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Thermal Hall effect in insulating quantum materials

The Innovation 2022年第5期3卷 3-4页

作者： Shucheng Guo Youming Xu Ran Cheng Jianshi Zhou Xi Chen Department of Electrical and Computer Engineering University of CaliforniaRiversideRiversideCA 92521USA Department of Physics and Astronomy University of CaliforniaRiversideRiversideCA 92521USA Materials Science and Engineering Program Department of Mechanical EngineeringUniversity of Texas at AustinAustinTX 78712USA

The emerging field of quantum materials involves an exciting new class of materials in which charge,spin,orbital,and lattice degrees of freedom are intertwined,exhibiting a plethora of exotic physical *** materials include,but are not limited to,superconductors,topological quantum matter,and systems with frustrated spins,which enable a wide range of potential applications in biomedicine,energy transport and conversion,quantum sensing,and quantum information processing。

关键词： properties. quantum topological

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Fully rubbery synaptic transistors made out of all-organic materials for elastic neurological electronic skin

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Nano Research 2022年第2期15卷 758-764页

作者： Hyunseok Shim Seonmin Jang Jae Gyu Jang Zhoulyu Rao Jong-ln Hong Kyoseung Sim Cunjiang Yu Materials Science and Engineering Program University of HoustonHoustonTX 77204 USA Department of Chemistry Seoul National UniversitySeoul 08826Republic of Korea Department of Chemistry Ulsan National Institute of Science and Technology(UNIST)Ulsan 44919Republic of Korea Department of Mechanical Engineering University of HoustonHoustonTX 77204 USA Department of Biomedical Engineering University of HoustonHoustonTX 77204USA Department of Electrical and Computer Engineering University of HoustonHoustonTX 77204 USA Texas Center for Superconductivity University of HoustonHoustonTX 77204USA

Neurologic function implemented soft organic electronic skin holds promise for wide range of applications,such as skin prosthetics,neurorobot,bioelectronics,human-robotic interaction(HRI),***,we report the development of a fully rubbery synaptic transistor which consists of all-organic materials,which shows unique synaptic characteristics existing in biological *** synaptic characteristics retained even under mechanical stretch by 30%.We further developed a neurological electronic skin in a fully rubbery format based on two mechanoreceptors(for synaptic potentiation or depression)of pressure-sensitive rubber and an all-organic synaptic *** converting tactile signals into Morse Code,potentiation and depression of excitatory postsynaptic current(EPSC)signals allow the neurological electronic skin on a human forearm to communicate with a robotic *** collective studies on the materials,devices,and their characteristics revealed the fundamental aspects and applicability of the all-organic synaptic transistor and the neurological electronic skin.

关键词： synaptic transistor stretchable electronic skin all-organic

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Nonlinear optical characterization of Ag2Se and PbSe colloidal quantum dots using 1030 nm femtosecond pulses

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Optical and Quantum Electronics 2024年第12期56卷 1-17页

作者： Ganeev, Rashid A. Bejoy, Namitha Brijit Piatkowski, Piotr A. Boltaev, Ganjaboy S. Aslanov, Sergey V. Zvyagin, Andrey I. Smirnov, Mikhail S. Ovchinnikov, Oleg V. Alnaser, Ali S. Materials Research Center College of Arts and Science American University of Sharjah Sharjah26666 United Arab Emirates Department of Optics and Spectroscopy Voronezh State University Voronezh394018 Russia TIIAME National Research University Tashkent100000 Uzbekistan Department of Sciences Western Caspian University BakuAZ1001 Azerbaijan Department of Physics College of Arts and Sciences American University of Sharjah Sharjah26666 United Arab Emirates Materials Science and Engineering Program College of Arts and Sciences American University of Sharjah Sharjah26666 United Arab Emirates

Nonlinear optical characteristics of chemically prepared silver selenide (Ag2Se, 3.7 nm) and lead selenide (PbSe, 6.3 nm) colloidal quantum dots (QDs) are investigated using the 1030 nm femtosecond pulses. Ag2Se QDs demonstrated two-photon absorption followed by saturable absorption. PbSe QDs initially showed the saturable absorption at small intensities of 1030 nm probe pulses, followed by reverse saturable absorption at stronger excitation. The difference in the positive nonlinear optical absorption mechanisms in these two QD colloids is attributed to their different bandgaps. The studied QD colloids exhibited the Kerr-induced positive nonlinear refraction. Transient absorption studies of the QDs showed that photoexcitation creates a hot exciton that forms band-edge exciton within 1.2 ps after excitation. Most of the electron-hole pairs further recombine through band-to-band recombination with a time constant of 1490 ps. Furthermore, the results from the transient absorption studies indicate the contribution of trap-assisted recombination occurs on a time scale exceeding that of the experimental time window. © The Author(s), under exclusive licence to Springer science+Business Media, LLC, part of Springer Nature 2024.

