SiC substrate, and the interfacial thermal boundary resistance at the GaN/SiC interface were determined. Results were validated by performing thermal imaging and modeling of a transmission line measurement (TLM) structure fabricated on the GaN-on-SiC wafer. © 2023 IEEE.

关键词： High electron mobility transistors

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Application of Plant-Based Coagulants and Their Mechanisms in Water Treatment:A Review

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Journal of Renewable Materials 2024年第4期12卷 667-698页

作者： Abderrezzaq Benalia Kerroum Derbal Zahra Amrouci Ouiem Baatache Amel Khalfaoui Antonio Pizzi Higher Normal School of Constantine Ali Mendjeli Nouvelle VilleConstantine25000Algeria Laboratory of Process Engineering for Sustainable Development and Health Products(GPDDPS) Department of Process EngineeringNational Polytechnic School of ConstantineConstantine25000Algeria Department of Environmental Engineering Laboratoire de Recherche sur le Médicament et le Développement Durable(ReMeDD)University of Salah Boubnider Constantine 3El Khroub25012Algeria Laboratory LIPE Faculty Process EngineeringUniversity of Constantine 3Ali Mendjeli Nouvelle VilleConstantine25000Algeria Laboratoire d’Etude et Recherche sur le Matériau Bois(LERMAB).Ecole Nationale Supérieure des Technologies et Industries du Bois(ENSTIB)—University of Lorraine Epinal88000France

This review describes the mechanisms of natural *** provides a good understanding of the two key processes of coagulation-flocculation:adsorption and charge neutralization,as well as adsorption and *** factors have influence the coagulation/flocculation process,including the effect of pH,coagulant dosage,coagulant type,temperature,initial turbidity,coagulation speed,flocculation speed,coagulation and flocculation time,settling time,colloidal particles,zeta potential,the effects of humic acids,and extraction density are *** bio-coagulants derived from plants are *** impact of organic coagulants on water quality,focusing on their effects on the physicochemical parameters of water,heavy metals removal,and bacteriological water quality,is *** methods of extraction and purification of plant-based coagulants,highlighting techniques such as solvent extraction and ultrasonic extraction,are *** also examines the parameters that influence these *** methods and principles of purification of coagulating agents,including dialysis,freeze-drying,ion exchange,electrophoresis,filtration,and centrifugation,are ***,it evaluates the sustainability of natural coagulants,focusing on the environmental,technical,and economic aspects of their *** the end of this review,the readers should have a comprehensive understanding of the mechanisms,selection,extraction,purification,and sustainability of plant-based natural coagulants in water treatment.

关键词： Bio-coagulants coagulating agents extraction water treatment

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Binderless low silica X zeolite for methane separation from binary CO2/CH4 biogas stream: A comprehensive experimental and computational study

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Journal of Industrial and engineering Chemistry 2025年 149卷 705-719页

作者： Yadav, Tushar R. Shrotri, Aadesh R. Kate, Pranjali N. Devasia, George Niphadkar, Prashant S. Mali, Nilesh A. Krishnamurty, Sailaja Bokade, Vijay V. Nandanwar, Sachin U. Catalysis and Inorganic Chemistry Division CSIR-National Chemical Laboratory Pune411 008 India Physical and Materials Chemistry Division CSIR-National Chemical Laboratory Pune411 008 India Chemical Engineering & Process Development Division CSIR-National Chemical Laboratory Pune411 008 India Ghaziabad201 002 India

This study presents the synthesis of binderless Na-LSX (B-Na-LSX) and binderless NaK-LSX (B-NaK-LSX). XRD, SEM, EDS, and N2 physisorption were used for characterization of samples. Computational modelling of prepared sorbent was performed for the fundamental understanding of zeolite topology and adsorption behaviour. The breakthrough experiments are used to evaluate the adsorption capacities on CO2/CH4 (40/60 vol%) binary biogas stream. The results were compared with commercial Na-LSX (C-Na-LSX). The breakthrough adsorption capacity of B-Na-LSX was 3.08 mmol g−1 and 0.29 mmol g−1 of CO2 and CH4, respectively, at 300 K and 1 bar. CO2 sorption capacity of B-Na-LSX was ∼11 % and ∼17 % higher than B-NaK-LSX (2.77 mmol g−1) and C-Na-LSX (2.56 mmol g−1), respectively. DFT study reveals that the higher adsorption of CO2 over CH4 was attributed to higher charge transfer from CO2 to zeolite framework. Dual-bed six-step Pressure Swing Adsorption (PSA) was performed on B-Na-LSX at 6 bar. ∼232 cycles were run with above 98 % of CH4 purity and ∼74 % of recovery. The life-cycle test of sorbent was studied. It was implied that the designed sorbent is effective to produce the high purity of CH4 and can be utilized for a longer period for CH4 production. © 2025 The Korean Society of Industrial and engineering Chemistry

