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Advancing physical intelligence for autonomous soft robots

Science robotics 2025年第102期10卷 eads1292页

作者： Chi Chen Pengju Shi Zixiao Liu Sidi Duan Muqing Si Chuanwei Zhang Yingjie Du Yichen Yan Timothy J White Rebecca Kramer-Bottiglio Metin Sitti Tetsuya Iwasaki Ximin He Department of Material Science and Engineering University of California Los Angeles Los Angeles CA USA. Department of Chemical and Biological Engineering University of Colorado Boulder Boulder CO USA. Materials Science & Engineering Program University of Colorado Boulder Boulder CO USA. School of Engineering & Applied Science Yale University New Haven CT USA. School of Medicine and College of Engineering Koç University Istanbul Turkey. Department of Mechanical and Aerospace Engineering University of California Los Angeles Los Angeles CA USA.

Achieving lifelike autonomy remains a long-term aspiration, yet soft robots so far have mostly demonstrated rudimentary physical intelligence that relies on manipulation of external stimuli to generate continuous motion. To realize autonomous physical intelligence (API) capable of self-regulated sensing, decision-making, and actuation, a promising approach is creating nonlinear time-lag feedback embedded within materials, where a constant stimulus elicits delayed responses to enable autonomous motion. This Review explores such feedback mechanisms, traces the evolution of physically intelligent robots, outlines strategies for embedding API in soft robots under diverse environments, and further discusses challenges and future directions beyond simple locomotion.

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Real-time 3D analysis during electron tomography using tomviz

arXiv

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arXiv 2022年

作者： Schwartz, Jonathan Harris, Chris Pietryga, Jacob Zheng, Huihuo Kumar, Prashant Visheratina, Anastasiia Kotov, Nicholas A. Major, Brianna Avery, Patrick Ercius, Peter Ayachit, Utkarsh Geveci, Berk Muller, David A. Genova, Alessandro Jiang, Yi Hanwell, Marcus Hovden, Robert Department of Material Science and Engineering University of Michigan Ann ArborMI United States Kitware Inc Clifton ParkNY United States Argonne Leadership Computing Facility Argonne National Laboratory LemontIL United States Department of Chemical Engineering University of Michigan Ann ArborMI United States The Molecular Foundry Lawrence Berkeley National Laboratory BerkeleyCA United States School of Applied and Engineering Physics Cornell University IthacaNY United States Advanced Photon Source Argonne National Laboratory LemontIL United States National Synchrotron Light Source II Brookhaven National Laboratory UptonNY United States Applied Physics Program University of Michigan Ann ArborMI United States

The demand for high-throughput electron tomography is rapidly increasing in biological and material sciences. However, this 3D imaging technique is computationally bottlenecked by alignment and reconstruction which runs from hours to days. We demonstrate real-time tomography with dynamic 3D tomographic visualization to enable rapid interpretation of specimen structure immediately as data is collected on an electron microscope. Using geometrically complex chiral nanoparticles, we show volumetric interpretation can begin in less than 10minutes and a high-quality tomogram is available within 30 minutes. Real-time tomography is integrated into tomviz, an opensource and cross-platform 3D data analysis tool that contains intuitive graphical user interfaces (GUI), to enable any scientist to characterize biological and material structure in 3D. © 2022, CC BY.

关键词： Graphical user interfaces

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Corrigendum to “Synthesis and characterization of eco-friendly chitosan-based waterborne polyurethanes and their ultraviolet degradation properties” [Polymer Degradation and Stability, 233 (2025) 111169]

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Polymer Degradation and Stability 2025年 236卷

作者： Chun-Ta Wei Jhu-Lin You Kai-Yen Chin Shu Mei Chang Shun-Yi Jian An-Yu Cheng Department of Chemical & Materials Engineering Chung Cheng Institute of Technology National Defense University Taoyuan 335 Taiwan System Engineering and Technology Program National Chiao Tung University Hsinchu 300 Taiwan Institute of Organic and Polymeric Materials Research and Development Centre for Smart Textile Technology National Taipei University of Technology Taipei 10608 Taiwan Department of Material Engineering Ming Chi University of Technology New Taipei 24301 Taiwan Center for Plasma and Thin Film Technologies Ming Chi University of Technology New Taipei 243303 Taiwan