关键词： Semiconductor quantum dots

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Spin-orbit-locked hyperbolic polariton vortices carrying reconfigurable topological charges

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eLight 2022年第1期2卷 143-153页

作者： Mingsong Wang Guangwei Hu Saroj Chand Michele Cotrufo Yohannes Abate Kenji Watanabe Takashi Taniguchi Gabriele Grosso Cheng‑Wei Qiu Andrea Alù Photonics Initiative Advanced Science Research CenterCity University of New YorkNew York CityNY 10031USA Department of Electrical and Computer Engineering National University of SingaporeSingapore 116083Singapore Department of Physics and Astronomy The University of GeorgiaAthensGA 30602USA Research Center for Functional Materials National Institute for Materials ScienceTsukubaIbaraki 305‑0044Japan International Center for Materials Nanoarchitectonics National Institute for Materials ScienceTsukubaIbaraki 305‑0044Japan Physics Program Graduate CenterCity University of New YorkNew YorkNY 10016USA

The topological features of optical vortices have been opening opportunities for free-space and on-chip photonic technologies,e.g.,for multiplexed optical communications and robust information *** a parallel but disjoint effort,polar anisotropic van der Waals nanomaterials supporting hyperbolic phonon polaritons(HP2s)have been leveraged to drastically boost light-matter *** far HP2 studies have been mainly focusing on the control of their amplitude and scale *** we report the generation and observation of mid-infrared hyperbolic polariton vortices(HP2Vs)associated with reconfigurable topological ***-shaped gold disks coated with a flake of hexagonal boron nitride are exploited to tailor spin-orbit interactions and realise deeply subwavelength *** complex interplay between excitation spin,spiral geometry and HP2 dispersion enables robust reconfigurability of the associated topological *** results reveal unique opportunities to extend the application of HP2s into topological photonics,quantum information processing by integrating these phenomena with single-photon emitters,robust on-chip optical applications,sensing and nanoparticle manipulation.

关键词： Hyperbolic polariton vortex Light-matter interactions Spin-orbit interaction Topological charge Reconfigurability

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Goldilocks Energy Minimum: Peptide-Based Reversible Aggregation and Biosensing (Vol 15, Pg 42293, 2023)

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ACS APPLIED materials & INTERFACES 2023年第41期15卷 48838-48838页

作者： Yim, Wonjun Retout, Maurice Chen, Amanda A. Ling, Chuxuan Amer, Lubna Jin, Zhicheng Chang, Yu-Ci Chavez, Saul Barrios, Karen Lam, Benjamin Li, Zhi Zhou, Jiajing Shi, Lingyan Pascal, Tod A. Jokerst, Jesse V. Materials Science and Engineering Program University of California San Diego La Jolla California 92093 United States Department of Nano and Chemical Engineering University of California San Diego La Jolla California 92093 United States Shu Chien-Gene Lay Department of Bioengineering University of California San Diego La Jolla California 92093 United States Department of Radiology University of California San Diego La Jolla California 92093 United States

Colorimetric biosensors based on gold nanoparticle (AuNP) aggregation are often challenged by matrix interference in biofluids, poor specificity, and limited utility with clinical samples. Here, we propose a peptide-driven nanoscale disassembly approach, where AuNP aggregates induced by electrostatic attractions are dissociated in response to proteolytic cleavage. Initially, citrate-coated AuNPs were assembled via a short cationic peptide (RRK) and characterized by experiments and simulations. The dissociation peptides were then used to reversibly dissociate the AuNP aggregates as a function of target protease detection, i.e., main protease (Mpro), a biomarker for severe acute respiratory syndrome coronavirus 2. The dissociation propensity depends on peptide length, hydrophilicity, charge, and ligand architecture. Finally, our dissociation strategy provides a rapid and distinct optical signal through Mpro cleavage with a detection limit of 12.3 nM in saliva. Our dissociation peptide effectively dissociates plasmonic assemblies in diverse matrices including 100% human saliva, urine, plasma, and seawater, as well as other types of plasmonic nanoparticles such as silver. Our peptide-enabled dissociation platform provides a simple, matrix-insensitive, and versatile method for protease sensing.