关键词： Gas adsorption

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Metagenomic analysis revealing the metabolic role of microbial communities in the free amino acid biosynthesis of Monascus rice vinegar during fermentation

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Food Science and Human Wellness 2024年第4期13卷 2317-2326页

作者： Hang Gao Jian Zhang Li Liu Lijun Fu Yan Zhao Germán Mazza Xin Zhang Beijing Academy of Food Sciences 100068 BeijingChina Institute for Research and Development in Process Engineering Biotechnology and Alternative Energies(PROBIENCONICET-UNCo)8300 NeuquénArgentina

Free amino acid(FAA)is the important component of vinegar that infl uences quality perception and consumer *** is one of the major metabolites produced by microorganisms;however,the microbial metabolic network on FAA biosynthesis remains *** metagenomic analysis,this work aimed to elucidate the roles of microbes in FAA biosynthesis during Monascus rice vinegar *** profiles from functional analyses showed 14 dominant genera with high contributions to the metabolism *** metabolic network for FAA biosynthesis was then constructed,and the microbial distribution in different metabolic pathways was *** results revealed that 5 functional genera were closely involved in FAA *** study illuminated the metabolic roles of microorganisms in FAA biosynthesis and provided crucial insights into the functional attributes of microbiota in vinegar fermentation.

关键词： Monascus rice vinegar Metagenomic analysis Free amino acid synthesis Metabolic pathway Microbial distribution

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Anchoring Pt nanoparticles and Ti_(3)C_(2)T_(x)MXene nanosheets on CdS nanospheres as efficient synergistic photocatalysts for hydrogen evolution

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Science China(Technological Sciences) 2022年第12期65卷 3020-3028页

作者： JIANG JiZhou XIONG ZhiGuo WANG HaiTao XIANG Kun WU PingXiu ZOU Jing School of Environmental Ecology and Biological Engineering School of Chemistry and Environmental EngineeringKey Laboratory of Green Chemical Engineering Process of Ministry of EducationEngineering Research Center of Phosphorus Resources Development and Utilization of Ministry of EducationNovel Catalytic Materials of Hubei Engineering Research CenterWuhan Institute of TechnologyWuhan 430205China Semiconductor Electronic Special Gas of Hubei Engineering Research Center Jingzhou 434000China

The development of a new-fashioned functional nanomaterial with an outstanding photocatalytic hydrogen evolution reaction(HER)activity under visible-light irradiation is a sustainable and promising strategy to cope with the increasingly serious global energy ***,an advanced ternary photocatalytic HER catalyst,in which the Pt nanoparticles and Ti_(3)C_(2)T_(x)nanosheets are synchronously anchored on the surface of CdS nanospheres(Ti_(3)C_(2)T_(x)/Pt@CdS),is elaborately constructed via acid etching,sel-freduction,and solvothermal ***,the synergistic promoting effect between Ti_(3)C_(2)T_(x)and Pt on the charge transfer of CdS effectively hinders the backtransfer of electrons to recombine with holes,resulting in a high-effective utilization of photoexcited *** obtained Ti_(3)C_(2)T_(x)/Pt@CdS possesses a superior photocatalytic HER activity compared to that of single active component *** work demonstrates the great potential of MXene materials in constructing high performance photocatalysts.

