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作者： Ramasamy, Sivasamy Banjerdpongchai, David Park, PooGyeon Center of Excellence in Intelligent Control Automation of Process Systems Department of Electrical Engineering Faculty of Engineering Chulalongkorn University Bangkok Thailand Department of Electrical Engineering Pohang University of Science and Technology Pohang Korea Republic of

One of the most important goals of theoretical ecologists is to find a strategy for controlling the chaos in ecological models to maintain healthy ecosystems. We investigate the influence of fear and the supply of additional food to predators in a delayed tri-trophic food chain model, where interference among the species is determined by Holling type-II functional response. The proposed model incorporates the fact that the growth rates of prey and middle predators are decreased due to the fear of middle and special predators, respectively. The additional food is supplied to both predators by either nature or external agencies. Furthermore, the poisoned prey in the predator's environment is taken into account. In the proposed model, we use two time delays: one for the growth term of the middle predator and another for the gestation delay of the special predator. We determine the conditions for the existence of ecologically feasible equilibrium points and their local and global stability. In addition, we establish the conditions for the existence of Hopf bifurcation around interior equilibrium to seek periodic behavior in nondelayed and delayed models. Numerical investigations are performed to justify the proposed theoretical findings through phase portraits, time series of solutions, and bifurcation diagrams. We observe that the chaotic dynamics of a tri-trophic food chain model can be controlled by the proper choice of the fear effect and by supplying additional food parameters. As a result, our findings provide more ecological insights into the dynamics of the delayed tri-trophic food chain model with the fear effect and additional food supply. © 2023 John Wiley & Sons, Ltd.

关键词： Hopf bifurcation

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Universality class of machine learning for critical phenomena

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science China(Physics,Mechanics & Astronomy) 2023年第12期66卷 63-70页

作者： Gaoke Hu Yu Sun Teng Liu Yongwen Zhang Maoxin Liu Jingfang Fan Wei Chen Xiaosong Chen School of Systems Science and Institute of Nonequilibrium Systems Beijing Normal UniversityBeijing 100875China Data Science Research Center Faculty of ScienceKunming University of Science and TechnologyKunming 650500China State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

Herein,percolation phase transitions on a two-dimensional lattice were studied using machine learning *** reveal that different phase transitions belonging to the same universality class can be identified using the same neural networks(NNs),whereas phase transitions of different universality classes require different *** on this finding,we proposed the universality class of machine learning for critical ***,we investigated and discussed the NNs of different universality *** research contributes to machine learning by relating the NNs with the universality class.

关键词： universality class machine learning percolation

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Promoting effect of d-band center and in-situ precipitation strategy on sulfur evolution reaction

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Journal of Energy Chemistry 2025年第5期104卷 740-748页

作者： Jun Pu Yun Tan Jiasen Yin Zihan Shen Shoujie Liu Kai Zhang Lei Zhou Yagang Yao Key Laboratory of Functional Molecular Solids Ministry of Education Anhui Provincial Engineering Laboratory for New-Energy Vehicle Battery Energy-Storage Materials College of Chemistry and Materials Science Anhui Normal University National Laboratory of Solid State Microstructures College of Engineering and Applied Sciences Jiangsu Key Laboratory of Artificial Functional Materials Collaborative Innovation Center of Advanced Microstructures Nanjing University State Key Laboratory of Multiphase Complex Systems Institute of Process Engineering Chinese Academy of Sciences School of Materials Science and Engineering Anhui University School of Energy and Power Engineering Jiangsu University Department of Electrical Engineering Eindhoven University of Technology

The slow conversion of polyphase in lithium-sulfur （Li-S） batteries not only intensifies the shuttle effect of lithium polysulfides （LiPSs）,but also causes the continuous accumulation of inactive sulfur species,resulting in rapid capacity attenuation and sluggish dynamic ***,the promoting effect of atomic interface stress on sulfur reaction was investigated via CoFe-CoFe2O4heterogeneous nanosheets with a cavity *** strain force induced by the in-situ precipitation of Co Fe bimetallic alloy in oxide matrix increased the d-band center,which was conducive to the interaction between catalyst and Li *** sulfur cathode based on this two-dimensional （2D） nanosheet design showed an extremely high capacity of 751 mAh g-1at 4 *** with a sulfur loading of 5.55 mg cm-2,its area capacity was still as high as 7.15 mAh ***,the enhanced stability greatly improved the practical potential of Li-S batteries.

