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比较三种稳定剂对FeS纳米颗粒的稳定效果及对水土中镉的固定与去除性能的影响

Journal of Central South University 2024年第4期31卷 1064-1075页

作者：田舒婷赵东叶霍丽娟马骏杨睿 Department of Environmental Science School of Environment and ResourcesTaiyuan University of Science and TechnologyTaiyuan 030024China Environmental Engineering Program Department of Civil&Environmental EngineeringAuburn UniversityAuburnAL 36849USA Department of Civil Constructionand Environmental EngineeringSan Diego State UniversitySan DiegoCA 92182USA

本研究评估了三种多糖稳定剂(羧甲基纤维素钠(CMC)、羧甲基淀粉钠(CMS)和一种水溶性淀粉)用于稳定FeS纳米颗粒的有效性,并测试了相应稳定化纳米颗粒在水和土壤中固定Cd^(2+)的性能。使用0.010 wt%CMC、0.025 wt%CMS或0.065 wt%淀粉可获... 详细信息

本研究评估了三种多糖稳定剂(羧甲基纤维素钠(CMC)、羧甲基淀粉钠(CMS)和一种水溶性淀粉)用于稳定FeS纳米颗粒的有效性,并测试了相应稳定化纳米颗粒在水和土壤中固定Cd^(2+)的性能。使用0.010 wt%CMC、0.025 wt%CMS或0.065 wt%淀粉可获得完全稳定的FeS纳米颗粒(100 mg/L FeS)。CMC-FeS表现出较高的zeta负电位,淀粉-FeS保持中性,而CMS-FeS则表现出中等负电位。CMCFeS对Cd^(2+)的吸附速率最快,吸附容量也最高。当用100 mg/L CMC-FeS或CMS-FeS处理一种含Cd土壤(58.3 mg/kg Cd)后,Cd的TCLP浸出率分别降低了88.4%和68.0%。CMC-FeS和CMS-FeS均可在模型土壤中运移,显示出其在土壤中原位固定Cd^(2+)方面的潜力。土壤穿透曲线实验表明,CMC-FeS在4.5个孔体积,CMS-FeS在约25个孔体积处几乎完全穿透。柱实验结果表明,当用55个孔体积的CMC-FeS或CMS-FeS悬浮液(100 mg/L)处理该含Cd土壤后,Cd的水浸出率分别降低了98.2%和98.0%。根据目标污染物、材料在土壤中的传输特性和材料成本,可找到这三种稳定剂在土壤修复中的最佳应用。

关键词：硫化铁纳米颗粒稳定剂重金属污染物固定土壤修复地下水污染

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Effect of Impregnation of Liquid Sodium Silicate on Thermal Properties of Paper

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Palpu Chongi Gisul/Journal of Korea Technical Association of the Pulp and Paper Industry 2022年第6期54卷 60-67页

作者： Park, Gwon-Hui Kim, Younglae Cho, Byoung-Uk Department of Paper Science & Engineering College of Forest and Environmental Sciences Kangwon National University Korea Republic of Program of Paper Material Science & Engineering College of Forest and Environmental Sciences Kangwon National University Korea Republic of

Heat-resistant insulators are the core materials in fire doors and are directly related to people’s safety in a fire. Heverever, there needs to be a material that possesses heat resistance and insulation with reasonable production cost. To develop a core material for fire doors based on recycled paper, such as copy paper and linerboard, were impregnated with liquid sodium silicate and the effects of the sodium silicate content on the thermal properties of paper were investigated. It was observed that liquid soidum silicate can be used as a flame retardant when manufacturing fire door core materials. Imprenation of liquid sodium silicate delayed both glowing and burning temperatures along with an increased weight of residues after combustion over 750℃. Hence, it is possible to manufacture an incombustible material based on recycled papers by adding liquid sodium silicate and inorganic materials that do not themally decompose over 750℃. © 2022 Korean Technical Assoc. of the Pulp and Paper Industry. All rights reserved.

关键词： Impregnation

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Comparison on Efficiency of Iron and Aluminum Nanoparticles for Methylene Blue Removal from Aqueous Solutions

Comparison on Efficiency of Iron and Aluminum Nanoparticles ...

