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Agrosystem engineering, Technology & Applications (AGRETA), IEEE International Conference on

作者： Jonathan E. Pa-a Erwin P. Enriquez Department of Chemistry Silliman University Dumaguete City Philippines Department of Chemistry and Program in Materials Science and Engineering School of Science and Engineering Ateneo de Manila University Quezon City Philippines

The NH 2 -graphene/polyaniline composites are synthesized by in situ electropolymerization of aniline monomer and NH 2 -functionalized graphene (“NH 2 -graphene”) sheets in acidic electrolyte solution by constant-potential coulometry. Cyclic voltammetry and FTIR analyses confirm the covalent attachment of polyaniline backbone onto NH 2 -graphene in the composite. Having the same functional moieties (NH 2 -group), the polyaniline nanofibers are grafted laterally forming ’synapses’ resulting in improved charge-transfer reaction and stability of the composite. This link is believed to be ’phenazine-like’ microstructure formed at the edges of graphene sheets as evidenced by SEM and TEM images. The voltammograms of the NH 2 -graphene/polyaniline composite films coated onto pencil lead graphite electrodes (PLGE) exhibit remarkable increase in the current density relative to the bare PLGE and polyaniline-coated PLGEs. Based on the electrochemical impedance spectroscopy (EIS) measurements, the enhancement in the electrochemical properties of the composite may be due to the good chargetransfer redox activity of polyaniline fibers that are grafted onto the NH 2 -graphene sheet. The composite film also demonstrated photo-responsive property which could be useful for sensing or photovoltaic cell design.

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Accelerating Degradable Composite Breakdown Using Citrus Processing Side Streams

ACS Sustainable Resource Management

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ACS Sustainable Resource Management 2024年第2期1卷 344-354页

作者： Aline V. Duarte Laís T. Possari Lívia M. G. Gonçalves Baltus C. Bonse Talita R. Rigolin Sílvia H. P. Bettini Graduate Program in Materials Science and Engineering Federal University of Sao Carlos Rod. Washington Luiz 235 São Carlos 13565-905 Brazil Department of Materials Engineering Centro Universitário FEI 09850-901 São Bernardo do Campo Brazil Department of Materials Engineering Federal University of Sao Carlos Rod. Washington Luiz 235 São Carlos 13565-905 Brazil

Daily, vast amounts of waste are produced in the orange juice industry, a large part of which is reused in low-added-value products. In this work, orange vesicle fiber residues from the juice sieving stage were plasticized by extrusion, producing a thermoplastic citrus pulp (TCP). This pulp was incorporated into poly(butylene succinate) (PBS) at up to 50 wt %. The influence of TCP on the molar mass, morphology, tensile properties, rheological behavior, and biodeterioration of PBS in soil was evaluated. Highly flexible compounds with elongations similar to those of PBS were produced. Scanning electron microscopy analyses suggested good dispersion between the TCP and PBS phases, verified after acid extraction of pectin. Rheological analyses indicated the presence of strong interactions in the interconnected network formed by pectin gel, percolation of TCP lignocellulosic fibers, or both. Analyses of mass loss by burial in soil showed that the higher the TCP content in PBS is, the higher and faster the biodeterioration is. Size exclusion chromatography analyses indicated that the greater the concentration of TCP and the better dispersed it was in the compounds, the lower molar masses populations appeared in PBS, indicating higher rates of degradation of PBS in the presence of TCP. This innovative approach not only reuses the waste produced in the orange juice industry but also demonstrates the potential for obtaining environmentally friendly compounds.

