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arXiv 2025年

作者： Kazempour, Ali Sisakht, Esmaeil Taghizadeh Okyay, Mahmut Sait Jiang, Xiao Sato, Shunsuke Park, Noejung Department of physics Payame Noor University PO BOX Tehran119395-3697 Iran Department of Physics Ulsan National Institute of Science and Technology Ulsan689-798 Korea Republic of Materials Science and Engineering Program Department of Chemical and Environmental Engineering University of California-Riverside RiversideCA92521 United States Center for Computational Sciences University of Tsukuba Tsukuba305-8577 Japan

Ultrafast optical control of ferroelectricity based on short and intense light can be utilized to achieve accurate manipulations of ferroelectric materials, which may pave a basis for future breakthrough in nonvolatile memories. Here, we demonstrate that phase manipulation of electric field in the strong field sub-cycle regime induces a nonlinear injection current, efficiently coupling with the topology of band structure and enabling dynamic reversal of both current and polarization. Our time-dependent first-principles calculations reveal that tuning the phase of linearly or circularly polarized light through time-varying chirp, or constant carrier envelop phases within sub-laser-cycle dynamics effectively breaks the time-reversal symmetry, allowing the control over current and electronic polarization reversal over multi-ferroelectric states. Our time- and momentum-resolved transverse current analysis reveal the significance of Berry curvature higher order poles in the apparent association between the odd (even) orders of Berry curvature multipoles to odd (even) pseudo-harmonics in driving polarization dynamics reversal. We suggest that these phase manipulations of short pulse waveform may lead to unprecedented accurate control of nonlinear photocurrents and polarization states, which facilitate the development of precise ultrafast opto-ferroelectric devices. © 2025, CC BY.

关键词： Ferroelectricity

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Stable Cycling of Sodium All-Solid-State Batteries with High-Capacity Cathode Presodiation

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Advanced Energy materials 2025年第0期

作者： Tang, Wei Xu, Dapeng Wu, Junlin Lee, Dong Ju Fuqua, Alexander Li, Feng Jeon, Yuju Bian, Wenjuan Chen, Zheng Aiiso Yufeng Li Department of Chemical and Nano Engineering University of California La Jolla San DiegoCA92093 United States Program of Materials Science and Engineering University of California La Jolla San DiegoCA92093 United States Energy and Environment Science and Technology Idaho National Laboratory Idaho FallsID83415 United States Sustainable Power and Energy Center University of California La Jolla San DiegoCA92093 United States

Sodium all-solid-state batteries (NaSSBs) with an alloy-type anode (e.g., Sn and Sb) offer superior capacity and energy density compared to hard carbon anode. However, the irreversible loss of Na+ at the alloy anode during the initial cycle results in diminished capacity and stability, impairing full-cell performance. This study presents an easy-to-implement cathode presodiation strategy by employing a Na-rich material to address these challenges. Leveraging the high theoretical capacity and suitable voltage window, Na2S is chosen as the Na donor, which is activated by creating a mixed electron-ion conducting network, delivering a high capacity of 511.7 mAh g−1. By adding a small amount (i.e., 3 wt.%) of Na2S to the cathode composite, a NaCrO2 || Sn full cell demonstrated capacity improvement from 90.8 to 118.2 mAh g−1 (based on cathode mass). The capacity-balanced full cell can thus cycle to more than 300 times with >90% capacity retention. This work provides a practical solution to enhance the full-cell performance and advance the transformation from half-cell to full-cell applications of NaSSBs. © 2025 Wiley-VCH GmbH.

关键词： Solid-State Batteries

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High Spatial Resolution Terahertz Time-Domain Imaging of Murine Pancreatic Ductal Adenocarcinoma Tissues

High Spatial Resolution Terahertz Time-Domain Imaging of Mur...