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Imaging Atomic-Scale Chemistry from Fused Multi-Modal Electron Microscopy

arXiv

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arXiv 2022年

作者： Schwartz, Jonathan Di, Zichao Wendy Jiang, Yi Fielitz, Alyssa J. Ha, Don-Hyung Perera, Sanjaya D. Baggari, Ismail El Robinson, Richard D. Fessler, Jeffrey A. Ophus, Colin Rozeveld, Steve Hovden, Robert Department of Materials Science and Engineering University of Michigan Ann ArborMI United States Mathematics and Computer Science Division Argonne National Laboratory LemontIL United States Advanced Photon Source Facility Argonne National Laboratory LemontIL United States Dow Chemical Co. MidlandMI United States Department of Material Science and Engineering Cornell University IthacaNY United States School of Integrative Engineering Chung-Ang University Seoul Korea Republic of Department of Physics Cornell University IthacaNY United States The Rowland Institute at Harvard CambridgeMA United States Department of Electrical Engineering and Computer Science University of Michigan Ann ArborMI United States National Center for Electron Microscopy Molecular Foundry Lawrence Berkeley National Laboratory BerkeleyCA United States Applied Physics Program University of Michigan Ann ArborMI United States

Efforts to map atomic-scale chemistry at low doses with minimal noise using electron microscopes are fundamentally limited by inelastic interactions. Here, fused multi-modal electron microscopy offers high signal-to-noise ratio (SNR) recovery of material chemistry at nano- and atomic- resolution by coupling correlated information encoded within both elastic scattering (high-angle annular dark field (HAADF)) and inelastic spectroscopic signals (electron energy loss (EELS) or energy-dispersive x-ray (EDX)). By linking these simultaneously acquired signals, or modalities, the chemical distribution within nanomaterials can be imaged at significantly lower doses with existing detector hardware. In many cases, the dose requirements can be reduced by over one order of magnitude. This high SNR recovery of chemistry is tested against simulated and experimental atomic resolution data of heterogeneous nanomaterials. © 2022, CC BY.

关键词： Electron microscopy

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Shape Permanence in Diarylethene-Functionalized Liquid-Crystal Elastomers Facilitated by Thiol-Anhydride Dynamic Chemistry

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Angewandte Chemie 2022年第11期134卷

作者： Tayler S. Hebner Maciej Podgórski Sudheendran Mavila Timothy J. White Christopher N. Bowman Department of Chemical and Biological Engineering University of Colorado Boulder 596 UCB Boulder CO 80309 USA Department of Polymer Chemistry Institute of Chemical Sciences Faculty of Chemistry Maria Curie-Sklowdowska University M. Curie-Sklodowska Sq. 5 20-031 Lublin Poland Material Science and Engineering Program University of Colorado Boulder 596 UCB Boulder CO 80309 USA

Diarylethene-functionalized liquid-crystalline elastomers (DAE-LCEs) containing thiol-anhydride bonds were prepared and shown to undergo reversible, reprogrammable photoinduced actuation. Upon exposure to UV light, a monodomain DAE-LCE generated 5.5 % strain. This photogenerated strain was demonstrated to be optically reversible over five cycles of alternating UV/Visible light exposure with minimal photochrome fatigue. The incorporation of thiol-anhydride dynamic bonds allowed for retention of actuated states. Further, re-programming of the nematic director was achieved by heating above the temperature for bond exchange to occur (70 °C) yet below the nematic-to-isotropic transition temperature (100 °C) such that order was maintained between mesogens. The observed thermal stability of each of the diarylethene isomers of over 72 h allowed for decoupling of photo-induced processes and polymer network effects, showing that both polymer relaxation and back-isomerization of the diarylethene contributed to LCE relaxation over a period of 12 hours after actuation unless bond exchange occurred.

关键词： Liquid Crystal Elastomers Covalent Adaptable Networks Shape Memory Diarylethene Robotics

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Transparent, low-autofluorescence microECoG device for simultaneous Ca2+ imaging and cortical electrophysiology in vivo

Transparent, low-autofluorescence microECoG device for simul...