关键词： 2D nanosheets D-band center In-situ precipitation Li-S batteries Strain effect

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Synthesis of interfacial electric field-enhanced CdS/CdxZn1-xS/ZnO ternary heterojunction by lye dissolution etching mechanism for photocatalytic H2 production and CO2 reduction

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材料科学技术（英文版） 2025年第1期204卷 152-165页

作者： Qi Li Shengchao Yang Yufan Huang Yuwei Liang Chunling Hu Min Wang Zhiyong Liu Yanlong Tai Jichang Liu Yongsheng Li School of Chemistry and Chemical Engineering Shihezi University/Key Laboratory of Green Process for Chemical Engineering/Key Laboratory for Chemical Materials of Xinjiang Uygur Autonomous Region/Engineering Center for Chemical Materials of Xinjiang BingtuanShihezi UniversityShihezi 832003China Shanghai Institute of Ceramics Chinese Academy of SciencesShanghai 200050China School of Chemistry and Chemical Engineering Shihezi University/Key Laboratory of Green Process for Chemical Engineering/Key Laboratory for Chemical Materials of Xinjiang Uygur Autonomous Region/Engineering Center for Chemical Materials of Xinjiang BingtuanShihezi UniversityShihezi 832003China Key Laboratory of Human-Machine Intelligence-Synergy Systems of Chinese Academy of Sciences(CAS) Shenzhen Institutes of Advanced TechnologyShenzhen 518055China School of Chemistry and Chemical Engineering Shihezi University/Key Laboratory of Green Process for Chemical Engineering/Key Laboratory for Chemical Materials of Xinjiang Uygur Autonomous Region/Engineering Center for Chemical Materials of Xinjiang BingtuanShihezi UniversityShihezi 832003China Lab of Low-Dimensional Materials Chemistry Key Laboratory for Ultrafine Materials of Ministry of Education School of Materials Science and Engineering East China University of Science and Technology ShanghaiShanghai 200237China

The difficulty in fabricating a multifaceted composite heterojunction system based on CdxZn1-xS limits the enhancement of photocatalytic *** the present scrutiny,novel ZnO/CdxZn1-xS/CdS com-posite heterojunctions are successfully prepared by the alkaline dissolution etching *** internal electric field at the interface of Ⅰ-type and Z-scheme heterojunction improved the effective charge *** ZC 8 sample exhibits excellent photocatalytic performance and the H2 production efficiency is 15.67 mmol g-1 h-1 with good stability up to 82.9％in 24-hour *** performance of CH4 and CO capacity in the CO2RR process is 3.47 μmol g-1 h-1 and 23.5 μmol g-1 h-1,*** photogener-ated accelerated charge transport is then examined in detail by in situ X-ray photoelectron spectroscopy(ISXPS)and density functional theory(DFT)*** work presents a new idea for the synthe-sis of CdxZni-xS solid-solution-based materials and provides a solid reference for the detailed mechanism regarding the electric field at the heterojunction interface.

关键词： Photocatalysis Interface electric field Composite heterostructure Photocatalytic mechanism CdxZn1-xS solid-solution

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Heterojunctioned CuO/Cu_(2)O catalyst for highly efficient ozone removal

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Journal of Environmental sciences 2023年第3期125卷 340-348页

作者： Guojun Ma Wenxiang Tang AnqiWang Le Zhang Jian Guan Ning Han Yunfa Chen Key Laboratory of Science and Technology on Particle Materials Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemical Engineering Sichuan UniversityChengdu 610065China

In recent years, near surface ozone pollution, has attracted more and more attention,which necessitates the development of high efficient and low cost catalysts. In this work,Cu O/Cu_(2)O heterojunctioned catalyst is fabricated by heating Cu_(2)O at high temperature, and is adopted as ozone decomposition catalyst. The results show that after Cu_(2)O is heated at180℃conversion of ozone increases from 75.2% to 89.3% at mass space velocity 1,920,000cm^(3)/(g·hr) in dry air with 1000 ppm V ozone, which indicates that this heterojunction catalyst is one of the most efficient catalysts reported at present. Catalysts are characterized by electron paramagnetic resonance spectroscopy and ultraviolet photoelectron spectroscopy,which confirmed that the heterojunction promotes the electron transfer in the catalytic process and creates more defects and oxygen vacancies in the Cu O/Cu_(2)O interfaces. This procedure of manufacturing heterostructures would also be applicable to other metal oxide catalysts, and it is expected to be more widely applied to the synthesis of high-efficiency heterostructured catalysts in the future.

关键词： Cu_(2)O Ozone decomposition CuO Heterojunction

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Long Text Classification Using Pre-Trained Language Model for a Low-Resource Language 6

Long Text Classification Using Pre-Trained Language Model fo...

