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Emerging contaminants:A One Health perspective

The Innovation 2024年第4期5卷 140-170,139页

作者： Fang Wang Leilei Xiang Kelvin Sze-Yin Leung Martin Elsner Ying Zhang Yuming Guo Bo Pan Hongwen Sun Taicheng An Guangguo Ying Bryan WBrooks Deyi Hou Damian EHelbling Jianqiang Sun Hao Qiu Timothy MVogel Wei Zhang Yanzheng Gao Myrna JSimpson Yi Luo Scott XChang Guanyong Su Bryan MWong Tzung-May Fu Dong Zhu Karl JJobst Chengjun Ge Frederic Coulon Jean Damascene Harindintwali Xiankui Zeng Haijun Wang Yuhao Fu Zhong Wei Rainer Lohmann Changer Chen Yang Song Concepcion Sanchez-Cid Yu Wang Ali El-Naggar Yiming Yao Yanran Huang Japhet Cheuk-Fung Law Chenggang Gu Huizhong Shen Yanpeng Gao Chao Qin Hao Li Tong Zhang Natàlia Corcoll Min Liu Daniel SAlessi Hui Li Kristian KBrandt Yolanda Pico Cheng Gu Jianhua Guo Jianqiang Su Philippe Corvini Mao Ye Teresa Rocha-Santos Huan He Yi Yang Meiping Tong Weina Zhang Fidèle Suanon Ferdi Brahushi Zhenyu Wang Syed AHashsham Marko Virta Qingbin Yuan Gaofei Jiang Louis A.Tremblay Qingwei Bu Jichun Wu Willie Peijnenburg Edward Topp Xinde Cao Xin Jiang Minghui Zheng Taolin Zhang Yongming Luo Lizhong Zhu Xiangdong Li DamiàBarceló Jianmin Chen Baoshan Xing Wulf Amelung Zongwei Cai Ravi Naidu Qirong Shen Janusz Pawliszyn Yong-guan Zhu Andreas Schaeffer Matthias C.Rillig Fengchang Wu Gang Yu James M.Tiedje State Key Laboratory of Soil and Sustainable Agriculture Institute of Soil ScienceChinese Academy of SciencesNanjing 210008China University of Chinese Academy of Sciences Beijing 100049China Department of Chemistry Hong Kong Baptist UniversityHong KongChina HKBU Institute of Research and Continuing Education Shenzhen Virtual University ParkShenzhenChina Technical University of Munich TUM School of Natural SciencesInstitute of Hydrochemistry85748 GarchingGermany School of Resources&Environment Northeast Agricultural UniversityHarbin 150030China Climate Air Quality Research UnitSchool of Public Health and Preventive MedicineMonash UniversityMelbourneVICAustralia Faculty of Environmental Science&Engineering Kunming University of Science&TechnologyKunming 650500China Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria College of Environmental Science and EngineeringNankai UniversityTianjin 300350China Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control School of Environmental Science and EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Ministry of Education Key Laboratory of Environmental Theoretical Chemistry South China Normal UniversityGuangzhouGuangdong 510006China Department of Environmental Science Baylor UniversityWacoTXUSA Center for Reservoir and Aquatic Systems Research(CRASR) Baylor UniversityWacoTXUSA School of Environment Tsinghua UniversityBeijing 100084China School of Civil and Environmental Engineering Cornell UniversityIthacaNY 14853USA Key Laboratory of Microbial Technology for Industrial Pollution Control of Zhejiang Province Zhejiang University of TechnologyHangzhou 310014China School of Environmental Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China Laboratoire d’Ecologie Microbienne Universite Claude Bernard Lyon 1UMR CNRS 5557UMR INRAE 1418VetAgro Sup69622 VilleurbanneFrance Department of Pla

environmental pollution is escalating due to rapid global development that often prioritizes human needs over planetary *** global efforts to mitigate legacy pollutants,the continuous introduction of new substances remains a major threat to both people and the *** response,global initiatives are focusing on risk assessment and regulation of emerging contaminants,as demonstrated by the ongoing efforts to establish the UN’s Intergovernmental Science-Policy Panel on Chemicals,Waste,and Pollution *** review identifies the sources and impacts of emerging contaminants on planetary health,emphasizing the importance of adopting a One Health *** for monitoring and addressing these pollutants are discussed,underscoring the need for robust and socially equitable environmental policies at both regional and international *** actions are needed to transition toward sustainable pollution management practices to safeguard our planet for future generations.