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作者： Zátonyi, A. Madarász, M. Szabó, O. Lőrincz, T. Hodován, R. Rózsa, B. Fekete, Z. Research Group for Implantable Microsystems Faculty of Information Technology and Bionics Pázmány Péter Catholic University Budapest Hungary Microsystems Laboratory Institute for Technical Physics and Material Sciences Centre for Energy Research HAS Budapest Hungary Doctoral School of Chemical Engineering and Material Sciences University of Pannonia Veszprém Hungary Laboratory of 3D Functional Network and Dendritic Imaging Institute of Experimental Medicine HAS Budapest Hungary János Szentágothai PhD Program Semmelweis University Budapest Hungary Roska Tamás Doctoral School of Sciences and Technology Pázmány Péter Catholic University Budapest Hungary

Objective. Multimodal neuroimaging approaches are beneficial to discover brain functionalities at high spatial and temporal resolution. In our work, a novel material composition of a microECoG device relying on Parylene HT and indium-tin-oxide (ITO) is presented, which facilitates two-photon imaging of Ca2+ signals and concurrent recording of cortical EEG. Approach. Long-term stability of the interfaces of the transparent microdevice is confirmed in vitro by electrochemical and mechanical tests. The outstanding optical properties, like high transmittance and low auto-fluorescent are proven by fluorimetric measurements. Spatial resolution of fluorescent two-photon imaging through the microECoG device is presented in transgenic hippocampal slices, while concurrent recording of Ca2+ signals and cortical EEG is demonstrated in vivo. Photoartefacts and photodegradation of the materials are also investigated in detail to provide safety guidelines for further use in two-photon in vivo imaging schemes. Main results. Two-photon imaging of Ca signals can be safely performed through the proposed transparent ECoG device, without significant distortion in the dimensions of detected neuronal structures or in the temporal signaling. In chronic use, we demonstrated that fluorescent Ca signals of individual neurons can be clearly recorded even after 51 d. Significance. Our results give a firm indication that highly transparent microECoG electrode arrays made of Parylene HT/ITO/Parylene HT multilayer are excellent candidates for synergetic recording of optical signals and EEG from intact brains with high resolution and are free of electrical and optical artefacts. © 2020 IOP Publishing Ltd.

关键词： Electrophysiology

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MOF-derived spinel NiMn2O4/CoMn2O4 heterojunction and its application in a high-performance photocatalyst and supercapacitor

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Journal of Environmental chemical engineering 2023年第5期11卷

作者： Lee, Kuen-Chan Hsiao, Yu-Sheng Sung, Ming-Yen Chen, Yi-Lun Wu, Nian-Jheng Huang, Jen-Hsien Cho, Er-Chieh Weng, Huei Chu Hsu, Shih-Chieh Department of Science Education National Taipei University of Education No. 134 Section 2 Heping E. Road Da-an District Taipei City106 Taiwan Ph.D. Program in Medical Neuroscience College of Medical Science and Technology Taipei Medical University 250 Wuxing Street Taipei City110 Taiwan Department of Materials Science and Engineering National Taiwan University of Science and Technology No. 43 Section 4 Keelung Road Da-an District Taipei10607 Taiwan Department of Clinical Pharmacy School of Pharmacy College of Pharmacy Taipei Medical University 250 Wuxing Street Taipei City110 Taiwan Université Paris-Saclay CNRS Institut des Sciences Moléculaires d′Orsay Orsay91405 France Department of Green Material Technology Green Technology Research Institute CPC Corporation No. 2 Zuonan Rd. Nanzi District Kaohsiung City81126 Taiwan Department of Mechanical Engineering Chung Yuan Christian University No. 200 Chungpei Rd Chungli District Taoyuan City32023 Taiwan Department of Chemical and Materials Engineering Tamkang University No. 151 Yingzhuan Road Tamsui District New Taipei City25137 Taiwan