关键词： Beverages Carbohydrates Fibers Polymers Soils

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Evidence of magnetoelectronic electromagnon-mediated transport in flexoelectronic heterostructures

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Physical Review B 2023年第16期107卷 165305-165305页

作者： Anand Katailiha Paul C. Lou Ravindra G. Bhardwaj W. P. Beyermann Sandeep Kumar Department of Mechanical Engineering University of California Riverside California 92521 USA Department of Physics and Astronomy University of California Riverside California 92521 USA Materials Science and Engineering Program University of California Riverside California 92521 USA

The superposition of atomic vibrations and flexoelectronic effect gives rise to a cross correlation between free charge carriers and temporal magnetic moment of phonons in conducting heterostructures under an applied strain gradient. The resulting dynamical coupling is expected to give rise to quasiparticle excitations called magnetoelectronic electromagnons that carry electronic charge and temporal magnetic moment. Here, we report experimental evidence of magnetoelectronic electromagnons in the freestanding degenerately doped p-Si based heterostructure thin film samples. These quasiparticle excitations give rise to long-distance (>100 μm) spin transport, demonstrated using spatially modulated transverse magnetothermoelectric and nonlocal resistance measurements. The magnetoelectronic electromagnons are nonreciprocal and give rise to large magnetochiral anisotropy (0.352A−1T−1) that diminishes at lower temperatures. The superposition of nonreciprocal magnetoelectronic electromagnons gives rise to longitudinal and transverse modulations in charge carrier density, spin density, and magnetic moment, demonstrated using the Hall effect and edge dependent magnetoresistance measurements, which can also be called inhomogeneous magnetoelectronic multiferroic effect. These quasiparticle excitations are analogous to photons where time dependent polarization and temporal magnetic moment replace electric and magnetic field, respectively, and most likely topological because they manifest topological Nernst effect. Hence, the magnetoelectronic electromagnon can potentially give rise to quantum interference and entanglement effects in conducting solid state systems at room temperature in addition to efficient spin transport.

关键词： Flexoelectricity Magnetic coupling Magnetotransport Spin current Spin-phonon coupling Doped semiconductors Multiferroics

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Glycerol Electrooxidation over Precision-Synthesized Gold Nanocrystals with Different Surface Facets

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Precision Chemistry 2024年第3期2卷 103-111页

作者： Hansen Mou Fang Lu Zechao Zhuang Qiaowan Chang Lihua Zhang Xiaobo Chen Yugang Zhang Jingguang G.Chen Department of Chemical Engineering Columbia UniversityNew YorkNew York 10027United States School of Chemical Engineering and Bioengineering Washington State UniversityPullmanWashington 99164United States Center for Functional Nanomaterials Brookhaven National LaboratoryUptonNew York 11973United States Materials Science and Engineering Program State University of New York at BinghamtonBinghamtonNew York 13902United States Chemistry Division Brookhaven National LaboratoryUptonNew York 11973United States

Electrochemical glycerol oxidation(EGO)emerges as a promising route to valorize glycerol,an underutilized byproduct from biodiesel production,into value-added *** study employed three types of gold(Au)nanocrystals with controlled shapes to elucidate the facet-dependent electrocatalytic behavior in ***,rhombic dodecahedral,and cubic Au nanocrystals with{111},{110},and{100}facets,respectively,were precisely synthesized with uniform size and *** dodecahedra exhibited the lowest onset potential for EGO due to facile AuOH formation,while octahedra showed enhanced electrochemical activity for glycerol oxidation and resistance to ***-situ FTIR analysis revealed that Au{111}surfaces selectively favored C_(2) products,whereas Au{100}surfaces promoted C_(3) product formation,highlighting the significant effect of facet orientation on EGO performance and informing catalyst design.