关键词： pollution planet contaminants

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The Role of Fe(Iv) in the Zero-Valent Iron Biochar Activated Persulfate System for Treatment of Contaminants of Emerging Concern

SSRN

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SSRN 2024年

作者： Peng, Guilong Gong, Wenwen He, Dandan Wang, Xiao Yan, Yuting Dionysiou, Dionysios D. Blaney, Lee Institute of Quality Standard and Testing Technology Beijing Academy of Agriculture and Forestry Science Beijing100097 China State Key Laboratory of Resource Insects College of Sericulture Textile and Biomass Sciences Southwest University Chongqing400715 China Environmental Engineering and Science Program Department of Chemical and Environmental Engineering University of Cincinnati CincinnatiOH45221 United States University of Maryland Baltimore County Department of Chemical Biochemical and Environmental Engineering BaltimoreMD21250 United States Yibin Academy Southwest University Yibin China

In this paper, Fe(IV) was analyzed in the zero-valent iron biochar (ZVI-BC) activated persulfate (PS) process with methyl phenyl sulfoxide (PMSO) as the probe compound. Without a reaction terminator, PMSO degradation continued during the sample holding time, resulting in significant errors in the kinetics analysis. When 1 mM NaNO2, 1 mM NH2OH, 10 mM Na2S2O3, and 10 mM dimethyl sulfoxide were used as terminators, the analytical interference to PMSO and its oxidation product, methyl phenyl sulfone (PMSO2), was reduced to a negligible level, enabling detection by high performance liquid chromatography. In addition to Fe(IV), free radical (i.e., SO4•–, •OH, O2•–) and nonradical (i.e., 1O2) reactive species were also involved in the ZVI-BC/PS system;however, Fe(IV) was the predominant reactive species. Generally, organic contaminants with electron-donating moieties rapidly reacted with Fe(IV), and the relative contribution of Fe(IV) to overall contaminant degradation decreased as the solution pH was increased. Overall, this study provided new insights into the quantitative analysis of Fe(IV) in the ZVI-BC/PS system and its application to treatment of organic contaminants in solutions with variable water quality. © 2024, The Authors. All rights reserved.

关键词： Sodium compounds

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Critical Review on the Abatement Of Endocrine Disrupting Compounds In Iron-Based Materials Catalyzed Persulfate Systems: Reactive Species, Reaction Mechanisms, and Perspectives

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SSRN 2024年

作者： Sun, Ye Huang, Ying Zheng, Shujie Chen, Haojia Yang, Yan Ji, Hongbing Han, Changseok School of Chemical Engineering and Light Industry School of Environmental Science and Engineering Guangdong University of Technology Guangzhou510006 China School of Environment Hangzhou Institute for Advanced Study UCAS Hangzhou310024 China School of Chemistry and Chemical Engineering Guangxi Key Laboratory of Petrochemical Resource Processing and Process Intensification Technology Guangxi University Nanning530004 China Synergy Innovation Institute of Guangdong University of Technology Shantou515041 China Department of Environmental Engineering INHA University Incheon22212 Korea Republic of Program in Environmental and Polymer Engineering Graduate School of INHA University Incheon22212 Korea Republic of

Persulfate-based advanced oxidation processes have emerged as promising technologies for mitigating endocrine-disrupting compounds (EDCs) in wastewater treatment. Economically viable Fe-based materials with tailored properties have demonstrated significant efficacy in activating persulfate for the decomposition of EDCs through both radical-routes (•OH, SO4•−, and O2•−) and non-radical routes (1O2, surface activated PS complex, and high-valent Fe species). This review summarized the latest advancements in the persulfate activation mechanisms mediated by Fe-based materials, categorized by Fe valence states and the types of reactive species. Furthermore, it critically assesses the influence of active sites of Fe-based catalysts on persulfate activation pathways and summarizes the selective reaction of reactive species towards EDCs. Despite these advancements, several challenges persist in non-radical route-dominated persulfate activation, particularly regarding the impact of Fe-Fe distance on the reactive species and the catalytic role of Fe-based materials for reactions between inorganic ions and persulfate. This review proposes prospective research directions, provides design strategies, and expands the application of Fe-based materials in PS activation for effective EDC abatement in real situations. © 2024, The Authors. All rights reserved.

