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Electronic and magnetic properties of the topological semimetal candidate NdSbTe

Physical Review B 2020年第23期101卷 235161-235161页

作者： Krishna Pandey Rabindra Basnet Aaron Wegner Gokul Acharya Md Rafique Un Nabi Jiangwei Liu Jian Wang Y. K. Takahashi Bo Da Jin Hu Materials Science and Engineering Program Institute for Nanoscience and Engineering University of Arkansas Fayetteville Arkansas 72701 USA Department of Physics University of Arkansas Fayetteville Arkansas 72701 USA Research Center for Functional Materials National Institute for Materials Science Tsukuba Ibaraki 305-0047 Japan Institute for Materials Research and Center for Spintronics Research Network Tohoku University Sendai 980–8577 Japan Research Center for Magnetic and Spintronic Materials National Institute for Materials Science Sengen 1-2-1 Tsukuba Ibaraki 305-0047 Japan Research and Services Division of Materials Data and Integrated System National Institute for Materials Science Tsukuba Ibaraki 305-0044 Japan

ZrSiS-type materials represent a large material family with unusual coexistence of topological nonsymmorphic Dirac fermions and nodal-line fermions. As a special group of ZrSiS family, LnSbTe (Ln=lanthaniderare−earth) compounds provide a unique opportunity to explore new quantum phases due to the intrinsic magnetism induced by Ln. Here we report the single-crystal growth and characterization of NdSbTe, a previously unexplored LnSbTe compound. NdSbTe has an antiferromagnetic ground state with field-driven metamagnetic transitions similar to other known LnSbTe, but exhibits distinct enhanced electronic correlations characterized by large a Sommerfeld coefficient of 115mJ/molK2, which is the highest among the known LnSbTe compounds. Furthermore, our transport studies have revealed the coupling with magnetism and signatures of Kondo localization. All these findings establish NdSbTe as a platform for observing phenomena arising from the interplay between magnetism, topology, and electron correlations.

关键词： Magnetic order Magnetotransport Topological phases of matter Magnetic systems Single crystal materials Strongly correlated systems Topological materials Magnetic techniques Specific heat measurements Transport techniques

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Dynamic Insights of Developing functional Nanomaterials for Clean Energy and Microelectronics

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Microscopy and Microanalysis 2024年第SUPPLEMENT_1期30卷

作者： Yang, Judith C Hwang, Sooyeon Camino, Fernando Chemical and Petroleum Engineering Department University of Pittsburgh Pittsburgh PA United States Physics and Astronomy Department University of Pittsburgh Pittsburgh PA United States Center for Functional Nanomaterials Brookhaven National Lab Upton NY United States Materials Science and Engineering Program & Department of Mechanical Engineering State University of New York at Binghamton Binghamton NY United States

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Rücktitelbild: Robust, Ultrafast and Reversible Photoswitching in Bulk Polymers Enabled by Octupolar Molecule Design (Angew. Chem. 16/2024)

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Angewandte Chemie 2024年第16期136卷

作者： Long Fang Ziwei Lin Yang Zhang Bin Ye Jing Li Qishan Ran Xiaotong Wang Meijia Yang Prof. Zhongke Yuan Prof. Xiaofeng Lin Prof. Dingshan Yu Prof. Xudong Chen Prof. Quan Li Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education Key Laboratory of High Performance Polymer-based Composites of Guangdong Province GBRCE for Functional Molecular Engineering School of Chemistry Sun Yat-sen University Guangzhou 510006 China School of Computer Science and Engineering Sun Yat-sen University Guangzhou 510275 China Institute of Applied Physics and Materials Engineering University of Macau Taipa Macao SAR 999078 China School of Chemical Engineering and Light Industry Guangdong University of Technology Guangzhou 510006 China Guangdong Laboratory of Chemistry and Fine Chemical Industry Jieyang Center Jieyang 515200 China Institute of Advanced Materials and School of Chemistry and Chemical Engineering Southeast University Nanjing 211189 China Materials Science Graduate Program Kent State University Kent OH 44242 USA

