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Organic X-Ray Image Sensors Using a Medium Bandgap Polymer Donor with Low Dark Current

Energy & Environmental Materials 2024年第6期7卷 230-237页

作者： Jong-Woon Ha Seung Hun Eom Bo Kyung Cha Seyeong Song Hyeong Ju Eun Jong H.Kim Jong Mok Park BongSoo Kim Byoungwook Park Seo-Jin Ko Sung Cheol Yoon Changjin Lee In Hwan Jung Do-Hoon Hwang Department of Chemistry Chemistry Institute for Functional MaterialsPusan National UniversityBusan 46241Korea Division of Advanced Energy Materials Research Center Korea Research Institute of Chemical Technology(KRICT)Daejeon 34114Korea Electro-Medical Device Research Center Korea Electrotechnology Research Institute(KERI)Ansan 15588Korea Graduate School of Carbon Neutrality School of Energy and Chemical EngineeringUlsan National Institute of Science and Technology(UNIST)Ulsan 44919Korea Department of Molecular Science and Technology Ajou UniversitySuwon 16449Korea Research Center for Advanced Specialty Chemicals Korea Research Institute of Chemical TechnologyUlsan 44412Korea Department of Chemistry Ulsan National Institute of Science and Technology(UNIST)Ulsan 44919Korea Department of Organic and Nano Engineering Human-Tech Convergence ProgramHanyang University222 Wangsimni-roSeongdong-guSeoul 04763Korea

The development of portable X-ray detectors is necessary for diagnosing fractures in unconscious patients in emergency ***,this is quite challenging because of the heavy weight of the scintillator and silicon *** weight and thickness of X-ray detectors can be reduced by replacing the silicon layer with an organic *** study presents a novel bithienopyrroledione-based polymer donor that exhibits excellent photodetection properties even in a thick photoactive layer(~700 nm),owing to the symmetric backbone and highly soluble molecular structure of *** ability of bithienopyrroledione-based polymer donor to strongly suppress the dark current density(Jd~10−10 A cm^(−2))at a negative bias(−2.0 V)while maintaining high responsivity(R=0.29 A W−1)even at a thickness of 700 nm results in a maximum shot-noise-limited specific detectivity of D_(sh)^(*)=2.18×10^(13)Jones in the organic *** organic photodetectors are developed by slot-die coating for use in X-ray detectors,which exhibit D_(sh)^(*)=2.73×10^(12)Jones with clear rising(0.26 s)and falling(0.29 s)response times upon X-ray *** reliability is also proven by linear response of the X-ray detector,and the X-ray detection limit is 3 mA.

关键词： low dark current low detection limit organic photodetector printable X-ray

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Magnetism Measurements of Two-Dimensional van der Waals Antiferromagnet CrPS_(4)Using Dynamic Cantilever Magnetometry

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Chinese Physics Letters 2024年第10期41卷 123-128页

作者： Qi Li Weili Zhen Ning Wang Meng Shi Yang Yu Senyang Pan Lin Deng Jiaqiang Cai Kang Wang Lvkuan Zou Zhongming Zeng Zhaosheng Wang Jinglei Zhang Anhui Province Key Laboratory of Condensed Matter Physics at Extreme Conditions High Magnetic Field LaboratoryHFIPSChinese Academy of SciencesHefei 230031China Science Island Branch of Graduate School University of Science and Technology of ChinaHefei 230026China School of Advanced Manufacturing Engineering Hefei UniversityHefei 230601China Suzhou Institute of Nano-tech and Nano-bionics Chinese Academy of SciencesSuzhou 215123China

Recent experimental and theoretical work has focused on two-dimensional van der Waals(2D vdW)magnets due to their potential applications in sensing and spintronics *** measurements of these emerging materials,conventional magnetometry often encounters challenges in characterizing the magnetic properties of small-sized vdW materials,especially for antiferromagnets with nearly compensated magnetic ***,we investigate the magnetism of 2D antiferromagnet CrPS_(4)with a thickness of 8nm by using dynamic cantilever magnetometry(DCM).