关键词： Endocrine disrupters

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Evidence for autotrophic growth of purple sulfur bacteria using pyrite as electron and sulfur source (vol 90, e00863, 2024)

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APPLIED AND environmental MICROBIOLOGY 2024年第9期90卷 e00863-24-e00863-24页

作者： Alarcon, Hugo V. Mohl, Jonathon E. Chong, Grace W. Betancourt, Ana Wang, Yi Leng, Weinan White, Jason C. Xu, Jie Environmental Science and Engineering Program the University of Texas at El Paso El Paso Texas USA Department of Mathematical Sciences the University of Texas at El Paso El Paso Texas USA Border Biomedical Research Center the University of Texas at El Paso El Paso Texas USA Department of Earth Environmental and Resource Sciences the University of Texas at El Paso El Paso Texas USA The Connecticut Agricultural Experiment Station New Haven Connecticut USA The National Center for Earth and Environmental Nanotechnology Infrastructure Blacksburg Virginia USA School of Molecular Sciences Arizona State University Tempe Arizona USA

Purple sulfur bacteria (PSB) are capable of anoxygenic photosynthesis via oxidizing reduced sulfur compounds and are considered key drivers of the sulfur cycle in a range of anoxic environments. In this study, we show that Allochromatium vinosum (a PSB species) is capable of autotrophic growth using pyrite as the electron and sulfur source. Comparative growth profile, substrate characterization, and transcriptomic sequencing data provided valuable insight into the molecular mechanisms underlying the bacterial utilization of pyrite and autotrophic growth. Specifically, the pyrite-supported cell cultures (“py”’) demonstrated robust but much slower growth rates and distinct patterns from their sodium sulfide-amended positive controls. Up to ~200-fold upregulation of genes encoding various c- and b-type cytochromes was observed in “py,” pointing to the high relevance of these molecules in scavenging and relaying electrons from pyrite to cytoplasmic metabolisms. Conversely, extensive downregulation of genes related to LH and RC complex components indicates that the electron source may have direct control over the bacterial cells’ photosynthetic activity. In terms of sulfur metabolism, genes encoding periplasmic or membrane-bound proteins (e.g., FccAB and SoxYZ) were largely upregulated, whereas those encoding cytoplasmic proteins (e.g., Dsr and Apr groups) are extensively suppressed. Other notable differentially expressed genes are related to flagella/fimbriae/pilin(+), metal efflux(+), ferrienterochelin(−), and [NiFe] hydrogenases(+). Characterization of the biologically reacted pyrite indicates the presence of polymeric sulfur. These results have, for the first time, put the interplay of PSB and transition metal sulfide chemistry under the spotlight, with the potential to advance multiple fields, including metal and sulfur biogeochemistry, bacterial extracellular electron transfer, and artificial photosynthesis.

关键词： purple sulfur bacteria pyrite anoxygenic photosynthesis transcriptomic sequencing cytochrome iron sulfur cluster Allochromatium vinosum

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Metal-Doped Carbon-Supported/Modified Titanate Nanotubes for Perfluorooctane Sulfonate Degradation in Water：Effects of Preparation Conditions, Mechanisms, and Parameter Optimization

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SSRN 2022年

作者： Zhu, Yangmo Xu, Tianyuan Zhao, Dongye Environmental Engineering Program Department of Civil and Environmental Engineering Auburn University AuburnAL36849 United States School of Resource and Geosciences China University of Mining and Technology Jiangsu Xuzhou221116 China Department of Civil Construction and Environmental Engineering San Diego State University 5500 Campanile Drive San DiegoCA92182 United States