Metal oxide heterojunctions have attracted considerable attention in photocatalyst and supercapacitor applications. In this study, NiMn2O4/CoMn2O4 (NMO/CMO) heterojunctions were synthesized using ternary metal-organic frameworks (MOFs) as precursors. After calcination at 500 °C, the as-prepared NMO/CMO composite maintains the porous sheet-like morphology of the ternary MOF, exhibiting a highly porous structure. The heterostructured NMO/CMO composite demonstrates enhanced photocatalytic performance compared with pure NMO and CMO. This enhancement may be attributed to the well-aligned energy levels at the NMO/CMO interface, which effectively reduces charge recombination and facilitates the efficient transport of photogenerated carriers. In addition, the NMO/CMO heterojunction exhibits enhanced supercapacitor performance owing to the increased number of active redox sites and reduced charge transfer resistance. When tested at 3 A/g, the NMO/CMO composite displays a higher capacitance (756.4 F/g) than pure NMO (579.6 F/g) and CMO (519.6 F/g) and remarkable rate capability, maintaining a capacitance of 639 F/g even at 10 A/g. Notably, asymmetric supercapacitors fabricated using NMO/CMO and activated carbon can achieve an energy density of 32.18 W h/kg at 750 W/kg and superior cycling life, retaining 92.1% of its initial capacitance after 3000 cycles. © 2023 Elsevier Ltd

关键词： Heterojunctions

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Bioenergy knowledge, perception and attitude among students at Jambi state senior high school

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Journal of Physics: Conference Series 2021年第1期1816卷

作者： Nazarudin M P H Hasibuan B Haryadi Nurhayati Ulyarti Hadiyanto Chemical Engineering FST University of Jambi Jambi Indonesia Energy and Nano Material Centre LPPM Universitas Jambi Jambi Indonesia Center of Excellent on Bio-Geo Material and Energy Universitas Jambi Jambi Indonesia Master of Enviromental Study Program University of Jambi Jambi Indonesia Master of Science Education Program University of Jambi Jambi Indonesia

Bioenergy is one of the renewable energies which is predicted to be a main energy in the next few years. It can play the important role to change the current fossil fuel-based energy into a green energy which has a low carbon footprint. A research about how to develop a bioenergy have been done by a lot of reseacher. However, especially in Indonesia, there is just few research to study about bioenergy from societal aspects poin of view such as the understanding and awarness of bioenergy among citizens. In this research, we have investigated senior high school students' knowledge, perceptions, and attitudes interconected to bioenergy with online survery. The survey instrument used in the study was adopted from P. Halder's study. The data was collected from students at senior high school th (SMAN 10) Jambi City. The results showed that the students awareness of bioenergy perceived from school, home, and social media have significant effects on their knowledge, perceptions and attitudes related to bioenergy. Among 211 students as respondent (N), we found 70.62% believe that they understand well the concept about bioenergy, 5.21% believe that they understand it very well, and the rest believe that they do not understand it. This understanding reflects to their willingness to use a bioenergy in their daily life, in which 71.70% respondents agree to use bioenergy, 25.47% respondents can not decide, and only 2.83% do not want to use it. To find the relationship among the variables, a multiple regression was conducted. A statistical analysis showed that the model for knowledge as a function of attitudes and perception does not fit the data therefore this model is rejected. However, both model for attitudes as function of perception and knowledge, and also perception as function of attitudes and knowldeges fit the data hence the models are accepted. In other words, attitudes of students who will use/not use bioenergy, is significantly affected by their perception about bioen

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Overcoming the surface paradox: Buried perovskite quantum dots in wide-bandgap perovskite thin films