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6th International Conference on Information and Computer Technologies, ICICT 2023

作者： Yohannes, Hailemariam Mehari Amagasa, Toshiyuki University of Tsukuba Systems and Information Engineering Tsukuba Japan University of Tsukuba Center of Computational Science Tsukuba Japan

ISBN: (纸本)9798350300956

Text classification is an essential task of Natural Language processing (NLP) that intends to classify texts into predefined classes. Most recent studies show that transformer-based pre-Trained language models such as BERT and RoBERTa have achieved state-of-The-Art performance in several downstream NLP tasks. Despite their advantages, these models suffer from one primary drawback of the restricted input size. Because of this limitation, they cannot operate the entire input long texts. This paper presents an approach that utilizes the self-Attention mechanism to address the bottleneck of most pre-Trained language models of long input texts in the case of Amharic, regarded as a low-resourced language. Specifically, our method carefully investigates the significance of each word in the dataset using a self-Attention mechanism. Then identify and select the most relevant words according to their attention scores. Finally, we train our model on the filtered text. Our results show that the approach achieves better performance in terms of accuracy compared to the baseline model. © 2023 IEEE.

关键词： Classification (of information)

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Tuning the atomic configuration environment of MnN_(4) sites by Co cooperation for efficient oxygen reduction

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Journal of Energy Chemistry 2023年第7期82卷 547-559,I0012页

作者： Jing Wang Haihong Zhong Jun Yang Huiyu Li Pinggui Tang Yongjun Feng Dianqing Li State Key Laboratory of Chemical Resource Engineering Beijing Engineering Center for Hierarchical CatalystsCollege of ChemistryBeijing University of Chemical TechnologyBeijing 100029China College of Science Hainan UniversityHaikou 570228HainanChina State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China

Carbon-based N-coordinated Mn(Mn-N_(x)/C)single-atom electrocatalysts are considered as one of the most desirable non-precious oxygen reduction reaction(ORR)candidates due to their insignificant Fenton reactivity,high abundance,and intriguing electrocatalytic ***,current MnN_(x)/C single-atom electrocatalysts suffer from high overpotentials because of their low intrinsic activity and unsatisfactory chemical ***,through an in-situ polymerization-assisted pyrolysis,the Co as a second metal is introduced into the Mn-N_(x)/C system to construct Co,Mn-N_(x)dual-metallic sites,which atomically disperse in N-doped 1D carbon nanorods,denoted as Co,Mn-N/CNR and *** electron microscopy and X-ray absorption spectroscopy(XAS)techniques,we verify the uniform dispersion of CoN4and MnN4atomic sites and confirm the effect of Co doping on the MnN_(4) electronic *** functional theory(DFT)calculations further elucidate that the energy barrier of ratedetermining step(^(*)OH desorption)decreases over the 2 N-bridged MnCoN_(6) moieties related to the pure MnN_(4).This work provides an effective strategy to modulate the local coordination environment and electronic structure of MnN_(4) active sites for improving their ORR activity and stability.

关键词： Dual-atom sites Oxygen reduction reaction M-Nx/C catalysts Coordination environment Electronic structure Synergistic effect

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MXene Key Composites:A New Arena for Gas Sensors

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Nano-Micro Letters 2024年第10期16卷 350-391页

作者： Yitong Wang Yuhua Wang Min Jian Qinting Jiang Xifei Li Hubei Province Key Laboratory of Systems Science in Metallurgical Process Wuhan University of Science and TechnologyWuhan 430081People's Republic of China Key Materials and Components of Electrical Vehicles for Overseas Expertise Introduction Center for Discipline Innovation Institute of Advanced Electrochemical Energy and School of Materials Science and EngineeringXi'an University of TechnologyXi'an 710048People's Republic of China College of Materials Science and Engineering Fuzhou UniversityFuzhou 350108FujianPeople's Republic of China

With the development of science and technology,the scale of industrial production continues to grow,and the types and quantities of gas raw materials used in industrial production and produced during the production process are also constantly *** gases include flammable and explosive gases,and even contain toxic ***,it is very important and necessary for gas sensors to detect and monitor these gases quickly and *** recent years,a new two-dimensional material called MXene has attracted widespread attention in various *** abundant surface functional groups and sites,excellent current conductivity,tunable surface chemistry,and outstanding stability make them promising for gas sensor *** the birth of MXene materials,researchers have utilized the efficient and convenient solution etching preparation,high flexibility,and easily functionalize MXene with other materials to pre-pare composites for gas *** has opened a new chapter in high-performance gas sensing materials and provided a new approach for advanced sensor ***,previous reviews on MXene-based composite materials in gas sensing only focused on the performance of gas sensing,without systematically explaining the gas sensing mechanisms generated by different gases,as well as summarizing and predicting the advantages and disadvantages of MXene-based composite *** article reviews the latest progress in the application of MXene-based composite materials in gas ***,a brief summary was given of the commonly used methods for preparing gas sens-ing device structures,followed by an introduction to the key attributes of MXene related to gas sensing *** article focuses on the performance of MXene-based composite materials used for gas sensing,such as MXene/graphene,MXene/Metal oxide,MXene/Transition metal sulfides(TMDs),MXene/Metal-organic framework(MOF),MXene/*** summarizes the advantages and disad