Metal-doped, activated carbon (AC) supported titanate nanotubes (Me/TNTs@AC) have been shown promising for photocatalytic degradation of per- and polyfluoroalkyl substances (PFAS). However, the preparation recipe of these adsorptive photocatalysts has not yet been optimized in terms of type and content of precursor materials and the metal dopants as well as synthesizing conditions. To address this knowledge gap, we prepared TNTs@AC based on a commercial TiO2 and six different ACs at varying AC:TiO2 ratios and under different hydrothermal conditions. In addition, a suite of dopant metal ions, including Fe3+, Bi3+, Ga3+, In3+, Co2+, Cu2+, and Mn2+, were compared to gauge their effect on the material photoactivity. Moreover, the effect of the calcination temperature was also tested. The photocatalytic performance of Me/TNTs@AC was evaluated based on their effectiveness in defluorination of pre-sorbed perfluorooctane sulfonic acid (PFOS) after 4-h UV irradiation. Based on the experimental results, the highest photocatalytic mineralization efficiency (66.2%) of PFOS was achieved using Ga/TNTs@AC prepared under the following conditions: Filtrosorb-400® = 50 wt.%, Ga = 2 wt.%, hydrothermal treatment temperature = 130 ℃, hydrothermal duration = 72 h, and calcination temperature = 550 ℃. To understand the underlying mechanisms, selected materials were characterized via X-ray diffraction, the BET surface area and pore volume, UV-vis diffuse reflectance spectrometry, and photoluminescence. The results revealed that the superior photoactivity of Ga/TNTs@AC is attributed to the Ga-facilitated formation of pure crystallized anatase phase during the calcination, high UV light absorption, formation of microscale hybrid AC-anatase-Ga phases, and oxygen defects induced by Ga3+. The information can facilitate preparation and optimization of composite photocatalysts for efficient adsorption and photocatalytic degradation of PFAS in water. © 2022, The Authors. All rights reserved.

关键词： Activated carbon

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Ultrathin-shell epitaxial Ag@Au core-shell nanowires for high-performance and chemically-stable electronic, optical, and mechanical devices

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Nano Research 2021年第11期14卷 4294-4303页

作者： Yangzhi Zhu Sanggon Kim Xuezhi Ma Peter Byrley Ning Yu Qiushi Liu Xiaoming Sun Da Xu Sangshan Peng Martin C.Hartel Shiming Zhang Vadim Jucaud Mehmet R.Dokmeci Ali Khademhosseini Ruoxue Yan Department of Chemical and Environmental Engineering Bourns College of EngineeringUniversity of California-RiversideRiversideCA92521USA Terasaki Institute for Biomedical Innovation Los AngelesCA90064USA Department of Electrical and Computer Engineering University of California-RiversideRiversideCA92521USA State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical TechnologyBeijing100029China State Key Laboratory of Chemo/Biosensing and Chemometrics College of Chemistry and Chemical EngineeringHunan UniversityChangsha410082China Department of Bioengineering University of California-Los AngelesLos AngelesCA90095USA Department of Electrical and Electronic Engineering The University of Hong KongHong KongChina Material Science and Engineering Program University of California-RiversideRiversideCA92521USA

Silver nanowires (AgNWs) hold great promise for applications in wearable electronics, flexible solar cells, chemical and biological sensors, photonic/plasmonic circuits, and scanning probe microscopy (SPM) due to their unique plasmonic, mechanical, and electronic properties. However, the lifetime, reliability, and operating conditions of AgNW-based devices are significantly restricted by their poor chemical stability, limiting their commercial potentials. Therefore, it is crucial to create a reliable oxidation barrier on AgNWs that provides long-term chemical stability to various optical, electrical, and mechanical devices while maintaining their high performance. Here we report a room-temperature solution-phase approach to grow an ultra-thin, epitaxial gold coating on AgNWs to effectively shield the Ag surface from environmental oxidation. The Ag@Au core-shell nanowires (Ag@Au NWs) remain stable in air for over six months, under elevated temperature and humidity (80 °C and 100% humidity) for twelve weeks, in physiological buffer solutions for three weeks, and can survive overnight treatment of an oxidative solution (2% H2O2). The Ag@Au core-shell NWs demonstrated comparable performance as pristine AgNWs in various electronic, optical, and mechanical devices, such as transparent mesh electrodes, surface-enhanced Raman spectroscopy (SERS) substrates, plasmonic waveguides, plasmonic nanofocusing probes, and high-aspect-ratio, high-resolution atomic force microscopy (AFM) probes. These Au@Ag core-shell NWs offer a universal solution towards chemically-stable AgNW-based devices without compromising material property or device performance.