关键词： magnets Magnet

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Exploring the Correlation Between Surface Roughness, Surface Energy, nano-indentation, Electrical Properties, and Magnetic Characteristics of Annealed Co40Fe40Dy20 Thin Films Deposited on Si(100) Substrates

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Journal of Electronic Materials 2024年第8期53卷 4498-4511页

作者： Liu, Wen-Jen Chang, Yung-Huang Hsu, Shuo-Ting Fern, Chi-Lon Chen, Yuan-Tsung Tsao, Shin-Ying Lin, Shih-Hung Department of Materials Science and Engineering I-Shou University Kaohsiung840 Taiwan Bachelor Program in Industrial Technology National Yunlin University of Science and Technology 123 University Road Section 3 Yunlin Douliou64002 Taiwan Graduate School of Materials Science National Yunlin University of Science and Technology 123 University Road Section 3 Yunlin Douliou64002 Taiwan Department of Electronic Engineering National Yunlin University of Science and Technology 123 University Road Section 3 Yunlin Douliou64002 Taiwan

The impact of film thickness and annealing temperature on the structural, electrical, magnetic, and mechanical properties of cobalt–iron–dysprosium (Co40Fe40Dy20 ) thin films deposited on Si(100) substrates have been investigated. X-ray diffraction (XRD) analysis confirmed the film's crystalline microstructure, featuring dysprosium oxide, Dy2O3(440), and cobalt oxide, Co2O3(422) and Co2O3(511), crystallographic phases. Surface energy measurements indicated a noticeable reduction in surface energy following annealing treatments, which could be ascribed to the alleviation of residual stress and enhanced atomic arrangement, resulting in a more stable film structure with reduced surface energy. The film exhibited a decreasing trend in hardness with increasing thickness, and film resistivity was significantly responsive to alterations in thickness and annealing temperature. Notably, the Co40Fe40Dy20 film demonstrated exceptional characteristics, featuring a high saturation magnetization (Ms) of 675 emu/cm3 and a low coercivity (Hc) of 9.5 Oe. Further analysis of magnetic domains and hysteresis loops revealed that larger and brighter domains were associated with higher Hc. To sum up, the surface roughness of CoFeDy films under various annealing temperatures played a pivotal role in shaping their magnetic, electrical, adhesive, and optical characteristics. An improved low-frequency alternating current magnetic susceptibility (χac) value was achieved by minimizing the pinning effect on domain walls through surface smoothing. Moreover, smoother surfaces displayed heightened carrier conductivity, resulting in a decrease in electrical resistance. On the whole, Co40Fe40Dy20 films exhibited outstanding soft magnetic properties, encompassing high saturation magnetization, low coercivity, exceptional mechanical attributes, and decreased surface energy. Graphical Abstract: (Figure presented.) © The Minerals, Metals & Materials Society 2024.

关键词： Magnetic susceptibility

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Mesoporous WO_(3)-Dot-Decorated Flexible Electrodes for the Determination of Industrial Pollutants

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Energy & Environmental Materials 2025年第2期8卷 273-283页

作者： Aneesh Koyappayil Hyunho Seok Gwan Hyun Choi Sachin Chavan Sangho Yeon Sihoon Son Anna Go Jinhyoung Lee Keon-Woo Kim Dongho Lee Hyun-Bin Choi Hyeong-U Kim Jin Kon Kim Taesung Kim Min-Ho Lee School of Integrative Engineering Chung-Ang UniversitySeoul 06974South Korea SKKU Advanced Institute of Nanotechnology(SAINT) Sungkyunkwan UniversitySuwon 16419Korea Materials Architecturing Research Center Korea Institute of Science and Technology(KIST)Seoul 02792Korea School of Mechanical Engineering Sungkyunkwan UniversitySuwon 16419Korea National Creative Research Initiative Center for Hybrid Nano Materials by High-level Architectural Design of Block Copolymer Pohang University of Science and Technology(POSTECH)PohangGyungbuk 37673Korea Department of Semiconductor Convergence Engineering Sungkyunkwan UniversitySuwon 16419Korea Semicondcutor Manufacturing Research Center Korea Institute of Machinery and Materials(KIMM)Daejeon 34103Korea Department of Nano-Mechatronics University of Science and Technology(UST)Daejeon 34113Korea

