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Endotaxial Polytype engineering: Enhancement of Incommensurate Charge Density Waves in TaS2

Microscopy and microanalysis : the official journal of Microscopy Society of America, Microbeam Analysis Society, Microscopical Society of Canada 2023年第1期29卷 1646-1647页

作者： Sung, Suk Hyun Kezer, Pat Agarwal, Nishkarsh Goh, Yin Min Schnitzer, Noah Baggari, Ismail El Sun, Kai Kourkoutis, Lena F. Heron, John T. Hovden, Robert Department of Materials Science and Engineering University of Michigan Ann Arbor MI United States Department of Physics University of Michigan Ann Arbor MI United States Department of Materials Science and Engineering Cornell University Ithaca NY United States Rowland Institute at Harvard University Cambridge MA United States Kavli Institute at Cornell for Nanoscale Science Ithaca NY United States School of Applied and Engineering Physics Cornell University Ithaca NY United States Applied Physics Program University of Michigan Ann Arbor MI United States

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Improving the True Cycling of Redox Mediators-assisted Li-O_(2) Batteries

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Energy & Environmental materials 2021年第2期4卷 201-207页

作者： Deqing Cao Fengjiao Yu Yuhui Chen Xiangwen Gao State Key Laboratory of Materials-oriented Chemical Engineering College of Chemical EngineeringNanjing Tech UniversityNanjingJiangsu 211816China Materials Science and Engineering Program and Texas Materials Institute University of Texas at AustinAustinTX 78712USA State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China

The application of redox mediators has been considered as a promising strategy to boost the performance of aprotic Li-O_(2)***,the issues brought with redox mediators,especially on the Li anode side have been ***,we propose a facile approach of preparing a gel polymer membrane that not only allow uniform Li plating/stripping withlarge current densities over extended cycling but also inhibit the diffusion of redox mediators and avoid redox shuttling,self-discharge,and internal *** importantly,the gel polymer membrane prevents the penetration of O_(2)and superoxide intermediates from the Li ***,it ensures the successful application of both lithium anode and redox mediators in Li-O_(2)batteries to achieve the desired high capacity and rate ***,it helps understand the benefit and problems of added redox mediators and reactive oxygen species so that theperformance of such Li-O_(2)batteries can be truly evaluated.

关键词： gel polymer electrolyte Li-O_(2)batteries redox mediator redox shuttle effect

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Design of Mixed-Dimensional QDs/MoS2/TiO2 Heterostructured Resistive Random-Access Memory with Interfacial Analog Switching Characteristics for Potential Neuromorphic Computing

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ACS Applied Electronic materials 2024年第3期6卷 1581-1589页

作者： Tang, Shin-Yi Shih, Yu-Chuan Shen, Ying-Chun Cyu, Ruei-Hong Chen, Chieh-Ting Yang, Tzu-Yi Chaudhary, Mayur Peng, Yu-Ren Kuo, Yao-Ren Miao, Wen-Chien Yu, Yi-Jen Lee, Ling Kuo, Hao-Chung Chueh, Yu-Lun Department of Materials Science and Engineering National Tsing Hua University Hsinchu30013 Taiwan College of Semiconductor Research National Tsing Hua University Hsinchu30013 Taiwan Semiconductor Research Center Hon Hai Research Institute Taipei11492 Taiwan Ph. D. Program in Prospective Functional Materials Industry National Tsing Hua University Hsinchu30013 Taiwan Department of Electrophysics College of Science National Yang Ming Chiao Tung University Hsinchu30010 Taiwan Instrument Center National Tsing Hua University Hsinchu30013 Taiwan Department of Photonics Institute of Electro-Optical Engineering National Yang-Ming Chiao Tung University Hsinchu30010 Taiwan Department of Physics National Sun Yat-Sen University Kaohsiung80424 Taiwan Department of Materials Science and Engineering Korea University Seoul02841 Korea Republic of