关键词： epitaxial growth core-shell nanowire plasmonic waveguides atomic force microscopy(AFM)probe transparent electrode wearable electronics

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Effect of double coating on microencapsulation of levofloxacin using the particles from gas-saturated solutions process as a controlled-release system

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Discover Chemistry 2025年第1期2卷 1-13页

作者： Sharmin, Tanjina Takeshita, Toshihiro Ouchi, Mikio Yoshida, Koji Znad, Hussein Saptoro, Agus Sarker, Zaidul Islam Irie, Keiichi Satho, Tomomitsu Nioh, Atsushi Masuda, Takaaki Muneyoshi, Yuuki Terayama, Suzuko Mishima, Kenji Department of Chemical Engineering Faculty of Engineering Fukuoka University Fukuoka Japan Research Institute of Composite Materials Fukuoka University Fukuoka Japan Resource Circulation Faculty of Environmental Engineering Fukuoka University Fukuoka Japan Faculty of Sciences Fukuoka University Fukuoka Japan Western Australian School of Mines: Minerals Energy and Chemical Engineering Faculty of Science and Engineering Curtin University Perth Australia Department of Chemical Engineering Faculty of Engineering Curtin Malaysia Graduate School Miri Sarawak Malaysia Department of State Program and Food Science Northern Marianas College Saipan USA Faculty of Pharmaceutical Sciences Fukuoka University Fukuoka Japan Yokohama Research Center Pola Chemical Industries Yokohama Japan

A novel double-coating technique was employed to encapsulate levofloxacin (LVF), a potent antibacterial drug, using the particles from gas-saturated solutions (PGSS) process to achieve extended release. The primary coating utilized glyceryl tristearate (GT), a lipid with a high melting point (72 °C), followed by a secondary coating with trimyristin (TM), a lipid with a lower melting point (52 °C). For comparison, a single-coating approach was also explored, using the biocompatible polymer poly-(ε-caprolactone) (PCL). The resulting particles were characterized for their shape, size, and LVF encapsulation efficiency, with confirmation of LVF entrapment provided by Fourier transform infrared (FTIR) spectroscopy, and X‐ray powder diffraction (XRD) analysis. The particles, with an average diameter of 95.3 ± 16.5 μm, exhibited an encapsulation efficiency of up to 92.1 ± 2.5%. Furthermore, in vitro release studies revealed that the double-coated microcapsules effectively suppressed the initial burst release and provided controlled, extended release of LVF (t30D = 36.3%), demonstrating the efficiency of this encapsulation method for prolonged drug delivery.

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Ozone pollution induced-yield loss of major staple crops in China and effects from COVID-19

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Journal of environmental Sciences 2025年 157卷 804-820页

作者： Haiyang Liu Siyuan Wang Guangsheng Chen Zhaozhong Feng Di Liu Wenxiu Zhang Shufen Pan Hanqin Tian State Key Laboratory For Ecological Security of Regions and Cities Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing 100085 China University of Chinese Academy of Sciences Beijing 100049 China College of Environmental and Resource Sciences Zhejiang A&F University Hangzhou 311300 China School of Ecology and Applied Meteorology Nanjing University of Information Science and Technology Nanjing 210044 China Department of Engineering and Environmental Studies Program Boston College Chestnut Hill MA 02467-9991 USA Center for Earth System Science and Global Sustainability Schiller Institute for Integrated Science and Society Boston College Chestnut Hill MA 02467-9991 USA Department of Earth and Environmental Sciences Boston College Chestnut Hill MA 02467-9991 USA