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Back Cover: Robust, Ultrafast and Reversible Photoswitching in Bulk Polymers Enabled by Octupolar Molecule Design (Angew. Chem. Int. Ed. 16/2024)

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Angewandte Chemie International Edition 2024年第16期63卷

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Robust, Ultrafast and Reversible Photoswitching in Bulk Polymers Enabled by Octupolar Molecule Design

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Angewandte Chemie 2024年第16期136卷

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Revealing the Dominance of the Dissolution-Deposition Mechanism in Aqueous Zn−MnO2Batteries

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Angewandte Chemie 2023年第6期136卷

作者： Yadong Li Yuhao Li Qingshan Liu Yongshuai Liu Tiansheng Wang Mingjin Cui Prof. Yu Ding Prof. Hongsen Li Prof. Guihua Yu College of Physics Qingdao University Qingdao 266071 China Center of Energy Storage Materials & Technology College of Engineering and Applied Sciences Jiangsu Key Laboratory of Artificial Functional Materials National Laboratory of Solid State Microstructures and Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 P. R. China Materials Science and Engineering Program and Walker Department of Mechanical Engineering The University of Texas at Austin Austin TX 78712 USA

Zn−MnO 2 batteries have attracted extensive attention for grid-scale energy storage applications, however, the energy storage chemistry of MnO 2 in mild acidic aqueous electrolytes remains elusive and controversial. Using α-MnO 2 as a case study, we developed a methodology by coupling conventional coin batteries with customized beaker batteries to pinpoint the operating mechanism of Zn−MnO 2 batteries. This approach visually simulates the operating state of batteries in different scenarios and allows for a comprehensive study of the operating mechanism of aqueous Zn−MnO 2 batteries under mild acidic conditions. It is validated that the electrochemical performance can be modulated by controlling the addition of Mn 2+ to the electrolyte. The method is utilized to systematically eliminate the possibility of Zn 2+ and/or H + intercalation/de-intercalation reactions, thereby confirming the dominance of the MnO 2 /Mn 2+ dissolution-deposition mechanism. By combining a series of phase and spectroscopic characterizations, the compositional, morphological and structural evolution of electrodes and electrolytes during battery cycling is probed, elucidating the intrinsic battery chemistry of MnO 2 in mild acid electrolytes. Such a methodology developed can be extended to other energy storage systems, providing a universal approach to accurately identify the reaction mechanism of aqueous aluminum-ion batteries as well.

关键词： Aqueous Batteries Dissolution-Deposition Mechanism Energy Storage Mechanism Zinc-Ion Batteries

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Coconut waste to green nanomaterial: Large scale synthesis of N-doped graphene nano sheets

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Nano-Structures and Nano-Objects 2023年 36卷

作者： Siburian, Rikson Tang, Liang Wei Alias, Yatimah Tok, Alfred Iing Yoong Goei, Ronn Simanjuntak, Crystina Tarigan, Kerista Paiman, Suriati Goh, Boon Tong Anshori, Isa Kurniawan, Cepi Postgraduate Program Department of Chemistry Faculty of Mathematics and Natural Sciences Universitas Sumatera Utara Medan 20155 Indonesia Department of Chemistry Faculty of Mathematics and Natural Sciences Universitas Sumatera Utara Medan 20155 Indonesia Carbon and Frankincense Research Center Universitas Sumatera Utara Medan 20155 Indonesia Department of Chemistry Faculty of Science Universiti Malaya Kuala Lumpur 50603 Malaysia University Malaya Centre for Ionic Liquids (UMCiL) Universiti Malaya Kuala Lumpur 50603 Malaysia School of Materials Science and Engineering Nanyang Technological University 50 Nanyang Avenue Singapore 639798 Singapore Department of Physics Faculty of Mathematics and Natural Sciences Universitas Sumatera Utara Medan 20155 Indonesia Physics Department Faculty of Science Universiti Putra Malaysia Selangor (Serdang) Seri Kembangan 43400 Malaysia Low Dimensional Materials Research Centre Department of Physics Faculty of Science University of Malaya Kuala Lumpur 50603 Malaysia Biomedical Engineering Department School of Electrical Engineering and Informatics Bandung Institute of Technology Bandung 40132 Indonesia Research Center of Nanoscience and Nanotechnology Bandung Institute of Technology Bandung 40132 Indonesia Chemistry Department Faculty of Mathematics and Natural Sciences Universitas Negeri Semarang Semarang 50229 Indonesia Functional Material Research Center Universitas Negeri Semarang Semarang 50229 Indonesia