Resistive random-access memory (RRAM) is one of the most promising candidates for next-generation nanoscale nonvolatile memory devices and neuromorphic computing applications. In this study, we developed a novel mixed-dimensional design for RRAM devices, incorporating zero-dimensional quantum dots (QDs), two-dimensional MoS2, and a TiO2 switching layer to achieve prominent interfacial switching behaviors. Compared with typical filamentary RRAM devices, the proposed heterostructure featured a light-sensitive QDs/MoS2 layer that allowed for bias-controllable resistive changes during the set and reset processes without abrupt switching. This was endowed by effective electron-hole pair separations upon excitation and the generation of a thin molybdenum oxide (MoOx) layer due to the accumulation of oxygen ions at the interface between MoS2 and TiO2. The ITO/QDs/MoS2/TiO2/Pt RRAM device exhibited an on/off ratio of 10 with improved endurance under 515 nm laser illumination and wavelength-dependent resistive switching behavior, making it useful for multilevel storage. Furthermore, the heterostructured device demonstrated synaptic characteristics with enhanced potentiation and depression nonlinearities and asymmetry factors, revealing its potential for future neuromorphic applications. © 2024 American Chemical Society.

关键词： Titanium dioxide

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Technology Roadmap for Flexible Sensors

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ACS NANO 2023年第6期17卷 5211-5295页

作者： Luo, Yifei Abidian, Mohammad Reza Ahn, Jong-Hyun Akinwande, Deji Andrews, Anne M. Antonietti, Markus Bao, Zhenan Berggren, Magnus Berkey, Christopher A. Bettinger, Christopher John Chen, Jun Chen, Peng Cheng, Wenlong Cheng, Xu Choi, Seon-Jin Chortos, Alex Dagdeviren, Canan Dauskardt, Reinhold H. Di, Chong-an Dickey, Michael D. Duan, Xiangfeng Facchetti, Antonio Fan, Zhiyong Fang, Yin Feng, Jianyou Feng, Xue Gao, Huajian Gao, Wei Gong, Xiwen Guo, Chuan Fei Guo, Xiaojun Hartel, Martin C. He, Zihan Ho, John S. Hu, Youfan Huang, Qiyao Huang, Yu Huo, Fengwei Hussain, Muhammad M. Javey, Ali Jeong, Unyong Jiang, Chen Jiang, Xingyu Kang, Jiheong Karnaushenko, Daniil Khademhosseini, Ali Kim, Dae-Hyeong Kim, Il-Doo Kireev, Dmitry Kong, Lingxuan Lee, Chengkuo Lee, Nae-Eung Lee, Pooi See Lee, Tae-Woo Li, Fengyu Li, Jinxing Liang, Cuiyuan Lim, Chwee Teck Lin, Yuanjing Lipomi, Darren J. Liu, Jia Liu, Kai Liu, Nan Liu, Ren Liu, Yuxin Liu, Yuxuan Liu, Zhiyuan Liu, Zhuangjian Loh, Xian Jun Lu, Nanshu Lv, Zhisheng Magdassi, Shlomo Malliaras, George G. Matsuhisa, Naoji Nathan, Arokia Niu, Simiao Pan, Jieming Pang, Changhyun Pei, Qibing Peng, Huisheng Qi, Dianpeng Ren, Huaying Rogers, John A. Rowe, Aaron