关键词： Pt nanoparticles Ti_(3)C_(2)T_(x)MXene CdS nanospheres synergistic catalytic effect photocatalytic HER

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High-performance Si-Containing anode materials in lithium-ion batteries: A superstructure of Si@Co-NC composite works effectively

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Green Energy & Environment 2022年第1期7卷 116-129页

作者： Qiongguang Li Yanhong Wang Jing Yu Menglei Yuan Qiangqiang Tan Ziyi Zhong Fabing Su School of Chemical Engineering University of Chinese Academy of Sciences100049BeijingChina State Key Laboratory of Multiphase Complex Systems CAS Key Laboratory of Green Process EngineeringInstitute of Process EngineeringChinese Academy of SciencesBeijing100190China Zhongke Langfang Institute of Process Engineering Fenghua Road No 1Langfang Economic&Technical Development ZoneHebei Province065001China College of Engineering Guangdong Technion Israel Institute of Technology(GTIIT)241 Daxue RoadJinping DistrictShantou515063China Technion Israel Institute of Technology(IIT) Haifa32000Israel Institute of Industrial Chemistry and Energy Technology Shenyang University of Chemical TechnologyShenyang110142China

To mitigate the massive volume expansion of Si-based anode during the charge/discharge cycles,we synthesized a superstructure of Si@Co±NC composite via the carbonization of zeolite imidazolate frameworks incorporated with Si *** Si@Co±NC is comprised of Sinanoparticle core and N-doped/Co-incorporated carbon shell,and there is void space between the core and the *** using as anode material for LIBs,Si@Co±NC displayed a super performance with a charge/discharge capacity of 191.6/191.4 mA h g^(-1)and a coulombic efficiency of 100.1%at 1000 mA g^(-1)after 3000 cycles,and the capacity loss rate is 0.022%per cycle *** excellent electrochemical property of Si@Co±NC is because its electronic conductivity is enhanced by doping the carbon shell with N atoms and by incorporating with Co particles,and the pathway of lithium ions transmission is shortened by the hollow structure and abundant mesopores in the carbon ***,the volume expansion of Si nanoparticles is well accommodated in the void space and suppressed by the carbon host *** work shows that,through designing a superstructure for the anode materials,we can synergistically reduce the work function and introduce the confinement effect,thus significantly enhancing the anode materials’electrochemical performance in LIBs.

关键词： Confinement effect Work function regulation Doping Hollow core-shell structure Si anode

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Characterization of dielectric barrier discharge reactor with nanobubble application for industrial water treatment and depollution

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South African Journal of Chemical engineering 2022年 40卷 246-257页

作者： Luvita, V. Sugiarto, A.T. Bismo, S. Intensification Process Laboratory Chemical Engineering Faculty of Engineering Universitas Indonesia Kampus UI Depok 16424 Indonesia Technical Implementation for Instrumentation Development Unit – BRIN Bandung Indonesia

The performance of wet and advanced oxidation processes is considered to have many weaknesses concerning ozone and peroxone, specifically their characteristics against persistent organic compounds, as well as nitrogen-ammonia and amine-phenolic-based compounds. This is necessary to increase and improve the performance of the utilized plasma reactor, specifically the finer bubble size, as well as the intensity and reactivity (chemical reaction barriers) of the reacting species, to have a smaller impact on mass transfer or diffusivity in polar solvents. Therefore, this study aims to analyze the hydrodynamic characterization and several tests of the most important physicochemical parameters of a prototype nanobubble plasma ozone reactor, which is a reaction vehicle integrating the synergistic effect of a cold field. This reactor was used with a nanobubble-producing nozzle in a PFR (plug flow reactor), to increase the absorption ability of the plasma by water. The results showed that the oxygen and ozone solubilities, H₂O₂ production, and the synergy of these species were strongly influenced by the electric voltage, feed gas flow rate, and the O₂ purity used in the injection system. © 2022

关键词： Dielectric barrier discharge Nanobubble Ozone Plasma Reactor

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Advanced carbon nitride-based single-atomphotocatalysts

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SusMat 2024年第5期4卷 70-113页

作者： Zifan Zhang Kun Xiang Haitao Wang Xin Li Jing Zou Guijie Liang Jizhou Jiang School of Environmental Ecology and Biological Engineering School of Chemistry and Environmental EngineeringKey Laboratory of Green Chemical Engineering Process of Ministry of EducationEngineering Research Center of Phosphorus Resources Development and Utilization of Ministry of EducationNovel Catalytic Materials of Hubei Engineering Research CenterWuhan Institute of TechnologyWuhanChina Institute of Biomass Engineering Key Laboratory of Energy Plants Resource and UtilizationMinistry of Agriculture and Rural AffairsSouth China Agricultural UniversityGuangzhouChina Hubei Key Laboratory of Low Dimensional Optoelectronic Materials and Devices Hubei University of Arts and ScienceXiangyangChina