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2023 AIChE Annual Meeting

作者： Mostafa, Mohamed K. Sadek, Ahmed H. Cairo Egypt Environmental Engineering Program Zewail City of Science Technology and Innovation Giza Egypt Giza Egypt

This review demonstrates a comparative study of methylene blue (MB) dye removal from aqueous solutions using zero-valent iron (nZVI) and zero-valent aluminum (nZVAl) nanoparticles. The results indicated that at pH 6, nZVI dosage 10 g/L, initial MB concentration 10 mg/L, temperature 30 °C, and stirring rate 150 rpm, the equilibrium time was 30 min achieving a removal efficiency of approximately 100% for nZVI. While for nZVAl, the results indicated that at an initial MB concentration of 10 mg/L, pH 10, nZVAl dosage 1.0 g/L, stirring rate 200 rpm, and temperature 30 °C, the removal efficiency of approximately 99.0% was achieved within an equilibrium time of 90 min. Moreover, the adsorption data of MB fitted well to the Freundlich isotherm model (R2: 0.9358) and pseudo-second-order kinetic model (R2: 0.9976) for adsorption by nZVI. Also, the isotherm adsorption data were best fitted by the Freundlich isotherm model (R2: 0.9569), while the kinetic data were well described by the pseudo-second-order model (R2: 0.9999) for adsorption by nZVAl. From the aforementioned results, it is clear that both nZVI and nZVAl showed very high efficiency in removing methylene blue from aqueous solutions with a slight difference in favor of nZVI. © 2023 American Institute of Chemical Engineers. All rights reserved.

关键词： Aluminum

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Habitat modelling of escolar fish (Lepidocybium flavobrunneum, Smith 1843) in the southwestern Indian Ocean using remote sensing data

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International Journal of Remote Sensing 2024年第23期45卷 8722-8741页

作者： Sihombing, Riah Irawati Ray, Aratrika Mondal, Sandipan Lee, Ming-An Environmental Biology and Fisheries Science National Taiwan Ocean University Keelung City Taiwan Center of Excellence for Ocean Engineering National Taiwan Ocean University Keelung City Taiwan Doctoral Degree Program in Ocean Resource and Environmental Changes National Taiwan Ocean University Keelung City Taiwan

Escolar (Lepidocybium flavobrunneum) belongs to Gempylidae family, is a top predator species that plays a crucial role in the marine ecosystem. However, limited information is available regarding their spatial-temporal variations in habitat, while habitat suitability index (HSI) modelling has been widely used in recent years for conservation, fisheries, and ecology. We compared an Arithmetic Mean Model (AMM) and a Geometric Mean Model (GMM) to gain insights into their habitat distribution. Fishery data were collected from the southwestern Indian Ocean between 2010 and 2014. Ten oceanographic remote sensing data sets were compiled, and four of them were selected based on their higher R 2 values obtained from Generalized Additive Model (GAM), Boosted Regression Trees (BRT), and Random Forest (RF) analyses for constructing the model combination. Meanwhile, Suitability Index (SI) curves were employed to determine the habitat suitability range for escolar. environmental parameters were combined using a step-wise approach and applied for both AMM and GMM. The models were evaluated based on the Lowest Akaike Information Criterion (AIC) value. Eventually, AMM was chosen over GMM with the AIC value was 28.49 and 31.25, respectively. The selected model combination of AMM was Sea Surface Height (SSH), Oxygen (O), and Sea Surface Temperature (SST) meaning these parameters influenced the distribution of escolar. The SI curve of the chosen model indicated the habitat range for each parameter as follows: SSH (0.61–0.69 m), O (222–230 mmol m−3), and SST (18.7–21.1°C). The most suitable habitat for escolar was observed within the coordinates 36 ºS-30 ºS and 28 ºE-36 ºE. Thus, this method is demonstrated in a case study where just presence data are provided and the incorporation of remote sensing environmental factors is gathered. This result could help improve escolar fishery management in the southwestern Indian Ocean. © 2023 The Author(s). Published by Informa UK Limited, trading

关键词： Fisheries

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Applicability of Electrical Resistance Method to Moisture Transfer Measurement in Paste Using Mineral Admixture 2nd

Applicability of Electrical Resistance Method to Moisture Tr...