Schmidt, Oliver G. Sekitani, Tsuyoshi Seo, Dae-Gyo Shen, Guozhen Sheng, Xing Shi, Qiongfeng Someya, Takao Song, Yanlin Stavrinidou, Eleni Su, Meng Sun, Xuemei Takei, Kuniharu Tao, Xiao-Ming Tee, Benjamin C. K. Thean, Aaron Voon-Yew Trung, Tran Quang Wan, Changjin Wang, Huiliang Wang, Joseph Wang, Ming Wang, Sihong Wang, Ting Wang, Zhong Lin Weiss, Paul S. Wen, Hanqi Xu, Sheng Xu, Tailin Yan, Hongping Yan, Xuzhou Yang, Hui Yang, Le Yang, Shuaijian Yin, Lan Yu, Cunjiang Yu, Guihua Yu, Jing Yu, Shu-Hong Yu, Xinge Zamburg, Evgeny Zhang, Haixia Zhang, Xiangyu Zhang, Xiaosheng Zhang, Xueji Zhang, Yihui Zhang, Yu Zhao, Siyuan Zhao, Xuanhe Zheng, Yuanjin Zheng, Yu-Qing Zheng, Zijian Zhou, Tao Zhu, Bowen Zhu, Ming Zhu, Rong Zhu, Yangzhi Zhu, Yong Zou, Guijin Chen, Xiaodong 08-03 Innovis Singapore 138634 Republic of Singapore Innovative Centre for Flexible Devices (iFLEX) School of Materials Science and Engineering Nanyang Technological University Singapore 639798 Singapore Department of Biomedical Engineering University of Houston Houston Texas 77024 United States School of Electrical and Electronic Engineering Yonsei University Seoul 03722 Republic of Korea Department of Electrical and Computer Engineering The University of Texas at Austin Austin Texas 78712 United States Microelectronics Research Center The University of Texas at Austin Austin Texas 78758 United States Department of Chemistry and Biochemistry California NanoSystems Institute and Department of Psychiatry and Biobehavioral Sciences Semel Institute for Neuroscience and Human Behavior and Hatos Center for Neuropharmacology University of California Los Angeles Los Angeles California 90095 United States Colloid Chemistry Department Max Planck Institute of Colloids and Interfaces 14476 Potsdam Germany Department of Chemical Engineering Stanford University Stanford California 94305 United States Laboratory of Organic Electronics Department of Science and Technology Campus Norrköping Linköping University 83 Linköping Sweden Wallenberg Initiative Materials Science for Sustainability (WISE) and Wallenberg Wood Science Center (WWSC) SE-100 44 Stockholm Sweden Department of Materials Science and Engineering Stanford University Stanford California 94301 United States Department of Biomedical Engineering and Department of Materials Science and Engineering Carnegie Mellon University Pittsburgh Pennsylvania 15213 United States Department of Bioengineering University of California Los Angeles Los Angeles California 90095 United States School of Chemistry Chemical Engineering and Biotechnology Nanyang Technological University Singapore 637457 Singapore Nanobionics Group Department of Chemical and Biological Engineering Monash University Clayton Australia 3800 Monash

