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A brief review of preparation and applications of monolithic aerogels in atmospheric environmental purification

Journal of Environmental sciences 2025年第3期149卷 209-220页

作者： Linfeng Nie Shuangde Li Mengjie Cao Ning Han Yunfa Chen State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Key Laboratory of Science&Technology on Particle Materials Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China

Monolithic aerogels are promising candidates for use in atmospheric environmental purification due to their structural advantages,such as fine building block size together with high specific surface area,abundant pore structure,***,monolithic aerogels possess a unique monolithic macrostructure that sets them apart from aerogel powders and nanoparticles in practical environmental clean-up *** review delves into the available synthesis strategies and atmospheric environmental applications of monolithic aerogels,covering types of monolithic aerogels including SiO_(2),graphene,metal oxides and their combinations,along with their preparation *** particular,recent developments for VOC adsorption,CO_(2)capture,catalytic oxidation of VOCs and catalytic reduction of CO_(2)are ***,challenges and future opportunities for monolithic aerogels in the atmospheric environmental purification field are *** reviewprovides valuable insights for designing and utilizing monolithic aerogel-based functional materials.

关键词： Monolithic aerogel Environmental purification Catalysis Adsorption

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Multi-Scale Time Series Segmentation Network Based on Eddy Current Testing for Detecting Surface Metal Defects

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IEEE/CAA Journal of Automatica Sinica 2025年第3期12卷 528-538页

作者： Xiaorui Li Xiaojuan Ban Haoran Qiao Zhaolin Yuan Hong-Ning Dai Chao Yao Yu Guo Mohammad S.Obaidat George Q.Huang the School of Intelligence Science and Technology University of Science and Technology Beijing the Beijing Advanced Innovation Center for Materials Genome Engineering the Key Laboratory of Intelligent Bionic Unmanned Systems and the Institute of Materials Intelligent Technology Liaoning Academy of Materials IEEE the Department of Computer Science Hong Kong Baptist University the School of Computer and Communication Engineering Key Laboratory of Advanced Materials and Devices for Post-Moore Chips Ministry of Education University of Science and Technology Beijing the Beijing Advanced Innovation Center for Materials Genome Engineering University of Science and Technology Beijing the School of Computer and Communication Engineering University of Science and Technology Beijing the King Abdullah Ⅱ School of Information Technology The University of Jordan the Department of Computational Intelligence the School of Computing SRM University the School of Engineering The Amity University The Hong Kong Polytechnic University

In high-risk industrial environments like nuclear power plants, precise defect identification and localization are essential for maintaining production stability and safety. However, the complexity of such a harsh environment leads to significant variations in the shape and size of the defects. To address this challenge, we propose the multivariate time series segmentation network(MSSN), which adopts a multiscale convolutional network with multi-stage and depth-separable convolutions for efficient feature extraction through variable-length templates. To tackle the classification difficulty caused by structural signal variance, MSSN employs logarithmic normalization to adjust instance distributions. Furthermore, it integrates classification with smoothing loss functions to accurately identify defect segments amid similar structural and defect signal subsequences. Our algorithm evaluated on both the Mackey-Glass dataset and industrial dataset achieves over 95% localization and demonstrates the capture capability on the synthetic dataset. In a nuclear plant's heat transfer tube dataset, it captures 90% of defect instances with75% middle localization F1 score.

关键词： Eddy current testing nondestructive testing semantic segmentation time series analysis

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Predicting Knowledge Graph Updates from Edit Histories 26th

Predicting Knowledge Graph Updates from Edit Histories

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26th International Conference on Information Integration and Web Intelligence, iiWAS 2024

作者： Okura, Maiki Amagasa, Toshiyuki Graduate School of Systems and Information Engineering University of Tsukuba Tsukuba Japan Center for Computational Science University of Tsukuba Ibaraki Tsukuba Japan

ISBN: (纸本)9783031780899

Knowledge graphs (KGs) are inherently incomplete and require continuous maintenance to keep up with the latest status of the target domain. Various studies have been conducted to automate this maintenance, but it still relies heavily on human labor. To alleviate such a burden, predicting updates in KGs is useful for maintaining KGs. In this study, we focus on predicting which entities to be updated in KGs containing many entities. Our basic idea is to exploit the KG’s structural information and the edit history, making it possible to predict entities likely to be updated in the next time interval. We have constructed a dataset including edit history based on Wikidata, a general-purpose knowledge graph, and developed a method to predict entities that will be updated based on link relations and edit history, and confirmed their usefulness through experiments. © The Author(s), under exclusive license to Springer Nature Switzerland AG 2025.

关键词： Edit history Knowledge graph Update prediction

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Stability and bifurcation analysis of delayed tri-trophic food chain model in poisoned environment with fear effect and additional food

Stability and bifurcation analysis of delayed tri-trophic fo...