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2023 Conference on Lasers and Electro-Optics, CLEO 2023

作者： Chakraborty, Debamitra Mills, Bradley N. Cheng, Jing Komissarov, Ivan Gerber, Scott Sobolewski, Roman Materials Science Graduate Program University of Rochester RochesterNY14627-1299 United States Laboratory for Laser Energetics University of Rochester RochesterNY14623 United States Department of Surgery University of Rochester Medical Center RochesterNY14642 United States Department of Electrical and Computer Engineering University of Rochester RochesterNY14627-0231 United States

We developed a terahertz time-domain spectroscopy system to generate high-resolution 2-dimensional images of paraffin-embedded murine pancreatic ductal adenocarcinoma tissues using the refractive index and absorption ... 详细信息

ISBN: (纸本)9781957171258

关键词： Tissue

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Alginate-based bioink for organoid 3D bioprinting: A review

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Bioprinting 2022年 28卷

作者： Leonardo, Michael Prajatelistia, Ekavianty Judawisastra, Hermawan Materials Engineering Study Program Faculty of Mechanical and Aerospace Engineering Institut Teknologi Bandung Indonesia Materials Science and Engineering Research Group Faculty of Mechanical and Aerospace Engineering Institut Teknologi Bandung Indonesia

As a 3D cell culture, organoids have been researched thoroughly to model the human biology system in advancing disease treatment and drug development. A novel way to create an organoid is using bioink, consisting of polymeric materials and living cells, to fabricate a hydrogel scaffold through the 3D bioprinting method. Alginate has the potential to be developed as a bioink due to its good biocompatibility, low toxicity, and ease of processing method. However, studies are still required to obtain an optimum alginate-based bioink. Alginate is insufficient in terms of the cell-binding site;thus, mixing it with supplementary gelatin material can be employed to optimize further the printability, mechanical properties, and biocompatibility of alginate-based bioink. The addition of gelatin material, in addition to increasing the binding site, also makes the process of making bioink easier due to the thermoresponsive nature of gelatin. The alginate-based bioink can be further optimized depending on gelatin concentration to produce appropriate density and rheological value of bioink. The addition of gelatin into alginate-based bioink will also significantly affect the printability of bioink and the mechanical properties of resulted hydrogel scaffold, which need to be considered appropriately. The alginate-based bioink also showed good biocompatibility regarding cell viability and biological performance. This paper focuses on the relationship between the structure and properties of alginate-based bioink, the 3D bioprinting processing parameters, and the implementation of resulted hydrogel scaffold and organoid. © 2022 Elsevier B.V.

关键词： 3D bioprinting Alginate Bioink Gelatin Hydrogel scaffold

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Cr is not an acceptor in β−Ga2O3

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Physical Review materials 2025年第5期9卷 054606-054606页

作者： Cassandra Remple Benjamin L. Dutton Joel B. Varley John S. McCloy Matthew D. McCluskey Materials Science & Engineering Program Washington State University Pullman Washington 99164-2711 USA Department of Physics and Astronomy Washington State University Pullman Washington 99164-2814 USA Institute of Materials Research Washington State University Pullman Washington 99164-2711 USA Lawrence Livermore National Laboratory Livermore California 94551-0808 USA

The intensity of red Cr3+ photoluminescence (PL) in monoclinic gallium oxide (β−Ga2O3) is suppressed by n-type conductivity, an effect that has been attributed to a Cr deep acceptor level in the bandgap. In n-type material, such an acceptor level would be occupied, resulting in the Cr2+ oxidation state and the absence of Cr3+ PL. To test this model, n-type β−Ga2O3 crystals co-doped with Cr and Zr (a donor) were grown from the melt. The samples show Cr3+ optical absorption bands and a high free-electron concentration of 4×1018cm−3. If Cr were an acceptor, then it would be fully compensated and therefore would not exhibit the Cr3+ optical signature. Hybrid functional calculations indicate that Cr occupies the substitutional octahedral Ga(II) site and that the Cr2+ state is energetically unfavorable, i.e., Cr is not an acceptor. Weak Cr3+ PL was observed in the Cr/Zr co-doped samples. The quenching of PL may be caused by a transfer of energy to free electrons, a nonradiative process that would reduce the emission intensity.