关键词： MXene Compound material Gas sensor Gas sensitive preparation Gas sensitivity performance

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engineering of Fe d-band center in Fe_(3)O_(4)/CeO_(2)hetero-nanoparticles via orbital coupling for high-efficiency oxygen reduction electrocatalysis

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Nano Research 2025年第1期18卷 129-139页

作者： Jiayi Liu Jingwen Yin Yingzi Lin Mingxin Pang Huan Pang Songtao Zhang Lin Xu Jun Yang Yawen Tang Jiangsu Key Laboratory of New Power Batteries Jiangsu Collaborative Innovation Center of Biomedical Functional MaterialsSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing 210023Chin a 2 State Key Laboratory of Multiphase Complex Systems Center of MesoscienceInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou 225009China Testing Center Yangzhou UniversityYangzhou 225009China

The deliberate engineering of the d-band center of metal site represents an effective strategy to boost the intrinsic electrocatalytic performance toward the oxygen reduction reaction(ORR).Herein,following a heterointerfaceinduced orbital coupling rationale,we report a judicious design of an efficient ORR electrocatalyst consisting of Fe_(3)O_(4)/CeO_(2)hetero-nanoparticles in-situ encased into N-doped carbon nanofibers(abbreviated as Fe_(3)O_(4)/CeO_(2)@N-CNFs hereafter).The theoretic calculations uncover that the Fe_(3)O_(4)/CeO_(2)heterointerface-triggered orbital coupling can cause the down shift of the d-band center positions of Fe sites,which leads to the weakened chemisorption of oxygenated groups and lowered energy barrier for the potential-determining step,ultimately dramatically boosting the ORR intrinsic *** a consequence,the well-designed Fe_(3)O_(4)/CeO_(2)@N-CNFs display admirable ORR activity with a half-wave potential of 0.84 V and outstanding structural/electrochemical stability in an alkaline electrolyte,surpassing the commercial Pt/C benchmark and a majority of recently reported Fe_(3)O_(4)-based *** encouragingly,the Fe_(3)O_(4)/CeO_(2)@N-CNFsincorporated Zn-air battery outperforms the Pt/C-assembled counterpart with higher power density,larger energy density,and excellent cycling stability,serving as a competent candidate for ORR-involved renewable energy *** study offers an innovative approach for the rational manipulation of the d-band center and interfacial electron behavior of active sites toward the optimization of electrocatalytic performance.

关键词： hetero-nanoparticles electrospinning interfacial engineering orbital coupling oxygen reduction reaction

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Boosting C_(2)H_(6)/C_(2)H_(4) separation via the precise electrostatic modulation of synthetic 1D channel at atomic level

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Nano Research 2024年第11期17卷 10083-10087页

作者： Salamanti Ainiwaner Hengcong Huang Jia-Jia Zheng Fengting Li Xue-Tong Yang Yang-Yang Guo Fangli Yuan Ming-Shui Yao Yifan Gu College of Environmental Science and Engineering State Key Laboratory of Pollution Control and Resource Reuse Tongji University Shanghai 200092 China Laboratory of Theoretical and Computational Nanoscience National Center for Nanoscience and Technology Chinese Academy of Sciences Beijing 100190 China Skate Key Laboratory of Mesoscience and Engineering Institute of Process Engineering Chinese Academy of Sciences Beijing 100190 China Chinese Academy of Sciences University of Chinese Academy of Sciences Beijing 100049 China

The regulation of gas sorption via simple pore modification is crucial to molecular recognition and chemical ***,a rational pore surface electrostatic modulation in synthetic one dimensioned(1-D)channel is demonstrated to boost ethane/ethylene(C_(2)H_(6)/C_(2)H_(4))selectivity for one-step extraction of C_(2)H_(4) from C_(2)H_(6)/C_(2)H_(4) *** the precise modulation of the surface charge arrangement with negatively charged moieties in the 1-D channel of a metal—organic framework(MOF),enhanced C_(2)H_(6)—host framework and decreased C_(2)H_(4)—host framework electrostatic interactions were obtained,which resulted in an obvious improvement in adsorption ***,the breakthrough separation performance rendered the obtained MOF an efficient adsorbent for C_(2)H_(4) purification from C_(2)H_(6)/C_(2)H_(4) *** combined detail theoretical studies prove that the gas sorption selectivity is remarkably sensitive to framework electrostatic change even in the case of pore surface modification at the atomic *** results are of fundamental importance to the design of porous materials for challenging separation tasks.

关键词： metal—organic framework ethane/ethylene separation ethane—selective MOF adsorption electrostatic modulation

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