关键词： colorimetric biosensor DLVO theory reversible aggregation dissociation peptide matrix-insensitive SARS-CoV-19

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Elevated temperature-driven coordinative reconstruction of an unsaturated single-Ni-atom structure with low valency on a polymer-derived matrix for the electrolytic oxygen evolution reaction

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Nanoscale 2024年第15期16卷 7467-7479页

作者： Patil, Rahul Rajput, Anubha Matsagar, Babasaheb M. Chen, Norman C. R. Ujihara, Masaki Salunkhe, Rahul R. Yadav, Praveen Wu, Kevin C.-W. Chakraborty, Biswarup Dutta, Saikat Electrochemical Energy & Sensor Research Laboratory Amity Institute of Click Chemistry Research & Studies Amity University Noida India Department of Chemistry Indian Institute of Technology New Delhi India Department of Chemical Engineering National Taiwan University Taipei10617 Taiwan Molecular Science and Technology Program Taiwan International Graduate Program Academia Sinica Taiwan National Taiwan University Taiwan Graduate Institute of Applied Science and Technology National Taiwan University of Science and Technology Taipei Taiwan Materials Research Laboratory Department of Physics Indian Institute of Technology Jammu India Synchrotron X-ray Facility Raja Ramanna Centre for Advanced Technology Rajendra Nagar Madhya Pradesh 452013 Indore India

A high-temperature pyrolysis-controlled coordination reconstruction resulted in a single-Ni-atom structure with a Ni-Nx-C structural unit (x = N atom coordinated to Ni). Pyrolysis of Ni-phen@ZIF-8-RF at 700 °C resulted in NiNP-NC-700 with predominantly Ni nanoparticles. Upon elevating the pyrolysis temperature from 700 to 900 °C, a coordination reconstruction offers Ni-Nx atomic sites in NiSA-NC-900. A combined investigation with X-ray absorption spectroscopy, X-ray photoelectron spectroscopy, and soft X-ray L3-edge spectroscopy suggests the stabilization of low-valent Niδ+ (0 −2 was achieved. The cell potential recorded with Pt(−)/(+)NiSA-NC-900/NF was much lower than that obtained for other cells, i.e., Pt(−)/NF and NF(−)/(+)NF, which enhances the potentials of low-valent NiSAs for insightful understanding of the OER. At a constant applied potential of 1.61 V (vs. RHE) for 12 h, an small increase in current for initial 0.6 h followed by a constant current depicts the fair stability of catalyst for 12 h. Our results offer an insightful angle into the OER with a coordinatively reconstructed single-Ni-atom structure at lower valency ( © 2024 The Royal Society of Chemistry.

关键词： Reaction kinetics

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Unravelling the strong interplay for interfacial magnetic switching in metal-organic-based spintronics

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Journal of materials Chemistry C 2024年第11期12卷 3931-3942页

作者： Chen, Wan-Ting Yu, Li-Chung Lin, Jiu-Hua Cheng, Su Ling Shiu, Hung Wei Lai, Yu-Ling Chu, Ying-Hao Chin, Yi-Ying Wang, Jeng-Han Hsu, Yao-Jane National Synchrotron Radiation Research Center Hsinchu30076 Taiwan Graduate Program for Science and Technology of Accelerator Light Sources National Yang Ming Chiao Tung University Hsinchu30076 Taiwan Department of Materials Science and Engineering National Tsing Hua University Hsinchu30013 Taiwan Department of Chemistry National Taiwan Normal University Taipei11677 Taiwan Department of Photonics National Cheng Kung University Tainan70101 Taiwan Department of Physics National Chung Cheng University Chiayi62102 Taiwan

Organic semiconductors are promising building blocks for multifunctional spintronics. The spinterface plays a key role in affecting the magnetic properties of the performance of spin-based devices. Herein, we reveal the strong interfacial interplay affecting the magnetic switching at the interface of the synthetic paramagnetic tris(8-hydroxyquinoline)iron(iii) (Feq3) layer on the ferromagnetic surface. In combination with synchrotron-based analysis and density functional theory (DFT) calculations, we observed that the robust magnetic interactions of the Co/Feq3 system were strongly influenced by the interfacial reaction between Co and Feq3. As the charge transferred from the contacted Co to Feq3, the central iron was reduced from Fe(iii) to Fe(ii) and hybridized with the 8-hydroxyquinoline, causing spin polarization at the interface. The reduced central Fe(ii) exhibited apparent ferromagnetic ordering after contact with the ferromagnetic Co substrate. With increasing the Feq3 layer thickness, the central Fe reverted to its original Fe(iii) state, resulting in the disappearance of ferromagnetic ordering. The thickness dependence of the Feq3 layer on the magnetic response could be used to tune the spinterface properties and thus the interfacial magnetic interplay. These findings reveal the effect of the strong interfacial redox on the spinterface and open up a promising approach for the use of metal-organic materials in oragnic spintronic devices. © 2024 The Royal Society of Chemistry.

关键词： Organometallics

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Photolithography Patterning of Organic Light-Emitting Diodes Using Solvent Resistant Electron Transport materials

Photolithography Patterning of Organic Light-Emitting Diodes...