关键词： Electrochemical glycerol oxidation Precision synthesis Shaped nanocrystals Au nanocrystals SAXS In-situ FTIR

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X-photon 3D lithography by fs-oscillators:wavelength-independent and photoinitiator-free

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Light(Advanced Manufacturing) 2024年第4期5卷 89-101页

作者： Dimitra Ladika Antanas Butkus Vasileia Melissinaki Edvinas Skliutas Elmina Kabouraki Saulius Juodkazis Maria Farsari Mangirdas Malinauskas Institute of Electronic Structure and Laser Foundation for Research and Technology-Hellas70013 HeraklionGreece Department of Materials Science and Technology University of Crete70013HeraklionCrete Laser Research Center Faculty of PhysicsVilnius UniversitySaulėtekio Ave.10LT-10223 VilniusLithuania Optical Sciences Centre and ARC Training Centre in Surface Engineering for Advanced Materials(SEAM) School of ScienceSwinburne University of TechnologyMelbourneAustralia WRH Program International Research Frontiers Initiative(IRFI)Tokyo Institute of Technology Nagatsuta-choMidori-kuYokohamaJapan

Laser direct writing employing multi-photon 3D polymerisation is a scientific and industrial tool used in various fields such as micro-optics,medicine,metamaterials,programmable materials,etc.,due to the fusion of highthroughput and fine features down to hundreds of *** limitations of technology applicability emerge from photo-resin properties,however any material modifications can strongly affect its printability,as photoexcitation conditions alter as *** we present wavelength-independent 3D polymerisation using low peak power laser *** pulse repetition rate and fast laser direct writing was employed for advancing additive manufacturing out of the SZ2080^(TM)photo-resist without any *** of 517 nm,780 nm,and 1035 nm are shown to be suitable for producing 300 nm polymerized features even at high-up to 10^(5)μm/s-writing *** of organic-inorganic ratio in hybrid material results in shift and decrease of the dynamic fabrication window,yet not prohibiting the *** energy deposition per focal volume is achieved due to localized heating enabling efficient 3D *** spatio-selective photo-chemical crosslinking widens optical manufacturing capacity of non-photo-sensitive materials.

关键词： 3D polymerisation Nonlinear absorption Multi-photon absorption Laser direct writing Additive manufacturing Material engineering Organic-inorganic polymers SZ2080^(TM) Photosensitizer

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Self-templated formation of cobalt-embedded hollow N-doped carbon spheres for efficient oxygen reduction

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Nano Research 2021年第8期14卷 2819-2825页

作者： Ayaz Mahsud Jianian Chen Xiaolei Yuan Fenglei Lyu Qixuan Zhong Jinxing Chen Yadong Yin Qiao Zhang Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesJoint International Research Laboratory of Carbon-Based Functional Materials and DevicesSoochow University199 Ren’ai RoadSuzhou 215123China School of Chemistry and Chemical Engineering Nantong UniversityNantong9 Seyuan RoadNantong226019China Department of Chemistry Materials Science and Engineering programand UCR Center for CatalysisUniversity of CaliforniaRiversideCA 92521USA

The slow kinetics at the cathode of oxygen reduction reaction(ORR)seriously limits the efficiencies of fuel cells and metal-air ***,the state-of-the-art ORR electrocatalyst,suffers from high cost,low earth abundance,and poor *** a self-templated strategy based on metal-organic frameworks(MOFs)is proposed for the fabrication of hollow nitrogen-doped carbon spheres that are embedded with cobalt nanoparticles(Co/HNC).The Co/HNC manifests better ORR activities,methanol tolerance,and stability than commercial Pt/*** high ORR performance of Co/NHC can be attributed to the hollow structure which provides enlarged electrochemically active surface area,the formation of more Co-N species,and the introduction of *** work highlights the significance of rational engineering of MOFs for enhanced ORR activity and stability and offers new routes to the design and synthesis of high-performance electrocatalysts.