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2nd International Conference on Sustainable Civil engineering and Architecture, ICSCEA 2021

作者： Aoki, Takahiro Ogawa, Yuko Kawai, Kenji Civil and Environmental Engineering Program Graduate School of Advanced Science and Engineering Hiroshima University 1-4-1 Kagamiyama Higashihiroshima Japan

ISBN: (纸本)9789811933028

Concrete is a porous material which has the ability to hold moisture stably inside. Since moisture is closely related to the deterioration of concrete structures, it is important to understand the moisture transfer in concrete in order to maintain the concrete structure appropriately. The electrical resistance method is one of non-destructive methods to investigate the moisture in concrete and the moisture transfer can be assessed with time by using one specimen. However, the electrical resistance may be affected by mineral admixtures in concrete. Although previous studies on the effects of mineral admixtures on the electrical resistance have been conducted, there are still many unclear points. Therefore, the purpose of this study is to assess the applicability of the electrical resistance method to moisture transfer measurement in paste containing mineral admixtures by focusing on the moisture transfer in the drying process. The moisture transfer in the hardened cement paste using fly ash and blast furnace slag with water-to-binder ratios of 0.35 and 0.55 was investigated by the electrical resistance method. Stainless steel rods of 0.9 mm in diameter were placed at an interval of 4 mm in the specimen. The calibration test was also conducted to obtain the relationship between the electrical resistivity and the internal relative humidity of the specimen. The result showed that the specific resistance of the specimen containing mineral admixtures was higher than that of the specimen without mineral admixtures. It was observed that at the drying period of 70 days, the internal relative humidity at a depth of 4 mm from the exposed surface was almost the same as the surrounding relative humidity. It is possible to know the change in the internal relative humidity distribution in the cement paste using mineral admixtures during the drying process by performing the calibration test appropriately. © 2023, The Author(s), under exclusive license to Springer Nature Singapore P

关键词： Concretes

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Direct Multi-group Cross-sections via NJOY+OJOYU for PWR and FLiBe-MSR Reactor Systems

Direct Multi-group Cross-sections via NJOY+OJOYU for PWR and...

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2023 Transactions of the American Nuclear Society Annual Meeting and Technology Expo, ANS 2023

作者： Wang, Meng-Jen Simpson, Michael Sjoden, Glenn E. Nuclear Engineering Program Department of Civil and Environmental Engineering University of Utah United States Department of Material Science and Engineering University of Utah United States

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Sulfur-doped hard carbon hybrid anodes with dual lithium-ion/metal storage bifunctionality for high-energy-density lithium-ion batteries

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Carbon Energy 2023年第1期5卷 71-81页

作者： Sungmin Cho Jong Chan Hyun Son Ha Yeonhua Choi Honggyu Seong Jaewon Choi Hyoung-Joon Jin Young Soo Yun Program in Environmental and Polymer Engineering Inha UniversityIncheonSouth Korea KU-KIST Graduate School of Converging Science and Technology Korea UniversitySeoulSouth Korea Departmant of Chemistry and Research Institute of Natural Science Gyeongsang National UniversityJinjuSouth Korea Department of Polymer Science and Engineering Inha UniversityIncheonSouth Korea Division of Energy Engineering Kangwon National UniversityGangwon-doSouth Korea

Bifunctional hybrid anodes(BHAs),which are both a high-performance active host material for lithium-ion storage as well as a guiding agent for homogeneous lithium metal nucleation and growth,exhibit significant potential as anodes for next-generation high-energy-density lithium-ion batteries(LIBs).In this study,sulfur-doped hard carbon nanosphere assemblies(S-HCNAs)were prepared through a hydrothermal treatment of a liquid organic precursor,followed by high-temperature thermal annealing with elemental sulfur for application as BHAs for *** a carbonate-based electrolyte containing fluoroethylene carbonate additive,the S-HCNAs showed high lithium-ion storage capacities in sloping as well as plateau voltage sections,good rate capabilities,and stable *** addition,high average Coulombic efficiencies(CEs)of~96.9%were achieved for dual lithium-ion and lithium metal storage *** the LIB full-cell tests with typical NCM811 cathodes,the S-HCNA-based BHAs containing~400 mA h g^(−1) of excess lithium led to high energy and power densities of~500Wh kg^(−1) and~1695Wkg^(−1),respectively,and a stable cycling performance with~100%CEs was achieved.

关键词： hard carbon hybrid anode lithium-ion batteries lithium metal anode lithium metal batteries sulfur-doped carbon

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Chevrel phase: A review of its crystal structure and electrochemical properties

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Progress in Natural science:Materials International 2023年第1期33卷 8-15页

作者： Meng Liu Guocheng Lv Tianming Liu Hao Liu Lingchang Kong Lintao Tian Wenxiu Rao Yuxin Li Libing Liao Juchen Guo Engineering Research Center of Ministry of Education for Geological Carbon Storage and Low Carbon Utilization of Resources Beijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes National Laboratory of Mineral Materials School of Materials Science and Technology China University of Geosciences(Beijing) School of Science China University of Geosciences Materials Science and Engineering Program University of California-Riverside Department of Chemical and Environmental Engineering University of California – Riverside

Chevrel phase compounds have attracted increasing attention as electrochemical energy storage materials and electro-catalysts. Benefiting from their unique crystal structure, Chevrel phase compounds can not only function as the host structures for reversible intercalation of a broad range of cations, but also exhibit high catalytic activity in electrochemical reduction reactions. Here we provide an overview of recent progress in the development of Chevrel phase materials including new understanding of structural features, synthetic methods, and electrochemical properties. A brief conclusion and perspectives on the future development of Chevrel phase materials are also provided.