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作者： Ramasamy, Sivasamy Banjerdpongchai, David Park, PooGyeon Center of Excellence in Intelligent Control Automation of Process Systems Department of Electrical Engineering Faculty of Engineering Chulalongkorn University Bangkok Thailand Department of Electrical Engineering Pohang University of Science and Technology Pohang Korea Republic of

One of the most important goals of theoretical ecologists is to find a strategy for controlling the chaos in ecological models to maintain healthy ecosystems. We investigate the influence of fear and the supply of additional food to predators in a delayed tri-trophic food chain model, where interference among the species is determined by Holling type-II functional response. The proposed model incorporates the fact that the growth rates of prey and middle predators are decreased due to the fear of middle and special predators, respectively. The additional food is supplied to both predators by either nature or external agencies. Furthermore, the poisoned prey in the predator's environment is taken into account. In the proposed model, we use two time delays: one for the growth term of the middle predator and another for the gestation delay of the special predator. We determine the conditions for the existence of ecologically feasible equilibrium points and their local and global stability. In addition, we establish the conditions for the existence of Hopf bifurcation around interior equilibrium to seek periodic behavior in nondelayed and delayed models. Numerical investigations are performed to justify the proposed theoretical findings through phase portraits, time series of solutions, and bifurcation diagrams. We observe that the chaotic dynamics of a tri-trophic food chain model can be controlled by the proper choice of the fear effect and by supplying additional food parameters. As a result, our findings provide more ecological insights into the dynamics of the delayed tri-trophic food chain model with the fear effect and additional food supply. © 2023 John Wiley & Sons, Ltd.

关键词： Hopf bifurcation

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Synthesis of interfacial electric field-enhanced CdS/CdxZn1-xS/ZnO ternary heterojunction by lye dissolution etching mechanism for photocatalytic H2 production and CO2 reduction

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材料科学技术（英文版） 2025年第1期204卷 152-165页

作者： Qi Li Shengchao Yang Yufan Huang Yuwei Liang Chunling Hu Min Wang Zhiyong Liu Yanlong Tai Jichang Liu Yongsheng Li School of Chemistry and Chemical Engineering Shihezi University/Key Laboratory of Green Process for Chemical Engineering/Key Laboratory for Chemical Materials of Xinjiang Uygur Autonomous Region/Engineering Center for Chemical Materials of Xinjiang BingtuanShihezi UniversityShihezi 832003China Shanghai Institute of Ceramics Chinese Academy of SciencesShanghai 200050China School of Chemistry and Chemical Engineering Shihezi University/Key Laboratory of Green Process for Chemical Engineering/Key Laboratory for Chemical Materials of Xinjiang Uygur Autonomous Region/Engineering Center for Chemical Materials of Xinjiang BingtuanShihezi UniversityShihezi 832003China Key Laboratory of Human-Machine Intelligence-Synergy Systems of Chinese Academy of Sciences(CAS) Shenzhen Institutes of Advanced TechnologyShenzhen 518055China School of Chemistry and Chemical Engineering Shihezi University/Key Laboratory of Green Process for Chemical Engineering/Key Laboratory for Chemical Materials of Xinjiang Uygur Autonomous Region/Engineering Center for Chemical Materials of Xinjiang BingtuanShihezi UniversityShihezi 832003China Lab of Low-Dimensional Materials Chemistry Key Laboratory for Ultrafine Materials of Ministry of Education School of Materials Science and Engineering East China University of Science and Technology ShanghaiShanghai 200237China

The difficulty in fabricating a multifaceted composite heterojunction system based on CdxZn1-xS limits the enhancement of photocatalytic *** the present scrutiny,novel ZnO/CdxZn1-xS/CdS com-posite heterojunctions are successfully prepared by the alkaline dissolution etching *** internal electric field at the interface of Ⅰ-type and Z-scheme heterojunction improved the effective charge *** ZC 8 sample exhibits excellent photocatalytic performance and the H2 production efficiency is 15.67 mmol g-1 h-1 with good stability up to 82.9％in 24-hour *** performance of CH4 and CO capacity in the CO2RR process is 3.47 μmol g-1 h-1 and 23.5 μmol g-1 h-1,*** photogener-ated accelerated charge transport is then examined in detail by in situ X-ray photoelectron spectroscopy(ISXPS)and density functional theory(DFT)*** work presents a new idea for the synthe-sis of CdxZni-xS solid-solution-based materials and provides a solid reference for the detailed mechanism regarding the electric field at the heterojunction interface.