In this paper, a breakthrough was achieved in large-scale production of N-doped Graphene Nano Sheets (N-GNS) using coconut fruits. The main objectives were to produce N-GNS on a large scale and assess its electrical conductivity. The process involved two key steps: first, producing GNS from coconut fruits through pyrolysis, and then generating N-GNS by doping with nitrogen using ammonia solution at room temperature. Various analytical techniques were used to characterize the produced N-GNS, including X-ray Diffraction (XRD), Scanning Electron Microscopy with Energy Dispersive Spectroscopy (SEM-EDS), Transmission Electron Microscopy (TEM), X-ray Photoelectron Spectroscopy (XPS), Raman spectroscopy, and electrochemical cyclic voltammetry and electrochemical impedance spectroscopy. The XRD data indicated that the C (002) peak of N-GNS shifted to a higher 2θ value (2θ = 24.72°) compared to GNS (2θ = 23.86°), suggesting an incorporation of nitrogen into carbon structure in N-GNS. This was further supported by XPS data, which identified N-pyridine (BE = 402.0 eV) and C-N (BE = 286.8 eV) in N-GNS. TEM images showed that N-GNS had a flat surface, and the distance between graphene layers slightly expanded (0.36 nm) compared to graphene layers (0.34 nm). SEM images and EDX data validated the morphology, resembling honeycomb lattices, with a significant content of N atoms. Raman data successfully identified the D-band and G-band in N-GNS, further validating its production. Most importantly, N-GNS exhibited electrical conductivity, making it a promising candidate for conductive and supporting materials in various applications. The significance of this research extends beyond N-GNS production, opening up new avenues for the sustainable synthesis of valuable nanomaterials from coconut fruit waste, contributing to both graphene technology and environmental conservation. © 2023 Elsevier B.V.

关键词： C-sp2 Electrical conductivity Graphene nano sheets N-graphene nano sheets N-pyridine XPS

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Valley lifetimes of conduction band electrons in monolayer WSe2

arXiv

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arXiv 2020年

作者： Ersfeld, Manfred Volmer, Frank Rathmann, Lars Kotewitz, Luca Heithoff, Maximilian Lohmann, Mark Yang, Bowen Watanabe, Kenji Taniguchi, Takashi Bartels, Ludwig Shi, Jing Stampfer, Christoph Beschoten, Bernd 2nd Institute of Physics JARA-FIT RWTH Aachen University Aachen52074 Germany Department of Physics and Astronomy University of California RiversideCA92521 United States Department of Chemistry and Materials Science & Engineering Program University of California RiversideCA92521 United States Research Center for Functional Materials National Institute for Materials Science 1-1 Namiki Tsukuba Ibaraki305-0044 Japan International Center for Materials Nanoarchitectonics National Institute for Materials Science 1-1 Namiki Tsukuba Ibaraki305-0044 Japan Forschungszentrum Jülich Jülich52425 Germany

One of the main tasks in the investigation of 2-dimensional transition metal dichalcogenides is the determination of valley lifetimes. In this work, we combine time-resolved Kerr rotation with electrical transport measurements to explore the gate-dependent valley lifetimes of free conduction band electrons of monolayer WSe2. When tuning the Fermi energy into the conduction band we observe a strong decrease of the respective valley lifetimes which is consistent with both spin-orbit and electron-phonon scattering. We explain the formation of a valley polarization by the scattering of optically excited valley polarized bright trions into dark states by intervalley scattering. Furthermore, we show that the conventional time-resolved Kerr rotation measurement scheme has to be modified to account for photo-induced gate screening effects. Disregarding this adaptation can lead to erroneous conclusions drawn from gate-dependent optical measurements and can completely mask the true gate-dependent valley dynamics. Copyright © 2020, The Authors. All rights reserved.