关键词： Chevrel phase Electrochemical properties Energy storage Electro-catalysis

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environmental Disinfection Based on Mobile Intelligent Networking Highly Efficient Ultraviolet Light Machines

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Aerosol and Air Quality Research 2024年第2期24卷 1-10页

作者： Chung, Chun-Yen Sung, Wen-Tsai Wang, Lin-Chi Siami, Lailatus Santos, John Paul Computer and Game Development Program Kun Shan University Tainan710303 Taiwan Department of Electrical Engineering National Chin-Yi University of Technology Taichung411030 Taiwan Department of Marine Environmental Engineering National Kaohsiung University of Science and Technology Kaohsiung81157 Taiwan Department of Environmental Engineering Chung Yuan Christian University Taoyuan32023 Taiwan Department of Civil Engineering Chung Yuan Christian University Taoyuan32023 Taiwan

Since 2019, the world has suffered from the outbreak of the "Coronavirus Disease (COVID)-19 pandemic. This study used the principle of Ultraviolet (UV)-C disinfection to produce a mobile high-power UV-C sterilizer. It focused on combining intelligent control systems, human sensors, and Internet of Things (IoT) systems to carry out disinfection tasks in unmanned indoor spaces. Because of its mobile nature, the sterilizer could be moved at any time in various learning, research, and activity rooms for disinfection. In addition to manually controlling the sterilizer, a Wi-Fi or Narrowband (NB)-IoT-enabled remote control was provided to start the disinfection process. In order to prevent ultraviolet light from harming the human body, sensors were employed self-acting to detect the presence of people and turn off the ultraviolet light when people were detected in the area. At the same time, a camera on the sterilizer would capture an image and notify the relevant personnel through a LINE notification, to prevent the human body from being exposed to ultraviolet light, causing harm to the teachers and students on campus. During operation, voice broadcast reminders and a status indicator could provide information about the operation status. After disinfection, users could view the disinfection process through a mobile device application or a webpage, which would automatically notify relevant personnel of the disinfection status through a LINE notification. In this way, the disinfection progress could be updated at anytime, anywhere and the current disinfection status in the classroom could be displayed in real-time, allowing teachers and students on campus to carry out teaching and learning in a safe and secure environment. © The Author(s).

关键词： Internet of things

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Unsaturated Strength of Tage Tuff and Its Water Retention Drying Curve

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Zairyo/Journal of the Society of Materials science, Japan 2024年第3期73卷 212-219页

作者： Kotabe, Haruhiko Togashi, Yota Hatakeyama, Ken Osada, Masahiko Civil and Environmental Engineering Program Graduate School of Science and Engineering Saitama University Shimo-Okubo Sakura-ku Saitama338-8570 Japan Integrated Technical Support Center Research Organization Saitama University Shimo-Okubo Sakura-ku Saitama338-8570 Japan

Strength loss of sedimentary rocks due to water content changes is an important issue in the civil engineering field. Assuming disasters associated with rainfall and drying, it is important to identify unsaturated strength properties for gradually varying moisture contents. Water retention curves are needed to describe unsaturated strength properties. The high suction acting in the case of rock presents a challenge in identifying the suction. In particular, identifying the water retention drying path is difficult. This study propose a method to identify the drying paths using uniaxial compressive strength and tensile strength of Brazilian test. Uniaxial compression and Brazilian tests were performed on specimens with varying water content in the drying pass to investigate changes in their mechanical properties. Strength and stiffness were found to be approximately halved in the wet condition compared to the dry condition. Simplified Mohr-Coulomb failure criteria are also identified using uniaxial compressive and tensile strength. The cohesion decreases with increasing water content, while the angle of shear resistance is independent of changes in water content. Suction at each saturation level was back-analyzed using the detected cohesion and shear resistance angles to identify the water retention drying curve. The water retention drying curves identified were compared with the water retention wetting curve identified by another method to confirm the validity of the proposed method. ©2024 The Society of Materials science, Japan.

关键词： Sedimentary rocks

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