Surface ozone (O 3 ) pollution showed a continuous increasing trend during the recent decades in China, posing an increasing threat to food security. A wide range of yield reductions have been reported and thus more studies are needed to narrow down the uncertainty resulting from spatiotemporal accuracy of O 3 metrics and extrapolation methods. Based on a high spatial resolution (0.1°) hourly surface O 3 data, here we analyzed the spatiotemporal O 3 pollution patterns and impacts on yield, production and economic losses for wheat, rice, and maize in China during 2005–2020. The accumulated O 3 exposure over a threshold of 40 ppb (AOT40) increased by 10 % during 2005–2019, and a decrease of 5.56 % was observed in 2020 due to the COVID-19 lockdowns. Rising O 3 pollution reduced national level wheat, rice and maize yields by 14.51 % ± 0.43 %, 11.10 % ± 0.6 %, and 3.99 % ± 0.11 %, respectively. A Business-As-Usual projection suggested that the relative yield loss (RYL) would potentially reach 8 %–18 % at the national scale by 2050 if no emission control is implemented. COVID-19 lockdowns in 2020 led to significantly reduced RYL for maize (0.52 %) and rice (2.17 %) but not for wheat (0.11 %), with the largest reduction (1.88 %–9.4 %) in North China Plain, highlighting the potential benefits of emission control. Our findings provided robust evidence that rising O 3 pollution has significantly affected China's crop yields, production and economic losses, underscoring the urgent need to curb O 3 pollution to safeguard food security, particularly in densely populated and industrialized regions.

关键词： Emission control

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World environmental and Water resources Congress 2021

World Environmental and Water Resources Congress 2021

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World environmental and Water resources Congress 2021: Planning a Resilient Future along America's Freshwaters

作者： Pasha, M. Fayzul K. Lundeen, Alex Weathers, Matthew Smith, Brennan Dept. of Civil and Geomatics Engineering California State Univ. FresnoCA United States Environmental Sciences Division Oak Ridge National Laboratory Water Power Program and Energy-Water Resource Systems Group Oak RidgeTN United States

ISBN: (纸本)9780784483466

Given the extent of a water distribution system (WDS) and its complexity and dependency on energy, it is important to observe, understand, and quantify the impact of WDS hydraulics on its energy consumption and energy flow. This observation will help to develop comprehensive knowledge in WDS energy management, which will eventually help WDS design and operation. This study observes the impacts of WDS model reduction on WDS hydraulics and hence on energy flow. Adding or removing a node can increase or decrease the number of pipes, and hence it changes the flow pattern and non-linear hydraulics of the system. This study ventures to answer the question how much change in system reduction can cause what amount of change in the system hydraulics and energy flow. The study developed a series of reduced models by removing nodes and observed the impacts of model reduction on system hydraulics and energy flow. Energy balance models have been set up for each of the reduced models separately to accomplish this goal. Results show that the total inflow energy and total outflow energy separately remain the same or fluctuate very minimally for all the reduced models. As the model reduces its size, the pumping energy also decreases but not significantly. However, as the model reduces its size, the pipe friction energy increases significantly compared to the pumping energy as the system average velocity increases even after the total length of the pipe is reduced. In this study, from the original model to the final reduced model, the system average velocity and friction loss increase by 54% and 95%, respectively. © ASCE.

关键词： Hydraulics

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Correction to: The perception of plastic waste and composition of boathouse waste in floating villages on Tonlé Sap Lake, Cambodia (Clean Technologies and environmental Policy, (2024), 10.1007/s10098-024-03108-2)

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Clean Technologies and environmental Policy 2025年 1-1页

作者： Habuer Fujiwara, Takeshi Vin, Spoann Chandara, Phat Tsukiji, Makoto Environmental Management Course Architecture Civil Engineering and Environmental Management Program School of Engineering Okayama University 3-1-1 Tsushima Naka Kita-Ku Okayama700-8530 Japan Department of Economic Development Faculty of Development Studies Royal University of Phnom Penh Russian Federation Boulevard Toul Kork Phnom Penh12156 Cambodia Department of Natural Resource Management and Development Faculty of Development Studies Royal University of Phnom Penh Russian Federation Boulevard Toul Kork Phnom Penh12156 Cambodia

In this article, the author’s name Habuer was incorrectly written as Mongolian Habuer. Incorrect version: Mongolian Habuer1 · Takeshi Fujiwara1 · Spoann Vin2 · Phat Chandara3 · Makoto Tsukiji1 Corrected version: Habuer1 · Takeshi Fujiwara1 · Spoann Vin2 · Phat Chandara3 · Makoto Tsukiji1 The original article has been corrected. © The Author(s) 2025.

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