关键词： Photocatalysis Interface electric field Composite heterostructure Photocatalytic mechanism CdxZn1-xS solid-solution

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engineering of Fe d-band center in Fe_(3)O_(4)/CeO_(2)hetero-nanoparticles via orbital coupling for high-efficiency oxygen reduction electrocatalysis

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Nano Research 2025年第1期18卷 129-139页

作者： Jiayi Liu Jingwen Yin Yingzi Lin Mingxin Pang Huan Pang Songtao Zhang Lin Xu Jun Yang Yawen Tang Jiangsu Key Laboratory of New Power Batteries Jiangsu Collaborative Innovation Center of Biomedical Functional MaterialsSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing 210023Chin a 2 State Key Laboratory of Multiphase Complex Systems Center of MesoscienceInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou 225009China Testing Center Yangzhou UniversityYangzhou 225009China

The deliberate engineering of the d-band center of metal site represents an effective strategy to boost the intrinsic electrocatalytic performance toward the oxygen reduction reaction(ORR).Herein,following a heterointerfaceinduced orbital coupling rationale,we report a judicious design of an efficient ORR electrocatalyst consisting of Fe_(3)O_(4)/CeO_(2)hetero-nanoparticles in-situ encased into N-doped carbon nanofibers(abbreviated as Fe_(3)O_(4)/CeO_(2)@N-CNFs hereafter).The theoretic calculations uncover that the Fe_(3)O_(4)/CeO_(2)heterointerface-triggered orbital coupling can cause the down shift of the d-band center positions of Fe sites,which leads to the weakened chemisorption of oxygenated groups and lowered energy barrier for the potential-determining step,ultimately dramatically boosting the ORR intrinsic *** a consequence,the well-designed Fe_(3)O_(4)/CeO_(2)@N-CNFs display admirable ORR activity with a half-wave potential of 0.84 V and outstanding structural/electrochemical stability in an alkaline electrolyte,surpassing the commercial Pt/C benchmark and a majority of recently reported Fe_(3)O_(4)-based *** encouragingly,the Fe_(3)O_(4)/CeO_(2)@N-CNFsincorporated Zn-air battery outperforms the Pt/C-assembled counterpart with higher power density,larger energy density,and excellent cycling stability,serving as a competent candidate for ORR-involved renewable energy *** study offers an innovative approach for the rational manipulation of the d-band center and interfacial electron behavior of active sites toward the optimization of electrocatalytic performance.

关键词： hetero-nanoparticles electrospinning interfacial engineering orbital coupling oxygen reduction reaction

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Dynamic Self-Triggered Control for Nonzero-Sum Games of Unknown Nonlinear Constrained systems via Generalized Fuzzy Hyperbolic Models

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IEEE Transactions on systems, Man, and Cybernetics: systems 2025年第5期55卷 3506-3518页

作者： Liu, Fan Su, Hanguang Zhang, Huaguang Luo, Biao Wang, Jiawei Northeastern University School of Information Science and Engineering Shenyang110004 China Northeastern University School of Information Science and Engineering State Key Laboratory of Synthetical Automation for Process Industries Shenyang110004 China Central South University School of Automation Changsha410083 China Northeastern University National Frontiers Science Center for Industrial Intelligence and Systems Optimization Shenyang110819 China

In this article, a novel adaptive dynamic programming algorithm is devised to handle the multiplayer nonzero-sum (NZS) games of completely unknown nonlinear systems, subject to state and input constraints under the dynamic self-triggered mechanism. Initially, in order to eliminate the demand for system dynamics, a generalized fuzzy hyperbolic model based identifier is established, which only relies on input-output data. Then, the equivalent transformation of the reconstructed system is implemented by virtue of barrier functions. With the aid of the nonquadratic utility function, the Hamilton-Jacobi equation of the NZS game is derived. After that, an adaptive critic scheme with experience replay is employed to acquire the Nash equilibrium solution. Furthermore, a novel dynamic self-triggered rule is proposed with the dead-zone operation, which not only significantly reduces source consumption but also overcomes the implementation difficulty of monitoring hardware in the event-triggered mechanism. Moreover, the stability of the system and the uniform ultimate boundedness of the critic weights are guaranteed. Ultimately, two simulation examples are given to validate the feasibility of the developed method. © 2025 IEEE.

关键词： Adaptive algorithms

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Deep transfer learning technique to detect white blood cell classification in regular clinical practice using histopathological images

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Multimedia Tools and Applications 2025年第9期84卷 5699-5723页

作者： Davamani, K. Anita Jawahar, Malathy Anbarasi, L. Jani Ravi, Vinayakumar Al Mazroa, Alanoud Robin, C. R. Rene Computer Science and Engineering Sathyabama Institute of Science and Technology Chennai India Leather Process Technology Division CSIR-Central Leather Research Institute Chennai India School of Computing Science and Engineering Vellore Institute of Technology Vellore India Computer Science and Engineering Sri Sairam Engineering College Sirukalathur India Center for Artificial Intelligence Prince Mohammad Bin Fahd University Khobar Saudi Arabia Department of Information Systems College of Computer and Information Sciences Princess Nourah bint Abdulrahman University Riyadh11671 Saudi Arabia