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International Symposium, Seminar, and Exhibition, Display Week 2024

作者： Yu, Hyunjin Yeong So, Eun Eun, Kyunghyun Jun Jung, Byung Kim, Myungwoong Lee, Jin-Kyun Yeob Lee, Jun School of Chemical Engineering Sungkyunkwan University 2066 Seobu-ro Jangan-gu Suwon-si Gyeonggi-do16419 Korea Republic of Department of Materials Science and Engineering University of Seoul Seoul02504 Korea Republic of Department of Chemistry and Chemical Engineering Inha University Incheon22212 Korea Republic of Program in Environment and Polymer Engineering Inha University 100 Inha-ro Michuhol-gu Incheon22212 Korea Republic of

In this paper, we develop a novel approach to achieve ultra-high resolution in organic light-emitting diodes (OLEDs) through a photolithography patterning process. It is important to apply a solvent resistant electron transport layer (ETL) in the photolithography pattering of OLED because of solution coating process of photoresist on the ETL. Therefore, a solvent resistant ETL named 2,7-bis(4,6-diphenyl-1,3,5-triazin-2-yl)-9,9′-spirobi[fluorene] (SBF-Trz) was developed and employed as the ETL of OLEDs. The SBF-Trz demonstrated excellent solvent resistance during photolithography process and enabled device performances comparable to those of the conventional OLED without any photolithography process. It was found that the SBF-Trz ETL is appropriate as the ETL of the OLED patterned by photolithography due to good electron transport property, good stability, and good solvent resistance. © 2024, John Wiley and Sons Inc. All rights reserved.

关键词： Reactive ion etching

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Synthesis of poly(lactide-co-glycolide) containing high glycolide contents by ring-opening polymerization as well as their structural characterizations, thermal properties, morphologies, and hydrophilicity

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Journal of Applied Polymer science 2023年第3期140卷

作者： Phan, Van Hoang-Khang Tai, Yi-Hsin Chiang, Tai-Chin Yu, Chin-Yang Department of Materials Science and Engineering National Taiwan University of Science and Technology Taipei Taiwan Global Development Engineering Program National Taiwan University of Science and Technology Taipei Taiwan

Random copolymers, poly(l-lactide-r-glycolide) are synthesized by one-pot ring-opening polymerization of l-lactide and glycolide in the presence of stannous octoate and 1-dodecanol. Block copolymers, poly(l-lactide-b-glycolide) are synthesized by ring-opening polymerization of l-lactide to generate poly(l-lactide) first and then further ring-opening polymerization of glycolide in the presence of poly(l-lactide) and stannous octoate. The composition ratio of l-lactide and glycolide is determined by the integration of the corresponding signals from 1H NMR spectra, which is consistent with the feeding ratio. Very few hetero-sequences can be observed for block copolymers due to well-defined microstructures. The block copolymers are more thermally stable than that of the random copolymers. The degree of crystallinity of the bock copolymers is relatively high compared to that of the random copolymers. The image of the block copolymers determined by field-emission scanning electron microscopy (FESEM) shows partial aggregate domains containing spherical particles with an average diameter of around 200 nm, which is very different from that of the random copolymers. Block copolymers are more hydrophilic than that of the random copolymers due to the ordered structure and amphiphilic behavior of the block series. © 2022 Wiley Periodicals LLC.

关键词： Microstructure

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Interfacial challenges for all-solid-state batteries based on sulfide solid electrolytes

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Journal of Materiomics 2021年第2期7卷 209-218页

作者： Shuo Wang Ruyi Fang Yutao Li Yuan Liu Chengzhou Xin Felix H.Richter Ce-Wen Nan State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing100084China Materials Science and Engineering Program and Texas Materials Institute The University of Texas at AustinAustinTX78712United States Institute of Physical Chemistry&Center for Materials Research Justus-Liebig-University GiessenHeinrich-Buff-Ring 17D-35392GiessenGermany State Key Laboratory of Bio-fibers and Eco-textiles Institute of Biochemical EngineeringCollege of Materials Science and EngineeringQingdao UniversityQingdao266071China

Sulfide solid electrolytes(e.g.,lithium thiophosphates)have the highest room-temperature ionic conductivity(-10^(-2) S cm^(-1))among solid Li-ion conductors so far,and thus have attracted ever-increasing attention for high energy-density and safety all-solid-state batteries(ASSBs).However,interfacial issues between sulfide electrolytes and electrodes have been the main challenges for their applications in *** interfacial instabilities would occur due to side reactions of sulfides with electrodes,poor solid-solid contact,and lithium dendrites during charge/discharge *** this review,we analyze the interfacial issues in ASSBs based on sulfide electrolytes,and in particular,discuss strategies for solving these interfacial issues and stabilize the electrode-electrolyte ***,a perspective of the interfacial engineering for sulfide-based ASSBs is provided.

关键词： Sulfide solid electrolytes Interfacial engineering All-solid-state batteries Li-metal protection

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