Humans rely increasingly on sensors to address grand challenges and to improve quality of life in the era of digitalization and big data. For ubiquitous sensing, flexible sensors are developed to overcome the limitations of conventional rigid counterparts. Despite rapid advancement in bench-side research over the last decade, the market adoption of flexible sensors remains limited. To ease and to expedite their deployment, here, we identify bottlenecks hindering the maturation of flexible sensors and propose promising solutions. We first analyze continued...challenges in achieving satisfactory sensing performance for real-world applications and then summarize issues in compatible sensor-biology interfaces, followed by brief discussions on powering and connecting sensor networks. Issues en route to commercialization and for sustainable growth of the sector are also analyzed, highlighting environmental concerns and emphasizing nontechnical issues such as business, regulatory, and ethical considerations. Additionally, we look at future intelligent flexible sensors. In proposing a comprehensive roadmap, we hope to steer research efforts towards common goals and to guide coordinated development strategies from disparate communities. Through such collaborative

关键词： soft materials mechanics engineering flexible electronics conformable sensors bioelectronics human-machine interfaces body area sensor networks technology translation sustainable electronics

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Two-Layer High-Throughput:Effective Mass Calculations Including Warping

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engineering 2022年第3期8卷 74-80页

作者： Andrew Supka Nicholas A.Mecholsky Marco Buongiorno Nardelli Stefano Curtarolo Marco Fornari Department of Physics&Science of Advanced Materials Program Central Michigan UniversityMount PleasantMI 48859USA Department of Physics&Vitreous State Laboratory The Catholic University of AmericaWashingtonDC 20064USA Department of Physics&Department of Chemistry University of North TexasDentonTX 76203USA Center for Autonomous Materials Design Duke UniversityDurhamNC 27708USA Department of Mechanical Engineering and Materials Science Duke UniversityDurhamNC 27708USA

In this paper,we perform two-layer high-throughput *** the first layer,which involves changing the crystal structure and/or chemical composition,we analyze selected Ⅲ-Ⅴ semiconductors,filled and unfilled skutterudites,as well as rock salt and layered *** second layer searches the full Brillouin zone(BZ)for critical points within 1.5 eV(1 eV=1.602176×10^(-19)J)of the Fermi level and characterizes those points by computing the effective *** introduce several methods to compute the effective masses from first principles and compare them to each *** approach also includes the calculation of the density-of-states effective masses for warped critical points,where traditional approaches fail to give consistent results due to an underlying non-analytic behavior of the critical *** demonstrate the need to consider the band structure in its full complexity and the value of complementary approaches to compute the effective *** also provide computational evidence that warping occurs only in the presence of degeneracies.

关键词： High-throughput Electronic structure Band warping Effective mass

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Wave propagation in meta-sandwich beams 16

Wave propagation in meta-sandwich beams

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Health Monitoring of Structural and Biological Systems XVI 2022

作者： Joubaneh, Eshagh Farzaneh Ma, Jihong Department of Mechanical Engineering University of Vermont BurlingtonVT05405 United States Materials Science Program University of Vermont BurlingtonVT05405 United States

ISBN: (数字)9781510649729

ISBN: (纸本)9781510649712

Acoustoelastic metamaterials are widely used as composite cores in sandwich beams. However, discussions on the application of metamaterials in face sheets have been sporadic. In this work, we parametrically explore the dynamic behaviors of sandwich beams with metamaterials as face sheets. In addition to the capability of phonon dispersion modulation using periodic face sheets, the relative positions of top and bottom face sheets can further break their spatial symmetry and thus opens more bandgaps that are not achievable with one-dimensional periodic beams. Our study has implications for the design of sandwich beams to mitigate damages induced by vibrations in various engineering and industrial applications. © 2022 SPIE

关键词： Metamaterials

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Diffractive Imaging of Transient Electronic Coherences in Molecules with Electron Vortices

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Physical Review Letters 2025年第7期134卷 073001-073001页

作者： Haowei Wu Haiwang Yong Department of Chemistry and Biochemistry University of California San Diego La Jolla California 92093 USA Program in Materials Science and Engineering University of California San Diego La Jolla California 92093 USA

Direct imaging of transient electronic coherences in molecules has been challenging, with the potential to control electron motions and influence reaction outcomes. We propose a novel time-resolved vortex electron diffraction technique to spatially resolve transient electronic coherences in isolated molecules. By analyzing helical dichroism diffraction signals, the contribution of electronic populations cancels out, isolating the purely electronic coherence signals. This allows direct monitoring of the time evolution and decoherence of transient electronic coherences in molecules.

关键词： Molecules

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Creep-recovery deformation of 304 stainless-steel springs under low forces

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Mechanics of materials 2024年 193卷

作者： Tsai, Ming-Yen Chang, Shou-Yi Zhang, Yulin Yang, Fuqian Lee, Sanboh Department of Materials Science and Engineering National Tsing Hua University Hsinchu300 Taiwan Chongqing Institute of Green and Intelligent Technology Chinese Academy of Sciences Chongqing400714 China Materials Program Department of Chemical and Materials Engineering University of Kentucky LexingtonKY40506 United States