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Self-Healable Sandfish Scale-Inspired Scalable Triboelectric Layer for Hybrid Energy Harvesting in Desert Environment

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Small 2024年第4期21卷 e2404637页

作者： Chen, An-Rong Parashar, Parag Sharma, Manish Kumar Shih, Jing-Siang Yeh, Hsuan-Yu Lin, Yen-Jui Kaswan, Kuldeep Fan, Kai-Po Chen, Po-Yu Lin, Zong-Hong Department of Materials Science and Engineering National Tsing Hua University Hsinchu30013 Taiwan Department of Biomedical Engineering National Taiwan University Taipei10617 Taiwan Institute of Biomedical Engineering National Tsing Hua University Hsinchu30013 Taiwan International Intercollegiate Ph.D. Program National Tsing Hua University Hsinchu30013 Taiwan

In deserts, sedimentation from frequent dust activities on solar cells poses a substantial technical challenge, reducing efficiency and necessitating advanced cost-inefficient cleaning mechanisms. Herein, a novel sandfish scale-inspired self-healing fluorinated copolymer-based triboelectric layer is directly incorporated on top of the polysilicon solar cell for sustained hybrid energy harvesting. The transparent biomimetic layer, with distinctive saw-tooth microstructured morphology, exhibits ultra-low sand adhesion and high abrasion-resistant properties, inhibits sedimentation deposition on solar cells, and concurrently harvests kinetic energy from wind-driven sand particles through triboelectric nanogenerator (TENG). The film exhibits a low friction coefficient (0.149), minimal sand adhesion force (27 nN), and a small wear area (327 µm2). In addition, over 2 months, a solar cell with the sandfish scale-inspired structure demonstrates only a 16% decline in maximum power output compared to the bare solar cell, which experiences a 60% decline. Further, the sandfish scale-based TENG device's electrical output is fully restored to its original value after a 6-h self-healing cycle and maintains consistent stable outputs. These results highlight the exceptional advantages of employing biomimetic self-healing materials as robust triboelectric layers, showcasing sustained device stability and durability for prolonged use in harsh desert environments, ultimately contributing to a low cost-of-electricity generation paradigm. © 2024 Wiley-VCH GmbH.

关键词： Nanogenerators

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Improved gas-phase infrared analysis of nitrobenzene using nanoporous silica preconcentrator

Improved gas-phase infrared analysis of nitrobenzene using n...

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Optical Sensors, Sensors 2021 - Part of OSA Optical Sensors and Sensing Congress 2021

作者： Day, Coco Hutter, Tanya Department of Chemistry University of Cambridge Lensfield Road CambridgeCB2 1EW United Kingdom Department of Mechanical Engineering Materials Science and Engineering Program Texas Materials Institute The University of Texas at Austin AustinTX78712 United States

Gas-phase infrared (IR) is often insufficiently sensitive to detect low-vapor-pressure explosives. A nanoporous silica preconcentrator was used to achieve a three-fold sensitivity enhancement of gas-phase IR for nitro... 详细信息

ISBN: (纸本)9781557528209

关键词： Nitrobenzene

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Large magnetic anisotropy and magnetostriction in thin films of CoV2O4

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Physical Review materials 2023年第1期7卷 014408-014408页

作者： Sangsoo Kim Christie J. Thompson Yan Xin Christianne Beekman National High Magnetic Field Laboratory Florida State University Tallahassee Florida 32310 USA Department of Physics Florida State University Tallahassee Florida 32306 USA Materials Science and Engineering Program Florida State University Tallahassee Florida 32310 USA

Spinel cobalt vanadate CoV2O4 has been grown on (001) SrTiO3 substrates. Using torque magnetometry experiments, we find that the previously observed temperature-induced anisotropy change, where the easy axis changes from the out-of-plane [001] direction to a biaxial anisotropy with planar <100> easy axes, occurs in a gradual second-order structural phase transition. This paper characterizes this transition and the magnetic anisotropies in the (001), (100), and (1¯10) rotation planes, and explores their field dependence up to 30 T. Below 80 K, hysteretic features appear around the hard axes, i.e., the out-of-plane direction in (1¯10) and (010) rotations and the planar <110> directions in (001) rotations. This is due to a Zeeman energy that originates from the lag of the magnetization with respect to the applied magnetic field as the sample is rotated. The appearance of the hysteresis, which persists up to very high fields, shows that the anisotropy at low temperature is rather strong. Additionally, field-dependent distortions to the symmetry of the torque response in increasing applied fields shows that magnetostriction plays a large role in determining the direction and magnitude of the anisotropy.