Single-atom catalysts(SACs)have rapidly become a hot topic in photocatalytic research due to their unique physical and chemical properties,high activity,and high *** many semiconductor carriers,the special structure of carbon nitride(C3N4)perfectly meets the substrate requirements for stabi-lizing SACs;they can also compensate for the photocatalytic defects of C3N4 materials by modifying energy bands and electronic ***,devel-oping advanced C3N4-based SACs is of great *** this review,we focus on elucidating efficient preparation strategies and the burgeoning photo-catalytic applications of C3N4-based *** also outline prospective strategies for enhancing the performance of SACs and C3N4-based SACs in the future.A comprehensive array of methodologies is presented for identifying and char-acterizing C3N4-based *** includes an exploration of potential atomic catalytic mechanisms through the simulation and regulation of atomic catalytic behaviors and the synergistic effects of single or multiple ***,a forward-looking perspective is adopted to contemplate the future prospects and challenges associated with C3N4-based *** encompasses considerations,such as atomic loading,regulatory design,and the integration of machine learn-ing *** is anticipated that this review will stimulate novel insights into the synthesis of high-load and durable SACs,thereby providing theoretical groundwork for scalable and controllable applications in the field.

关键词： atomic catalytic mechanism carbon nitride improvement strategies photocatalytic applications single-atom catalysts

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Removal enhancement of persistent basic fuchsin dye from wastewater using an eco-friendly, cost-effective Fenton process with sodium percarbonate and waste iron catalyst

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Environmental Science and Pollution Research 2024年第31期31卷 43673-43686页

作者： Aouni, Saoussen Imene Ghodbane, Houria Merouani, Slimane Lakikza, Imane Boublia, Abir Yadav, Krishna Kumar Djelloul, Chawki Albakri, Ghadah Shukri Elboughdiri, Noureddine Benguerba, Yacine Laboratory of Physics for Matter and Radiation Mohamed Cherif Messadia-Souk Ahras University P.O. Box 1553 Souk Ahras41000 Algeria Laboratory of Environmental Process Engineering Department of Chemical Engineering Faculty of Process Engineering University Salah Boubnider-Constantine 3 P.O. Box 72 Constantine25000 Algeria Département de Génie des Procédés Faculté de Technologie Université Ferhat ABBAS Sétif-1 Sétif19000 Algeria Faculty of Science and Technology Madhyanchal Professional University Ratibad Bhopal462044 India Environmental and Atmospheric Sciences Research Group Scientific Research Center Al-Ayen University Thi-Qar Nasiriyah64001 Iraq Laboratory of Reaction Engineering Faculty of Mechanical Engineering and Process Engineering USTHB Algiers Algeria Department of Teaching and Learning College of Education and Human Development Princess Nourah bint Abdulrahman University P.O. Box 84428 Riyadh11671 Saudi Arabia Chemical Engineering Department College of Engineering University of Ha’il Ha’il81441 Saudi Arabia Chemical Engineering Process Department National School of Engineers Gabes University of Gabes Gabes6029 Tunisia Ferhat Abbas Setif 1 University Setif Algeria

Abstract: In this comprehensive investigation, we evaluate the efficacy of the Fenton process in degrading basic fuchsin (BF), a resistant dye. Our primary focus is on the utilization of readily available, environmentally benign, and cost-effective reagents for the degradation process. Furthermore, we delve into various operational parameters, including the quantity of sodium percarbonate (SPC), pH levels, and the dimensions of waste iron bars, to optimize the treatment efficiency. In the course of our research, we employed an initial SPC concentration of 0.5 mM, a pH level of 3, a waste iron bar measuring 3.5 cm in length and 0.4 cm in diameter, and a processing time of 10 min. Our findings reveal the successful elimination of the BF dye, even when subjected to treatment with diverse salts and surfactants under elevated temperatures and acidic conditions (pH below 3). This underscores the robustness of the Fenton process in purifying wastewater contaminated with dye compounds. The outcomes of our study not only demonstrate the efficiency of the Fenton process but highlight its adaptability to address dye contamination challenges across various industries. Critically, this research pioneers the application of waste iron bars as a source of iron in the Fenton reaction, introducing a novel, sustainable approach that enhances the environmental and economic viability of the process. This innovative use of recycled materials as catalysts represents a significant advancement in sustainable chemical engineering practices. Graphical abstract: (Figure presented.). © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024.

关键词： Iron

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