arXiv

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arXiv 2025年

作者： Zhang, Hao Pasha, Altaf Metcalf, Isaac Zhou, Jianlin Staunstrup, Mathias Zhu, Yunxuan Liao, Shusen Ssennyimba, Ken Chen, Jia-Shiang Reddy, Surya Prakash Thébaud, Simon Hou, Jin Shuai, Xinting Mandani, Faiz Sidhik, Siraj Jones, Matthew R. Ma, Xuedan Balakrishna, R. Geetha Susarla, Sandhya Ginger, David S. Katan, Claudine Kanatzidis, Mercouri G. Bawendi, Moungi G. Natelson, Douglas Tamarat, Philippe Lounis, Brahim Even, Jacky Mohite, Aditya D. Department of Chemical and Biomolecular Engineering Rice University HoustonTX77005 United States Applied Physics Program Smalley‐Curl Institute Rice University HoustonTX77005 United States Centre for Nano and Material Sciences Jain University Jain Global Campus Kanakapura Karnataka Bangalore562112 India Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Université de Bordeaux LP2N Talence France Institut d’Optique CNRS LP2N Talence France Department of Physics and Astronomy Rice University HoustonTX77005 United States Center for Nanoscale Materials Argonne National Laboratory LemontIL60439 United States School for Engineering of Matter Transport and Energy Arizona State University TempeAZ85281 United States UMR 6082 CNRS INSA de Rennes Rennes35708 France Department of Chemistry Rice University HoustonTX77005 United States Department of Chemistry University of Washington Box 351700 SeattleWA98195-1700 United States UMR 6226 Rennes35000 France Department of Chemistry Northwestern University EvanstonIL United States Department of Chemistry Massachusetts Institute of Technology 77 Massachusetts Avenue CambridgeMA02139 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States

Colloidal perovskite quantum dots (PQDs) are an exciting platform for on-demand quantum, and classical optoelectronic and photonic devices. However, their potential success is limited by the extreme sensitivity and low stability arising from their weak intrinsic lattice bond energy and complex surface chemistry. Here we report a novel platform of buried perovskite quantum dots (b-PQDs) in a three-dimensional perovskite thin-film, fabricated using one-step, flash annealing, which overcomes surface related instabilities in colloidal perovskite dots. The b-PQDs demonstrate ultrabright and stable single-dot emission, with resolution-limited linewidths below 130 μeV, photon-antibunching (g2(0)=0.1), no blinking, suppressed spectral diffusion, and high photon count rates of 104/s, consistent with unity quantum yield. The ultrasharp linewidth resolves exciton fine-structures (dark and triplet excitons) and their dynamics under a magnetic field. Additionally, b-PQDs can be electrically driven to emit single photons with 1 meV linewidth and photon-antibunching (g2(0)=0.4). These results pave the way for on-chip, low-cost single-photon sources for next generation quantum optical communication and sensing. © 2025, CC BY.

关键词： Photons

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Ultrafast Formation of Charge Transfer Trions at Molecular-Functionalized 2D MoS2Interfaces

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Angewandte Chemie 2024年第30期136卷

作者： Yuancheng Jing Kangkai Liang Nicole S. Muir Hao Zhou Zhehao Li Joseph M. Palasz Jonathan Sorbie Chenglai Wang Scott K Cushing Clifford P. Kubiak Zdeněk Sofer Shaowei Li Wei Xiong Department of Chemistry and Biochemistry University of California San Diego 9500 Gilman Drive MC 0358 La Jolla California 92093-0358 United States Material Science and Engineering Program University of California San Diego 9500 Gilman Drive MC 0418 La Jolla California 92093-0418 United States Division of Chemistry and Chemical Engineering California Institute of Technology 1200 E California Blvd MC 127–72 Pasadena California 91125 United States Department of Inorganic Chemistry University of Chemistry and Technology Prague Technická 5 166 28 Prague 6 Czech Republic

In this work, we investigate trion dynamics occurring at the heterojunction between organometallic molecules and a monolayer transition metal dichalcogenide (TMD) with transient electronic sum frequency generation (tr-ESFG) spectroscopy. By pumping at 2.4 eV with laser pulses, we have observed an ultrafast hole transfer, succeeded by the emergence of charge-transfer trions. This observation is facilitated by the cancellation of ground state bleach and stimulated emission signals due to their opposite phases, making tr-ESFG especially sensitive to the trion formation dynamics. The presence of charge-transfer trion at molecular functionalized TMD monolayers suggests the potential for engineering the local electronic structures and dynamics of specific locations on TMDs and offers a potential for transferring unique electronic attributes of TMD to the molecular layers.

关键词： charge transfer trion Time-resolved interfacial-sensitive spectroscopy sum frequency generation molecular- functionalized monolayer TMD

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