关键词： Magnetic anisotropy Magnetic phase transitions Structural properties

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In Situ Anchoring Polymetallic Phosphide Nanoparticles within Porous Prussian Blue Analogue Nanocages for Boosting Oxygen Evolution Catalysis

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Nano Letters 2021年第7期21卷 3016-3025页

作者： Zhang, Guangxun Li, Yanle Xiao, Xiao Shan, Yang Bai, Yang Xue, Huai-Guo Pang, Huan Tian, Ziqi Xu, Qiang School of Chemistry and Chemical Engineering Yangzhou University Yangzhou Jiangsu 225009 China Ningbo Institute of Materials Technology and Engineering Chinese Academy of Sciences Ningbo Zhejiang 315201 China Department of Materials Science and Engineering SUSTech Academy for Advanced Interdisciplinary Studies Southern University of Science and Technology (SUSTech) Shenzhen 518055 China Institute for Integrated Cell-Material Sciences (ICeMS) Kyoto University Yoshida Sakyo-ku Kyoto 606-8501 Japan

The controllable synthesis of metal-based nanoclusters for heterogeneous catalytic reactions has received considerable attention. Nevertheless, manufacturing these architectures, while avoiding aggregation and retaining surface activity, remains challenging. Herein, for the first time we designed NiCoFe-Prussian blue analogue (PBA) nanocages as a support for in situ dispersion and anchoring of polymetallic phosphide nanoparticles (pMP-NPs). Benefiting from the porous surfaces and the synergistic effects between pMP-NPs and the cyano groups in PBA, the NiCoFe-P-NP@NiCoFe-PBA nanocages exhibit a significantly enhanced catalytic activity for oxygen evolution reaction (OER) with an overpotential of 223 mV at 10 mA cm-2 and a Tafel slope of 78 mV dec-1, outperforming the NiCoFe-PBA nanocubes, NiCoFe-P nanocages, NiFe-P-NP@NiFe-PBA nanocubes, and CoFe-P-NP@CoFe-PBA nanoboxes. This work not only offers the synthesis strategy of in situ anchoring pMP-NPs on PBA nanocages but also provides a new insight into optimized Gibbs free energy of OER by regulating electron transfer from metallic phosphides to PBA substrate. © 2021 American Chemical Society.

关键词： controlled synthesis in situ anchoring oxygen evolution catalysis polymetallic phosphide nanoparticles porous Prussian blue analogue nanocages

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Multiplex Magnetic Biosensor Microarrays Facilitate Personalized Vaccination Schedules for Sars-Cov-2 Variants

SSRN

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SSRN 2024年

作者： Um, Hyun-Kyung Kim, Songeun Wang, Shan X. Lee, Jung-Rok Department of Mechanical and Biomedical Engineering Ewha Womans University Seoul03760 Korea Republic of Graduate Program in Smart Factory Ewha Womans University Seoul03760 Korea Republic of Department of Materials Science and Engineering Stanford University Stanford CA94305 United States Department of Electrical Engineering Stanford University Stanford CA94305 United States

Rapid, sensitive, multiplexed antibody detection technologies are essential for assessing vaccine efficacy and recipient immunity against viruses. As severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2) variants continue to emerge, and the fact that novel viruses may pose potential threats in the near future, personalized vaccines can be precisely tailored to an individual’s measured immunity to help mitigate the symptoms of infection and viral spread. Here, we present giant magnetoresistive (GMR) biosensor microarrays for the quantitative multiplexed detection of antibodies against SARS-CoV-2 variants. The multiplexed GMR biosensor microarrays demonstrated high sensitivity, comparable to that of the single-plex enzyme-linked immunosorbent assay, enabling multiplexed measurements using blood obtained from finger pricks. Additionally, the GMR biosensor microarrays demonstrated compatibility with clinical samples and could detect variant-specific antibodies in serum, allowing for the assessment of current immunity status. Notably, an increased concentration of antibodies against the Omicron variant was clearly observed two weeks after receiving an Omicron-based booster vaccination. These results indicate that GMR biosensor microarrays offer a practical point-of-care tool for monitoring humoral immunity and guiding personalized vaccination schedules, thereby supporting immunity management against SARS-CoV-2 and future viral threats. © 2024, The Authors. All rights reserved.

关键词： Giant magnetoresistance

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