This study demonstrates the fabrication of mesoporous tungsten trioxide(WO_(3))-decorated flexible polyimide(PI)electrodes for the highly sensitive detection of catechol(CC)and hydroquinone(HQ),two environmental ***-inorganic composite dots are formed on flexible PI electrodes using evaporation-induced self-assembly(EISA)and electrospray *** EISA process is induced by a temperature gradient during electrospray,and the heated substrate partially decomposes the organic parts etched by O_(2) plasma,creating mesoporous *** pulse voltammetry and cyclic voltammetry demonstrate a linear correlation between analyte concentration and the electrochemical *** studies support the spontaneous adsorption of CC and HQ molecules on model WO_(3) *** proposed sensor shows high sensitivity,a wide linear range,and a low detection limit for both individual and simultaneous determination of CC and *** sample analysis on river water confirms practical *** WO_(3)-decorated PI electrode presents an efficient and reliable approach for detecting these pollutants,contributing to environmental safety measures.

关键词： catechol flexible sensor hydroquinone mesoporousWO_(3) simultaneous determination

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Conformal Ultrasound Patch for Real-Time Blood Flow Monitoring 38

Conformal Ultrasound Patch for Real-Time Blood Flow Monitori...

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38th IEEE International Conference on Micro Electro Mechanical Systems, MEMS 2025

作者： Lee, Taemin Park, Jongcheol Kim, Il-Seop Bang, Sangho Jung, Joontaek Lee, Hyunjoo J. Korea Advanced Institute of Science and Technology School of Electrical Engineering Korea Republic of National NanoFab Center Office of Nano Convergence Technology Korea Republic of Healcerion Co. Ltd. Korea Republic of

ISBN: (纸本)9798331508890

Wearable ultrasound systems are opening up new ultrasound applications that were previously not possible with conventional handheld probes, such as continuous blood flow monitoring, which address unmet clinical needs. The wearable ultrasound systems are rapidly advancing in terms of array order, array size, conformality with human skin, and form factors. Despite these advancements, current fabrication and packaging methods remain time-intensive and lack scalability, while the acoustic interface is inefficient for prolonged monitoring sessions. To address these issues, we present a two-dimensional (2D) conformal ultrasound patch developed for real-time continuous blood flow monitoring. A 2D conformal ultrasound patch is fabricated through a stable and efficient anisotropic conductive film (ACF) bonding and packaged with a silk layer which serves both as an adhesive and as an effective acoustic interface, enhancing long-term usability. A single element of the 2D array exhibits a transmit sensitivity of 5.7 kPa/Vpp and a receive sensitivity of 2.4 mVpp/kPa, which is 8.7 times higher than that of a commercial hydrophone. These acoustic properties are sufficient to monitor blood flow at 2 cm depth of the skin. © 2025 IEEE.

关键词： Piezoelectricity

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Tracking Control in Presence of Obstacles and Uncertainties for Bioinspired Spherical Underwater Robots

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Journal of Bionic Engineering 2023年第1期20卷 323-337页

作者： Chunying Li Shuxiang Guo Jian Guo Graduate School of Engineering Kagawa UniversityTakamatsuKagawa761-0396Japan Key Laboratory of Convergence Medical Engineering System and Healthcare Technology the Ministry of Industry and Information TechnologySchool of Life Science and TechnologyBeijing Institute of TechnologyBeijing100081China Tianjin Key Laboratory for Control Theory and Applications in Complicated Systems and Intelligent Robot Laboratory Tianjin University of TechnologyBinshui Xidao Extension 391Tianjin300384China

During marine missions,AUVs are susceptible to external disturbances,such as obstacles,ocean currents,etc.,which can easily cause mission failure or *** this paper,considering the strong nonlinearities,external disturbances and obstacles,the kinematic and dynamic model of bioinspired Spherical Underwater Robot(SUR)was ***,the waypoints-based trajectory tracking with obstacles and uncertainties was proposed for SUR to guarantee its safety and ***,the Lyapunov theory was adopted to verify the stability and the Slide Mode Control(SMC)method is used to verify the robustness of the control *** addition,a series of simulations were conducted to evaluate the effectiveness of proposed control *** tests,including path-following,static and moving obstacle avoidance were performed which verified the feasibility,robustness and effectiveness of the designed control ***,a series of experiments in real environment were performed to verify the performance of the control *** simulation and experimental results of the study supplied clues to the improvement of the path following capability and multi-obstacle avoidance of AUVs.