关键词： Landforms

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Rambutan-like morphology of NiO as a potential high-performance supercapacitor electrode

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AIP Conference Proceedings 2024年第1期3026卷

作者： Siti Wihdatul Himmah Ni Luh Wulan Septiani Shofarul Wustoni Ahmad Nuruddin Brian Yuliarto Doctoral Program of Engineering Physics Faculty of Industrial Technology Institut Teknologi Bandung Bandung 40132 Indonesia. Advanced Functional Materials Research Group Faculty of Industrial Technology Institut Teknologi Bandung Bandung 40132 Indonesia. Research Center for Advanced Materials National Research and Innovation Agency (BRIN) Komplek Puspiptek South Tangerang 15314 Banten. Biological and Environmental Science and Engineering King Abdullah University of Science and Engineering Thuwal 23955-6900 Saudi Arabia. Research Center for Nanosciences and Nanotechnology (RCNN) Institute Technology Bandung (ITB) Bandung 40132 Indonesia.

Nickel oxide (NiO)-based supercapacitor electrodes have attracted great attention due to the ultra-high theoretical specific capacitance. NiO, as a typical pseudocapacitive, is considered to be the most promising candidate as an electrode material for supercapacitors. Herein, the NiO nanostructures directly grown on the Ni foam have been successfully designed and synthesized via the hydrothermal method. The optimal Ni foam/NiO electrode exhibits a high specific capacity of 93.2 C/g at a current density of 5 mV/s. The enhanced electrochemical performance of Ni foam/NiO electrodes is due to the unique morphological architecture which facilitates open access and promotes electrolyte ion/electron transport.

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Electronic and Magnetic Properties of Topological Semimetal Candidate NdSbTe

arXiv

引用

arXiv 2020年

作者： Pandey, Krishna Basnet, Rabindra Wegner, Aaron Acharya, Gokul Un Nabi, Md Rafique Liu, Jiangwei Wang, Jian Takahashi, Yukiko Da, Bo Hu, Jin Materials Science and Engineering Program Institute for Nanoscience and Engineering University of Arkansas FayettevilleAR72701 United States Department of Physics University of Arkansas FayettevilleAR72701 United States Research Center for Functional Materials National Institute for Materials Science TsukubaIbaraki305-0047 Japan Institute for Materials Research Center for Spintronics Research Network Tohoku University Sendai980-8577 Japan Research Center for Magnetic and Spintronic Materials National Institute for Materials Science Sengen 1-2-1 TsukubaIbaraki305-0047 Japan Research and Services Division of Materials Data and Integrated System National Institute for Materials Science TsukubaIbaraki305-0044 Japan

ZrSiS-type materials represent a large material family with unusual coexistence of topological nonsymmorphic Dirac fermions and nodal-line fermions. As a special group of ZrSiS-family, LnSbTe (Ln = Lanthanide rare earth) compounds provide a unique opportunity to explore new quantum phases due to the intrinsic magnetism induced by Ln. Here we report the single crystal growth and characterization of NdSbTe, a previously unexplored LnSbTe compound. NdSbTe has an antiferromagnetic ground state with field-driven metamagnetic transitions similar to other known LnSbTe, but exhibits distinct enhanced electronic correlations characterized by large a Sommerfeld coefficient of 115 mJ/mol K2, which is the highest among the known LnSbTe compounds. Furthermore, our transport studies have revealed the coupling with magnetism and signatures of Kondo localization. All these findings establish NdSbTe as a new platform for observing novel phenomena arising from the interplay between magnetism, topology, and electron correlations. Copyright © 2020, The Authors. All rights reserved.

关键词： Topology

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