关键词： cobalt self-templated metal organic framework hollow sphere oxygen reduction reaction

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A Runaway Electron Avalanche Surrogate for Partially Ionized Plasmas

arXiv

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arXiv 2025年

作者： Arnaud, Jonathan S. McDevitt, Christopher J. Tang, Xian-Zhu Nuclear Engineering Program Department of Materials Science and Engineering University of Florida GainesvilleFL32611 United States Theoretical Division Los Alamos National Laboratory Los AlamosNM87545 United States

A physics-constrained deep learning surrogate that predicts the exponential "avalanche" growth rate of runaway electrons (REs) for a plasma containing partially ionized impurities is developed. Specifically, a physics-informed neural network (PINN) that learns the adjoint of the relativistic Fokker-Planck equation in steady-state is derived, enabling a rapid surrogate of the RE avalanche for a broad range of plasma parameters, motivating a path towards an ML-accelerated integrated description of a tokamak disruption. A steady-state power balance equation together with atomic physics data is embedded directly into the PINN, thus limiting the PINN to train across physically consistent temperatures and charge state distributions. This restricted training domain enables accurate predictions of the PINN while drastically reducing the computational cost of training the model. In addition, a novel closure for the relativistic electron population used when evaluating the secondary source of REs is developed that enables improved accuracy compared to a Rosenbluth-Putvinski source. The avalanche surrogate is verified against Monte Carlo simulations, where it is shown to accurately predict the RE avalanche growth rate across a broad range of plasma parameters encompassing distinct tokamak disruption scenarios. © 2025, CC BY.

关键词： Fokker Planck equation

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Design and Characterization of Octave Spanning, 1-THz Kerr Frequency Microcombs in Silicon Nitride

Design and Characterization of Octave Spanning, 1-THz Kerr F...

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2024 Conference on Lasers and Electro-Optics, CLEO 2024

作者： Melton, Tristan Aldhafeeri, Alwaleed Chin, Hsiao Hsuan Rukh, Lala Colación, Gabriel M. Drake, Tara E. Wong, Chee Wei Mesoscopic Optics and Quantum Electronics Laboratory University of California Los AngelesCA90095 United States Optical Science & Engineering Program Center for High Technology Materials University of New Mexico AlbuquerqueNM87106 United States Dept. of Physics & Astronomy University of New Mexico AlbuquerqueNM87106 United States

We design microresonators for octave-spanning soliton frequency comb generation in silicon nitride. We lock the repetition rate via an electro-optic comb and achieve phase noise of -130-dBc/Hz, with the resultant modu... 详细信息

ISBN: (纸本)9781957171395

关键词： Silicon nitride

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Searching for quantum nonthermodynamic phenomena

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Physical Review E 2025年第5期111卷 054108-054108页

作者： Yu Qiao Program of Materials Science and Engineering University of California–San Diego La Jolla California 92093 USA and Department of Structural Engineering University of California–San Diego La Jolla California 92093-0085 USA

Recent research on the fundamentals of statistical mechanics has led to an interesting discovery. With locally nonchaotic barriers, as Boltzmann's H theorem is inapplicable, there exist nontrivial nonthermodynamic systems that can produce useful work by absorbing heat from a single thermal reservoir without any other effect, thereby breaking the boundaries of the second law of thermodynamics. The previous analyses used classical mechanical models. In the current investigation, the study is extended to quantum mechanics. First, we reiterate that the Fermi-Dirac distribution and the Bose-Einstein distribution are compatible with the generalized Maxwell's relations, which demonstrates the general robustness of the framework of quantum statistical mechanics. Next, we analyze a set of simple-step scattering problems. When the system is in contact with a thermal reservoir, a bound state inherently follows the second law of thermodynamics, while a scattering state may not. The root cause is associated with the nonlocal nature of the wave function. It implies that the nonthermodynamic phenomena favor unquantized energy and localized wave packets, exhibiting a tendency to occur in “semiclassical” setups.

关键词： Statistical mechanics

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Design and Characterization of Octave Spanning, 1-THz Kerr Frequency Microcombs in Silicon Nitride

Design and Characterization of Octave Spanning, 1-THz Kerr F...

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CLEO: Applications and Technology in CLEO 2024, CLEO: A and T 2024 - Part of Conference on Lasers and Electro-Optics

关键词： Silicon nitride

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