The deformation behavior of materials at high temperatures determines the structural stability of mechanical structures under high-temperature service conditions. In this work, we prepare helical springs from 304 stainless-steel wires and study creep-recovery deformation of the helical springs under small forces at temperatures of 475–575 °C. In contrast to most methods reported in the literature, we use Kelvin representation of the Burgers model with a nonlinear dashpot in series connection to analyze the creep-recovery deformation of the helical springs and suggest the deformation mechanisms of the diffusion of interstitial atoms and dislocation generation/annihilation in transient creep and recovery of the helical springs under small forces. For the creep deformation, the stress exponent and activation energy for the plastic flow of the nonlinear dashpot are 2 and 57.8 kJ/mol, respectively, and the activation energy for the deformation flow of the linear dashpot is 41.8 kJ/mol. The nonlinear dashpot does not play any role in the recovery deformation, and the formation energy of defects for the recovery deformation of the helical springs is 51.4 kJ/mol. The approach used in this work provides a simple method to use a phenomenological model with a nonlinear dashpot to capture the power-law creep deformation of metallic materials. © 2024

关键词： Activation energy

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Insights into the Structural and Thermodynamic Instability of Ni-Rich NMC Cathode

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ACS Sustainable Chemistry and engineering 2023年第18期11卷 6978-6987页

作者： Tran, Ngoc Thanh Thuy Lin, Che-An Lin, Shih-Kang Research Center National Cheng Kung University Tainan701 Taiwan Department of Materials Science and Engineering National Cheng Kung University Tainan701 Taiwan Program on Smart and Sustainable Manufacturing Academy of Innovative Semiconductor and Sustainable Manufacturing National Cheng Kung University Tainan70101 Taiwan

The Ni-rich LiNi1-x-yMnxCoyO2 (NMC) layered oxides have been promising materials to replace the LiCoO2 commercial cathode due to their high operation voltages, low cost, and enhanced capacity. However, structural instability is the main drawback of the Ni-rich NMC system, leading to capacity fading, which prevents its commerce application. While numerous efforts have been made to comprehend and overcome this issue, there remains a lack of systematic phase stability analysis which is an essential factor to be addressed. Herein, systematic first-principles calculations were performed in this study to reveal the structural, oxidation, and phase stability of Ni-rich NMC during delithiation. This is the first report on competing phases of Ni-rich NMC at various states of charge (SoCs). The compounds with the spinel and rock salt structures formed during delithiation and oxygen evolution takes place at highly delithiation cases, which are likely the origins of capacity fading and crack formation at the surface. This work also outlined the thermodynamic foundation of doping and oxidation state gradient-based core-shell strategies for resolving the instability and enhancing the capacity retention of Ni-rich NMC layered oxides as cathode materials in Li-ion batteries. © 2023 American Chemical Society.

关键词： Cathodes

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Correlation between the Morphology of Carbon Nanofibers and the Transport Characteristics of Li-Ions in a Lib Anode Under Fast Charging Conditions

SSRN

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SSRN 2023年

作者： Cho, Hang In Lee, Sung Hoon Park, Chong Rae WCU Hybrid Materials Program Department of Materials Science and Engineering Research Institute of Advanced Materials Seoul National University Seoul08826 Korea Republic of

Energy storage materials for electric vehicles and energy storage systems must be able to supply high capacity quickly, which requires efficient Li-ion transport within the anode active material. The transport of Li ions through a battery system can lead to concentration polarization and subsequent overpotential, which can limit the electrochemical performance, especially under fast charging conditions. To overcome these limitations, it is important to control solvated Li-ion transport and design an anode material with a rational approach. One way to achieve this is by controlling the morphology of carbon nanofibers (CNFs) to create ion transport channels. A facile method for this was investigated using an immiscible polymer blend electrospinning system and interpreting a ternary phase diagram. The effects of the morphology and space characteristics of each CNF on the electrochemical performance were studied, particularly the rate capability and cycle stability under fast charging conditions. These characteristics were analyzed in terms of the transport properties of the electrochemical species in different types of ion channels. © 2023, The Authors. All rights reserved.

关键词： Electrospinning

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