关键词： Path following Obstacle avoidance Bioinspired.Spherical underwater robot(SUR) Lyapunov theory

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Examining the Impact of Expression Fragmentation and Number Redundancy on Financial QA task

Examining the Impact of Expression Fragmentation and Number ...

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2025 IEEE International Conference on Big Data and Smart Computing, BigComp 2025

作者： Lee, Yoonjae Ki, Kyung Seo Gweon, Gahgene Kim, Bugeun Seoul National University Graduate School of Convergence Science and Technology Korea Republic of Seoul National University Interdisciplinary Program in Artificial Intelligence Korea Republic of Chung-Ang University Department of AI Korea Republic of

The goal of financial QA is to generate solution equations by solving problems about financial reports. Current financial QA models can suffer from two issues: expression fragmentation and number redundancy. We conduct experiments to examine the impact of the two issues. The experimental results show that addressing the expression fragmentation issue in financial QA using EPT improves the execution accuracy by 0.09, and alleviating the number redundancy issue by removing redundant numbers in the input of the FinQANet generator improves the execution accuracy by 0.07. © 2025 IEEE.

关键词： Carrier sense multiple access

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Amorphous BaTiO_(3) Electron Transport Layer for Thermal Equilibrium-Governed γ-CsPbl_(3) Perovskite Solar Cell with High Power Conversion Efficiency of 19.96%

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Energy & Environmental Materials 2024年第3期7卷 291-302页

作者： Changhyun Lee Chanyong Lee Kyungjin Chae Taemin Kim Seaeun Park Yohan Ko Yongseok Jun Department of Energy Environment Policy and Technology Graduate School of Energy and Environment(KU-KIST Green School)Korea UniversitySeoul 02841Republic of Korea Nano Electronic Materials and Components Research Center Gumi Electronics and Information Technology Research Institute(GERI)Gumi 39171Republic of Korea Energy Materials Research Center Clean Energy Research DivisionKorea Institute of Science and Technology(KIST)Seoul 02792Republic of Korea

Compared to organic-inorganic hybrid perovskites,the cesium-based allinorganic lead halide perovskite(CsPbI_(3))is a promising light absorber for perovskite solar cells owing to its higher resistance to thermal ***,additional research is required to reduce the nonradiative recombination to realize the full potential of CsPbI_(3).Here,the diffusion of Cs ions participating in ion exchange is proposed to be an important factor responsible for the bulk defects inγ-CsPbI_(3)*** based on first-principles density functional theory reveal that the[PbI_(6)]^(4-)octahedral tilt modifies the perovskite crystallographic properties inγ-CsPbI_(3),leading to alterations in its bandgap and crystal *** addition,by substituting amorphous barium titanium oxide(a-BaTiO_(3))for TiO_(2)as the electron transport layer,interfacial defects caused by imperfect energy levels between the electron transport layer and perovskite are ***-resolution transmission electron microscopy and electron energy loss spectroscopy demonstrate that a-BaTiO_(3)forms entirely as a single phase,as opposed to Ba-doped TiO_(2)hybrid nanoclusters or separate domains of TiO_(2)and BaTiO_(3)***,inorganic perovskite solar cells based on the a-BaTiO_(3)electron transport layer achieved a power conversion efficiency of 19.96%.