Leukemia, a malignant disease characterized by the rapid proliferation of specific types of white blood cells (WBC), has prompted increased interest in leveraging automatic WBC classification system. This study presents the design of a robust WBC classification system, integrating deep learning with microscopic image analysis. The proposed classification model is designed to categorize blood cells into four distinct groups: eosinophil, lymphocyte, monocyte, and neutrophil. The study employs a Kaggle image dataset for comprehensive learning. The dataset comprises 12,500 microscopic images used to categorize the four blood cell groups. To enhance performance and reduce the likelihood of overfitting, transfer learning techniques are employed. Six deep transfer learning models namely VGG16, ResNet50, AlexNet, MobileNet, GoogLeNet, and EfficientNetBO are used for feature extraction and classification. The results of the experiments show that VGG16 and MobileNet demonstrated enhancements compared to other pre-trained models when evaluated on both augmented and original datasets. A diverse set of evaluation criteria was employed to thoroughly assess the effectiveness of medical image classification. Notably, the VGG16 and MobileNet models accurately predicted Lymphocytes and Monocytes with a 100% accuracy rate, and Eosinophil and Neutrophil with rates of 99.35% and 99.81%, respectively. This research work empower medical practitioners, particularly in the field of pathology and hematology by providing advanced tools for accurate blood cell classification. The proposed VGG16 and MobileNet models hold promise for simplifying WBC classification, improving decision-making processes, and ultimately advancing patient care in the medical domain. © The Author(s), under exclusive licence to Springer science+Business Media, LLC, part of Springer Nature 2024.

关键词： Deep learning

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Geometric Probability on a Lattice with the 15th Type of Convex Pentagon as a Fundamental Region

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Acta Mathematica Sinica,English Series 2025年第4期41卷 1213-1230页

作者： Jiangfu Zhao Jun Jiang Hai Liu Department of Mathematics and Physics Fujian Jiangxia University College of Science Wuhan University of Science and TechnologyHubei Province Key Laboratory of Systems Science in Metallurgical Process National Engineering Research Center for E-learning Central China Normal University

In 2015,a group of mathematicians at the University of Washington,Bothell,discovered the 15th pentagon that can cover a plane, with no gaps and ***,research on its containment measure theory or geometric probability is *** this study,the Laplace extension of Buffon's problem is generalized to the case of the 15th *** the solving process,the explicit expressions for the generalized support function and containment function of this irregular pentagon are *** addition,the chord length distribution function and density function of random distance of this pentagon are obtained in terms of the containment function.

关键词： Buffon lattice containment function generalized support function Geometric probability tessellation

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Promoting effect of d-band center and in-situ precipitation strategy on sulfur evolution reaction

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Journal of Energy Chemistry 2025年第5期104卷 740-748页

作者： Jun Pu Yun Tan Jiasen Yin Zihan Shen Shoujie Liu Kai Zhang Lei Zhou Yagang Yao Key Laboratory of Functional Molecular Solids Ministry of EducationAnhui Provincial Engineering Laboratory for New-Energy Vehicle Battery Energy-Storage MaterialsCollege of Chemistry and Materials ScienceAnhui Normal UniversityWuhu 241002AnhuiChina National Laboratory of Solid State Microstructures College of Engineering and Applied SciencesJiangsu Key Laboratory of Artificial Functional MaterialsCollaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093JiangsuChina State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Materials Science and Engineering Anhui UniversityHefei 230601AnhuiChina School of Energy and Power Engineering Jiangsu UniversityZhenjiang 212013JiangsuChina Department of Electrical Engineering Eindhoven University of TechnologyEindhoven MB 5600the Netherlands

The slow conversion of polyphase in lithium-sulfur(Li-S)batteries not only intensifies the shuttle effect of lithium polysulfides(LiPSs),but also causes the continuous accumulation of inactive sulfur species,resulting in rapid capacity attenuation and sluggish dynamic ***,the promoting effect of atomic interface stress on sulfur reaction was investigated via CoFe-CoFe_(2)O_(4)heterogeneous nanosheets with a cavity *** strain force induced by the in-situ precipitation of Co Fe bimetallic alloy in oxide matrix increased the d-band center,which was conducive to the interaction between catalyst and Li *** sulfur cathode based on this two-dimensional(2D)nanosheet design showed an extremely high capacity of 751 mAh g^(-1)at 4 *** with a sulfur loading of 5.55 mg cm^(-2),its area capacity was still as high as 7.15 mAh cm^(-2).Meanwhile,the enhanced stability greatly improved the practical potential of Li-S batteries.

关键词： 2D nanosheets In-situ precipitation Strain effect D-band center Li-S batteries

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