关键词： amorphous BaTiO_(3) electron transport layer moisture γ-CsPbI_(3)

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Effect of Surface Roughness on the Magnetism, nano-indentation, Surface Energy, and Electrical Properties of Co60Fe20Dy20 Films on Si (100) Substrate

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Journal of Electronic Materials 2024年第4期53卷 1752-1762页

作者： Liu, Wen-Jen Chang, Yung-Huang Chiang, Chia-Chin Chen, Yuan-Tsung Lin, Chih-Chien Chen, Pei-Ling Lin, Shih-Hung Department of Materials Science and Engineering I-Shou University Kaohsiung840 Taiwan Bachelor Program in Industrial Technology National Yunlin University of Science and Technology 123 University Road Section 3 Yunlin Douliou64002 Taiwan Department of Mechanical Engineering National Kaohsiung University of Science and Technology Kaohsiung City80778 Taiwan Graduate School of Materials Science National Yunlin University of Science and Technology 123 University Road Section 3 Yunlin Douliou64002 Taiwan Department of Electronic Engineering National Yunlin University of Science and Technology 123 University Road Section 3 Yunlin Douliou64002 Taiwan

In this study, we focused on depositing a target material, cobalt-iron-dysprosium (Co60Fe20Dy20), onto silicon (Si) (100) substrates with thickness varying from 10 nm to 50 nm through a direct-current (DC) magnetron sputtering technique. The subsequent step involved subjecting the samples to an hour-long annealing process in a vacuum annealing furnace at temperatures of 100°C, 200°C, and 300°C. To assess the elemental composition of the CoFeDy films, energy-dispersive X-ray spectroscopy (EDS) was employed. An observed trend indicated an increase in low-frequency alternating-current magnetic susceptibility (χac) with the increasing thickness. Remarkably, the CoFeDy films exhibited their peak χac following annealing at 300°C, with an optimal resonance frequency of 50 Hz. After annealing at 300°C, the CoFeDy film’s surface energy peaked at 50 nm. The magnetic, electrical, and adhesive properties of the CoFeDy films were notably influenced by surface roughness at different annealing temperatures. Atomic force microscopy (AFM) analysis revealed a gradual reduction in film roughness post-annealing, corresponding to smoother surfaces indicative of a weaker domain wall pinning effect, heightened carrier conductivity, and increased liquid spreading. Collectively, these outcomes contributed to diminished χac, reduced electrical resistance, and enhanced adhesion. Graphical Abstract: (Figure presented.) © The Minerals, Metals & Materials Society 2024.

关键词： Adhesion

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An EMG-Based Biomimetic Variable Stiffness Modulation Strategy for Bilateral Motor Skills Relearning of Upper Limb Elbow Joint Rehabilitation

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Journal of Bionic Engineering 2023年第4期20卷 1597-1612页

作者： Ziyi Yang Shuxiang Guo Keisuke Suzuki Yi Liu Masahiko Kawanishi Graduate School of Engineering Kagawa UniversityTakamatsuKagawa761-0396Japan Key Laboratory of Convergence Medical Engineering System and Healthcare Technology School of Life Science and TechnologyBeijing Institute of TechnologyBeijing100081China National Rehabilitation Center for Persons with Disabilities Tokorozawa359-8555Japan Faculty of Medicine Kagawa UniversityTakamatsuKagawa761-0793Japan

Bilateral rehabilitation systems with bilateral or unilateral assistive robots have been developed for hemiplegia patients to recover their one-side ***,the compliant robotic assistance to promote bilateral inter-limb coordination remains a challenge that should be *** this paper,a biomimetic variable stiffness modulation strategy for the Variable Stiffness Actuator(VSA)integrated robotic is proposed to improve bilateral limb coordination and promote bilateral motor skills *** Electromyography(EMG)-driven synergy reference stiffness estimation model of the upper limb elbow joint is developed to reproduce the muscle synergy effect on the affected side limb by independent real-time stiffness ***,the bilateral impedance control is incorporated for realizing compliant patient-robot *** experiments were carried out to evaluate the tracking performance and investigate the multiple task intensities’influence on bilateral motor skills *** results evidence the proposed method could enable bilateral motor task skills relearning with wide-range task intensities and further promote bilateral inter-limb coordination.

关键词： Biomimetic stiffness modulation Compliant physical human-robot interaction(pHRI) Electromyography(EMG) Variable stiffness actuator(VSA) Rehabilitation robotics Synergy-based control Skill relearning

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